EVALUATION OF ALTERNATIVE
    SECONDARY OZONE AIR QUALITY STANDARD!
               January 1979
    Strategies and Air Standards Division
Office of Air Quality Planning and Standards
    U.S. Environmental Protection Aqency
       Research Triangle Park, NC

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                      TABLE OF CONTENTS


Section                                                          Page
  1.0     Introduction
  2.0     Method of Analysis for Preliminary Estimate of
          Reduction in Yield for Commercially Important
          Crops ........................     2

  3.0     Preliminary Estimate of Ozone Damage to
          Commercial Farm Crops ................     9

  4.0     Preliminary Estimate of Ozone Damage to
          Other Vegetation ..................     14

  5.0     Examination of Available Evidence on Yield Reduction
          in Field Exposures ..................   16

  6.0     Ozone Damage to Materials and Reduction in
          Visibility .....................     19

  7.0     Summary and Conclusions ...............     21

          References .....................     23

          Figure 3-3 .....................     24
          Table 1 .......................     25
          Table 2 .......................     26
          Table 3 .......................     28
          Table 4 .......................     32
          Table 5 .......................     33
          Table 6 .......................     34
          Table 7 .......................     35
          Table 3 .......................     36

          Attachment 1
          Attachment 1
          Attachment 3
          Appendix A
          Appendix 3
          Appendix C

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1.0  Introduction
     It has been found that ambient concentrations of ozone are re-
sponsible for economic losses that arise from accelerated aging of
certain materials (e.g., rubber cracking, dye fading, and paint weathering)
and damage to vegetation (e.g., foliar injury, growth reduction, and yield
reduction), and are associated with visibility degradation in some
areas. This analysis attempts to quantitatively assess the difference in
damages associated with alternative secondary ozone standard levels.
     It should be emphasized that the estimates for reduction in damage
to forest products, farm crops, and ornamentals are primitive due to
the extremely limited data base correlating yield reduction and short-
term low-level ozone exposure.  The analysis used a first-cut approach
to obtain an upper-boundary estimate on reduction of damage for major
farm crops.  Damage was estimated both in terms of growth and yield
reductions and economic losses.  Economic losses were estimated to
provide an indicator of damage across crop types.  Reduction in ozone damage was
estimated for 90% of the major farm crops for which the U.S. Department
of Agriculture (USDA) recorded economic data (3).  EPA consulted with
several plant pathologists to obtain an improved estimate for reduction
in damage.  In addition, the available evidence relating long-term ozone
field exposures to yield reduction in commercial crops and indigenous
flora were examined and the implications of these studies for the selection
of an appropriate secondary standard level were explored.  Finally, for
materials and visibility, EPA concluded that there is no identifiable difference
in economic damage between the alternative standards.
                                 1

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 2.0 Method of Analysis  for  Preliminary  Estimate of Reduction  in Yield
     For  Commercially  Important Crocs
     The  criteria  document  (2) estimates that damage to vegetation
 resulting from current ambient oxidant exposures may be approaching
 $300 million  (1974 dollars)  at the  farm  level.  The goal of this analysis
 is to  estimate the incremental reduction in yield that might result from
 adoption  of alternative  annual peak hourly average ozone secondary standards
 (0.08  ppm, 0.10 ppm, or  0.12 ppm).  For the standard levels under considera-
 tion,  the available evidence indicates that the air quality parameter
 that will  determine the  amount of vegetation injury is the 6-  to 3-hour
 average concentration which  accompanies the permitted hourly average
 peaks.  SPA analyzed 123 site-years of ozone or total oxidant  data from
 stations  that were diversified in nature, ranging from "center-city -
 industrial" to "rural -  agricultural".  The results of this analysis are
 presented  in Attachment  1.   Annual-asak 3-hour ozone (or oxidant)
 concentrations are plotted as a function of annual peak hourly average
 concentrations in  Figure 1 of that attachment.  As can be seen from
 the figure, there  is a considerable- variability in this relationship. ;?A
 chose  to  use an upper-boundary cur/e which envelops most of the data
 in Figure  1 to establish the maximum 3-hour average cancantraticn "hat
 could  be exoectad  to occur if a given hourly average standard  level
were achieved.  Thus a 0.08  ppm hourly average standard level
should prevent 0.07 ppm, 3-hour average, from being exceeded more

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than once per year.  Similarly, a 0.10 ppm hourly average standard level
should prevent 0.09 pom, 8-hour average, from being exceeded and a 0.12
com hourly average standard level should prevent 0.10 ppm, 8-hour
average from being exceeded more than once per year.  The following pre-
liminary analysis is based upon two comparisons:  (1) allowing only one
0.10 ppm/8-hour versus 0.09 ppm/ 8-hour peak exposure oer year and (2)
allowing only one 0.09 ppm/8-hour versus 0.07 ppm/8-hour peak exposure
per year.
     In order to evaluate the reductions in yield or growth for alternative"
standard levels, it is necessary to have a dose-response function relating
ozone concentrations and duration of exposure to percent yield reduction
or damage.  Larsen and Heck have developed a mathematical model that
quantitatively predicts the extent of foliar injury in certain classes
of crops due to single, acute exposures as a function of ozone concentration
and exposure time (6).  Dr. Ralph Larsen (U.S. EPA) has applied this mathematical
node! to the 1135 data points evaluated in the 1977 National Academy of
Sciences report (4).  The results of this analysis are presented in
Attachment 2 and utilized in Tables 2 and 3 of this report (pp. 26-31).
     It should be cautioned that foliar injury is an imprecise measure
of the effect of ozone on Plant growth and/or yield.  The Con/all is
Environmental Research Laboratory (CERL) of U.S. EPA has recently funded
a case study in California to evaluate the economic effects of air
pollution on agricultural crops.  The study will utilize data
which are currently being generated to measure yield effects.  The
objective of the study is to develop a generalized economic methodology

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 for  evaluating  direct  and  secondary  impacts on agricultural crop
 yields.   Unfortunately,  the  results  of this recently  initiated
 study will not  be  available  for  some time.   However,  section 5.0
 of this  report  examines  the  available evidence relating yield
 reduction and growth parameters  for  commercial crops  and native
 vegetation to seasonal ozone doses.
     For the purposes  of this analysis, a first-cut estimate was
 made based on the  assumption that the acute foliar injury response
 to the peak exposure permitted by the standard can be  used to predict
 biomass  (growth) and yield reduction caused by chronic exposure to
 ozone levels up to and including the peak value permitted by the
 standard.   Regarding  this assumption, Or. Walter Heck (Research
 Leader,  Southern Region, USDA, Raleigh, NC) estimated that the ratio of
 the percent damage (yield reduction) to acute foliar  injury percentage
 may be as low as 1:2 or  as high as 1:1 (see Attachment 3).
     In discussions with plant pathologists arcund the country,
 EPA was cautioned that while there appears to be a fair amount of
 correlation between foliar injury percentage and biomass reduction,
 there is a great degree  of variability in the relationship between
biomass reduction and  reduction in yield (the economically imoortant
parameter for most craps),   "or example,  significant damage or yield
reduction can occur in some crops without any noticeable foliar
injury.   Conversely,  it  is  possible to have significant foliar

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injury and biomass reduction and yet have no noticeable effect on
yield, as illustrated in Table 4.  The timing of an air pollution
episode in the crop's life cycle and the presence of other environ-
mental stresses (e.g., drought conditions) are often crucial
determinants of how much yield and/or biomass reduction will  result
from a given degree of foliar injury.
     Another important caveat is the fact that the Larsen and Heck
equations were derived from studies which generally exposed plants in
greenhouses under the most likely conditions to produce injury "(e"."g.V~~
high humidity, high soil moisture, and medium temperature).  The levels
of injury suggested by the Larsen and Heck model  almost certainly
exaqaerate the amount of damage for the significant portion of the U.S.
crop which is grown under less sensitive conditions (e.g., low humidity,
low soil  moisture).  These less sensitive conditions are particularly
found in the central and northern plains regions  of the United States.
     The commercial crops studied are divided into the following categories
depending upon which part of the plant is of economic value:   foliar
(tobacco, hay), seed (corn, wheat), root (potatoes, onion) and
fruit (oranges, tomato).  For foliar type crops it is assumed that
there is no threshold, i.e., any foliar injury percentage will  result
in some yield reduction.  However, for non-foliar type crops, the
assumption made is that only foliar injury greater than 5 percent will
lead to yield reduction.  The selection of a 5 percent threshold value

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 is a conservative estimate based on the comments  of several  researchers
 to the effect that 5 to 20 percent foliar injury  is usually  required
 before there is a detectable reduction in biomass and/or yield  in
 sensitive plants.
      Using the above assumptions,  a percent_damage (yield  reduction)
 is determined using the foliar injury  data from Attachment 2  for each
 major commercial  croo known to be  sensitive to low ozone levels.  The
 difference in oercent damage associated with alternative standard
 levels is listed  in Tables 2 and 3  as  A	% damage.   However,  in
 order to  compare  damages  across  crop types, EPA used  the economic
 indicator of crop values  as a convenient measure  or surrogate for
 yield reduction effects.
      The  daca needed  to enable conversion of i  *  damage to a dollar
 measure are:
      (1)   the economic  value  of  production of each  crop at the farm
           level;
      (2}   the percentage  of each croo  that is of a  sensitive or
           intermediate  cultivar  (i.e.,  variety).
      The  aroduction value  of  each major crop is obtained frcm the U.S.
 Department of Agriculture  (3)  and is in  terms of 1377 oroduction and
 dollars.  A  first-cut, systematic estimate of the share of :he total
 crop  that is  of a sensitive  (or  intermediate)  variety is calculated by
 one of two methods.  3oth methods rely on Table 11-24. in the National
Academy of Sciences (NAS)  ozone document (*•}  which categories the
 varieties examined by olant researchers as sensitive, intermediate,  or

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resistant.  Where four or more cultivars for a crop are listed,  it is
assumed that the percent of sensitive (intermediate) cultivars for that
crop (as reported in Table 11-24) is equivalent to the sensitive
(intermediate) fraction of the crop oresently being grown on the nation's
farms.  Therefore, since 12 cultivars for oats are listed and 5  of them
are in the sensitive category, then 6/12 or 50 percent of the oats grown
are assumed to be of the sensitive variety.  Where fewer than 4  cultivars
of a given crop are listed, a percentage of sensitive cultivars  for that
tyoe of crop (i.e., seed, foliar, fruit, or root)  is used to determine
the share of the crop that is sensitive.  For example, fewer than 4
cultivars are listed for sweet corn in Table 11-24, but 24 percent of  the
seed-type cultivars fall in the sensitive category.  Therefore,  it is
assumed that roughly 24 percent of the sweet corn  grown is of a  sensitive
variety.
     To put the above assumptions into proper perspective it should be
recognized that the commercial lifespan of most cultivars is no  more
than ten years, and indeed can be considerably shorter.  Many of the
cultivars listed in the MAS tables are either no longer grown, or are  of
only minor commercial  sianificanca.  Nonetheless,  for a preliminary
estimate of ozone-related crop damage EPA chose to use the NAS breakdown
of cultivar sensitivity as a rough approximation of the sensitivity of
crops presently being grown on the nation's farms  due to the limited
data base and resources available for this study.

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      Utilizing the above estimates and -the assumptions upon which they
 are based, the difference in economic loss between two alternative ozone
 standards is calculated by (1) multiplying the difference in percent damage
 for the sensitive crops, the share of the crop that is sensitive, and
 the economic value of the total production at the farm level for each......
 crop and (2) multiplying the difference in percent damage for the intermediate
 crop, the share of the crop that is intermediate, and the economic value
 of the total production at the farm level for each crop, and (3) summing the
 products for all  major commercial  crops.
[Differential
 Annual  Economic
 Loss,  in 1977
 dollars and
!oraduction
n
d * Damage
for sensi-
tive crop i
n !~i % Damage
* Z for interme-
1=1 diate crop i
V -i
 * of crop that
jjs sensitive

\% of crop that !
jis intermediate
H~              J
r!977 value
 of production
 for crop i
| 1977 value   1
 of production?
                                                                 ror croo
      In  determining the reduction in yield and growth associated with  a
 0.07  ppm/3-hour as  opposed to  a  0.09 ppm/8-hour exposure  (Table  2),  it
 was found that  for  crops of intermediate  sensitivity  the  A "  damage  is
 zero  or  nearly  zero for the crops considered.   Thus no loss data for
 intermediate  crops  appears in  Table  2.  However,  in comparing a  0.09
 ppm/3-hour and  a 0.10  ppm/8-hour exposure (Table  3),  ozone carnage to
 intermediate  craps  was  included  because the  5  percent injury  threshold
 is exceeded for some crops for a peak exposure greater than 0.09 ppm/
 3-hour average.

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     The above estimate of the annual  difference in economic loss
associated with alternative standards  assumes that production will
remain at 1977 levels and that the value or price per unit for each crop
would remain unchanged even if more of the crop were produced due to
reduced ozone levels.
3.0  Preliminary Estimate of Ozone Damage to Commercial  Farm Crops
     Using the above-mentioned assumptions an upper-boundary (worst-
case) estimate was made to identify which crops might be responsible for
the bulk of the reduction in damages.   It was found that the
vast majority of the estimated loss was accounted for by the following 6
crops:  corn for grain, cotton, hay, soybeans, tobacco,  and wheat.   In
addition, the systematic approach outlined above was not helpful  in
providing even a first-cut estimate for several important crops.
Therefore, in order to obtain more realistic estimates of the reduction
in damage to these major farm crops associated with alternative standards,
various plant experts were consulted with on the assumptions used in the
initial analysis and the total values  obtained.  3ased on these con-
versations, the first-cut estimates were revised for several crops, and
original estimates were made for several  others.  These improved results
are shown in Tables 2 and 3. The following oaragraphs detail the bases
for these revisions.
     Dr. Al Heagle (Plant Pathologist, U.S. Department of Agriculture,
Raleigh, NC) has suggested that the percent of field corn (corn for
grain) that is of a sensitive variety is probably on the order of one-
half of the percentage of sweet corn that is sensitive.   Since the
systematic estimate of this percentage was the same for both crops,
this recommendation lowered the damage estimates for field corn by

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 50 percent from the first-cut estimate.   Tables 2 and 3 have been
 revised to incorporate this suggestion.
      The first-cut estimate of the incremental  reduction in damage to
 tobacco was  from $94 to S190 million (0.09  ppm/S-hour vs.  0.07 ppm/8-hour).
 This  was based on the systematic  estimate that  70 percent  of the  tobacco —
 crop  is of a sensitive variety.   This  estimate  is almost certainly too
 high.   In North Carolina,  where nearly 50%  of the U.S.  tobacco crop is
 grown,  the maximum annual  ozone (weather fleck) damage  in  the period .1_9_7_3^_.
 1977  occurred in 1976.   The estimated  disease loss was  only 0.38  percent
 or S3.555 million for that year (5).   Or. Furney Todd of M.C.  State
 estimated in personal  communications that about 23 percent of the North
 Carolina flue-cured tobacco crop  (types  11-H)  consists  of the variety
 Speight 3-23 and that this variety was the  most sensitive  of the  flue-
 cured types  presently grown.   However, he believed that  Soeight G-23
 would fall  in  the intermediate category  using the MAS classification
 system.  Or.  Todd also  mentioned that most of  the ozone  (weather ^lec!<)
 damage  was to  the lower leaves of  the  tobacco plants.   There  is currently
 a  surolus  of these  leaves  on  the market  and farmers are  being  encouraged
 to destroy these leaves.   Thus at present there is little,  if  any,  ozone-
 related  economic  damage  to  the tobacco crop in  North  Carolina.
     For Burley  Type  31  tobacco, which makes up  roughly  31  percent  of
 total  tobacco  croo, Or.  Hadden (Univ. of Tennessee) estimated  that  the
maximum weather  fleck  (ozone) damage suffered in  recent years was  around
0.5 oercent  of the croo.   Since 3urley Type 31  and flue-cured  types  11-
1-J- make UD 91 oercent of the total tobacco crown  and are of intermediate

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or resistant susceptibility to ozone,- the maximum fraction of the
tobacco crop that could be of a sensitive variety is 9 percent.  Tables 2
and 3 have been revised in accordance with this upper-boundary estimate.
     Dr. Todd also estimated that 26 percent of the total  tobacco crop
nationwide was of an intermediate varie±y.  This value is  used in  -   -
generating the reduction-in-loss estimate in Table 3 for intermediate
sensitivity tobacco.
     We also consulted Or. H.E. Heggestad of the U.S. Department of
Agriculture at Beltsville, MO regarding his work with cotton.  While he
noted that some cultivars were found to be more sensitive  than others,
he offered his judgment that no cotton tested would show a difference in
yield for either of the alternative standards under consideration.
Tables 2 and 3 reflect his judgment.
     EPA also sought expert advice on the impact that environmental
factors (such as soil moisture and type, humidity, tamperatura,  etc.) as
well as the timing of an ozone pollution episode in a crop's life cycle
might have on the yield response of that crop.
     It is generally recognized that the timing of a peak  pollutant
exposure in a crop's life cycle can have a considerable impact on the
response of that crop to the pollutant.  Plant pathologists have shown
that for non-foliar type crops the most susceptible period occurs from
onset of flowering through fruit development.  According to Dr.  Heagle
(U.S. Department of Agriculture), this period is highly dependent on
the crop.  For corn, soybeans, and wheat, however, he indicated that
the most susceptible period is about 1 month.  Since peak  man-caused
                                   11

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 ozone values typically occur in the 5-month period from May through
 September (see Table 1 in Attachment 1), it seems reasonable to
 hypothesize that there is a 20 percent chance that in  a particular
 location one of these crops might sustain yield reduction  losses  •
 as a result of the peak ozone level.   EFA has amended  the  results  of
 its preliminary analysis in accordance with this  estimate  by incorporating*
 this correction factor for seed and fruit crops in Tables  2 and 3  in the
 column listing the percentage of the  crop that is sensitive (or inter-
 mediate) .	
      Environmental  conditions such  as  soil  moisture, humidity,  and
 temperature  are known  to be important  factors  in  determining the
 response of  plants  to  pollutant challenges.   Several experts cautioned
 that foliar  injury  studies such as  these on which Tables 2  and  3
 are based  are  generally  conducted in greenhouse chambers under  ex-
 perimental conditions  which,  as nearly  as  is  possible,  are  optimal  for
 producing  injury.   This  means that  the  results  presented in  Tables  2  and 2
 are an overestimate of the damage associated with the alternative
 standards, since the analysis  assumes  that  environmental conditions
 throughout the  nation  are  optimal for producing injury when  the peak
ozone  levels occur.  Such  is  clearly not  the case,  since tne  3reat
 Plains, Mountain, and  Southwest regions of  the  country generally have
environmental conditions  (dry soil and  low humidity) which are less
conducive to ozone-related damage than  are the  humid, moist-soil regions
of  the East and South  and  the irrigated farm areas of California.   The
estimates of damage for crops such as wheat which are largely grown  in the

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less susceptible regions of the country are consequently inflated.  EPA
was not able to modify Tables 2 and 3 to correct for this bias, however,
because the available data do not permit a reasonably accurate breakdown
of the nation's crop production into areas of differing environmental
conditions in relation to pollution damage susceptibility.
     Several researchers emphasized the fact that there are alternative
approaches to the reduction of ozone-related damage to commercial  crops.
One option is for the agricultural sector to substitute more resistant
cultivars for susceptible ones in regions of the country where ozone
levels are high.  Researchers are developing new cultivars  that are
specifically bred to be more resistant to air pollutants.  In some cases,
chemical protectants can be applied to sensitive crops to reduce or
eliminate ozone-related damage.
     It should, however, be realized that the alternatives  described
above also involve costs.  The costs associated with research, application
and testing of chemical protectants, changes in harvesting  equipment and
procedures, reduced quality or yield for some of the substitute cultivars,
etc., would have to be calculated for a complete and thorough cost-
benefit analysis.  In addition,  the question of equity would have to be
addressed, for it is the farmer who would bear the additional expense
associated with the pollution generated by industry and automobiles.
Que to the limited data available, EPA does not have the ability to
address this issue in any greater detail at this time.
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      Where possible, Tables 2 and 3 have been revised to incorporate the
 suggestions of the plant experts.consul ted.   Consequently,  EPA believes
 that these tables represent the best estimates  that can presently be made
 using the foliar injury data base to compare the  nationwide reductions  in
 yield of commercially important crops associated  with alternative short-term
 (annual  peak hourly average) secondary ozone standards.  The results of  this
 preliminary analysis indicate that the incremental  damage between a  0.12 ppm
 peak hourly average standard and a 0.10  ppm  peak  hourly average  standard
 ranges  from SO.14 to $0.29  billion per year, while  the  incremen-tal--4am*c-e
 between  a  0.10  ppm and a 0.08 ppm standard ranges from  SO.18 to  SO.36 billion
 per  year.   Compared with the 1977 nationwide total  of crop  production evaluated
 in -his  analysis,  S50.5 billion per year, these incremental  damages  are  G.3-
 0.5% and 0.4-0.7*,  respectively.   Because the analysis  was  net corrected for
 temperature,  humidity and soil  moisture, these estimates  ire conservative,
 tending  to  overstate the potential  impact.   Given the uncertainty in  the data
 and  the  conservatism in the  estimates, EPA does not  consider these -impacts  to
 be significant.
 4.0   Preliminary  Estimate of Ozone  Damage to  Other Vegetation
      The preceding  section presented  quantitative estimates  of the reduction
 in damage to  commercial  farm crops  which would result from  attainment of
 alternative ozone standards.   It  should be realized  that  current  ambient
 ozone levels  also cause  damage  to our national forests  and  parks, to  commercial
 timber growth, and  to commercial  and  home-grown ornamentals.
      It is very difficult to quantify adequately the  importance of natural
 ecosystems to the public welfare, and consequently to provide -nonetary estimates
of the impacts of oxidant pollution on natural ecosystems. While  there have

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been important advances made in the economic methodology to measure the
benefits of or damages to natural ecosystems (e.g., willingness-to-pay
approaches), the state of the art is not sufficiently developed to
distinguish the incremental difference involved with the alternative
ozone standards being considered.
     Using the systematic methodology discussed previously for farm  	
crops, a crude (worst-case) estimate can be made of the maximum reduction
in damage to all commercial forestry and ornamental products associated
with the alternative standards.  In 1972, the total value for_all_j:ommercial
forestry products was 32.9 billion.  If the percentage of the sensitive
trees grown is equivalent to the fraction of tree species listed in
Table 11-24 (reference 4) that are sensitive (20") and the difference in
damage for the 0.09 pern vs. 0.07 ppm/8-hr levels is about 12 percent
(the value obtained using the all-sensitive-trees equation for foliar
injury data), then for the case where percent yield reduction is assumed
to equal percent foliar injury, the annual reduction in damage is:
     (20%) (12S) (32.9 billion) = 370 million (1972 dollars) or 2A%
Thus, the range of the estimate given in Table 2 is 335-70 million per
year (0.09 ppm/8-hr vs. 0.07 ppm/8-hr).
     A similar crude estimate can be made for commercial ornamentals and
shrubs using the all-sensitive-plants equation:
     (92) (8%) ($1.3 billion) = $9 million (1974 dollars) or Q.7%
     (0.09 ppm/8-hrs vs. O.Q7 ppm/8-hr).
     The range of the estimated reduction in damage to ornamentals would
be $5 - 39 million per year for exposure to a 0.07 ppm/8-hour-average
as opposed to exposure to a 0.09 ppm/3-hour-average.
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      The preceding estimates  contain  the  same  conservative  assumptions
 discussed in section 3.0 for  the farm crop  analysis.   Consequently,
 these estimates  also tend to  overstate the  potential  impact.
      Quantitative  estimates of damage to  home-grown crops,  ornamentals,
 and shrubs  were  not made due  both  to  the  lack  of  information on how much
 of each  type of  vegetation is  grown and the difficulty of placing an
 economic value estimate  on damage  to  shrubs and plants. These plants may
 be damaged  by ozone such that  their appearance is marred but still the
 plant  continues  to  survive.  Since these  plants are not subject to any
 market mechanism,  it is  very difficult to place an economic value on the
 partial  damage that is caused  by exposure to ozone.
 5.0  Examination of Available  evidence on Yield Reduction in Field Exposures
     Section  3.0 detailed specific revisions which were made in the
 first-cue,  systematic estimate of croo damage associated with alternative
 ozone  standards, based a a*the  suggestions received from several  plant
 experts.  However,  a more basic criticism of this approach was offered
 by several  researchers in relation to  its underlying assumotion that
 greenhouse  foliar injury data  is a valid  indicator with which to project
yield  reduction in  crops excosed in the field.   As was noted previously,
the environmental conditions  in the field may not be nearly so optimal
for producing injury as those  typically used in greenhouse chamber
studies.
     In order to determine whether or not croo  yield reductions  would
actually  occur at any of the  alternative standards, £?A evaluated  the
                                 15

