c/EPA
             United States
             Environmental Protection
             Agency
             Environmental Monitoring
             Systems Laboratory
             P.O. Box 93478
             Las Vegas NV 89193-3478
EPA/600/R-93/094
May 1993
             Research and Development
Radium in Water
Intercomparison Study

A Statistical Evaluation of
the March 5,1993 Data
                                             55UGR92NRO.COV-27

-------
             Radium in Water
          Intercomparison Study
             March 5, 1993
      Environmental Protection Agency
Environmental Monitoring Systems Laboratory
            Las Vegas, Nevada

-------
            UNITED STATES ENVIRONMENTAL PROTECTION AGENCY
                        OFFICE OF RESEARCH AND DEVELOPMENT
               ENVIRONMENTAL MONITORING SYSTEMS LABORATORY-LAS VEGAS
                                  P.O. BOX 93478
                            LAS VEGAS, NEVADA 89193-3478
                                   (702/798-2100)
Dear Participant,
   Enclosed are the results of the Nuclear Radiation Assessment Division (EMSL-LV)
Intercomparison Study for Radium in Water; March 5, 1993.

   The known value for each analysis was determined by gravimetric methods,
checked by chemical analyses performed by EMSL-LV's Radiochemistry Laboratory,
and compared to the participating laboratories' grand average.
   The expected precision, determined by the known value, was taken from "Table
3. Laboratory Precision:  One Standard Deviation Values and Control Limits for
Various Analyses", which is based on data accumulated over the years by the
Intercomparison Program, and can be found in the Environmental Radioactivity
Laboratory Intercomparison Studies Program and Radioactive Standards Distribution
Program information brochure.

   Please take a few minutes to review this report and the analytical data your
laboratory submitted to us.  If there are any apparent discrepancies, please notify
us immediately.

   We encourage you to make use of the computer-automated data-entry system that
has been in place for some time now. As the number of participants increases, and
it becomes unrealistic for us to receive results by mail or FAX, the computer system
will be our only avenue for accepting data.

   If you have any questions or comments,  please send a message via the data-entry
system or contact Frank Novielli at 702/798-2159 or Patricia Honsa at 702/798-2141.

                                          Sincerely,
                                          Frank Novielli
                                          Senior Chemist
                                          Radioanalysis Branch
Enclosure

-------
               NOTICE

This material has been funded wholly by
the U.S. Environmental Protection Agency.
It has been subject to the Agency's review,
and has been approved for publication as
an EPA document.

-------
           EMSL-LV Intercomparison Study:  Radium in Water,  5-Mar-1993         1/14
   The following pages consist of separate sections for each of the nuclides in this study with four
parts per section.  After the first, each part is separated from the next by a new page or a thick
horizontal bar.  The first page of each section is a statistical summary for the nuclide and starts
with a statement of the known value, the control limits, and the warning limits.

   The warning limits are placed at two normalized standard deviations above and below the
known value and the control limits are three normalized standard deviations above and below
the known value.  If you keep control charts, these values will be useful for anticipating problems
with the accuracy of your analytical methods.

   The coin shaped pie chart at the top of the summary page shows the fate of all the samples
sent out in number and percentage terms.  The pie chart starts at the top and rotates clockwise.
The first sector represents those participants who submitted analytical results within both the
warning and control limits. The next sector represents those who are in the warning region but
not out of control. The third sector represents those who are out of control, but have passed
the outlier test. The fourth sector represents those who have failed the outlier test. The last
sector represents those participants who have failed to respond properly. This is the case if no
analytical results were returned, or less than three determinations were  reported, or If the results
were received too late.  The reeding on the edge of the coin is spaced at one percent intervals, and
the sector shading becomes darker as the data reliability decreases. Sectors with zero width are
not shown.

   The table in the center shows a number of statistical quantities calculated from the submitted
data based on the mean and median values in relation to the known value, both before and after
outlier removal. The lower pie chart uses the same construction as the upper chart and shows
the distribution of properly submitted data in terms of deviation from the known value divided
into sectors representing  one, two, three, and greater than three normalized standard deviations.

   The second part is an  alphabetical listing, in lab-code order, of submitted data and several
calculated quantities. An entry that is shaded has been rejected because of one of the reasons
listed above or failure of the outlier test. The fifth and sixth columns are a measure of laboratory
precision. The Range analysis is a normalized value that you may use to keep precision control
charts. If this value is between 2.0 and 3.0, your analytical process precision is in the warning
zone; if it exceeds 3.0 it is out of control. The eighth and ninth columns are the differences from
the mean of all non-outliers and from the known value, respectively. A tag symbol may appear in
the last column. Each page with tags has a symbol definition summary at the bottom.  If there is
no tag symbol, the data is within the control limits, but it may be in the warning zone.

   The third part is a three-column  listing of result average, tag symbol, and lab-code in average
order excluding those labs not responding properly. In this order, all outliers and out-of-control
results appear at the top  or bottom of the list.

   The last part is two bar chart displays showing frequency distributions of responding
participants. The first chart places the known value at the center and a  bar at each 0.2 unit of
expected precision.  The second chart places the mean of the reported measurements at the center
and a bar at each 0.2 unit of standard deviation. In both cases, a bar includes those results within
0.1 unit up to the maximum of six. Any results more than six units from the center value are
shown cumulatively by a shaded bar one past the sixth unit. If the central tendency of the known
value distribution falls away from the center, an error in accuracy is indicated. If the distribution
is broad, poor precision is indicated. The mean value distribution is similar but uses the average
and standard deviation of reported results as its basis.

-------
2/14        EMSL-LV Intel-comparison Study: Radium in Water, 5-Mar-1993


     The Range Analysis(R + SR) is calculated from the range, mean range and standard error of
  the range values.  The range is the difference between the maximum and minimum results for the
  laboratory. The mean range is calculated by multiplying the expected precision by 1.693(for three
  results).  The standard error of the range is calculated by multiplying the mean range by 2.575(for
  three results), subtracting the mean range from this product, and dividing the result by 3. If the
  range is greater than the mean range, then the range analysis is calculated by subtracting the
  mean range from the range, dividing the result by the standard error of the range and adding 1.
  If the mean range is greater than or equal to the range, then the range analysis is calculated by
  dividing the range by the mean range.

     The normalized deviation of the mean from the grand average is calculated from the deviation
  of the mean from the grand average and the standard error of the mean values. The deviation of
  the mean from the grand average is calculated by subtracting the grand average from the
  average of the laboratory's three results. The standard error of the mean is calculated by
  dividing the expected precision by the square root of 3(the number of results). The normalized
  deviation of the mean from the grand average is calculated by dividing the deviation of the mean
  from the grand average by the standard error of the mean.

     The normalized deviation of the mean from the known value is calculated from the deviation of
  the mean from the known value and the standard error of the mean values.  The deviation of the
  mean from the known value is calculated by subtracting the known value from the average of the
  laboratory's three results.  The standard error of the mean is calculated by dividing the expected
  precision by the square root of 3(the number of results). The normalized deviation of the mean
  from the known value is calculated by dividing the deviation of the mean from the known value by
  the standard error of the mean.

