THE CAPE COD AQUIFER
           MANAGEMENT PROJECT (CCAMP)

  A MASS-BALANCE NITRATE MODEL FOR
  PREDICTING THE EFFECTS OF LAND USE
      ON GROUNDWATER QUALITY IN
MUNICIPAL WELLHEAD PROTECTION AREAS
                                       Eastham
                CCAMP WAS UNDERTAKEN BY:
         U.S. ENVIRONMENTAL PROTECTION AGENCY, REGION I
       U.S. GEOLOGICAL SURVEY, MASSACHUSETTS DISTRICT OFFICE
     MASSACHUSETTS DEPT. OF ENVIRONMENTAL QUALITY ENGINEERING
     CAPE COD PLANNING AND ECONOMIC DEVELOPMENT COMMISSION

                  IN COOPERATION WITH:

        THE TOWN OF BARNSTABLE AND THE TOWN OF EASTHAM

     	IDLY 1988	

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                                      9O1388OO7
  A  Mass-Balance  Nitrate  Model  For
  Predicting The  Effects Of Land Use On
  Groundwater  Quality  In   Municipal
  Wellhead Protection Areas
                      By

                Michael H. Frimpter
               U.S. Geological Survey
              Water Resources Division

                John J. Donohue, IV
Massachusetts Department of Environmental Quality Engineering
               Division of Water Supply

                 Michael V. Rapacz
Massachusetts Department of Environmental Quality Engineering
           Division of Water Pollution Control
                    July 1988

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                TABLE    OF    CONTENTS



   Section                                                        Page

Table of contents                                                  i

List of figures                                                    ii

List of tables                                                     iii

Abstract                                                           1

Introduction                                                       2

Hydrogeologic setting                                              3

Previous Nitrate Loading Approaches:                                6
Relation Between Nitrate Loading and
Housing Density in the Zone of Contribution

Proposed Approach:  Accounting for Nitrate                         8
from All Sources Within Municipal Wellhead
Protection Areas

Applications
   Example No. 1                                                  13
   Example No. 2                                                  15
   Example No. 3                                                  16
   Example No. 4                                                  18

Assumptions and Qualifications                                    20

Conclusion                                                        22

References Cited                                                  23

General References                                                24

Appendix A:  Nitrate Concentrations Associated                    A-l
With Varying Land Uses (pp. A1-A8)

Appendix B:  Directions for the Preparation of a                  B-l
Computerized Spread Sheet for the Nitrate Loading
Calculations (pp. B1-B4)

Appendix C:  List of Acronyms, Chemical Formulas                  C
and Mathematical Symbols Used

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                          LIST OF FIGURES
Figure                        Title
                Hydrogeologic section of a pumped
                well in a valley fill aquifer
                Block diagram of house lot showing
                inflow of nitrate diluted with
                recharge from precipitation
                Block diagram of municipal wellhead
                protection area (Zone II) to a public
                supply well
                Sources of nitrate and zones of con-              10
                tribution to a municipal supply well
                pumped at 1 million gallons and 0.5
                million gallons per day
                Map view of glacial valley aquifer                19
                showing the zones and stream that con-
                tribute water to a public supply well
                                 ii

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                          LIST OF TABLES
Table No.                       Title
                    Summary of nitrate loads from sep-             13
                    tic systems for average one day
                    period  -  one million gallon per
                    day well (in liters and milligrams
                    per day)
                    Summary of solid nitrate loads                 14
                    - in milligrams per day
                    Increase in nitrate load due to                15
                    proposed hospital development - one
                    million gallon per day public supply
                    well
                    Summary of nitrate loads from septic           17
                    systems for average one day period
                    • 0.5 million gallon per day public
                    supply well (in liters and milligrams
                    per day)
                    Summary of solid nitrate loads - 0.5           17
                    million gallon per day well
                                iii

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           A MASS-BALANCE NITRATE MODEL FOR PREDICTING THE EFFECTS
       OF LAND USE ON GROUNDWATER QUALITY IN WELLHEAD PROTECTION AREAS

                                     by '"     '

   Michael H. Frimpter, U.  S. Geological Survey,  Water Resources Division
   John J. Donohue, IV, Massachusetts Department of Environmental Quality
                    Engineering, Division of Water  Supply
    Michael V. Rapacz, Massachusetts Department of Environmental Quality
              Engineering,  Division of Water Pollution Control
                               ABSTRACT
 A  mass-balance  accounting  model   can be used  to  guide  the management  of
 septic  systems  and  fertilizers to control  the  degradation of  groundwater
 quality  in  zones  of  an  aquifer  that  contribute water to public  supply
 wells.  .   The nitrate nitrogen concentration  of the  mixture in the well can
 be  predicted  for steady-state conditions, by calculating  the concentration
 that  results  from  the total weight of nitrogen and  total volume of water
 entering  the  zone  of  contribution to the  well.   These  calculations will
 allow  water  quality  managers to predict the nitrate  concentrations that
 would  be  produced  by  different   types  and levels of  development,  and  to
 plan  development  accordingly.     Computations   for  different  development
•schemes  provide  a  technical  basis  for planners  and  managers to compare
 water  quality  effects  and  to select  alternatives  that  limit nitrate
 concentration in wells.

 Appendix  A  contains tables of nitrate loads and water  volumes  from  common
 sources  for  use with the accounting model.   Appendix B describes the pre-
 paration  of  a  spreadsheet  for   the  nitrate loading  calculations  with a
 software package generally available for desktop  computers.

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Introduction

    Protection  of  groundwater  quality  for  public  water supply use has
become  a  priority  environmental  issue.   In recent years, one ubiquitous
cause  of  degradation  of groundwater quality has been nitrate contributed
by  subsurface wastewater disposal systems  and agricultural activities.  In
New  England,  where  shallow, unconsoli'dated aquifer systems provide large
quantities  of  public  drinking water and also receive large quantities of
wastewater,  the  potential for water quality degradation is a primary con-
cern.    In  order  for these two potentially conflicting activities to co-
exist  within  acceptable  limits,  the interrelation between withdrawal for
water  supply  and  wastewater  discharge  needs  to be accurately defined.
This definition requires a characterization of the aquifer system and quan-
tification of the contribution of nitrate to groundwater from land use.

    The  purpose of this paper is to provide an approach for evaluating the
cumulative  effects  of nitrogen contributing land uses on water quality in
public  supply  wells.  The procedure involves the summation of all nitrate
sources  within  a municipal wellhead protection area (Zone II) of a public
supply  well  to  predict  resultant steady-state nitrate concentrations at
the well head.

    Specifically,  the  paper  presents a mass-balance accounting equation,
tables  of  nitrate  nitrogen concentrations and flow volumes (Appendix A),
general  model  examples  and  directions  for the preparation of a comput-
erized spreadsheet for the mass-balance accounting model (Appendix B).

    The  proposed approach departs from previous nitrate loading approaches
used  in Massachusetts, by comprehensively accounting for nitrate inputs to
a  subset  subdivision of the aquifer system the Municipal Wellhead Protec-
tion Area (Zone II).  Properly applied, this approach will provide the nec-
essary scientific foundation for planning development through land use man-
agement,  to  keep  nitrate  concentrations at the well head below a chosen
threshold  value.  Anyone intending to apply this approach needs a thorough
understanding  of  the  Applications  and  Qualifications  section  of this
paper.

    Nitrate  was  chosen as the contaminant of concern for several reasons:
Nitrate  acts  as a conservative chemical species in groundwater; it is not
sorbed  by  aquifer  materials  nor  does it enter into most chemical reac-
tions.   Although nitrogen may be introduced to groundwater in several dis-
solved  forms,  the  proposed approach assumes that all nitrogen in ground-
water  is  converted  to nitrate before reaching a public supply well.  The
principal  mechanism  by  which nitrate is attenuated is by dilution.  Sec-
ondly,  two  health  hazards  are  related to the consumption of water con-
taining  large  concentrations of nitrate (or nitrite); induction of methe-
moglobinemia,  particularly in infants, and potential formation of carcino-
genic  nitrosamines  (National  Research  Council, 1977).  Because of  these
health  related  concerns,  the U.S. Environmental Protection Agency (1975)
has  established  a  maximum  contaminant  level for nitrate as nitrogen in
drinking  water  at  10  mg/L  (milligrams  per  liter).   Nitrate, as used

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hereafter  in this report, refers to nitrate as nitrogen.   In addition,  the
results  of  a  study in Australia suggest that the consumption of drinking
water  containing  elevated  concentrations  of nitrate during pregnancy is
associated  with  a  significantly  increased risk of malformations in off-
spring  (Dorsch, 1984).  Although nitrate may not be the cause of malforma-
tions,  it  is  associated  with  their presence.  It has been demonstrated
that  nitrate  is a geochemical indicator for other more toxic contaminants
associated  with  wastewater  (Dorsch,  1984,  Dewalle,  1985  and LeBlanc,
1984).

Acknowledgments

    The  authors express their appreciation to the Cape Cod Aquifer Manage-
ment  Project  (CCAMP)  project  for providing the impetus and forum to re-
search  and develop this document.  The CCAMP was initiated in 1985 for the
purpose  of examining the adequacy of groundwater programs at all levels of
government  and  for developing or recommending modifications of these pro-
grams.   Members of the project included the Cape Cod Planning and Economic
Development  Commission,  the  Massachusetts  Department  of  Environmental
Quality  Engineering,  the U. S. Environmental Protection Agency, Region I,
and  the  U.  S. Geological Survey.  This report is one of several products
of  the  CCAMP  intergovernmental  collaboration.  The authors also greatly
appreciate  the  assistance  of Ms. H. Gile Beye in preparing Appendix B, a
user's guide to simplify data handling.

Hydrogeologic Setting

    Glacial  outwash  and  ice contact deposits of sand and gravel form the
most  productive  aquifers  in  Massachusetts and New England.  These water
table  aquifers  are most commonly less than 25 feet below land surface and
less  than  100  .feet  thick.    They are typically located either on broad
plains  or  in  low  valley  areas  adjacent  to the streams of the region.
Because  these  aquifers  are recharged from the land immediately overlying
them,  groundwater  quality is highly dependent on local land uses.  Massa-
chusetts  has  developed  an approach to managing groundwater quality which
focuses  management  efforts  on  the  land  which  recharges  that part of
aquifers which contribute water to wells.               "     "

    The  delineation  of  the land area that provides'recharge to a pumping
well  is a prerequisite for the application of the methodology set forth in
this  paper.   In Massachusetts, the land surface that contributes recharge
to  a  public supply well is referred to as Zones II and III by the Depart-
ment  of  Environmental  Quality  Engineering.'   Zone  II and Zone III are
defined  in  310  CMR  24.00  (the  Massachusetts  Aquifer Land Acquisition
Program Regulations, 1983) and shown in Figure 1.

    Zone  II (the Municipal Wellhead Protection Area) is defined in 310 CMR
24.00  as  "The  area of an aquifer that recharges a well [the land surface
which  overlays  that  part of the aquifer that recharges a well] under the
most  severe  recharge  and  pumping  conditions  that can be realistically
anticipated.    It  is  bounded by the groundwater divides that result from
pumping  the  well  and by the contact of the edge of the aquifer with less
permeable materials such as till and bedrock."

