O EPA REPORT NUMBER 72-PC-ll AIR EMISS CHAMPION INTERNATIONAL Pasadena, Texas UNITED STATES ENVIRONMENTAL PROTECTION AGENCY Office of Air and Waste Management Office of Air Quality Planning and Standards Emission Measurement Branch Research Triangle Park. North Carolina ------- SOURCE TEST REPORT EPA No.: 72-PC-ll. Particulate and Gaseous Emissions From A Kraft Pulp Hill U. S. PLYWOOD - CHAMPION PAPERS Pasadena, Texas EPA Contract No.: 68-02-0232 Task No.: 7 Environmental Engineering, Inc. 2324 Southwest 34th Street Gainesville, Florida 32601 ------- TABLE OF CONTENTS Page Number(s) I. INTRODUCTION 1 II. SUMMARY AND DISCUSSION OF RESULTS 2-6 TABLE 1 - TRS Daily Averages 4 TABLE 2 - Participate and Sulfur Dioxide Emissions 5 TABLE 3 - Carbon Dioxide, Oxygen, and Carbon Monoxide Concentrations 6 TABLE 4 - Nitrogen Oxide Concentrations No. 6 Recovery Furnace Outlet 6 III. PROCESS DESCRIPTION AND OPERATION 7-16 Figure 1 - Flow Diagram of Recovery Furnace and Black Liquor Oxidation System .... 8 TABLE 5 - Summary of the Recovery Furnace Process Data 13 TABLE 6 - Sodium Sulfide Concentrations in Black Liquor Fed to the Direct Contact Evaporator 14 TABLE 7 - Summary of Process Data for the Black Liquor Oxidation System 15 TABLE 8 - Summary of Process Data for the Electrostatic Precipitator 16 IV. LOCATION OF SAMPLING POINTS 17-18 Figure 3 - Top View of Particulate Sampling Ports 18 V. SAMPLING AND ANALYTICAL PROCEDURES 19-32 Figure 4 - GC Gas Sampling System 21 Figure 5 - Barton Sampling System 23 Figure 6 - Particulate and S0? Train 26 Figure 7 - C02> 02> and CO Sampling System ... 30 ------- I.. INTRODUCTION In accordance with Section 111 of the Clean Air Act as amended of 1970, the Environmental Protection Agency is charged with the establishment of performance standards for new stationary sources which may contribute significantly to air pollution. These standards are based upon the best air pollution control technology that has been demonstrated. This report presents the results of an extensive source testing program conducted at Champion Paper Company, Pasadena, Texas, June 3-9, 1972, to obtain data for a partial basis in consideration of new source performance standards in the kraft pulping industry. Stack emissions were measured from the chemical recovery boiler for particulate, sulfur dioxide, reduced sulfur compounds, oxides of nitrogen, carbon dioxide, carbon monoxide, and oxygen. Emissions from the first and second stages (individually vented) of the black liquor oxidation system were also measured for sulfur dioxide and reduced sulfur. The recovery boiler utilizes a cascade direct contact evaporator and strong black liquor oxidation and exit gases are controlled with an electrostatic precipitator. Reduced sulfur compounds were measured by flame photometric gas chromatography and coulometric titration. Carbon monoxide and carbon dioxide were measured with infrared analyzers and oxygen was monitored with a paramagnetic oxygen analyzer. All other stack emissions were measured with .EPA reference methods. 1 ------- II. SUMMARY AND DISCUSSION OF RESULTS Table 1 summarizes results of gaseous sulfur determinations utilizing both flame photometric and coulometric detection systems. All summary results are reported in terms of TRS as hLS. TRS is defined as hydrogen sulfide plus methyl mercaptan plus dimethyl sulfide plus dimethyl disulfide; all compounds are reported as hydrogen sulfide. It should also be noted that dimethyl disulfide (RSSR) con- centrations, determined with the chromatographic system, are assumed to yield twice those concentrations when considered as hydrogen sulfide. Complete gaseous sulfur data is contained in Appendix A. Results from the particulate emission tests on the recovery furnace are shown in Table 2. Emission rates were calculated on the basis of the moisture