     A complete explanation of the statistical calculations involved in the report may be found in the
  Environmental Radioactivity Laboratory Intercomparison Studies Program information brochure
  [Draft Revision of EPA-600/4-81-004], available from Frank Novielli, EMSL-LV, 702/798-2159.

-------
             EMSL-LV Intercomparison Study: Radium in Water,  5-Mar-l993
                                   3/14
Radium-226                         Statistical Summary                      152 Participants
The known value of this nuclide is 9.8 pCi/1 with an expected precision of 1.5; the control limits
are 7.2 to 12.4; the warning regions are 7.2 to 8.1 and 11.5 to 12.4
28(18.4 %) Failed to respond
13(8.6%) Outliers *
5(3.3 %) Out of control '
     but not an outlier


         Statistic
                . 92(60.5 %) Within all limits
Respondents
14(9.2 %) In warning zone
        but within control


           Non-outliers
Mean
Std. Dev.
Variance
%Coef. ofVar.
% deviation of mean from known value
Norm. dev. of mean from known value
Median
% deviation of median from known value
Norm. dev. of median from known value
     11.27
      8.66
     74.97
     76.83
     15.00
      0.17
      9.80
      0.00
      0.00
  Grand Avg 9.81
              1.26
              1.58
             12.81
              0.10
              0.01
              9.73
             -0.68
             -0.05
18(14.5 %) More than 3 norm. S.D. ,
16(12.9 %) Between 2 and 3 norm. S.D.
            ,62(50.O %) Within 1 norm. S.D.
                           of known value
     28(22.6 %) Between 1 and 2 norm. S.D.

-------
4/14
EMSL-LV Intercomparison Study: Radium in Water, 5-Mar-1993
Radium-226
Lab Res. 1
A
AE
AF
AI
AJ
AK
AL
AP
AW
AZ
BA
BC
BG
BH
BK
BL
BM
BN
BO
C
CA
CE
CG
CJ
CK
cs
DB
DE
DT
DZ
E
EB

- EH* s;
9.4
10.5
8.7
10.0
11.3
9.8
9.1
11.6
7.9
10.6
9.7
11.0
11.1
8.2
9.7
9.2
10.1
9.6
9.0
12.3
9.2
7.3
9.0
7.8
9.4
10.2
8.3
8.0
10.7
9.2
11.1
10.5

'<*v V,
Res. 2
9.5
10.7
8.6
9.4
11.0
9.0
8.8
10.8
7.6
8.7
10.4
11.0
10.7
8.4
9.6
9.4
10.4
9.7
9.1
11.3
8.7
8.8
10.7
7.6
10.0
11.2
8.6
8.0
10.9
9.6
10.9
10.5

% •.' v f ' •.-•
Res. 3
9.6
10.9
8.9
9.9
11.4
10.4
9.4
11.2
8.3
9.5
9.7
11.8
10.9
9.0
9.7
9.8
10.3
9.5
8.8
12.1
10.0
8.6
10.3
7.6 -
10.0
9.7
9.3
8.0
10.5
9.4
11.1
10.0


Exper.
Sigma
0.10
0.20
0.15
0.32
0.21
0.70
0.30
0.40
0.35
0.95
0.40
0.46
0.20
0.42
0.06
0.31
0.15
0.10
0.15
0.53
0.66
0.81
0.89
0.12
0.35
0.76
0.51
0.00
0.20
0.20
0.12
0.29


Rnganal
(R + SR)
0.079
0.158
0.118
0.236
0.158
0.551
0.236
0.315
0.276
0.748
0.276
0.315
0.158
^0.315
0.039
0.236
0.118
0.079
0.118
0.394
0.512
0.591'
0.669
0.079
0.236
0.591
0.394
0.000
0.158
0.158
0.079
0.197


Average
9.50
10.70
8.73
9.77
11.23
9.73
9.10
11.20
7.93
9.60
9.93
- 11.27
10.90
8.53
9.67
9.47
10.27
9.60
8.97
11.90
9.30
8.23
10.00
7.67
9.80
10.37
8.73
8.00
10.70
9.40
11.03
10.33

, , ..........
Normalized deviation
(grand-avg) (known) Tag
-0.36
1.03
-1.24
-0.05
1.64
-0.09
-0.82
1.60
-2.17
-0.24
0.14
1.68
1.26
-1.47
-0.17
-0.40
0.53
-0.24
-0.97
2.41
-0.59
-1.82
0.22
-2.48
-0.01
0.64
-1.24
-2.09
1.03
-0.47
1.41
0.60

',.
-0.35
1.04
-1.23
-0.04
1.66
-0.08
-0.81
1.62
-2.16
-0.23
0.15
1.69
1.27
-1.46
-0.15
-0.38
0.54
-0.23
-0.96
2.42
-0.58
-1.81
0.23
-2.46
0.00
0.65
-1.23
-2.08 i
1.04
-0.46
1.42
0.62 ;

',,,, ;, ' •
EO

ER
FE

FN
>!*«'
;FZ', '
• G€J'<
GN
GO
GQ
HE
HK
9.0

10.3
9.0

9.1
V'-\2&0;H
>yj 'x,2%;%
(y •< °« Y vf-s;"
v'!, 1&8;'*
10.6
"" '"2t8H'"<\
9.3
9.4
9.7

9.7
9.7

8.5
>'/18;4r^>>
,ss/17%£;M
'i,x~>^,---. /-7 >7^
'i,. "13;2'v,,l«"
10.2
3 -:28$> '*:•'';
10.3
9.2
9.3

10.2
8.9

8.9
'jttj&'l
;18l0A;
", >.><• --* v"
1&2
11.0
"MaV
10.2
9.5
• s No data submitted
0 s
Insufficient
data
x s
0.35 0.276

0.32 0.236
0.44 0.315

0.31 0.236
; ^3.37 4.046
'
:.":L63 1.345
0.40 0.315
: 0.29 0.197
0.55 0.394
0.15 0.118
TAG SYMBOLS
Determined to be an
9.33

10.07
9.20

8.83
21130
18,33:

1&07
10.60
28*13
9.93
9.37

outlier
-0.55

0.30
-0.70

-1.13
\ 13.27'V;
----9.84-, ,

6.07
0.91
21.16 ""
0.14
-0.51
ft = Above
Ji s Below
-0.54
1
0.31
-0.69 !
i
-1.12 i
IB.28 x
9^85 x
•
6.08 x
0.92 i
21.17 x ;
0.15 ;
-0.50
control limit j
control limit J

-------
EMSL-LV Intel-comparison Study: Radium in Water, 5-Mar-1993
Radium-226
Lab
HL
HP
r-HUf'i
HY
I
ID
J
JE
JG
^«INfi-
JS
JIX _
•"W;!*
'K^
.KK£
KH
KL
KZ
L
;\£A^
JLJtT
\o^ ^^^-*
'JLujOL^
'is"
LT
LZ
M
ME
v'MJNfl