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ozone field exposure data currently available in the criteria document
(summarized in Table 5) and in recent unpublished studies  (7,8,9)  by  Dr.
A. S. Heagle.  These data are not directly relevant to  the issue of
comparing alternative peak hourly average standards, since they  relate
crop yield reductions to the long-term (growing season)  mean  of  the
daily maximum 6- to 7-hour-average ozone concentrations.   Nevertheless,
EPA believes that some useful conclusions can be drawn  from an examination
of this evidence in conjunction with available air quality data.
     The five studies in Table 5 all demonstrated statistically  signi-
ficant growth and yield reductions in commercial varieties of alfalfa,
soybean, and sweet corn or in pine seedlings when the seasonal mean of
the daily maximum 6-hour-average ozone concentrations was  0.10 ppm. In
these studies ozone was added to a charcoal-filtered airstream to  produce
the exposure dosage.  Of the three studies in which crops  were exposed
to a seasonal mean of 0.05 ppm, one demonstrated statistically significant
growth reductions in alfalfa.  In this study of 0.05 ppm,  the alfalfa
did not receive any nitrogenous nutrients; the ozone exposure apparently
affected the ability of the alfalfa to symbiotically fix atmospheric
nitrogen.  The bulk of this evidence suggests that for normally  fertilized
agricultural crops, the threshold for significant growth or yield  reductions
lies between 0.05 and 0.10 ppm for a seasonal mean of the  daily  maximum
6- to 7-hour-average concentrations.
     Or. Heagle's studies (7,8,9) examined the effect of long-term ozone
exposures on the yield of several commercial varieties  of  field  corn,
spinach, and winter wheat grown in open-top field chambers.  The first

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 two studies have been accepted  for publication  and  the  third study will
 be submitted shortly; these  studies are  attached as Appendixes A, 3, and
 C.  The  exposure  protocol  in  these  studies  differed  from  those discussed
 above  in  that the crops  received different ozone doses by the addition
 of different but constant concentrations of ozone to non-filtered ambient
 air for 7 hours  per  day  (approximately 0930 to  1630 hours EOT).  The
 results of these studies  are summarized  in Table 5, along with an ambient
 exposure  study on tomatoes by O.C.  Maclean and  R.E. Schneider (10).  On
 balance,  this evidence indicates a  threshold for significant yield  -• 	 -
 reductions  in several commercial crops between  0.06 pom and 0.10 ppm for
 a  seasonal  mean  of the daily maximum 7-hour average ozone concentration.
 It  is particularly interesting  to note that in  the field corn study (7),
which had a  significant yield response threshold between 0.11 and 0.15
ppm seasonal mean  7-hour-average, the foliar injury response threshold
was less  than 0.07 ppm seasonal mean, demonstrating that field corn can
                                                *
sustain some injury with no loss of yield.
     The rationale for selection of the seasonal mean of the daily
maximum 7-hour-average ozone concentration  as  the air quality parameter
with which to correlate yield reduction caused by ozone exposures is
presented by reference 3:
     Previous methods of describing ambient pollutant doses  include
     seasonal means, weekly means,  24-hour  means, ppm hours, peak hourly
     means, and a number of hours above a set  concentration.  None of
     these methods adequately describe the  dose from a biological standpoint
     because pollutant dose - plant response curves  are .not  linear and
     plants may respond differently to pollutants at different  times
     during growth.  Doses have also been described  in  terns of oercentage
     of time or number of hours above set concentrations  intervals,  but
     neither of these metnoas consider the  timing of exposure to  given

-------
     concentrations in relation to plant growth stage or time of day.
     In our experience, the 7 hour/day (0930 to 1530 hour EOT) and 24
     hour/day means, adequately characterize the dose from a biological
     standpoint.
     The connection between this long-term dose characterization and the
annual peak hourly average standard format under evaluation is difficult
to establish definitively.  A few examples may be cited:  In Raleigh,
North Carolina a peak hourly average of 0.14 ppm was observed when the
ambient air seasonal mean 7-hour-average concentration in Dr. Heagle's
winter wheat study (9) was 0.06 ppm.  A peak hourly average oxidant
value of 0.20 ppm was measured in Yonkers, Mew York in conjunction" with"
the 0.07 ppm seasonal mean 7-hour-average concentration calculated from
reference 10.  The results of an analysis of EPA's air quality data
files presented in Table 2 and Figure 2 of Attachment 1 demonstrate that
the relationship between peak hourly average values and long-term mean
7-hour-average concentrations is quite variable.  However, the data do
seem to indicate that attainment of a peak hourly average standard level
of 0.12 ppm would prevent a seasonal mean daily-maximum 7-hour-average
concentration of O.Q6 ppm from being exceeded.  As a result, EPA concludes
that the evidence currently available does not suggest that a peak
hourly average ozone secondary standard any lower than 0.12 ppm is
necessary on the basis of ozone-related yield reduction effects in
vegetation.
6.0  Ozone Damage to Materials and Reduction in Visibility
     Materials damage resulting from ozone can be described as an acceleration
of aging processes; for example, rubber cracking, dye fading, and paint
weathering.  In contrast to the effects of ozone on vegetation, these

                              19

-------
 effects  are linearly dependent on the total  ozone dose  sustained  by the
 material.   As  a result,  the annual  average concentration  will  determine
 the rate  at which  material  is  damaged,  as  discussed  in  the  criteria
 document  (2).   Any nonzero  ozone  concentration  (including natural  background
 levels) will contribute  to  the deterioration  of sensitive materials over
 a  sufficient exposure duration.   While  peak  1-hour ozone  concentrations
 in  urban areas  tend to be considerably  higher than in rural  areas
 remote from man-made emission  sources,  the annual average concentrations
 observed in these  areas  are  essentially the same, as illustrated  in
 Tables 7 and 3.  This finding  is  believed  to  be  due  to  the  impact  of
 very low urban-area nighttime  ozone concentrations on the annual  average
 values; nighttime  ozone  levels  in remote areas  are not  reduced as  much
 from the daytime levels  due  to  the absence of scavenging  by  man-made
 urban pollutants (e.g.,  nitrogen oxices and hydrocarbons).   As peas ozone
 levels in urban areas are Deduced through  control of man-made pollutants,
 scavenging  will also  be  reduced resulting  in  little  if  any change  in the
 annual average.  Consequently, no effect-based  rationale  can be of-ersd
 to  -decide the level  of the secondary  standard needed to protect materials.
Accordingly, a secondary standard more stringent  than the primary  standard
does not appear necessary on the basis of ozone damage  to materials.
     The criteria document states that there  is a limited amount of data
suggesting  an association between ambient ozone and visibility degradation,
particularly in the Los Angeles area.   The final version of  the criteria
document contains a diagram  (Figure 3-2, attached) that depicts a  gcod
correlation for the Los Angeles basin between visibility reduction  (as
measured by the extinction coefficient)  and Z-'icur-average maximum  ozone

                                  20

-------
concentrations.  However, inspection of the data reveals no obvious
relationship between visibility reduction and maximum ozone concentrations
at and below 0.12 ppm.  Furthermore, the criteria document states that
the Los Angeles evidence on the impact of ozone-related control  measures
on haze does not have universal validity, as indicated by the case of
Denver, for example, where the haze problem appears to be caused by
primary aerosols.  On the basis of the available information, EPA does
not believe that a secondary standard more stringent than the primary
standard is necessary to prevent visibility deterioration.  	
7.0  Summary and Conclusions
     This report has produced a quantitative estimate of the yield
reduction impacts of alternative peak hourly average ozone standards
based on the foliar injury data base.  Several experts questioned the
validity of this analysis because of its underlying assumption that
greenhouse chamber foliar injury data is a reliable indicator of yield
reduction in field crops.  Because of these criticisms, EPA believes the
preliminary estimates given in Tables 2 and 3 do not provide an accurate
indication of the damages associated with the alternative standard
levels considered, but rather are considerable overestimates.
     Consequently, EPA has evaluated the data currently available in the
criteria document (summarized in Table 5) and in other recent studies
(summarized in Table 6) relating long-term ozone field exposures and
yield reduction in commercially important crops and indigenous flora. On
the basis of this information and an examination of air quality data,
EPA has concluded that there is currently no evidence indicating the

-------
need for a peak hourly average ozone secondary standard any lower than
0.12 ppm on the basis of ozone-related yield reduction effects  in vegetation,
     Furthermore, EPA's assessment of the available information regarding
materials damage and visibility deterioration indicates that a  secondary
standard more stringent than 0.12 ppm is unnecessary to protect against
these effects as we!1.
                              22

-------
                              REFERENCES
1.   U.S. Environmental  Protection Agency,  Assessment  of  Welfare
     Effects and the Secondary Air Quality  Standard  for Ozone, June
     1978.

2.   U.S. Environmental  Protection Agency,  Air Quality Criteria for
     Ozone and other Photochemical Oxidants,  Publication  No.  EPA-600/ 8-
     78-004, April 1978 (preprint).

3.   Department of Agriculture, Crop Values 1975-1976-1977, Washington,
     DC, January 18, 1978.

4.   National Academy of Sciences (MAS),  Ozone and Other  Photochemical
     Oxidants. MAS, Washington, DC,  1977.

5.   Todd, Furney, Extension-Research on  Wheels;  Summary Report of  1977
     Data, North Carolina Agricultural  Extension  Service, November,
     1977.

6.   Larsen, R.I. and W.W.  Heck.   "An air quality data analysis system
     for interrelating effects, standards,  and needed  source  reductions:
     Part 3.  Veaetation Injury."  J. Air Pollution  Control Assoc.
     26(4): 325-333, 1976.

7.   Heagle, A.S., R.B.  Philbeck, and VI.M.  Knott, "Thresholds  for  injury,
     growth, and yield loss caused by ozone on field corn hybrids."
     Phytopathology, 1979 (In Press).

8.   Heagle, A.S., R.B.  Philbeck, and M.S.  letchworth, "Injury and yield
     responses of spinach cultivars  to chronic doses of ozone  in open-
     top field chambers."  Journal of Environmental  Quality,  1979  (In
     Press).

9.   Heagle, Allen S., Suzanne Spencer and  Michael 3.  Letchworth,  "Yield
     Responses of Winter Wheat Cultivars  to Chronic  Doses of  Ozone."
     (Draft, to be submitted for publication  in 1979).

10.  Maclean, D.C., and R.E. Schneider.  "Photochemical oxidants  in
     Yonkers, Mew York:   Effects on  yield of  bean and  tomato." J.  Environ.
     Qua!. 5_(1): 75-78, 1976.
                              23

-------
   14
   10
i_   3
•Z  4
u
X
LU
       BSC3t AT PEAK OZONE (BASSO ON TWO HOUR
      AVERAGED OATA FROM LOS ANGELES AREA)
              (SUMMER 1973)
   (SUMMER 1972)
        0 ROUBIOOUX (RIVERSIDE)   * PASADENA
         A WESTCOVINA
         a POMONA
         • DOMINGUE2 HILLS
            (TORRANCE)
• RIVERSIDE
» POMONA
* HAR8OR FvVY.
  (DOWNTOWN LA)
O 3LIMP FLIGHT  '
  19/6/73!
  1315-1500 PST
                                        BLIMP    _
         NO AcHOSOL IN THE ATMOSPHERE
            !        I        I       I
     )      0.1      0.2      0.3      0.4     0.5     0.5
                   03. ppm (MAXIMUM)
      Figure 3-3. Corralation between 3SCat anci rnaximal
      ozone concentration.
                        37
      from Air Quality Critaria  for 3zane and
      other ^loiiccnsrncai  jx'aants,  /o;'j~e  :.
      Office of ^ssearcr. anc CaveVcpmen', j.S.  E


-------
                               TABLE  1
          SELECTED VEGETATION GENERA  AND SPECIES  GROUPED 3Y
                        SENSITIVITY TO OZOfiE

Sensitive                        intermediate           Res-is-tan-t—
Sean (4)a
Cucumber (1)
Oats (6)
Soybean (14)
Spinach (4)
Tobacco (35)
Tomato (7)
Sean (5)
Cucumber (2)
Oats (5}
Soybean (19)
Spinach (3)
Tobacco (12)
Tomato (5)
Bean (5)
Cucumber (1)
Oats (1)
Soybean (5)
Spinach (1)
Tobacco ( 1 )
Tomato (3)
aMumbers in parentheses  (  ) are the numbers  of  varieties  of the species
for which reports of ozone response were reviewed  in  the  MAS report.
(reference 4).
                                £.3

-------
                                        I/..ULE  2

          Preliminary tbliuiJiL'S of KtUiiut ion in Annual  tconomic D
to fdim Crops,  forust fvoilmts, anil lii•ii.uiu.-iiUls (G.07ppin/8-lir. vs
.  0.09p|iin/8-Ur.)
Crop
- foliar
r - Kool
i> - fruit
apples (fr)
tin Icy (s)
beans, dry
edible d]_
broccoli (f)
cabbaije (f)
'corn, for
corn, sweet
U)
;cotton
cucumber (fr)
jrupes (fr)
Iwy (f)
'oats (s)
onions (r)
juranyes (fr)
leanuls (s)
potatoes (r)
foliar injury
(F.I.)
O.O/ 0.09
piii/t nrs ppm/8tui
a
a
10
a
a
a
a
" a" "
a
a
13
2
a
8
a
a
16
16
20
16
16
16
16
16
16
16
23
. 6 '
16
16
16
16
type of equations
used for fol iar
iajury Values
1) sensit ive plants
11 sensitive plants
II sensit ive beans
11 sensitive plants
II sensitive plants
til sensitive plants
ill sensitive plants
ill sensitive plants
ill sensitive plants
ill sensitive plants
til sensitive hay
ill sensitive oats
ill sensitive plants
ill sensitive plants
ill sensitive plants
all sensitive plants
% IJamaye (if 1 . 1 . - Yield
tetlucliou (Y.K. ) tar
:oliar lype crops Ji.d V.K.
-f .l.-b.Oi; for otner crops
O.O/ 0.09
3
3
6
a
a
3
3
3
3
3
13
0
3
3
3
3
II
11
Ib
16
16
11
11
11
II
D
23
I
A* Damage if
V ft -t I in
1:1
8
a
10
a
a
a
a
a
a
a
10
; 1
n a
1 D a
n
n
11
8
-' - 	 i
Value of
t rop
illilliu: i)
621
714
358
88
176
12.887
220
4,014
136
776
6,742
853
227
648
771
17275
of crop
hat is
ens it ive
5
5
5
51
51
2
5
0.
5
7
30
10
26
JO
1
25
Value of
Sfllb it ive
crop
30
40
20
40
90
260
10
0
10
50
2000
90
60
60
10
320
A Oaiuaye (SMi Dions)
Y.U.:F.l. Y.R.:1.I.
1:2 1:1
1
1
1
2
4
2
3
2
3
' 7
10 i 20
" L?
0
0
0 ! 1
, : 4
100 200
0
2
3
0
13
1
5
~5
'
26

-------
                                 Table 2 (cont.)

          Preliminary  Estimates of Reduction  in  Annual Economic Damage
to Farm Crops,  forest  Products, and Ornamentals  (0.07ppm/8-hr. vs. O.G9ppm/8-hr.)
Crop
f - Foliar
r = Knot
fr - Fruit
s = Seed
rice (s)
sorghum (s)
soybeans (s)
spinach (f)
tobacco (f)
tomato (fr)
iwlieat (s)

sub-total
(farm crops)

forest crops
jornamentals
:and shrubs
i
i
TOTALS

i
i
foliar injury
(F. .)
0.07 0.09
prn/Bhrs ppm/3hrs
a
10
2
8
15
4
8



9
8




16
20
9
16
25
10
16



2)
16




Type of equations
used for foliar
injury values
all sensitive plants
all sensitive
sorghum
all sensitive
oybfidns
all sensitive plants
11 sensitive tobacco
all sensitive tomato
ill sensitive plants



ill sensitive trees
ill sensitive plants




% Damage (if F.I.- Yield
(eduction (Y.R.) for
Foliar type crops and Y.R.
=F.I.-5.0'i for o:iicr crops
0.07 0.09
)pm/8l»rs 'iiiii.'lilirs
3
5
0
8
15
0
3



9
8


11
15
4
16
25
5
11



21
16

&% Damage if
Y.R.:F.l. is
1:1
8
10
4
8
10
5
8



12
8
I
i

t


Value of
crop
S.'iill ions)
929
1.357
9,945
24
2,294
914
4,677

50,650

2,900
1,300


!

of crop
hat is
ensitive
5
5
7
50
9
9
5



20
9



t
i 	 	
Value of
ens it ive
crop
SHill ions)
50
70
700
A Uamage (SMillions)
Y.R.:F.I. Y.R.iF.l.
1:2 1:1
2
3
14
10 0
210 10
80
4
7
28
1
21
2 4
230 | 9 i 19



580
120




t
180 : 360

35
5

220


70
9

440



-------
                                        IAIIU  3
        I'rcl imliiary I ^Uuiati.'i ut  UuUucliuu  in Annual tcuitomic
farm Lru|is,  li)ii-"jl I'ruiluulii, and di aumuiil.1 IL (0.09|i|iin/tl  lir'. v
(I. I0|)|uii/ll-l,r.]
1 1 U|l
- 1 ul iar
i - l(c,ui
li - 1 mil
d|>|l|ui (fl)
J|)|ilei (fr)
barley (i)
barluy (b)
IICMI, tlry
H.anu, dry
Ill0tl.0li (t)
JIULCllli (I)
1
LjUUillJO ( f )
calibaot; (f)
LUIII, t»r
•jrain .(il ...
LIIIII, lor
.urn, 'jWuut
:urn, bwuiil
i ul lull
uc,ullUur (1,
lullar injury
if. •)
u.o'j o.io
16
1
16
1
20
0
16
1
16
1
16
*
16
b
0
16
21
2
21
2
26
t
21
2
21
2
21
7
21
1
0
21
ype ol initial uiiii
uiccl fur ful iar
11 iuiiill ivu |j|anli
i Ian Is
all ifnti i t ivu planlt,
;i|anLi
.11 .unsUlveULM,,,
};jui;^iiniwiiuiu v
all ii-'in 1 1 i vc jijanli
j)l Inluruiudialo
lldllli
,11 Se,,Sillvo,,l-,,lS
<)anli
il 1 Suiib lUvu |)|anlb
ill iliU.-1'incil laU;
,11 S^iliv, ,-laats
,) 1 inltiriucdialu tun
ill luiisljul plants
,11 .un.itivu planl,,
% Uamayc- (It l-'.l.- ticlJ
(cdutiiuii (y.U.) fur
ol iar ly|>0 crup^ ami y.lt.
-F.I. -5. OX lor oi.i^r cruu^
0-09 o. |0
II
0
1)
0
11,
0
16
1
16
1
II
0
11
0
0
II
16
0
16
0
21
0
21
2
21
2
16
2
16
2
0
16
.Ti OilMUlIC it
1:1
&
a
5
0
6
0
&
1
5
1
5
2
I 5
2
0
5
VdUlU Ul
621
62)
714
714
3M1
3SU
UU
IM
176
176
12. UU/
12.UU7
220
220
4.014
136
ol crop
lint ii
eiiiitivo
&
5
5
13
5
U
61
(33)
51
(32)
2
13
6
13
0
5
Value ol
intur-
WUll'iuMu)
30
,30)
40
(90)
20
(30)
40
(30)
90
!\ Uiuiuiju (Si'.il 1 ions)
V . ft . : 1 . 1 . y.U : 1 . 1 .
1:2 1:1
1
0
1
0
\
0
2
0
2
0
2
0
• 1
0
5
0
2 f 4
(6(i) o : l
260
(16oO)
10
(30)
"'
10
6
17
1)
U
0
0
.3
34
1
1
0
i 	
0

-------
                                  I Alii L 3 (lout.)
to
  I'rel iminary F.sl imalet.  of  IU;dm:l ion in /Uimul hconomic
Crops, forest Products,  and Ornamentals (0.0'jppm/B fir- vs. 0.lOppw/H-hr.)
Crop
t - Foliar
I - ItOOl
1 1' - F ru i t
s - Seed
cucumber (fr)

ji apes (fr)
jrapeb (tr)
>ay (t)

.ay (t)
DdlS (S)
IjdlS (S)
unions (r)
I
jnions (r)

,1-amjes (fr)
ifdiiges (tr)
ledliuts (s)
•»'•'-"'"«' <*>
iurijliuiit (s)
.oybeans (s)

Soybeans (s)

foliar i
(F .1
0.0'J

1

16
1
23

1
6
0
16

1

16
1
16
1 16
1
'J

4

njury
• '
0. 10
ppin/hlirs
2

2'
2
28

2
8
0
21

2

21
2
2)
21
2
13

5


fype of equal ions
used for fol i ar
injury values
all intermediate
)1 dills
all sensitive plants
all intermediate
all sens it ive hay

dl 1 intermediate hay
all sensitive oats
^ln!icrl"ediale
all sensitive plants

all intermediate
plants
all sensitive plants
all intermediate
p |ants
all sensitive plants
all sensitive plants
jjlants
dl 1 sensi t ive
soybeans
all intermediate
soybeans
'i Haulage ( i f
(eduction (Y.
Fo) iar tvjie c
-F.I.-5.T\ fu
0.0'J

0

11
0
23

1
1
0
11

0

11
0
11
II
0
4

0
F.I.- Yield
K.) for
rops and Y.ii.
r ottter crops
0. 10
1 tiu/iibrs
0

16
0
20

2
3
0
1C

0

16
0
16
1C
0
U

0


A# Damaijc if
Y l( •!" 1 is
1:1
0

5
0
5

1
2
0
5

0

5
0
5
i 5
0
4 :

0 1
1...


Vdllld of
c rop

136

776
776
6,742

6,742
853
853
227

227

648
648
771
1,357
1,357
9,U45

-g.94-5

A of crop
hat is
ens it ive

led i ale)
10

7
10
30

(50)
10
8
26

(42)

10
10
1
5
13
7

11
Value of
sens it iv«
(inler-
iiediatc')

$Mi 11 ions)
(10)

54
(80)
2,100

(3,400)
90
(70)
60

(100)

60
(60)
10
70
(IftO)
670

(1100)


6 Uamayu
Y H *l 1
1:2
0

i
0
50

17
1
0
2

0

2
0
0
2
0
14

0
— ^' — —" i

Si'li 11 ions)
Y . « . : F . 1 .
1:1
0

3
0
100

' 34
2
0
3

0

3
0
0
3
0
28

0

-------
                                     IAllll 3  (LuiiI.)

           l'i cl tin I luii y I jllmuli-'i ul  lli.ilui I inn in Annual  trunumii  i,_,,m.ji.
to I arm Crop.,  loiu.l IVi-ilncl.. ami Oi n..iiiuiilal., (0.09ppilanl:
;lil..tc'i"isUUiB
all •Juu-,lliv-: plant:
al) iflluniU--l|a-L'
al 1 -L'n.il Ivu plant.
dl) intuniieiliali.
li)eul-i. ... ... .
all ..un.itivi.
all int t:i'niijil i at tj
luljacixi
all -.cniil ivu
l!!.llslli-
al 1 Inl urnicilljle
all .uliSilivt: plant
al 1 1 n t c l ineil i jlc




i Oailla.e ( ll .1 .- YlilJ
(-.•Um:l ion (V.K. ) lur
ol iai lyini erupt, and Y.R.
-1 . 1 . -i . O.i lor uihcr crups
0.0'J O.|0
16
1
12
0
12
0
25
1
«»
0
12
0




21
3
16
0
16
0
31
2
9
0
16
0




At Uauiayu if
Y.li.:l.l. it,
1:1
5
2
4
0
4
0
6
1
4
0
4
0


i
1

V_)u. Ul
i.i'Hi |
s:m: i.i.i..
24
24
1.275
1.275
929
929~
2.294
2.294
914
914
4.677
4.677
50.650



1C of i.iu|j
Llidl It.
iun'. i livu
[inU:r-
c.lijlu)
50
(3U)
25
(50)
_
13
9
(26)
9
U
5
13
	


.alui' ul
-,Cll-> 1 I i VI!
inler-
iiL-tliali.')
t-rop
(tMilliun.)
12
(9)
320
(640)
(50)
(120)
210
(600)
«0
(/O)
230
(610)
	 	 -


A Uauiatji. (i"' 1 1 lon-j)
Y.l(.:f.l. Y..\.:KI.
1:2 1:1
0
0
6
0
1
0
1
0
13
0
- 2
0
6 j 13
3 j 6
2 1 3
o : o
5
0
140


9
„ _ .
290



-------
                                                      I              TAUIt  3 (ConI.)
                                           Preliminary' Cat iiiiatus of ((eduction  in Annual  economic
                                 to I arm Crops, forest; Products, am) Ornamentals  l0.09ppm/8-lir.  vs.  0.10ppm/8-hr.)
JQiJ
Crop
= 1 ol iar
-- KliOt
r - fruit
= Seed


rest
ouucts
rest
oJucls
namentals
'i.&!irul)S... _
•itamentals
id shrubs
!•.>- total
Hal - all
Delation








foliai- j
(r.
0.0'J
pr.'i/chrs


21
/
16
0










njury
-)
0. 10
ppin/Ohrs


28
9
21
1










lype of oijudt ions
used for foliar
injury values


all sensitive trees
all intemiedidte
trees
all sensitive plants
all intermediate
anuiueftials.










