SEPA
              United States
              Environmental Protection
              Agency
              Office of Air Quality
              Planning and Standards
              Research Triangle Park NC 27711
EPA-450/4-79-014
September 1979
              Air
Graphic  Arts:
An AP-42 Update

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                                                  EPA-450/4-79-014
                             GRAPHIC ARTS:
                             AN  AP-42 UPDATE
                    PACIFIC ENVIRONMENTAL  SERVICES,  INC.
                              1930  14th  Street
                      Santa Monica, California  90404
                          Contract No. 68-02-2583
                           Work Assignment  No.  12
                    EPA Project Officer:   Audrey McBath


                                Prepared  for

                    U.S. ENVIRONMENTAL  PROTECTION AGENCY
                     Office of Air, Noise and  Radiation
                Office of Air Quality Planning and Standards
               Research Triangle Park,  North  Carolina 27711
                               September  1979                    Property Of
                                                                 EPA Li::rc;y
                                                                RTP LO 27711
                     Pacific Environmental Services, INC.

CORPORATE AND ENGINEERING  1930 14th Street  Santa Monica. California 90404  Telephone (213) 450-1800
    MIDWEST OPERATIONS  465 Fullerton Avenue  Elmhurst, Illinois 601 26  Telephone (31 2) 530-7272

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This report is issued by the U.S. Environmental Protection Agency to
report technical data of interest to a limited number of readers.
Copies are available free of charge to Federal employees, current con-
tractors and grantees, and nonprofit organizations - in limited quan-
tities - from the Library Services Office  (MD-35), U.S. Environmental
Protection Agency, Research Triangle Park, North Carolina 27711; or,
for a fee, from the National Technical Information Service, 5285 Port
Royal Road, Springfield, Virginia 22161.
This report was furnished to the U.S. Environmental Protection Agency
by Pacific Environmental Services, Inc., 1930 14th Street, Santa
Monica, California 90404.  The contents of this report are reproduced
herein as received from Pacific Environmental Services, Inc.  The
opinions, findings, and conclusions expressed are those of the authors
and not necessarily those of the Environmental Protection Agency.
Mention of company or product names is not to be considered as an
endorsement by the Environmental Protection Agency.
                   Publication No. EPA-450/4-79-014
                                    n

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                   TABLE OF CONTENTS
                                                        Page

FIGURES	  iv

TABLES 	  iv

INTRODUCTION	   1

GRAPHIC ARTS	   2

4.9.1 Process Description	   2

     4.9.1.1  General	   2
     4.9.1.2  Web Offset Lithography	   3
     4.9.1.3  Ueb Letterpress	   5
     4.9.1.4  Rotogravure	   5
     4.9.1.5  Flexography	   9

4.9.2  Emissions and Controls	  10

     4.9.2.1  General	  10
     4.9.2.2  Web Offset Lithography	  11
     4.9.2.3  Web Letterpress	  13
     4.9.2.4  Rotogravure	  13
     4.9.2.5  Flexography	  15

REFERENCES FOR SECTION 4.9	  17

BACKGROUND DOCUMENT	  19
                             m

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                               FIGURES
Number                                                          Page

 4.9-1   Web offset lithography publication printing line
           emission points	  4
 4.9-2   Web letterpress publication printing line emission
           points	  6
 4.9-3   Rotogravure and flexography printing line emission
           poi nts	  8
                               TABLES
Number

 4.9-1
 4.9-2
                                                       Page
Typical parameters for computing solvent emission
  from uncontrolled web offset lithography, web
  letterpress, rotogravure and flexography printing
  1i nes	
Estimated control technology efficiencies for web
  offset lithography, web letterpress,  rotogravure
  and flexography printing lines	
12


16

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                             INTRODUCTION

    As the Table of Contents indicates, this report was written for
inclusion in EPA Publication No. AP-42, Compilation of Air Pollutant
Emission Factors.  A preliminary draft of this section was begun when
the draft version of the Control Techniques Guideline (CTG) document
on "Graphic Arts" became available in April 1978.  This work was
performed under Work Assignment No. 7 of EPA Contract No. 68-02-2583.
The publication date of the CTG document was subsequently postponed
from July to December 1978, so completion of this AP-42 section was
likewise delayed and was completed under Work Assignment No. 12 of the
contract.
                                   -1-

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4.9  GRAPHIC ARTS

4.9.1  Process Description

4.9.1.1  General--The term  "graphic arts" as used here means four
basic processes of the printing industry: web offset lithography, web
letterpress, rotogravure and flexography.  Screen printing and manual
and sheet fed techniques are not included in this discussion.

