NERC-LV-539-30 FINAL REPORT OF THE RADIOLOGICAL SURVEILLANCE PROGRAM FOR THE PROJECT GASBUGGY PRODUCTION TEST May 15, 1973 to November 6, 1973 by the Monitoring Applications Laboratory National Environmental Research Center U. S. ENVIRONMENTAL PROTECTION AGENCY Las Vegas, Nevada Published August 1974 This work performed under a Memorandum of Understanding No. AT(26-1)-539 for the U. S. ATOMIC ENERGY COMMISSION ------- This report was prepared as an account of work sponsored by the United States Government. Neither the United States nor the United States Atomic Energy Commission, nor any of their employees, nor any of their contractors, subcontractors, or their employees, make any warranty, express or implied, or assume any legal lia- bility or responsibility for the accuracy, completeness or use- fulness of any information, apparatus, product or process disclosed, or represent that its use would not infringe privately-owned rights. Available from the National Technical Information Service, U. S. Department of Commerce, Springfield, VA 22151 Price: Paper copy $5.45; microfiche $1.45 ------- NERC-LV-539-30 FINAL REPORT OF THE RADIOLOGICAL SURVEILLANCE PROGRAM FOR THE PROJECT GASBUGGY PRODUCTION TEST May 15, 1973 to November 6, 1973 by the Monitoring Applications Laboratory National Environmental Research Center U. S. ENVIRONMENTAL PROTECTION AGENCY Las Vegas, Nevada Published August 1974 This work performed under a Memorandum of Understanding No. AT(26-l)-539 for the U. S. ATOMIC ENERGY COMMISSION ------- ABSTRACT A production test of the Project Gasbuggy nuclear-stimulated natural gas well (GB-ER) was conducted from May 15, 1973, through November 6, 1973. This test was sponsored by the El Paso Natural Gas Company, the Atomic Energy Commission, and the U. S. Bureau of Mines. The test well, located about 88 km (55 mi) east of Farmington, New Mexico, had been shut-in for about 42 months since an earlier production test. Data furnished by the El Paso Natural Gas Company indicate that a total of about 49 Ci of 3H and about 4.7 Ci of 85Kr was released into the atmosphere during the flaring of about 3.03 million cubic meters (107 MMCF) of natural gas. For the purpose of determining the impact of the production test on the environment, environmental monitoring was provided by the U. S. Environmental Protection Agency, National Environmental Research Center-Las Vegas. Aerial and ground surveillance teams collected environmental samples prior to, during, and after the production test. During the environmental monitoring program, samples of air were analyzed for 85Kr, and samples of atmospheric moisture, vegetation, soil, precipitation, and surface water were analyzed for H. Based upon wind patterns and aircraft trackings, samples were collected where the maximum concentrations of these nuclides would be expected to be found. In addition, aerial and ground sampling was done where maximum concentrations were most likely to be found at times of the day during which maximum and minimum atmospheric mixing conditions occurred. Also, contaminated water removed from the gas was stored and injected into the flare at higher than normal rates dur- ing most of the surveillance operations. Out of 13 compressed air samples collected during the production test, one had a 85Kr concentration (21 ± 1.0 pCi/m3) which was higher than normal and may indicate a contribution from the production test. Tritium levels above esti- mated background (1000 pCi/1 H20) were found in some samples of each type of environmental media collected with the exception of surface water. From the highest concentration of 3H measured in atmospheric moisture samples, it is concluded that any direct exposure to hypothetical off-site receptors was below ------- 0.4% of the Concentration Guide for a suitable population sample in an un- controlled area as listed in the Atomic Energy Commission's Manual, Chapter 0524, "Standards for Radiation Protection." The analytical results of post-flaring sample collection showed concen- trations of 3H above estimated background on 10 out of 25 post-flaring vegeta- tion samples that were collected from all four compass quadrants surrounding the flare stack. One of 25 soil samples collected showed a concentration of 3H slightly above the estimated background. There are no guides for vegetation or soil; however, all vegetation samples collected were native uncultivated shrubs which would not constitute additional exposure to the off-site popula- tion. ii ------- TABLE OF CONTENTS Page ABSTRACT i LIST OF FIGURES iv LIST OF TABLES v INTRODUCTION 1 GENERAL OPERATIONAL PROCEDURES 3 Aerial Surveillance 3 Ground Monitoring 4 Analytical Procedures 5 PRE-FLARING SAMPLE COLLECTION RESULTS 1973 7 Sampling Procedures 7 Results 7 FLARING SURVEILLANCE PROCEDURES AND RESULTS MAY 1973 9 May 19. 1973 9 May 20. 1973 10 May 21. 1973 11 Results of Aerial Operations 12 Ground Monitoring Results 13 FLARING SURVEILLANCE PROCEDURES AND RESULTS JULY 1973 14 July 25, 1973 14 July 26. 1973 15 Results of Aerial Operations 16 Ground Monitoring Results 16 POST-FLARING SAMPLE COLLECTION AND RESULTS NOVEMBER 1973 17 Sampling Procedures 17 Results of Post-Flaring Sample Collection 17 SUMMARY AND CONCLUSION 18 REFERENCES 20 iii ------- LIST OF FIGURES No. Page 1. Gasbuggy Sampling Locations 22 2. Close-in Gasbuggy Sampling Locations 23 3. Variation of Natural Gas Flow Rate During Flaring Period 24 iv ------- LIST OF TABLES No. Page 1. Quantities of Natural Gas Flared and Radioactivity Released 25 During Project Gasbuggy Production Test May 15 - November 6, 1973 2. Analytical Results of Pre-Flaring Water and Precipitation 28 Samples Collected May 1973, for Project Gasbuggy Production Test 3. Analytical Results of Pre-Flaring Atmospheric Moisture Samples 29 Collected May 1973, for Project Gasbuggy Production Test 4. Analytical Results of Pre-Flaring Compressed Air Samples 30 Collected May 1973, for Project Gasbuggy Production Test 5. Analytical Results of Pre-Flaring Vegetation Samples Collected 31 May 1973, for Project Gasbuggy Production Test 6. Analytical Results of Pre-Flaring Soil Samples Collected May 33 1973 7. Analytical Results of Aircraft Atmospheric Moisture Samples 35 Collected May 1973, for Project Gasbuggy Production Test 8. Analytical Results of Aircraft Compressed Air Samples Collected 36 May 1973, for Project Gasbuggy Production Test 9. Analytical Results of Water Samples Collected May 1973, for 37 Project Gasbuggy Production Test 10. Analytical Results of Atmospheric Moisture Samples Collected 38 May 1973, on the Ground for Project Gasbuggy Production Test 11. Analytical Results of Vegetation Samples Collected May 1973, 40 for Project Gasbuggy Production Test 12. Analytical Results of Soil Samples Collected May 1973, for 41 Project Gasbuggy Production Test ------- No. Page 13. Analytical Results of Aircraft Atmospheric Moisture Samples 42 Collected July 1973, for Project Gasbuggy Production Test 14. Analytical Results of Aircraft Compressed Air Samples Collected 43 July 1973, for Project Gasbuggy Production Test 15. Analytical Results of Atmospheric Moisture Samples Collected 44 July 1973, on the Ground for Project Gasbuggy Production Test 16. Analytical Results of Water Samples Collected July 1973, for 45 Project Gasbuggy Production Test 17. Analytical Results of Vegetation Samples Collected July 1973, 46 for Project Gasbuggy Production Test 18. Analytical Results of Soil Samples Collected July 1973, for 47 Project Gasbuggy Production Test 19. Analytical Results of Compressed Air Samples Collected July 48 1973, on the Ground for Project Gasbuggy Production Test 20. Analytical Results of Post-Flaring Water Samples Collected 49 November 1973, for Project Gasbuggy Production Test 21. Analytical Results of Post-Flaring Vegetation Samples Collected 50 November 1973, for Project Gasbuggy Production Test 22. Analytical Results of Post-Flaring Soil Samples Collected 52 November 1973, for Project Gasbuggy Production Test vi ------- INTRODUCTION Under a Memorandum of Understanding between the Atomic Energy Commission (AEC) and the Environmental Protection Agency (EPA), the EPA's National Environmental Research Center-Las Vegas (NERC-LV) carried out a program of off-site radiological surveillance for a Project Gasbuggy production test during 1973. Project Gasbuggy was a joint Government-Industry project for the purpose of testing the feasibility of increasing the yield of natural gas wells by detonating a nuclear device below the gas-bearing formation, thus increasing the permeability of the host rock. The detonation took place on December 10, 1967, about 88 km (55 mi) east of Farmington, New Mexico. This report describes the procedures and results of the NERC-LV surveillance program. This surveillance consisted of the collection of environmental samples on the ground during pre-flaring, flaring, and post-flaring periods. During flaring operations, periodic in-cloud aerial sampling and tracking were done with an EPA aircraft. The surveillance was a continuation of Project Gasbuggy