SMQ
OX
OY
P
PB
Res. 1
8.7
_^11.6w
O@.y§F%lk
™ ^
13.6
rann-^r^
9.1
12.6
9.4
^A ^ iii^ic^
12.0
9.6
?S*fS£
yf^",8.jP
^rS^l/S
9.5~
11.1
8.1
_,JLH~ -
^yV?^1 x:'i*
ib.o
^.....^ * ^j,..,-.™^^
s«;\;>, ^ ' ,ys J « ~v k-j?
	 "4.9""
9.6
10.4
9.5
	 ._9.9w
^^Y^^^^f1^^^^


"""^ii.o'™
14.0
9.9
10.2
9.6
10.3
9.9
8.8
__8;2_
S»S^"^IS^
X\3$\s* ^^SJi''1 "^ K^1" "•."§•
1I8IWI8!
"16.2
7.9
10.7
11.0
Res. 2 Res. 3
8.9
12.7_ ^_
if^^i^k^l5^.-
8.3
11.5
7.2
9.1
12.4
8.9
?:S?v21:§'.:^*:;xu
11.0
,._9.8^_.,
-;5Jy;2.5j^i~V-
^.r 7:5r..-"'
Tt.^^^VvJx,;
9.2
8.0
8.2
12.1
l%2^i^
12.3
$t ;K™ " ."*£« t^yr" * f \j
^> , ;^,xs j^XY- -'
'7.8
9.8
10.6
10.0
^ ^^10.2^ __
s^^? ' JSviV %>^ k

SiSfikSi^
loiaT 	
3.1
10.5
9.8
9.3
10.0
9.7
8.8
__10.4 	
S^^'ipFS^Vp5^
** £ -N "S11 ^x^ '^\''<;'- X"^ % •. "• ••' ••
^JijQ3l2!t:^
	 "io"e 	
8.2
7.2
10.9
7.8
13.4
Ltf ^ :
9.4
9.5
6.9
9.6
12.9
11.1
:22;6
11.0
9.9
1 M '
7.8 "
\ -." v
9.4
9.9
8.3
12.7
v*5x_ :
13.0
;v^s% w^A ^
" " ^C s *+
- 6.0
9.4
10.5
12.5
^ 10.5
j;JVv^v'

v|-^ ;
ii.o
12.1
9.7
10.6
9.9
9.9
9.5
8.8
_12.4_
KJX^"*?^-''
-i"--^ S S^J ^^
JS^iy
10.1
8.6
9.2
11.4
• s No data submitted
0 s
Insufficient
data
x =
Exper.
Sigma
0.59
0.91
- !"~ ,- v\
0.64
2.05
0.62
0.29
0.25
1.15
0:72
0.58
0.15
0.12
0.68

0.15
1.56
0.10
0.35

1.57
'-,.-"»•

1.20
0.20
0.10
1.61
0.30
!\ - ' ' '' I

,r-;x-5---* \s- ;\,»
0.40
5.82
0.42
0.40
0.30
0.21
0.20
0.00
2.10
C^N ^ *" "^ ,,
s\ ^ •• s
;v -7.05 /
0.26
0.35
1.76
0.26
5/14 J
Rng anal Normalized deviation
(R + SR) Average (grand-avg) (known) Tag
0.433
0.709
,„*, ~\
0.433
2.170
0.473
0.197
0.197
0.866
0.512
0.394
0.118
0.079
0.512

0.118
1.420
0.079
0.236
.- " ".
1.345

••* •• s
0.945
0.158
0.079
1.345
0.236
v % X


0.276
7.271
0.315
0.315
0.236
0.158
0.158
0.000
2.245


8.396
0.197
0.276
1.720
0.197
8.47
_ 12.57 ^^
;~'\™A--,xfW1elL
9.03
	 11.53
6.70
9.27
12.63
9.80
- *"< - 21;7-7V- \.
11.33
9.77
•• * * ^V%v V.% N^. SS ^ ^
8J03
\ -:%i> , >-:- : '
9.37
9.67
8.20
12.30
% ^ \ Is
11.77
s S ^A A S \ % W \ S , WVV
, ""° " \ " "^* ^"^
6.07
9.60
10.50
10.67
10.20
" - % ^^i^^^--.------^^, 5ss-.

11 \^ ^ ^;j %xo
10.77
9.73
10.03
10.20
9.60
10.07
9.70
8.80
	 10.33
; " "" o - ^" ' * v ^ r^ T"1; x^t" v
s -. ^ ^ " s •. 1 s V
. .^V V98;9a*"»;-v
10.30
8.23
9.03
11.10
TAG SYMBOLS
Determined
to be an
outlier
-1.55
3.18
/"t^^ff^;
-0.90
1.99
-3.59
-0.63
3.26
-0.01
•ik8~i"xv'
1.76
-0.05
^B£2.: ..
-2.05
\>* " :"•' -_ x
-0.51
-0.17
-1.86
^^2.87
*i*T~".\"3/
2.26
^ s j , „ „ _ \ ->s
*^* X-- , ,^,|
-4.32
-0.24
0.80
0.99
0.45
#K,^5\: ' '-xi^
iS - v % "•

1.10
-0.09
0.26
0.45
-0.24
0.30
-0.13
-1.17
_0.60__
X"" J^,1- "• •• •.*'''•:!'
^s^*^ •".•• ^ ••^C''"' C "
T02'Q1-- ^-.^^'"^
0.57
-1.82
-0.90
1.49
It 5= Above
Ji = Below
-1.54
3.19 It
"-'^-V^K^^** ;n-
-0.89
2.00
"-3.58 Ji "
-0.62
3.27 It
0.00
13:82 X
1.77
-0.04
-8.51 x,
-2.04
x« -\ - "V •
-0.50
-0.15
-1.85
2.89
-'> , X;;', \ ,*• ,
2.27

^- , Q,
'-4.31 'Ji
-0.23
0.81
1.00
0.46
', " ' -- ;;' «! "

:-'\.;'^-- • - -
1.12
-0.08
0.27
0.46
-0.23
0.31
-0.12
-1.15
_0;62 ; _
,5, ™ , ^ .,«? J «~^,
*• •. i •.*" ^ '"" \ ^ "" •. "• **
L02.92 iVx
0.58
-1.81
-0.89
1.50
control limit
control limit

-------
6/14 EMSL-LV Intercomparison Study: Radium in Water, 5-Mar-1993
Radium-226
Lab Res. 1
PC
PG
PP
Pt
PV
PW
PX
PY
Q
QB
QJ
QQ
QU
QX
QZ
R
RC
; KD
RF
RL
RM
RN
RV
RW
RZ
S
SA
sc
SD
SF
SI
SM:
ss
ST
SW
sz
T
TA
TG
'TH-
TI
tk
TL
• =
0 s
'V v''^ "* " "
10.7
10.5
\"< ';V
9.2

9.8
' ' ~*v
11.1
10.1

;• 25,6
9.3
Res. 2
"' ' " >5- J > ^
10.0
10.7
y;— "-'••-'-;- -•
10.3
' > "' '' '
10.2
, -:;v • -- ,
12.1
10.2
;/"^;;~
9.2
9.4 9.2
Res. 3
,\^ - . ,
11.5
10.7