content determined from a separate moisture test instead of the condensed moisture in the impingers. The reason for this is that the evaporation rate of the isopropanol in the impingers was found to be excessive based upon previous tests. The third and fourth impingers, which contained 3% hydrogen peroxide, were analyzed for sulfur dioxide by using barium perchlorate titrations. The data are also included in Table 2. Complete particulate and sulfur dioxide data are contained in Appendix B. Daily mean concentrations for oxygen, carbon dioxide, and carbon monoxide are presented in Table 3. The results are reported on a dry ------- gas basis. Complete results of the gas concentrations at 15-minute intervals are included in Appendix C. The results from the nitrogen oxide emission testing are summarized in Table 4. Complete NO data are included in Appendix B. A ------- Table 1 TRS DAILY AVERAGES (Coulometric and Flame Photometric Detection) U. S. PLYWOOD - CHAMPION PAPERS Pasadena, Texas Date 6-3-72 6-4-72 6-5-72 6-6-72 6-7-72 6-8-72 6-9-72 Source PPT Outlet PPT Outlet PPT Outlet PPT Outlet PPT Outlet PPT Outlet 1st Stage BLO (5) 2nd Stage BLO Flame Photometric Detection ppm (1) 2.02 (2) 1.41 (3) 1.40 1.54 0.77 1.58 38.90 23.25 Ibs/hr 1.54 1.06 1.06 1.16 0.58 1.20 1.21 0.62 Ibs/ADTP Coulometric Detection ppm 4.1 2.9 2.7 2.5 2.9 3.1 48.8 6.8 Ibs/hr 3.13 2.19 2.04 1.88 2.19 2.35 1.52 0.18 Ibs/ADTP . (1) Parts per million by volume - Dry Gas Basis (2) H2S only (3) RSR & RSSR (4) }^S & RSH (5) BLO - Black Liquor Oxidation ------- • TABLE 2 PARTICULATE AND SULFUR DIOXIDE EMISSIONS Date Time Began Time End Barometric Pressure, In. Hg Absolute Meter Orifice Pressure Drop, In.'H20 3 Vol. Dry Gas @ Meter Conditions, ft Average Gas Meter Temperature, °F. Vol. Dry Gas @ S.T.P.*, ft Stack Gas Moisture, %,Volume % C02 % 02 % CO % N2 Average Stack Gas Temperature, °F. Stack Pressure, In. Hg Absolute Stack Gas Velocity @ Stack Cone!. ., fpm Stack Gas Flow Rate @ S.T.P.", scfm Net Time of Test, min. Percent Isokinetic Particulate Concentrations, grains/scf Front half and Filter Total Particulate Emissions, Ibs/hr Front half nnd Filter Total Particulate Emissions, Ibs/ton Front half and Filter 1 S02 Emissions, Ibs/hr Run #1 6/3/72 12:45 18:23 30 0.14 42.431 86 41.312 25.5 10.4 10.7 0 78.9 314.2 30.07 4633 141512 180 113.4 0.085 0.184 103.32 223.04 4.13 8.92 14.77 Run 12 6/5/72 9:25 13:05 30 0.14 42.530 87 41.333 25.3 10.7 11.4 0 77.9 304.2 30.07 4683.6 145321 200 99.4 0.096 • 0.199 110.07 248.18 4.40 9.93 63.82 Run #3 6/6/72 9:52 13:32 30 0.09 45.294 89 43.853 21.9 11.8 10.1 0 78.1 302.6 30.07 4554.1 148042 200 103.5 0.092 0.197 116.51 250.03 4.66 10.00 Neg. i Based upon 600 tons ADP/day ------- Table 3 Carbon Dioxide, Oxygen, and Carbon Monoxide Concentrations Date 6/3/72 6/4/72 6/5/72 6/6/72 6/7/72 6/8/72 Daily Averages CO (ppm) • 153 93 84 95 102 51 co2 % 10.4 8.2 10.7 11.8 12.9 11.1 o2 % 10.7 11.4 11.4 10.1 10.1 9.9 Table 4 Nitrogen Oxide Concentrations No. 6 Recovery Furnace Outlet Date 6/3/72 6/5/72 6/6/72 Time 1605 1830 1400 1630 1700 1440 1535 1600 NOX, ppm 19.3 19.8 19.8 24.2 17.9 20.2 34.3 34.5 ------- III. PROCESS DESCRIPTION AND OPERATION The Champion International Plant at Pasadena, Texas is a complete mill, producing 600 tons of fine paper and newsprint per day from its own bleached kraft pulp and groundwood. The EPA test program at this mill was limited to two facilities; the black liquor oxidation system, and the recovery furnace system. These systems are a small but important part of the plant complex, and are part of the process for recovering spent cooking chemicals from the kraft pulping operation. Diagrams of both systems are shown in Figure 1. Process Description A. General The mill produces kraft pulp by cooking wood chips in white liquor, a water solution of sodium hydroxide and sodium