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                DRAINAGE DIVIDE
                  ZONE I - 400 FOOT RADIUS ABOUT PUBLIC SUPPLY WELL
                  ZONE II - LAND SURFACE OVERLAYING THE PART OF THE
                          AQUIFER THAT CONTRIBUTES WATER TO THE WELL

                  ZONE III - LAND SURFACE THROUGH AND OVER WHICH WATER
                          DRAINS INTO ZONE II
          -.._..-  DRAINAGE DIVIDE

               ***  DIRECTION OF WATER FLOW
       FIGURE 1:  Hydrogeologic section of a pumped well in a valley-
                                 fill aquifer
    Zone   III is defined as  "That  land area beyond the area of Zone II from
which surface water and groundwater drain into Zone II.   The surface drain-
age  area  as  determined  by   topography  is  commonly  coincident with the

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groundwater  drainage  area  [groundwater  divides in the upland materials]
and  will be utilized to delineate Zone III.   In some locations,  where sur-
face water and groundwater drainage are not coincident,  Zone III shall con-
sist of both the surface drainage area and the groundwater drainage area."

    Zone  II  and . Zone  III  are  two-dimensional  map  projections  of  a
three-dimensional  subsurface  volume.   As such, the proper delineation of
Zone  II and Zone III should account for significant aspects of the surface
water  and  groundwater hydrogeology:  when a well is pumped,  the resulting
Zone  II and associated Zone III represent a state of physical equilibrium.
This  state  of  physical  equilibrium  is  reached  (after days, weeks, or
months),  and  maintained  when  the withdrawal from the aquifer because of
pumping  is  balanced  by  various  recharge  mechanisms.  These mechanisms
include:    areal recharge from precipitation; recharge from induced infil-
tration  of  surface  water;  recharge  from subsurface wastewater disposal
systems;  and recharge from overland runoff and groundwater that drain from
Zone  III  into  Zone  II.  An accurate delineation of Zone II and Zone III
would  account  for  these  various  recharge  mechanisms in their relative
proportions.    For  a more detailed treatment of the determination of Zone
II  and  Zone  III  see  (Massachusetts Department of Environmental Quality
Engineering, 1986 and Donohue, 1986).

    Within  Zone  II,  all  groundwater flow is toward and converges at the
well.    This results in a complete mixing effect of the water (and associ-
ated contaminants) at the well as it is withdrawn from the aquifer.

    The  mass-balance  accounting  model presented in this paper is used to
predict  nitrate  concentrations  at  the  municipal wellhead.  The concen-
trations predicted represent steady-state conditions at the wellhead.

    In  the  field,  steady-state  conditions are reached when physical and
dilution  equilibrium  are attained.  Physical equilibrium is attained when
the  volume of water contributed by the various recharge mechanisms matches
the  amount  of  water  withdrawn.  Dilution equilibrium is attained at the
wellhead  when  the  concentration  of  nitrate nitrogen in the various re-
charge  mechanisms  stabilizes,  and  that  recharge  (water and associated
nitrate  nitrogen)  has  had  sufficient time to move from the most distant
regions  of  the Zone II to the wellhead.  Steady-state conditions may take
tens  of  years or more to achieve, after nitrate loads to the Zone II have
stabilized.    The amount of time necessary to achieve steady-state depends
on the rate of movement of groundwater in the Zone II being considered.

    In  summary, the delineations of Zone II and Zone III are important be-
cause  water  of  impaired quality recharging the groundwater system within
these  areas  ultimately  will affect the quality of water at the wellhead.
When  steady-state conditions have been reached, the water quality observed
at  the  wellhead  represents the sum of the constituents (ratio of nitrate
to  the  volume  of  water  pumped) entering the Zone II.  Accordingly, the
management  of  nitrate loading within the Zone II and Zone III areas is an
effective  approach  to  prevent contamination of municipal supply wells by
nitrate.

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       Previous Nitrate Loading Approaches:  The Relationship Between
                    Nitrate Loading and Housing Density
    Previous  work  on  calculating  nitrogen  loading  to ground water for
Massachusetts  has  focused  on  the determination of the minimum house lot
size  (Figure  4) that could be allowed on an aquifer recharge area without
violating  the  nitrate  limit  (10  mg/L nitrate as nitrogen) for drinking
water  (Cape Cod Planning and Economic Development Commission, 1978).   This
approach  was  based  on  a  mass-balance  mixture  equation  described  as
follows.     The  average nitrate load and water volume from a septic system
were  estimated  and  the  average  nitrate  load from a lawn was estimated
using  information available in the literature (see Appendix A).   To deter-
mine  the  quantity of recharge required to dilute the nitrate to the limit
of  10  mg/L, these estimates of water volume and nitrate load were substi-
tuted  in  a mixture equation similar to the one shown below.  All nitrogen
from  the septic system and fertilizer is assumed to be oxidized to nitrate
after  traveling  through  the  aquifer to the public supply well. Although
the  nitrate limit for drinking water is 10 mg/L, a planning goal of 5 mg/L
was  adopted  by  the Cape Cod Planning and Economic Development Commission
to  ensure  that  the  health  standard  would be rarely exceeded (Cape Cod
Planning  and Economic Development Commission, 1978).  The mixture equation
could be written as:

                           LOAD OF NITRATE
CONCENTRATION  -           	
                           VOLUME OF WATER
              or,
                    LOAD FROM RECHARGE  +  LOAD FROM SOURCES
CONCENTRATION  -   	
                           TOTAL VOLUME OF WATER

Where  load  from  recharge equals recharge volume times nitrate concentra-
tion in recharge (0.05 mg/L nitrate as nitrogen) for Cape Cod, Mass.).

    The  house lot nitrate loads used were 5 pounds per person per year and
9  pounds  per  year per lawn, or 1090 x 10  rag (milligrams) for a 3-person
household.   The volume of wastewater return flow was 65 gallons per person
for  3  persons  for  365  days,  or  7 x 10  gallons (27 x 10  liters) per
household  per  day.     Solving the equation for recharge volume (in cubic
feet),  then  dividing  by the annual recharge rate (1.33 feet per year), a
lot  size  of  59,250  ft  (square feet) (Figure 2) was calculated as being
required  to  capture  sufficient  recharge  to  dilute  the mixture to the
5 mg/L nitrate planning goal.

    For  the  Cape  Cod  208  Water Quality Management Plan, this value was
adjusted  to  43,560  square  feet,  or  1 acre, for areas zoned for single
family  housing  (Cape  Cod  Planning  and Economic Development Commission,
1979)  "after  allowing  for  standard  percentages of roads and open space
associated  with  residential  development."  Land use data for housing and

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                                                     GROUND WATER FLOW
                                                     TO PUBLIC SUPPLY WELL
    NOT TO SCALE
FIGURE 2:  Block diagram of house lot showing  inflow of nitrate
            diluted with recharge from precipitation

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open  space supporting this adjustment were not provided (Cape Cod Planning
and  Economic  Development  Commission,1979).     With  use  of  the nitrate
accounting  model described in the next section of this report,  the need to
provide  open  space  data  to  justify  the  adjustment  to 1 acre lots is
eliminated.

    The  conclusion that a housing density of one house per acre would meet
the  planning  goal  of  5  mg/L nitrate translated into a general planning
guideline  to  protect  groundwater  quality.   This calculation provided an
average  limit  on  housing density where groundwater quality is to be pro-
tected.    For  the protection of groundwater quality, this housing density
guideline,  or  some  adaptation  of it, has been adopted by many towns and
incorporated in their land use zoning ordinances and development plans.

Proposed Approach:  Nitrate Loading From All Sources In Municipal Wellhead
                               Protection Areas
    The  intent  of this guide and the following equation is to offer a com-
prehensive  approach to limiting nitrate degradation from all sources in the
zones  that  contribute water to public supply wells (Zone II,  as defined by
the  Massachusetts Department of Environmental Quality Engineering, Division
of  Water  Supply (Fig. 3).  Nitrogen from all sources is assumed to be oxi-
dized  to  nitrate  before  entering a public supply well.  The mass-balance
accounting  model described here is for prediction of future conditions.  It
is  for steady-state conditions in which all of the nitrate and water enter-
ing the Zone II are in equilibrium with and equal to that withdrawn for pub-
lic supply.  Currently observed low concentrations of nitrate are not neces-
sarily  indicative  of  future  concentrations because many years may be re-
quired  to  reach steady state conditions.  On the basis of slow movement of
groundwater,  as  determined  in  the  Cape Cod aquifer (LeBlanc, 1984), the
steady-state  condition  is  estimated  to  take tens of years or more to be
approached  in  most  parts  of  the Cape Cod aquifer.  This method also re-
quires  that  only  a  small  percentage (less than 25 percent) of the water
withdrawn  is  discharged to and recharges groundwater within Zone II.  If a
large  part  of  the water produced by a public supply well were returned to
the  zone  that  contributes  water to the well (Zone II), then recycled ni-
trate  would  dominate  the effects of dilution from precipitation and other
recharge  sources,  and nitrate would increase and exceed 10 mg/L.  Wells so
affected  by  recycled  nitrate will eventually produce water with more than
10  mg/L  nitrate.  For these wells, the approach described here is ineffec-
tive.    For most wells, this approach is effective because most public sup-
ply wells serve areas much larger than their Zone II.

    Although  there  are reasons for ground-water quality protection outside
of  the  Zone  II  , this paper is limited to activities within the wellhead
protection  area  (Zone  II)  (Fig.  4) that affect nitrate concentration in
water  from  the  public  supply well.  This approach is an expansion of and
more  complete  use of the mass-balance dilution equation used previously to
determine  a maximum average housing density on Cape Cod.  An example of the
equation and its accounting for all sources follows:

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                ZONE OF
             CONTRIBUTION
PUMPING
WATERi
 LEVEL
                                 AQUIFER
                            NOT TO SCALE
FIGURE 3:  Block diagram of a municipal wellhead protection area
          (Zone II) to a public supply well showing the zone
          that contributes water to  the well

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                                  10.
                                                  NOT TO SCALE
FIGURE 4:    Sources  of  nitrate  and zones of contribution to a public
             supply  well  pumped  at  1 million gallons per day (Mgal/d
             and 0.5 million gallons per day (Mgal/d)

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Nitrate
concentration
in well water
        Cw~
                                     11
                   Nitrate load from precipitation + nitrate load from sources