8.6

10.4
/ , -
12.9
10.9
'V' ^
29.6
8.6
9.3
Exper.
Sigma
s^
0.75
0.12

0.86

0.31
,>
0.90
0.44
2,10
0.38
0.10
"" * '""' " A\^ ^^ '' '''' '' 'w'% " ^" >WV ""tj.1" *"* ' '' • -y ;.; _ 	 / • - - -.-
-' i8J&; :-'
12.8
12.1
11.8
11.9
7.9
9.7
9.3
9.7

9.1
9.3
10.4
7.4
• •- • , x 4.9
8.7
9.8
;' v\«#"'
10.2
9.7
10.5
_, '- -, ' *-\
,' \lfiL«U
- , ---<'
12.1
;; , ™ '••>;•" —
8.1
-;"-;^18iS1'-\\c-- -
10.8
11.7
12.7
9.6
8.3
8.7
9.0
'., ,S>.7_ ^
' " v'-~ ! " ' " ' ,
9.2
9.3
12.9
7.3
- 4ft* r -
8.5
9.8
:•'" ^>H
9.7
9.6
JL0.8_
"'' 'moi -

11.2
";/-- ' -/'- -
7.3
-"- i8';6 ,-
12.7
11.0
12.2
10.2
8.4
10.0
9.1
10.0
~.
9.5
10.2
11.3
7.2
:,V-'4:9".
8.3
9.6
. Sty
8.7
9.8
10.5
13.5

13.0

5.9
No data submitted
Insufficient
data
x =
>. -•• vO.17 --
1.13
0.56
0.45
1.19
0.26
0.68
0.15
0.17

0.21
0.52
1.27
0.10
<,V''>(M)6"—
0.20
0.12
;';V 7,05 *
0.76
0.10
0.17
1.39

0.90

1.11
Rng anal Normalized deviation
(R + SR) Average (grand-avg) (known) Tag
„- - ' ' '•
0.591
0.079
> -
0.669

0.236

0.709
0.315
2,020
0.276
0.079

0.118
0.788
0.433
0.354 '
0.906'
0.197
0.512
0.118
0.118

0.158
0.354
0.984
0.079
0;000
0.158
0.079
9.671
0.591
0.079
0.118
0.984

0.709

0.866
'" -: "V-V
10.73
10.63
t
9.37

10.13

12.03
10.40
28;00 :
9.03
9.30

18.70
12.10
11.60
12.23
10-57
8.20
9.47
9.13
9.80

9.27
9.60
11.53
7.30
4.90
8.50
9.73
15.73
9.53
9.70
10.60
15.10

12.10

7.10
TAG SYMBOLS
Determined
to be an outlier
:V-, ^v''-
1.07
0.95

-0.51

0.37
, ^v
2.57
0.68
21,00
-0.90
-0.59
sV1- "'•••.
10*27 ;
2.64
2.07
2.80
0.87
-1.86
-0.40
-0.78
-0.01

-0.63
-0.24
1.99
-2.90
/»5.'67'M *
-1.51
-0.09
6;84
-0.32
-0.13
0.91
6.11

2.64

-3.13
11 = Above
' "- - , " V
1.08
0.96

-0.50

0.38
,-
2.58
0.69
21:02
-0.89
-0.58

10.28
2.66
2.08
2.81
0.89
-1.85
-0.38
-0.77
0.00

-0.62
-0.23
2.00
-2.89
-6,66
-1.50
-0.08
6.85
-0.31
-0.12
0.92
6.12

2.66

-3.12
control
•11 = Below control
, •;• -


•^ •

•

• '

9
*
X


•
X








'"" •




X


X


X
•

»
li
limit
limit

-------
EMSL-LV Intel-comparison Study: Radium in Water, 5-M ar-1993 7
/14 1
Radium-226
Lab
JKjf
,,,,TV,
.XL
•"$$
UE
UI
UL
UN
W
X
Y
Z
Res. 1 Res. 2
~* 	 7.0 	 _ 8.6
,II^?-1™1,JM,
^-^,,M~-^.^.^?5L
	 "~8?6 	 "9.5"
10.0 9.4
8.1 8.9
11.4 10.4
7.7 9.7
11.6 11.2
9.7 10.1
10.1 10.1
Exper.
Res. 3 Sigma
8.0 0.81
10.1 0.46
H"_i?»-®r - p-?6.
*~~6.8 	 1.37
9.2 0.42
8.5 0.40
10.9 0.50
8.9 1.01
10.8 0.40
9.9 0.20
10.0 0.06
Rng anal
(R + SR)
0.630
0.315
0.276
1.120
0.315
0.315
0.394
0.788
0.315
0.158
0.039
Normalized deviation
Average (grand-avg) (known)
7.87 -2.24 -2^23
10.63 _0.95 _ 0.96
9.30 :0;59_,1 -°'58
8.30 -1.74 -1.73
9.53 -0.32 -0.31
8.50 -1.51 -1.50
10.90 1.26 1.27
8.77 -1.20 -1.19
11.20 1.60 1.62
9.90 0.10 0.12
10.07 0.30 0.31
Tag
>r>rj*
r. , •*»•

* ":







Data sorted by Laboratory Average
Average Tag

























• =
2.43 x
4.90 x
6.07 U
6.70 U
7.10 U
7.30
7.67
7.87
7.93
8.00
8.03
8.20
8.20
8.23
8.23
8.30
8.47
8.50
8.50
8.53
8.73
8.73
8.77
8.80
8.83
No data submitted
0 = Insufficient data
Lab
JY
SM
LS
ID
TL
SI
CJ
TQ
AW
DE
K
RV
KZ
OY
CE
UE
HL
UL
SS
BH
DB
AF
W
OB
FN
Average
8.97
9.03
9.03
9.03
9.10
9.13
9.20
9.27
9.27
9.30
9.30
9.30
9.33
9.37
9.37
9.37
9.40
9.47
9.47
9.50
9.53
9.53
9.60
9.60
9.60
Tag

f























TAG SYMBOLS
Lab
BO
QZ
P
HY
AL
RZ
FE
SC
J
U
R
CA
EO
PV
KH
HK
DZ
RW
BL
A
UI
SZ
SD
NH
LT
Average Tag
9.60
9.60
9.67
9.67
9.70
9.70
9.73
9.73
9.73
9.77
9.77
9.80
9.80
9.80
9.90
9.93
9.93
10.00
10.03
10.07
10.07
10.07
10.13
10.20
10.20
1? s Above control
x = Determined to be an outlier il = Below control
Lab
BN
AZ
KL
BK
T
NT
ST
MY
AK
A I
• IX
S
•JG
CK
Y
ME
BA
( G
N
7.
NO
KR
I'X
NG
ME
limit
linvit

-------
8/14 EMSL-LV Intercomparison Study: Radium
Radium-226
Average Tag
10.27
10.30
10.33
10.33
10.37
10.40
10.50
10.57
10.60
10.60
10.63
10.63
10.67
10.70
10.70
10.73
% responding labs
10- — 	 — -_-