sulfide. The spent cooking solution, called black liquor, is treated to regenerate cooking solution. During regeneration, the black liquor is concentrated in evaporators and then burned in a recovery furnace. At the furnace bottom, inorganic chemicals are recovered as a sodium carbonate-sodium sulfide smelt. The molten smelt is tapped off and dissolved in water. The resulting mixture, called green liquor, is drawn from the dissolving tank and treated with lime to complete the regeneration of cooking solution. Heat released in the recovery furnace from combustion of the black liquor is used to generate process steam and to complete the evaporation of additional black liquor. The recovery furnace, sometimes called a ------- Contact Evaporator iquor Atnosphore black liquor let Sta-;-: Oxidation lc-ctrostot 'reel pita tor black — liquor (oxidized) Atmosphere 2nd Starjc Oxidation air Stack Figure 1 . Flov/ Oiagrar: of ".ocovary Furnace and Black Liquor .Oxidation systo,.i. 8 ------- recovery boiler, employs water walls and boiler tubes to absorb part of the available heat. Combustion gases leave the furnace at about 700°F and go to a direct contact evaporator; black liquor, fed counter- currently to this unit, contacts the hot gases directly and is evaporated to a solids content of about 60 percent. The concentrated liquor is sprayed into the furnace; combustion gases leaving the direct contact evaporator are cleaned in an electrostatic precipitator and then vented to the atmosphere through a tall stack. Chemical reactions between the combustion gases and black liquor in the direct contact evaporator can generate hydrogen sulfide. To inhibit these reactions the black liquor is first sparged with air in a two stage oxidation system. Oxidation converts sulfide in the liquor to thiosulfate and effectively reduces subsequent hydrogen sulfide formation. B. Recovery Furnace System The test unit was installed in 1958 and designated the #6 recovery furnace. This furnace was designed by Babcock and Nil cox for a heat input of 575 million BTU per hour, equivalent to a pulp production rate of 650 tons per day. Associated with this furnace is a cascade direct contact evaporator. A portion of the product steam is used to blow soot from the boiler tubes. Tubes are cleaned continuously, one section at a time. ------- C. Oxidation System The oxidation system was designed by Champion to oxidize strong black liquor by sparging with air in two sequential stages. The first stage was installed in 1951 and the second stage in 1967." In each stage, air is blown through the black liquor and vented through a cyclone to the atmosphere. Number 2 heating oil is pumped to the second stage at about 15 gallons per hour to inhibit foaming, and each stage has a foam breaker. Black liquor from the cyclones and foam breakers are recycled. The oxidation system serves two recovery furnaces with a total equivalent pulp production of 900 tons per day. D. Electrostatic Preci pita tor The precipitator was designed for a collection efficiency of 98 percent and installed by the Koppers Company in 1958. Inlet gas is divided into three parallel chambers, and each chamber has three fields. The inlet fields of chambers 1 and 2 are coupled electrically; the center fields of chambers 2 and 3 are also coupled. Accordingly, the precipitator has seven separately controlled sections. Rappers operate every 2 1/2 minutes; during each cycle the inlet sections rap for 5 seconds, followed by the center sections for 10 seconds, and the outlet sections for 15 seconds. Salt cake drops to the hoppers and is recycled to the recovery furnace by circulating black liquor. Process Operation During testing, records were kept of process variables for the recovery furnace, electrostatic precipitator, and the black liquor 10 ------- oxidation system. Wherever