COMMUNITY WATER SUPPLY SURVEY:
     SAMPLING AND ANALYSIS FOR
    PURGEABLE ORGANICS AND TOTAL
            ORGANIC CARBON
    H.J. BRASS AND M.J. WEISNER
               USEPA
  TECHNICAL SUPPORT DIVISION, ODW
          CINCINNATI, OHIO
                s>
           B.A. KlNGSLEY
         SRI INTERNATIONAL
        CHEMISTRY LABORATORY
       MENLO PARK, CALIFORNIA
PRESENTED AT THE AWWA ANNUAL MEETING,
 WATER QUALITY DIVISION, JUNE 9, 1981

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  THE CWSS CONTAINS DATA FROM 1189
SAMPLES REPRESENTING 452 UTILITIES.

INCLUDED ARE:
o  325 SAMPLES FROM 106 SURFACE
     HATER SUPPLIES
o  801 SAMPLES FROM 330 GROUND
     WATER SUPPLIES
o  63 SAMPLES FROM 16 SUPPLIES
     USING COMBINED SURFACE AND
     GROUND WATERS

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 SUPPLIES SURVEYED AND SAMPLES COLLECTED
1
2
3
H
5
6
7
SIZE CATEGORIES
(PERSONS SERVED)
25-99
100
500
1,000
2,500
5,000
10,000
- M99
-999
-2,499
- 4,999
- 9,999
- 99,999
NUMBER
SUPPLIES
57
120
63
71
37
38
63
NUMBER
SAMPLES
108
226
122
209
106
109
309
SAMPLES REQUESTED
PER CATEGORY '•
RAW AND FINISHED
RAW AND FINISHED
RAW AND FINISHED
RAW, FINISHED, AND
1 DISTRIBUTION
RAW, FINISHED, AND
1 DISTRIBUTION
RAW, FINISHED, AND
1 DISTRIBUTION
RAW, FINISHED, AND
                                     3 DISTRIBUTION
TOTAL       152         1189

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PURGEABLE ORGANIC COMPOUNDS ANALYZED
  INCLUDED:

TR1HALOMETHANES
CHLOROFORM              DIBROMKHLOROMETHANE
BROMODICHLOROMETHANE    BROMOFORM

ALL TERMINAL SAMPLES ANALYZED-  REDUCED
SAMPLES ANALYZED IF TTHM IN TERMINAL
SAMPLE > 5 UG/L-

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PURGEABLE ORGANICS ANALYSIS INCLUDED:

OTHER SPECIFIC COMPOUNDS
CARBON TETRACHLORIDE    Ll.l-TRICHLOROETHANE
CHLOROBENZENE           TRICHLOROETHYLENE
1,2-DICHLQRQETHANE      BENZENE
Ł15. * TTWIS-1,2-        TOLUENE
  DICHLOROETHYLENE      XYLENES (ALL ISOMERS)
TETRACHLOROETHYLBIE

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  TOTAL ORGANIC CARBON
ANALYSES ALSO PERFORMED

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 CAUTION IN DATA INTERPRETATION

D  SAMPLES WERE 1-2 YEARS OLD PRIOR
   TO ANALYSIS.  LOW  MOLECULAR
   WEIGHT AROMATICS AND  IN  SOME
   CASES UNSATURATED  HALKARBONS
   MAY HAVE DEGRADED.
   -  FREQUENCIES OF  OCCURRENCE AND
      CONCENTRATIONS  FOR AFFECTED
      COMPOUNDS REGARDED As MINIMUM
      VALUES*

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 CAUTION IN DATA INTERPRETATION

o  SAMPLES COLLECTED A SINGLE TIME
   MAY NOT BE REPRESENTATIVE  OF
   OVERALL HATER QUALITY.