                                      Total volume of water

                 Cr x (Vw -0.9 x (V1+V2+...+Vn)) + < 1^+1.2+... +!<„>
                                         w
where:   C,
         w
        V.
         w
c1+c2-K..+cn
                       nitrate  concentration  of  ground water at the well,
                       in milligrams per liter;

                       volume  of  withdrawal  from  well  in liters (volume
                       must  be  converted  to liters because concentrations
                       are calculated in milligrams per liter;

                       nitrate  concentration in recharge from precipitation
                       in milligrams per liter;

                       nitrate  load  in  milligrams from individual sources
                       where  L  -  C  x V, when load is calculated from the
                       volume  and  nitrate  concentration  of effluent from
                       the source;

                       nitrate concentration in individual sources;  and

                       volume  of  water  used  by  each source before dis-
                       charge to septic system, in liters.
The  load  of  nitrate in recharge from precipitation is the product of ni-
trate  concentration  in  recharge  (C )  times  the volume of recharge de-
rived  from  precipitation  after  adjustment for water from other recharge
sources    (V..-0.9   x   (Vi+V2+...+V )).       Nitrate   concentration   in
                                                Cape Cod (C ) was estimated
groundwater  recharge  from  precipitation  on
as  0.05  mg/L on the basis of an analysis of the frequency'distribution of
nitrate  concentration  in  groundwater.    Thirty  percent  of about 5,000
groundwater  samples  from Cape Cod had nitrate concentrations of 0.05 mg/L
or less.
                                 a  summation
                                 zone.     The
                                               of the loads of nitrate from
                                               term  0.9  x  (V1+Vo+...+Vn)
The  term  (L^+  L2+...+1^)  is
all   sources   within      the  	    	  	  ...   __  , L  /      n-
represents  the  quantity  of  water  returned to the aquifer by the septic
systems  and  other return flows and is subtracted from the withdrawal rate
to  obtain  the quantity of recharge from precipitation that will reach the
well.    The  value  of  the  term  Vj+V2+..-+V  would have been determined
for  delineation  of the zone of contribution (Zone II) and therefore would
be  available  for  substitution  in  the mass-balance nitrate calculation.
The  sum  of the volumes of waste water are multiplied by 0.9 to adjust for
a  10  percent loss by evapotransporation as estimated in the previous work

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                                     12
 by  CCPEDC.     Nitrogen 15  be  introduced  to  the  ground  in  the  reduced state
 (ammonium)   but  is   oxidized   to   nitrate nitrogen  in  the well water.   For
 liquid .sources,   C^  and  V^   are  the  concentration of nitrogen  in nitrate
 nitrogen   equivalents  and  volume of water contributed  by  the  first source,
 respectively,; .  C^> and.-.. A^  .the second  source,   and  Cn  and Vn  are the
 last  (nth)  source.These  data are compiled,  summed and substituted in the
 equation   to  calculate  an estimate of  the nitrate nitrogen  concentration
 for  ground  water  at  the well (C ).  It is  repognizedthatvthis calcula-
 tion  is   an  estimate  that approximates the  concentration  of nitrate at a
 public supply well  under several simplifying  conditions,  none of which are
 expected   to  be  fully met  in  an actual situation.   The process of denitri-
 fication   of groundwater has not yet been described  in  sufficient detail to
 allow  its  inclusion  in these calculations and is  omitted.   The resulting
 influence of   this   omission   on   the  calculation  is  expected to be small
 because  of  the   low  .rate of the denitrification  in  groundwater,  but the
 calculation  should   result .itira slightly higher estimate than would actu-
 ally  occur.   Other  inaccuracies of the  calculated  concentration may be
 introduced  by the   imprecision with  which the individual  loads are esti-
 mated, the  imprecision of  the mapping  of the  municipal wellhead  protection
 area  (Zone  II), and  the areal  variation of  recharge from  precipitation
 over  the Zone.  The nitrate concentrations  calculated  by  this approach are
 intended   to  be   a   guide  for broad  decisions on  limiting land uses that
 increase   nitrate nitrogen in water  supply  wells.  The  significance of
 nitrate  as  a contaminant and an indicator  of contamination  for public
 health in drinking water is described in  the introduction  to this report.

 Applications

     The  prediction   of  nitrate concentration   at   a  well  by the dilution
 accounting  approach  can  be   used to  evaluate  the  potential  for exceeding
 nitrate  concentration  health limits or  planning goals.   Dilution account-
 ing  calculations also can be used to  assess  the relative effects of vari-
 ous  specific   land   uses  or   levels   of development on water quality.  In
 these  applications,  nitrate   dilution accounting is a water  quality plan-
 ning  and management  tool that can be used to  guide decisions.   To calcu-
.late  nitrate  concentrations in milligrams per liter, the  water volumes and
 nitrate  weights   given in  many references and in Appendix A of  this report
 must  be   converted  to the  metric units.  Some examples of calculations and
 discussion  of their  potential use for  planning and management  of ground-
 water quality  follow.

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                                            13
        Example No. 1: Effects of existing and proposed land uses on the nitrate
concentration for a well
Dumped at 1 million gallons per dav (Fi
e. 4)
Table No. 1 - Summary of nitrate loads from septic systems for average one day period
for a well pumped at 1 million gallons per day (in liters and milligrams per day)
SOURCE F10W
(eallons/d)
1.
2.
3.
4.
5.
6.
7.
8.
9.
10.
11.
12.
1/2 acre housing
High school
65/person
20/student
Fast food 150/seat
Restaurant (table seat) <
Fast Food 350/seat
Restaurant (counter seat)
One acre housing
Condominium
Shopping center
Office building
Gas station
Church
Motel A
Motel B
13. Hospital
Totals (VJ+V9+...+V,,;
65/person
65/person
60/employee
15/employee
500/island
3/seat
75/person
75/person
200/bed
)
• UNITS VOLUME CONCENTRATION** LOAD
(•variable) QitersAD (me/L} (me./d)
400 people
1,000 students
70 seats
10 seats
200 people
120 people
50 employees
25 employees
2 islands
200 seats
40 people
160 people
60 beds
98,410
75,700
39,740
13,250
49,210
29,520
11,360
1,420
3.785
2,270
11,355
45,420
45,420
426,860 (L,
40
40
40
35
40
40
40
40
40
40
35
35
35
+LO+ . . . +LI •
3,936,400
3,028.000
1,589,700
463,750
1,968,400
1,180,800
454,400
56,800
151,400
90,800
397,425
1,589,700
1,589,700
,) 16,497,275
Note:   Values  are  selected  from  Appendix  A,  nitrate concentrations in effluent were
        increased  by  5  mg/L based on the assumption that public water supply would not
        exceed  the  5 mg/L planning goal,  the 453,592 milligram per pound conversion was
        rounded  to 454,000 milligrams per  pound,  and a conversion factor of 3.785 liters
        per gallon was used.  Volume was rounded to nearest 5 liters.

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                                           14
           Table No.  2 -  Summary of solid nitrate  loads  in milligrams  per day

14.
15.
SOURCE
Lawns (5,000 ft2)
Horses @ 1,200 Ib
UNITS
100 lawns
6 horses
NITRATE
(pounds/d)
0.025*
0.027/100
MILLIGRAMS/POUND
454,000
Ib 454,000
LOAD
fmpAn
1,135,000
882.580
        each                                of animal

    Total            (L14+L15>                                              2,017,580
 Note:  Based on 9 Ibs/yr of nitrate leaching into the groundwater >system from 5,000
          ft  of lawn (Cape Cod Planning and Economic Development Commission, 1979)


 (Vl + V2 +...+V13) =   426,860 liters

 (Lx + L2 +...+L15) =   2,017,580 + 16,497,275 = 18,514,855


By  substituting  the  calculated total volume and total load in the mixture equation
described  above,  the  concentration' of nitrate at the pumped well can be calculated
as follows:

Calculation No. 1

            Cr x 
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                                     15
  Example No.2:  Prediction of the effect of a proposed forty bed addition
                      to the hospital in Example No.l.
     The   predicted 4.94 mg/L concentration is close to the planning goal of
 5   mg/L.    The  advisability of permitting a proposed 40-bed addition to the
 hospital   (fig.   6,   table 3) in  the zone of contribution can be determined
 by  predicting   its   effect  on   nitrate  concentration  in  the  well.  To
 calculate  the   nitrate   concentration  that would result with the hospital
 addition,   the   estimated additional  water  volume and additional nitrate
 load  can  be   added to the previously determined totals and the new totals
 substituted in  the equation.


 Table  No.  3 - Increase in nitrate load due to proposed hospital addition
      SOURCE        FLOW        UNITS      VOLUME    CONCENTRATION   LOAD
     	(gal/d)      (variable)   Qiters/d)     (mg/L)	(me/d)
 16.   Hospital
      addition     200/bed      40 beds       30,280          35      1,059,800
 Calculation No.  2

 (Vj+V2+...+V14)  +  V16  = 457,140  liters


       (L1+L2+...+L16)  - 19,574,655  milligrams


        Cr  x (Vw-0.9 x  (7^2+...+V)) + (1^+1^+.
-Cw	
                             Vw
        0.05x(3,785,000-0.9x(457,140))  + 19,574,655
 Cw
                    3,785,000


 Cw - 5.22 mg/L (nitrate)


     Calculation  No.   2  includes  the  water  volume and nitrate load that
 would  be caused by the hospital addition,  and exceeds the planning goal of
 5  mg/L.   If the planning goal is to be upheld, then the conclusion must be

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                                    16
to  deny  approval  of the hospital addition as proposed.   In this way,  the
nitrate  accounting  equation  becomes  a decision-making tool for limiting
the  amount  of nitrate discharged to the wellhead protection area.  It  can
also  be  used to compare various potential development plans and to select
future  development  alternatives.     For  example,   the effect of sewering
could  be  predicted  by  subtracting  the  load  of  nitrate that would be
sewered rather than discharged within the Zone II.


Example  No.  3:   Effects of existing land uses in Example No.l on nitrate
for the same well with pumping reduced to 0.5 million gallons per day

    This  example  considers  a  nonuniform distribution of nitrate sources
and  a  reduced pumping rate.  Because a well may-not be pumped at the same
rate  every  year  and  because  there  is no guarantee that the sources of
nitrate  will  be  uniformly  distributed  within the zone of contribution,
additional  calculations  are  advisable.    If  a  lower  pumping  rate is
assumed,  then  the  predicted  zone  of  contribution  to the well will be
correspondingly  smaller  and closer to the well.  See Figure 4 which shows
the  zone  of  contribution  for a well pumped at 1 million gallons per  day
and  a  smaller  zone  of contribution for the same well when pumped at  0.5
million  gallons  per  day.    By summing the water volume and nitrate load
produced  by  the  sources within the smaller zone and solving the equation
to  predict  the  nitrate  concentration  at  the  well,  it is possible to
determine  whether  the  5  mg/L planning goal would be exceeded at a lower
pumping  rate.    Comparison  of  the two nitrate concentration predictions
under  different  pumping  rates would also indicate whether the sources of
nitrate  are  uniformly  distributed  within the larger wellhead protection
area, or whether they are concentrated close to or far from the well.