process monitors were available, operating conditions that affect emission rates were recorded. The raw process data sheets and a key explaining the entries are included in the Appendix D. A. Recovery Furnace The process records, as well as statements by the operators, indicate that during the tests the recovery furnace was operated normally. The observed ranges of major operating, variables are given in Table 5; where information is available from the company, the design and normal values are also shown. As seen from the table, black liquor feed rate, solids content, and steam temperature, pressure, and production rate, were all within a few percent of normal; reduction ratio was greater than 95 per- cent, as proper. (Reduction ratio, determined from green liquor samples, is the concentration of sodium sulfide divided by the sum of sodium sulfide and sodium carbonate concentrations.) These records show that the furnace received a normal charge and performed its major functions (production of smelt and steam) in a normal way during the tests. Many operating parameters (such as distribution of furnace combustion air, manner of spraying feed liquor, etc.) affect furnace emissions. Those that could be monitored were recorded. There is no indication from the records or from operators' statements that unusual practices were followed. The sodium sulfide concentration in black liquor fed to the direct contact evaporator is a process variable of special interest, because of its strong influence on the generation of hydrogen sulfide. Sulfide levels are determined routinely by the Company and were made available for the 11 ------- test period. As shown in Table 6, sulfide levels were frequently unde- tectable; the highest levels (June 5 and 6) caused no measurable increases in hydrogen sulfide emissions. B. Black Liquor Oxidation System A limited amount of process data was obtained June 9 during tests on the oxidation system. Readings of the available process monitors were recorded on data sheets included in the appendix. These data are sum- marized in Table 7. As far as known from the process data and statements by the operators, the oxidation system was operated normally during the test. C. Electrostatic Precipitator Precipitator operation was monitored during all the furnace tests. Primary current, secondary current, and secondary voltage in each of the seven control sections were recorded hourly. The raw data sheets are included in the appendix. These data are summarized in Table 8; information supplied by Champion International on design and normal operating conditions is included where available. During most of the particulate sampling the precipitator was operated normally. The major exception occurred in the first run; during the last hour of sampling, the primary current in one control section dropped from about 78 to 46 amperes. (Particulate emissions, however, were lowest for this run.) The second run was postponed a day until the precipitator was repaired. When the faulty section was cleaned out and several damaged collector plates were welded into place, normal current was restored. 12 ------- Table 5. SUMMARY OF THE RECOVERY FURNACE PROCESS DATA Operating Condition Black Liquor Feed Rate Black Liquor Solids Content (r) Steam Production v; Steam Temperature Steam Pressure Reduction Ratio'6' Units GPM Wt. % 103 Ib/hr °F psig x Design^3 200(b) 67 299 750 375 During Item No. \ Test on Data ' Normal 6/3-8/72 Sheets 208 214-223 65 64.2-66.5 225^ 200 - 255 700 670 - 750 330 321 - 357 95.7 - 97.1 10 14 1 4 5 ^'Information supplied by Champion. International. * 'Calculated by Champion International from design heat input using current operating parameters. (c) v 'Net production, not including steam used for soot blowing in the recovery furnace. * 'Original design did not contemplate current rate of saturated steam usage for soot blowing. 