% Dative (if
liecJuction (Y
'oliar type c
=F.I.-5.0X fc
0.0'J
ipiu/Qhrs


21
7
16
0







i


F.l.= Yield
R.).for
rops and Y.K.
r otUer crops
0. 10
P(.'.n/!;iirs


28
9
21
1








1

A% Damage if
Y li -F 1 is
1:1


7
2
5
1







i


Value of
(; cop
SMil) ions)


2,900
2,900
1,300
1,300








1

% of crop
Ih.U is
sensitive
( i ntor-
iied iale[


20
(20)
9
(21)

•








Value of
sens i Live
(inter-
media to)
(SMil lions)


580
(580)
126
(270)



»






A Damage
Y.U.:F.I.
1:2


20
6
3
2
30
170








(SMil lions)
Y . It . : f I
1:1


41
12
• 6
3
CO
350









-------
                                                       Taole A
-iant specias 3.
i C'jltivar (cv.i '
Alfalfa,
cv. vernal
Saan,
cv. "into



Tuc'jraer,
cv. Ohio Mcsiac
jnion,
cv. Spartan Era
.'.adisn,
cv. Cnerry Sail a
r adisn,
cj. Cnerry Belle
3oytaan
cv . rood
in.l 2ar-
Soystan,
cv. 3are

3*eet ccn,
:•, . jalcen '-fidget
i?C1"'*-3
"ccacco,
cv. 3el —3
"aoacco,
cv. 3ur:ey-21
Tomato ,

*No statistical
*»*ta statistical
^Statistically
"Scat'sfcal !y
•jrowtfi and yield xesoonsas of Plants to Qiona Exposures, Compares uith roiiir Injury Response
froc U.S. EPA, Assessment of Welfare Effects and tne Secondary Air Duality Stanaard for Ozona,
June 1978.
concantration. Exposure pattern: ?1ant growth 3r yield ?oliar injury Type 3f 2ef«rsnc<
ppm* Surtier of hours!*), rasponsa, 5 'ssuction resoonsa, '. incr. Exposure
days(d), 4 w«e.t;
I*, root i'risa ;*»; 	
O.IQ(-) 3.h/d, 5d/w, 2* 2!*, top frssn s«;- ;3»
*i', root 'rash. *t;
0.3S'.*5 5h/d, 133d 3*. sass yield; 19* :-nci3sad fijic = =
22*. slant fresn *t;
3.13'!*} ih/d, 133d 55?, sasc yield; 37^
55?, Plant -resn 3.35opn(-j A3d 22?, laaf fresn »t; . "7- opsn-cop -"ijic '.,iO
3.2s.;-> 3h/d, 5d/w, AJ !*, leaf cry ^t; 3 ;raernausa 3C.79
3r-«», stam cry »t;
A2??, root cry »t;
O.CS(-J 3h/d, 5d/w, lw Mo significant rscuctions traca greennjusa 30,79
O..20(+) 2.5h/d, 3d/w, 15w 1*-, fruit yield; extensive, con- greannojsa £S
32?*, too dry wt; sidaraole amount
11**, root dry <*t; af cafoiiation
2.35(-) 2.5 n/d, 3o/w, 15* 45*-, fruit yield; extensive, ji-iost
72?*, toe dry »t; cpmoletaly
j3*», root dry 
-------
                                                         TABLE 5
                         Effects of Long-term Controlled Ozone Field Exposures on Growth and Yield of
                         Selected Plants (Excerpted from U.S. EPA, Air quality Criteria for Ozone ana
                         Other Photochemical Oxidants, April 1973,
Plant Species
1 Cul tivar (cv. )
Alfalfa, Cv.
'•'esa-Sirsa


Pine, Pcnaerosa
J'ne, western
.•ihica
Soyoean, Cv.
:are

S.veet Corn, Cv.
Golden Midget

Exposure Pattern
0, Concentration, and Duration:
?pma hours (h) 1 days(d)
0.05 7h/d, 63d
0.10 Sh/d, 70d

0.10 5h/d, 125d
0.10 5/hd, 12Sd
0.05 Sh/d, 133d
0.10 Sh/d, 133d
0.05 5h/d, Sid
0.10 5h/d, 54d
Type of
Exposure
Chamber
Enclosed
Enclosed

Enclosed
Enclosed
Eric lo sea
Enclosed
Enclosed
Enclosed
Plant growth or
yield response, ", re-
duction from controls
30*, cop irv-wt, 	
(Harvest 1 )"
50*, 'OP dry wt.
; Harvest 2;
20*. top dry wt.
..Harvest 2,
50**, too ciry wt.
•; harvest 3
12. root 'enqth
21 , sten cry •»'.
25*, root dry >jc.
I''*, fol iace -iry wt.
9, stem cry «t.
3, saec yield
22, 3 lane fresh wt .
55*, seed yiela
65*, plant fresh ,vt.
9, kernel dry wt.
-15*, kernel dry -.vc.
Criteria
Document
Reference
63


13i
;3i
133

'32

i AM  references specified both che .nonitoring technique  ana the calibration procedure,  except in the case
:f reference 53 zhat infomation ^as ootained by correspondence with the authors.

* Statistically significant difference from controls at the 5% confidence level.

*~ Statistically significant difference frcn controls at  the IX confidence level.


                                                           33

-------
                                                         T 1 Ol "* •"
                                                         .ASLi i


                            Effects 3f Long-carrt Ancient (ana AugKtentaaj Ozone .ria!a £xsosures en the  Meld

                            of Selected P
Plant Soecies, treatment Seasonal Mean of
lurncer of 7-hour-averaga
Caitivars Qj concentration, ppirr3
-



'ield lorn '3) AA
0) •a
5, karnei *t.
-2
7 '
25*
1 1 , Shoot fresn wt.
33** " :' ~' " ~
57** "
il»
12, sasd it.
T '
13*
30*
33**, fry it fresn .-/t.
^aferanc,

7



3



9



10
" "raat~ent AA is 'jnenclosad. 'IF treatments are lon-filtaraa poen-cap field cnamoers "3csiving

3
^


:
.3



(in raferences 7, 3, anc 9) additional coses
All "?farancas specif ^a
-------
                   Table 7.  Oxidant Levels in 23 Urban Areas

                                                   a  90,91
                             of the U.S., 1964-1975
Location
Ca.rcen, :U
Corpus Christi , TX
Ges Moires, I A
Louisville, K>'
vaTiaronec'<, NY
Vemohis, T'i
Newport, jg/tt (ppm)
53
90
53
30
70
90
72
89
97
99
54
94
34
95
91
77
95
32
90
33
95
55
94
93
97
95
N/A
N/A
N/A
N/A
N/A
N/A
N/A
N/A
N/A
table obtained after 19"
ier data measured total
es having valia cata for
y, the sites :reser,tea i
375 (0.19)
365 (0.19)
505 {0.25}
241 (0.12)
241 (0.12)
192 (0-10)
133 (0.10)
362 (0.18)
136 (0.09)
352 (0.13)
309 (0.16)
313 (0.16)
253 (0.13)
225 (0.1 i)
254 (0.13)
305 (0.16)
297 (0.15)
321 -.0.16)
155 (C.03)
225 (0.11)
552 (0.2?)
155 (0.03)
270 (0.14)
245 .0.13;
130 (0.07;
150 (0.03)
950 (0.43)*
340 f 0^.43)*
4^0 (0.22J*
440 (0.22)-
360 (0.13)*
570 (0.29)*
400 (0.201*
230 '0.14)*
3:0 :o.is;*
310 (0.16)*
220 (0.11)*
250 (0.13)*
44 (0.022)
40 '0.020)
38 (0.019;
41 (0.021)
44 (0.022;
47 <'0.024)
55 (0.034)
18 (0.009)
13 (0.009)
23 (0.012)
25 (0.013)
27 (0.014)
23 (0.012)
38 '0.019)
47 (0.024) . .„..
41 (0.021)
20 .'0.015)
24 (0.017)
32 (0.015)
53 (0.027)
50 (Q.028)
30 (0.015'.'
41 {0.021;
0 '0.020)
24 '0.012)
19 -0.310)
32 (O.G42)
71 (0.035)
71 (0.035;
71 (0.033)
51 (0.031)
59 (0.230)
59 (0.330)
"1 (0.036)
57 (0.029)
37 '0.019)
55 (0.023)
'Q were measured by ozone-soecific
oxidants. Also, post-1970 aata .
-------
                                                           I/U1I I- 'I

                                         it/nne Air ({ujliiy la Iteiuito
jtaliun Location fluvatton Ixlcnl of
(lumber Above Mean IUIJ .Months
bcM level, (Yeari of
i» Observation)
1 (Jul 1 Uyulu, MA 6i! (!) (|'J/4-/6)
•f. Mcltae. Mi 9/1) |'j (|'J/4-/l.)
3 un Site, Ml lou;? io (iy/6 /i.)
4a Uhlle liiver, 01 I!)'j0-I6i?b II, (|9/4-/nl
4b • 16 (19/4/6)
4< IU (l'J/4 /6)
!»<• II lo Ulanco, CO 1'JOO I'J (I9/4-/6)
!ib i!lOO I'J (|'J/4-/6)
6 Iriu I'eak. COC ^/30 '.t (I'J/M
/ Converse Co., UY N/A 6 (l'J/4)
11 imilti Face Mln., ML IlilU 23 ()lJ/1-/6)
'J Manna foa. III 3400 i'\ (ll-/!i)
10 /iujb|iltze, 3UOO 2] (CJ/4-/6)
tle^t liei-iiiany
Avij. Conceu.
aver I'eriuJ
Ex/iiniried,
•jb (O.(tfH)
// (0.03'J)
116 (0.044)
/!> (0.03U)
/I (0.036)
6/ (0.034)
S6 (O.O^j)
'jS (O.l>'.  ll'A. Ass,eiiineiil of We II are lllucli  and I In; Vn.ondary Air ()ual ily |Slandard for 0/une. June  I'J/H.

                                                                                 I

-------
                              ATTACHMENT 1
                       Air Quality Data Analyses

     This attachment describes two  analyses performed on ozone and
oxidant air quality data available in EPA's Storage and Retrieval  of
Aerometric Data (SAROAO) system.   In the first analysis, the relation-
ship between annual peak 1-hour and 3-hour average concentrations  was
evaluated.  This was used in the  preliminary approach presented in
sections 2.0 through 4.0 estimating ozone damage to vegetation using
the foliar injury data base.  The second analysis examined the relation-
ship between annual peak 1-hour average concentrations and the long-term
(growing season) mean of the daily maximum 7-hour average concentrations.
This was used in section 5.0 for  comparison with studies examining long-
term ozone field exposures on growth and yield reduction in vegetation,
1.   Annual peak 1-hour and 3-hour average concentrations
         In section 2.0 through 4.0, a preliminary estimate of the ozone
damage to vegetation was attempted using foliar injury data which  are
based on acute responses of plants to single short-term ozone exposures.'
The foliar injury  data suggested that the peak 3-hour average concen-
tration might, under prevailing atmospheric conditions, be the controlling
factor for determining the amount of foliar injury associated with given
alternative 1-hour average standard levels.  Consequently, EPA conducted
an  analysis of air quality data to determine the relationship between
these parameters.

-------
                                   2
          Ozone  or  total oxidant  data  from  123  site-years  (45  stations
 in  25  states) for  the  period  1975  through  1973 were  analyzed  to  compare
 annual  peak  1-hour  and 3-hour average  concentrations.   These  site-years
 constitute approximately  50 percent of the  data contained  in  5AROAD  for
 the control  sites  (i.e.,  stations  whose concentrations  are highest)  of the
 90 Air  Quality  Control Regions (AQCS)  containing urbanized areas with popu-
 lations  greater than 200,000.  The site-years to be  analyzed  were  selected
 in order of  increasing AQC3 number; this procedure should minimize any
 selection bias  in the  analysis.  Descriptions of the site-years  (extent
 of data,  location,  station type, etc.)  are  given in Table  1 of this
 attachment.  The station  types vary in nature from "center city-industrial"
 to "rural-agricultural."
          To permit  a tractable computer treatment of the problem, concen-
 trations were reduced  to  parts per hundred million (ppnm); the results of
 the analysis are reported in  this  unit. One pphm is equal to 0.31 pern
 (or 19.5 ug/m-  at 25°C  and 101.3 kilopascals).  This translation aeleted
one significant digit  ror most data (e.g., 0.137 ppm became 14 pphm;
Q.G05 Ppm rounded up;.
         For each site-year,  a computer program calculated 3-nour average
concentrations  far each day's data for the 3-hour periods starting at
12:01  a.m.,  1:01 a.m., and so forth on through 4:01 p.m., so that every
1-hour average value was included  in at least one 2-hour average comauta-
ticn,   Where a full  3 hours'  worth of data was not in the data tank  for a
given  start time,  3. multiple-hour average value was computed on the  oasis
of the number of hours of data that were available.  "Thus, if only 4 hours

-------
                                  3
of data were present for a given 3-hour period, the multiple-hour
average value computed was actually only a 4-hour average.  This data-
handling procedure could be expected to bias the 8-hour to 1-hour
average relationship on the high side by computing higher.(ostensible)
3-hour average values than the data warrant.  Consequently,  the output
of this computation was checked against the raw data for those instances
when the annual peak (ostensible) 3-hour average value seemed high
(within 2 pphm of the corresponding 1-hour average value).  As a result,
adjustments were made in the annual peak 8-hour average value for
5 site-years.  In addition, clearly anomalous peak 1-hour average values
were deleted for 5 site-years.
         Table 1 presents the corrected results of this computation.  A
plot of annual peak 3-hour average concentrations as a function of annual
peak I-hour average values is given in Figure 1.  As can be seen from the
figure, there is a considerable variability in this relationship.  EPA
chose to use an upper-boundary curve which envelops most of the data in
Figure 1 to establish the maximum 3-hour average concentration that
could be expected to occur if a given hourly  average standard level were
achieved.  Thus, attainment of a 0.08 ppm hourly average standard whose
permitted frequency of exceedance  is one day per year snould prevent
0.07 opm, 3-hour average,  from being exceeded more  than once per year.
Similarly, a 0.10 opm hourly average standard should prevent 0.03 opm,
8-hour average, from being exceeded and a 0.12 ppm  hourly average standard
should prevent 0.10 ppm, 8-hour  average from being  exceeded more than once
per year.  These relationships are used in  section  2.0 through 4.0  in the
preliminary damage estimates.
         In section 3.0 the pofnt was made that most of the annual peak
concentrations occurred  in the period May through September.  From  Taole  ;
it can be seen that the  annual peak 1-hour  average  concentration occurrec

-------
                                  4
during  this period  for 36  (or  73  percent)  of  the  site  years,  and of  the
remainder  18  (or  15 percent) had  no  data in the months May-September.
1.   Seasonal mean of  the daily maximum  7-hour  average  values
        As noted  in section 5.G,  the  available information  on yield
reduction  in vegetation resulting from  long-tern  ozone exposures
indicates  the  importance of the long-term  (growing  season)  mean  of
the  daily maximum 5-  to 7-hour average  ozone concentrations.  Consequent-
ly,  EPA conducted an  analysis of  the  available air  duality  data  to
determine what long-term mean might be  expected to  accompany a O.lZppm
annual peak 1-hour  average standard whose  permitted  frequency of excee-
dance is one day per year.
        The currently available evidence regarding  the  effects of
long-tern ozone exposures on growth and yield reduction  in  vegetation
is discussed in section 5.3 and summarized in Taoles 5  znc  5.  This
evidence indicates  that the threshold for  significant  growth and  yield
reduction in commercially important croos  and inaigenous vegetation  lies
between 0.06 and Q.lGppm for a 1- to 4-nonth mean of the daily maximum
5- to 7-hour average concentrations.  SPA  chose to use  the  Z-Tionth
mean of the daily maximum 7-hour  average concentration  as a reasonably
conservative parameter for evaluating the  protectiveness of a O.lZppm
annual pea.k 1-hour  average standard.
        Ozone or total oxidant aata were analyzed for  the 23^ site-years
in the period 1975-1973 contained in SARCAu for the control sites of
the 90 AQC2 containing urbanized areas with populations  greater  than
2CG,OCC.  Of these,  171 site-years had  a valid 2-month ~ean in the
:eriaa '-'ay througn  Seotemcer;  these site-years are describes ;:

-------
                               5
A valid 2-month mean v/as defined as two consecutive months with at
least 30 daily maximum 7-hour average values in the 2 months.  (One
site-year was included that did not have any 2 months consecutive but
otherwise fit the criterion.)  Table 2 presents the maximum 2-month
mean of the daily maximum 7-hour average values as well as the peak
1-hour average concentration in the period May through September,
and Figure 2 depicts the results graphically.  Figure 2 demonstrates
that the relationship between these parameters is quite variable, but
there is definitely a trend in the direction of increasing 2-month means
as the peak 1-hour average increases.
        In order to use Table 2 and Figure 2 to evaluate the protective-
ness against yield reduction effects of a peak 1-hour average standard
whose level is Q.12ppm and whose freauency of exceedance is one day per
year, it is necessary it introduce one cornolicating factor.  The "peak
1-hour value" column in Table 2 does not exactly correspond uO the stan-
dard level, since the peak 1-hour value is by definition the very
highest hour recorded in the May-September period (except for corrections
in the values of 7 site-years to delete anomalous data), whereas the
standard permits one daily maximum 1-hour average value per year (as
a 3-year average) to exceed the standard level .  For a standard level
of 0.12ppm, che expected peak 1-hour average is 0.13ppm.  Consequently,
a peak 1-hour average concentration of 0.13ppm or less would be expected
to attain the Q.12?pm 1-hour average standard.
        From Figure 2 and Taole 2, it can be discerned that of the
13 site-years with peak 1-hour average values less than or equal uO
0.13ppm, only 5 (or 12%) 'nave maximum 2-month means in excess of

-------
0.06 ppm (5 pphm).  Of those 5 site-years, none had 2-month means as high
as 7 pphm.   In contrast, of the 123 site-years whose peak 1-hour average
value exceeds 13 pphm, 33 (or 56 percent) had 2--nonth means in excess of
5 pphm.
        On balance, these data seem to indicate chat attainment of  a
Q.12ppm 1-hour average standara (with an expected exceedance frequency
of one day per year) would generally prevent a O.Ooppm 2-month mean
of daily maximum 7-hour average values from being exceeded.  Consequently,
EPA believes that the evidence currently available does  not suggest that a
peak 1-hour average standard any lower than Q.12ppm is necessary on the
•basis of ozone-related yield reduction effects in vegetation.

-------
RELATIONSHIP  Of- ANMUAL PEAK l-||oUll
     TABLE  J.
0-IIOUR AMEHAGH OY.OHE (OR  OXIOANT) CONCE/
31
33


5|TIT CODE
01 1300003 G0|
10351-0001 FOI
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n
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-------
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-------
                                       ATTACHMENT 2
                    UNITED STATES ENVIRONMENTAL PROTECTION AGENCY
  DATE:   October 24, 1978

SUBJECT:   Qzone  Leaf injury
           Ralph  Larsen
           Environmental Applications Branch, MD, ESRL (MO-80)

    T0:     Harvey Richmond
           Pollutant Strategies Branch, CAQPS (MD-12)
          This  is  in response to your request for calculations of expected
          percent  leaf injury in plants exposed to 8-hcur-average ozone con-
          centrations of 7, 9, or 10 pphm (last three columns of attached
          Table 3).

          Computer programs have been revised to produce Tables 1 and 2 (given
          to you October 12), and now 3.  Table 2 lists each observation of
          ozone leaf injury for each plant variety.  These input data have
          been  processed by a multiple regression program to calculate the
          three parameters of Or. Heck and my plant injury model and the
          expected percent leaf injury after an S-hcur exposure to ozone
          concentrations of 7, 9, or 10 pphm.

          Table 1  pools observations by integer plant numbers.  (The plant
          names following the commas do not apply.)  For instance, the 55
          observations of Pinto 3ean (plant 3.1), the 1 observation of Seeway
          3ean  (plant 3.2), and the 6 observations cf White Sanilac Bean
          (plant 3.4) have been pooled to give the 52 observations for beans
          that  comprise the input that gives the resulting plant injury
          parameters listed in Table 1.  Note that the large number of Pinto
          Bean  observations will weight the results towards that plant.  If
          you want to alter the weighting of the observations of the separate
          varieties comprising a pooled calculation, please let me know and
          I will try to revise the computer programs to do so.

          The computer program to produce Table 3 has just been completed.
          It allows pooling by plant number.  For sensitive tobacco, for
          instance, line 5GC states that all plant numbers between 20.0 and
          20.99 will first be pooled.

          Line  510 indicates that plant numbers between 22.0 and 23.9 will
          also  be  included in that pool.  Table 2 lists all of the available
          input data.  If you would like any of that data pooled in ways
          different than in Table 3, please give me the line title and the
          plant numbers you wish included in each susceptibility under that
          title, and I will run it for you.  Note that the plant number for
          the same plant name differs' among the three susceptibilities.

-------
 I  hope this  information  will  be  helpful  to  you,  Harvey.   If  I  can  be  of
 any further  assistance,  please let  me  know.

                              Addendum

      The  computer program  to  which  Dr. Larsen  refers  has  not been  included.
 Regarding his  statement  that  in  Table  1  the plant  variety names  do not
 apply, the comouter  printout  has  been  modified so  that variety names
 appear only  when  the data  pooled  are from that variety alone.  In all
 tables, the  concentrations  appearing in  the "INJURY THRESH"  (injury
 threshold) columns are for  1  percent response; the numbers appearing  in
 the "SUSC" (susceptibility) column  signify  the following  classification:
 (1)  sensitive,  (2) intermediate,  and (3) resistant.

      In Table 2,  the numbers  appearing in the  "EFFECT TYPE OR  N" column
 in  the lines presenting  individual  plant response observations refer  to
 one  of the following effect types:  (1)  foliar injury, (2) chlorophyll
 reduction, (3) yield reduction,  (4) leaf area  reduction,  (5) respiration
 increase,  (5) root dry weight reduction, and (7) tap dry  weight  reduction.
 The  numbers  that  appear  in  this column in the  lines summarizing  the
 observations for  each plant or variety are  the number of  observations
 presented  for that plant (variety), effect  type, and susceptibility.  In
 Table  1,  the data are summarized  by effect  type, starting with the
 effect type  1, cycling through the plant numbers and susceptibilities
 before proceeding to effect type  2, etc.

      In Taole 2,  the numbers appearing in the  ''TYPE CCNC  I'1ST" (tyoe  of
monitoring instrument) column nave  the following meaning: (1)  ampercmetric
neutral buffered  potassium  iodice (NBKI)  calibrated by 2  percent color-
 imetrlc ,'IBKI, (2! amoerometric '(3KI uncalibrated, (3)  ultraviolet -non i tori ng
 instrument (late  1950's), (-}  Atlas iodometric,  (5; wet chemistry (20
percent),  and (5) unknown.

     The numoers  that appear in the "MULT CORR CQEF"  (multiple correlation
coefficient)  column  are R values.  The fraction of variance in the data
explained by the  .node! would be .12.

     In Table 2,  the numbers in the '"REF" (reference)  column indicate
reference numbers in Chacter 11  of the 1975 draft of the National Academy
of Sciences document, Ozone and Other Photochemical Gxidants.  Only tne
docket copies of  this report contain these references.

     In order for the multiple regression orogram to  calculate the
parameters of the Larsen-Heck  model, and  hence calculate percent  injury
-or tne specified 3-hour average  concentrations,  there must be opservations
at more than  one  exoosure duration.   The  wider the range of exposure
durations, the better the model's predictions.   This  fact provides the
basis  for  certain comments  in  the margin  of Table 1 as to the validity
of the mocel's predictions.