   Printing may be performed on coated or uncoated paper and on other
surfaces, as in metal decorating and some fabric coating (see 4.2
Industrial Surface Coating).  The material to receive the printing is
called the substrate.  The  distinction between printing and paper
coating, which may employ rotogravure or  lithographic methods, is that
printing invariably  involves the application of ink by a printing
press.  However, printing and paper coating have the following
elements in common:
   • Application of a  relatively high  solvent content material
     to the surface of a moving web or film
   • Rapid solvent evaporation by movement of heated air across
     the wet surface
   • Solvent laden air exhausted from  the system
   Printing inks vary widely  in composition, but all consist of three
major components:

   • Pigments, which produce  the  desired colors  and  are  composed
     of finely divided organic and  inorganic materials
   » Binders, the solid components  that lock the pigments to the
     substrate and are composed of  organic resins and polymers, or
     in some inks, oils and rosins
                                    -2-

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   • Solvents,  which  dissolve or disperse the pigments  and binders  and
      are  usually  composed  of  organic  compounds

The  binder  and  solvent  make up the "vehicle"  part  of the  ink.   The
solvent evaporates  from the ink  into  the  atmosphere  during the  drying
process.

4.9.1.2   Web  Offset Lithography—Lithography, the  process  by which
about 75  percent  of books  and pamphlets and an  increasing  number  of
newspapers  are  now  printed, is characterized  by a  planographic  image
carrier  (i.e.,  the  image and  nonimage areas are on the  same plane).
The  image area  is ink wettable and water  repellant,  and the nonimage
area is chemically  repellant  to  ink.   The solution used to dampen the
plate may contain 15  to 30 percent isopropanol, if the  Dalgren
dampening system  is used.8 when  the image is  applied to a  rubber
covered  "blanket" cylinder, which then transfers the wet  inked  image
onto the  substrate, the process  is known  as  "offset" lithography.
When a web  (i.e., a continuous roll)  of paper is employed  with  the
offset process, this  is known as web  offset printing.   Figure 4.9-1
illustrates a web offset lithography  publication printing  line. A web
newspaper printing  line contains no dryer because  the ink  contains
very little solvent,  and somewhat porous  paper  is  generally used.

   Web offset employs "heatset"  (i.e., heat-drying offset) inks that
dry  quickly.  For publication work,  the inks  contain about 40 percent
solvent,  and  for  newspaper work, 5 percent solvent is used.  In both
cases, the  solvents are usually  petroleum derived  hydrocarbons.11
For  publication work, the  web is printed  on both sides  simultaneously
and  passed  through  a  tunnel or floater dryer  at about 200-290°C  (400-
£%ii
•9ae°F).   The  dryer  may  be  hot air or  direct flame.  Approximately 40
percent of  the  incoming solvent  remains in the  ink film and more  may  be
                                    -3-

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            <»••
                   Thermal  or
                   Catalytic  (
                   Incinerator •

                              '
                                     Ink Solvent and



r •* •
1
1
1
i- —


Thermal Degradation
Products
;
Heat i
Excr
*
l
Danger '
L__J

— 	 1
Shell
and
flat
Tube
Heat
Exchanger
Co
prc
orn
°2
air

                        Exhaust (an
                                                   I
                            Fan
                       [ Filter
                                                                                              Combustion
                                                                                              products
                                                                                              •Unburned
                                                                                              or n a nic s
                                                                                              02 depleted
                                                                                                 Fresh air
                                                          Filter
                                              Fan
                                              Gas
                                                    Air Heater
                                                    for dryer
                                           Ink  Solvent and
                                         Thermal Degradation
                                             Products
                  Heatset  Ink
Wash-up
solvents
      Water and
      Isopropaf
      vapor
        Neb
                                                                                            Printed Web (6 ,
                                   Water and
                                   isopropanol vapor
                Water1
Isopropanol
(With Dalgren
Dampening System)
               Figure 4.9-1.   Web offset  lithography  publication printing

           line emission points  (dashes  show  optional control  equipment).
                                                             11
                                                  -4-