13 ------- Table 6. SODIUM SULFIDE CONCENTRATIONS IN BLACK LIQUOR FED TO THE DIRECT CONTACT EVAPORATOR Date 1972 3 - 4 4 5 5 6 6 i i 7 3 9 Time 24 hour 1330 0700 1430 0730 1500 0745 1530 0645 0710 1315 0640 Sodim Sulfide^ gra^s/litcr 0.0 0.117 0.0 0.390 0.0 0.2£5 0.156 0,195 0.0 0.0 0.0 (a) Determined by Champion International by potentiometric titration. 14 ------- Table 7. SUMMARY OF PROCESS DATA FOR THE BLACK LIQUOR OXIDATION SYSTEM Stage 1 Operating Condition Black Liquor Feed Rate Air Feed Rate Air Feed Pump Pressure Units GP;i SCR! psig Design 535 6000 G Morr.ial 542 During Test (6/9/72) 350 - 500 not Measured G 1/4 - G 1/2 Statie 2 1 \ "t \~ Air Our inn last Operating Condition rr~~ j ^-4--, t '*. v; o • \Lt vv- Feed P-j.np Pressure Units CCF,I PS13 Ocsiqn 3000 C formal (J/S/72) nr\ t1 n,'i;i c : i r ••»."• 6 3/4 NOTE: Stage 2 liquor feed rate is not measured; it is slightly less than stage 1 because of evaporative water losses in stage 1. 15 ------- Table 8. SUMMARY OF PROCESS DATA FOR THE ELECTROSTATIC PRECIPITATOR Operating Condition Gas Volume Gas Temperature Inlet Loading Outlet Loading Efficiency Primary Current Primary Voltage Secondary Voltage Secondary Current Units 103 ACFM °F gr/SDCF gr/SDCF amps volts 103 volts Design 281 325-350 2.5-6.0 0.05^ 98 90 440 65 Normal 265 325 4.0 97.5 85-95 45-60 During Test 6/3,5,6/72 273-281 303-314 0. 085-0. 096^ 46 - 96(c) 310 - 400 325 - 490 (a) (b) (c) Texas Air Control Board method; similar to EPA Method 5. EPA Method 5; front half only. Primary current in one control section was low for about 30 minutes; minimum current at all other times during particulate testing was 70 amps. 16 ------- IV. LOCATION OF SAMPLING POINTS The outlet stack from the electrostatic precipitator on the No. 6 recovery furnace was sampled at the rectangular duct entering tnto the vertical stack, as shown in Figures 2 and 3. The traverse points sampled in each of the four ports are as follows: Distance From Sample Point No. Inside Hall, In. 1 5 3/4 2 17 1/4 3 28 3/4 4 40 1/4 5 51 3/4 6 63 1/4 7 74 3/4 8 86 1/4 9 97 3/4 10 109 1/4 NOTE: The traverse points were utilized for determination of particulates, gas volumes, moisture and other necessary stack gas parameters. The gaseous constituents were extracted from the source gas stream based upon the assumption that the gases were homogeneously mixed. Therefore, gaseous sulfurs, nitrogen oxides, carbon dioxide, oxygen and carbon monoxide were sampled from relatively fixed points in the gas handling system. 17 ------- Electrostatic Precipitator 3-Ducts Manifold Four Participate Sampling Ports Gas Sampling Ports V Stack SIDE VIEW OF MO. 6 RECOVERY FURNACE GAS OUTLET Figure 2 6 I. 21" | 30" I 22" |S" ^^iro1 &~*y- f'~<^ ^-4'? •"•• 6 6 (!) 6 Flow . TOP VIEW OF PARTICULATE SAMPLING PORTS .Figure 3 18 ------- V. SAMPLING AND ANALYTICAL PROCEDURES Chromatographic Sampling System Figure 4 illustrates the ;ystem which v/as emoloyed in conveying the gases from the source to the sensing equipment. The stainless steel probe and Teflon sampling line were maintained at temperatures exceeding the dew point of the source gases. The sampling line consisted of an insu.lated, electrically heated 1/4-inch Teflon tube. The sample gases were transmitted to the heated dilution box where they were split into two separate streams. One stream was conveyed to the vacuum source and wasted to minimize lag time in the sampling line. The remainder of the flow was diluted with nitrogen by an amount sufficient to lower the dew point of the gases below ambient temperature. A portion of this diluted sample was injected into the chromatograph through the Gas/Liquid Chromatograph (GLC) sampling valve. The remainder of the diluted gas was wasted through the vacuum source. Chromatographic Analysis Gaseous