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PURGEABLE COMPOUNDS ANALYZED BY
        PURGE AND TRAP
       GAS CHROMATOGRAPHY
QUANTIFICATION LIMIT     0-5 UG/L

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iU




I
ut
ui
K
 10
 I

15
20
    25



TIME (min)
 I

30
35
 I

40

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l/>
UJ
at
2


o

                                                       X
                                                       a
i
5
                i
                to
 I

15
20     26

TIME (mini
30 40
 i
45
60

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    TOTAL ORGANIC CARBON MEASURED
            USING DOHRMANN
            DC-54 ANALYZER


QUANTIFICATION LIMIT      100-200 UG/L

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SEPARATE EVALUATION OF INFORMATION
o  TRIHALCMETHANES
o  OTHER SPECIFIC ORGANIC CHEMICALS
o  TOTAL ORGANIC CARBON

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TRIHALOMETHANES

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TRIHALOMETHANE INFORMATION NOW
AVAILABLE FOR THE FIRST TIME
FOR A LARGE NUMBER OF SUPPLIES
IN SMALLER POPULATION SIZE
CATEGORIES (25-100,000 PERSONS).

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DATA EVALUATED ACCORDING TO SUPPLY

o  RAW HATER SAMPLES NOT INCLUDED-
o  VALUES FOR FINISHED AND DISTRIBUTION
   SAMPLES AVERAGED TO YIELD A SINGLE
   THM VALUE FOR EACH SUPPLY.

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  CHLOROFORM PREDOMINATED  IN
      SURFACE WATERS;
BROMINATED TWs PREDOMINATED
      IN GROUND WATERS

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REQUENCIES OF OCCURRENCE  GREATER
  IN SURFACE YS GROUND WATER
SUPPLIES, EXCEPT FOR BROMOFORM
WHERE REQUENCIES WERE GREATER
       IN GROUND WATERS

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                     COMMUNITY WATER SUPPLY SURVEY
                          TRIHALCMETHANE DATA
                         SURFACE WATER SUPPLIES
    COMPOUND
CHLOROFORM
BROMODICHLORO-
  METHANE
DIBROMOCHLORO-
  METHANE
BROMOFORM
TOTAL TRIHALO-
  METHANE
POSITIVES
PER
SUPPLIES
102/105
99/105
70/105
W105
RANGE
<0.5-700
<0.5-62
<0.5-<6
<1.0-5.7
POSITIVES
MEAN MEDIA)
90
12
5.0
2.1
61
8-2
3.2
1.3
                           CONCENTRATION, UG/L
                                        ALL VALUES
                                       ŁAN   MEDI
                                        87      60
                                         12
                  6.8
                                                 1.5
102/105    <0.5-720    110
70
100     66

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                     COMMUNITY WATER SUPPLY SURVEY
                          TRIHALOMETHANE DATA
                         GROUND WATER SUPPLIES
    COMPOUND
CHLOROFORM
BROMODICHLORO-
  METHANE
DIBROMOCHLORO-
  METHANE
BROMOFORM
TOTAL TRIHALO-
POSITIVES
   PER
SUPPLIES
 107/315
                 CONCENTRATION,  UG/L
             POSITIVES        ALL VALUES
 RANGE     MEAN   MEDIAN     MEAN   MEDIAN
<0-5-220    8-9     3-0       3.0    <0-5
 10V315    <0.5-51     5.8
                    3.5
 107/315    <0.5-32     6.6     4.1
  81/315    <1.0-110    11      3-0
                  132/315    <1.0-280    24
                                12
1.9
2.2
2-8
9.9
<0.5
<0-5
<1.0
<1.0

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       THM CONCENTRATIONS HIGHER IN
          SURFACE AS OPPOSED TO
          GROUND WATER SUPPLIES