surveillance programs starting with pre-detonation, detonation, re-entry and initial flaring operations. The results of previous Gasbuggy surveillance programs have been reported earlier.1"^ The purpose of this test was to obtain data which would provide a more thorough understanding of the reservoir characteristics of the chimney and fracture zones created by the initial detonation after the well had been closed-in for about 42 months since a previous production test. Details of the purpose and nature of this flaring operation have been described by the U.S. Atomic Energy Commission.6 Briefly, the test consisted of an initial rapid draw-down phase, a steady-pressure phase with low flare rates, and a final rapid pressure draw-down phase accompanied by high rates of gas flar- ing. The initial draw-down phase began on May 15, 1973, and the well was shut-in on November 6, 1973. Table 1 lists the cumulative gas flared, the average gas flaring rate, and the estimated quantities of radionuclides released for consecutive 7-day ------- periods. In addition, Table 1 shows when EPA aircraft and mobile monitors were conducting their surveillance activities. As shown in Table 1, water that had been extracted from the natural gas and stored in tanks was intro- duced into the flare as steam principally at the beginning and end of the flaring period. Water was removed from the gas so that more accurate flow- rate measurements could be made. The later water injection, in the form of steam injected into the flare, was done for the production test to simplify disposal of the 3H contaminated water. The information provided in Table 1 was furnished by the El Paso Natural Gas Company.7 Surveillance for the Gasbuggy production test was first begun with pre- flaring sample collection on May 3-8, 1973, for the purpose of establishing a base-line for comparing results obtained during flaring and post-flaring surveillance. Following the pre-flaring sampling, flaring surveillance opera- tions were undertaken during May 19-21, 1973, when maximum flow and steam injection occurred, and during July 25-26, 1973, a period when steady flow at a reduced rate had been established. A final post-flaring surveillance opera- tion was conducted during November 6-8, 1973. Each operation is treated as complete in itself and includes the specific description of operational procedures and results. A discussion of the total environmental impact is presented in the Summary and Conclusion section. ------- GENERAL OPERATIONAL PROCEDURES From previous surveillance programs for Project Gasbuggy, the radionu- clides of primary concern had been identified as 3H and 85Kr.2 In air these nuclides may both be of public health significance, whereas in other environ- mental media, such as water, vegetation, and soil, only the 3H may be a potential hazard due to its relatively rapid assimilation into the environment in the form of moisture. Krypton-85 is chemically inert and does not readily combine with most environmental media. For these reasons all surveillance attempts were directed toward the detection of both 3H and 85Kr in air and to the detection of 3H in other environmental media such as water, vegetation, and soil in areas surrounding the test well. Aerial Surveillance Aerial surveillance was provided by an EPA turbo-Beech aircraft equipped with an Environment/One Condensation Nuclei Monitor (CNM) and air sampling equipment. The CNM was used to detect and track the effluent plume discharged from the 15-meter flaring stack because the plume was invisible, and radio- activity levels were too low to be detected with conventional instruments. The CNM measured the concentration of condensation nuclei, generated by flar- ing operations, per unit volume of air. The CNM output was recorded on a strip- chart recorder located in the aircraft crew chief's instrument panel. This chart was annotated with names of appropriate landmarks on the ground so that the record of plume location could be used to position mobile monitors. Because of the anticipated low radioactivity levels, samples were collected only from the plume, to the extent possible. Air samples were collected in a one-cubic-meter plastic bag which was filled in approximately 10 seconds while the aircraft passed through the plume at a speed of about 160 knots, true air speed. A compressor then drew the air from the bag through a canister of 13X molecular sieve for collection of water vapor and compressed the remainder of the sample into a tank. The adsorbed water vapor was analyzed for 3H, and the compressed air sample was analyzed for 85Kr and radioxenon. ------- Ground elevation at the 15 m (50 ft) flare stack was 2190 m (7200 ft) above mean sea level (MSL).* Terrain within 3.2 km (2 mi) of the flare stack varied from 2130 m (7000 ft) to 2260 m (7400 ft). The general procedure was to perform an initial spiral descent from approximately 900 m (3000 ft) above the surface at a 1.6 km (1.0 mi) radius from the flare stack. A descent rate of 150 m (500 ft) per minute was maintained. This spiral descent identified the height of the plume and its direction of movement. Several passes were then made across the plume near the surface in order to locate positions for placement of mobile ground monitors. Because of the inherent delay in the CNM response (on the order of 2 to 5 seconds), these passes were made on reciprocal headings to obtain a fix on the plume centerline and edges. In most cases, a mobile monitor was then positioned downwind of the plume, and an aerial grab sample was collected over his location with a one-cubic-meter bag. When possible, the procedure was repeated farther downwind out to a distance of 8.0 km (5.0 mi). During the May and July sampling periods, the aircraft at- tempted to locate the effluent beyond 8.0 km (5.0 mi) of the flare stack. The maximum distance at which plume material was detected was 11 km (7.0 mi). Ground Monitoring In addition to the normal complement of equipment for the collection of water, vegetation, air, and other environmental samples, the NERC-LV mobile monitors were equipped with sampling apparatus designed for sampling 3H in atmospheric moisture and for sampling noble gases. Each monitor carried several molecular sieve sampling heads for atmospheric moisture collection. The heads consisted of a polyvinylchloride cylinder, 12.7 cm (5 in) long and 6.3 cm (2.5 in) in diameter, containing 300 g of 13X molecular sieve. The intake end of the sampling head held a 7.6-cm (3-in) diameter particulate filter (used primarily to prevent the introduction of foreign substances), and the outlet was equipped with a pipe-fitting attached to a dry-gas meter. Airflow was provided by a portable vacuum pump powered by a 12-volt battery. *A11 elevations in this report are above MSL unless otherwise stated. ------- Special 24-volt DC air compressors were carried by several monitors for the collection of compressed air samples. The air was pumped into a pressure tank until a pressure of 2.8 MPa (400 psig) was obtained. This was approxi- mately equal to one cubic meter of air at atmospheric pressure at the sampling altitude. For soil collection, a 30.5-cm (12-in) square steel frame, 2.5 cm (1 in) deep, was pressed into the ground until it was level with the surface. Soil within the frame was then removed with a trowel. All of the soil samples were collected to a depth of 2.5 cm (1 in) except for profile samples taken at Station 9 (Figure 1). These profile samples are identified in the tables. Analytical Procedures Sample analysis was done at the NERC-LV laboratory. Each atmospheric moisture sample was transferred to a heating vessel where the water was elutri- ated at 350° C with a dry He purge. Recovery of water from the absorber nor- mally exceeded 95%. This water was then re-distilled to eliminate possible interference by other contaminants. The 3H concentration in the re-distilled water was determined by liquid scintillation spectrometry. This was accomplished by taking 5 ml of the recovered water, 5 ml of a 3H standard (for counting effi- iency), and 5 ml of 3H-free water (for instrument background). The solution was then diluted with 20 ml of a dark-adapted scintillation cocktail. The sample, standard, and background mixtures were counted for 200 minutes in a liquid scintillation spectrometer optimized for 3H.8 The minimum detectable concentration (MDC) for 3H was determined to be about 200 pCi/1 of H20 at the 95% confidence level, based upon the 200-minute count and 5 ml of atmospheric water. Snow and surface water samples were re-distilled and analyzed in the same manner as the water from the molecular sieves. Moisture from vegetation and soil samples was recovered by vacuum distillation. The recovered water was re- distilled and analyzed in the same manner as the water from the molecular sieve samples. ------- Compressed air samples, about one cubic meter in volume, were analyzed for 85Kr and radioxenon by gas chromatography and liquid scintillation tech- niques as described by Stevenson and Johns.