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thermally degraded in a direct flame dryer.  The web passes over
chill rolls prior to folding and cutting.  For newspaper work, no
dryer is used, and most of the solvent  is believed to remain  in the
ink film on the paper.^

4.9.1.3  Web Letterpress—Letterpress is the oldest form of printing
(limited to movable types) and still predominates in periodical and
newspaper publishing, although numerous major newspapers are  convert-
ing to web offset.  In letterpress printing, the image area is raised
relative to the nonimage area, and the  ink is transferred to  the paper
directly from the image surface.  The image carrier may be made of
metal or plastic.  Only web presses using solvent-borne inks  are
discussed here because letterpress newspaper and sheet fed printing
use oxidative-drying inks which are not a source of volatile  organic
emissions.  Figure 4.9-2 shows one unit of a web publication
letterpress line.

   Publication letterpress printing uses a paper web that is  printed
on one side at a time and dried after each color is applied.  The inks
employed are heatset and usually contain about 40 volume percent sol-
vent.  The solvent in high-speed operations is generally a selected
petroleum fraction akin to kerosene and fuel oil, with a boiling point
of 200-370°C (4'00-700°F).13

4.9.1.4  Rotogravure--!n gravure printing, the image area is
engraved or "intaglio" relative to the  surface of the image carrier,
which is a copper plated steel cylinder that is usually also  chrome
plated to enhance wear resistance.  The gravure cylinder rotates in an
ink trough or fountain.  The ink is picked up in the engraved area,
                                   -5-

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                  Thermal
                Incinerator
                               Heat
                           I   Exchanger
                           I	
                                                                  i
                                                                  I
                                                                  Notary
                                                                  ~"  Head
                                                                  lExchor
                                  Comb istm-
                                  products
                                  Unb.irned
                                  organics
                                  C> Depleted
Web


















Exn

















lust

















18















nf



i





*^





Fan
/-
V
P
Heatset Ink
1








GD





•




»•

J





\ filter |

































,


c



















1 ] Tresh air
filter




Fan
•N
1





Air








i












Heater


For


Dryer





I Gas
















1 L 	
I
t
I
i
i
i
i
' only when
Gas , catalytic
' i unit is
_ _ _ * _ _ 1 , used here
Catalytic j J
—Incinerator . ]
,1
1 ,
l-r --J1

ST\

Solvent and thermal
degradation product*








Wash-up
solvents
Tunnel
or
Floater f*)\
Dryer ^—

















) Supply fan
Air and smoke

Chill

©

                                     Printed Web

                                        (4)
                                             I
Air
                                                               Air
                                                                           Cool water
            Figure  4.9-2.   Web  letterpress publication  printing
        line emission points  (dashes  show optional  equipment).
                       11
                                      -6-

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and excess ink is scraped off the  nonimage  area with a steel  "doctor
blade".  The image is transferred  directly  to the web when  it is
pressed against the cylinder by  a  rubber  covered impression  roll.
The product is then dried.  Rotary gravure  systems are known  as
"rotogravure" presses.

   Rotogravure can reproduce illustrations  with excellent color con-
trol, and it may be used on coated or uncoated paper, film,  foil and
almost every other type of substrate.   Its  use is concentrated in  (1)
publications and advertising such  as newspaper supplements,  magazines
and mail order catalogues; (2) folding  cartons and other flexible
packaging materials; and (3) specialty  products such as wall  and
floor coverings, decorated household paper  products, vinyl  upholstery
and health products.  Figure 4.9-3 illustrates one unit of  a  publica-
tion rotogravure press.  Multiple  units are required for multiple
color printing.

   The inks used in rotogravure  publication printing contain from  55
to 95 volume percent low boiling solvent, and they must have low vis-
cosities.  Typical gravure solvents  include alcohols, aliphatic naph-
thas, aromatic hydrocarbons, esters, glycol-ethers, ketones  and nit-
roparaffins.  Water based inks are in regular production use in some
packaging and specialty applications, such  as sugar bags.