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                                            17
          Table No. 4  - Summary of nitrate loads from septic systems for average
              one day  period  - 0.5 million gallon per day public supply well
SOURCE FLOW
( gallons /d)
1.
2.
3.
4.
5.
6.
7.
1/2 acre housing
High school
Condos
Shopping center
Office building
Gas station
Motel B
Totals
65/person
20/student
65/person
60/employee
15/employee
500/island
75/person
(L! + L2+.
UNITS
(variable)
300 persons
1,000 students
120 persons
50 employee
25 employee
2 island
160 persons
. .+L7)
VOLUME
(liters/d)
73,807
75,700
29,523
11,355
1,419
3,785
45.420
241,009 (V
CONCENTRATION
(me/L)
40
40
40
40
40
40
35
i + v2+...+v7)
LOAD
(mg/d)
2,952,300
3,028,000
1,180,920
545,200
56,760
151,400
1.589.700
9,504,280
              Table No. 5  Summary of solid nitrate loads for average one day
                  period  - 0.5 million gallon per  day public  supply well


8.
SOURCE
Lawns
(5,000 ft2)
UNITS
(variable)
50
NITRATE
(pounds /d)
0.025
MILLIGRAMS/POUND
CONVERSION
454,000
LOAD
(me/d)
567,500
Calculation No. 3

(Vj+V2+...+V7)  -  241,010 liters

(L1+L2+...+Lg)  =  10,071,780 milligrams

                  Cr x (Vw-0.9x(V1+V2+...+Vn))
  Cw  -
  Cw  -
                                          *w
                     .05 x (1,892,500-0.9 x (241,010)) + 10,071,780
                                      1,892,500
  Cw  •=  5.37 mg/L nitrate

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                                    18
    In  this example, because the loading sources were more heavily concen-
trated  close  to  the  well,  the  nitrate concentration predicted for the
smaller  zone of contribution is higher than that calculated for the larger
zone,  violating the 5 mg/L planning goal.   Similarly, calculations of load
can  be  expanded to account for larger areas of contribution if additional
pumping is planned.


Example No. 4:  Application to glacial-valley aquifers

    Most  public supply wells in New England are in glacial-valley aquifers
bounded  by  less  permeable  till  and bedrock uplands and by streams.  To
account  for  nitrate loading in these aquifers, some additional components
must  be  added  to the dilution accounting equation.  Where a well derives
part  of its yield from induced infiltration from a stream (figs. 1 and 5),
the   quantity  of  water  (Vg)  and  nitrate  concentration  (Cg)  of  the
stream  water  must be entered into the accounting.  Similarly, where water
drains  from beyond the aquifer into the zone that contributes water to the
well  (Figs.  1  and  5),  the  volume of that water (Vjjj) and the nitrate
concentration  of  that  water  C^jj  must  be  entered  in the accounting.
These  considerations  result  in  the  following expansion of the dilution
accounting equation:


Concentration   precipitation load + source load + stream load + Zone III load
 at public    = 	'•	
supply well                    total volume of water pumped
    or,

     Cr x (Vw~Vs~VIII"^'^ x (vl+ V2+1 ' >+Vn^+^Ll+L2+'''+I^^+^Vs x Cs^+^VIII x CIII^
                                     Vw
    Where the new terms are:
    V_ =    Volume of induced infiltration from streams,  in liters:
     o

            volume of drainage from Zone III into Zone II, in liters;

    Cs =    nitrate concentration in induced infiltration, in milligrams per
            liter; and

            nitrate concentration of drainage from Zone III to Zone II, in
            milligrams per liter.

    The  volume of water from streams and the volume of water from Zone III
are  essential  ingredients  for the determination of the zone of contribu-
tion  to a well (Donohue, 1986 and Morrissey, 1987) and,  therefore,  must be
available  wherever the zone of contribution (Zone II) has been determined.

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                                    19
            ZONE 1-400 foot radius about public supply well
                                                            NOT TO SCALE
            ZONE Ih-Land surface overlaying the part of the aquifer that contributes
                      water to the well
            ZONE Ill-Land surface through and over which water drains into Zone II

       	DRAINAGE DIVIDE
FIGURE 5:  Idealized map view of glacial-valley aquifer showing the zones
           and stream which contribute water ,to a public supply well

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                                    20
In  Massachusetts ,   nitrate concentration data for streams may be available
from  the  Division  of  Water  Pollution Control or samples may have to be
collected  for  chemical  analysis.   Estimates of the nitrate concentration
of  water  draining  from Zone III could be made from a dilution accounting
calculation  for  that  zone,  or chemical analysis of representative water
samples might be used.

    Appendix  B  is  a  computer  spreadsheet  for applying this accounting
approach  to  a public supply well in the most complicated case where there
are  contributions  from  surface  water and from Zone (III) outside of the
aquifer.    If  no water is contributed from these sources, as on Cape Cod,
then zeros are entered for Vs, C ,  V-r-r-r, and
    From  inspection  and  comparison  of the calculated nitrate loads from
various  sources ,   a  relative ranking of the importance of the sources can
be  developed.  Once the nitrate loading data are entered into an automatic
spreadsheet,  such  as  shown  in  Appendix  B  of  this report, only minor
modifications  are  necessary  to make sensitivity analyses to test for the
consequences  of different development levels or scenarios .   Assessment and
comparison  of  the  potential  effects  of all sources through the nitrate
accounting  process  described  here assists in the recognition of greatest
threats  to  water  quality  and  corresponding selection of priorities and
scale of groundwater quality management efforts.

ASSUMPTIONS AND QUALIFICATIONS

1.  The  nitrate  accounting approach described here provides the necessary
    information  for land use decisions that will limit groundwater contam-
    inants  in  the  wellhead  protection  area of wells completed in water
    table  aquifers.    The  approach  is appropriate for contaminants that
    are   attenuated predominantly by dilution and that may be tolerated in
    the  1-to  500-mg/L  range of concentration, such as nitrate, chloride,
    and  total dissolved solids.  The approach should not be used to manage
    or  evaluate  threats  from other types of contaminantion, such as sol-
    vents  and  fuels.   The nitrate predictions that result are approxima-
    tions  of long-term average concentrations, which are imprecise in that
    actual  concentrations  may  be  expected  to  be  above  and below the
    average.    For  this  reason, a planning standard, or goal, of 5 mg/L,
    which  is lower than the 10 mg/L health standard, has been advocated by
    the  Cape  Cod Planning and Economic Development Commission and is used
    in the examples in this guide .

2.  The  approach  assumes  that, under steady-state withdrawal conditions,
    all  of  the water and nitrate withdrawn from the well are derived from
    the  zone of contribution for the well, and that only some of the water
    withdrawn  is  returned to the zone of contribution as return flow.  In
    those  situations  where  a well derives some of its yield from induced
    infiltration  from  streams or other surface water bodies, the quantity
    and  quality of induced infiltration need to be entered in the account-
    ing.    The  quantity  of water derived from induced infiltration would

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                                    21
    have  been computed in order to delineate the zone of contribution and,
    therefore,  would  be  available  for  nitrate  calculations.   In those
    situations  where a well derives some of its yield from an area of till
    upland  beyond  the  boundary  of  the  aquifer  from  which ground and
    surface  water  drain  (Zone  III),   the  quantity  and quality of such
    drainage need to be entered in the accounting.

3.  The  formula  predicts  concentration  at  the  well under steady-state
    conditions  where  all  of  the  water from the zone of contribution is
    mixed.   Individual plumes with elevated concentrations of contaminants
    would  be  expected  to  emanate  from septic systems and other sources
    within  the zone of contribution.  Therefore, the prediction should not
    be  used  to determine contaminant concentration at other points within
    the  aquifer, or to determine the concentration in any smaller (private
    domestic supply) wells within the zone of contribution.

4.  The  contaminant  (nitrate) is considered to act conservatively.  It is
    not  absorbed or adsorbed by aquifer materials.  Attenuation is assumed
    to  occur  only  through the process of dilution.  Some diminishment of
    nitrate  through  other processes is known to occur, but the quantities
    affected  are  not  large  enough  to  be  considered  in  these  gross
    calculations.

5.  The  zone  of contribution to the well is assumed to remain constant in
    size  and  shape  for  application  of  the nitrate accounting approach
    described  here.   Actually, the size of the zone is expected to become
    smaller  as  more return flow from septic systems recharges the zone of
    contribution,  but  additional  recalculations of the zone of contribu-
    tion  would most likely be expensive and have an unacceptably high cost
    to  benefit ratio.  Therefore, this assumption results in protection in
    a  zone  slightly larger than may actually contribute water to the well
    and  is therefore considered conservative if sources are uniformly dis-
    tributed.    Recharge  to the aquifer is assumed to be uniform over the
    zone  of  contribution.  Where variations of aquifer properties or sur-
    face  drainage  characteristics  cause  irregular  distribution  of re-
    charge,  both  the delineation of the zone of contribution and the cal-
    culation  of  contaminant concentration would have to take those varia-
    tions  into  account.    Under such conditions, the predictive approach
    described in this guide may not be accurate.

6.  For  the  examples  shown  here,  return flow of public supply water is
    estimated  to  be  10  percent less than the quantity of water supplied
    because  of  evaporation  and  transpiration from outdoor uses and from
    septic  system  leach  fields.    Future research may indicate that the
    return  flow from septic systems is somewhat different.  The 10 percent
    value  is  based  on  the  findings  of  Cape Cod Planning and Economic
    Development  Commission  and estimates for Long Island, New York.  Soil
    conditions  over other aquifers will most  likely allow different rates
    of evaporation and transpiration.

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                                    22
7.  On  the  basis  of  nitrate  analyses of about 5,000 water samples from
    shallow  wells  on  Cape  Cod, the nitrate concentration of groundwater
    recharge  was  estimated  to  be  0.05  mg/L  for  the examples in this
    guide.   The concentration of nitrate in recharge may vary considerably
    from  region  to  region primarily because of differences in quality of
    precipitation, soils, and geology.  Application of the nitrate account-
    ing  approach  described here needs to take these local geochemical and
    hydrologic conditions into consideration.

8.  It  is  necessary  to demonstrate that the sources of nitrate are rela-
    tively  uniformly  distributed within the zone of contribution by using
    the  technique  for  predicting  nitrate concentrations at the well for
    lower  withdrawal  rates.    Without  application of the prediction for
    lower  withdrawal  rates,  it  would  be  possible  for land uses to be
    concentrated  about  a well in such a pattern that although the nitrate
    planning  goal is not exceeded at the maximum withdrawal rate, it might
    be  exceeded  at  some  lower  withdrawal  rate.  This is a significant
    consideration,  because  withdrawal  rates  from an individual well are
    commonly changed from time to time.
CONCLUSION:

    This  nitrate  accounting  approach  can  be  used  to  predict nitrate
concentrations  in  public  supply  wells.    These  predictions will allow
planners  and  managers  to recognize what level of incremental development
will  cause violations of nitrate planning goals thereby signaling the need
to  cease further development of nitrate loading activities within the zone
of  contribution.    Alternatively, predictions may be used to indicate the
level  of  development  at  which  sewering within the zone of contribution
would  be  needed  to  limit nitrate contamination of a public supply well.
Most  importantly,  this  nitrate  accounting approach provides a technical
basis  for  evaluating future alternative development plans and for compar-
ing  tradeoffs  between  various  land  uses  and  development proposals in
groundwater quality protection areas.

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                                     23
                               REFERENCES CITED
 1.    Bear,  Jacob,   1979,  Hydraulics  of  Groundwater:    New  York,  N.Y.,
      McGraw-Hill,  Inc.,  569 p.

 2.    Cape   Cod  Planning and Economic Development Commission (CCPEDC) 1978,
      Environmental  Impact  Statement  and 208 Water Quality Management Plan
      for Cape  Cod, Vol.  1 and Vol. 2, 340 p.