o  TTHM MEAN CONCENTRATIONS FOR POSITIVES
   SURFACE WATERS          110 UG/L
   GROUND WATERS            24 UG/L

o  TTHM MEDIAN CONCENTRATIONS FOR ALL SUPPLIES
   SURFACE WATERS           65 UG/L
   GROUND WATERS         < LO UG/L

o  MAXIMUM TTHM CONCENTRATIONS
   SURFACE WATERS          720 UG/L
   GROUND WATERS           210 UG/L

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 COMMUNITY WATER SUPPLY SURVEY
TTHM CONCENTRATIONS RELATED TO
   POPULATION SIZE CATEGORY
     SURFACE WATER SOURCES
POPULATION
 CATEGORY
NUMBE^POSITIVES
NUMBER SUPPLIES
                        CONCENTRATION. UG/L
MEAN    MEDIAN
JEAN
                                           YAU)ES
                                             fcDIAN
All
1
2
3
1
5
6
7
102/105
1/1
17/18
11/12
21/21
M/W
13/W
25/25
110
15
130
170
81
130
86
81
70
15
61
86
91
110
66
59
100
15
120
160
81
130
80
81
66
15
51
30
91
110
61
59

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                       COMMUNITY  WATER  SUPPLY SURVEY
                      TTHM CONCENTRATIONS  RELATED TO
                         POPULATION SIZE CATEGORY
                           GROUND WATER SOURCES
POPULATION
 CATEGORY
   ALL
    1
    2
    3

    5
    6
    7
NUMBER SUPPLIES

    132/315
      7/51
     26/95
     22/47
     28/52
     13/18
     1V23
     22/29
21
19
W
25
29
29
20
29
CONCENTRATION
VES
MEDIAN
12
5.5
8.8
13
13
27
17
12
, UG/L
ALL
MEAN
9.9
2-6
3.8
12
15
21
12
22

VALUES
MEDIAN
< 1
< 1
< 1
< 1
< 1
10
2.7
3-5

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SUPPLIES EXCEEDING MCL FOR TTHMs

 (BASED ON NON-REDUCED SAMPLES)
SURFACE WATERS        39 PERCENT
                     (41 OF 105)
GROUND HATERS          1 PERCENT
                      <<1 OF 315)

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   TTHM CONCENTRATIONS IN
   REDUCED SAMPLES WERE
 GENERALLY 50-65 PERCENT
OF TERMINAL CONCENTRATIONS

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OTHER SPECIFIC ORGANIC
      CHEMICALS

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OTHER SPECIFIC ORGANIC CHEMICALS (SOCs)

 INFORMATION AVAILABLE FOR LARGE NUMBER
   OF SUPPLIES IN SMALLER POPULATION
SIZE CATEGORIES (25 - 100,000 PERSONS).

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o  DATA EVALUATED ACCORDING TO SUPPLY

   -  RAW, FINISHED, AND DISTRIBUTED WATERS
        CONSIDERED.
   -  SAMPLE WITHIN A SUPPLY HAVING THE
        HIGHEST CONCENTRATION OF AN
        INDIVIDUAL COMPOUND USED TO DEVELOP
        STATISTICAL DATA.

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   FOR HALOCARBONS, FREQUENCIES OF
OCCURRENCE AND HIGHEST CONCENTRATIONS
    WERE IN GROUND WATER SUPPLIES.

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FREQUENCIES OF OCCURRENCE OF AROKAT1C
     COMPOUNDS SLIGHTLY HIGHER IN
        SURFACE AS OPPOSED TO
        GROUND WATER SOURCES.

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             PERCENT OCCURRENCE AND MAXIMUM
                     CONCENTRATIONS
                       AROMATICS

                           PERCENT                MAXIMUM
COMPOUND                  OCCURRENCE          CONCENTRATION, UG/L
                      GROUND    SURFACE       GROUND    SURFACE
BENZENE                 1.6       1.0            
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                     COMMUNITY WATER SUPPLY SURVEY
                         ORGANIC CHEMICAL DATA
                         SURFACE WATER SUPPLIES
                                                 CONCENTRATION, UG/L
        COMPOUND
CARBON TETRACHLORIDE
CHLOROBENZENE
1,2-DICHLOROETHANE
CIS + TRANS-L2-
  DIQCORO^HYLENE
TETRACHLOROETHYLENE
1,1,1-TRICHLOROETHANE
TRICHLOROETHYLENE
BENZENE
TOLUENE
XYLENES
POSITIVES
PER
SUPPLIES
3/106
0/106
0/106
0/106
3/106
3/106
0/106
1/100
3/100
7/100
RANGE
<0.5 -
-
-