   Rotogravure is similar to letterpress  printing in that the web  is
printed on one side at a time and  must  be dried after the application
of each color.  Thus, for four color, two-sided publication  printing,
eight presses are employed, with each press  including a pass  over  a
                                   -7-

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Tottmosp

here
Traces of
water and
solvent

i
i Solv
T Hot water
1 Solvent Still l
J — " i I" ~\ Mixture
^ ' Condenser | ^ ' Decanter | Warm
i 	 	 | I 	 Jwater | 	 _,
Ji Cool water
Steam Plus
Solvent Vapor f ~\
fc* 1 ^B_^^.i«-.^«
Adsorber j products
,_ 	 	 J r__ 1 .
1

1 Activated Carbon [^ "^ J
1 Adsorber j ' 	 T~P
1 1 GasT 1 ,
                                                                      Air 'Water
                                                   Solvent-laden air
Web
Ink
1 •








Ink Fountain








^^^^^^




i i

Press
(One
Unit)
(D







^ 1


Steam Drum or


(3)

^



r*hi 1 1 Rnllc

©




^Air f IT T |T Cool weier
1 1 f Heat Alr
Alr from
steam,
hot water,
or hot air
Printed
  Web
         Figure 4.9-3.  Rotogravure and flexography printing line
       emission points (dashes  show optional control  equipment).11
                                   -8-

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steam drum or through a hot air dryer at 38-93°C  (100-200°F), where
nearly all of the initial  solvent  is removed.3

4-9.1.5  F1exography--In flexographic printing, as in  letterpress, the
image area is raised above the surface of the plate.   The distinction
is that flexography uses a rubber  image carrier and alcohol based
inks.  The process is usually web  fed and is employed  for medium or
long multicolor runs on a  variety  of substrates,  including heavy
paper, fiberboard, metal and plastic foil.  The major  categories of
the flexographic market are flexible packaging and laminates, multi-
wall bags, milk cartons, gift wrap, folding cartons, corrugated paper-
board (which is sheet fed), paper  cups and plates, labels, tapes, and
envelopes.  Almost all milk cartons and multiwall bags and half of
flexible packaging are printed by  this process.

   Steam set inks, employed in the "water flexo"  or "steam set flexo"
process, are low viscosity inks of a paste consistency that are gelled
by water or steam.  Steam  set inks are used for paper  bag printing,
and they produce no significant emissions.  Water based  inks, usually
pigmented suspensions in water, are also available for some flexo-
graphic operations, such as the printing of multiwall  bags.

   Solvent-based inks are  used primarily in publication  printing, as
shown in Figure 4.9-3.  Like rotogravure, flexography  publication
printing uses very fluid inks, containing about 75 volume percent or-
ganic solvent.  The solvent, which must be compatible  with rubber, may
be alcohol or alcohol mixed with an aliphatic hydrocarbon or  ester.
Typical solvents also include glycols, ketones and ethers.  The inks
dry by solvent absorption  into the web and by evaporation, usually in
high velocity steam drum or hot air dryers, at temperatures below
              3 13
120°C (250°F). '    Like letterpress publishing,  the web is printed
                                   -9-

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on only one side at a time.  The web passes over chill rolls after
drying.

4.9.2  Emissions and Controls

4.9.2.1  General—Significant emissions from printing operations con-
sist primarily of volatile organic solvents.  Such emissions vary with
the printing process, ink formulation and coverage, press size and
speed, and operating time.  The type of paper, coated or uncoated, has
little effect on the quantity of emissions, although  low levels of
organic emissions are derived from the paper stock during drying.^
High volume web fed presses such as those discussed in Section 4.9.1
are the principal sources of solvent vapors.