^ The MDC for these radionuclides at the 95% confidence level is 5 pCi/m3 and 2 pCi/m3, respectively. ------- PRE-FLARING SAMPLE COLLECTION AND RESULTS MAY 5-8, 1973 Sampling Procedures During the pre-flaring sampling program, 17 locations were selected within a 32-km (20-mi) radius of the flare stack. Three ponds within an 11-km (7-mi) radius of the flare stack were selected for surface water samples. Not all types of samples were collected at all of the 17 pre-selected sampling locations. During the pre-flaring sampling period, 2 compressed air, 10 atmospheric mois- ture, 17 vegetation, 18 soil, 3 water, and 2 snow samples were collected. Fig- ures 1 and 2 show the sampling locations. Other sampling locations numbered 18 and higher were added during the production test. Results Since one of the two compressed air samples was lost, only one result for 85Kr prior to flaring operations was available. This sample showed a 85Kr con- centration of 17 ± 1.0 pCi/m3 of air. This is similar to values reported in the literature. Andrews10 reported a mean concentration of 16 ± 4.0 pCi/m3 (± two standard deviations) which was calculated from the results of weekly samples collected from a continuously-operated air sampler at Las Vegas, Nevada, over the twelve-month period April 1972 through March 1973. Also, from estimates of projected releases of 85Kr from nuclear facilities throughout the world, Bernhardt * predicted that the atmospheric concentration of 85Kr would be 13 pCi/m3 in 1970 and 25 pCi/m3 in 1975. Tables 2 through 6 show the analytical results and the two-sigma counting errors of all other samples collected prior to flaring operations. The ranges and averages of the 3H concentrations in each sample type are as follows: ------- Sample Type Surface water Snow Soil Vegetation Atmospheric moisture No. of Samples 3 2 18 17 10 3H Concentration, pCi/1 Maximum Minimum <240 410 500 1200 650 ± 240 ± 240 ± 260 ± 240 <240 380 ± 250 <240 <240 <200 H20 Average <240 400 323 570 390 In the computation of the average concentrations, the values less than the MDC were set equal to the MDC. The two-sigma counting error is given for each maximum and minimum concentration above the MDC. The pre-flaring samples were collected as a cursory check on background concentrations of 3H with the understanding that seasonal and geographical variations in background can not be precisely defined with the limited num- ber of samples collected. During a surveillance program for Project Gasbuggy in previous years, a 3H background concentration of about 1000 pCi/1 of water was used.2 Although 3H concentrations have been known to occasionally vary above this concentration, such as the 1200 pCi/1 concentration for a pre- flaring vegetation sample, the 1000 pCi/1 value for background is used through- out this report with the acknowledgment that the background concentration is variable. ------- FLARING SURVEILLANCE PROCEDURES AND RESULTS MAY 19-21, 1973 May 19, 1973 During the morning of May 19, 1973, the aircraft flew a mission to determine characteristics of drainage winds and to collect air samples at a time when no tritiated water was being injected into the flare. Mobile monitors were not involved in the morning sampling effort. Until 0930 hours the plume was moving 330° from the flare stack following a ridge along the north side of Leandro Canyon (Figure 1). A grab sample was collected at 0905 hours, 1.9 km (1.2 mi) northwest of the flare stack at an altitude of 2440 m (8000 ft). In this area the terrain ranges in altitude from 2190 m (7200 ft) to 2260 m (7400 ft). At 0917 hours, a spiral descent was started. The top of the plume was identified at 2590 m (8500 ft) with the maximum concentrations of nuclei at 2320 m (7600 ft). Condensation nuclei concentration at 2440 m (8000 ft) during sampling was within a factor of two of the concentration measured at 2320 m (7600 ft) during the spiral descent. At 0939 hours, the plume was again detected at 1.6 km (1 mi) east of the flare stack at an altitude of 2350 m (7700 ft). At 0946 hours, a spiral descent was started 3.7 km (2.3 mi) east of the flare stack where the plume top was found to be at 2680 m (8800 ft) with the maximum concentration of nuclei at 2320 m (7600 ft) over ground elevation of 2200 m (7200 ft). A grab sample was collected in two halves at the plume centerline on two successive passes at 2320 m (7600 ft) at 1002 hours. Unstable atmospheric conditions caused moderate turbulence and direc- tional instability of the plume as well as vertical mixing. At 1002 hours, the plume width at 3.7 km (2.3 mi) east of the flare stack was about 7 km (4.5 mi). The morning mission was terminated at that time. On the afternoon of May 19, at 1330 hours, the aircraft returned to the area along with the mobile monitors for the purpose of conducting a coordinated ------- aerial-ground sampling mission. Water injection into the flare had beguii at 1200 hours and was continued until 1600 hours. Malfunction of the CNM pre- vented plume detection until 1405 hours when a spiral descent was started 2.1 km (1.3 mi) east of the flare stack. The plume top was found at 2900 m (9500 ft). Mobile monitors were sent to Stations 18 and 19 (Figure 2) to start atmospheric moisture sampling and to collect vegetation and soil samples. Meanwhile, the maximum concentration of nuclei was found at 2590 m (8500 ft) and an aerial grab sample was collected at that elevation at 1423 hours over Station 19, 1.6 km (1 mi) at 110° from the flare stack. Further investigation by the aircraft indicated the plume base to be above ground level. Highly unstable atmospheric conditions soon made plume detection impossible and the aerial and ground operations were terminated at approximately 1500 hours. May 20, 1973 Water injection into the flare began at 0800 hours. Difficulties with the CNM prevented making measurements until 0857 hours. Without aircraft tracking information, and assuming that downslope drainage winds were sim- ilar to those on May 19, mobile monitors were directed to begin atmospheric moisture sampling at Stations 8, 11, and 20 (Figure 2). Doppler radar results showed westerly winds over the mobile monitor locations varying from 5 knots at the surface to 20-25 knots 910 m (3000 ft) above the surface. The CNM began functioning properly and a spiral descent was begun on a 1.6-km (1-mi) radius around the flare stack at 0900 hours. The plume top was found at 2740 m (9000 ft) with the maximum concentration of nuclei at 2590 m (8500 ft). Mobile monitors were sent to Stations 18 and 19 to begin sampling, and an aerial grab sample was collected over Station 19. This sample was taken at 2590 m (8500 ft) at 0925 hours. The aircraft established a north-south pattern about 8.0 km (5 mi) east of the flare stack. The pattern showed the plume to be centered at 75° from the flare stack. A mobile monitor started atmospheric moisture sampling at this location (Station 21) at 1020 hours. A spiral descent by the aircraft 10 ------- over Station 21 showed the plume top at 3350 m (11,000 ft), with the maximum concentration of nuclei at 3200 m (10,500 ft). Most of the plume material was above 2740 m (9000 ft), but some material was detected down to 30 m (100 ft) above ground level, which is 2160 m (7100 ft) at this location. At this time, the plume seemed to be centered over Station 21 with the north edge passing over Station 9 and the south edge passing over Station 19. Mobile monitors were directed to take compressed air samples at Stations 19 and 20. A second spiral descent was made by the aircraft in the vicinity of Station 21 where the plume centerline was located at 2740 m (9000 ft). A grab sample was taken at this point at 1040 hours. Because of fluctuating plume height due to turbulence, this sample may not have been collected at the center- line. Malfunction of the CNM prevented an afternoon mission. Vegetation and soil samples were collected at Stations 8, 9, 11, 18, 19, 20, and 21 (Figures 1 and 2). May 21. 1973 Mobile monitors arrived in the area at 0645 hours and determined that the direction of the downwind drainage winds was generally NNW of the flare stack. Mobile monitors were sent to Stations 8, 11, and 20 where they began atmospheric moisture sampling. The Station 8 monitor began sampling at 0725 hours, and Stations 11 and 20 at 0715. Injection of water into the flare was supposed to have started at 0700 hours; however, some problems were encountered which delayed water injection until 0725 hours. The aircraft began tracking at 0745 hours and the plume material was found to be on a heading of 330° from the flare stack. A grab sample was collected over Station 20 at an altitude of 2320 m (7600 ft) at 0800 hours. Indications were that the plume was moving in a more northerly direction and by 0815 hours, the plume was centered on a 30° trajectory. The mobile monitor at Station 11 then started another atmospheric moisture sample at 0800 hours. In addition, an atmospheric moisture sample was started at Station 22 at 0825 hours. 