-6 -4
% responding labs
ID- -----------

-6 -4
• s No data submitted
0 = Insufficient data

DC
Lab
BM
OX
OF
EB
CS
QB
LZ
RN
TA
GO
TU
PP
M
DT
AE
PG
in Water, 5- Mar- 199 3

ita sorted by Laboratory Average
Average Tag Lab Average
10.77
10.90
10.90
11.03
11.10
11.20
11.20
11.23
11.27
11.33
11.53
11.53
11.60
11.77
11.90
12.03
Frequency distribution
I •• •
_«••_• lIllllll.lB.
MS 12.10
UN 12.10
BG 12.23
E 12.30
PB 12.57
X 12.63
AP 15.07
AJ 15.10
BC 15.73
JS 18.33
SF 18.70
I 20.10
RL 21.30
LB 21.77
C 28.00
Q 28.13
98.93

-
_•_• — •• •
-2 0 +2
Normalized deviation of the mean from the known value
Frequency distribution
• •••
	 ..••_• I|||||I|.|B.
Normalized deviation of the mean from
TAG SYMBOLS


.1 • 	 B. m
+2
the grand average
IN
x s Determined to be an outlier U =

Tag



tr
n
X
X
X
X
X
X
X
X
X
X
X



+4



+4
* Above control
= Below control

Lab
TI
RF
RM
L
HP
JE
GN
TG
SW
FZ
RD
TN
FP
JN
QX
GQ
OS

S !
S

N
76
limit
limit

-------
             EMSL-LV Intel-comparison Study: Radium in Water, 5-Mar-1993
                                   9/14
Radium-228                         Statistical Summary                      152 Participants
The known value of this nuclide is 18.5 pCi/1 with an expected precision of 4.6; the control limits
are 10.5 to 26.5; the warning regions are 10.5 to 13.2 and 23.8 to 26.5
48(31.6 %) Failed to respond .
1 (0.7 %) Outliers •
7(4.6 %) Out of control •'
     but not an outlier


         Statistic
                • 91 (59.9 %) Within all limits
Respondents
-•-• 5(3.3 %) In warning zone
           but within control


              Non-outliers
Mean
Std. Dev.
Variance
%Coef. ofVar.
% deviation of mean from known value
Norm. dev. of mean from known value
Median
% deviation of median from known value
Norm. dev. of median from known value
     17.69
      3.74
     13.98
     21.13
     -4.38
     -0.22
     18.13
     -1.98
     -0.10
    Grand Avg 17.81
                 3.54
                12.50
                19.85
                -3.72
                -0.19
                18.43
                -0.36
                -0.02
8(7.7 %) More than 3 norm. S.D. •«
5(4.8 %) Between 2 and 3 norm. S.D.
            .65(62.5 %) Within 1 norm. S.D.
                           of known value
     26(25.O %) Between 1 and 2 norm. S.D.

-------
10/14 EMSL-LV Intel-comparison Study: Radium in Water,
5-Mar-1993

}
Radium-228

Lab
A
AE
AF
AI
AJ
AK
AL
AP
AW
AZ
BA
BC
BG
BH
BK
sir
BM

BN
BO
C
CA
CE
CG
CJ
CK
cs
DB
DE
DT
DZ
B,-
EB
EH
EO
' TSTt" '
jsiit,..
FJ2-'..
r •?
• FN
FP
FZ

'GCT-
GN
GO
GQ
HE
HK

Res. 1
18.9
17.9
19.7
18.9
21.0
19.6
16.0
11.7
13.6
22.5
17.1
19.1
-„, -!• ..*>,' "•.-
18.1
19.5
; .V-V'-JH-
18.4

';'" /'V^;
17.3
21.5
20.5
20.1
24.7
18.0
15.6
19.7
13.1
22.0
18.3
17.3
' v"" -•••• •• •••;' ,
15.4
""-'",. -'^ _ *;
17.0
"" "" •'"XJ'^i s% f.f "" ^ ,
-'•• '*''- »V''>' ''
;', ,''> *'• -/ ' >V,
*/ * * ^ ** "-. j' X -Sjv.
13.0
15.5
14.0


7.0
\. , \ 'f ,
14.7
17.4
18.2

Res. 2
18.9
16.6
19.9
18.5
20.9
19.5
19.8
9.2
14.3
19.8
18.3
19.9
- - -A-'--,-
19.9
18.4
"""v... * •• Jf s
19.1

"?-' • -^ '<*;:
17.4
21.8
19.8
19.4
23.1
22.0
17.5
21.8
13.7
21.6
18.9
17.1
"'••',- -- ty
, i?-!.
' „ < \ X •?
17.7
, , 1 Y,-;,- "',",-
,'> "'" ' -\ '-
* '""f « *"'»"i'
' * t * ' /* '•'-.'^
13.3
16.3
7.3

""*"'""""
7.1
, J,. fV ->„ ,v;
15.0
16.7
18.8

Res. 3
19.0
17.3
21.8
19.9
20.8
20.6
16.4
10.5
14.5
19.2
18.1
20.3
^ " - A
20.2
18.3
; i-' v ">v-- ;
20.2

-_ ",'V}-;;^-"
16.8
21.3
22.0
19.6
22.5
18.0
19.2
21.5
12.5
21.4
18.3
16.9
,:,,' ^ '„
15.5
"-^,'~\ \>™
17.4
'*''^?-5'1>*"-"<1 ~',>'f'\\
-- "f '! '' ' "
-v">V' > / \>'--,~
^%t * ^ ^ ^ ^A
12.8
14.6
19.0

;." "y ^ '' "i'-»"
7.2
; !-? , '- - ,<•
15.1
15.1
18.3
• = No data submitted
0 s
Insufficient
data
X s
Exper.
Sigma
0.06
0.65
1.16
0.72
0.10
0.61
2.09
1.25
0.47
1.76
0.64
0.61

1.14
0.67

0.91

- •"•f" ' , -•". ,
0.32
0.25
1.12
0.36
1.14
2.31
1.80
1.14
0.60
0.31
0.35
0.20
jj j ''
0.06
j \
0.35
J^ Trf ' -
" ^'',
"%S *.
/ -.'
0.25
0.85
5.87

--':-"
0.10

0.21
1.18
0.32
Rnganal
(R + SR)
0.013
0.167
0.270
0.180
0.026
0.141
0.488
0.321
0.116
0.424
0.154
0.154

0.270
0.154

0.231


0.077
0.064
0.282
0.090'
0.282
0.514
0.462
0.270
0.154
0.077
0.077
0.051

0.013

0.090




0.064
0.218
1.957


0.026

0.051
0.295
0.077
Normalized deviation
Average
18.93
17.27
20.47
19.10
20.90
19.90
17.40
10.47
14.13
20.50
17.83
19.77

19.40
18.73

19.23


17.17
21.53
20.77
19.70
23.43
19.33
17.43
21.00
13.10
21.67
18.50
17.10

15.43

17.37




13.03
15.47
13.43


7.10

14.93
16.40
18.43
TAG SYMBOLS
Determined
to be an outlier
(grand-avg) (known)
0.42
-0.21
1.00
0.48
1.16
0.79
-0.16
-2.77
-1.39
1.01
0.01
0.74
, \;
0.60
0.35