   Total annual emissions from the industry in 1976 were estimated to
be 340,000 MT (380,000 tons).  Of this total, lithography emits 28
percent, letterpress 18 percent, gravure 41 percent and flexography 13
percent.^

   Most of the solvent contained in the ink and used  for dampening and
cleanup eventually finds its way into the atmosphere, but some solvent
remains with the printed product as it leaves the plant and is re-
leased to the atmosphere later.  Overall solvent emissions can be
computed from Equation 1 using a material balance concept, except in
cases where a direct flame dryer is used and some of  the solvent is
thermally degraded.
                                   -10-

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          Etotal=T
where
     Etotal = to1:al solvent emissions including those from the
              printed product, kg  (pounds)

     T      = total solvent usage  including solvent contained in ink,
              kg (pounds)

   The solvent emissions from the  dryer and other components that are
connected to the main exhaust system can be computed from Equation 2.
The remaining solvent leaves the plant with the printed product and/or
is degraded in the dryer.

          Edryer = SI   (100 - P)                             (2)
           aryer  100     100
where
     E .      = solvent  emissions from dryer, kg (pounds)

     I       = ink usage in kg (pounds)

     S and P = factors  from Table  4.9-1

4.9.2.2  Web Offset Lithography—Emission points on web offset litho-
graphy publication printing lines  include:  (1) the ink fountains, (2)
the dampening system, (3) the plate and blanket cylinders, (4) the dryer,
(5) the chill rolls and  (6) the product.  Emission point numbers refer to
Figure 4.9-1 .

   Alcohol is emitted from points  2 and 3.  Washup solvents are a small
source of emissions from points 1  and 3.  Drying is the major source be-
cause 40 to 60 percent  of the ink  solvent is removed from the web during
this process (emission  point 4).
                                    -11-

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  The quantity of web offset emissions may be estimated from Equation 1
  or from Equation 2 and the appropriate parameters from Table 4.9-1.
  Table 4.9-1.  TYPICAL PARAMETERS FOR COMPUTING SOLVENT EMISSIONS FROM
  UNCONTROLLED WEB OFFSET LITHOGRAPHY, WEB LETTERPRESS, ROTOGRAVURE AND
                       FLEXOGRAPHY PRINTING LINES3
Process
WEB OFFSET
Publ ication
Newspaper
WEB LETTERPRESS
Publication
Newspaper
ROTOGRAVURE
FLEXOGRAPHY
Typical Solvent
Content of Ink
(percent)
S

40
5

40
0
75
75
Typical Solvent Remaining in
Product and Destroyed in Dryer
(percent)
P

40 - hot ai r dryer
60 - direct flame dryer
100

40
(not applicable)
2 - 7
2 - 7
Emission
Factor
Rating

A
B

B

C
C
a References 1 and 14.  For certain packaging products, the amount of
  solvent retained is regulated by the FDA.
                                      -12-

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4-9.2.3  Web Letterpress—Emission points on web  letterpress publica-
tion printing lines are:  (1) the press  (which includes the image
carrier and inking mechanism),  (2) the dryer, (3) the chill rolls and
(4) the product.  Emission point numbers refer to Figure 4.9-2.

   Web letterpress publication  printing  produces  significant emis-
sions, primarily from the ink solvent, about 60 percent of which is
lost from the drying process  (point 2).  Wash-up  solvents  are  a small
source of emissions (point 1).  The quantity of emissions  can  be com-
puted as discussed above for  web offset.

   Letterpress publication printing uses a variety of papers and inks
that lead to problems in emission control, but losses can  be reduced
by use of a thermal or catalytic incinerator, either of which  may be
coupled with a heat exchanger.

4.9.2.4  Rotogravure—Emissions from  rotogravure  printing  occur at
(1) the ink fountain, (2) the press,  (3) the dryer and (4) the chill
rolls.  Emission point numbers  refer  to  Figure 4.9-3.  The dryer is
the major emission point, because most of the VOC in the low boiling
ink is removed during drying.   The quantity of emissions can be com-
puted from Equation 1 or from Equation 2 and the  appropriate para-
meters from Table 4.9-1.

   Ventilation systems are necessary  to  minimize  solvent loss  around
the ink fountain and at the chill rolls  (points 1 and 4).  Fume in-
cinerators and carbon adsorbers are the  only devices that  have a high
efficiency in controlling vapors from rotogravure operations (points
1 to 4).
                                    -13-

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   Solvent recovery by carbon adsorption  systems has been quite suc-
cessful at a number of large publication  rotogravure plants. These
presses use a single, water immiscible solvent  (toluene) or a simple
mixture that can be recovered in approximately the proportions used in
the ink.  All new publication gravure plants are  being designed to
include solvent recovery.