11 ------- The aircraft began a spiral descent around the flare stack at 0830 hours at an altitude of 2900 m (9500 ft), and descended to within 61 m (200 ft) of the surface. The plume material was found to be rising nearly vertically due to very light winds. Several spiral descents and ascents were accomplished during the next hour; however, no plume material was found beyond 1.6 km (1 mi) of the flare stack. At about 0840 hours, a slight indication of plume material was found at 30 m (100 ft) above ground level at 0.4 km (0.25 mi) northwest of the flare stack. A mobile monitor had already started atmospheric moisture sampling at Station 18. Aircraft tracking continued to indicate that the plume was rising nearly vertically above the flaring stack and that unstable air was causing direc- tional instability of the plume material. At about 0945 hours, wind speeds increased causing the plume to move along the surface on an ESE direction. A mobile monitor started atmospheric moisture sampling at Station 23, 3.5 km (2.2 mi) at 126° from the flare stack at 1004 hours. Shortly thereafter, wind speeds decreased and the plume again began rising vertically. The aircraft took a final grab sample at 3050 m (10,000 ft) 3.2 km (2 mi) southeast of the flare stack at 1025 hours. Water injection ceased at 1015 hours when the stored water was exhausted so that this sample may not have been from that portion of the plume containing injected water. The aerial mission was terminated at this time. Surface water samples were collected at Stations 27 through 31, and veg- etation samples were collected at Stations 17, 22, and 23. In addition, soil samples were collected at Stations 22 and 23. The ground monitoring mission was terminated by 1200 hours. Results of Aerial Operations Tables 7 and 8 list the analytical results of all samples collected by the aircraft during the May 19-21 surveillance mission. Of the seven aerial atmospheric moisture samples that were collected, four contained concentrations of 3H above 1000 pCi/1 of H20. The maximum concentration of 3H was 2800 pCi/1 of H20. This concentration expressed as 24 ± 2.9 pCi/m3 of air is 0.04% of the Concentration Guide specified in the AEG Manual, Chapter 0524, for a suitable 12 ------- population sample in an uncontrolled area.12 The associated compressed air samples did not show concentrations of 85Kr that could definitely be considered to be above background except for the sample collected at an azimuth of 330° and a distance of 1.9 km (1.2 mi) from the flare stack on May 19. This sample, which had a 85Kr concentration of 21 ± 1.0 pCi/m3, was slightly higher than all others collected during the period May 19-21 and higher than the 95% con- fidence interval of the annual average of 85Kr concentrations measured in Las Vegas.10 Since an atmospheric moisture sample collected at the same time showed a 3H concentration above background, it is possible that a portion of this 85Kr concentration was the result of flaring operations. Ground Monitoring Results Tables 9 through 12 list the results of all samples collected on the ground with the exception of two compressed air samples collected at Stations 19 and 20. The compressed air sample from Station 19 was lost in analysis. The sample from Station 20, collected between 0910 and 0940 hours on May 20, had a 85Kr concentration of 15 ± pCi/m3. Of the 16 molecular sieve samples collected, five showed concentrations of 3H above 1000 pCi/1 H20. The maximum 3H concentration was 4100 ± 310 pCi/1 H20 (14 ± 1.1 pCi/m3 of air) at Station 18, 1.4 km (0.9 mi) 77°. This is less than 0.02% of the Concentration Guide for continuous exposure for a suitable population sample in an uncontrolled area.12 Only one vegetation sample showed a 3H concentration that was above the estimated background of 1000 pCi/1 H20, and none of the soil samples exceeded the estimated background. A vegetation sample collected at Station 18 had a 3H concentration of 1200 pCi/1 H20. Since this sample was collected at the same location as the highest atmospheric moisture sample, it is possible that the slightly elevated 3H concentration was the result of flaring operations. Five surface water samples were collected at Stations 27 through 31 within 16 km (10 mi) of the flare stack. None of the five samples showed elevated levels of 3H. 13 ------- FLARING SURVEILLANCE PROCEDURES AND RESULTS JULY 25-26, 1973 July 25. 1973 The aircraft began tracking at 0705 hours. From the usual spiral descent and ascent, the plume was detected 1.8 km (1.1 mi) west of the flare stack at 0730 hours, between the ridge north of Leandro Canyon and Station 25. Mobile monitors were sent to Stations 8 and 24, and started atmospheric moisture sampling. A compressed air sample was also taken at Station 24. Water in- jection started at 0700 hours and ended at 1050 hours when the stored water was exhausted. In the air the plume was detected at 2350 m (7700 ft) over terrain of 2320 m (7600 ft) 4.8 km (3 mi) at 260° from the flare stack. A grab sample was collected in two halves on passes over Station 27 at 0746 and 0754 hours. The first pass was at 2260 m (7400 ft) and the second was at 2230 m (7300 ft). The ground elevation along this route is 2160 m (7100 ft). The heading of the plume was determined to be about 260° from the flare stack and a ground monitor was positioned at Station 25 where an atmospheric moisture sample was started at 0811 hours. At 0830 hours, the aircraft located the plume starting at the flare stack and continuing down Leandro and La Jara Canyons to Highway 17; then west along Vaqueros Canyon. Plume contact was maintained the entire length of this pass at an elevation of about 60 m (200 ft) above the surface. Mobile monitors were dispatched to Stations 11 and 13 to obtain atmospheric moisture samples. At 0839 hours, an aerial grab sample was collected at the junction of La Jara and Vaqueros Canyons, at 2070 m (6800 ft) about 60 m (200 ft) above the surface 8.0 km (5 mi) at 300° from the flare stack. A third grab sample was collected at 0931 hours 2010 m (6600 ft) in Vaqueros Canyon 8.0 km (5 mi) at 290° from the flare stack. This sample was collected about 30 m (100 ft) above the canyon floor of 2010 m (6500 ft). The aerial mission was concluded at this time. Mobile monitors collected vegetation and soil samples at all stations where atmospheric moisture samples were taken (Stations 8, 11, 13, 24, and 25). This terminated the surveillance for July 25. 14 ------- July 26, 1973 A spiral descent by the aircraft starting at 0730 hours, identified the plume top about 2260 m (7400 ft) between 260° and 290° from the flare stack. Prior to this time mobile monitors had been sent to Stations 8 and 13 to try to sample early morning drainage winds. Atmospheric moisture samp- ling was started at Station 13 at 0625 hours, and at Station 8 at 0717 hours. Based upon the aircraft information, other mobile monitors were sent to Stations 24 and 26 where they collected atmospheric moisture samples. By 0750 hours the wind speed had decreased to near zero moving slowly to the northwest. A pass over Station 25 at 2190 m (7200 ft) at 0757 hours, indicated a slight trace of plume material. An aerial grab sample was col- lected at 0817 hours at 2440 m (8000 ft) between Leandro Canyon (300°) and Station 25. Following a spiral descent around the flare stack a second grab sample was taken at 2320 m (7600 ft), 1.3 km (0.8 mi) from the flare stack between 270° and 300°. By 0851 hours the plume was identified at 2350 m (7700 ft) 330° from the flare stack about 2 km (1.2 mi) out. By 0908 hours the plume was still moving in the same direction and was detected over La Jara Canyon at 2290 m (7500 ft), 4.8 km (3 mi) from the flare stack. A grab sample was taken at 0913 hours between 6.4 km (4 mi) and 8.0 km (5 mi) at 2320 m (7600 ft) on a heading of 320°. Based upon the trajectory established by the aircraft, a mobile monitor was sent to Station 20 and began atmospheric moisture sampling at 0920 hours. Aerial tracking was terminated at 1000 hours with the last contact at 1.6 km (1 mi) to 3.2 km (2 mi) north of the flare stack. At that time (0940 hours) the Doppler radar showed the winds over the surface to be about 2 knots from 180°. Vegetation samples were collected at Stations 9, 17, 18, 19, 20, and 23. Soil samples were collected at Stations 9, 18, 19, 20, 23, and 26. The soil sample at Station 9 was a profile sample consisting of surface to 2.5 cm (1 in) 2.5 cm to 7.6 cm (3 in), and 7.6 cm to 15.2 cm (6 in). Surface water samples were collected at Stations 27, 28, 30, and 31. This terminated the surveillance for July 26. 