-------
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                                                   CAtCULATEO  INJURY  PARAMETERS TOR  PI AN TS  EXPOSIO TO 01 CN E.
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25
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25
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25
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25
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25
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25
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EIFECT STO CEO CEO INJURY I Nl UR Y Til IT 31 IN J COM: M U. T * IN J AT 8 MR
TYPE CEO MEAN HEAN LIME PPIIH RATIO C OR fl IP IH CONC OF
RTF OK N DEV AT T 1 MR SL(PE 1 II R 3 IK 8 II R HE O/ TH IS C OE F 7 9 10
214
214
214
214
214
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214
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449
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52
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-------
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-------
TAULE   2 (CONTINUED!.   OBSER V IT ION S ANO  CALCULATED INJURY PARAMETERS FOR PUNTS EXPOSED TO  OZONE.
EXPOS NUMBER TYPE
DURAT CONC INJURY OF DEV CONC
PLANT HR PPHM X Z IMST
10.
10.
10.
10.
10.
IB.
IB.
10.
10.
10.
10.
IB.
10.
20.
ill.
20.
20.
211.
20.
20.
20.
20.
2(1.
20.
21).
20.
211.
20.
20.
20.
2(1.
20.
20.
20.
20.
300
1UO
'llJI)
500
500
mo
too
700
TOO
QUO
DUO
'Jin
•JOU
100
100
U)U
11)0
101
101
101
Ul 1
111)
110
110
111)
120
120
120
120
130
130
130
130
I'lO
110
SOYBE
2.0
SOYHE
2.0
SOYUE
2.0
SOYDC
2.0
SOYflE
2.0
SOYBE
2.0
SOYUE
2.0
2.0
2.0
rou t£
3.0
3.0
3.0
IN.
.50
AN.
50
UN.
50
AN,
50
AN.
50
AN.
50
IN.
8
'15
30
CO*
15
22
JO
CL ARK
GO
CL ARK 63
GG
CUTLER
61

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2

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GG
LEE
70
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7 9
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0
1
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TOBACCO. MARYLAND
3.0
3.0
3.0
15
22
30
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3.0
3.0
3.0
15
22
30
TOU ACCO.
3.0
3.0
3.0
15
22
30
TOU ACCO.
3.0
3.0
15
22
35
38
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3G
30
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33
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27
31
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10
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-.31
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59
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-.31
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G
-------
I AUK   i  (CONIINU(U).  OBSEHVU IONS AND CMCU1MLU  INJURY PMUMIIIUS fOHPI_»NlS  EXPOSCO 10  OlOHf.
1
1
P L » N 1
21). I'll)
2U. I'lO
20. 150
20. I'jO
20. ISO
20. 150
21). 1!»0
20. 15 0
21). ISO
20. II. (1
20.if, 0
20. 1CU
20. ILO
20. ICQ
20. 160
211. 100
20. I/O
2(1. I/O
20. 170
20. U(l
211. 1MI
20. HI)
21). HO
20. 1UU
20. ioo
20. IHU
20. IUO
2(1. IUO
20. IUC1
20. IUO
20. no
2U. I'll)
20. rill
20. DO
20. Uil
20. DO
20. 110
20. 200
20.200
txpos
JUIU1 CONC
lilt I'PIIM
1 .0 JO
iuii v:cu.
1.0 JO
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2.0 SO
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1011 V.-CO.
1.0 U)
1.5 20
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IUII 
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IUII «CCO.
1.0 JO
1 .0 20
1 .0 JO
J.O 10
J.O 20
1..0 10
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1.0 JO
1.5 20
2 .() JO
1.0 10
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IUU CCO.
2.0 21
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J07
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504
-.71

m-t
;
-------
TABLE   2  ICONTlNUfDI.   OBSEHVITIONS »ND  (MLCULUEO  INJURY PARAMETERS FOR PUNTS  EXPOSED  TO OZONC.
EXPOS NUHOER TYPE
DURAT CONC INJURY OF OEV CONC
PLANT IIR PPHM t 2 IHST
20. 2O 1
20.20 1
20.201
20.210
20.210
20. 210
20.21(1
20. 210
20.210
20. 220
20. 220
20. 220
20.220
20.220
20.220
20. 230
20.230
20.230
20.230
20.230
20. 2MO
20. 2'lO
20.2'lO
20.2'lO
20.2'lO
20.2'tO
20.250
20.250
20.250
20.250
20.250
20.25H
20. 2GO
20.260
20.260
20. 260
20. 26 H
20.260
2.5 IB
2.5 3t
101) 1C CO,
2.0 30
2 -5 12
2.5 10
2.5 36
J.O 20
TOU ACCO.
2.0 30
2.5 12
2.5 10
2.5 36
3.0 20
TOO «C CO •
2.0 30
2.5 12
2.5 IB
2.5 36
3.0 20
T t\H RT" P f\ m
I UU RU L- U f
2.0 30
2.5 12
2.5 10
2.5 3f.
J.O 20
TOO HCCO,
2.0 30
2.5 12
2.5 18
2.6 36
3.0 20
ion ncco.
2 .0 30
2.5 12
2.5 18
2.5 36
J.O 20
roo iccot
J2
51
COKEB 187
51
17
3M
66
32

i
i
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5 10.01 22 .MM
I
1
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1
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INJURY THW Ul 1NJ CONC MULT t IN J AT 0 MR
rpim RATIO CORR rp m CONC OF
I III! 3 IIR 0 IIR MED/TIIRS COEF 7 9 10


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                                                350

-------
IAIUL   2  ICUNI iNUtO I.   imSHIVUlOHS »NO  CUCUlUtO 1HJUI1V PMUHlirilS rOII PIOUS  CXPOSfU  10  070NC.
IXPOS NUhUltl llTI't tfltCl SIO CJEU QIO 1NJUKY UUURY IHUfSH 1HJ COMC HUH X 1MJ kl B III)
11 II IHl CUNC 1 NJUHT OF DtV CUNC 1 Yl't GEO HI *M H(«N 1. INI I'l'IIH I) U IO C OH R fP IN C ONC Or
I'lAHl till PI'IIH t Z IN SI SOSC 111) 01) N OfV *I 1 1 III! SL (VI I lilt .1 UK B UK HtO/ IllltS COEI 7910
20.2/0
2U. 210
211.2/0
20.2110
20.280
20.2UQ
20.2UO
20.2UII
20.280
20.2'JO
20.2)0
20.210
20.200
20.230
2(1. 2UQ
20. JUO
20. 100
20.JUO
20. JUO
2U.3UO
20. JUO
211. JUO
20. JUO
20. JUO
20.300
20. UIO
20. .100
2 (1 . JU 0
20. JtlO
2(1. JU I)
20. JOI)
21). JOU
20. -UIO
20. JOO
20. UK)
20. JUO
21). JUO
20. 1UU
20. .(00
2 0 . M 0
20. JOO
20. IUO
20. JIM)
2 U . Ill 0
2.S
2.!i
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2.0
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2.5
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2 358
2 358
358
2 358
2 358
2 358
2 I 358
2 1 3Sa
1 358
2 1 15 U
2
2
2
2

2
2
2
2
2
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
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1
1
1
I
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1
35a
350
358
358
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6
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G4
G<4
C'l
138
212
212
212
214
214
214
214
214
214
2lli
217
217
217
217
217
217
21 /
217
217
217
217
21 /
217
1
1
3 2.13 2J .I1C
1
1
1
1
1
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1
1
1
t
1
5 1.79 GC -1.17 17 5 1 3.9 .87 G3 .1 77.9 B2 .9
1
1
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1
1
1
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1
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1
1
1
1
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1
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1
1
t
1
1
1
1
1
1
1
1
1
1

-------
TABLE   2  (CONTINUED).   OBSERVATIONS UJO  CM.CUMIED  INJURY P*R»METERS FOR PUNTS EXPOSED  TO OZONE,
PLANT
2 0. 30 0
20. 300
20.300
20.300
20.300
20.300
20.300
20. 30 U
20.31)0
20.3(10
20.300
20.300
2U.300
20.300
20.300
20. MO
20. 31)0
20.3UO
20.300
20.300
20. 3011
20.3UU
20.300
20.300
20.31)0
20.3UO
20.3UO
20.300
2(1. 3OO
20.3UO
20.300
20.300
20. 300
2U. 300
20. -WO
20.30 1
20.301
20. i) 1
20. 30 I
2 0. 3fJ 1
2 U. 30 1
?0. 31 0
20. 31 U
2 U. 31 0
2 0. 3L 0
20. 32 0
CXPO:
OUIM
11)1
2.0
2.0
2.0
2.0
2.0
2.0
2.0
2.0
2.0
2.0
2.0
3 .0
3.0
3.0
2.0
2.0
2.0
2.0
2.0
2.0
1.5
1.5
i.r,
1.5
1.5
1.5
1.0
2.0
2.0
2.0
3.0
3.0
1 .0
4-0
TOO
2.0
2.5
2.5
2.5
3.0
100
2.5
2.5
2 .5
TOO
2 .5
r CONC
PPIIM
10
10
10
It
It
22
22
22.
28
28
28
25
50
75
27
10
It,
22
28
21
5
1,0
15
20
30
35
20
10
to
20
10
20
10
20
HCCQt
30
12
ia
3k
20
«CCOi
12
ia
3b
ceo.
12
INJOflY
t
1
9 9
12
20
MO
21
32
77
40
73
83
4'J
75
7 2
33
1
13
10
64
30
0
10
0
55
ao
a a
3
0
4
3 1
26
35
25
Mb
OL WJ
13
14
39
73
4 4
SPEIQI T
35
4 1
8 7
9' El Ul T
3 3
Nunocn
OF DEV
z
-2.33
2.33
-1.10
-.84
-.25
-.71
-.47
.74
-.25
.51
.95
-.02
.67
.58
-.44
-2.33
-.08
-.25
.36
-.20
-3.72
-1.28
-3.72
.13
.04
1.18
-1.88
-3.72
-1.75
-.50
-.G4
-.38
-.67
-.10

-.18
-1.08
-.28
.61
-.15
G-3
-.38
-.23
1.13
0-7
- .44
TYPE
CONC
INST
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
1
1
1
1
1
1
6
6
6
6
6
6
G
6

2
2
2
2
2

2
2
2

2
SOSC
1
1
1
1
1
1
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001 OtH ARIIOU
-3.72
-1.0%
-.67
-2.33
-1.88
- i-ia
-.61
-.23
1.75
-3.72
-.31
.25
-.99
-.55
.99
NNSCOTT
-3.72
-1.01
-.GI
4KE
-3.72
- 1.01
-.G7






i
i
i
i
i
i
i
i
i

i
i
i

i
i
i
. Ulllir SUEET
10
15
20
. L
50
•1'J
25
75
20
GO
50
U
S
25
V) JNO
15
3 9
1
1 9
7
57
17
-3.72
-1.65
-.G7

-1.01
-.28
-1.75
-.02
-1.10
.18
-.08











LlflCl SID CIO OCO IHOIlif 1HIOIIY HIDE Ml IHJ CONC HOL 1 X IN J *l 8 III)

SUSC
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2

IMF
211
211
211
ia
ia
ia
52
52
52
211
211
211
214
211
211
211
214
211
211
211
211
52
52
52
52
52
52
52
52
52
52
52
52
52
211
211
211
211
211
211
214
1YPC CEO ME*tl HE1N LINI PPIIM IMT10 CORR n' IM CONC OF
on H OCV »T I 1 III! SLOPE 1 IIH 3 IM 8 IIR HCO/HIRS COfF 7 9 10
1
1
9 1.35 51 -.OB 25 23 21 2.0 .93 .0 .U .0
1
1
2
1
1
1
1
I
I
1
1
1
1
1
i
i
i
i
15 i.51 fid -.38 ?0 U 4 2.B .90 3 .9 1.6
1
1
1
3 1.25 21 .95
1
1
1
3 1.25 21 .95
1
1
1
3 1.25 22 .99
1







-------
TABLE   2  (CONTINUED*.   OBSERVATIONS  tNO CM-CULUED INJURY ptRtHETERS TOR Pt«MTS  EXPOSTD TO OZOMC.
EXPOS NUMBER TYPE
DUIMT CONC INJURY OF DEV CONC
PLANT I»R PPIIH « Z INST '
1 2 . 10 0
12. 100
12. 1(JQ
12.200
12.200
12.2110
1 2 . 20 (1
12.200
1 1 . 20 0
12. 21/0
12.200
12.200
12.200
13.100
13. 100
13.200
13. ZOO
13.2110
13.2UO
is. loo
it. ion
1C. 100
1C. 100
in. ion
IU. 100
10.100
IB. ion
la. 100
1 a . 2U o
IB. 200
IQ.2UU
1 0 . ?O P
10.20(1
10. 311 II
10.300
18.300
18. 300
10. 300
IB. 'if)0
7.0 10 5 -1.65
7.0 (»0 57 .18
cotiNt GOLU:N cnoss
.5 50 11 -1.23
.5 9'J 28 -.56
1.0 25 1 -2.33
1.0 75 5 'J .23
2.0 20 13 -1.13
2.0 GO GO .17
1.0 50 70 .52
7.0 tO 7 -1.18
7.0 '10 GO .25
CORN. P10NCCR SOI
1.0 25 10 -.25
CUCUMBER. CHIC400 PICKLING
1.0 25 7 -1.18
1.0 50 1 0 -.38
1.0 9'J GG .41
CUCUMBER. L ONG HtRKCTER
8.0 25 3t, -.36
L »RCM» CUIUPE «N
1.5 70 16 -.10
tCflUCE. PUiK OREEN BOSTON
1.0 10 0 -3.72
i.o ia B -i.m
1.0 22 5 -1.G5
'(.0 31 12 -.20
OATS. C.I . 7575
1.0 10 0 -3.72
1.0 13 15 -1.01
1.0 22 21 -.71
1.0 31 11 -.15
OUTS. C.I. 7578
1.0 10 0 -3.72
1.0 I'J 13 -1.13
1.0 22 38 -.31
1.0 31 BG 1.00
OATS. CHRION
2.0 16 6 -1.56
1
1

I
i
i
i
i
i
i
i
i

i

i
i
i

i

i

i
i
i
i

i
i
i
i

i
i
i
i

i
susc
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
EFFECT SIO fif 0 OEQ INJURY INJURY ll(RCy< INJ CONC HULT t INJ U 8 MR
TYPE GEO ME*N HEIN LINE PPIIM IUTIO CORR PPIM CONC OF
RTF OR N OEV »T T 1 Hit SLOPE 1 IIR 3 MR 8 UR MF.O/TIIRS COEF 7 3 10
211
211
211
211
2ii
211
211
211
211
211
211
211
211
133
133
211
211
211
211
112
112
119
119
49
19
19
I'J
19
19
19
19
19
19
19
I'J
19
10
19
211
1
1
9 2.10 03 -.11 15 9 6 5.7 .99 1 .fl 3.9 5.3
1
1
1
I
1
1
1
1
1
9 1.91 BO -.57 10 10 5 1.5 .91 2 .E G. 0 8.2
1
1
1
1
1
3 2.07 79 .98
1
1
1
1
I
1
1
1
1 1.39 33 .90
I
1
1
I
1 1.36 29 .90
1
1
1
1
1 1.26 21 1.00
1

-------
2 ICGNIINOCU t.
                                       uio  cucuuuu in juny putiHiuns roitriuus cxrosro  10 ozone.
I'l AMI
        I XI'OS               NUMOEW TYI'C
        niiiur  CUHC IN Jin y  ur bcv cone
         mi   I'i'iiH     x       z   IN si
1 U.100
1 U. '11)0
10.100
i a . UK)
iu. bun
1U.MHI
iu.a>n
lu.uin
I a. 11)0
19. 100
20. 100
20. 100
20. 100
20. 100
20. 100
20. 100
20. 100
21 . 100
21. 100
21.200
21.200
21. 300
21.300
21. 300
21.3UO
2|. 300
21. 100
21.300
22. 100
!i. 100
22. 100
22. UIO
22. UIO
22.200
22.200
22.200
22.200
22.200
2.0
2.0
30
60
22
71
-.77
.55
1
i
OMSt CI-IHIIUI) 61
1.0
1 .0
1 .0
1.0
041S.
2.0
ON 1 (114.
I .5
3.0
3.U
3.U
J.I)
C.O
I'Elinii
U .0
PINE.
O.I)
1'lNl.
1 .0
2.0
2.0
1 .0
U .0
a.o
I'llU.
1.0
'» .0
'< .U
1 .0
10
19
22
31
0 »IWY
10
SU3>«
30
15
30
SO
60
30
»• U)
2U
4USIII
25
-MCK
50
25
25
25
10
25
VIMU1
10
15
25
35
I'CJIHSf HI*.
1 .0
1 .0
1.0
1.0
10
15
25
Ib
I'OUJit 11 M.
0
16
39
tl

1 5

10
10
21
23
66
1C

23
UN
35

5
5
I 6
10
5
60
111 4
0
10
25
60
E CKt
0
0
10
J'j
I' MIL
-3.72
-.99
-.28
.36

-1.01

-1.28
-1.28
-.7i
-.71
.11
-.10
E
-.71

-.38

-1.65
-1.65
-.99
-.25
-1.65
.25

-3.72
- 1.28
-.67
.25
M'OIMT
-3.72
-3.72
- 1.28
-.30
i
i
i
i

2

2
2
2
2
2
2

1

1

1
1
1
1
1
1

2
2
2
2

2
2
2
2
HIKKELSOH
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
211
214
211
1'J
19
19
13
19
111
ill
67
67
17
67
6)
67
67
112
112
112
112
111
111
111
111
111
111
111
310
310
3'iU
ViO
310
ViO
310
I'lO
3'iQ
310
1
1
3
1
1
I
1
*
1
i
1
1
1
1
1
1
6
1
1
1
1






6
1
1
1
1
1
1
1
1
1
1


1.93 11




1.31 25








2.27










1.71




1.11 30




1.10 11
                                           CIUCI SIU CIO   010  JNJUIIY  1NJUIIY JIIHESII  1NJ  CONC  MULT * 1NJ  U  8 UN
                                             lYl'C  CEO MEM!  HUN  I. INI        TPIIM       IIUIO    CORR Fl'IH CONC OF
                                  susc HIK   on  N  new »i  \  i  nn siau   i MM  3 UK a nit HFU/IIIRS  con    7    a   10
                                                                                                          .99
                                                                                                           .90
                                                                     107
                                                                            .70
                                                                                                    6.7
                                                                                                   .98
5 .9 1 0. *  U .0
                                                                           -.75    27
                                                                                        12
                                                                                                    3.6
                                                                                                           .89
                                                                                                           .95
                                                                                                           .95
                                                                                                                 2 M  6.1  9.2
 2 3 . 20 0  I . 5
                              .07

-------
TABLE   2 CCONrlNUCDI.  OBSERVATIONS AND CALCUHTEO  INJURY PARAMETERS TOO TUNIS  EXPOSFD 10  OZONE.
        txros               NUMBER
        OURAT CONC INJURY  OF 0 CV  CONC
EFFECT  SID CEO   OEO  INJURY INJURY  THRESH   INJ CONC MULT t IN J  AT  8 II fl
 TYPE   CEO ME IN  Mf AN  LINE         PPIIM       RATIO   CORR Pt> IH CONC  OF
PLANT
23.200
23.301)
23.300
2 3 . 40 0
2 3 . 40 0
z 3 . so n
23.500
2 3 . 00 0
2 3 . tU 0
2 4 . 1U f.l
24. 1UU
24.200
24.200
25. 100
25. 100
25. inn
2!>. 11)0
2 5 . 10 0
25. 100
2 S . 10 0
25.100
25. 100
25. 100
20. 11)0
20. 100
20. 100
20.101
20. 101
20. 101
20.110
20.110
20. lltl
20. 110
20. UO
20. 110
20. 120
II R PPIIM
t
z
INST
it MUSK. RED nor
1.5 35
RADISH. C
1.5 35
RADISH, f.
I .5 35
24
-.71
1
ALVALRONDO
24
-.71
1
«RLY SCARLET OLOOE
23
-.74
1
RADISH. FRENCH OREAKFAST
l.S 35
17
-.95
1
RADISH. ICICLE
2.0 25
S *r FL 0 WE R
2.0 25
3 AF FL 0 Ut R
1.0 15
1-0 30
1.0 GO
2.0 15
2.0 30
2.0 00
4.0 15
4.0 30
4 .0 00
SOUQIUH.
1.5 30
l.S 70
SOYBE AH.
1.5 30
1.5 70
SOYBE AN.
2.0 IB
2.11 30
2.0 CO
1.5 30
1.5 70
SOYDE AN.
1.5 30
32
• FR10
45
t NE IH
1
7
59
4
4 0
7 0
30
44
90
H RUN
1
48
«SOY
4
29
u:r
i
15
4 3
3
4 5
a; OTT
1
-.17

-.13
ASKA-10
-2.33
-1.10
.23
-1.75
-.05
.77
-.36
-.15
1.75

-2.33
-.05

-1.75
-.55

-2.33
-1.04
-.18
-1.80
-.13

-2.33
2

2

1
1
1
1
1
1
1
1
1

1
t

1
1

1
1
1
1
1

1
susc
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
RFF
449
449
449
449
443
449
449
4'|5
449
256
250
256
256
214
214
214
214
214
214
211
214
214
211
S4G
54 G
54 G
SQG
54G
540
214
214
214
540
54 G
214
540
OR N OEV AT T 1 HR SLOP! I MR 3 IIR 8 )IR MEO/THRS COEF 7 9 10
1
1
1
1
1
1
1
I
I
1
1
I
1
1
1
1
1
1
1
1
1
1
9 1.78 59 -.07 15 7 4 3.9 i 97 10 J] 1 9. 8 25 .3
1
1
2
1
1
2
1 I
1
1
1
1
5 1. 01 130 -l.il 33 10 3 4.0 .99 15 JO 27.0 33.2
1

-------
1AOIE   2  ICONUNU(Q).   OUSEftVAIIUNS ANO  CAltulOEl)
I'tlltHtUflS
                          EXPOSfl)  10 OZONC.
tXI'OS
PUHAI COUC
I'l.ANI III! ri'llH
2fc. 120
2C. 120
2fc. ljn
2C.1JO
2C.130
/I.. 1'iU
2t. mo
2C. lt>0
2t.iso
2(.. 11.0
2L. ICO
2C. If 0
2C-170
2C. 1UU
2b. iao
2t. 100
2fc. 1'JO
2 C . 20 II
2 C . 20 0
ZC.2UO
26.?J)1
2 C . 20 I
2 (..«)»
2C. JUO
2C. 300
26. tun
2 1. Mill
2t, U)()
21,. UJU
2t. tOO
2t. tOO
2 fc . tO 0
2t. tOP'
2b.MH>
2L. LOO
2k. tUO
1.5 70
SOY DC IN»
1 .'j JO
I .b JO
SUYUC AN.
2.0 SO
SOVttt »N.
2.0 bQ
SOYUI AN*
2 .U bt)
surui AN.
2.0 SO
SUV tit ANf
2.0 SO
SOY tit AN>
2.0 SO
SUYW AN.
1 .5 30
I .'j TO
SOYUt AM.
2 .0 !.0
•iOYUt AM.
1 .5 30
i.s /a
SOY lit AH,
.5 Gt
.5 65
.S CS
.S Q^
.5 85
.5 85
1.0 15
1 .0 <<5
1.0 16
i.o to
1.0 CO
NUHUIlt lYI'C
INJUHY Of OEV COHC
t 2 IN SI
11
IKAVtHSt
fc
29
UAYNt
5 b
AUK SOY
52
INS
55
UlINT ItlU
51
OOUCN
It
-.IB

-1.5G
-.55

.13

.05

.13

.15

-.10
1

1
1

2

2

2

2

2
1'. I . 101550
15
-.13
2
f. i . 15717%
10
25
01 11' Pi. W A
5 J
YUI1K
1
1C
U AH K b i
J
4
6
7
I 0
21
7
0
11
21
2 t
-1.28
-,67
61
.oa

-1.75
-.16

-1.88
-1.75
-1.56
-1.1B
-,ao
-.81
-1.16
-1,11
-1.08
-.81
- ,U 7
1
1

2














1
susc
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
tuici s ru cto uto iNOJitr IMJUIIY niric^u JNJ CONG nut i t JHJ AY a un
lYI't ULO HC »H M(AH LINt PI'MH rt At 10 CURR IV IIM COMC OF
ii (T un H otv AI i i tin sttrt i un 3 nit a tin neo/tiiRS coir 7 'j 10
5lb
bib
516
SIC
5iG
J82
-J82
5BZ
362
J02
382
1112
302
302
3112
3B2
382
SIC
SIC
51 £
302
382
SIC
SIC
510
13'J
139
139
13 'J
li'J
lia
U'J
130
130
13')
130
1
2
1
1
2
1
1
1
1
1
1
I
i
1
i
i
1
i
i
2
1
1
1
1
2
1
1
1
1
1
1
1
1
1
I
1

-------
TABLE   2  CCONTINUIO).   OBSERVATIONS  4ND  CtLCULllEl)  INJURY PARAMETERS  FOR PUNTS EXPOStO  TO OZONE.
I
[
PLANT
26.500
2G.ain
2C..5UO
2 G . UJ 0
26. U10
2G. MO
2G. 500
2G.SOO
2 1 . 50 (t
26. 500
26. 500
26. 500
26. SOU
26. U1Q
2b. 500
26.500
26. 500
2G.GUU
2G.GUO
20. von
2G. TOO
26. TOO
26.000
2G. QUO
2 G . BO 0
2G.U10 i
26.900
26. 'JUU
27. 100
27. UJD
27. 100
27. 100
27. 100
27. 100
27. 100
27. 100
27.100
27. 100
27. 100
27. 1UU
27. 100
20. 100
LXPOS
>UR»T CONC
MR PPIIM
1.0 60
2.0 35
2.U 35
2.0 35
2.0 so
2.0 50
2.0 50
1 .0 25

1.5 30
1.5 70
sortie KHf
1.5 30
1.5 70
SOYOE *N.
1.0 &
1.0 15
1.0 25
1.0 30
1.0 50
1.0 Q3
2.0 0
2.11 15
2-0 30
'l.O (1
1.0 IS
•t.tl 30
SPINtClli
.5 50
INJURY
I t
2B
1 B
22
22
M 3
44
48
13
16
21
26
31
38
45
12
43
U RE
57
DELH M
12
4 n
IK RK
1
57
lUWKtYl
5
44
KENT
0
0
0
1
73
96
0
0
25
0
3
7 7
N> nniL ^
27
NUHOCR
OF OEV I
z
-.50
-.92
-.77
-.77
-.18
-.15
-.05
-1.13
-.99
-.01
-.64
-.50
-.31
-.13
-1.18
-.IB

.18

-1.18
-.02

-2.33
.18

-1.65
-.15

-3.72
-3.72
-3.72
-2.33
.Gl
1.75
-3.72
-3.72
~.C7
-3.72
-1.8B
.74
40
-.&!
TYPE
CONC
IN 5T
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1