 3.    Cape   Cod  Planning and Economic Development Commission (CCPEDC) 1979,
      Water  Supply  Protection   Project  - Final Report:  ..Barnstable, Bourne,
      Brewster,  Dennis, Yarmouth,  20 p.

 4.    Dewalle,   F.B.  Kalman, D.A., Norman, 6., Plews, 6., 1985, Determination
      of toxic  chemicals  in   effluent  from  household septic tanks:  U.S.
      Environmental  Protection  Agency, Water Engineering Research Laboratory
      EPA/600/S2-85/050,  9 p.

 5.    Donohue,   J.  J.  IV, 1986,  "Zone II Determination:  A Case Study of Two
      Hydrogeological  Investigations,"  Proceedings  of  the  Third  Annual
      Eastern   Regional Ground Water Conference, National Water Well Associa-
      tion,  Dublin/Ohio,  pp. 54-63.

 6.    Dorsch,   M.M.,   1984,   "Congenital Malformations and Maternal Drinking
      Water  Supply  in Reval, South Australia, American Journal of Epidemio-
      logy,  Vol.  119, No. 4, pp.  473-486.

 7.    LeBlanc,   D.R.,  19B4, "Sewage Plume in a Sand and Gravel Aquifer, Cape
      Cod,   Massachusetts,"  U.S.  Geological Survey Water Supply Paper 2218:
      Washington,D.C.,  Government Printing Office, 28 p.   /

 8.    LeBlanc,   D.R.,  Guswa,  J.H., Frimpter, M.H. and Londquist, C.J. 1987,
      "Ground-Water  Resources   of Cape  Cod, Massachusetts," U.S. Geological
      Survey   Hydrologic  Atlas 692,   Washington,  D.C.,  U.S.  Government
      Printing  Office,  4  pis., scale 1:48,000.

 9.    Massachusetts  Aquifer  Land Acquisition  Program Regulations  (310 CMR
      25.00),   1983,   Massachusetts Department of  Environmental Quality Engi-
      neering,  Division of Water Supply,  Boston, Massachusetts, 4 p.

 10.   Massachusetts  Department   of  Environmental Quality Engineering, Divi-'
      sion   of   Water  Supply, 1986, Hydrogeologic Study Requirements  for the
      Delineation  of  Zone II and Zone  III  for New Source Approvals,  Boston,
      MA, 11 p.                             (
                                                                            ^
 11.   National   Research  Council, 1977,  "Drinking  Water and Health", Washing-
      ton, National Academy of Sciences,  939 p.

 12.   U. S. Environmental Protection Agency, 1975, Water programs,  national
,  '    interim   primary drinking  water  regulations, V. 40, No.  248, Wednesday,
      December  24,  1975,  Part  IV, p.  59566-59587.                      '    ^

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                                    24

                          GENERAL REFERENCE LIST
 1.   Anderson  -  Nichols  and  Co.,   Inc.,   1985,  Edgartown Water Resource
     Protection Program - Final Report

 2.   Bear,   Jacob,  1979,  Hydraulics  of  Groundwater:     New  York,  N.Y.,
     McGraw-Hill,  Inc.

 3.   Belfit,  G.,  1986, Personal communication concerning fertilizer appli-
     cation  rates  to   golf  courses  on  Cape Cod:   Cape Cod Planning and
     Economic Development Commission  (CCPEDC).

 4.   Bennett,  E.R.,   Leach,  L.E.,   Enfield,  C.G.  and Walters,  D.M.,  1985,
     Optimization of nitrogen removal by rapid infiltration:   U.S. Environ-
     mental Protection Agency, EPA/600/S2-85/016.

 5.   Cape  Cod Planning and Economic Development Commission (CCPEDC),  1979,
     Water  Supply  Protection Project - Final Report:   Barnstable, Bourne,
     Brewster, Dennis,  Yarmouth.

 6.   Cape  Cod  Planning  and  Economic  Development   Commission  (CCPEDC),
     1978,   Environmental Impact Statement and 208  Water Quality Management
     Plan for Cape Cod, Vol. 1 and Vol. 2.

 7.   Clark,  B.,  1986,  Communication  concerning  fertilizer  application
     rates,  leaching rates and grass types on Cape Cod:  Barnstable County
     Extension Service - personal communication.

 8.   Cooper,  R.,   1986,  Communication  concerning  fertilizer components,
     application   rates,   potential   for  leachability  or  uptake,  and
     fertilization  rates:    UMASS,   Amherst,  MA, Dept. of Plant and Soil
     Sciences.

 9.   Cornell  University,  1974,  Nitrogen  utilization   by crops:  Cornell
     Field Crops Handbook.

10.   Deubert,  K.H.,   1986,  Communications  concerning  nitrogen loading in
     the  form  of fertilizers for cranberry bogs:  Wareham,  MA.  Cranberry
     Experiment Station - personal communication.

11.   Dewalle,  F.B.,   Kalman, D.A.,  Norman, G., Plews, G., 1985, Determina-
     tion  of toxic chemicals in effluent from household septic tanks: U.S.
     Environmental    Protection   Agency,    Water    Engineering   Research
     Laboratory, EPA/600/S2-85/050.

12.   Dickey,  E.G.  and Vanderholm,  D.E., 1981, Vegetative filter treatment
     of livestock feedlot runoff:  J. Environ. Quality., Vol. 10, No.  3.

13.   Douglas,  D.F.   1986,  Literature  Review  of  the Cumulative Impact of
     On-Site  Sewage  Disposal Systems on Nitrate - Nitrogen Concentrations
     in  Ground  Water:    Ground  Water Management Section.   Department of
     Water Resources and Environmental Engineering, State of Vermont.

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                                     25
14.  Dorsch,  M.M.,   1984,   "Congenital  Malformations and Maternal Drinking
     Water  Supply  in  Rural  South  Australia:     A  Case-Control  Study,"
     American  Journal  of  Epidemiology,  the John  Hopkins  University of
     Hygiene and Public Health.

15.  Eckenfelder,  W.W.  Jr., 1970,  Water quality engineering for practicing
     engineers:  Boston, MA,  Cahner  Books International,  Inc.

16.  Edwards,  W.M.,   Chister,  F.W.  and Harrold,  L.L.,  1971,  Management of
     barnlot  runoff  to  improve downstream  water quality:  International
     Symposium on Livestock Wastes pp. 48-50, 1971.

17.  Gerhart,  J.M.,   1986, Ground-water recharge and its effects on nitrate
     concentrations  beneath  a manured field site in Pennsylvania:  Ground-
     water, Vol. 24,  No. 4, July-August.

18.  Harper,  J.,  1983,  Turf  and  garden fertilizer handbook:  Washington,
     D.C., The Fertilizer Institute.

19.  Hem,  J.D., 1970, "Study and Interpretation  of Chemical Characteristics
     of  Natural  Water,"  U.S.   Geological  Survey Water Supply Paper 2218:
     Washington, United States Government Printing Office.

20.  Heufelder,  G.,   1986,  Barnstable  County  Board  of  Health, Personal
     communication.

21.  Hinisk,  W.W.,   1978,   Forty questions  and  answers on manure:  Penn-
     sylvania State University,  College of Agriculture,  Leaflet No. 213.

22.  Holyoke,  V.,  1981,  Manure  is  not  an evil:    New England Farmer.
     October 1979.

23.  LeBlanc,  D.R.,   1984, "Sewage  Plume in a Sand and Gravel Aquifer, Cape
     Cod  Massachusetts,"  U.S.   Geological  Survey Water Supply Paper 2218:
     Washington, United States Government Printing Office.

24.  Litchfield,  J.H.,  Meat,  fish,  and poultry processing wastes:  Water
     Pollution Control Federation, Volume 56, Number 6.

25.  Livestock waste facilities handbook.

26.  MacQueen,  M.,  1986,   Pilgrim  Resource  Conservation  and Development
     Council, Middleboro, MA, personal communication.

27.  Metcalf  &  Eddy,  Inc.  1972,  Wastewater:  collection, treatment, dis-
     posal:  New York, McGraw Hill.

28.  National  Research Council, 1977, "Drinking Water and Health," Washing-
     ton, National Academy of Sciences.

-------
                                     26
29.  North  Carolina  State  University,  1978,  Best management practices for
    . agricultural  nonpoint source control:   Biological and agricultural en-
     gineering department,  North Carolina State University,  Raleigh,  N.C..

30.  Tchobanoglous,   G.,  rev.,  1979,  Wastewater engineering:   treatment dis-
     posal, reuse:  New York, McGraw-Hill.

31.  Tchobanoglous,   G.,   Theisen, H.,  and Eliasses, R.,  1977, Solid wastes:
     engineering  principles  and  management issues:  New York,  McGraw-Hill
     Book Company.

32.  U.S.  Environmental  Protection Agency,  1977,  Process design manual for
     land  treatment of municipal wastewater:  U.S. Environmental Protection
    ., Agency,  Office  of  Water  Program  Operations,  EPA  625/-77-008 (COE
     EM1110-1-501).

33.  U.S. Environmental Protection Agency, 1984, Handbook for septage treat-
     ment  and  disposal:    U.S.  Environmental Protection Agency,  Environ-
     mental Research Laboratory, Ohio,  EPA 625/6-84-009.

34.  U.S.  Environmental  Protection  Agency,  U.S. Army Corps of Engineers,
     U.S. Department of Interior, U.S.  Department of Agriculture,, 1981, Pro-
     cess  design  manual  for land treatment of municipal wastewater:  U.S.
     Environmental  Protection  Agency,  Center  for  Environmental Research
     Information, EPA/625/1-81-013 (COE EM1110-1-501).

5.   U.S.  Environmental  Protection  Agency,  1977,  Alternatives for small
     wastewater treatment systems, EPA/625/4-77-011.

36.  U.S.  Environmental  Protection  Agency,  October  1975, Process design
     manual  for  nitrogen  control:    U.S.  Environmental Protection Agency,
     Office of Technology Transfer, Washington, D.C.

37.  U.S.  Department  of Agriculture,  U.S.  Environmental Protection Agency,
     1979,  Animal  waste  utilization  on  cropland  and pastureland:  USDA
     Utilization research report No.  6, EPA - 600-2-79-069.

38.  United  States  Geological, Survey,   1986,  Personal communication con-
     cerning  water  quality  analysis for public water supply wells on Cape
     Cod; Water Resources Division -  Boston,  MA.

39.  Wehrmann,  A.E.,   1983,  Potential nitrate contamination of groundwater
     in  the  Roscoe area,  Winnebage County,  Illinois:   Champaign, Illinois:
     Illinois State Water Survey.

40.  Wells,  R.G.,  1986,  Communications  concerning the .appropriate appli-
     cation  rates  for  fertilizers:    Washington,  D.C.,   The  Fertilizer
     Institute.

41.  Young,  R.A.,  Huntrods,  T.  and  Anderson, W., 1980,  Effectiveness of
     Vegetated  buffer  strips in controlling pollution from feedlot runoff:
     Journal of Environmental Quality,  Vol.  9,  No.  3, 1980.