15 ------- Results of Aerial Operations Tables 13 and 14 list the results of aerial operations for the July 25-26 flaring. Six atmospheric moisture samples were collected by the aircraft. Tritium concentrations were of the same magnitude as the May flaring surveil- lance with four samples above background and a maximum of 4000 ± 300 pCi/1 H20 in a sample collected 1.8 km (1.1 mi) from the flare stack on an azimuth of 260°. This concentration, expressed as 48 ± 3.6 pCi/m3 of air was 0.07% of the Concentration Guide for a suitable population sample in an uncontrolled area.12 Associated compressed air samples did not show ^5Kr concentrations above anticipated background. The compressed air samples were also analyzed for radioxenons. No concentrations of radioxenons were found above the detec- tion limit of 2.0 pCi/m3 of air. All samples with 3H concentrations above 1000 pCi/1 were collected during injection of water on July 25. Ground Monitoring Results Tables 15 through 19 list the analytical results of all samples collected by ground monitors. Ground level sampling of atmospheric moisture showed definite concentrations of 3H above background at Stations 8, 11, 13, 24, and 25. All of these Stations, with the exception of Station 13, were within 2 km (1.2 mi) of the flare stack in a sector from 220° to 341°. Station 13 was 8 km (5 mi) from the flare stack on an azimuth of 300°. The maximum concentration of 3H occurred at Station 11, 0.5 km (0.3 mi) at 341° from the flare stack. This concentration was 49,000 pCi/1 H20, which was equivalent to 300 pCi/m3 of air. This was about 0.4% of the Concentration Guide for a suitable population sample. All of the above samples were collected on July 25, 1973 during which time water was being in- jected into the flare. Vegetation and soil samples showed concentrations of H above background at Station 11. A vegetation sample collected on July 25 at Station 11 had a 3H concentration of 22,000 pCi/1 H20, and a soil sample collected at the same location had a 3H concentration of 5800 pCi/1 H20. Four surface water samples were also collected. None of the samples o showed elevated levels of 3H. 16 ------- POST-FLARING SAMPLE COLLECTION AND RESULTS NOVEMBER 6-8, 1973 Sampling Procedures Post-flaring environmental samples were collected from the Gasbuggy Project area on November 6, 7, and 8, 1973. Of the 26 soil and vegetation sampling locations used throughout the flaring period, vegetation and soil samples were collected at all stations except two. Only vegetation was collected at Station 17, and only soil was collected at Station 26. Shut-in of the test well was accomplished at 1235 hours on November 6; however, water containing H was steamed until November 7. A few of the more remote samples were collected on the morning of November 6, but were considered to be post- flaring samples. Only three of the five water sampling locations were sampled. No water was available at Bullsnake Pond and John Mills Lake (Stations 29 and 31). Results of Post-Flaring Sample Collection Tables 20, 21, and 22 list the analytical results of all samples collected after flaring was completed. Post-flaring vegetation sampling results showed levels of 3H above back- ground in all four compass quadrants surrounding the flare stack. Of the 25 stations where vegetation was collected, ten had concentrations of 3H greater than 1000 pCi/1 of H20. No obvious pattern existed in relation to distance and direction for those stations where elevated levels of 3H were found. The maxi- mum concentration of 3H was found in a vegetation sample at Station 20, 2 km (1.2 mi) 330°. This sample had a 3H concentration of 26,000 pCi/1 of H20. This value is about five times greater than the next highest vegetation sample (5500 pCi/1 H20) which was collected at Station 21, 8.2 km (5.0 mi) 75°. Of the 25 stations where soil samples were collected, only Station 10 0.5 km (0.3 mi) 102°, had a concentration of 3H above 1000 pCi/1 H20. This sample contained 1700 pCi/1 H20 of 3H. Three surface water samples were collected. None of these samples showed H concentrations above background. 17 ------- SUMMARY AND CONCLUSION During the production test conducted at the Project Gasbuggy site from May 15 to November 6, 1973, natural gas containing 85Kr and 3H was flared continuously. On several occasions tritiated water, which had been removed from the natural gas, was converted to steam and injected into the flaring plume. The flow rate at which the natural gas was flared varied as shown on Figure 3. Figure 3 also shows when steam containing 3H was injected into the flaring plume and when aerial and ground sampling was conducted by NERC-LV personnel. The primary radionuclides of concern were identified from previous surveillance programs for Project Gasbuggy to be 3H and 85Kr, of which a total of 48.93 Ci and 4.69 Ci, respectively, was released into the atmosphere during this production test.7 Aerial sampling detected concentrations of 3H above background levels in the plume on each mission flown during the periods May 19-21 and July 25-26. The concentrations of 85Kr in all air samples collected during flaring operations were considered to be at background levels (~17 pCi/m3), except for one sample collected on May 19 which had a 85Kr concentration of 21 ± 1.0 pCi/m3. This concentration is less than 0.02% of the Concentration Guide for a suitable population sample in an uncontrolled area.12 The highest concentration of H detected in aircraft samples was 48 ± 3.6 pCi/m3 of air in a sample collected on July 25 at an elevation of 2290 m (7500 ft), 1.8 km (2.8 mi) at 260° from the flare stack. This concentration is less than 0.07% of the Concentration Guide for continuous exposure to a suitable population sample in an uncontrolled area.12 Mobile monitors on the ground, who were positioned in the plume downwind of the stack by personnel in the aircraft, also collected atmospheric moisture samples containing 3H above estimated background during each sampling period in May and July. The highest 3H concentration in atmospheric moisture samples collected by mobile monitors on the ground was collected at Station 11, an unpopulated location, on July 25. This concentration, which was 300 pCi/m3 of air, is less than 0.4% of the Concentration Guide for a suitable population sample in an uncontrolled area.12 18 ------- Tritium concentrations above estimated background concentrations were found in some vegetation and soil collected during the July 25-26 surveillance operations and the November 6-8 post-flaring surveillance; no elevated 3H concentrations were detected in these sample types during the May 19-21 sur- veillance. No surface water samples showed concentrations of 3H above estimated background. The highest 3H concentration in vegetation (26,000 pCi/1 of H20) was measured in a sample collected at Station 20 on November 7, 2 km (1.2 mi) 333° from the flare stack. The highest 3H concentration in soil (1700 pCi/1 H20) was measured in a sample collected at Station 10 on November 7, 0.5 km (0.3 mi) 102° from the flare stack. From the highest concentrations of 3H which were measured in atmospheric moisture samples, it is concluded that any direct exposures to the off-site population were all below 0.4% of the Concentration Guide for this radio- nuclide. There are no concentration guides for 3H in vegetation or soil. However, all vegetation samples were native, uncultivated shrubs, which are not used for human consumption or known to be of consideration in the food chain of area residents. All concentrations of radionuclides detected should be considered as maximum since considerable effort was made to sample at times, places, and under atmospheric conditions when plume material was most likely to be on or near the surface at maximum concentrations. In addition, much of the sampling of atmospheric moisture was done when stored, tritiated water was being deliberately injected at higher than normal rates into the flare. References to exposures to a suitable population sample are more hypothetical than real, since all samples containing concentrations of 3H above estimated background were collected at unpopulated locations. 19 ------- REFERENCES 1. "Report of Off-Site Surveillance for Project Gasbuggy," SWRHL-99r. Southwestern Radiological Health Laboratory, U.S. Department of Health, Education and Welfare, Las Vegas, Nevada, February 1970. 2. "Environmental Surveillance for Project Gasbuggy Production Test Phase," SWRHL-lOOr. Southwestern Radiological Health Laboratory, U.S. Depart- ment of Health, Education and Welfare, Las Vegas, Nevada, June 1970. 3. "Project Gasbuggy Off-Site Radiological Safety Report, GB-2R, Phase I Program," SWRHL-105r. Southwestern Radiological Health Laboratory, U.S. Department of Health, Education, and Welfare, Las Vegas, Nevada, July 1970. 4. McBride, J. R. and D. Hill, "Off-Site Radiological Surveillance for Project Gasbuggy, June 1967 - July 1968." Radiological Health Data and Reports, Volume 10, No. 12, December 1969. Page 535. 5. "Results of Sampling Natural Gas Wells in the Vicinity of Project Gas- buggy," NERC-LV-539-9, National Environmental Research Center, U.S. Environmental Protection Agency, Las Vegas, Nevada, February 1973. 6. "Environmental Assessment, Project Gasbuggy 1973 Gas Production Test Rio Arriba County, New Mexico." U.S. Atomic Energy Commission, Nevada Operations Office, Office of Effects Evaluation, Las Vegas, Nevada, December 1972. 