0.53

•• 'A %, -. .. .••,
-0.24
1.40
1.11
0.71
2.12
0.57
-0.14
1.20
-1.77
1.45
0.26
-0.27

-0.90

-0.17


"..'',-. ''
.••- v f s .•
-1.80
-0.88
-1.65


-4.03

-1.08
-0.53
0.23
ft = Above
U = Below
0.16
-0.46
0.74
0.23
0.90
0.53
-0.41
-3.02
-1.64
0.75
-0.25
0.48

0.34
0.09

0.28

*
-0.50
1.14
0.85
0.45
1.86
0.31
-0.40
0.94
-2.03
1.19
0.00
-0.53

-1.15

-0.43




-2.06
-1.14
-1.91

-, -.
-4.29

-1.34
-0.79
-0.03
control
control
Tag


*




li




- 1


*


••












•

" *

,

' •





» -
U
•



limit
limit

-------
EMSL-LV Intercomparison Study: Radium in Water,
5-Mar-1993
11/14]
Radium-228

Lab
HL
HP
5HUr
HY
I
; • V,N sv. « -. N^S
T^k^ ^
•• l*»x, t
ID
J
JE
JG
W5S^ - ""!:%'*X

V;5^*v'^i£
JS
JX

!¥1!
K

^KKy?
KH
KL
KZ
L
S,-^S •.-. W AJW •.
V->TT YA ^ 5
^V '^^sSvs'XX

^ TIOXs
"--" r"
l|IiM/
LS
v.""T " ^""•\!
^•^MitOt''^
"M
ME
SM'OI
MS
(SS'W s* > •i'W^
f^MYI
N
NG
NH
NO
NT
' 'OB\
OF
OS
OX
OY
P
PB

Res. 1
15.7
_17.8
^^•X^H;
16.9
16.7
••^ttv- XV " <: ^ ' x «,^v. •^•^•••- ^
>^xis ;Ckii ,>f s
',?-, ,\ s; , >v«.
10.5
20.3
16.2
23.1
^x-v ^^^^•^^^^^••••^x'-X

^ V!H£* sV^KssV^X^S^^
	 ~2i"o"™"
16.5

>?"%o"S^5 -Q^
18.2

rc£»c4i c$i' -3?
"'17.5"
21.5
17.7
20.6
^w.v^^w^^yj.v^v^I.I.V.VAy.w
i^\ ^ ^\5? ^v -\^ ^-.-^ ^ \
•X^.^SX'x\Jv!'.\ \X\^'-\V i\"^^

^^^VC^T^i:^ ^ ^ \ °*
^-V^V^'^ly "^f. •"-
^x^lf^i^v^
16.0™""
18.1 ^
"'"""24!o'"
13.4^

14.6
'^JJ^'^-X^V^X^ A1"^" ""
^ ^iSS ^r^H^U
20.2
21.1
16.0
10.8
20.6
*;5 - "'y^r 7 ;
16.2
" ^28.2"
18.8
9.2
13.8
20.6

Res. 2
18.4
19.0
"\rt^->vv^
^••\^ x.j\ s hv- ^
15.8
17.3
5 1^% ^ %x' s ••^•^•-''^ ^
•• ••'••" 0^\ ^ s "• * v >.
•• ^ ^f. ^ s^ v -. ^ S
10.5
21.1
14.9
17.8
s^\^ ""tT'c? * ""^ ^tr

°\xv^ S ^OX1"
22.0
17.6


sS '•XsXl^X \>. X s ^ •> ^
21.5

:s\\~»2^;SS
20.5
21.3
17.7
20.7
X^^V ^^vw-v. ^ ^
^"" ~^^\ ^'-••-.f \X" ^^
•• ^ ^ ^ ^ -^x^^ ^ I-^'

\^X^^ ^->\S^\ 'x^l;''
^1-1 *-v%'™"^*-
^!^liit^
22.0
19.7
24^0
14.1

13.4
^ X ," °"^V^O^
^i'SV-^l?,
20.2
20.9
12.3
10.0
21.4
(\c -" }:<°x
17.2
21.6
18.5
10.4
10.9
20.5

Res. 3
15.7
20.0
.vw;' •- \
17.1
14.3
"-•voo^"^ % T'l'VNxs'5 %
•> \ '^''V^1-'- ^ ^ "• "• *• •• s
v. 51 ^% V '•• % Vs """"V %
10.0
20.8
17.4
20.0
s-.«sw«\i^^^ «.^%%w w^ ^ ^

v,1" O^-.'lC.'' /"" \^v
21.0
15.5

^"^N>"u.s6• ^ ? o- s;c- ss h
& *\ "• x - %* V''^1' v
19.0
19.3
17.7
20.0
V.y.'.'.'. S v.-.'-W'* N ^^C ^ ,_!;•••• v
"" •. ^ "NX ^ s -.-i v_v >-x's
XSC %•>'* ^ -^ ti? £ •• ^^ ••;'"'•*•'•

^^ % J $*l* s """^x ^ v
^'"i-"' 0^ ^ s-.^^-^^ ••
;;;^:^;x.%y\j
• 19.0
18.8
23.0
15.0
4.t&" •. i'Vi;t \ :'-x\~-
f ;*8~ISV- o ^ -S\
14.3
"*^\^*S^CV^ X, ""%\s
^^LX^fei^^-^ "
18.6
21.1
18.4
9.6
21.0
^A^l , -
14.0
23.8
19.0
10.0
16.1
20.6
• = No data submitted
0 s
Insufficient
data
x =
Exper.
Sigma
1.56
1.10
; ; !
0.70
1.59
SX "" "" ^ •• T


0.29
0.40
1.25
2.66
\c s - __ w w •. %^


0.58
1.05

^ ' - 0.21 *, "
2.29

x-t '!-
1.35
1.22
0.00
0.38
V V, •- s X V •.

-. ^J ^_ % 1\ ^ -.< •- ^ *

' Xs \ * -- -.
, ' - ;,
t;-! "'-,'-; -.-;•-
3.00
0.80
0.58
0.80
^;v< • >>/
0.62
•^

0.92
012
3.07
0.61
0.40

1.64
3.36
0.25
0.61
2.61
0.06
Rnganal
(R + SR)
0.347
0.282
s __•>'"'- v ^
0.167
0.385
* - - - - x"


0.064
0.103
0.321
0.681
" •• ^ •- *"*•• v j *•


0.128
0.270

, -^|-;—
0.565

1 > , -^ ,. ;•
0.347
0.282
0.000
0.090
V W V, -.V.V V sv
•• , ^
"• ^ t t% s ""• •, viv> ^ ^ \
-. * " ^" •- % "" *. "%
s ^\ s "" •• '' "" "* s
\N ^

0.770
0.205
0.128
0.205
-.^^'•^t
0.154
"•X. \\ \ ''^^^
:*l - - -
0.205
0.026
0.783
0.154
0.103
- , < \
0.411
0.847
0.064
0.154
0.668
0.013
Normalized deviation
Average
16.60
18.93
, , , '~ ' > vL' -
16.60
16.10
' " s ^ •-•• •• ; -• 5; % *
^ ''^ ^ v ^ ^ ^