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                                               APPENDIX A

                      NITROGEN CONCENTRATIONS ASSOCIATED WITH DIFFERENT LAND USES
Page         Section          Title

A-1             1             Sewage Flow Volumes and Nutrient Concentrations
A-4             2             Animal Feedlot Nitrogen Production
A-5             3             Nutrient Utilization by Crops, Trees and Ground Cover
A-6             4             Uastewater Treatment Facilities
A-7             5             Septage Pits and Lagoons
A-7             6             Cranberry Bogs and their Fertilization
A-7             7             Fertilizers and Lawns
A-9             8             Nutrient Input from Lawn Fertilizers
A-10            9             Nitrogen Leachability
A-12           10             Golf Courses
A-13           11             Precipitation  .
                                                 TABLES

Page         Table            Title

A-1 •          1A              Sewage flow volumes and nitrate concentrations
A-4           2A              Feedlot Wastes
A-4           2B              Influence of Time and Wind Speed on Nitrogen Losses
A-5           3A              Nutrient Utilization by crops, trees and commonly occurring ground cover
A-6           4A              Nitrogen removal variations
A-8           7A              Common Grass Types
A-11          9A              Nitrogen Leachability

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                                   Section  1.
                                                  Sewage  Flow Volumes and Nutrient Concentration
The following Table 1A is a list of sewage flew volumes commonly discharged from commercial,  recreational  and domestic  land  uses.
The nitrate nitrogen figure presented is the concentration of nitrate nitrogen expected to be generated,  assuming  ammonia  nitro-
gen has been bacterially oxidized and is in the nitrate form.
                                          Table 1A - Sewage Flow Volumes and Nitrate Concentrations
           Land Use
Unit
  Flow-GPD/
Person or Unit
                                                                                 Concentration
                                                                                of NOj-N mg/l
                                                                      Ibs.  NCyN/
                                                               1000  gallons of  Wastewater
                                                               Cone.
                                                               in mg/l       Ibs. NC-N.
1)  Restaurants
   'A.  food service-lounge tavern
    B.  thruway service area
        thruway service area
    C.  short order
    0.  bars, cocktail lounge
    E.  average type
        average type
    F.  cafeteria
    G.  mess hall
    H.  coffee shop

2)  Schools
    A.  day/cafeteria
    B.  day/cafeteria showers
    C.  day
    D.  high school
    E.  elementary
    F.  boarding
seat
table seat
counter 'seat
person
person
seat
meal
seat
person
person
person
person
person
person
person
person
35
150
350
4
2-20
35
7
150
15
250
10-15
20
10
20
10
75
                                           35-40
                                           35-40
                                           30-35
                                           35-40
                                           35-40
                                           35-40
                                           35-40
                                           30-35
                                           30-35
                                           30-35
                                           35-40
                                           30-35
                                           35-40
                                           30-35
                                           35-40
                                           30-35
                                                   10
                                                   30
                                                   35
                                                   40
                                                   45
                                                   50
                                                  100
0.08
0.25
0.29
0.33
0.38
0.42
0.83
                                                                     A-1

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                                       Table 1A • Sewage Flow Volumes and Nitrogen Concentrations   -  continued
                                          Table 1A • Sewage Flow Volunes and Nitrate Concentrations
            Land Use

3)   Parks/Campgrounds
     A.   developed campground
     B.   camp/mess hall
     C.   day camp/no meals
     D.   luxury camp/private bath
     E.   traitor/toilet/bath
     F.   trailer village
     G.   trailer dump station
     H.   lodge/cabin
     I.   picnic parks/toilets
     J.   park/shower/toilet
     K.   swimming pool/beaches

4)   Hospitals
     A.   hospital
     B.   hospital
     C.   prison

5)   Recreation
     A.   fairgrounds/daily
     B.   assembly halls
     C.   theatre/auditoriun/inside
     D.   theatre/outside/food stand
     E.   gymnasium
     F.   country club-resident  type
     G.   country club-transient/meals
     H.   church
     I.   bowling alley
     J.   skating rink (3000  gpd+)
    Units
    person
    person
    person
    person
2 1/2 persons
    person
    per site
    person
    person
    person
    person
    bed
    person
    person
    person
    person
    person
    car
    person
    person
    person
    seat
    alley
    seat
  Flow-GPO/
Person or Unit
      25
      15
      10
    75-100
   125-150
      35
      50
      50
     5-10
      10
    10-15
      200
   125-200
      175
       1
       2
      3-5
      3-5
      3-25
     20-100
     17-30
       3
    100-200
       5
                                                                                                                    Potential
                                                                                                                  Concentration
                                                                                                                 of NOj-N mg/l
35-40
35-40
35-40
30-35
30-35
35-40
35-40
35-40
35-40
35-40
35-40
30-35
30-35
30-35
35-40
35-40
35-40
35-40
30-35
30-35
35-40
35-40
35-40
30-35
                                                                              A-2

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                                    Table 1A • Sewage Flow Votunes and Nitrate Concentrations -  continued
          Land Use

6)   Commercial.
     A.   gas stations
     B.   gas stations
     C.   office building
     D.   office building
     E.   barber shop/beauty parlor
     f.   dry good store
     G.   stores -
     H.   stores
     I.   shopping center
        Units
        island
        vehicle
        person
        1000 ft.2
        seat
        100 ft. 2
1st 25 ft.  of frontage
   additional 25 ft.
        employee
   Flow-GPO/
Person or Unit
    300-500
      10
     10-15
      75
     100
       5
     450
     400
      60
                                                                                                                     Potential
                                                                                                                   Concentration
                                                                                                                  of  NOj-N  rag/I
 35-40
 35-40
 35-40
 35-40
 30^35
 35-40
 35-40
 35-40
 35-40
7)   Dwellings
     A.   private - pub/priv.  water supply
     B.   apartments/private wells
     C.   single/multiple
     D.   general
     E.   hotels
     F.   motels
     G.   boarding house1
     H.   mobile home park
     I.   co I leges,: boardi ng • schoo I s
     J.   residence 'homes/apartments
     K.   dormitory, bunkhouse
     L.   construction camp
     M.   private dwellings
        person
        person
        per bedroom
        person
        person
        person
        •person
        site
        person
        person
        person
        person
        110 gal
     50-70
     75-100
     110
      55
     50-100
     50-75
     50-75
     200
     50-65
      75
      50
      50
10-15,000 ft2
 30-35
.30-35
 30-35
 30-35
 35?40
 30-35
 30-35
 35-40
,35-40
 35-40
 35-40
 35-40
 30-35
Some  of  the  flow/unit  values  appearing  in  the  above, table  have  been  taken  from  "310  CMR  15.00"  The  State  Environmental  Code-Title
5   Minimum   requirements   for  the  subsurface  disposal  of  sanitary  sewage."   -Title  5  provides  flow  estimates • for  varying  land  uses.
These values are to be used when sizing a leaching area as part of a subsurface wastewater disposal system.

The   potential   concentration   of   NO,-N   mg/1   values   have   been  taken  from  planning  documents  and  sampling  date  collected  by  the
Massachusetts   Department   of   Environmental  'Quality'  Engineering.      The  -values :  wilt  vary  depending  on  water  use  practices.    For
example,   a   business   that   employs   strict   water   conservation   techniques  and  hardware  will  have  a  higher  concentration  of  NOj-N
when measured as milligrams per liter.
                                                                               A-3

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                                                    Section 2 - Animal Feedlot Nitrogen Production

                             Table 2A presents the nitrogen production potential common to animal feedlot waste products:

                                                              TABLE ZA -  FEEDLOT WASTES

                                                                                                              Ibs/day of nitrogen per
                        Animal                                                                                   100 Ibs of animal
                                                                                                                   without loss	
                      Dairy Cattle                    .                                                                0.040
                      Beef Cattle                                                                                     0.034
                      Finishing pig                                                                                   0.045
                      Sow and litter                                                                                  0.060
                      Sheep                                                                                           0.045
                      Horses                                                                                          0.027
                      Chickens                                                                                        0.087
                      Ducks                                                                                           0.142


Generally one ton (2000 Ibs) of manure  is composed of 1380  Ibs. solid and 620  Ibs. of liquid.  The liquid portion of  manure is
immediately available for plant uptake.  Only a small percentage of the solid  portion is available the first year, prior to bacte-
riological breakdown of solids in the soils.  The potency of manure is greatly decreased because of failure to utilize the liquid
portion and excessive nitrogen loss from solids by ammonia  volatilization, due to volatilization and evaporation.


                                             TABLE 2B • INFLUENCE OF TINE AND WIND SPEED ON NITROGEN LOSS

                                                                         Percent Total nitrogen lost

                      Manure spread                                   Ho wind                                 8 1/2 moh wind

                      12 hrs. 3 68°F                                  7.7 percent                              25 percent
                      36 hrs. a 68°F                                  23 percent                               31 percent
                      7 days a 68°F                                   36 percent                               37 percent


Manure that is not collected and applied promptly and properly has very limited value.  Ten tons of potent manure (20,000 Ibs) is
comparable in nutrient value to 500 pounds of a 10-6-10 (nitrogen-phosphorous-potash) commercially available fertilizer.

                                                                               A-4

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                                                Section 3  -  Nutrient Utilization by Crops. Trees, and Ground Cover


Uhen considering the amount of nitrogen available to leach throughout vegetated top soils and surficial deposits,  the nitrogen uptake poten-
tial of the ground cover must be considered.  Table 3A presents values from the literature describing the nitrogen uptake potential  for sev-
eral crops and ground covers.

                                          TABLE  3A -  NITROGEN UTILIZATION  BY CROPS AND COMMONLY-OCCURRING GROUND COVER *

                                                                                                                           pounds of nitrogen
          Vegetative Type                                                                                                  per acre per year

          corn                                                                                                                     250
          grass-legume hay                                                                                                         300
          oats                                                                                                                      60
          sunnier annuals                                                                                                           200
          pines  (trees)                                                                                                           27-62
          mixed coniferous                                                                                                        36-71
          deciduous (trees)                                                                                                       44-88
          alfalfa                                                                                                                  450
          bromegrass                                                                                                               165
          coastal bermuda grass                                                                                                    500
          reed canary grass
          rye grass                                                                                                                210
          sweet clover                                                                                                             157
          tall fescue                                                                                                              118
          barley                                                                                                                    62
          cotton                                                                                                                    66
          milomaize                                                                                                                 81
          soybeans                                                                                                                  94
          kentucky bluegrass                                                                                                     178-240
          quackgrass                                                                                                             210-250
          orchardgrass                                                                                                           225-310
          grain sorghum                                                                                                            120
          potatoes                                                                                                                 205
          wheat                                                                                                                    143


*  Values used are approximations from current literature.  The values presented include the nitrogen fixed from the air  as N and nitrate
       nitrogen  in soils.  To achieve these  values the  plant must be harvested.

                                                                               A-5

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                                                           Section 4 - Wastewater Treatment Facilities
Different  levels of sanitary wastewater treatment provide varying levels of nitrogen compound removal.  Nitrogen remaining after treatment
will presumably be converted to the nitrate form some distance from the subsurface discharge point.  Water quality analysis conducted for
municipal  wells on Cape Cod supports this presumption.  Host samples collected contain nitrate but very limited nitrogen in the ammonia
form.