7. Correspondence over period May 29, 1973 to November 14, 1973, from Eddie W. Chew, Energy Resource Development, El Paso Natural Gas Company, El Paso, Texas, to Peter K. Fitzsimmons, Radiological Operations Division, U.S. Atomic Energy Commission, Las Vegas, Nevada. 8. Johns, F. B., "Southwestern Radiological Health Laboratory Handbook of Radiochemical Analytical Methods," SWRHL-11. Southwestern Radiological Health Laboratory, U.S. Department of Health, Education and Welfare, Las Vegas, Nevada, March 1970. 20 ------- 9. Stevenson, D. L. and F. B. Johns, "Separation Technique for the Deter- mination of 85Kr in the Environment," IAEA-SM-148/68. International Atomic Energy Agency, Vienna, 1971. 10. Andrews, V. E. and D. T. Wruble, "Noble Gas Surveillance Network, April 1972, through March 1973." U.S. National Environmental Research Center, Environmental Protection Agency, Las Vegas, Nevada. Presented at Noble Gases Symposium, Las Vegas, Nevada, September 1973. 11. Bernhardt, D. E., A. A.Moghissi, J. A. Cochran, "Atmospheric Concentrations of Fission Product Noble Gases," U.S. Environmental Protection Agency, National Environmental Research Center, Las Vegas, Nevada. Presented at Noble Gases Symposium, Las Vegas, Nevada, September 1973. 12. "Standards for Radiation Protection," U.S. Atomic Energy Commission Manual, Chapter 0524. U.S. Atomic Energy Commission, Washington, D.C., September 1973. 21 ------- S3 ft (B O (U C 09 CO B- OQ f O O O CO GASBUGGY ,« FLARE STACK ------- GASBUGGY FLARE STACK Figure 2. Close-in Gasbuggy Sampling Locations 23 ------- MAY M IS SEPTEMBER MB IT OCTOBER li t> 25 NOVEMBER 1973 Figure 3. Variation of Natural Gas Flow Rate During Flaring Period ------- Table 1. Quantities of Natural Gas Flared and Radioactivity Released During Project Gasbuggy Production Test May 15-November 6, 1973 Ul Volume of Seven-Day Natural Gas Flaring Period Flared Ending Midnight (MMCF) 5/21b'C 5/28 6/4 6/7C Totals for First Drawdown 6/13C 6/20 6/27 7/4 7/11 7/18 7/25d 8/1 8/8 8/15 8/22 8/29 25.692 24.050 16.957 4.713 71.412 2.880 .731 .867 1.298 1.284 1.257 1.105 1.054 1.034 .938 .937 .807 85Kr Released (Ci) 1.28 1.24 0.88 0.21 3.61 0.12 0.02 0.02 0.04 0.04 0.04 0.03 0.03 0.03 0.03 0.03 0.02 3H Released in Gas (Ci) 6.09 6.33 5.13 1.55 19.10 0.68 0.10 0.13 0.25 0.26 0.25 0.22 0.21 0.21 0.17 0.17 0.14 3H Released by Steam Total 3H Injection into Flare Released (Ci) (Dates) (Ci) 3.30 5/16,19,20,21 9.39 3.37 5/24,28 9.70 4.50 5/29,30, 6/1,3 9.63 2.61 6/5,6 4.16 13.78 32.88 0.68 0.10 0.13 0.25 0.26 0.25 0.90 7/25 1.12 0.21 0.21 0.17 0.17 0.14 ------- Table 1. Quantities of Natural Gas Flared and Radioactivity Released During Project Gasbuggy Production Test May 15-November 6, 1973 Seven-Day Flaring Period Ending Midnight 9/5 9/12 9/19 9/26 10/3 10/10 10/17 10/23° Totals for Steady Pressure Phase 10/29C 11/5 ll/7C>e Totals for Second Drawdown Totals for Production Test Volume of Natural Gas Flared (MMCF) .802 .809 .677 .574 .676 .654 .506 .393 19.283 9.230 7.214 .450 16.894 107.589 85Kr Released (Ci) 0.02 0.02 0.02 0.01 0.02 0.01 0.01 0.01 0.57 0.28 0.22 .01 0.51 4.69 3H Released in Gas (Ci) 0.14 0.14 0.11 0.10 0.11 0.10 0.08 0.06 3.63 2.36 1.82 .10 4.28 27.01 3H Released by Steam Total 3H Injection into Flare Released (Ci) (Dates) (Ci) 0.14 0.14 0.11 0.10 0.11 0.10 0.08 0.06 0.90 4.53 2.58 10/26,27,29 4.94 3.75 10/31,11/2,4,5 5.57 .91 11/6,7 1.01 7.24 11.52 21.92 48.93 ------- •a All data supplied by El Paso Natural Gas Company. Gas flow measurements were made by El Paso Natural Gas Company. Radioactivity measurements were made by Eberline Instrument Corporation. Ground and aerial surveillance was conducted on May 19, 20, and 21, 1973. •\ "Represents flow for periods not sevei 6.5 days, and 0.5 days respectively. Q Represents flow for periods not seven full days long: 6.5 days, 2.5 days, 6.5 days, 5.5 days, Ground and aerial surveillance was conducted on July 25 and 26, 1973. n Ground surveillance was conducted on November 6-8, 1973. ------- Table 2. Analytical Results of Pre-Flaring Water and Precipitation Samples Collected May 1973, for Project Gasbuggy Production Test Station No. 30 27 10 11 29 Azimuth and Distance (°) (km)3 151 10.5 (6.5) 269 1.3 (0.8) 102 0.5 (0.3) 341 0.5 (0.3) 71 4.8 (3.0) Date /Time Collected Source 5/3 1130 Pond 5/5 1145 Pond 5/6 0945 Snow 5/6 1000 Snow 5/6 1225 Pond 3H Concentration (PCi/l H£0) <240 <240 380± 250 410± 240 <240 a = Distance in miles is given in parentheses. 28 ------- Table 3. Analytical Results of Pre-Flaring Atmospheric Moisture Samples Collected May 1973, for Project Gasbuggy Production Test Azimuth and Station Distance No. (°) (km)a 8 305 1.8 (1.1) 10 102 0.5 (0.3) 11 341 0.5 (0.3) 7 43 5.0 (3.1) 9 53 2.1 (1.3) 13 300 8.0 (5.0) 15 280 17.9 (11.1) 3 46 16.1 (10.0) 5 356 10.9 (6.8) 12 241 10.1 (6.3) Date /Time on Date /Time off 5/5 5/5 5/5 5/5 5/5 5/5 5/6 5/6 5/6 5/6 5/6 5/6 5/6 5/6 5/7 5/7 5/7 5/7 5/7 5/7 1415 1500 1535 1620 1405 1450 1135 1235 1015 1115 1040 1140 1200 1300 1140 1240 1130 1240 0930 1030 Volume (m3) 6.43 7.79 5.01 8.10 9.27 5.04 9.89 8.64 7.87 8.47 Altitude Above MSL (m)a 2160 (7100) 2190 (7200) 2190 (7200) 2070 (6800) 2130 (7000) 1980 (6500) 2010 (6600) 2220 (7300) 2190 (7200) 2130 (7000) 3H Concentration (pCi/1 H20) (pCi/m3 air) 240± 240 <200 240± 240 590± 240 650± 240 550± 240 460± 240 480± 240 330± 240 <200 1.2± 1.2 <0.1 1.0± 1.0 2.5± 1.0 2.7± 1.0 2.3± 1.0 1.9± 1.0 2.1± 1.0 1.5± 1.1 <0.1 a = Altitude in feet above mean sea level (MSL) and distance in miles are given in parentheses. 29 ------- Table 4. Analytical Results of Pre-Flaring Compressed Air Samples Collected May 1973, for Project Gasbuggy Production Test Azimuth and Station Distance No. (°) (km)3 8 305 1.8 (1.1) 9 53 2.1 (1.3) Date/Time on Date/Time off 5/5 5/5 5/5 5/5 1050 1117 1235 1305 Altitude Volume Above MSL 85Kr Xe (m3) (m) (pCi/m3 air) (pCi/m3 air) 0.968 2160 17± <2.0 (7100) 1.0 Samples lost in analyses a = Altitude in feet above mean sea level (MSL) and distance in miles are given in parentheses. 30 ------- Table 5. Analytical Results of Pre-Flaring Vegetation Samples Collected May 1973, for Project Gasbuggy Production Test Station No. 8 9 10 11 6 7 13 14 15 1 2 3 4 5 Azimuth and Distance (°) (km)a 305 53 102 341 10 43 300 273 280 34 49 46 73 356 1.8 (1.1) 2.1 (1.3) 0.5 (0.3) 0.5 (0.3) 9.3 (5.8) 5.0 (3.1) 8.0 (5.0) 19.3 (12.0) 17.9 (11.1) 35.4 (22.0) 20.6 (12.8) 16.1 (10.0) 20.1 (12.5) 10.9 (6.8) Date /Time Collected 5/5 5/5 5/5 5/5 5/6 5/6 5/6 5/6 5/6 5/7 5/7 5/7 5/7 5/7 1115 1300 1530 1315 1320 1150 1115 1345 1230 0940 1130 1220 1040 1215 Mois ture Content (%)b 51 58 62 59 58 71 76 66 68 70 66 62 61 66 3H Concentration (pCi/1 H20) (pCi/kg veg.) <240 570± 250 1200± 260 530± 250 380± 260 500± 240 530± 260 440± 260 560± 260 570± 250 550± 260 490± 260 670± 250 720± 240 <120 330± 140 740± 160 310± 150 220± 150 360± 170 400± 200 290± 170 380± 180 400± 180 360± 170 300± 160 410+ 150 280+ 160 31 ------- Table 5. (continued) Analytical Results of Pre-Flaring Vegetation Samples Collected May 1973, for Project Gasbuggy Production Test Station No. 12 16 17 Azimuth and Moisture Distance Date/Time Content (°) (km)a Collected (%)b 241 10.1 5/7 0945 68 (6.3) 154 10.5 5/8 1000 66 (6.5) 77 0.8 5/8 1000 63 (0.5) % Concentration (pCi/1 H20) (pCi/kg veg.) 480± 240 670± 250 610± 250 330± 160 440± 160 380± 160 a = Distance in miles is given in parentheses. b = Based upon sample wet weight. All samples were native, uncultivated shrubs. 32 ------- Table 6. Analytical Results of Pre-Flaring Soil Samples Collected May 1973, for Project Gasbuggy Production Test Station No. 8 9 9C 9d 10 11 6 7 13 14 15 1 2 Azimuth and Distance (°) (km)a 305 53 53 53 102 341 10 43 300 273 280 34 49 1.8 (1.1) 2.1 (1.3) 2.1 (1.3) 2.1 (1.3) 0.5 (0.3) 0.5 (0.3) 9.3 (5.8) 5.0 (3.1) 8.0 (5.0) 19.3 (12.0) 17.9 (11.1) 35.4 (22.0) 20.6 (12.8) Date /Time Collected 5/5 5/5 5/5 5/5 5/5 5/5 5/6 5/6 5/6 5/6 5/6 5/7 5/7 1100 1250 1300 1245 1530 1330 1305 1210 1100 1330 1215 0915 1110 Moisture Content 20 8.6 15 16 6.1 9.1 14 12 13 10 21 11 14 3H Concentration (pCi/1 H20) (pCi/kg soil) 360+ 260 330± 240 310+ 260 <260 400+ 240 430± 240 <260 290± 240 340+ 240 500± 240 <240 <240 410± 240 71± 51 28± 21 50± 39 <42 24± 15 39± 22 <36 35± 29 43± 30 51+ 25 <50 <26 57± 34 33 ------- Table 6. (continued) Analytical Results of Pre-Flaring Soil Samples Collected May 1973, for Project Gasbuggy Production Test Station No. 3 4 5 12 16 Azimuth and Distance (°) (km)3 46 16.1 (10.0) 73 20.1 (12.5) 356 10.9 (6.8) 241 10.1 (6.3) 154 10.5 (6.5) Mois ture Date /Time Content Collected (%)b 5/7 1200 19 5/7 1100 11 5/7 1200 6 5/7 0930 11 5/8 1015 8.5 3H Concentration (pCi/1 H20) (pCi/kg soil) 330± 260 <240 360± 240 260± 240 <260 64± 50 <26 21± 14 28± 26 <22 a = Distance in miles is given in parentheses. b = Based upon sample wet weight. c = This sample was collected at a depth of 2.54 cm to 7.62 cm (1 to 3 in). d = This sample was collected at a depth of 7.62 cm to 15.2 cm (3 to 6 in). 