2

1
1

1
1

I
1

1
1
1
I
1
1
1
1
1
1
1
1

1
susc
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
t
RET
139
139
139
139
139
139
139
139
139
139
139
139
139
5
-------
2 icoHiiuium.   oBStnvuioNS ANO ctLCuuuu  iMJtmv PMJMicitns rou PUNTS txi>osrn TO OZONE.
LXI'OS
DIIIUI CONC
PLANT III) I'I'IIM
28. 10 U
20. 1011
28. 100
2(1. 100
28. IUO
2(1. 100
2U. 100
2U. 100
28.10 0
2'J. 100
2'J. 100
2!). 100
29. 100
JO. 100
in. too
IU. 100
30. 100
JO. 100
10. 100
JO. IUO
jo. 100
111. 10 1
3(1. 10 1
JO. 110
SO. 110
10. 120
JO. 120
HI. no
JO. 1JO
IU.200
JO. 200
ID. ZOO
30.2UO
JO. 200
10.2110
30. «)0
J(J. JOO
30.3UU
JO. J0(l
lU.'iOO
.5
1.0
1.0
2.0
2.0
1.0
7.0
1 .0
SOU
1.0
1.0
1.0
99
25
75
20
60
50
10
10
i N.IUHY
s
51
7
50
6
56
37
0
1 1
mmuiii
OF OCV
z
.10
- 1.18
.00
-1.56
.15
-.33
-3.72
-.35
tiff
CONC
insr
i
i
i
i
i
i
i
i
*SII. SIMMtll
25
50
99
suiss cm
2.0
2.0
2.0
2.0
2.0
2.0
2.0
(Oil
2.0
too
2.0
rou
2.0
rou
2.0
rou
2.0
2.0
2.0
2.0
2.0
run
1.0
1.0
1.0
ion
2.0
JO
27
10
16
22
20
21
4CCOi
27
t£CO»
27
ceo.
27
4CCO.
27
VJCO.
27
10
16
22
20
4CCO.
25
50
99
ceo.
10
2
25
66
-2.05
-.67
.11
IUt (OHUMOOK 0
1 3
7
0
1
2
3 3
1 3
d 1 U
1 1
1C N Utt
8
-1.13
-1.18
-3.72
-2.33
-2.05
-.11
-l.U

- 1.23
12
-l.il
i
i
i
UN \
2
2
2
2
2
2
2

2

2
uiiirt uoto
7
NC-a5
6
11: in i b;
10
0
7
11
5 2
I£L C
6
10
61
It I UJ
0
- 1.18

-1.56
I
-1.28
-3.72
-1.18
-1.08
.05

- 1.56
-.25
.28

-3.72
2

2

2
2
2
2
2

1
1
1

2
SUSC
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
CITLC1 SIU OEO UtO IHJUKY INJUHY IIIRT.MI IN J CONC HUL 1 * IN J %T 8 IIH
1YPE 010 HUM MUN I. JNI FPIIH fWJO COHH PP IN CONC OF
HIF on H uru u r i tin stcrr i nn 3 mi o HR nn>/nirc COEF ^ 9 10
211
211
211
211
211
211
211
211
211
211
211
211
211
6
351
361
361
3C1
361
3G3
6
351
351
351
351
351
351
351
351
351
3d
361
361
361
351
211
211
211
211
3fcl
1
1
1
i
i
i
i
i
9 1.83 JO -.01 17 17 17 1.1 .96 .0 .0 .1
1
i
1
3 1.75 76 1.00
1
1
1
1
1
1
1
7 1.19 11 .91
1
1
1
1
1
1
1
1
1
1
1
1
1
5 1.11 32 .92
1
1
1
3 2-12 73 .97
1

-------
TABLE   2  (CONTINUED).   OBSERVATIONS »NU C»LCUHTEO INJURY  P*R»MEICRS  TOR PLANTS EXPOSED TO OZONE.
EXPOS NUHQCR TYPE
DUR»T CONC INJURY OF UEV CONC
PLANT Illl PPIIH t 7 IHST
JO. 1110
30.4UO
J 0.100
30.1(10
30. ion
JO- MO
30.500
iU.SU 0
JO. 500
JU.5UO
30.UJO
ju.sun
JO. !XJO
JO. M)0
jo. coo
JO. COO
ju.con
JO. COO
jo. to a
JO. GOO
JO. tOO
jo. ran
JO. 7IJO
JO. 7110
jo. /no
JO. 700
JO. 7110
JU. TOO
JO. 700
ja. onu
jo. nau
to. win
50. BOO
JO. BOO
jo. isio
JO. UQO
JO. QUO
jo. QUO
ju.'jin
jo. am
JU. 'MO
JU. 900
2.0 1C
2.0 22
2.0 2B
2.0 21
ion *cco.
i.n 20
l.O JO
2.0 20
2.0 JO
J.U 20
J.O JO
4.0 20
1 .0 JO
TOO CCOt
L.O JO
1.5 20
2.0 JO
J.U 10
J.O 20
G.O 10
TOO *CCO,
2.0 10
2.0 It
2 .0 22
2.0 2U
J.O 25
'J.O 50
J.O r 5
100 
-------
lAUlt   2 ICONI IIIUEO I.   OUSEDVOlOHi UNO  CMCUMItU 1NJUHV l'»MHIltllS (OKI'IINIS EXPOSED  TO OJOHf.
I'tANI
        i xros              NUHDER ni'C
        OUIUI CONC  INJURY Of  DCV CUNC
         UK   IM'IIN     *       Z
          fiiici sio GEO  oio   INJUN* INJURY nmrsii   INJ cure HUI.I  * JNJ «r a UK
           lYI'C  CEO Mt*N HE»N   LINE         fM'IIH       RUlO   CORK  H> IH  CONC OK
susc itrr   OH H  ocv u I i 1111  SLU-L   i tin  3  IIH e mi  tit u/i tins cotr    7    s   10
10.
30.
30.
31.
31.
31.
31.
II.
It.
31.
31.
31.
31.
32.
32.
32.
S2.
12.
32.
12.
12.
12.
12.
32.
32.
32.
32.
33.
31.
33.
33.
33.
33.
13.
•JUU
•joo
•jo ft
200
200
300
300
4UO
mo
MM)
too
LOO
U10
100
100
200
200
U1U
300
400
400
ujo
U10
too
(.00
JUO
All)
1110
tuo
100
100
11)0
100
IOO
3.0
3.0
I Oil
l.b
ion
1.5
ron
1 .5
I OH
1 .5
50
75
45
48
-.13
-.05
2
2
«CCO. UTIIII10M
10
tro. M*«
10
34
M'U.
26
*io. onto UR
40
33
«ro. OHIO uu
10
IOMUO, VE
1 .5
I OH
6.0
40
MO. VE
30
HJUIGIUSS.
6.0
50
36
14 Ml
26
13L
40
DELE
20
_

_
- 7
_
-25
-
7U7a
_

_
.41

.67

-44

.36

.64

.25
1

1

1

1

1

1
n ui-occruss
_
.84
1
roKEGims* luaiiioiii RED EESCUE
6 .0
30
lOlirWUSSi
6 .0
tun
6 .11
30
ECR4SS.
30
IUIIIUIUSS.
I, .11
30
lOREUIUSS •
6.0
30
IUKEOIUSS .
.5
.!>
.0
.n
.0
.0
.0
so
O'J
2£,
2J.
50
»!,
•J'J
60

.25
1
E4HURI RYEtilMSS
60
H4MI
60
Mfc IU
2U
P- 16
6(1

mi

.25
H RYtGH
.25
OH UUIEQIUS
-
.84
1
4SS
1
S
1
UCRHUnlGRtSS

n tuu «u N
0
42
0
4
2 U
5 a
52
-3
-
— 1
- 1
-


.25
1
HEO EESCUt
.12
.20
.12
.75
.58
.20
.05
1
1
1
1
1
1
1
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
2
352
352
352
448
448
448
448
440
'I'lll
448
448
440
4(1 8
44
44
44
kt
44
44
44
44
44
44
44
44
44
44
214
214
214
214
214
214
21 4
1
i
7 1 . 5'J
1
I
i
1
1
I
1
1
1
i
t
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
                                                                       34
                                                                                    12
                                                                                          21
                                                                                               37
                                                                                                      2.9
                                                                                                             .97
                                                                                                                     .U
                                                                                                                          .U
                                                                                                                               .0

-------
IADLE  2  CCOHJiNUtDI.   OBSERVATIONS  4NO C4LCUL4TED INJURY P*R*Mrit(jS FORPL4NTS  EXPOStO 10  020NF..
[XFOS
PUR4T CONC I
PLAN! MR PI'IIM
3 3 . 10 0
33.100
33. ion
33.100
33.11)0
33. 100
33. 100
3 3 . 1U 0
33.100
1. 100
1 . 10 0
1. 100
1. 100
1.200
1.200
1.2UO
1.2QO
1. 300
1.300
1.300
1.300
2.000
2.UJO
3.100
3. 100
3.100
3. 100
3.100
3. inn
3. 100
3.100
3. 1110
3. 100
4. 100
4. 100
'1.200
4.200
4. 300
4.300
4.400
2.0
2.0
2.0
2.0
2.0
4.0
7 .0
7.0
UHC 41 .
1.0
1.0
1.0
4LF 4LF
1 .0
4 .0
4 .0
15
20
30
60
CO
GO
10
40
UEIL
25
50
99
4. it
10
15
25
NUHOER TYPE
NJUHV OF OEV CONC
* Z IN SI
0
1 —
12
SO
59
74
0
4 b
S
1
a
67
RN AL
0
15
15
3.72
2.33
I. IB
.20
.23
.64
3.72
-.10

2.33
1.41
.44

3.72
1.04
1.04






1
1

1
1
1

1
1
1
4LF 4LF4. DU PUITS
4.0
4.0
4.0
4LF 4Lf
a.o
4Rno»v
.5
1 .5
1.0
1.0
2.0
2.0
4.0
7.0
7.0
10
15
25
4. 4t
25
IT 4'E
50
99
25
75
20
GO
50
10
40
4Z4LE 4. 4U
4 .0
DE4N,
4 .0
III UN.
4 .0
UE4N.
4.0
25
E4CLE
25
0
5
15
L4NIIC
0

0
0 -
0
0
0
0
3.72
1.G5
1.04

3.72

3.72
3.72
3.72
3.72
3.72
3.72
0 -3.72
0
0
SK 4
4

6
3.72
3.72

1.75

1.56
1
1
1

2

I
1
1
1
1
I
1
1
1

1

1
HARVEST EH
25
PROVI
25
1
Of R
2
2.33

2.05
1

1
susc
2
2
2
2
2
2
2
2
2
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
EFFECT SID CEO OEO IHaiRY INJURY THftf Sll 1NJ CONC MULT * IN J 4T 8 IIR
TYPE OEO HE4N ME4N LINT PPIIM R 41 10 CORR HP IM CONC OF
RtF OR N OEV 4T T 1 MR SLOPF 1 HR 3 IIR 8 IIR HEO/THRS COEF 7 9 10
214
214
214
214
214
214
214
214
214
214
214
214
214
52
52
52
52
52
52
52
52
340
340
214
214
214
214
214
214
214
214
214
214
109
109
109
109
109
109
109
1
1
1
1
1
1
1
1
15 1.47 81 -.4G 33 20 13 2.4 .91 J} .1 .1
1
1
I
3 1.G5 86 .98
1
1
1
3 1.43 30 .83
1
1
1
3 I. >t2 32 .93
1
1
1
1
1
1
1
1
1
1
1
9
I
1
1
1
1
1
1

-------
IAIHE   2  icONIlNUrut.   OUSERVlriONS  *NO CU.CUUlEU iHJUHY  ftlllHtUHS  FOR PUNTS  EXCOSfD  fO
IXI'OS NUHQCK IYTL
IJIJIUl COHC INJUUY OF UtV COHC
I'MNI Illl I'I'IIM 1 Z INir
1.400
1. 600
1 . 60 (I
!>. lUlt
5.100
5. 100
5. 100
(..CUD
t.OJO
b.WO
b.mo
b.mil
b.UlU
b.UOO
6 . 1C U
b. 100
b. 100
b. 10 11
b. 100
t.UJO
b. 1UO
b. 1UO
b. 10(1
b. 100
C. 101
b. 101
b. 101
b. 11(1
b. 11U
b. itn
b. 120
b. 120
b. 120
b. 1)0
b. UO
C. MO
b. HO
t. 1'lU
susc
UHN. SlUIMGltSS UUCK VU.ENI1NE 3
1 .(J 25 3
- l.BB
1
UUMt UNWH CHOP
1.0 25 0
1.0 50 0
1.0 3 1
1 .0 7 !. J 1
2.0 20 2
2.0 bO U
H.O !)0 6
1.0 10 0
7.0 HO 1
CMItYStUMI IMUI1 >
J.O 30 5
'1.0 tO lb
Cllll VSUUIMHUH.
i.O JO S
1.0 HO 15
CIIU Y SOI lilt HUH .
J.O iO S
1.0 10 «0
tlllltS*UJIIFHUH •
J.O 30 5
i| .0 10 
-------
TABLE   2 ICUNTlNUED t.  OBSERVATIONS »NO C*LCtJL»IEO  INJURY P»R*HtltHS FoRPLlNTS  EXPOSfO
OZONE.
EXPOS NUMBER TYPE
OUIUT CONC INJURY OF DEV CONC
PLANT HR PPHH t Z INST i SUSC.
G.
G.
G.
G.
G.
G.
G.
G.
G.
G.
G.
G.
G.
G.
G.
G.
G.
6.
G.
G.
G.
G.

G.
110
ISO
150
15(1
1GO
1GU
ISO
200
200
200
3UO
300
300
'lUO
100
100
500
too
51)0
MO
HID
GOO

700
6. TOO
G.
G.
G.
G.
G.
G.
G.
7.
7.
7.
7.
B.
TOO
co n
BOO
BUII

-------
I Mil I   2 CCONI INOCDI.   GUSEHViTIUNS INU C *l.COL* IE I)  INJUHV I'MUMtttOS roillMtHtS EXPOS I'D T t)  OtOHl.
        tXI'Oi               NUHllltt  Ul't

        OUI141  CONC INJUIIV  OF OEV  CONC
PI.ANI    Illl    Pl'lin     T       I    IN SI
          tirici  su» etc   oto  INJURY  INJURY  unitsii  IHJ  CONC HUL!  * INJ u a mi
           irrt   ccb ME MI  MC»N  i.INC.        PPIIH        nuio    conn  ivin CONC or
susc itir   on N   orv u T  i  iin si.trc   i MR 3  im  a 1111 nco/iuns coef    7910
 0.100  CONN.  SUUl
                                                  62
9. 1011
a. 100
a. too
a. too
9. 100
a. 100
9. 100
a . 20 o
a . 2u o
a. 200
a. 200
t .O
1.0
1.0
2.0
2.0
2.0
25
50
a a
15
30
60
co HUH. *a
1.0
1.0
1 .0
3.0
50
ad
a a
40
a. 200 coiioti. »a
10. 10(1
10. 100
10. 200
10.200
11. 100
i i . 10 a
11. 100
i
i
i
i
1
i
t
i
i
i
t
i
i
i
i
. 100
. 11) 0
. 100
. 100
. 10 0
. 100
. 100
. 100
. 100
. 100
. ion
. 100
. 100
.100
1. 100
t 1. 100

i. mo
12. 100

^.200
1 2 . 20 0
4 .0
CHOMN
4 .0
cnouii
.5
.5
1.0
1.0
1.0
1 .0
1 .0
2.0
2.0
2.0
2.0
2.0
4.0
4.0
'i.O
4 .0
) .0
7.0
25
V{ 1OI
25
VI 101
SO
•19
15
25
30
60
75
IS
20
50
60
60
15
10
50
60
10
40
CUCUHUIII t L
U.O
rut .
u.o
riu.
25
tui.su
25
4
15
2 /
b
1
6
M
5
25
95
40
-1.75
-1.04
-.61
-3.72
-2.33
-1.56

-1.65
-.67
1.65
-.25
1
t
1
1
1
1

2
2
2
2
1 » S J- 1
0
-3.72
1
. UllHUNU
0
-3.72
1
. ItHIIOIll
a
4 3
0
d
2
I U
3 a
0
2
G
a
3 3
1
7
32
ta
0
15
ONU
0

(1
-1.41
-.18
-3.72
-1.41
-2.05
-.92
-.31
-3.72
-2.05
-1.56
-1.34
-.44
-2.33
-1.40
-.47
-.92
-3.72
- 1.04
H III KCT til
-3.72

-3.72
1
i
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
I

2

2
OOOOHS
3
3
3
3
3
3
3
3
3
3
3
3
j
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
J
214
214
214
214
214
214
214
S29
529
523
529
529
52
52
52
52
214
214
214
214
214
214
214
214
214
214
214
214
214
214
214
21 't
214
214
214
340
340
340
340
1
1
1
I
1
i
6
1
1
1
1
4
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
1
ia
i
i
i
i
                                                            2.31
                                                            1.26
                                                                       128
                                                                               .96
                                                                        77    -.55
                                                                                      10
                                                                                     45
                                                                                           52  134
                                                                                           25
                                                                                                 15
                                                                                                        7.0
                                                                                                        1.7
                                                                                                               .97
                                                                                                               .90
                                                                                                                       JJ
                                                                                                                       .0
                                                                                                                            .0
                                                                                                                                 .0
                                                                                                                                 .0
                                                            l.UU
                                                                         91    -.14
                                                                                      25
                                                                                           21
                                                                                                 IB
                                                                                                        3.9
                                                                                                               .33
                                                                                                                       M
                                                                                                                            -O
                                                                                                                                  .0
 12. mo   a.i)
                            -3.72
                                                  I'll)

-------
TABLE  2  (CONTINUED).   OBSERVATIONS AND CALCULATED  INJURY  P*fl»METFRS FOR TUNIS EXPOSED  10 OZoNt.
PLANT
12.300
13. 100
13.100
11. 100
14. 100
1 4 . 1U 0
is,, inn
11>. 11)0
it. ID n
16. 11)1)
16. 100
IG. 100
IG. 100
16. 1OO
16. 100
iG.om
16. OK)
1 G . 01 0
iG. 01 n
IG. Oil)
16.200
11.200
1G.300
16. 30 U
1G.1UO
1 G . 40 0
1C. SOU
16.500
in. LO n
1C. LOU
1C. 711 0
1C. 7UO
16. 01)0
1 6 . 00 0
17. U)l)
EXPOS NUMBER
DURAT CONC INJURY OF OEV
MH PPMM * Z
Flit, UHITE
6 .0 25 G -1.56
Hi Ml OCX. EASTiDN
7.0 30 0 -3.72
7.0 SU U -3.72
HOLLY. ENGLISH
8.0 25 G -1.56
LARCH. JAPANESE
1.0 2b 2 -2.05
1.0 5(1 13 -1.13
1.0 93 54 .10
2.0 15 1 -2.33
2.0 30 5 -1.65
2.0 GO 30 -.31
TYPE
CONC
INST SUSC

2

1
1

2

1
1
1
1
I
1
LETTUCE. D»RK GI1CEN BOSTON
2.U 30 0 -3.72
2.0 60 4 -1.75
3.0 30 13 -1.13
3.0 60 3t -.50
M AP LE • S Ua H
1 .5 70 30 -.52
2
2
2
2

1
LETTUCE. GRAND lUPIDS FORCING
I 1.5 70 24 -.71
LETTUCE. IMPERIAL »45G
1.5 71) 21 -.71
LETTUCE. BUTTTR CRUNCH
1.5 70 21 -.71
LETTUCE. BIG BOSTON
1.5 70 13 -.88
LETTUCE. ROMIINE
1.5 7f) 11 -1.23
LETTUCE. SIMPSON. BLACK
1.5 70 10 -1.28
LETTUCE. CHEAT LAKES
1.0 25 0 -3.72
1

I

1

1

I
SEEDED
1

1
3
3
3
3
3
3
3
3
3
3 •
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
EFFECT STD GEO CEO INJURY INJURY THRESH IHJ CONC MULT t IN J AT B MR
TYPE GEO MEAN ME»N LINE PPItM RATIO CORR TV IIH CONC OF
RET OR N DEV AT T 1 lilt SLCI'T 1 II R 3 HR 8 M R MED/ THRS COEF 7 9 10
340
340
340
17
17
17
340
310
211
211
211
211
211
214
211
223
229
229
229
229
119
119
119
449
449
449
44G
449
449
449
149
449
449
449
211
1
1
1
1
1
2
1
1
I
1
1
1
1
1
6 1.91 98 -.35 21 14 10 4.7 .99 .2 .6 .9
1
1
1
1
1 1.70 1055 -2.53 304 19 2 3.5 .96 67.9 82.6 87.2
1
1
1
1
1
1
I
1
1
I
1
1
I
1
1

-------
lAUlt    2  (CUI4TIMUI 01-   UUSCHtftTIUHS tMU  Cit.Clll.MtU  IHJIMY  I'MUrtlltltS roRt'LifllS  CXPOSt'O 10 OZOUC.
tXI'OS
OUIM1 COIJC
(M*H1 Illl I'f'IIH
7.
1.
7.
U.
U.
U.
ia.
to.
1ft-
Itt.
13.
ia.
la.
i a.
la.
ia.
la.
20.
20-
20.
21).
20.
20.
20.
tQ.
21).
20.
21.
21.
21.
21.
21.
21.
21.
21.
21.
21.
21.
21.
21.
1UO
Jllll
l&O
100
1011
J0l>
ion
100
too
100
1110
100
inn
1(10
inn
uto
11)0
too
mo
m a
11)0
Ull)
ino
100
100
100
11) 0
HM
111 V
an
Ull
no
no
HO
110
120
120
120
120
130
1
t
.0
.0
50
a a
UUMlllU lYI't
INJURY OF 01V CONC
X I lMi.1
6 -1.56
1U -.05
1
i
SUSC
3
3
(MIS. ClINIllM) 61 4
1
1
1
2
2
2
.0
.11
.0
.0
.0
.0
2'j
50
au
it
10
Ml
a
10
2 9
0
1 —
i a
1
i
.11
.28
-.55
3
.72
2.33
-
.00
i
i
i
i
i
i
UNION
1
1
1
2
2
2
.n
.0
.0
.0
.0
.0
25
50
aa
15
30
CO
0
i
2
i
3
20
oiicmnn ciuss. poi


i
1
2
2
i)
7
7
.5
.!»
.0
.0
.0
.(I
.0
.0
.U
•JO
au
25
75
20
60
50
10
40
flltlUlNCil.
1
1






1
1
1
1'
1
.n
.0
.0
I TUN!
.0
.0
.0
IT UNI
.0
.0
.0
25
50
a a
0
1 (i
0
2i
0
IS
i a
0
i
h 0 IU CUT
0
\
11
3
2
2
2
I
-
.72
.33
.05
.33
.00
.01
i
i
t
i
i
i
omc
1
-
.72
.33
1.72
-
4
1
—
j
I

3
2
I
-fll
.72
.01
.till
.72
.75
EYES
.72
.33
.00
i
i
i
i
i
1
i
I
1

1
i
i
I. Hilt JllNS
2!i
50
13
n
12
47
3
1
-
.72
.10
.33
i
i
t
4. It 0 HtCIC
25
!iO
a a
i num.
.0
25
0
1
30
UtUH 1UH
(I
3.72
1
-

.10
.52

3.72
i
i
1

i
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
LIllCl S.IU UfO GttO IMJURV tttJURY UHtf Sit IHJ CUHC HUl « t IHJ IT 8 IIR
IVI't CtO HE»M HC*H I.1NI PI'IIH fUTIO COHfl 0> IH CONC Of
IMF DU N IHV Mil lilt SLcrC 1 IIR 3 lilt 6 IIR Hi D/ 11IRS COtf 7 a 10
211
211
211
211
211
211
21 H
211
211
211
211
211
211
211
211
il'i
211
211
2t1
211
211
211
211
211
211
211
211
162
162
162
162
162
162
162
162
162
162
162
162
162
1
1
3 1.15 36 ' 1^00
1
i
i
i
l
i
t, 2.11 112 .53 20 37 61 5.7 .92 M .0 .0
1
1
1
1
1
i
t 2. 1O 531 -2.02 ta 6 X 7.7 .97 It Jl 55.1 GO.l
1
t
1
1
t
1
1
1
1
3 1.S7 136 ~.<*D <»0 3i 21 2.B .91 .0 .0 .0
1
1
1
3 1.68 171 1.00
1
1
1
3 1. 50 101 .36
1
1
1
3 1.8,1 113 .37
1