   Some smaller rotogravure operations, such as those that  print and
coat packaging materials, use complex solvent mixtures in which many
of the solvents are water soluble.  Thermal incineration with heat
recovery is usually the most feasible control option for such oper-
ations.  With adequate primary and  secondary heat recovery, the amount
of fuel required to operate both the incinerator and the dryer system
can be reduced to less than that normally required to operate the
dryer alone.

   In addition to thermal and catalytic incinerators, pebble bed in-
cinerators are also available.  Pebble bed  incinerators combine the
functions of a heat exchanger and a combustion  device, and  can achieve
a heat recovery efficiency of 85 percent.

   VOC emissions can also be reduced by using low solvent inks.
Water-borne inks, in which the volatile portion contains up to 20
volume percent water soluble organic compounds, are used extensively
in rotogravure printing of multiwall bags,  corrugated paperboard and
other packaging products, although  water  absorption into the paper
limits the amount of water-borne ink that  can be printed on thin stock
before the web is seriously weakened.
                                    14-

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4.9.2.5 Flexography—Emission points on flexographic printing lines
are (1) the ink fountain, (2) the press, (3) the dryer and (4) the
chill  rolls.  Emission point numbers refer to Figure 4.9-3.  The dryer
is the major emission point, and emissions can be estimated from Equa-
tion 1 or from Equation 2 and the appropriate parameters from Table
4.9-1.

   Ventilation systems are  necessary to minimize solvent loss around
the ink fountain and at the chill rolls (points 1 and 4).  Fume incin-
erators are the only devices that have proven highly efficient  in  con-
trolling vapors from flexographic operations  (points 1 to 4).   VOC
emissions can also be reduced by using water-borne  inks, which  are
used extensively in flexographic printing of  packaging products (refer
to Section 4.9.2.4).

   Table 4.9-2 shows estimated control efficiencies for the  printing
operations discussed herein.
                                    -15-

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  Table 4.9-2.  ESTIMATED CONTROL TECHNOLOGY EFFICIENCIES FOR WEB
       OFFSET LITHOGRAPHY, WEB LETTERPRESS, ROTOGRAVURE AND
                    FLEXOGRAPHY PRINTING LINES
Emission Technology
      Application
  Reduction in
Organic Emissions
    (percent)
 Carbon adsorption
 Incineration3
 Water-borne inks"
Publication rotogravure
  operations
Web offset lithography

Web letterpress

Packaging rotogravure
  printing operations

Flexographic printing
  operations
Some packaging rotogravure
  printing operations0

Some flexographic packaging
  printing operations
      95e

      95*
      60d



     65-75d


      60d
a Direct flame  (thermal)  catalytic  and  pebble  bed.  Three  or more
  pebble beds in a system have a  heat recovery efficiency  of 85
  percent.

b Inks  in which the  solvent  portion consists of  75  volume  percent
  water and 25  volume  percent organic solvent.

c with  less demanding  quality requirements.

d Reference 3.  Overall  emission  reduction  efficiency.

e Reference 12.  Efficiency  of volatile  organic  removal—does  not
  take  into account  capture  efficiency.

f Reference 13.  Efficiency  of volatile  organic  removal--does  not
  take  into account  capture  efficiency.
                                  -1C-

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 References for Section 4.9
 1.   "Air Pollution Control  Technology  Applicable  to 26 Sources of
     Volatile Organic  Compounds",  Office  of  Air Quality Planning and
     Standards,  U.S.  Environmental  Protection  Agency,  Research
     Triangle Park, NC,  May  27,  1977.

 2.   Peter N. Formica,  Controlled  and Uncontrolled Emission Rates and
     Applicable  Limitations  for  Eighty  Processes,  EPA-340/1-78-004,
     U.S. Environmental  Protection Agency, Research Triangle Park,
     NC,  April  1978.

 3.   Edwin J. Vincent  and William  M.  Vatavuk,  Control  of  Volatile
     Organic Emissions  from  Existing  Stationary Sources,  Volume VIII:
     Graphic Arts - Rotogravure  and"F1exography,  EPA-450/2-78-033,
     U.S. Environmental  Protection Agency, Research Triangle Park,
     NC,  December 1978.