34 ------- Table 7. Analytical Results of Aircraft Atmospheric Moisture Samples Collected May 1973, for Project Gasbuggy Production Test Azimuth and Distance (°) (km)a 330 95 110 110 75 330 145 1.9 (1.2) 3.5 (2.2) 1.6 (1.0) 1.6 (1-0) 8.0 (5.0) 2.3 (1.4) 3.3 (2.0) Date/Time Volume Collected (m3) 5/19 0905 0.605 5/19 1002 0.785 5/19 1423 0.786 5/20 0925 0.787 5/20 1040 0.490 5/21 0800 0.714 5/21 1025 0.792 Altitude Above MSL (m)3 2440 (8000) 2320 (7600) 2590 (8500) 2590 (8500) 2740 (9000) 2320 (7600) 3050 (10,000) 3H Concentration (pCi/1 H20y (pCi/m3 air) 2800± 340 1400± 270 690± 340 2500± 280 860± 290 1300± 270 910± 260 24± 2.9 11± 2.1 5.7± . 2.8 12± 2.7 9.5± 3.2 12± 2.4 6.3+ 1.8 a = Distance in miles and altitude in feet above mean sea level (MSL) are shown in parentheses. 35 ------- Table 8. Analytical Results of Aircraft Compressed Air Samples Collected May 1973, for Project Gasbuggy Production Test Azimuth and Distance (°) (km)3 330 95 110 110 75 330 145 1.9 (1.2) 3.5 (2.2) 1.6 (1.0) 1.6 (1.0) 8.0 (5.0) 2.3 (1.4) 3.2 (2.0) Date /Time Collected 5/19 0905 5/19 1002 5/19 1423 5/20 0925 5/20 1040 5/21 0800 5/21 1025 Volume (m3) 0.605 0.785 0.786 0.787 0.490 0.714 0.792 Altitude Above MSL (m) 2440 (8000) 2320 (7600) 2590 (8500) 2590 (8500) 2740 (9000) 2320 (7600) 3050 (10,000) 85Kr Concentration (pCi/m3 air) 21± 1.0 16± 1.1 17± 1.1 18± 1.1 16± 1.0 14± 1.0 12± 1.0 a = Altitude in feet above mean sea level (MSL) and distance in miles are given in parentheses. 36 ------- Table 9. Analytical Results of Water Samples Collected May 19731 for Project Gasbuggy Production Test Station No. 27 28 29 30 31 Azimuth and Distance (°) (km)a 269 1.2 (0.8) 40 5.2 (3.3) 71 4.8 (3.0) 151 10.4 (6.5) 47 16.1 (10.0) Date/Time Collected Source 5/20 0905 Pond 5/21 1315 Pond 5/21 1300 Pond 5/21 1135 Pond 5/21 0645 Pond 3H Concentration (pCi/1 H20) 350± 250 320± 250 440± 250 470± 250 330± 250 a = Distance in miles is given in parentheses. 37 ------- Table 10. Analytical Results of Atmospheric Moisture Samples Collected May 1973, on the Ground for Project Gasbuggy Production Test Azimuth and Station Distance No. (°) (km)a 18 19 11 20 8 18 19 21 9 11 20 8 11 77 110 341 333 305 77 110 75 53 341 .333 305 341 1.4 (0.9) 1.6 (1.0) 0.5 (0.3) 2.0 (1.3) 1.7 (1.1) 1.4 (0.9) 1.6 (1.0) 8.2 (5.1) 2.0 (1.3) 0.5 (0.3) 2.0 (1.3) 1.7 (1.1) 0.5 (0.3) Date/Time on Date/Time off 5/19 5/19 5/19 5/19 5/20 5/20 5/20 5/20 5/20 5/20 5/20 5/20 5/20 5/20 5/20 5/20 5/20 5/20 5/21 5/21 5/21 5/21 5/21 5/21 5/21 5/21 1445 1545 1445 1545 0900 1000 0905 1005 0920 1020 0940 1032 0942 1044 1020 1150 1045 1145 0715 0755 0715 0815 0725 0840 0800 0900 Volume (m3) 6.66 i 9.58 6.66 7.85 6.49 7.25 7.42 8.84 6.97 4.14 8.16 5.86 5.69 Altitude Above MSL 3H Concentration (m)a (pCi/1 H20) (pCi/m3 air) 2160 (7100) 2130 (7000) 2190 (7200) 2290 (7500) 2160 (7100) 2160 (7100) 2130 (7000) 2160 (7100) 2130 (7000) 2190 (7200) 2290 (7500) 2160 (7100) • 2190 (7200) 4100± 310 • iooo± 260 1500± 260 540± 240 570± 240 2900± 290 880± 240 370± 230 300± 240 510± 240 630± 240 320± 240 450± 250 14+ 1.1 3.3± 0.86 8.7± 1.5 3.0± 1.3 3.2± 1.3 15± 1.5 4.1± 1.1 1.8± 1.2 1.4± 1.1 3.1± 1.4 3.3± 1.2 1.8± 1.3 2.5+ 1.4 38 ------- Table 10. (continued) Analytical Results of Atmospheric Moisture Samples Collected May 1973, on the Ground for Project Gasbuggy Production Test Azimuth and Station Distance No. (•) (kn)a 18 77 1.4 (0.9) 22 31 1.6 (1.0) 23 126 3.5 (2.2) Date/Time on Volume Qate/Time off (m3) 5/21 5/21 5/21 5/21 5/21 5/21 0825 8.72 0925 0832 5.75 0924 1004 7.72 1105 Altitude Above MSL , v3 (m) 2160 (7100) 2130 (7000) 2230 (7300) 3H Concentration (pCi/1 HO) (pCi/m3 air) 810± 260 1100± 600 3201 230 4.3± 1.4 6.1% 3.3 1.2± 0.87 a - Altitude in feet above mean sea level (MSL) and distance in miles are given in parentheses. 39 ------- Table 11. Analytical Results of Vegetation Samples Collected May 1973, for Project Gasbuggy Production Test Azimuth and Moisture Station Distance Date/Time Content 3H Concentration No. (°) (km)a Collected (%)b (pCi/1 H2<3) (pCi/kg veg.) 18 19 8 9 11 18 19 20 21 17 22 23 a = b = 77 110 305 53 341 77 110 333 75 241 31 126 Distance in Based upon £ 1.4 (0.9) 1.6 (1.0) 1.7 (1.1) 2.0 (1.3) 0.5 (0.3) 1.4 (0.9) 1.6 (1.0) 2.0 (1.3) 8.2 (5.1) 10.0 (6.3) 1.6 (1.0) 3.5 (2.2) miles sample 5/19 5/19 5/20 5/20 5/20 5/20 5/20 5/20 5/20 5/21 5/21 5/21 is given wet weigh 1520 56 1500 56 1315 62 1105 63 0945 58 1010 66 1110 63 1000 72 1100 67 1240 69 0910 73 1030 60 in parentheses . it. All samples 880± 260 700± 240 500± 250 650+ 240 650± 250 1200± 260 59 0± 240 260± 250 740± 260 570± 250 590± 250 440± 250 490± 150 390± 130 310± 160 410± 150 370± 140 790± 170 370± 150 190± 180 500± 170 390± 170 430+ 180 260+ 150 were native, uncultivated shrubs. 40 ------- Table 12. Analytical Results of Soil Samples Collected May 1973, for Project Gasbuggy Production Test Station No. 18 19 8 9 11 18 19 20 21 22 23 Azimuth and Distance (°) (km)a '77 1.4 (1.9) 110 1.6 (1.0) 305 1.7 (1.1) 53 2.0 (1.3) 341 0.5 (0.3) 77 1.4 (1.9) 110 1.6 (1.0) 333 2.0 (1.3) 75 8.2 (5.1) 31 1.6 (1.0) 126 3.5 (2.2) Moisture Date/Time Content Collected (%)b 5/19 1500 1.2 5/19 1515 2.8 5/20 1325 4.3 5/20 1120 0.88 5/20 1005 2.0 5/20 1000 2.5 5/20 1110 5.8 5/20 1020 3.7 5/20 1100 0.92 5/21 0915 4.8 5/21 1030 1.7 3H Concentration (pCi/1 H20) (pCi/kg soil) 8501 260 580± 240 <230 430± 230 430± 230 770± 240 510± 240 470± 240 360± 230 460± 230 530+ 240 10± 3.1 16± 6.8 <9.9 3.8± 2.0 8.6± 4.6 19± 6.0 29± 14 17± 8.9 3.3± 2.1 22± 11 91± 4.1 a = Distance in miles is given in parentheses. b = Based upon sample wet weight. c = This sample was collected at a depth of 2.54 cm to 7.62 cm (1 to 3 in), d = This sample was collected at a depth of 7.62 cm to 15.2 cm (3 to 6 in), 41 ------- Table 13. Analytical Results of Aircraft Atmospheric Moisture Samples Collected July 1973, for Project Gasbuggy Production Test Azimuth and Distance (°) (km)3 260 300 290 260- 300 270- 300 320 1.8 (1.1) 8.0 (5.0) 8.0 (5.0) 1.8 (1.1) 1.3 (0.8) 8.0 (5.0) Date /Time Volume Collected (m3) 7/25 0746 0.798 7/25 0839 0.779 7/25 0931 0.781 7/26 0817 0.696 7/26 0846 0.851 7/26 0913 0.848 Altitude Above MSL / \SL (m) 2260 (7400) 2170 (6800) 2010 (6600) 2440 (8000) 2320 (7600) 2320 (7600) 3H Concentration (pCi/1 H20) (pCi/m3 air) 40001 300 1500± 270 2000± 270 990± 260 760± 240 760± 240 48± 3.6 15± 2.7 19± 2.5 13± 3.4 111 3.4 9.9i 3.1 a = Altitude in feet above mean sea level (MSL) and distance in miles is given in parentheses. 42 ------- Table 14. Analytical Results of Aircraft Compressed Air Samples Collected July 1973, for Project Gasbuggy Production Test Azimuth and Distance Date/Time Volume (°) (km) Collected (m3) 260 300 290 260- 300 270- 300 320 1.8 7/25 0746 0.798 (1.1) 8.0 7/25 0839 0.779 (5.0) 8.0 7/25 0931 0.781 (5.0) 1.8 7/26 0817 0.696 (1.1) 1.3 7/26 0846 0.851 (0.8) 8.0 7/26 0913 0.848 (5.0) Altitude Above MSL (m) 2260 (7400) 2170 (6800) 2010 (6600) 2440 (8000) 2320 (7600) 2320 (7600) 85Kr Concentration (pCi/m3 air) 13± 0.70 17± 1.4 13± 0.70 16± 1.0 13± 1.1 17± 0.70 a = Altitude in feet above mean sea level (MSL) and distance in miles are given in parentheses. 43 ------- Table 15. Analytical Results of Atmospheric Moisture Samples Collected July 1973, on the Ground for Project Gasbuggy Production Test Azimuth and Station Distance No. (°) (km)a 8 24 25 11 13 13 8 24 26 20 305 1.7 (1-1) 282 1.8 (1.1) 220 1.9 (1.2) 341 0.5 (0.3) 300 8.0 (5.0) 300 8.0 (5.0) 305 1.7 (1-1) 282 1.8 (1.1) 285 3.5 (2.2) 333 2.0 (1.6) Date/Time on Date/Time off 7/25 7/25 7/25 7/25 7/25 7/25 7/25 7/25 7/25 7/25 7/26 7/26 7/26 7/26 7/26 7/26 7/26 7/26 7/26 7/26 0736 0841 0740 0840 0811 0911 0855 0940 0902 1006 0625 0725 0717 0817 0809 0909 0815 0915 0920 1020 Altitude Volume Above MSL (m3) (m)a 6.86 2160 (7100) 7.22 2160 (7100) 7.45 2160 (7100) 6.23 2190 (7200) 7.08 1980 (6500) 6.15 1980 (6500) 7.87 2160 (7100) 8.87 2160 (7100) 9.38 2260 (7400) 9.24 2290 (7500) 3H Concentration (pCi/1 H20) (pCi/m3 air) 6900± 330 3900+ 280 46001 290 49,000± 630 1400± 250 <230 260+ 230 270± 230 <250 400± 230 33± 1.6 21± 1.5 26± 1.7 300± 3.9 8.8± 1.6 <1.7 1.8± 1.6 2.0± 1.7 <1.8 2.7± 1.5 a = Altitude in feet above mean sea level (MSL) and distance in miles is given in parentheses. 44 ------- Table 16. Analytical Results of Water Samples Collected July 1973, for Project Gasbuggy Production Test Station No. 30 27 28 31 Azimuth and Distance (°) (km)a 154 10.4 (6.5) 269 1.2 (0.8) 40 5.2 (3.3) 47 16.1 (10.0) Date /Time Collected 7/25 1230 7/26 0700 7/26 0800 7/26 0700 Source Pond Pond Pond Pond 3H Concentration (pCi/1 H20) 410± 230 450± 230 <240 400± 230 a = Distance in miles is given in parentheses. 45 ------- Table 17. Analytical Results of Vegetation Samples Collected July 1973, for Project Gasbuggy Production Test Station No. 8 11 13 24 25 9 17 18 19 20 23 Azimuth and Distance (°) (km)3 305 341 300 282 220 53 77 77 110 333 126 1.7 (1.1) 0.5 (0.3) 8.0 (5.0) 1.8 (1.1) 1.9 (1.2) 2.0 (1.3) 0.8 (0.5) 1.4 (0.9) 1.6 (1.0) 2.0 (1.3) . 