-------
TAULE   2 (CONTINUED!.   OUSERVATIONS AND  CALCULATED INJURY  PARAMETERS  fOR PLANTS  EXTOSCO  TO OZONE.
        EXPOS               NUMOER TYPE
        OUHAT  CONC JNJUI1Y OF DEV CONC
PLANT    IIR    f'PIIM     «      Z    INST
          EEEECT  STO GCO   CEO  INJURY INJURY  TIlRFSH   INJ CONC MULT * IN J  AT  0 MR
           TYPE   CEO MEAN  MEAN  LINE         PPMH        RATIO   CORR PP IM CONC OF
SOSC REF   OR N   OEV AT T  1 IIR SLITC   I MR  3  MR 0 IIR  MED/TIIRS COEE   7    9    10
21. 130
21.130
21. HO
?1.11«J
? i . i>t n
?1.1'|0
?i . 110
71. 150
21.100
?l. 150
21. ISO
2 1 . 16 0
21.100
21. ir>o
21. ICO
? 1.300
21.300
2 1 . 30 0
21.300
?i.'ion
zi.'ino
•/l.'iOQ
21.100
2 1 . HI 0
21.51)0
21.500
2 1 . so n
? i . MI o
?1.C(IO
?l.C(lf)
21. COO
21.700
21. 700
2 1 . 70 0
21.700
21.800
21. BOO
21. COO
1.0 50
1.0 00
PETUUIAt
1.0 25
i.O 50
i-n 99
f>ETUNH«
1.0 25
1 .U 50
1.0 03
ft TUNJA>
1 .[) 25
I .0 50
1 .0 00
PETUNId.
1.0 25
1 .0 50
1.0 09
PCTUHIlt
1.0 25
I .0 50
1.0 00
PEruMT*.
1.0 25
1.0 50
I .0 09
PETUNH.
1.0 25
1.0 50
1.0 90
PC rum*.
l-O 25
1.0 50
1.0 99
PETUril*.
1.0 25
1 .0 50
1.0 09
0 -3.72
7 -l.«»B
VICTORY
0 -3.72
1 -2.J3
22 -.77
PARTI PINK tPINKI
0 -3.72
1 -2.33
27 -.61
fE AClf OLOSSOH
1 -2.33
1 -2.33
38 -.31
tt-UE SCA
0 -3.72
1 -2.33
i -2.33
ULAC TIME
0 -3.72
I -2.33
1 -2.33
OICItRY OLOSSOH
0 -3.72
3 -i. an
10 -1.20
CA L Y PS 0
0 -3.72
3 -1. OB
25 -.67
ItACIITS K CREAM
0 -3.72
0 -3.72
2 -2.05
DLUE D AHUOE
1 -2.33
9 -1.31
30 -.31
1
1

1
1
1

1
1
1

1
1
1

1
1
1

1
1
1

1
1
1

1
1
1

1
1
1

1
I
1
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
1C2
162
162
162
1C2
162
162
162
162
162
162
162
162
162
162
162
162
162
162
162
162
162
162
162
162
1C2
162
162
1C2
162
1E2
162
162
1G2
162
1C2
162
162
1
1
3 1.05 300
1
1
1
3 1.60 111
1
1
t
3 1.56 133
1
1
1
3 1.98 153
I
1
1
3 2.68 701
1
1
1
3 2.60 701
1
1
1
3 1 .76 101
1
1
1
3 1.57 12B
1
1
1
3 2.20 685
1
1
1
                                                                                                               .86
                                                                                                              1.00
                                                                                                              1.00
                                                                                                               .06
                                                                                                               .87
                                                                                                               .87
                                                                                                               .96
                                                                                                               .99
                                                                                                               .86

-------
lAUlt   2 ICUNI1NUIU).   OUSERV4T10NS *NU CMCIU.UIO  INJURY  P*R*H[ltllS
PLANTS  tXPOSfl) 10 0/0t4t.
IXI'OS NllHBlll IV PE
DUIMT CONC INJURY Of I) TV CONC
PLANI MR PPIIH I 2 !N il > SUSC
21.
21.
21.
21.
21.
22.
22.
22.
22.
22.
22.
22.
22.
23.
23.
23.
23.
23.
23.
23.
23.
23.
23.
21.
23.
23.
23.
23.
23.
23.
23.
23.
23.
23.
23.
23.
25.
uno
9110
200
900
<-«)0
inn
100
200
200
300
300
100
100
U) 0
(VI 0
000
01)0
too
100
100
100
ion
200
20 n
200
200
200
300
300
300
100
100
100
500
too
win
100
Pi IUIII
1.0
1
1
.0
-0
Pt IUMI
8
P
8
''
8
P
a
.0
INI.
•n
IHI:.
.0
mi.
.n
PJNt.
1
1
1
.0
.0
.0
POlNSl
3
1
3
3
P
3
1
3
J
P
1
1
P
1
1
P
1
1
P

.0
.u
.0
-0
oinsr
.0
.0
.0
.0
oi tm
.n
.0
OIHU
.0
.0
uiir.i
.0
.0
OlNJI
.-,
»« fCJ
25
50
99
>r iw U-
Q
9
36

-3.72
-1.31
-.36

1
1
1
I, IIOULtlH
25
I'l ICII
25
lit U
25
6

U

Jl
-1.56

-J.72

-.50
2

2

2
SCOICH
25
UIUIE
25
50
99
II 1 A
30
15
(.0
75
III A.
30
15
60
75
III A.
25
35
II 1 A.
25
35
n i A.
25
35
II I A,
•-,0
16

1
2
1
III (0 .
5
20
10
10
-.99

-2.33
-2.05
-t.75
PINK. Will
-1.65
-.6*1
-.25
-.25
2

1
1
i
It VII)
2
2
2
2
AMflETIK IHGG
0
0
2 0
10
- 1.72
-.1.72
-.81
-.25
2
2
2
2
tCKESPOlNl C-l
0
25
U <«K
0
5
Will 1C
0
15
-3.72
-.67
II LI) ANN El
- 1./2
- 1. EH
UINEIIC
-1./2
-.13
2
2
11 III 0
2
2
III 110
2
2
M1KKEI Wllllt
5
- 1.65
1
3
3
3
3
i
3
1
3
3
3
3
3
i
3
3
3
3
3
3
3
J
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
llttCI Sll) CCO CtO INJURY INJURY Him ^11 INJ CONC HUM X INJ AT 8 MR
iri't OtO Hf UJ MMH I lilt PPIIH RMIO CORK PPIIM CONC OF
III) (111 N DCtf AI I I IIR Sl.(l>t 1 II n 3 lilt 8 lilt HCO/HIRS COtf 1 9 10
162
162
162
162
162
310
310
310
310
310
310
310
31(0
211
211
211
211
6U
GQ
6U
60
GO
68
68
60
CO
68
310
310
310
310
310
310
310
J10
310
211
3 1.90 122 1.00
1
1
1
3 i.51 101 .97
1
1
1
i
i
1
1
I
1
1
1
3 10.926605 1.00
1
1
1
1
1 1.86 78 .97
1
1
I
1
1 1.2 1 02 .90
1
1
2
1
1
2
1
1
2
1

-------
TABLE   2 (CONTINUUM.   OBSERVATIONS AND  CALCULUEO INJURY  PUttHEfniS  fOR PUNTS EXPOSED  16 OZONE.
EXPOS NUHUfR TYPE
DURIT CONC INJURY OF IHV CONC
PLANT MR PPIIM t Z INST
25. 100
25. 100
25. 100
2 5 . in o
25. 11)0
25. mo
25. 100
25.100
25. 100
25. 100
?5.ioo
25.100
20. 100
26. 100
20.200
2k. 21)0
2 G . 20 0
26.200
26.200
26. 300
2 6 . iO 6
2 6 . 30 0
26.300
2 b . M) (1
26.10-0
26.1UO
26. <<00
2 6 . <|0 0
2G.1UO
26. HIP
?b.50t)
2 6 . !>0 0
26. LOO
?G.tnn
26.600
20.100
2 B . 10 0
28. ZOO
28.200
20. 300
.5 99
1.0 25
1.0 25
1.0 50
1.0 75
1.0 93
2.0 20
2.0 GO

-------
        2  (cum
                    i.
cucuuuo  ift.iiiiiY
                                                                        r on nuns  txcosio 10
        CXI'US             NUHUtlt  ITI'l
        IJUIUl CONC 1NJUIY OF OEV  CONC
I* i-AMI    mi    iM'tm    «       2    mil
                                         SUSC II IF
        tirici  sio UEo  uro  INOJIIY  INJURY uint sii  INJ CONC nu.r  * INJ u a tin
          lYI'f   Ct 0 ME 4M HftM  I INt        f'PIIH       IMTJO   CORK  (rill  CUNC OF
          on  N   ocv M  r i mi suua   i  MR i tin a tin Hco/nms coin    ;    
-------
TAULE   2  (CONTINUED I.   OBSEI1V 4TION S  »NO CM.CULMEO  INJURY PlR4HlTER5  fORPLlNIS EXPOSED TO 020NE.
PLANT
3.
11.
1 1.
11.
11.
11.
11.
11.
11.
11.
23.
23.
31.
31.
31.
31.
31.
31.
0.
0.
8.
3.
3.
3.
100
0(10
mo
mo
win
QUO
con
C110
uno
aio
ion
100
100
100
100
100
100
1X10
inn
1110
100
100
1110
loo
1
20.100
20.
20.
20.
20.
20.
20.
20.
23.
23.
23.
9.
9.
9.
•in a
100
100
MID
800
liOQ
8UO
100
inn
100
100
HI a
icm
EXPOS HUHUER
OURM CONC INJURY OF OEV
MR PPIIH t Z
UE4N.
.5
1.0
2.0
2.0
2.0
2.0
2.0
1.0
PINTO
35
35
IS
25
35
35
15
35

a -i
20
1 -I
20
28
35
53
52

.11
.01
.75
.111
.50
.30
.00
.05
TYPE
CONC
INST

2
2
2
2
2
2
2
2
DUCKUEEO
1.0
II 40 ISM
l.S
1.0
1.0
1.0
1.0
25
• C V
99
50
50
99
99
TOH4TO. FBI
2.0
2.0
CORNt
12.0
12.0
UE4N«
2.0
2.0
2.0
33
33
SHEET
5
10
PINTO
10
20
30
TOR 1C CO. C4
2.0
2.0
2.0
10
20
30
11
4LIER
56
36
36
67
6 7
Ell ILL
12
3 -1

13 -1
15 -I

0 -3
60
63
LLUS DEL
0 -3
32
60
TOU4CCO. C4LLUS DEL
1.0
1.0
HMU'ill
2.0
2.0
2.0
25
25
• C 4V
10
20
10
31
39
4LIER
5 -I
2 1
21
.23

.15
.36
.36
.11
.11

.20
.86

.13
.01

.72
.25
.33
U3
.72
.17
.25
ri
.11
.28

.65
.01
.71
2

2
2
2
2
2

1
1

1
1

1
1
1

1
1
1

2
2

2
2
2
SUSC
2
2
2
2
2
2
?
2
2
2
2
2
2
2
2
2
2
2
1
3
1
1
I
1
1
1
1
1
1
1
1
1
2
2
2
1
1
1
ETFECT STD CEO OEO IMJJRY INJURY THRESH INJ CONC HW.T t INJ 4T 8 MR
TYPE CEO HE4N ME4N LINE PPIIH R4TIO CORR PP IH CONC OF
RTF OR H OEV 4T T 1 MR SLCTE 1 MR 3 MR 8 MR MED/TIIRS COEF 7 9 10
169
90
90
90
9(1
90
90
90
90
90
3
3
0
200
260
200
200
0
62
C2
62
117
117
117
11
11
1 1
11
11
11
11
11
3
3
3
S
S
5
1
2
2
2
2
2
2
2
i
8 1.09 62 -.11 11 9 6 1.1 .99 2.1 5.7 7.9
2
1
2
2
2 	
2
2
5 1.09 62 -.11 11 9 6 1.1 .96 2.1 5.7 7.9
3
3 - 	
2
1
1
2
5
5
5
3 1.29 23 .91
5 .....
5
5
3 1.31 25 .90
6
6
2
7
7
7

-------
uiut   2  icuNiiHurui.   OUSERVMIONS »NO  CILCUUUO INJiJiii rtR»Hi.itRS FOR Hitm cxposrn td o2oiic.
        LXI'OS              HUHUIII lYI'f
        OUI14I CUNC INJURY Of  OfV CONC
         tin   f'PiiH     *       i
                                           SUSC II (f
9.
9.
1 3.
13.
13.
13.
13.
21.
21.
21.
21.
b.
b.
5.
b.
*•
5.
5.
5.
b.
5.
1 1.
1 I.
11.
11.
u.
11.
31.
31.
5.
b.
5.
b.
5.
21.
100
100
ID a
100
100
100
100
200
200
100
100
100
100
too
mo
100
MO
300
3DO
jon
3110
100
100
100
too
inn.
100
100
100
21)0
200
?00
200
20 n
1110
21. 100
21. 100
21 . 100
2.0 00
cium*
2.0
2.0
2.0
2.0

10
20
10
UO
Pimm, a
1 .5
ronun
1 .5
IOHUO
2.0
2.0
2.0
2.0
IUO|)N1
2.0
2. a
2.0
2.0
10
. HtO
10
. HUM
10
20
in
UO
». u
10
20
10
UO
IHGOtm. Ml
2.0
2.0
2.0
2.0
col i us
1.0
t .0
10
20
10
00
, P«
f»0
•13
IOHUO. fin
2.0
2.0
2.0
2.0
o r (• on i
2.0
2.0
2.0
2.0
10
20
MO
00
4. s:
10
20
10
00
30
UN »
10
1C
21)
in
PHI
CO
-.5?
'2
GOLD IN HINDU
-1.20
- .99
-.81
-.25

.25
2
2
2
2

1
CIIEHRY .
a «.»
* VF
0
^
17
33
NO 4
0
0
17
50
ITU-
1,
7
11
1 7
lEt
33
1 0
(II 41
1
7
9
1 9
1.23

-3.72
-1.75
-.95
-.28

-3.72
-3.72
-.95
.00
1

2
2
2
2

2
2
2
2
T40SENOSCHON
-1.75
- 1.18
-I. on
-.95
H4IHUOU
-.11
-.OS
L
-1.75
- 1.1B
-1.31
-.UO
2
2
2
2

2
2

2
2
2
2
4IHF.Tt 4
0
0
5
1
-3.72
- 3.72
- 1.65
-1.11
2
2
2
2
1
1
1
1
i
i
i
t
i
i
i
2
2
2
2
2
2
2
2
2
2
2
2
2
2
a
2
2
2
3
3
3
3
3
1
3
3
3
5
5
5
S
5
5
5
110
111)
110
iia
s
5
S
5
5
5
5
S
5
S
5
5
S
b
S
200
200
200
b
b
5
5
5
5
5
5
!i
7
*
7
7
}
)
1
7
1
1
1
,
7
i
7
*
7
/
7
I
1
7
7
7
i
1
/
J
2
,
J
1
;
i
7
7
7
7

I.1U 1 10




8. 50 171








l.a; ao




l.cs an




12.03 715







12.30 Of)




IIIILI  SID Uf;o  uro  INJURY  INJURY IIIRESlI  INJ CONC  HUL 1 » INJ  U  6 MR
 I YPC   CIO Mt»N ME»N  LINT        PPIIM        IIUIO    COHR fVIIM CONC OF
 OR N   OCV U I I  MR SI (PE   I  MR 3 HR B  MR HtU/IMHS  COtf   7     9    10
                                                                                                             .HO
                                                                                                             .96
                                                                                                              .90
                                                                                                              .91
                                                                                                              .00
                                                                                                              .37

-------
TABLE   2  (CONTINUED).  OBSERVATIONS UNO CILCULUED INJURY P»R*MrTr.RS FOR PUNTS EXPOSTO TO  OZONC.
       EXPOS              NUMBER TYPE
       UWMT  CONC INJURY OF  DCV CONG
PLANT    MR    PPHH    t       2   INST
         EFFECT  STU oro  OEO  INJURY  INJURY THRESH  INJ CONC MULT t INJ u a IIR
           TYPE   GEO Hf_*N HUN  LINT        PPHn       R*TIO   CORR HP IM C OHC Or
susc Rrr   OR  N   orv AT T i IIP SLCPE   i IIR 3 MR o IIR MFD/TIIRS cotr   7910
21.
21.
21.
71.
21.
21.
21.
21.
21.
21.
21.
21.
21.
21.
21.
2.1.
32.
32.
32.
10 0
2110
200
200
200
2110
1110
100
ino
100
100
?00
200
200
200
200
100
1110
100
PETUNUi UONIN24
2.0
2.0
2.0
2.0
10
20
10
80
0
0
10
1
PETUNUt CAN* DI M-
z.n
2.0
2.0
2.0
10
20
10
aO
SNM'OIMGONr
2.0
2.0
2.0
2.0
10
20
10
80
SNAPDRAGON.
1.0
1.0
TOM 41
SO
19
[0. Flit
a
10
9
7
F LORAL
0
0
10
11 -
ROCKCT
15
21
EB ALL
3
1
1
i
.72
.72
.28
.10
2
2
2
2
ALL OOUOLE HIX
3
1
1
1

3
3
1
.72
.28
.31
.18
CARPET
.72
.72
.28
1.23

1
-

MIXTURE
.01
.81

2
2
2
2
FORMAL
2
2
2
2

2
2

3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
3
5
5
5
5
5
5
5
S
S
5
5
5
S
5
S
5
280
280
200
1 2.12 201
7
7
7
7
1 2.13 191
7
7
7
7
1 2.83 215
7
7
7
7
1 2.01 ICQ
7
7
2
.92




.87




.73




.90




-------
TABLE   1.   IMSHWMIOHS AND LALCULATIU  1N.HJIIY  PAItAMFTERS  FOIl  PLANfS EXPOSED TO OZONE.


I'l ANf
All. PI AN IS
All I'l. AN IS
All I'l AN IS
All UtANS EXCEI'f SOYUEANS
All BEAMS EXCEPT SOYBEANS
ALL COHN
riOWEHS (BEGONIA & POINSETTIA)
IIAY {ALTAI. FA & GltASSES)
HAY (All All A 1 CHASSIS)
(MflAMiNIAI S
SOIIWIIIH. MAIU1N
All SOYBEANS
All SOYBEANS
AIL iniJACEU
ALL IllllACCO
WES UIU UlMltEK (4 VARIETIES OF PINE)
IUEES IOH l.UMUEH (3 VAIIIEIIES OF PINE)
UIIIAI
* 1 - sensitive'
2 - tnleniieillalc
3 * rusl slant
" Hit L-sliulil - IX injury


SUSC*
1
2
3
1
2
2
2
I
2
2
2
1
2
1
2
|
2
2




NUMIIEIt SID
OF CEO
OUS DEV
450
342
260
62
10
IB
17
23

25
y
26
SO
203
59
10
.06
.67
.92
.75
.61
.00
.59
.91
.59
.61
.70
.51
.71
96
.711
.61
0 2.27
15 1.47




GEO
MEAN
1 lilt
30
72
174
35
72
Ul
60
45
57
60
59
72
94
39
70
49
119
Ul




IN JUDY
LINE
SLOI'E
-.40
-.46
-.27
-.42
-.37
-.51
-.32
-.54
-.37
-.34
-.67
-.73
-.66
-.49
-.33
-.63
-.74
-.46




INJUItY THRESH
PPIIM**
1 lilt
9
22
30
9
24
16
23
10
19
22
15
27
27
0
ID
16
21
33




3 IIR
6
13
20
6
16
9
16
6
13
15
7
12
13
5
13
0
9
20




0 (III
4
0
21
4
U
6
12
3
9
11
4
6
7
3
9
4
4
13




IN,) CONC
HAT 10
MED/ TIMS
4.3
3.3
4.6
3.7
3.1
5.0
3.0
4.5
2.9
3.0
3.9
2.6
3.5
4. a
3.0
3.0
6.7
2.4




MULT
CORK
COEF
.77
.05
.59
.00
.92
.95
.09
.03
.09
.07
.97
.77
.90
.75
.08
.91
.79
.91




% IN,) AF (1 IIR
WIM CONC OF
7.0 9.0 10.0
0.4 16.5 21.1
.4 1.4 2.3
.0 .0 .0
9.8 19.9 25.6
.1 .3 .6
2.2 4.9 6.6
.0 .2 .3
13.0 23.0 20.3
.2 1.0 1.9
.1 .3 .6
10.0 19.0 25.3
2.5 0.7 13.4
1.1 3.6 5.3
15.1 25.4 30.7
.3 .9 1.5
9.0 20.0 27.0
3.0 7.0 9.0
.0 .1 .1





-------
                                ATTACHMENT  3

             UNITED STATES  DEPARTMENT OF AGRICULTURE
                   SCIENCE AND EDUCATION ADMINISTRATION
                                                       1224 Gardner Hall, Botany Dept.
FEDERAL RESEARCH                                          NORTH CAROLINA STATE UNIVERSITY
SOUTHERN REGION                                           P. O. BOX  5186
                                                       RALEIGH. NORTH CAROLINA 2765O
                                                       September 27, 1978


     Subject:  Estimate of Economic Benefits Associated with Alternative
               Secondary Ozone Standards

     To:       Mr. Don Lokey               -                             - - •
               Mr. Harvey Richmond
               U. S. Environmental Protection Agency
               MD-12
               Research Triangle Park, NT. C. 27711

     I have scanned with interest  your development of the above subj_ec_t	
     matter.  You have made use of data that was generated for this use.
     I had hoped to do something like that for the MAS document but time
     did not permit.

     I have problems with some of  your assumptions but you have well stated
     these problems and have included comments from many people with whom
     vou have communicated.  Your  approach is clearly given, your caveats
     are well stated and your discussions with exoerts are well presented.
     I personally have no problems with your presentations.

     However, based on observations in field work here at NCSU, I have some
     of the same concerns voiced by Dr. Heggestad.  I will raise some
     questions without really giving you any answers.

     1.   I question the 0.07 and 0.09 pom 0  for 8 hrs when the hourly is
         0.08 and 0.10 respectively.

     2.   Further, if the hourly is 0.08 or 0.10 ppm, what would you expect to
         find in terms of numbers  of days from >lay - September when the 3 hr
         average each day would be above say 0.06 ppm?

     3.   I would tend coward a different ratio for the best and worst case
         of yield:injurv ratio.  The worst would be 1:1 and the best 1:2.
         This would not be for leafy crops used for human consumption where
         a 10:1 ratio could hold.

     4.   I would also stress the dangers of extrapolation from short term
         acute exposures with injury as the prime response to long term
         chronic exposures where harvested yield is Che prime concern.

     I still like vour approach and believe it is a first effort that should
     be submitted.  At the least,  it will make others seriously look at
     economic imoact.

-------
Paae 2
Mr. 3 on LsSwy
Mr. Harvey  Richmond

I vouid encourage you eo Look aC "he paper  by  Laraen and .rvself.  Larsen
cook, che 32-
-------
                              Appendix A
 1          Thresholds  for Injury, Growth, and Yield Loss


 2             Caused by Ozone on Field Corn Hybrids


 3          A.  S.  Heagle,  R.  3. Philbeck and W. M. Knott


 4       Plant  Pathologist and Agricultural Engineer, Southern Region,


 5  Science  and Education  Administration, U. S. Department of Agricul-


 6  ture,  Plant Pathology  Department, North Carolina State University,


 7  Raleigh,  N.  C.  27650;  and Research Associate, Botany Department, ___


 g  North Carolina State University, -Raleigh, N. C. 27650.


 9       Cooperative  investigations  of the U. S. Department of Agricul-


IQ  ture  and  the North  Carolina State University.  Paper number 5529 of


^j_  the Journal Series  of  the North  Carolina Agricultural Experiment


12  Station,  Raleigh, North Carolina 27650.


^3      Mention of commercial products or equipment by name does not


^  constitute  a guarantee or warranty__of the product by Che U. S.


T*  Department  of  Agriculture, or North Carolina State University and


,f  does nof imply its  approval to the exclusion of other products  that


 _  may be suitable.


        The  authors  thank Hans Hamann for statistical analyses and
18

    Michael  B.  Letchworth,  John W. Johnston and Janice L. Heard for


__  technical assistance.
20

        Accepted  for publication
22
                              ABSTRACT
23

   HEAGLE, A. S., R. 3. PHILBECK, and W. M. KNOTT. 1979.  Thresholds foi


        injury, growth, and yield loss caused by ozone on field corn

-------
                                                        Heagle et al. - 2
  1       hybrids.   Phytopathology 69:



  2                                                        ."'-      r


  3       A commercial field com, .Zea  nays L. ,  hybrid 'Cokar-16'  ' —
                                   ™'-M-"11-"    * '                         y


  4  was  exposed to four chronic doses  of ozone (0.,) in open-      —



  5  top  field  chambers from 25  days  after planting until maturity.  The



  5  different  doses war a  obtained by adding different but constant con-



  7  ceatrations  of 0_ to  the naturally varying  ambient concentrations  for



  g  7 .hr/day (0930 to 1530  hr) .  The threshold  0..  concentrations causing



  g  foliar injury  (betveen  0.02  and  0.07  ppm) were lower than concentra-



 IQ  tions  required to -decrease "kernel -yield : (between. -0*11 _and 0.15 pom).



 11  These  thresholds  were the same whether planes  were grown in pots



 j2  or in  the ground.   In the greenhouse,  the sensitivity of Coker 16  to



 «2  growth  effects  caused by chronic 0, exposures  was intermediate to



 ,.  that of two open-pedigree hybrids.   In the  field,  both open-pedigree



 ._  hybrids- were more sensitive  than Cokar 16.  Exposure  to a mean 7 hr/



 -^  day 0_ concentration of 0.15 ppm decreased - kernel  yield of the open—
 15       J


    pedigree hybrids  by 37-«0", but  that of Coker  15 was  decreased by  only


    -, -,<.