sulfur concentrations were determined with a Tracer Model 250 Gas/Liquid Chromatograph. This unit is equipped with a flame photometric detector which is specifically for sulfur compounds. Two analytical columns were utilized in the separation and analysis of the gaseous sulfur compounds. One was a 36-foot by 1/8-inch OD Teflon column packed with polyphenyl ether liquid phase on a solid support of grannular Teflon with stripper column. The second column, constructed of identical materials, v/as 8 feet long. Both columns were operated at 50°C. 19 ------- The 36-foot column was utilized for analyzing hydrogen sulfide, sulfur dioxide, and methyl mercaptan while the 8-foot column facilitated the analysis of dimethyl sulfide and dimethyl disulfide. The chromatograph was calibrated for hydrogen sulfide, sulfur dioxide, methyl mercaptan, dimethyl sulfide, and dimethyl disulfide, using the spinning syringe technique. 20 ------- Stack . XGlass J\\ 7 Wool Dilution Nitrogen Heated Sample ne 4"Teflon (_.J /. GC GAS SAMPLING SYSTEM Figure 4 ~(5?) Carrier Gas (N2) Gas Chromatograph GC Sampling Valve Vacuum Pump ,M: Rotameter ><) : Metering Valve ------- '•-• '.Couloinetric DatectoK.(Barton Titrator) •;.'."'••'• Figure 5' illustrates the system which was employed in conveying .",'• *'• "*• / ;..;;- '•'•'.- the gases from the source to the Barton Titrator. The stainless steel . probe and Teflon sampling line were maintained at temperatures exceeding the dew point of the stack gases. The sampling line was the same as the sampling line used with the GLC. The sample gases were transmitted to the Barton Titrator by a vacuum source. Barton Titrator Total reduced sulfur (TRS) concentrations were analyzed using a Barton Titrator, Model 400. Furnace gases were scrubbed through a 3% solution of potassium acid phthalate (KHP) which removes sulfur dioxide and a large fraction of water vapor from the sample gases. The sample gas was then introduced to a coulometric titration cell which utilizes hydrobromic acid (HBr) as an electrolyte. The electrolytic cell generates bromine from the HBr electrolyte which reacts with the sulfur compounds entering the titration cell. The quantity of current required to generate the excess bromine, to consume the sulfur compound, is proportional to the gaseous sulfur concentrations introduced. The current required to operate the titration cell is sensed and trans- mitted to a recorder where a continuous readout is accomplished. The recorded output is converted to TRS concentrations, as H?S from cali- bration data generated with the "spinning syringe" technique. 22 ------- Glass Wool Heated Sample Line 1/4" Teflon so2 Scrubbers Data Recorder Barton Titrator BARTON SAMPLING SYSTEM Figure 5 Flow Meter A X"—>> Micro f\'' jMetering Vjyvalve v Vacuum Pump ------- Sampling Procedure for Participate Emissions Prior to performing the actual participate emission tests, certain preliminary stack parameters had to be determined for the stack gases. This preliminary data included the average stack gas temperature, velocity head, moisture content, stack dimensions, and number of sampling points. The stack gas temperature was determined by using bimetallic ther- • mometers and a pyrometer. The approximate stack gas moisture content selected for setting the nomograph was based upon previous tests made on the same boiler. The final moisture content used in calculating the stack emissions from the recovery furnace was based upon the amount of condensate collected in the impingers and the silica gel from a separate moisture test. The sampling points selected and tiie respective stack gas velocities were determined by using Methods No. 1 and 2 of the Federal Register (Vol. 36, No. 247, December 23, 1971). Velocity head measurements were made by using a calibrated S-type pi tot tube with an inclined manometer. The