 4.   Communication with C. M.  Higby,  Cal/Ink,  Berkeley, CA, March 28,
     1978.

 5.   T.  W. Hughes, et  a!.. Prioritization of Air  Pollution from
     Industrial  Surface Coating  Operations,  EPA-650/2-75-019a. U.S.
     Environmental Protection  Agency, Research Triangle Park,  NC,
     February 1975.

 6.   Harvey F.  George,  "Gravure  Industry's Environmental  Program",
     Environmental Aspects of  Chemical  Use in  Printing Operations,
     EPA-560/1-75-005,  U.S.  Environmental  Protection Agency, Research
     Triangle Park, NC,  January  1976.

 7.   K.  A. Bownes, "Material of  Flexography",  ibid.

 8.   Ben H. Carpenter  and Garland  R.  Hilliard, "Overview  of Printing
     Processes and Chemicals Used", ibid.

 9.   R.  L. Harvin, "Recovery and Reuse  of Organic  Ink  Solvents", ibid.

10.   Joseph L.  Zborovsky, "Current Status of Web Heatset  Emission
     Control Technology", ibid.

11.   R.  R. Gadomski, et al., Evaluations  of  Emission and  Control
     Technologies in the Graphic Arts  Industries,  Phase I:  Final
     Report, APTD-0597, National Air  Pollution Control Administration,
     Cincinnati, OH, August  1970.
                                 -17-

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12.  R. R. Gadomski, et a!., Evaluations of Emissions  and Control
     Technologies In THe GrapFTc Arts Industries,  Phase  II:  Web~
     Offset and Metal Decorating Processess, APTD-1463,  U.S.
     Environmental Protection Agency, Research  Triangle  Park, NC,
     May 1973.

13.  Control Techniques for Volatile Organic Emissions from
     Stationary Sources, EPA-450/2-78-022,  U.S. Environmental
     Protection Agency, Research Triangle Park, NC,  May  1978.

14.  Communication with Edwin J. Vincent, U.S.  Environmental
     Protection Agency, Research Triangle Park, NC,  July 1979.
                                  -18-

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                        BACKGROUND DOCUMENT
                      SECTION 4.9  GRAPHIC ARTS
1.0  INTRODUCTION
     The section on Graphic Arts is organized as two separate
sections with five subsections each, as follows:
     4.9.1  Process Description
            4.9.1.1 General
            4.9.1.2 Web Offset Lithography
            4.9.1.3 Web Letterpress
            4.9.1.4 Rotogravure
            4.9.1.5 Flexograpy
     4.9.2  Emissions and Controls
            4.9.1.1 General
            4.9.1.2 Web Offset Lithography
            4.9.1.3 Web Letterpress
            4.9.1.4 Rotogravure
            4.9.1.5 Flexography
     Screen printing and manual techniques are not  included due to
the lack of available information.  Direct lithography,  in which the
image carrier prints the image directly onto the substrate, is also
not included because most lithographic operations are web offset
(although most  plants classified  under commercial lithography
operate with sheet fed equipment).  Sheet fed gravure is excluded
because it  is slow and little  used.  Of the three categories  of
letterpress printing, only web presses using solvent-borne inks are
discussed because
        Letterpress  newspaper  printing  (which  is  web  fed)  utilizes
        oxidant  drying  inks  composed  of  petroleum oils  and carbon
        black,  but  little or no  volatile solvent
        Letterpress  sheet fed  printing employs  nonsolvent  inks  that
            in  racks by air  oxidation at room  temperature
                                 -19-

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Moreover, flexographic newspaper printing, like letterpress
newspaper printing, uses oxidative drying inks and emits only ink
mist and paper dust, so this form of printing is also omitted from
Section 4.9.

2.0  EMISSION FACTORS (Table 4.9-1)

     The values for S, solvent content of ink, for web offset and
letterpress  were taken from Table 35 (pages 123-128) of Reference
11.  The information was obtained through mail surveys  (421 res-
ponses) and field visits (86) to printing establishments.  The
values for rotogravure and flexography were supplied by Ed Vincent
of ESED in a private communication.