18



19  -
         Chronic doses of ozone CO,) g^" injure foliage and decrease yield
20                                J

    of important crop species (5,  o, 11, 13, 14, 15).  Yiald of  sv.eet



    com,  Zea mays L. ,  'Golden ilidget', grown in field chambers  was de-



    creased by daily 7-hr exposures to 0.10 ppm of 0, CO. 10- ppm  of 0, =



    196  ^g/m  at 25 C  and 750 mm Hg)  but not by 0.05 ppm (.5).   Tieid of



    sveet  com was decreased substantially by exposure of planes to

-------
                                                        Heagle et al.  - 3
 1  ambient  oxidants  in open-top field chambers  in  California (14)  and


 2  by  exposure  in  a  greenhouse to 0.20 or 0.35  ppm of  0,  (11).   Cameron


 3  (2,  3) showed that  sweet corn had high heritability for response to


 4  foliar injury from  ambient oxidants in California.   There are no	


 5  reports  of the  effects of ambient oxidants or chronic  doses  of  0_


 5  on  field corn.


 7      Fertility  levels and growth media greatly  affect  the_sensitiv-_


 g  ity of plants to  0-,  Interactions between the  different nutrient  -


 g  elements and sensitivity seem to be complex  (1, 8),  but the  exact


10  relationships have  not been shown (10) .  Greenhouse studies  with


»»  potted pinto bean and tobacco showed that foliar  sensitivity to


12  oxidants is  greater in plants growing in artificial media such  as


.-  a peat:perlite mixture or vermiculite, than  in  plants  growing in


..  soil (9,  12).   However, foliar injury of tobacco  caused by ambient


    oxidants in  the field was four to five times less for  potted plants


    growja in a mixture  of peat:perlite:soil than for  plants grown in
16

    the  ground (4) -   No studies have compared the effects  of 0,  on  yield


    of  plants grown in  different growth, media.
18

        Previous field studies on the effects of ambient  oxidants  have
19

    been limited to determining the effects of one  dose, usually comparing
20

    plants grown in carbon-filtered (CF) air with, plants grown in non-


    filtered (N?) air.   From such studies, it is not  possible to determine


    the relative impact of different doses or to determine threshold


    doses for effects on injury, growth, and yield.


        The present  research, was conducted with, field  com to:  i)

-------
                                                        Heagla et al. - 4




 I   identify the range of sensitivity to 0, of several hybrids in a

 2   greenhouse,  ii)  determine threshold doses of 0. causing-injury _

     and  decreased growth and yield  of a cosnercial hybrid grown in .- —

     pots or  in the ground in field  chambers,  and iii)  relate the inj.u.ry

     and  growth effects of 0, in  the greenhouse to effects of 0- on

     yield in  the field.
 6
                           MATERIALS AND METHODS

          Greenhouse  study. - rive open-pedigree  and six cocnercial
 o
     field com,  Zea inays  L.,  hybrids  (Table 1) were tested for relative
 9                     -—

     sensitivity  to 0,.   Seeds were  planted  on 2-February 1976 in 4-licer
10                  J
    pocs, containing a 1:1:1  ratio  (by  volune) of sand:sandy-loan soil:

    ?ro-Mi:c 32.  Pro—Mis  EX  contains  seat and perlite  with nutrients
12                                    "
     (Premier Brands,  Inc., ^lev Tork.,  N.  ?.).   Plants were thinned to  1
13
    plant/pot and fertilized  7 days after planting  wich  2 g of fertilizer
U
    0-4-4-6,  N-P--Q .   Sight plants  per hybrid vere  exposed to Q,  or  carbon—
15                          "                                   J
    filtered  ^-^ in two field chambers  05)  installed in  a greenhouse.
16
    Plants were eznosed ta Q^ for 7 hr  G09QO  to 1500 hrs)  for 21  davs,
17
    starting  14 days after planting.  Ozone was generated by  ulcraviaiet
18
    lighr. Concentrations of Ov in. chaabers vere ncni-tored continuously
IS                             °
    during exposure with, a chesiluainescence 0, analyzer  (Model 3410A, Mon—
20
    itor  Labs Inc., San Diego, CA 92121) calibrated to a  1" neutral buffer-
21
    ad  KZ standard.  The sean hourly 0, concentrations during  the 21-day
22
    esposure.  period ranged froa Q.G6 to 0.13 ?pa.  The aean 7-hr 0., coccen—
23                                           "                    J
    tracion was 0.12  ppn (daily range: 0.08  to 0.17 ppn).  Tesperature
2*
    and relative humidity CP>H) i^- the greenhouse and exposure chambers
23

-------
                                                       Reagle et al. - 5
 *  ranged from 20 to 25 C and 35 to 70% KH respectively.  No supple-




 *  mental lighting was used.  One day after exposures ended', we esti-




 3  mated visible foliar injury on individual leaves in 5% increments"




 *  (0-100%).  Fresh weight of the stem and leaves (shoots) were   ~ ""




 5  measured.  Dry weights of shoots were measured after drying for




 6  2 days at 60 C.




 7       Field studies - threshold doses of ozone and effeac__of._plantr




 8  growth media. - Seeds of 'Coker 16'  were sown with a four-row planter




 9  on 6 May, 1976, -in rows spaced 95 cm in a 1.2 ha field of sandy-clay




10  and sandy-loam soil (Cecil and Appling, Typic hapludults).   Fertilizer




11  (14-0-14; N-P-K) was banded along each row at 500 kg/ha at planting.




12  Ammonium nitrate was applied in a strip along each row at 336 Jcg/ha,




13  34 days after planting.




14       Seeds were also planted on 6 May in 15-liter plastic pots con—




13  taining a 1:1:1 ratio (by volume) of sandy-loam soil (Appling,  Typic




16  hapludults) :sand:Pro-M±s 5X.   Plants were thinned to 1 plant/pot 21




17  days after planting.  Each plant was fertilized with 6 g of fertilizer




18  (14-4-6;  N-P-K), 24 days after planting and 5 g of ammonium nitrate,




19  34 days after planting.




20       Each plot (of a total of 25 in  5 blocks) initially consisted of




21  tvo 2.75  m rows of corn.  Plants in  alternate halves of each row were




22  removed to make room for plants in four 15-liter pots.   Pots were




23  partially buried leaving the top 5 to 10 cm uncovered.   The plants




24  growing in the ground were thinned to about one per each. 15 cm of




35  row,  leaving seven to eight plants in each, of the two alternate 1.33 m

-------
                                                         Heagle at al. - 6
  1 rows/plot.   Planes were watered to prevent wilt ing.  Com plants




  2 growing adjacent to plots were not disturbed.   Weeds wera controlled




  3 by hand.   Insects wera controlled vita carbaryl (1-napthy1 nethyl-




  4 carbanate)  or aalathion [S-(l,  2-bis[ethoxycarbony]ethyl) 0,0-di-—




  5 methyl  phosphorodithioate]  as  needed.




  6      Five  treatments (1 treatment/plot)  wera randomized within aach




  7 of the  five blocks.   One treatment was ambient air (AA) with no_chanbe:




  3 A  cylindrical (3  m-diaraeter) open-top  field chamber (4, 7)  was placed




  9  over  each of  the  four remaining plots  in each  block,  22 days after




10  planting.   Plants in one chamber/block,  continuously received charcoai-




jj_  filtered (CF)  air.   Plants  in  three chambers/block were exposed con-




^2  tinuously to  nonfilterad OIF) air (particuiata filtar only)  throughout




13  the sncner.   However,  starting  25  days afcar planting,  snail constant




j^  concentrations of  0^ wera added for 7  hr/day (0930  to 1530  hrs).   "The




I*  added 0^ resulted  in  thrae  different 0-  cur*/es  that followed the  daily




tg  fluctuations  of anbianc  oxidant  concentrations (Fig.  1).  One dose




,j  (NF-1) was near anbienc  concentracions and was  obtained by  adding




,« O.Q2 pen of 0, to  chaaber concentrations, thus  z^king up  for the  0^




«a lost in tie chanber air-handling systen.  Two  higher  doses wera ob.—




2Q tained by adding 0.06 ppm C^F-2) or 0.10 ppm CNF-3) of  0-.   Ozone was




-, added to the NF-1, NF-2, and UF-3 chambers for  7 hr/day for  33 days




-2 C31 >iay tnrough, 27 August).




        Ozone  was oroducad and dispensed as described previously  (.7) .




_, Ozone concentrations were monitored frcn the center of  the chamber




   at  midplant canopy haighr, as described previously C7) .

-------
                                                     Heagle et al.  - 7
 1       Plant height and leaf  emergence were  measured,  and estimates


 2  of  visible foliar chlorosis and necrosis  (injury) on individual -


 3  leaves  were made once each  week for 10  consecutive weeks,  starting"


 4  8 days  after exposures began:  Eights plants  in the  ground (four-	


 5  in  each row) and the  eight  plants  in pots  in  each plot  were labeled


 g  to  show plant position.before harvest.  Plants  in the ground adja-


 7  cent  to the chamber wall or pots were not  used  in measuring effects.


 g  Plants  were harvested 115 days-after-planting,  when  leaves in all


 o  treatments were  brown and a black  layer had formed in the  kernels.


»Q  Plant height and fresh weight of ears,  with husks and without husks,


«<  were  measured.   Ears  were dried to 12.5% moisture content  and


«-  weighed.   The total kernel  weight  and the  weight of  100 kernels/


.»  plant were measured.   Stovers were dried in the field for  42 days


,,  (10-25%-/moisture content) and weighed.

         Response of three hybrids. -  Plants of 'Coker 16'  sown on


    6 May were removed, and seeds of two open-pedigree hybrids,  FR. 532 x
16

    FR  619  (OP-1)  resistant, and H 95 x FR  64A (OP-2) sensitive,  and

    Coker 16  intermediate sensitivity, were planted on 24 May.   Seeds
18

    were  spaced 15 cm apart in  seven 45 cm  subrows  in tvo 2.75 a. rows
19

    in  each of three clots in three blocks.  The.  hybrid  positions were'
20

    randomized within each subrov.  Four seeds were planted at each
21
    position  but plants were thinned to one after 12 days.   Plants were


    fe^-ti'1i2ad with  336 kg/ha of ammonium nitrate and 336 kg/ha of 10-
23
    10-10;  N-P-K,  13 and  25 days, respectively, after planting.   Coker


    16  corn growing  in adjacent rows was maintained.

-------
                                                      Heagle st al. - 8
         Open-top  field  chambers were  inscalled  on 2 plots/block 25




   days  after planting.  Plants in one chamber  received carbon-fil-=_




   tered (C?) air for 24 hrs per day.  Those  in the other chamber ;




   received nonfiltered air for 24 'or/day with  0.10 ppm 0- added




 ^ (NF-4) for 7 hr/day for 32 days, starting  on 22  June and continuing




 * through 12 Sepcamber (29 to 111 days after planting).




 7                              RESULTS                      •		




 '       Greenhouse study.  - Foliar sympotoms  of 0,  exposure ranged - -




 5 froa  interveinal chlorosis and-surf ace necrosis-co-white-bifacial




10 necrosis on all 11 hybrids.




H      Among Che open-pedigree hybrids, H 95 x ?R  54A  (OP-2) vas  acre




12 sensitive and  (TR 37 :c H 34) :c ~a 25 more  resistant  to  0_ injury




13 than others (Table 1).   Overall, the connercial  hybrids vara  injured




1* less than were the csaen-oedigree hybrids. _ De«La.lb_XL 73  was conpar—




13 atively sensitive while Pioneer 3363A was relatively resistant.




16      Tie correlation coefficient between shoot fresh and shoot  dry




17 weights was 0.97.   Therefore,  Table 1 shows only shoot  fresh  weights.




13 Of  the open-pedigree hybrids,  shoot weight  of FR 532 ;c  ?r 519 (OP-i)




19 was 2.7, less because of  0_  and  shoot weight  (OP-2) was 53% less  than




20 the concrol C^aole 1).   The  range  of 0,  effects on shoot weight was




21 less among  the  commercial  hybrids  than  that for tha  open-pedigree




22 hybrids.   Scooc weight  of  Pioneer  3363A  was decreased lass (.27^) and




23 chat of Funk G  4545 more  (Ai")  than chat  of mosc other commercial




2A hybrids casted  (Table 1).




23      Field  studies  -  ozone concentrations.  -  Daily fluctuations in

-------
                                                    Keagle  et  al.  -9
 1 the. ambient 0^ concentrations are shown by the daily  7-hr  (0930
 2 to 1630 hr) and 24-hr means in Figure 1.  The mean diurnal 0,  fluctu-
 3 ations for various treatments are shown in Figure 2.  Except for
 4 several rainy days, the 7-hr mean 0. concentration greatly exceede'd
 5 the 24-hr mean 0, concentration, as would be expected by the diurnal
 6 pattern of 0^ concentrations, shown in Figure 2.  The overall mean
 7 1- and 24-hr 0. concentrations in ambient air (AA) and .those -for.. the
 8 various -chamber treatments- are shown -in Table 2, --The. daily. 7-hr __
 9 mean concentrations for the NF-1, NT-2, NF-3 or NF-4 treatments can
10 be easily determined by adding 0.01, 0.05, 0.09 or 0.09 pom,  respec-
11 tively, to the daily 7-hr AA means (Fig. 1).   The daily 24-hr mean
12 OT concentrations for the various NF treatments can also be calculated
13 using a common 0_ dose (87% of AA) for all NF creacments during the
1^ 17 hr when 0., was not added.   For example, the calculation to deter-
U mine a given 24-hr aean for NF-1 is:

16          24 hr mean for NF-1 =  7 (7-hr *F-1)  + 17 CNF 17)
                                                ^4
17 NF 17 is the common 17 hour daily mean for all NF  treatmencs:
18               24 hr AA - 7 hr AA (7/24)
        NF 17 =  -     -  x .3/
19
2Q      threshold doses of ozone and effects of plant-growth media. -
j-t Symptoms of foliar injury in  the  field  resembled those from green-
22 house exposures to 0,.   The initial  symptom was a faint interveinal
23 chlorosis which gradually increased  with continuing  exposure,  often
^culminating in complete chlorosis.
«.      The percentage injury o£ plants in pots and ground was similar,

-------
                                                       Eeagle  at  al.  - 10
    and were combined for each. 0, treatment  (Fig. 3).  The decreased in-




  * jury between weeks 2 and 4 was probably due to rapid growth, as jell




  ^ as to relatively low 0_ concentrations.  The difference in foliar




  * injury between-plants in the CF treatment (0.02 pom) and plants in




  * each of the other chamber treatments is an indication of the amount




  * of injury caused by 0.. rather than by normal senescence.  The thresh-




  7 old 0. concentration for significant foliar injury of Coker i5—was -




  8 between" 0".07 (NF-1)  and 0.11 ppm (NF-2)  (Fig.  3).  Chlorosis and




  9 necrosis of-foliage was greater in chambers at 0.07- CN"F-i)  or 0.02




10 (CF)  ppn 0., than that in the AA (0.06 ppm)  treatment from weeks 8




11 to  10 (Fig.  3).   .




12      There  were  no  significant 0.,  treatment :c media interactions for




13 any of the  growth or yield  measures taken.   Plants in chambers were




14 slightly  taller  than these  in the  AA treatment- (Liable 3) .   Plants sear




15  the center  of  the chambers  were  slightly taller  with slightly greater




16  kernel weight  than  those nearer  the chamber  wails,  but  these  differences




17  were  not  statistically  significant.   There ware  ao  significant 0,




13  treatment x chamber  position  interactions affecting growth.   The




15  threshold 0., dose for decreased height and weight of  stovers  was




20 higher for potted plants  than for planes  grown in the ground  (Table 3)




21 but the interaction was not significant  statistically.




22      Yields tended to decrease at a higher 0- level for potted  plants




23 than for slants  in the ground  (Table  3) but  there was no significant




Tjk 0, concentration :c media interaction.  Kernel weight oer olant  at 0.15
*>•»  j                                                w



25 pro of 0- was 30  g less than  that at  3.02 ppm for potted plants  and

-------
                                                       Heagle et al. - 11
 1 38  g  less  for  plants  in the  ground.   At  0.15  ppm,  kernel size (100



 2 wt) was  decreased  by  7  to  9% compared to a 13 to  16% decrease for



 3 kernel weight/plant,  showing that  0_  also caused  a decrease in num-~



 4 bers  of  kernels.



 5      A block x 0-  treatment  interaction  for yield of potted plants



 6 was partially  caused  by block-to-block fluctuations at  0.07 ppm of



 7 0, where the yield ranged  from 7%  greater to  13%  less than—tha-fe--ae- —



 8 0.02  ppm.-  Block-to-block-fluctuations were smaller-at-Q.11. ppm.



 9 However, for all blocks, the weight of kernels/plant_at 0.15 ppm were



10 less  (9  to  19%)" than  those at 0.02 ppm.   There-were-no- differences in--



11 0-, concentrations  that  accounted for  these fluctuations.



^2      Block x 0- treatment  effects  also occurred for growth, -and yield



13 of plants  in the ground, primarily due to variation at  0.02 ppm where



JA plants were-unusually small-in-block  3 and usually large in block 2.



•it In all blocks,  growth, and  yield of plants at  0.15  ppm was less than



»g that  at  0.02 ppm.



,7      response  of three  hybrids. -  Injury symptoms were  similar to



,o those in the threshold-dose  study  except for  bifacial necrosis which
.Lu


jo occurred on some leaves of both open-pedigree hybrids after several



-g weeks of exposure  in  the NF-4 treatment.



        Injury of  all hybrids was significantly  greater at 0.15 (NF-4)



-•than  that  at 0.02  (CF)  ppm 0., on all  dates, except injury was similar



7-in both  treatments for  Coker 16 after week 1  (Fig.  4).   The two open-



_.pedigree hybrids were -ore severely injured than  Coker  16  after weeks



   i, 2, 3  and 9.  But during intermediate  weeks, foliar injury of all

-------
                                                       Heagle et_ al.  - 12
 1 hybrids -as srnilar; about 15%  greacar  ac 0.15  ppm Chan at  Q.Q2  ppm




 2 o£ Q7.  Percentage injury of  the open-pedigree  hybrids  were siailar




 3 (<5% different), except after veek  3 vhea OP~1  vas sore severely*.ia-




 4 jured than OP-2.




 5      Plants of all hybrids were shorter and  the stovers weighed  less




 6 at 0.15 ppm than at Q.Q2 pan.  in all blocks (Table  4). .  A block 2 Q~




 7 treat-lent interaction for plant height  and weight  of  scovar-s vs-& - -




 8 caused primarily by greater effects of  0,-on all hybrids in-block




 9 1 than in other blocks. .. ..




10      The weight of kernels/plant at 0.15 ppm~vas 12;-37,-and 40" less




11 than -hat ac 0.02 ppm for Coker 15, OP-1,  and Q?-2, respectively;  the




12 weighz of 100 kernels -^as decreased by  15, 25,  and 30%  for  Cokar 16,




U OP-1,  and OP-2, respectively  CTabia 4).  These  values indicated  chat




H yield  decreases of Coker 15  vere caused-by decreased kerr.el  sizes




1* rather than by nuabers.  However,  vich.  the open-pedigree hybrids,




it yield  decreases vere apparently caused by decreased kernel  numbers  as





17




18




19




20




21




22




23




24




23

-------
                                                   Heagle et al. - 13
 1                              DISCUSSION




 2       Ozone concentrations in ambient air at our field site near 7




 3  Raleigh, N. C. depended mainly on regional weather patterns and ,.




 4  were representative of most of the southeastern United States.  The




 5  daily concentration curve was predictable, based on previous hourly




 6  concentrations during a given day, assuming no abrupt change in in-




 7  tensity of sunlight.   Hourly fluctuations in 0. concentrations_were_




 8  usually-less than-0.02 ppm.  The daily, —7r-hr, ambient 0__nieans, shown	




 9  in Figure 1, were generally within .04 ppm of the daily minimum and




10  maximum ---concentrations-during--daylight-hours,--—.	.v..




11       Threshold doses  of 0, for injury expression and effects on




12  growth were much lower than threshold doses for decreased kernel yield,




U  demonstrating that field corn can withstand some injury with no loss




l^  of yield.  The correlation between.injury,—growth, and yield effects




1«  across treatments-was often low.  The magnitude of the differences




lg  between treatments in the amounts of foliar injury and affects on




*7  stover weight were a  poor indication of  the magnitude of the effects




jo  on kernel weight.  For example,  at 0.11  ppm of 0-, the percentage of




je  foliar injury averaged about 17,  greater  than that at 0.02 ppm, stover




-Q  weight was decreased  by 23%, and yield was decreased by only 27..  At




?1  0.15 ppm, foliar injury was 10%  greater  than at 0.02 ppm of 0-, stover




_-  weight was decreased  by 45%, and yield was decreased by 15%.




         Differences in plant injury, growth, and yield in ambient air




    at 0.06 ppm of 0., C24-hr mean =  0.04)  and in chambers at 0.07 ppm




    (24-hr mean - 0.04)  (Table 3) provided an estimate of the chamber

-------
                                                        Heagle et al. - li
 *  affects,  assuming the snail  dose  difference between. 0930 to 1530 hr


 2 was not a factor.  The canses for  these differences are not known Jut


 3 are probably  related  to  =™a11_  differences in climate (i, 7).  While


 * the chambers  can. affect, plant  growth,  there are no reports where


 5 changes in light,  wind  speed,  or  tesrperature,  of the magnitude caused


 6 by the chambers,  have been shown  to  affect sensitivity to 0.,.   We found


 7 no significant Q^  treatment  x  chamber  position interactions—af-fecsiag-


 8 injury7" growth, 'or yield; - More-research-is--needed-to-det-erziine inter-


 9 actions between  various  environmental.factors  and plant response to


10 chronic doses of 0-,.


H      Threshold doses  for  injury,  growth,  and yield of the open-pedi-


12 gree hybrids was noc  determined,  but our  results indicated that all


13 thresholds would be lass  for the  two open-pedigree hybrids tested


Ifc than, for Goker 16.  The effects of 0, on  injury rather  than growth


15 under greenhouse conditions,  were a better  indicator of the reaction
              •

15 under field conditions.  It is not known  *«hy growth of  OP-1 was severely


j^7 affected in the field but not in  the greenhouse.


13


19


20


21


22


23


24


23

-------
                                                       Heagle et al. - 15
 1                           LITERATURE CITED



 2 1.  BREWER, R. F., F. 3. GUILLEMET, and R. K. CREVELING.  1961.  4



 3      Influence of N-P-K fertilization on incidence and severity  -



 4      of oxidant injury to mangels and spinach.  Soil Sci. 92:298-301.



 5 2.  CAMERON, J. W.  1975.  Inheritance in sweet corn for resistance



 6      to acute ozone injury.  J. An. Soc. Hort. Sci. 100:577-579.



 7 3.  CAMERON, J. W. and 0. C. TAYLOR.  1973.  Injury to sweet-corn	



 5      inbreds and hybrids-by--air-pollutants in the field and by ozone



 g      treatments in the greenhouse	J.-Environ.-Oual. 2:387-389.  - --



10 4.  HEAGLE, A. S., D. E. BODY, and W. W. KECK.  1973.  An-open-top



H      field chamber to assess the impacc of- air pollution on plants.



12      J- Environ. Qual. 2:365-368.



jj 5.  HEAGLE, A. S., D. E. BODY, and G. E. NESLY.  1974.  Injury and



i^      yield response of soybean to chronic doses of ozone and sulfur



j«      dioxide in the field.   Phytopathology 64:132-136.



16 6.  HEAGLE, A. S., D. E. BODY, and S. K. POUNDS.   1972.  Effect of



. -      ozone on yield of sweet corn.  Phytopathology 62:683-687.



,a 7.  HEAGLS, A. S., R. 3. PHTLBECK, H. E. ROGERS,  and H. 3. LETCEWORTH.
It)


1Q      1979.  Dispensing and monitoring ozone in open—top field chambers



_o      for plant effects studies.  Phytopathology 69:



   3.  HECK, W. ft".  1968.  Factors influencing expression of oxidant  .



_.,      damage to plants.  Ann.  Rev. Phytopath. 6:165-188.



   9.  HECK, tf. W., and J.  A.  DUNNI2TG.  1967.  The effects of ozone on



,,, .     tobacco and pinto bean as conditioned by several ecological



        factors.   J.  Air Poll. Contr. Assoc.  17:112-114.

-------
                                                       Keagla at al. - 16
 1 10.  HECK, w. W. ,  J. 3. MUDD,  and ?.  R.  MILLER.   1977.   Plane and




 Z       micro-organisms.  In:   "Ozone and  Other  Photochemical Oxidants."




 3       Chap. 11, Vol. 2, Nat.  Acad. Sci. ,  Washington,  D.  C.   (Ingress).




 ^ 11.  OSHIMA, R. J.  1273.  Effect of  ozone  on  a  commercial  sweet com




 $       variety.  Plant Disease Reporter 57:719-723.




 6 12.  SEIDMAN, G.,  I. J. EINDAWI, and  W. W.  HZCK.   1965.   Enviranaental




 7       conditions affecting the use of plants as  indicators-- o-f-a-ir- —




 8       pollution.   J. Air Poll. "Contr. Assoc.   15 T 153-170-.-




 9 13.  THOMPSON, C,  R. , Z. EENSEL,. and  G. XAIS.  -19.69.  .Effects, of




10       photochemical air pollutants -on Zinfandel  grapes.   Hortic. 3ci.




U       4:222-224.