sampling train configuration used during the tests consisted of the following: a stainless steel nozzle; a heated glass-lined probe; a heated glass-fiber filter; two Greenburg-Smith impingers with tips, each containing 100 ml of 80% isopropanol; two Greenburg-Smith impingers without tips, each containing 100 ml of 3% hydrogen peroxide; one Greenburg-Smith impinger without a tip, containing about 200 grams of silica gel; a flexible sample line; an air-tight vacuum pump; a 24 ------- dry-test meter; and finally a calibrated orifice with an inclined manometer (see Figure 6). Velocity head measurements were conducted simultaneously with the sampling at each point so that each point could be sampled isokinetically. The impinger portion fo the sampling train was feed down to collect the condensables, and to determine the actual stack gas moisture. 25 ------- 3. 4. 5. r, 10. 11. 12. 13. 14. 15. 16. 17. 18. T ^ i .> • 20. 20 Stainless steel nozzle Glass-lined probe (heated) Heated box (250°F) Glass-fiber filter and holder Ice bath Impingcr with Tip, 100 ml of 80% Isopropanol Impinger vn'th Tip, 100 ml of 80% Isopropanol Impinger without Tip,.100 ml of 3% Impinger without Tip, 100 ml n-c •?'•' u n 0 i o/j r>oUo Inpinger' with 200 grams of Silica Gel Thermometer Flexible sample line Vacuum gauge Coarse valve Fine valve Vacuum pump Drg-test meter Calibrated orifice Inclined manometer S-typs pi tot .tube 13 I n. 14 FIGURE 6 ' PARTICIPATE AND S02 TRAIN ------- Samp 1 e Recovery and Ana 1 ys e s of Pa r 11 c u 1 ate s Sample recovery from the particulate train was accomplished by. separating train components into the following containers: Container No. 1 - The previously weighed glass-fiber filter was placed into this container, then sealed and labeled. Container. No. 2 - All portions of the train from the nozzle through the front half of the filter holder were rinsed with acetone and the contents placed into a glass container, then sealed and labeled. . Container llo. 3 - The volume of liquid from the first and second impingers was measured and the contents placed into a glass container. Also, all sample-exposed surfaces between the filter and third impinger were rinsed with 80;i isopro- panol and placed into this Container, then sealed and labeled. Container No. 4 - The volume of liquid from the third and fourth impingers was measured and the contents placed into separate glass containers. All glassware between the second and fifth impingers was then rinsed with deionized, dis- tilled water and then added to each respective container. The liquid samples were then sealed and labeled. Only one sample container was used for both impingers used in the smelt dissolving tank sampling. Container No. 5 - The previously weighed silica gel was re- moved from the fifth impinger and placed into the original polyethylene jar and sealed. 27 ------- :•.. The samples recovered were analyzed as follows: Container No.. 1 - The filter and all loose material in the sealed petri dish were transferred to a tare glass weighing dish, desiccated, and dried to'a constant weight. Container No. 2 - The acetone washings were transferred to a tared beaker and evaporated to dryness at ambient temperature and pressure. It was desiccated and dried to a constant weight. Container No. 3 - The contents were transferred to a tared beaker, and then evaporated at 212°F. The residue was desic- cated and dried to a constant weight. Container No. 4 - The liquid contents were shaken, and then a 25 ml aliquot of each container was pipetted into separate 250 ml Erlennieyer flasks. One hundred ml of isopropanol, plus two to four drops of thorin indicator was added to each sample. The samples were titrated with barium perch!orate to a pink end point. Another duplicate sample and blank was titrated in the same manner as the first sample. Samples were analyzed at the plant site. Container No,. 