The Massachusetts regulatory agencies consider primary treatment of effluent to be removal of at least 25% of the five day Biological Oxy-
gen Demand (BOO,) 55X of the suspended solids and 85X of the floating solids and solids that settle out.  Secondary treatment is con-
sidered to be removal of at least 85X 800,  and suspended solids and removal of all settleable and floating solids.  Advanced treatment
is considered any treatment form exceeding secondary treatment.  Examples of advanced treatment would be the addition of a nitrification/de-
nitrification stage for nitrogen removal or carbon filtration or an air stripper for the elimination of volatile organic chemicals.
                                                             TABLE 4A  -   NITROGEN  REMOVAL  VARIATIONS
                  Treatment
                   Process

                   primary
                  secondary
                  advanced
                 (denitrification)
Nitrogen Removal
  Potential X

no removal 0-10X
none-slight 0-30%
    70-95X
         Total
 Nitrogen Concentration
  of Untreated Effluent
	ma/1	

          40
          40
          40
       Total
   POST Treatment
 Nitrogen Concentration
	mg/l	

      35-40
      25-40
       6-10
     In the Commonwealth of Massachusetts  treatment  plant  discharges  to  ground-waters are  required to discharge at or below the drinking
water standard for nitrates or total nitrogen (10 mg/l) if they are an industrial discharger, discharge over 150,000  gallons  per day of
sanitary wastewater or are considered by the regulatory agency to be in an environmentally sensitive area.   The use of  treatment plants  is
required for all industrial discharges and sanitary wastewater discharges over 15,000 gallons per day.   It  is highly  unlikely that the
State of Massachusetts would permit the construction of a municipal scale wastewater treatment plant within the delineated Zone II of a
public supply well.  Location of commercial and large scale residential  wastewater treatment plants  is  evaluated on a case by case basis
with drinking water supplies being considered the most important potentially impacted resource.
                                                                               A-6

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                                                          Section 5 - Septage Pits and Sanitary Lagoons
     Although great effort has been made by regulatory authorities  to phase  out  "septage pits" as a disposal option, several municipal and
private pits/lagoons exist throughout the Commonwealth.  Because of the less-dilute nature of septage the nitrogen levels (organic  nitrogen
and ammonia-nitrogen) available for conversion to nitrate greatly exceed sanitary wastewater.  The ammonia nitrogen levels commonly
observed in septage exceed 100 mg/l.  EPA documents reviewed suggested that 150 mg/l would be an appropriate design figure although total
nitrogen concentrations observed in septage samples often approach 400 mg/l.  One thousand gallons of septage  has the potential  to  generate
between 0.83 and 1.25 pounds of nitrate nitrogen.
                                                        Section 6 -  Cranberry  Bogs and Their  Fertilization

     Massachusetts is this countries highest bulk producer of  cranberries.   This  requires the use of thousands of acres of land for
cultivation and the use of tons of fertilizer to stimulate plant growth.  Between ten and forty pounds of nitrogen/acre/year are  applied to
cranberry bogs.  Thirty Ibs/acre/year is assuned to be the average application rate.  Nitrate applications are monitored carefully because
the plants will sprout leaves rather than berries if excessive quantities of nitrogen are applied.   It is therefore probable that a large
percentage of the nitrogen applied to the bogs is utilized by the plant.  Since the plant is harvested, very little plant decay matter is
available for bacteriological breakdown.  Very acidic, low pH environments associated with bogs do  not stimulate bacteriological  activity
necessary for the conversion to nitrate.  Surface water runoff via drainage ditches, flood channels or tributary streams associated with
bogs sometimes have elevated nitrate nitrogen concentrations.
                                                                 Section 7 -  Fertilizer and Lawns

     Fertilizers are applied to ground covers and crops to stimulate growth and  productivity.  The following table describes the lawn
fertilizer application rates suggested by the National Fertilizer Institute in their publication "Turf and Garden Fertilization Handbook".
The rates of application suggested should stimulate maximum plant growth under most circumstances.   The grasses listed are common  ground
covers found throughout Massachusetts and the fertilizers are readily available commercial products.
                                                                               A-7

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                                                                             Table 7A
                                                     Common Grass Types - Reconroended Fertilizer Application


Grass Type
Kentucky Blue
Kentucky Blue
Rye
Rye
Tall Fescue
Tall Fescue
Leafy Fescue
Leafy Fescue


Fertilizer
regular
slow release
regular
slow release
regular
slow release
regular
slow release

Ibs/ni trogen
1000 ft2/vear
2-3
3-4
3-5
4-6
3
3-4
2
4
Recommended
Nunber of
Applications
3
2
3
2
2
2
2
2
Most cultivated lawns include these grass types in varying percentages.  For example, an attractive,  durable,  well-maintained lawn may
include 40X Kentucky Blue grass, 30X fescue and 30X rye grass.


                                                         Section 8 -  Nutrient  Input from Lawn Fertilizers

The Long Island Cooperative Extension Service presented in a 1978 planning stud/, fertilizer application rates thought  to be typical  for
lawns on Long Island.  It was assumed that:

                          o     3 IDS of nitrogen are applied per 1000 ft /yr of lawn
                          o     most lawns are 5000 ft
                          o     1000 ft2 x 5 x 3 Ibs nitrogen = 15 IDS nitrogen/5000  ft2/yr
                          o     60% of nitrogen applied (15 Ibs) leached into groundwater
                          o     60% x 15 Ibs = 9 Ibs
                          o     nitrogen converted to nitrate form
                          o     9 Ibs nitrate nitrogen /5000 ft  lawn/yr leaches to groundwater
                                                                               A-8

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Many factors play a part in determining the quantity of nitrogen that teaches into groundwater.   When considering lawns the following fac-
tors appear to be of primary importance:


                 o      fertilizer application rate
                 o      type of fertilizer
                 o      soil type
                 o      precipitation/rates
                 o      type of plant/uptake potential
                 o      stage of plant growth
                 o      frequency of harvesting - cut and remove
                 o      nitrate in precipitation
                 o      conversion from nitrogen to nitrate
                 o      depth to water table


     Conversations  with  several  life long  residents  of Cape Cod suggest  that  the 3  lbs/1000 ft /yr figure utilized  in the Long Island 208
study might be excessive when discussing the average lawn on Cape Cod.  Golf courses on Cape  Cod, meticulously maintained apparently apply
on the average between 3 and 4 pounds of nitrogen per 1000 ft  per year.  It is highly unlikely that the average lawn on Cape Cod is
maintained to such rigorous standards.  For arguments sake we'll  assume that'the average lawn of Cape Cod receives  more than half the
fertilizer per unit area than that of a professionally maintained golf course.  In this case  a volume of 2 lbs/1000 ft  /yr could be used
as an average, stretching the application rate to 3 Ibs for green lawn enthusiasts.
                                                                Section 9  - Nitrate teachability

     Following a literature review and consultation with-people working in  the agricultural disciplines, it appears that there is a probable
range of values representing the percent of-nitrate leaching into groundwater through  vegetative cover and soils.   Nitrogen applied to the
lard surface from various fertilizers is presumed to be converted to nitrate and from  10-60%  of the volume initially applied will  reach
the groundwater as nitrate.  This large range of leaching nitrate is dependent  on the  factors listed above.  Values in the neighborhood of
45-50% might be most representative of the Cape Cod environment.   For the sake  of argument several  scenarios concerning fertilizer  applica-
tions are presented below:
                                                                               A-9

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                                                                        Table 9A
                                                                  Nitrogen Leachability
                     Application Rate
                    (lbs/1000 ft2/yr>
Average Lawn Size
   (ft2)
Nitrogen leaching
      (X)
Nitrate nitrogen volume
   available to
  groundwater (Ib/yr)
                            2
                            3
                            2
                            3
                            2
                            3
                            6
                            6
                            6
    6000
    6000
    6000
    6000
    5000
    5000
    5000
    5000
    5000
      10
      10
      45
      45
      60
      60
      10
      45
      60
       1.0
       1.5
       4.5
       6.75
       6.0
       9.0
       3.0
      13.50
      18.00
Assuming average lawn sizes to be approximately 5000 ft  (CCPEDC, 1979) these are the probable ranges of  nitrogen likely to  leach
into groundwater.  The application rate of 6 lbs/1000 ft /yr was used to demonstrate volumes that are generated by over-zealous or  in-
correct applications of lawn fertilizer.  As was mentioned earlier, grasses are most productive when a specific quantity of  fertilizer
is applied (per Table 7A).  Over fertilization may be harmful to the plants and results in excess nitrogen available to leach  into
groundwater.  In this case, more is definitely not better.

Lawn sizes and fertilizer application rates vary greatly from region to region and from home to home.  Local  conditions should be
evaluated to accurately predict the effects of lawns on groundwater quality.
                                                                         A-10

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                                                 Section  10  - Golf Courses



Fertilization rates for two golf course settings were available for review.  Both courses are situated on Cape Cod.

                                     Fertilization Rates  For Two Golf Courses on Cape Cod

                                                                                 Application Rate
                                              Area                              Ibs nitrogen/1000ft2/yr
                                           fairways                                  3.1-4.0
                                           greens                                    4.3-6.0
                                           tees                                      3.8
                                           rough                                     0-2.0

Since fairways generally constitute close to 90% of a golf course's total land area, the fertilizer application rates assigned to
fairways can be used to represent an overall application volume:

Ibs of nitrogen/acre/yr =

3.1-4.0 lbs/1000 ft2 X 43560 ft2/acre = between 135-17-lbs/acre/yr
                                            Section 11  - Recharge from precipitation


Thirty percent of about 5,000 groundwater samples from Cape Cod had nitrate notrogen concentrations of 0.05 mg/L  or less.   These ni-
trate concentrations are interpreted to result from recharge of precipitation in undeveloped areas without anthropogenic sources in the
recharge area.  Therefore, a recharge concentration, Cp, of 0.05 was used to calculate the nitrate load derived from'precipitation
for Cape Cod.  This value is significantly lower than the 2 year nitrate nitrogen average concentration of 0.26 mg/L measured in pre-
cipitation at Truro on Cape Cod.  The reduction of nitrogen concentration between precipitation and groundwater is apparently caused by
biological activity in the soil zone and at land surface.   Nitrogen loads in precipitation, soil,  and vegetative  conditions vary
greatly from place to place and nitrate concentrations values for recharge need to be developed from emperical  data representative of
the region for which the mass balance nitrate calculations are being made.


                                                                          A-11

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                                 APPENDIX B

        Directions for the Preparation of a Computerized Spreadsheet
                 for Automated Calculation of Nitrogen Loads
                               by H.  Gile Beye


    A  spreadsheet  to  calculate  nitrogen  loads can easily be set up with
Lotus  1-2-3  or  similar  software  packages.   A  working knowledge of the
software,  package  is  prerequisite to use of the spreadsheet.  The example,
shown  on  p.  B2 and described below, uses Lotus 1-2-3.   The spreadsheet is
set  up in seven parts.   Each part generates values to ultimately be used to
solve the nitrate-loading mass-balance equation.