10.33
20.73
16.17
20.30
«.-, ; w^% ^ \ ss s ..

s S". •• "• ••'•'"yV^
21.33
16.53

' «.- ;v' 4193' "S
18.93

"• •>" ° % *
19.10
20.70
17.70
20.43
vv ^vv\ s ss s s_v ^sws s s
•• s ^-.\ O s
"' , "•"""' ^^^ •. .> s^ VO

-- •> ^^
•-V "" ^
\ :>T' "\ -y '
19.00
18.87
23.67
14.17
>^\'(^
14.10
— .^ ^^ •, ^ ^
- ;v. K:^',"'^
19.67
21.03
15.57
10.13
21.00
*• ^ C'''''1'S'" ^ *
15.80
24.53
18.77
9.87
13.60
20.57
TAG SYMBOLS
Determined
to be an outlier
(grand-avg) (known) Tag
-0.46
0.42
"-L>,s " -"- \- s ,% ;t4vv!
-0.46
-0.64
•J^X '" ' ' " * •••tV'* X-. C-*1 %
•? ^ "" S """"N ••••""
^ ^ ^^ v ^ \% « V ^
-2.82
1.10
-0.62
0.94
...... w ; ^5 s^vssvsv v.x% ^ ss s s

\ ^Ssvlss , s°S sU •>"
1.33
-0.48

, y -4*85"' •'' ^K
0.42

* xJtV s •"'•S^':'- ""•• \*Nv ^
0.48
1.09
-0.04
0.99
V-^S ^ hS AVSSSSM •.-,•. VS V. SSSS %S
-.'"'•'• \s- ^ """• - '' -.-^ ^
^ "" o^s ^;^ -Xj1" C •* «. '•^

^ •• v V ° s V %'•• "" s * ^ " ^"
"• "•r^ ^ ^«s ••
/^^%fe^>^:~-
0.45
0.40
2.20
-1.37
^4:>^;§^'
-1.40
1 " ^ ^x^s _•• *s" c; Xs" v
t&; v^4\/ *c^- %; v;
0.70
1.21
-0.85
-2.89
1.20
~ " ' - \ ' - \ ' -
-0.76
2.53
0.36
-2.99
-1.59
1.04
ft s Above
& = Below
-0.72
0.16
*:AV., -;',•!,
-0.72
-0.90
JSS ff-.^ .V. ^ V V % ^
s "• % Xs ^ ••
s- S " •-
-3.08 Ji
0.84
-0.88
0.68
w^ v -. , ™ v. -. -, v •. ss s

S_ ^ " "" *
1.07
-0.74

sljJilV-'- -*X
0.16

, -\\-\v^ ~; • -v
0.23
0.83
-0.30
0.73
V V •- V.V. S-, ., •.•.-. S ,
•> •• : •.'*'' % ^
•.-. its*1 •>•>,_ •> "" V','' \-" tv ..
* "• •• •• V> s
•

, ^ S^;N " ^ • ^
0.19
0.14
1.95
-1.63
-;^>°\;y»- ^ s" --
-1.66
*~ ^ s
,\"- :> - - - v * ~
0.44
0.95
-1.10
-3.15 Ji
0.94
• 
-------
12 /
14 EMSL-LV Intercomparison Study: Radium in Water, 5-Mar-1993

Radium-228
Lab
PC
IsVt
pp
pf
PV
PW
PX
PY
Q
QB
QJ
QQ
Qtf
QX
QZ
BU
R(d
RD
RF
RL
RM
RN
RV
RW
RZ
S
SA
sc
SD
SF
SI
SM
SS
ST
SW
sx
sz
T
TA
TD
TG
TH
TI
TK
TL
Res. 1
f^tr?^:
"" ' *~ '-'
13.1
,' - •» ~\ ', ' • '
13.7


15.4
> • <:" ,>'V, V
, "?
H - :V'"'tM
' * ' *
27.9
15.6
"«v'v *TH:
\ ' ^ v
22.8
21.5
15.3
17.2
14.3
14.2
11.8
16.4
18.7
18.3
19.2
25.1
20.2
16.5
18.9
10.2
23.2
15.0
21.7
18.5
19.7
' ' - ",'''"

24.1
v'r \ '~- '"'-
16.0
Res. 2
'/fV^^tr
•o-.,- "<,*•• ; - -„•> v.
16.4
12.5

.--'- * - '"•" i'
13.0
.-„• •"",' ' '*• :%, -*"-

• *1 - >• '' ""',';
,, -'vv-',r-, :
27.3
15.3
; VVv-;, ;;;;.:',
20.4
18.7
15.3
18.8
15.1
14.5
12.2
17.5
14.1
' V
20.0
19.4
25.9
20.6
15.1
21.0
11.4
20.0
16.0
20.4
16.2
21.7
^ f-

, ff :
22.3
- . ,---' - - > •
19.0
Res. 3
^^v,;
'""•"' , ,- ,
16.6
17.5
' ; '". "",
•• -. ••
12.7
v-- /v,^
A
% J \' •. ,_
s ^ ~-f

26.7
15.8
- ~t " *\' '-,
19.3
19.5
14.9
15.0
15.4
14.4
11.6
21.7
12.6

19.1
20.6
31.8
23.0
14.3
22.0
10.1
19.4
17.0
21.2
18.8
19.2


,
24.8

16.4
• = No data submitted
0 a
Insufficient
data
X s
Exper.
Sigma
t'vv ;? v "
t '* ^
1.97
2.61
51 : '
1.48
A ' '-

1s _. ""

0.60
0.25

1.79
1.44
0.23
1.91
0.57
0.15
0.31
2.80
3.18
0.85
0.76
3.66
1.51
1.11
4.58
0.72
2.04
1.00
0.66
1.42
1.32


1.29

1.63
Rng anal Normalized deviation
(R + SR) Average (grand-avg) (known) Tag


0.449
0.642

0.347




0.154
0.064

0.449
0.360
0.051
0.488
0.141'
0.039
0.077
0.681
0.783
0.218
0.180
0.860
0.360
0.282
0.398
0.167
0.488
0.257
0.167
0.334
0.321


0.321

0.385
V '' •• '\ / •- ""' "J^1

15.37
14.57

13.70




27.30
15.57
,
20.83
19.90
15.17
17.00
14.93
14.37
11.87
18.53
15.13
19.13
19.73
27.60
21.27 .
15.30
20.63
10.57
20.87
16.00
21.10
17.83
20.20


23.73

17.13
TAG SYMBOLS
Determined
to be an
outlier
j ' f "" X "" •£'

-0.92
-1.22

-1.55
•.',-;?••

- •* *'*', ... '

3.57
-0.85
" '' J..'' ~-f '/
1.14
0.79
-1.00
-0.31
-1.08
-1.30
-2.24
0.27
-1.01
0.50
0.72
3.69
1.30
-0.95
1.06
-2.73
1.15
-0.68
1.24
0.01
0.90