5 - The spent silica gel was weighed at the site and recorded. The filter from Container No. 1, and the beakers from Containers No. 2 and 3 for each run were sent to the EPA project officer after the initial analysis for additional analyses. 28 ------- Sampling System for Oxygen, Carbon Dioxide, and Carbon Monoxide Figure 7 is a schematic.'-diagram of the sampling system. Source gases were drawn continuously through a glass-lined probe and polyethylene tubing to a moisture trap consisting of silica gel im- pingers immersed in an ice bath. Valves on the pressure side of the vacuum pump controlled the flow"of sample gas to the detectors. A bleed valve was provided to maintain adequate purging of the sample line. Gases to the oxygen and carbon monoxide detectors were passed through an ascarite bed to remove carbon dioxide which potentially interferes with the HDIR determination of carbon monoxide. Sample to the carbon dioxide detector v/as diluted with nitrogen to accommodate the range requirements of the detector. 29 ------- From Stack Ice Bath Silica Gel Midget Impinger w/Silica Ge"T To COp System ~1 f Ascarite Impinger Vent~«—£>; A CO Cal Gas Vent -MX A co2 Cal Gas Bleed V T Vacuum Pump To CO. On ,$_ystem CO NDIR °2 Paramagnetic Analv?er Flowmeter Dilution System NDIR C02, 02, and CO SAMPLING SYSTEM Figure 7 Flow —[Xh> V.ent Cal Gas -(X}>-Vent Dilution Nitrogen 30 ------- A Beckrcan model F-3 paramagnetic oxyg.cn analyzer capable of measuring 0 - 25f= oxygen was used for. CL detection. Beckman NDIR models 315-B and 315-A, respectively, were used in determining carbon dioxide and carbon monoxide concentrations. The instrument configura- tions were 0 - 5% CO,, and 0 - lOOOppm CO. All instruments were supplied with a lov/, medium and high range which were calibrated separately. The detectors were switched on and allowed to run continuously 24 hours per day for the entire sampling interval. Calibration All calibration gases were supplied and analyzed by Matheson Gas Products, Inc., Morrow, Georgia, and La Porte, Texas. The calibra- tion procedure was conducted prior to sampling each morning and was re- peated at the end of each day. Nitrogen was introduced into each instrument and the zero control was adjusted to obtain a steady "zero trace" on the recorder. Appropriate standards were then passed into the instruments at less than 100 cc/minute. The gain controls for each range were adjusted to provide maximum deflection and accuracy. Daily Operation Each morning after calibrating the instruments, charging the traps, and checking the probe, the system was assembled as shown in Figure >7. The dilution to the carbon dioxide detector was regulated to provide an accurate deflection range at a total flow rate less than 100 cc/minute. Flows for sample gas and dilution nitrogen were measured with a bubble tube. The recorder traces were observed and the ranges 31 ------- were adjusted throughout the sampling interval as required. Occasionally sampling was interrupted to obtain odor samples, charge traps, or to check the system. Sampling Procedure for jiitrogen Oxides Nitrogen oxide concentrations of the recovery furnace outlet gases were determined by using the EPA Method 7, which is described in the Federal Register (Volume 36, No. 247, December 23, 1971). Essentially, the method consisted of collecting a grab sample of the gas in an evacuated 2-liter flask containing a dilute sulfuric acid- hydrogen peroxide absorbing solution. The sample remained in the flask at least 16 hours, and was then placed in a glass storage bottle. Sodium hydroxide (IN) was then added to the sample until alkaline. The samples were taken back to the laboratory in Gainesville, Florida, and measured colorimetrically using the phenoldisulfonic acid procedure. 32 ------- |