3.5 (2.2) Date /Time Collected 7/25 7/25 7/25 7/25 7/25 7/26 7/26 7/26 7/26 7/26 7/26 1015 1000 1030 1010 0945 1120 0715 1100 0830 0945 1005 Moisture Content (%)b 58 60 58 66 55 56 57 63 66 52 52 3H Concentration (pCi/1 H20) (pCi/kg veg.) 920± 240 22,000± 460 480± 250 390± 240 680± 240 660± 240 760± 260 480± 250 360± 250 440± 240 530± 240 530± ' 140 13,000± 280 280± 150 260± 160 370± 160 370± 130 430± 150 300± 160 240± 170 230± 120 280± 120 a = Distance in miles is given in parentheses. b = Based upon sample wet weight. All samples were native, uncultivated shrubs. 46 ------- Table 18. Analytical Results of Soil Samples Collected July 1973, for Project Gasbuggy Production Test Station No. 8 11 13 24 25 9 9b 9C 18 19 20 23 26 Azimuth and Distance (°) (km) a 305 341 300 282 220 53 53 53 77 110 333 126 285 1.7 (1.1) 0.5 (0.3) 8.0 (5.0) 1.8 (1.1) 1.9 (1.2) 2.0 (1.3) 2.0 (1.3) 19.8 (12.5) 1.4 (0.9) 1.6 (1.0) 2.0 (1.3) 3.5 (2.2) 3.5 (2.2) Moisture Date/Time Content Collected (%)b 7/25 7/25 7/25 7/25 7/25 7/26 7/26 7/26 7/26 7/26 7/26 7/26 7/26 1010 1.6 0945 1.2 1045 1.7 1020 1.2 1000 1.8 0745 1.3 1100 4.8 1120 5.7 1105 1.3 0830 1.2 1000 1.2 1015 1.7 0830 1.5 3H Concentration (pCi/1 H20) (pCi/kg soil) 540± 240 5800± 310 370± 230 910± 240 520± 240 270± 230 300± 230 230± 230 380± 230 350± 230 370± 230 310± 230 380± 230 8.6± 3.8 70± 3.7 6.3± 3.9 11 ± 2.9 9.4± 4.3 3.5± 3.0 14± 11 13± 13 4.9± 3.0 4.2± 2.8 4.4+ 2.8 5.3± 3.9 5.7± 3.5 a = Distance in miles is given in parentheses. b = Based upon sample wet weight. All samples were native, uncultivated shrubs, c = This sample was collected at a depth of 2.54 cm to 7.62 cm (1 to 3 in). d = This sample was collected at a depth of 7.52 cm to 15.2 cm (3 to 6 in). 47 ------- Table 19. Analytical Results of Compressed Air Samples Collected July 1973, on the Ground for Project Gasbuggy Production Test Azimuth and Station Distance No. (°) (km)3 24 282 1.8 (1.1) 24 282 1.8 (1.1) Date/Time on Volume Date/Time off (m3) 7/25 7/25 7/26 7/26 0739 0.944 0805 0755 0.933 0826 85Kr (pCi/m3 air) 15± 0.7 14± 0.6 Xe (pCi/m3 air) <2.0 <2.0 a = Distance in miles is given in parentheses. 48 ------- Table 20. Analytical Results of Post-Flaring Water Samples Collected November 1973, for Project Gasbuggy Production Test Azimuth and Station Distance Date/Time No. (°) (km)a Collected Source 27 269 1.2 11/6 1600 Pond (0.8) 28 40 5.2 11/6 1415 Pond (3.3) 29 71 4.8 11/7 1245 Pond (3.0) ^H Concentration (pCi/1 H20) 380± 240 <240 <240 a = Distance in miles is given in parentheses, 49 ------- Table 21. Analytical Results of Post-Flaring Vegetation Samples Collected November 1973, for Project Gasbuggy Production Test Station No. 1 2 3 4 5 12 14 15 25 7 10 16 17 20 Azimuth and Distance C) (km)3 34 49 46 73 356 241 273 280 220 43 102 154 77 333 35.4 (22.0) 20.4 (12.8) 16.1 (10.0) 19.8 (12.5) 10.8 (6.8) 10.0 (6.3) 19.3 (12.0) 17.7 (11.1) 1.9 (1.2) 4.9 (3.1) 0.5 (0.3) 10.4 (6.5) 0.8 (0.5) 2.0 (1.3) Date/Time Collected 11/6 11/6 11/6 11/6 11/6 11/6 11/6 11/6 11/6 11/7 11/7 11/7 11/7 11/7 1115 1230 1000 1330 1145 1015 0915 1100 1545 1000 0845 1330 1600 1440 Moisture Content 58 48 43 51 38 38 41 33 42 38 20 48 41 49 3H Concentration (pCi/1 H20) (pCi/kg veg.) 680± 270 530± 260 1400± 390 860± 270 320± 260 3600± 430 330± 260 1400± 390 570± 260 910± 260 1400± 270 400* 260 2100± 280 26,000± 720 , 390± . 160 260± 120 600± 170 440± 140 120± 99 14001 160 140+ 110 4701 130 2401 110 3501 99 280+ 54 1901 120 8501 110 12,400+ 350 50 ------- Table 21. (continued) Analytical Results of Post-Flaring Vegetation Samples Collected November 1973, for Project Gasbuggy Production Test Station No. 21 23 6 8 9 11 13 18 23 22 24 Axiauth and Distance C) (tan)a 75 8.2 (5.1) 126 3.5 (2.2) 10 9.2 (5.8) 305 1.7 (1.1) 50 2.7 (1.3) 341 0.5 (0.3) 300 8.0 (5.0) 77 1.4 (0.9) 110 1.6 (1.0) 31 1.6 U.O) 282 1.8 (1.1) Moisture Date/Time Content Collected (Z)b 11/7 1045 27 11/7 1200 56 11/8 1000 44 11/8 1100 41 11/8 0915 25 . 11/8 1130 32 11/8 0845 50 11/8 1045 44 11/8 1130 36 11/8 1215 24 11/8 1015 .44 3H Concentration (pCi/1 H20) (pCi/kg veg.) 55001 330 1200± 380 740± 370 440± 260 700± 270 <260 1700± 390 600± 260 <260 18001 400 4001 260 1500± 890 . 6901 220 330+ 160 1801 110 1801 68 <830 8301 190 2601 110 <:94 4401 95 180+ 110 a = Distance in miles is given in parentheses. b = Based upon sample wet weight. All samples were native, uncultivated shrubs. 51 ------- Table 22. Analytical Results of Post-Flaring Soil Samples Collected November 1973, for Project Gasbuggy Production Test Station No. 1 2 3 4 5 12 14 15 25 26 7 10 16 Azimuth and Distance (°) (km)a 34 49 46 73 356 241 273 280 220 285 43 102 154 35.4 (22.0) 20.4 (12.8) 16.1 (10.0) 19.8 (12.5) 10.8 (6.8) 10.0 (6.3) 19.3 (12.0) 17.7 (11.1) 1.9 (1.2) 3.5 (2.2) 4.9 (3.1) 0.5 (0.3) 10.4 (6.5) Moisture Date/Time Content Collected (%)*> 11/6 1130 2.1 11/6 1245 4.4 11/6 1020 4.1 11/6 1400 3.2 11/6 1145 1.3 11/6 1015 2.2 11/6 0915 1.2 11/6 1100 2.0 11/6 1545 4.2 11/6 1515 3.1 11/7 1000 1.6 11/7 0945 5.8 11/7 1330 3.0 3H Concentration (pCi/1 H20) (pCi/kg soil) <240 280± 240 <240 340± 240 <230 260± 240 <230 240± 240 <240 260± 240 390± 240 1700± 260 350± 240 <5.1 12± 11 <9.8 11± 7.7 <3.0 5.9± 5.3 <2.8 4.8± 4.8 <11 8.4± 7.4 6.1± 1.6 99± 15 11± 7.2 52 ------- Table 22. (continued) Analytical Results of Post-Flaring Soil Samples Collected November 1973, for Project Gasbuggy Production Test Azimuth and Station Distance No. («) (km)a 20 21 23 6 8 9 9C 9d 11 13 18 19 22 24 a = b - c = d = 333 75 126 10 305 53 53 53 341 300 77 110 31 282 Distance in Based upon This sample This sample 2.0 (1.3) 8.2 (5.1) 3.5 (2.2) 9.2 (5.8) 1.7 (1.1) 2.0 (1.3) 2.0 (1.3) 2.0 (1.3) 0.5 (0.3) 8.0 (5.0) 1.4 (0.9) 1.6 (1.0) 1.6 (1.0) 1.8 (1.1) miles sample Moisture Date/Time Content Collected (%)b 11/7 11/7 11/7 11/8 11/8 11/8 11/8 11/8 11/8 11/8 11/8 11/8 11/8 11/8 is given 1500 1100 1200 0945 1100 0915' 0915 0915 1130 0915 1100 1145 1200 1015 4. 1. 1. 1. 2. 2. 5. 9. 2. 5. 1. 1. 2. 1. 0 9 9 6 8 0 4 5 3 3 9 6 4 8 3H Concentration (pCl/1 H20) (pCi/kg soil) 250± 240 350± 240 <240 280± 240- 470± 240 310± 240 510± 240 370± 240 <240 <240 530± 250 260± 240 <240 340± 240 1.0± 1.0 6.6± 4.6 <4.6 4.5± 3.8 13± 6.7 6.1± 4.8 27± 13 35± 23 <5.5 <13 10± 4.8 4.1± 3.8 <5.8 6.2± 4.3 in parentheses. wet weight. was collected was collected at a depth at a depth of of 2.54 7.62 cm to 7.62 cm cm to 15.2 cm (1 to 3 in). (3 to 6 in). 53 ------- DISTRIBUTION 1-15 National Environmental Research Center, Las Vegas, NV (15) 16 - 20 Edward Fleming, Jr., AEG/DAT, Wash., B.C. (5) 21 - 22 Martin B. Biles, AEC/DOS, Wash., D. C. (2) 23 - 24 Maj. Gen. Ernest Graves, Jr., AGM/MA, Wash., B.C. (2) 25 - 26 James L. Liverman, AEC/AGMBERSP, Wash., D.C. (2) 27 Mahlon E. Gates, Manager, AEC/NV, Las Vegas, NV 28 Robert H. Thalgott, AEC/NV, Las Vegas, NV 29 - 49 Robert R. Loux, AEC/NV, Las Vegas, NV (20) 50 Paul J. Mudra, AEC/NV, Las Vegas, NV 51 - 53 Bennie G. DiBona, AEC/NV, Las Vegas, NV (3) 54 David G. Jackson, AEC/NV, Las Vegas, NV 55 - 57 Technical Library, AEC/NV, Las Vegas, NV (3) 58 Frank E. Abbott, USAEC, Golden, CO 59 Harold F. Mueller, ARL/NOAA, AEC/NV, Las Vegas, NV 60 Gilbert J. Ferber, ARL/NOAA, Silver Spring, MD 61 Albert C. Trakowski, Acting Assistant Administrator for Research & Development, EPA, Wash., D.C. 62 William D. Rowe, Deputy Assistant Administrator for Radiation Programs, EPA, Wash., D.C. 63 William A. Mills, Dir., Div. of Criteria & Standards, ORP, EPA, Wash., D.C. 64 Ernest D. Harvard, Acting Director, Division of Technology Assessment, ORP, EPA, Wash., D.C. 65 Bernd Kahn, Chief, Radiochemistry & Nuclear Engineering, NERC, EPA, Cincinnati, OH 66 - 67 Charles L. Weaver, Director, Field Operations Division, ORP, EPA, Wash., D. C. (2) 68 Gordon Everett, Director, Office of Technical Analysis, EPA, Wash., D.C. 69 Kurt L. Feldmann, Managing Editor, Radiation Data & Reports, ORP, EPA Wash., D.C. 70 Regional Administrator, EPA, Region IX, San Francisco, CA 71 Regional Radiation Representative, EPA, Region IX, San Francisco, CA 72 Eastern Environmental Radiation Facility, EPA, Montgomery, AL 73 Library, EPA, Wash., D.C. 74 Kenneth M. Oswald, LLL, Mercury, NV ------- DISTRIBUTION (continued) 75 James E. Carothers, LLL, Livermore, CA 76 Alfred Holzer, LLL, Livermore, CA 77 Wayne R. Woodruff, LLL, Livermore, CA 78 Charles I. Browne, LASL, Los Alamos, NM 79 Jerome E. Dummer, LASL, Los Alamos, NM 80 Arden E. Bicker, REECo, Mercury, NV 81 Savino W. Cavender, REECo, Mercury, NV 82 Carter D. Broyles, Sandia Laboratories, Albuquerque, NM 83 George Tucker, Sandia Laboratories, Albuquerque, NM 84 Robert H. Wilson, University of Rochester, Rochester, NY 85 Richard S. Davidson, Battelle Memorial Institute, Columbus, OH 86 J. P. Corley, Battelle Memorial Institute, Richland, WA 87 - 91 Philip L. Randolph, EPNG, El Paso, TX (5) 92 William S. Twenhofel, USGS, Denver, CO 93 Alfred E. Doles, EIC, Santa Fe, NM 94 - 95 Charles H. Atkinson, USBM, Bartlesville, OK (2) 96 Miles Reynolds, Austral Oil Co., Houston, TX 97 Gerald R. Luetkehans, CER, Las Vegas, NV 98 Milford R. Lee, Conoco, Houston, TX 99 Robert L. Mann, Conoco, Casper, WY 100 John M. Ward, President, Desert Research Institute, University of Nevada Reno, NV 101 Charles Barton, ORNL, Oak Ridge, TN 102- 103 Technical Information Center, Oak Ridge, TN (for public availability) (2) ------- |