2.23

-0.26
ft = Above
^rf,*^v?
'•> ," '•" -' • > v~ /
-1.18
-1.48
" X-'- ' •"-
„ , • ': »,
-1.81
- . - •
• '
' * '
»
3.31 ft
-1.10
'' ': ! "• ,
0.88
0.53
-1.26
-0.56
-1.34
-1.56
-2.50
0.01
-1.27
0.24
0.46
3.43 ft
1.04
-1.20
0.80
-2.99
0.89
-0.94
0.98
-0.25
0.64
' -- - •
•
1.97
. • •
-0.51
control limit
JJ = Below control limit

-------
EMSL-LV Intercomparison Study: Radium
Radium-228

Lab Res. 1 Res. 2
TN 14.7 16.8
TQ ^ 17.7 _ 21.5
^mff^^t^*^^^*"1^^"^^
-;Tt^-5^&i- ^ ^IS v iS

*U 	 ^'""jgj" 	 ~ 1?'4
^^Y^j^^S ^^^^I^^^^X^I^-^^ S^?-l
•^ ss%J.»S>..i^ ^ ^li\:i\ ; ^^V:t^^il% s" ^V^x^^^^rV'',,
^W^^v^^^.-J^^^^^^^^i^
^J^I^il&S'>^^ffiS^S;ElS??!A^^^
UE 22.5 19.0
'X'iff^^^yy1^^^^^^^^^^

" j^p"-""' ..^^V*~*™^<_££ v~
W 15.8 16.7
J[_ 	 16.6 __ .18.2
xi! v^5£3i1^';SW«W? ^1K » ^ ^!1il
s •.-. \"^% *•'•'''' t^s'"v, -.^>.\ * *x\'"' NSXwii V •. s ^v. •i' *' '"1^\\ v \%*s
Z 18.7 18.5

Exper. Rng anal
Res. 3 Sigma (R + SR)
19.8 2.56 0.655
17.6 2.22 0.501
"^;v\^V^~" *•" ' '= ' ,> ! ' ' ''*"•
,;^vl/,\~ - - - , >\ -; -
|PfR; 'V/ "" "''.:> ^
16.9 0.55 ,0.141
i*^t\o ^T^^\X^- ^ xv ""••" -"" 'v\r"w -.'"•• ^ ^V11 ' " ••"
\ ^^ *s" w vHr ~" •• "
Kv^t:^s£vft'-\^ ^ "^ s \- - \ ^
hflS^ii^V^ v \,\^s,\ : ;- s ^'-
21.1 1.76 0.449
^lSJ?"?~f\A,"~ "V • •' 	 " ' ' ~ "
^ij;|||t:;^:,\ >A c- /?
^mi>16.7" '" 1.12 OA24
15.4 0.67 0.167
18.2 0.92 0.205
^\fi^s - -^,V; ,s ^ - - •' " !
^ lO^*'". s" sss'^i'1 •!' s *" "• v "
18.7 0.12 0.026
in Water, 5-Mar-1993 13

Normalized deviation
Average (grand-avg) (known)
17.10 -0.27 -0.53
18.93 0.42 0.16
: "•'» ;,,/ ~\ "^t. v ....„., xsS^^x; , \.,i ~'V-;"".
'•< - ,- Vv^— v^ ,-lJr^'"
1 ••fe^-jfs^^'"^^
16.87 -0.36 -0.62
^ ^ > '•••v^-C™':, " ^^^X1*"!: ^W^V* •• ^'"•^ ^«t '•>'•'"• ^ " v^r ^ v.1-1- v s ^
s ^ ^^ > ''^'"'C* "v N^'"v ^v'' "" •-; s ••
s ?:""\ \' ^%K,* s ^ %4^ ^v S '** * %
\, - - !." * s ^--"-v? ;«wi\*\-o \s^sV ^\V "
20.87 1.15 0.89
"T"""™ ~!"7™"~sTT' "7\ •""""" * ' * -
; ; ^ - ' ^:&li|:(v I - ;X* ,; x\ c . • -:
16.13 -0.63 -6"89
15.97 -0.70 -0.95
17.67 ,-0.05 -0.31
, '„ - r>~- ,i-V' '•!"•- '. ;/

18.63 0.31 0.05
/14 1
^

Tag


>r)« V
' «-^: '
^?

*\ ^"^t ™v;-
^ i ^ "•

/;s?x"


,',.;;-



* :' "
s%i

Data sorted by Laboratory Average
Average Tag
4.93 x
7.10 U
9.87 U
10.13 U
10.33 U
10.47 &
10.57
11.87
13.03
13.10
13.43
13.60
13.70
14.10
14.13
14.17
14.37
14.57
14.93
14.93
15.13
15.17
15.30
15.37
15.43
• = No data submitted
0 s Insufficient data
Lab Average Tag
JY 15.47
GN 15.57
OY 15.57
NO- 15.80
D3 15.97
AP 16.00
ST 16.10
RW 16.13
FN 16.17
DB 16.40
FZ 16.53
P 16.60
Q 16.60
MS 16.87
AW 17.00
ME 17.10
RV 17.10
PV 17.13
RN 17.17
GQ 17.27
S 17.37
RL 17.40
SM 17.43
PP 17.67
EB 17.70
TAG SYMBOLS
Lab Average Tag
FP 17.83
QZ 17.83
NH 18.43
OF 18.50
W 18.53
SX 18.63
I 18.73
UN 18.77
JE 18.87
HE 18.93
JX 18.93
HY 18.93
HL 18.93
U 19.00
RM 19.10
TN 19.10
DZ 19.13
TL 19.23
BO 19.33
AE 19.40
EO 19.67
AL 19.70
CK 19.73
X 19.77
KZ 19.90
tt s Above control
x = Determined to be an outlier M = Below control
Lab
T
BA
HK
DT
RZ
Z
BK
OX
LT
HP
A
TQ
K
LS
KH
AI
SC
BM
CJ
BH
N
CE
SD
BC
RF
limit
limit

-------
14 / 14 EMSL-LV Intel-comparison Study: Radium in Water, 5-Mar-1993
Radium-228

Average Tag
19.90
20.20
20.30
20.43
20.47
20.50
20.57
20.63
20.70
% responding labs

IU' -----------

° -6 ' -'4
% responding labs

10'

-6 -4


Data sorted by Laboratory Average
Lab
AK
TA
JG
L
AF
AZ
PB
SS
KL
Average Tag Lab
20.73 J
20.77 CA
20.83 RD
20.87 -UE
20.87 SW
20.90 AJ
21.00 NT
21.00 CS
21.03 NG
21.10 SZ
Average Tag
21.27
21.33
21.53
21.67
23.43
23.67
23.73
24.53
27.30 ft
27.60 ft
Frequency distribution

• ___ 1- •• 	
.. . ..•.hlll.lllill. ...
-2 0 +2 +4
Normalized deviation of the mean from the known value
Frequency distribution
|__l 	 _- 	 	 	 .
. -•• _ 	 	
•Illl . . -
-2 0 +2 +4
Normalized deviation of the mean from the grand average
7



Lab
SI
JS
c
DE
CG
M
TI
OS
QX
SF




+6




+6

• = No data submitted
0 s Insufficient data
       TAG SYMBOLS
x s Determined to be an outlier
ft s Above control limit
•U s Below control limit

-------