    The  first  part  of  the  spreadsheet,  summary of liquid nitrate loads,
contains  data  necessary  to  calculate the sum of liquid nitrate load from
different  land  uses  and  also to calculate the total volume of water con-
tributed  by the sources (VI + V2+...+Vn).  The spreadsheet software package
does  not  accommodate  subscripts, so the terms in the formula are modified
from  those  presented in the text.  The calculations are based on long-term
averages  for  an  arbitrary period of 1 day.   The first column in part 1 of
the  spreadsheet  is  labeled SOURCE.   Listed in this column is the land use
source  of  nitrate.     The  next  column  is labeled FLOW.  The flow is the
discharge  from the source in gallons per day per person, seat, employee, or
other  unit.  The next column is labeled UNITS; it lists the number of units
in  each  land  use  category.    The  names of the units can be included to
clarify  the  FLOW  and UNITS columns, as shown in the example.  To do this,
set  up  a separate column for the names (Lotus does not allow letters to be
listed  in  the  same column as numbers that will be used for calculations).
The  next  column is labeled VOLUME;  the volume is calculated by multiplying
FLOW,  UNITS  and a conversion factor of 3.7853 (liters per gallon).  To set
up  this  equation,  type an opening (left) parenthesis,  the cell address of
the  first  value  in  the FLOW column, an asterisk (*),  the cell address of
the  first  value  in  the  UNITS  column, another asterisk, 3.7853, and the
closing  (right) parenthesis.  The resultant value appears in the first cell
of  the  VOLUME column.   It represents the volume of discharge per land use,
in  liters  per  day.    Copy the formula into the other cells in the VOLUME
column  (use  the  copy  procedure  in the Lotus menu).  If data are missing
from  the  FLOW  and  UNITS column, a zero will appear in the VOLUME column.
This  will be automatically replaced by a value when the data are entered in
those  columns.    The  next  column  is  labeled CONCENTRA TION.  It is the
concentration  of  nitrate  for  each  land use listed.  The final column is
labeled  LOAD.   It is the total nitrate load per land use per day.  This is
the  product  of  the  VOLUME and the CONCENTRATION columns.  To compute the
load,  type  an  opening  (left)  parenthesis, the cell address of the first
value  in  the  VOLUME  column,  an  asterisk, the cell address of the first
value  in  the CONCENTRATION column,  and then a closing (right) parenthesis.
Copy  this  formula  into  each  cell  of  the LOAD column.  Then, total the
VOLUME  column by typing at the bottom "@SUM  (cell address of first value in
column..cell  address  of last value in column)."  Type only the information
            Use of product or trade names does not consitute endorsement by
the authors or their agencies.

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within  the  quotation marks, for example @SUM(G9..G22).   This will give the
value  for  (VI  +  V2+...+Vn)  in  the  final  nitrate loading .mass balance
equation.  To total the LOAD column, follow the same procedure.

    The  second  part  of  the  spreadsheet, summary of solid nitrate loads,
solves  an  equation which computes the load of solid nitrate, in milligrams
per  day.    The  procedure for setting up this equation is the same as that
used  for  the  liquid  nitrate  equation,  except  there will not be a FLOW
column.    When the LOAD values have been calculated,•total the column using
the  @sum  procedure.    The  total solid nitrate load is added to the total
liquid  nitrate load for a total load (LI + L2 +...+ Ln).   Set this up as an
equation  on  a  separate  line  in the spreadsheet.  The equation is "(cell
address  of  total liquid nitrate load + cell address of total solid nitrate
load)".

    The  third  part  of  the  spreadsheet  is  the nitrate concentration in
recharge  from precipitation (Cr).   This varies from case to case.  Enter on
this line the value to be used for the current case.

    The  fourth  part of the spreadsheet converts the volume of pumpage from
well  (Vw) from English (inch, pound) to Metric units (meter, gram).  Set up
the  equation  with  gallons per day in one column and the conversion factor
(3.7853)  to  change  gallons  to  liters  in the next column.  In the third
column,  type  "(cell address of the gallons per day value * cell address of
the  conversion  factor).   The  resultant  value, pumpage in liters per day,
will appear in the cell.

    Part  five of the spreadsheet,  nitrate load of induced infiltration from
streams,  is  the product of the volume of induced infiltration from streams
(Vs) and the nitrate concentration of the induced infiltration (Cs).

    Part  six  of the spreadsheet,  nitrate load of drainage from Zone III to
Zone  II,  is the product of the volume of drainage from Zone II'I to -Zone II
(VIII) and the nitrate concentration of the drainage (CIII).

    Part  seven  of  the  spreadsheet,  concentration  at well, is the final
equation.    The  equation  using  the variables defined in this spreadsheet
looks like this:

Cw = [Cr * [Vw-Vs-VIII -(0.9 * (VI + V2+...+Vn))] +  [(LI + L2
+ ...+Ln) + (Vs * Cs) + (VIII * GUI)] /Vw.
Set  this  up by typing an opening (left) parenthesis, the cell addresses of
the  values  that correspond to the variables in the equation, and a closing
(right)    parenthesis.      In   Lotus   syntax   it   looks   like   this:
"C39*(F46-(0.9*122))  + (I35+C53+C60)/F46."  The result is the concentration
of nitrate in mg/L at the well.


                                      B2

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    The  advantage in using a spreadsheet to solve this equation is that
the  effects  of  additional  or  different  land  uses  can  be  easily
evaluated.    If  additions  are  anticipated at the time of spreadsheet
generation,  set up extra rows for them.  When changes are made, test to
be sure that accuracy in the solution of the equations is preserved.

    The  software  package  Lotus 1-2-3 was used for this example.  How-
ever,  a  similar  spreadsheet can be designed with any software package
that  has  the  capability  to  perform  mathematical  functions.    This
appendix  describes a general format for structuring data to solve equa-
tions  by  means  of  a spreadsheet.  The format can be modified to meet
the requirements of other spreadsheet software.
                                      B3

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SUMHAHY OF UATEW VOLUMES ANII NlTKATt LOADS CALCULATED  PEN  DAY  IN  THE  ZONE OF CONTRIBUTION
     1) Suiiart) of liquid nitrate loads tig/day)
     SOURCE
     (Land use!

     1/3 Acre housing
     High School
     Fast Food table seats
     Fast Food counter seats
     1 Acre housing
     Condoiiniuis
     Shopping Center
     Office Building
     Gas Station
     Church
     Hotel
     Hotel
     Hospital
FLOW

( gallons/ day 1
65
SO.
150
350.
65
65
60
15
500
3
75
75.
200
.00
00
.00
00
.00
.00
.00
.00
.00
00
.00
00
.00
•
UNITS
' - VOLUME - CONCENTRATION -
• (varies)
/people
/people
/seat
/seat
/people
/people
/eiployee -
/eiployee -
/island -
/seat
/people
/people
/bed
400
1000
70
10
200
120
50
25
2
200
40
160
60
people
people
•seats
seats
people
people '•' -
employees -
employees -
islands -
scats
people
people
beds
(liters)
98117
75706.
39745
13248.
49208
29525
11355
1419
3785
2271.
11355
15123
45423
.80 ..-
00 .-
.65 -
55 -
.90 -
.34 -
.10 -
49 -
.30 -
18 -
.90 -
60 -
.60 -
dg/L)
40
40.
40
35.
40
40.
40
40
40
40.
35
35.
35

.00 -
00 -
.00 -
00 -
00 -
.00 -
.00 -
00 -
.00 -
00 -
.00 -
00 -
.00 -
LOAD
lig)
3936718
3028240
1599826
463699
1968356
1181013
454E36
56779
151412
90847
397456
1589826
1589826


.00
00
.'00
.25
.00
60
.00
.50
.00
.20
.50
00
.00
                                             Total VOLUME (VI  + V2 +...Vn)  =     426887.21     Total  liquid LOAD=  16498230.05
     2) Smeary of solid nitrate loads tig/day)
     SOURCE
     Lawns 5000 sq. ft.
     Horses P 1200 Ib each
                               UNITS
                             (varies)
                                    100  launs
                                      6  horses
 NITRATE
  libs)

-   0.025 /lawn
-   0.027 /100 Ibs
          of aniial
CONVERSION
  (•g/lb)

     454000
     454000
     Total Nitrate LOAD,  liquid and solid coibined (LI + L2 f...Ln)  =

     31 (Crl- Nitrate concentration in recharge frot precipitation.

                                        0.05 ig/L

     4) (Vwl- Voluie of puaipage froi well
                                                                            Total  solid  LOAD*
                                                                              17706778.05
 LOAD
 dg)

1135000.00
  73548.00
                                                                                                 1208548.00
                        VOLUME   CONVERSION
                         IGPD)  (GPD) x 3.7853
                       1000000
                                      3.7853
                                                     L/day

                                                    3785300
5)  Nitrate load of induced infiltration concentration froi streais

    (Vsl- Voluis of induced infiltration froi streais
    ICs)- Nitrate concentration in induced infiltration

    IVs * Cs) =                    0.00 ig

6)  Nitrate load of drainage froi Zonelll to Zonell

    (VIII)- Voluie of drainage froi Zonelll into Zonell
    (CUD- Nitrate concentration of drainage froi Zonelll to Zonell

    (VITI * CIIII -                0.00 ig

71 (Cul- Concentration of nitrate at well

Cu = [ Cr * CV« - Vs - VIII - 10.9 * (VI + V2 +...Vnll ] + (Li + L2 +...Ln)

                     Cw=           4.72 ig/L
                                                                                     0.00 L
                                                                                     0.00 ig/L
                                                                                     0.00 L
                                                                                     0.00 ig/L
                                                                                     IVs x Csl + (VIII x CIIII / Vu
                                                            B-4

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                                   Appendix C



        List of Acronyms, Chemical Formulas and Mathematical Symbols Used

ACRONYMS

BOD:          5 day Biological Oxygen Demand
CCPEDDC:      Cape Cod Planning Ahd Economic Development Commission
GPD:          Gallons Per Day
MGD:          Million Gallons Per Day
MG/L:         Milligrams Per Liter
USEPA:        United States Environmental Protection Agency
WHPA          Wellhead Protection Area

Mathematical Symbols

C :      Nitrate concentration in individual sources (mg/L)

Cr:      Nitrate nitrogen concentration in recharge from precipitation (mg/L)

Cs:      Nitrate concentration in induced infiltration (mg/L)

GW:      Nitrate nitrogen concentration at well (mg/L)

'"'III'   Nitrate concentration of drainage from Zone III to Zone II (mg/L)

L^:      Nitrate nitrogen load in milligrams for individual septic systems

V :      Volume  of  water  used by each source before discharge to septic system
        (liters)

V ':      Volume of induced infiltration from streams (liters)
 s

Vw:      Volume of withdrawal from well (liters)

        Volume of drainage from Zone III into Zone II (liters)


Chemical Formulas

N:      Nitrogen
N2:      Nitrogen (atmospheric)
N2:      Nitrite Nitrogen
N03:    Nitrate Nitrogen
NHo:    Ammonia Nitrogen
NH^:    Ammonia Nitrogen (ionized)

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