<0.5-
< 0-5 -
V
< 0.5 -
< 0.5 -
< 0-5-

2.2



3.0
7.0

0-64
6-1
24
POSITIVE
MEAN
1.3
-
-
-
1.5
2-8
-
0.64
2-5
4.3
POSITIVE
MEDIAN
1.2
-
-
-
0.92
0.88
-
0.64
0.85
0-93

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        COMPOUND
CARBON TETRACHLORIDE
CHLOROBENZENE
1,2-DICHLOROETHANE
CIS + TRANS-L2-
  DICHOTEFHYLENE
TETRACHLOROETHYLENE
1,U-TRICHLOROETHANE
TRICHLOROETHYLENE
BENZENE
TOLUENE
XYLENES
COffUNm WATER
SUPPLY SURVEY


ORGANIC CHEMICAL DATA
GROUND WATER SUPPLIES
POSITIVES
PER
SUPPLIES
6/330
1/330
4/329
8/330
18/330
: 15/330
14/330
5/307
2/307
8/307
RANGE
< 0.5 - 2.8
< 0.5 - 1.3
< 0.5 - 1.8
< 0-5 - 82
< 0-5 - 30
< 0.5 - 650
< 0.5 - 210
< 0.5 - 44
< 0-5 - 0.62
< 0.5 - 4.2
CONCENTRATION, UG/L
POSITIVE POSITIVE
MEAN MEDIAN
1,9
1.3
1.3
15
3.4
47
30
9.7
0.56
1.6
1.8
1.3
1-2
3.4
1.9
1.3
1.3
1.4
0.56
0.91

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 DATA FOR CHEMICALS OTHER THAN TWs
 EVALUATED ON TOE BASIS OF AT LEAST
ONE COMPOUND PER SUPPLY. STATISTICS
 PROVIDED BASED ON WATER SOURCE AND
     POPULATION SIZE CATEGORY.

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TOTAL
SIZE CATEGORY 7
SIZE CATEGORY 6
SIZE CATEGORY 5
SIZE CATEGORY 4
SIZE CATEGORY 3
SIZE CATEGORY 2
SIZE CATEGORY 1
                     COMMUNITY WATER SUPPLY SURVEY
                      SUPPLIES SHOWING OCCURRENCES
                        OF ONE ORGANIC CHEMICAL*
SURFACE WATER
M/106
7/25
1/M
I/M
3/21
2/12
0/19
0/1
(PERCENT)
(13.2)
(28.0)
(7.1)
(7.1)
(14.3)
(16.7)
(0)
(0)
GROUND WATER
   50/330
   13/29
    2/23
    V18
   1V53
    3/51
    9/100
    5/56
A  BASED ON THE PRESENCE OF AT LEAST ONE COMPOUND
   OTHER THAN THKs AND TOC-
(PERCENT)
  (15.2)
  (8.7)
  (22-2)
  (25.4)
  (5.9)
  (9.0)
  (8.9)

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    DATA EVALUATED BASED ON THE
  KCURRENCE OF FROM ONE TO FIVE
CHEMICALS PER SUPPLY-  STATISTICS
PROVIDED BASED ON WATER SOURCE AND
    POPULATION SIZE CATEGORY.

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                      COMMUNITY WATER SUPPLY SURVEY
                        MULTIPLE OCCURRENCE DATAA
                         SURFACE HATER SUPPLIES

                                          NUMBER OF CONTAMINANTS
 POPULATION
   SERVED                         aŁ     M     THREE     FOUR     FIVE
    25-199                       000
   500-2499                      221
  2500-9999                      200
10,000 - 99,999                    52        0
TOTAL                              9410
   SUPPLIES SHOWING ONE OR MORE OF THE FOLLOWING CONTAMINANTS:
   CARBON TETRACHLORIDE; CHLOROBENZENEj 1,2-DlCHLOROETHANEj
   CIS + TRANS-1 , 2-D 1 CHLOROETHYLENE I TETRACHLOROETHYLENEj
   TTLl-TRICHLOROETHANE; TRICHLOROETHYLENE; BENZENE; TOLUENE;
   AND XYLENE (ALL ISOMERS).