     Values for P, the solvent remaining with the product  or
destroyed in the dryer, were taken from Table 35 of Reference 11 for
web offset and web letterpress, except for the value for web offset
using a direct flame dryer, which was taken from Table  18  (page  113)
of Reference 12.  The data from Reference 11 were derived  from
surveys and the data from Reference 12 were derived from source
tests.  Values for P for rotogravure and flexography were  supplied
by Ed Vincent of ESED 
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The term "capture efficiency" refers to the efficiency of conveying
all solvent emissions to the inlet of the control device.  The term
"removal efficiency" refers to the efficiency of the control device
in removing all emissions that pass through it.

4.0  EMISSION FACTOR RATINGS

     The factors are essentially  based on the data  base  for  estima-
ting the parameters S and P in Table 4.9-1.  The factor  for  web  off-
set publication printing is rated A because it  is based  on  results
of a test program specifically designed to evaluate emissions.   The
factors for web offset newspaper  and web  letterpress publication
printing are rated B because they are based on  a combination of
engineering analysis and limited  test data.  The factors for roto-
gravure and flexography are rated C because they are based  on  engi-
neerng analysis and plant visits  and may  have been  derived  by  aver-
aging data from several plants that varied substantially from  each
other.  The numerical rankings are as follows:
Process
Web Offset
Publication
Newspaper
Web Letterpress
Publication
Rotogravure
Flexography
Measured
Emissions

17
9

9
0
0
Process
Data

9
9

9
8
8
Engineering
Analysis

10
10

10
9
9
Total

36
28

28
17
17
                                 -21-

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 . REPORT NCX

 EPA No. 450/4-79-014
 Tl T I C A & i K ._.. .	  ' '• ~ ~   " "~
                                   TECHNICAL REPORT DATA
                            (Please read Instructions on the reverse before completing)
                                                           3. RECIPIENT'S ACCESSION NO.
	:	• ~y*/ -r i .
 TITLE AND SUBTITLE



Graphic Arts:   An AP-42 Update
                                                           5. REPORT DATE
                                                           6. PERFORMING ORGANIZATION CODE
                                                            September  1979
 AUTHOR(S)
                                                           8. PERFORMING ORGANIZATION REPORT NO.
 K.  Wilson and V.  Scott
 PERFORMING ORGANIZATION NAME AND ADDRESS
 Pacific Environmnetal  Services, Inc.
 1930 14th Street
 Santa Monica, California 90404
                                                           10. PROGRAM ELEMENT NO.

                                                            2AA635
                                                           11. CONTRACT/GRANT NO.
                                                            68-02-2583
                                                            Work Assignment No. 12
 2. SPONSORING AGENCY NAME AND ADDRESS
 Office of Air Quality Planning and Standards
 U.S.  Environmental  Protection Agency
 Research Triangle  Park,  North Carolina  27711
                                                           13. TYPE OF REPORT AND PERIOD COVERED
                                                            Final;  April to August  1979
                                                           14. SPONSORING AGENCY CODE
15. SUPPLEMENTARY NOTES
 EPA Project Officer:   Audrey McBath
16. ABSTRACT
      This document  contains the text of  AP-42 Section 4.9,  Graphic Arts, written  in
 May 1979.  The  section includes a description of four graphic  arts processes  (web
 offset lithography,  web letterpress, rotogravure, and flexography), process flow
 diagrams, and emissions and controls discussions.  A method for estimating emissions
 using theoretically  derived equations  is also included.  A  background document which
 discusses, in some  detail, the derivation of emission quantification methodologies
 follows the Section  itself.
                                KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
                                              b.IDENTIFIERS/OPEN ENDED TERMS
                                                                         c.  COSATI field/Group
 emission factors
 air pollution  control
 evaporation  loss sources
 graphic arts industry
 solvent use
"18 DISTRIBUTION STATEMENT

 Unlimited
                                              19 SECURITY CLASS /This Report)
                                               Unclassified
21 NO OF PAGE!
   26
                                               20 SECURITY CLASS (This page)
                                                Unclassified
                                                                          22 PRICE
EPA Form 2220-1 (R«».4-77)   PBEVI
                           OUS EDITION IS OBSOLETE

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