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                      COMMUNITY WATER SUPPLY SURVEY

                        MULTIPLE OCCURRENCE DATAA

                          GROUND WATER SUPPLIES


                                          NUMBER OF CONTAMINANTS
 POPULATION
   SERVED                         m     M     THREE     FOUR     FIVE

    25-499                       832         10
   500 - 2499                     11       5        0         0        1

  2500-9999                      330         00

10,000 - 99,999                    920         11

TOTAL                             31      13        2         22


A  SUPPLIES SHOWING ONE OR MORE OF THE FOLLOWING CONTAMINANTS:
   CARBON TETRACHLORIDE; CHLOROBENZENEj 1,2-DICHLOROETHANEj
   CIS + TRANS-1,2-DICHLOROETHYLENEj TETRACHLOROETHYLENEj
   T7L1-TRICHLOROETHANE; TRICHLOROETHYLENEj BENZENE; TOLUENE;
   AND XYLENE (ALL ISOMERS)-

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DATA EVALUATED BASED ON COMPOUND
  CONCENTRATION AND FREQUENCY
DISTRIBUTION.  CHARACTERIZED BY
SIZE CATEGORY AND SOURCE WATER.

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                             COMMUNITY WATER SUPPLY SURVEY

                                FREQUENCY DISTRIBUT10NA

                               TEN SOCs - SURFACE HATER
                                                    NUMBER OCCURRENCES
POPULATION
SERVED
25-499
500-2499
2500-9999
10000-99999
TOTAL
POSITIVES
PER
SUPPLIES
0/20
5/33
2/28
7/25
1V106
I BELOW
OUAN.
LIMITS
100
85
93
72
87
0-5-5

4
2
6
12
CONCENTRATION RANGES, UG/L
>5-10 >10-50 >50-100 >100-500

1


1



1
1
>500





A  SINGLE OCCURRENCE AND HIGHEST CONCENTRATION USED IF MORE THAN
   ONE CHEMICAL OCCURRED IN A SUPPLY.

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                             COMMUNITY HATER SUPPLY SURVEY
                                FREQUENCY DISTRIBUTION*
                               TEN SOCs - GROUND WATERS
              POSITIVES   Z BELOW
POPULATION
SERVED
25-499
500-2499
2500-9999
10000-99999
TOTAL
PER
SUPPLIES
14/156
17/104
fi/41
13/29
50/330
OUAN.
LIMITS
91
84
85
55
85
0.5-5
11
13
6
10
40
>5-10
1
3


4
>10
2


2
4
    NUMBER OCCURRENCES
CONCENTRATION RANGES, UG/L
                                                             >50-100   >100-500   >500
                                                                                   1
                                                                                   1
A  SINGLE OCCURRENCE AND HIGHEST CONCENTRATION USED IF MORE THAN
   ONE CHEMICAL OCCURRED IN A SUPPLY-

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             ADDITIONAL HALXARBONS IDENTIFIED
                     BUT NOT QUANTIFIED

                                      OCCURRENCES
                            SURFACE WATER      GROUND WATER
      COMPOUND                SUPPLIES           SUPPLIES
U-DICHLOROETHANE                0                  H
U-DICHLOROETHYLENE              5                  W
METHYL CHLORIDE                   1                  0
VINYL CHLORIDE                    0                  1
                  TOTAL           6                  19

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            TOTAL ORGANIC CARBON

    SURFACE HATERS EXHIBITED HIGHER TOC
     CONCENTRATIONS THAN GROUND WATERS.

                        CONCENTRATION, UG/L
                        MEAN         MEDIAN
SURFACE WATERS          2600          2200
GROUND WATERS           1500          1000

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