1214.  THOMPSON, C.  R. , G. SATS, and J. W.  CAiMZRON.   1376.  Effects of




13       ambient photochemical air pollutants  on  growth, jlald and  aar




14       characters of tvo street cam hybrids.  J.  Environ.  Oual. 5:




13       410-412.




Ifi 15.  THOMSON, C. R. , and 0.  C. TAYLOR.    1969.  Effects of  air pollu-
J.7       cants on growth, leaf drop,  ruit drop, and yield of citrus  trees.



12       Envircn. 5ci. Technoi.   3:934-940.




19



20



21




22




23



24




23

-------
                                                      Heagle  at  al.  -  17
 1 Figure I.  Daily 24 and 7 hr (0930 co 1630 hr) mean ozone  concentrations

 2            in ambient air 4.8 km south of Raleigh, North Carolina.

 2            Ozone was added for 7 hr/day to ambient air  (AA)  chambers

 ^            from 31 May through 27 August (A-C) in the threshold-dose

 e            study and from 22 June through 12 September  (B-D) in  the

 g            three-hybrid study.

 j Figure 2.  Mean ozone concentrations at different -times • of "the~day In

 g            ambient air (AA) , carbon- fil-tered-airr -chambers- -(CF) ,  or non-

 *            filterad-air chambers with different. .concentrations of. .ozone ._.

1Q        ..   added (NF-1) , (NF-2) , (NF-3), (NT-4) for 7 hr/day.  Each

..            point is the mean from 31 May through 27 August,  1976, excepc

-_            for NF-4 which is the mean from 22 June through 12  September,
13

   Figure_3.  Foliar injury, at. 10 weekly intervals on  'Coker 16'  corn  grown
14
              in ambient air (AA) , carbon-f iltered-air chambers  CCF) ,  or

              nonfiltered-air CNF) chambers with different  concentrations
16
              of ozone added for 7 hr/day O^T-i, NF-2, NF-3).   Each  aoint  is
17
              the mean injury per leaf on 24 plants  C3 plants  in  2 growth
18
              media in each of 4 blocks).  Confidence intervals shown  are
19
              the LSD C? = 0.05) values for treatment .x growth media.
20
   Figure 4.  Percentage injury per leaf on three field corn hybrids grown

              in carbon-filterad-air CCF) or in nonfiltered-air chambers
22
              with 0.10 ppm ozone added for 7 hr/day  CNF-4) over  a nine-week
23
              period.  Each ooint is the mean -of- 12 plants  C4  plants in each
24
              of three blocks) .   Confidence intervals shown are the  LSD
23

-------
                                                        Heagle  a:  al.  -  13
 1             CL * 0-05) values for  craacaerit x hybrid.




 2




 3



 4




 5




 6



 7




 8




 9   .



10




11




12




13



14




15



16




17



ia




19



20



21




22




23



24




25

-------
                                                      Heagle et al. - 19
 Table  1.   Injury  and  growth  response  of  11  field  corn  hybrids  co  chronic

           doses of  ozone  in  a greenhouse.—
Hybrid
Open Pedigree
(FR 37 x H 84) x Va 26
FR 632 x H 94
FR 632 x FR 619 (OP-1)
B 73 x MO 17
H 95 x FR- 64A (OP-2)
Commercial
Pioneer 3368A
DeXalb XL 43
Coker 16
Funk G 4646
McNair x 170
DeKalb XL78
LSD 0.05 =
Foliar Injury—
(Leaves nos. 5,6,7,8)
(%)

24 ij
33 kl
34 kl
37 1
45 m
IS h
• 23 hi
1 23 hi ..
23 hi
25 ij
29 jk
5.3
Shoot Fresh Weight-
Control
(s)

98.8
74.3
55.8
61.4
71.7
73.2
75.3
86.3
73.0
83.7
72.7
Exposed ,
(% Loss)-7

37 kl
30 j
2 h
28 ij
63 n
27 i
29 ij
35 k
41 m
39 Ln -
38 1
2.8
— Plants were exposed to carbon-filtered .air  (control) or  to carbon-filtered
  air plus ozone (mean concentration of 0.12 ppm for 7 hr/day for  21  days,
  starting 14 days after planting.

— These leaves were chosen because no chlorosis or necrosis was present  on
  homologous leaves of control plants.  Each value is the mean of  32  leaves
  (4 leaves on each of 8 plants per cultivar) .  Means followed by  different
  letters are significantly different (LSD ?_ = 0.05).

—'Each value is the mean of 8 plants/cultivar..  .Means followed by  different
  letters are significantly different (LSD P_ =• 0.05).  '
^Percent loss is defined as 100 -  (    °       ')10°-
                                             v

-------
                                                        Heagle  et_ al.  -  20


 Table 2.   Mean ozone concentrations for 7 hr/day  (0930-1630 hr)  and  24

           hr/day in field studies to determine threshold doses  of ozone

           for significant affects on fiald corn hybrids.
Threshold-Dose Three-Hybrid
Study*' StudyH/.


Treatment
Anbiaat Air (AA)




Carbon-Filtered Air (C7)
Nonfiltered Air -r Q_
Nonfilcered Air ~ 0.,
Nonfilterad Air •*• 0,
j
3
a/,, ....
— iarasnoj.c coses o;
15 ' zrown ia oots o
per treatment cover
25 C and 760 nm of
(NF-i)^
(NI-2)-7
ozone for ef
7 hr/
day

0.06
0.02
0.07
0.11
0.15
facts on
r in the ground vera
the period
Eg, 0.10 ppa
from 31
of 0, =
24 hr/ 7 hr/
day day
ppn
0.04 Qj36 	
0.01 0.02
0.0" . —
0.05 —
0.06 —
0 . 15
. inj ury , grovth and yiald
determined. Mean concent
May through 27 August, 197
196 ug/m",
24 hr/
day

.. .0-04
0.01
—
0.06
of 'Coke:
rations
6. Ac
— The effects of ozone on injury,  growth  and  yield vera datamined for -vo
  open-oedigrae hybrids and for  'CoJeer  15'.   Mean concentrations per traat-
  aenc for 22 June  through 12 Septasber.

                                 :errcr3-cions -in  chanbers -for 7 hr per day
  (0930 to 1630 hr) .  Concentrations in NF chambers when Q, vas not added
  * AA cines 0.37.                                         J

-------
                                                       Heagle et  al.  - 21
 Table 3.   Growth and  yield of  'Coker  16'  field  corn  grown  in either  pots  or
           ground in ambient air with  no chamber (AA) ,  or in  open-top field
           chambers  and exposed continuously  to  charcoal-filtered  air (CF)
           or nonfiltered air with  three levels  of  0, added for  7  hr/day
           (NF-1, NF-2,  NF-3)£/
 Treatment
7 hr daily
mean 0.,
cone £_'
   ppm
    Growth Media Jt
                 b/
                                               Pots
                 Ground
AA
CF
NF-1
NF-2
NF-3
AA
CF
NF-1
NF-2
NF-3
AA
CF
NF-1
NF-2
NF-3
0.06
0.02
0.07
0.11
0.15
                             LSD 0.05
0.06
0.02
0.07
0.11
0.15
                             LSD 0.05
0.06
0.02
0.07
0.11
0.15
                             LSD 0.05
                                                    Plant Height -  cm
287
318
315
315
305
j
h
h
h
i
312
343
333
	 338--
323
k
h
i
- i
j
                           6.8
                   4.8
                                                                       c/
                                                  Weight  of  stover -  g—'
203
244
237
193
142
i
h
h
i
j
194
257
217
196
133
j
h
i
j
k
                          21.2
                  18.9
                                               Weight of kernels  g/plant—'
                                                                         d/
234.9 h
240.1 h
243.3 h
239.1 h
209.8  i
 11.0
221.3   j
239.1 hi
245.9 h
229.7  ij
201.5    k
                                           15.5
                                                                      d/
                                                Weight -2/100 kernels—'
AA
CF
NF-1
NF-2
NF-3

0.06
0.02
0.07
0.11
0.15
LSD 0.05
32.3 h
32.3 h
32.5 h
32.7 h
29.9 i
1.2
32.2 h
31.2 h
31.8 h
31.0 h
23.3 i
1.2
— Each value is the mean of 40 plants  (8 plants in each of 5 blocks).  Ozone was
  added  to  the inlet duct of nonfiltered air  (NF) chambers for  7 hr/day  to
  produce the 7 hr mean concentrations as shown.

—  Data  for each growth media were analyzed separately. Means for  a  given
   response measure and growth media followed by different letters are
   significantly different according to the LSD (?_ = 0.05) values  (.treatment) .

-------
                                                        Eeagle  e_t  al.  -22


— The aoisture content of stovers ranged from 10-25%.

— Tne values for kernel weights were adjusted to reflect a aoisture content
  of 15.5%

-------
                                                       Keagle et  al.  - 23
Table  4.  Growth and yield of three field corn hybrids grown in ambient  air
          with no chambers (AA), in charcoal-filtered-air open-top chambers
          (CF) or in nonfiltered-air open-top chambers with 0., added for 7
          hr/day (NF-4)£/                                    -1
Treatment

7 hr daily
mean 0., cone.



ppm
Coker
16
Effect per
OP-1
hybrid2-''

Plant Height
AA
CF
NF-4
0.
0.
0.
06
02
15
285
292
283
hi
h
i
256
259
240
j
j
k
OP- 2
- cm
227
233
212
.

1
kl
m
AA
CF
NF-4
AA
CF
NF-4
                        LSD 0.05 =
                             7.11
                                              Weight of stover - 'g—
0.06
0.02
0.15
295
301
136
h
h
i
90
90
56
j
-j
k
80
100
53
jk
j
k
                        LSD 0.05 =
                             27.7
                                                                       d/
                                           Weight of kernels - g/plant—'
0.05
0.02
0.15
213.5 h
214.5 h
188.9  i
126.3
130.5
 81.9
jk
jk
                        LSD 0.05 =
                             15.2
119.6  k
136.1 j
 82.1   1

    d/
                                              Weight - g/100 kernels—'
AA
CF
NF-4

0.06
0.02
0.15
LSD 0.05 =
33.5 h
34.7 h
29.6 i
1.75
30.5 i
30.4 i
22.7 j

25 . 7 k
27.7 j
19.4 1

—0.08 ppm ozone was added to ambient concentration in nonfilterad-air .chambers
  for 7 hr/day  (0930-1430 hr).  0, concentrations shown are means  for  (0930-
  1630 hr).

—Each value is the mean of 24 plants (8 plants in each of 3 blocks).  Means
  followed by different letters within a response measure are significantly
  different according to the LSD C?_ =-'0.0'5) values (treatment x hybrid).

— The moisture  content of stovers ranged from 10-252.

—The values shown have been corrected to reflect a moisture content of  15.5%.

-------
inure  i
               I     I      i     i     I      !
                7 HOUR MEi.M ( OD3O HOURS-I63O
               2-4 HOL'R MEAN
                              .'  U f,\\    ;.'
                             ^l.-fUi
                                r •! i 4
_ 1 1 1 	 	 -.{ — _
A3 CD
1 1 1 1 I I ! 1 1 1 1 !
                                                              9/13

     o.oo
         O5OO

-------
igurc. 3
        Mcrjr
    70
  ^ GO


  I

  U.


  5 50



  (T
   30
   20 -
   -0
                                                       ,0
        Figure
  SO
  SO —
£T 50
3
-3
Z


c ^o
_J
o
  30
  20
  10 -
              .
              Cf  t
                ' /,--
p	3
                                 - I
                                  c

                                W c t K

-------
                              Appendix  B
 1       Injury and Yield Responses of Spinach Cultivars to Chronic


 2               Doses of Ozone in Open-Top Field Chambers—


 3        A. S. Heagle, R. B. Philbeck, and M. B. Letchworth^-''  —


 $       Spinach (Spinacia oleracea L.) cultivars were exposed con-


 5  Cinuously during growth to carbon-filtered air or non-filtered


 g  ambient air in open-top field chambers.  Constant low concentrations


 j  of ozone (0_) were added to the varying ambient concentrations in


 a  the non-filtered-air chambers for 7 hr (0920 to 1620 hr EOT) per


 g  day.  There were significant differences in the amount~of~foliar"


,Q  injury and shoot growth decrease among 11 spinach cuV:ivars  exposed


.-  for 7 hr/day to 0.13 ppm of 0_; America, Winter Bloomsdale,  and


    Sevea-R were less sensitive to foliar injury than Chesapeake,


    E7brid-612, and Dixie Market.  Shoot growth of America and Viroflay


    w=s affected less and Hyfarid-612 and Dark Green Bloomsdale sore
14  	


^5  —   Cooperative investigations of the U. S. Department of Agriculture


^g  a=d the North Carolina State University.  Paper number 5516 of the


»7  journal series of the North Carolina Agricultural Experiment Station,


,g  Raleigh, North Carolina 27650.

    2/
-o  —   Plant Pathologist and Agricultural Engineer, Science and Education


2O  Administration, U. S. Department of Agriculture, Plant Pathology


21  Department, North Carolina State University, Raleigh, N. C.  27650;


    Research Assistant, Plant Pathology Department, North Carolina State


„.  University, Raleigh, N. C. 27650.


    —'   The authors thank Hans Hamann for statistical analyses and Suzanne
24

    Spencer, Madeleine Engel and John W. Johnston for their technical support.

-------
  1  than that of most other cultivars.  The cultivars Anerica, Winter




  2  Bloomsdale, Hybrid 7,  and Viroflay were exposed for 38 days co




  3  determine threshold doses of 0  for injury and yield effects.   The




  ^  threshold 7-hr/day mean 0, concentration for foliar injury was




  5  between 0.02 and 0.06  ppta..  The.threshold for significantly decreased




  g  shoot growth of most spinach cultivars was between 0.06 and 0.10 ppta.




  7  Shoot fresh weights of plants grown in the ground at 0.06, 0.10,




  a  and  0.13 ppm were 18,  37 and 69%  less, respectively, chan plants




  o  grown at 0.02 ppta.  Comparative values for potted plants grown in




 ._  a  1:1:1 oixture of sand:soil:Pro-Mix 3X were 4, 25, and 55%




     respactively.
11
12  Additional index words:   Oxidants,  plant growth




13
13




16




17




IS




19




20




21




22




23



24




25

-------
 1       Ozone  (0 ) is part of the photochemical oxidaut air pollution
 2  that occurs over widespread areas of the United States (14, 18).
 3  Reports of  foliar injury to plants from exposure to ambient doses
 4  of 0_ are common (11, 19), but there are relatively few reports of
 5  the effects of 0, on. yield under field conditions (5, 6, 7, 12,
 6  16, 17, 20, 21).
 •j       Commercial plantings of spinach (Spinacia oleracea L.) have
 a  been severely injured by photochemical oxidant pollution (3, 4, 15).
 o  Foliar symptoms from controlled exposure to 0^ are identical ~to~
,Q  symptoms in the field (4, 15).  There are no reports of the effects
. ,  of 0  on spinach yields, but several papers have reported  threshold
..  doses of 0  causing foliar symptoms in short-term (acute)  exposures
     (13, 15).   y^T^ng et al.  (15) found differential foliar sensitivity

 ,  a^cng six comercial cultivars exposed for 4 hr in a, greenhouse to
    0.10, 0.15, 0.20, or 0.25 ppm of 0_.  The cultivar America was
    slightly injured at 0.10 ppm, while Winter 31ooir.sda.le and  Bounty
16
,„  were injured at 0.15 ppm  (15).  Hill et al,  (.13) found  that  the
17
    injury threshold for four spinach cultivars, including  Hybrid  7,
IS
    was near 0.23 ppm for 2-hr exposures.  There are no reports  of the
    effects on  spinach of long-term (chronic) exposure to low  0_
20                                                             3
    concentrations .
21
         For recommendations of appropriate control strategies,  studies
22
    are needed  on the threshold doses of 0_ that can cause  iniurv  and
                                          3
24
23
    decrease crop yields.  The present study was designed to determine
    whether spinach cultivars vary in sensitivity to 0  and  to determine
25                                                    J

-------
  1   threshold doses of 0  for injury and decreased shoot yield.


  2   Spinach was exposed to low 0,  concentrations  for long periods in


  3   open-top field chambers (5).   The effaces  of  0- on. injury and


  4   yield  of 11 spinach cultivars  grown in  pots were measured.  Plants


  5   of  four cultivars- were grown in  the ground or in pots to determine


  g   whether edaphic conditions affected sensitivity.


  7                           MATERIALS AND METHODS


  .       Spinach (Spinacia oleraeea  L.)  seeds  were planted in 3.8-


  .   or  0.1-liter pots  containing a 1:1:1 ratio by voiune"~cff~~saad': ~~

                     4/
 ,Q   soil:Pro-Mix BX— .   Pro-Mix 3X is a cotnnercial aixture of peac


      aad periite with added nutrients (Premier  Brands,  Inc., New


      York,  N.  T.).   Planes  were chinned  to I/pot 9 days after planting.


      Planes grown is 3.8~liter pots were fertilized with 6 g/pct of


      14-4-5,  OT-P-E:}  on  12  September  and  with 3 g/?oc  of 10-10-10
14

      C2T-P-5)  on 5 October.


          Plants in 0.1  licar pots  wera  cransplantad into the ground
15

      ia  2.4 3 rows in clay-loani or  sandy-losa soil on  9 September.


      They were fertilized on 15 Septanber with  100 g/row of 10-10-10
ia

      Ol-P-tv)  placed in a  furrow, 8  cs. away froa the plants.
19

          Plants were watered as needed  to prevent wilting.   Insects
20   	
      4/
2*7   —   Mencion of connercial  products or equipment by nane does not


22    constitute  a guarantee  or  warranty of Che product  by the U.  5.


22   Deparcaent  of  Agriculture, or N'orth  Carolina  State University and


-A   does not  iaply  their approval  to  the exclusion of  other products


 «    chat siay  be  suitable.

-------
 1   were  controlled with weekly  applications of Carbaryl  (1-napthyl

 2   methylcarbaniate)  or a  commercial preparation of Bacillus

 3   thuringiensis.

 4         Open-top field exposure chambers  (5)  3-m  diameter x 2.4-m

 5   tall  were used.   In each of  two studies, plants were  exposed in

 f   chambers receiving charcoal-filtered air continuously or in chaia-

 •j   bers  receiving nonfiltered air continuously with 0. added for

 a   7 hr/day.   Ozone  was generated in  oxygen by silent electric

 _   discharge and constant concentrations  were dispensed  to the inlet

_Q   ducts of the nonfiltered-air (NF)  chambers for 7 hr/day (0920 to

     1020  hr EDI) as described previously  (8).  With this  method, we

     produced a  set of oxidant curves in the NF chambers  that had a

     constant relationship  to the changing  oxidant  concentrations in
ij                                      •
     arbi=-c air.  The daily 7 (0920 to 1620 hr) and 24 hr mean 0.
14                                                               ->
     concentrations at our  field  site from  10 September through

     17  October  1976 are shown in Figure 1. Ozone  concentrations were
16
     monitored in ambient air (AA) and  within chambers at  plant height
17
     using a monitoring system previously described (8).
13
                              Cultivar Sensitivity
19
           Seeds  of 11  cultivars (Table  2) were  planted in  3.8-liter
20
     pots  on 30  August 1976.   Two plants of each cultivar  were placed
21
     randomly in each  quadrant of eight chambers  (2 chambers in each of
22
     four  replicates).  Exposures began on  15 September and continued
23
     for 33 days.  Plants in 1 chamber/reulicate were  exposed continuously
24
     to  carbon-filtered air (CF). Plants  in the other chamber were
25

-------
  1   exposed continuously co  nonfiltered air with 0.08 ppa of 0_


  2   added to ambient  concentrations  for 7 hr/day (NF-4) .   The mean


  3   0. concentrations and diurnal fluctuations of 0_ for the CF and


  4   NF-4 treatments are  shown in Table 1 and Figure 2, respectively.


  5        The percentage  chlorosis and necrosis (in-jury) of individual


  6   leaves was estinated at  5Z increments (0-100%)  on 15  October.


  7   Plant shoots were harvested and  weighed on 19 October.  Shoots


  Q   were dried for 5  days at  70 C and weighed.  Analyses  of variance
  9   were performed and/'.LSD  (?_ =  0.05)  fces±s-we=a used as "a'aielH


 2£   separation technique when F  tests  were  significant.


 ^7                                 Dose Response


 J9         Seeds of the cultivars  America,  Winter Bloomsdale,  Hybrid 7,


 T,    and 7iroflav were planted on 31 August  1976.   Sixteen  chambers


 .,    vera used (faur chambers  in.  each of  four blacks).  Five  plants


 . -    of each cultivar grown  in 0.1-liter  pots were transplanted into

 15                                         '               '      7^
 ,~    the sround in. each of 2 rows/chamber  as shown in Figure  3.   The    ~
 16                                                               f-

      four plants nearest the chamber walls in each row were not used    •r-.f-sf-'

                                                                           _^*.«^J*^
      in data analyses.  Plants growing  in  the ground in one block, were     „_/
 Ho                                                                            ' ''
                                                                           ^S-r*-S
      subsequently discarded because of  poor  growth from an  unknown         -  -
 19                                                                          **-* '"'
                                                                             /}r
      cause in two plots.                                                   ^

20                              .                                            -
           Two plants of each cultivar grown  in the 3.8-licar  pots were    j^


      randomly placed on the ground in each of 4  quadrants/ chamber as       „_„„
22                                                                           >
                                                                           ^ ~-,2Z*
      shown in Figure 3.  Eight plants of Winter  Sloonsdale  and  Hybrid 7  ; ~'"~~
23                                                                          ,c*— ^.

      grown in 3.8-liter pots were placed in  an ambient-air  plot  (no        •;z
24                                                                         ^->-^

      chamber) in each block.                                              •'•''~Lss
23                                                                           f-

-------
  1        Exposures began on 10 September and continued for 38 days,

  2   Plants in. one chamber/block were exposed continuously to carfaon-

  3   filtered air.  Plants in 3 chambers /block, were exposed continuously

  4   to nonfiltered air, but in addition, each received a. different

  5   constant concentration of 0_ for 7 hr/day.  The mean added Q_

  g   concentrations were 0.01, 0.05, or 0.08 ppm for the NF-1, NF-2,

  7   and NF-3 treatments, respectively.  These additions resulted in

  g   7 hr/day mean concentrations for each treatment as shown in

  «   Table 1.  Figure 2 shows the mean diurnal concentratTaV~£Tuctua-

,Q   tions for each treatment.

--         Foliar injury and fresh weight responses were measured on

._   12 October and 13 October, respectively.  Plants were dried and

  _    weighed as- described previously.  Separate analyses of variance
             S           CAT.-V .....}
      &-£ LSD ass*s vara pes§£H:me4i for plants grown in each media.  A
l-»
      cs^biaad analysis was porforraed on plants in 3 blocks to determine

16
      vhsthar growth media affected the amount of loss in shoot weight
      caused by 0 .

                                     RESULTS
13
                              Cultivar Sensitivity
19
           Symptoms of foliar injury resembled those described previously
20
      (4, 15).  However, in this experiment, the major symptom was
21
      chlorosis rather than bifacial necrosis.  Foliar injury of  the
22
      11 cultivars ranged from 49 to 65% greatar at 0.13 ppm than at
23
      0.02 ppm (Table 2).  America, Winter Bloomsdale, and  Seven-R were
24
      less sensitive than Chesapeake, Hybrid-612, and Dixie Market.
25

-------
>-
  1        Thers were no obvious relationships between foliar injury

  2   and shoot fresh or dry weight (Table 2).  The correlation coefficients

  3   between injury and shoot fresh and dry weight were 0,069 and 0.052,


  4   respectively.  Percentage loss ia shooc fresh weight ac 0.13 ppzn


  5   03 ranged from 33% for Viroflay to 512 for Kybrid-612 (Table-2).

  5   If the effects oo shoot weight wera used as a measure of relative


  7   sensitivity, Aaerica and Viroflay ---are lass sensitive chan Hybrid-612,


  g   Dark. Green Bloomsdale, Seven-R, and Dixie Market.	


  «                                Dose—B.asponse


• Q         Injury on all four cultivars ia-crsased as the 0_ concantratior.


«.    incrsassd (Table 3).   The ozone trastaar.t and cultivar affects


-_    were significant but  thera was no significant cultivar x 0. treacseat intar-


.^    actiact in aichsr growth sadia.  The acsunt of foliar injury caused


, ,    b~ 0, was sizilar in  both siadia C'abla 3).   Mean foliar injury
1*4        J

      for all plazrs was 5, 38, and 35S at 0.05, 0.10, and 0.13 ppra of 5.,
              L6

                        Taa  corrslacion  coefficianc  across traacsents  becvean. shoot

                   frash weight and  shoot  dry  weight vas 0.97.   Therefore,  only cha
              13
                   effects of 0, on  shoot  fresh weight will be discussed further.
              19               3
                   The threshold 0   concantraticn  for decrsasad  growth depended
              20                  3
                   partially on the  growth nedia,  as vail ^s the culcivar (table 4);
              21
                   the interactions  between 0_ traaczaflt ar.d growth tnedia and between
              22                             3
                   0. treatment and  cultivar were  significant statistically but the
              23    3
                   three-way interaction vas not.  Tor th* cultivars cot2.bir.ad, the
              24
                   growth of ootred  plants  was decreased less by 0, than that of
              23             '                                     3

-------
                                      /7*.*r     (
  1   plants grown in the soil.  The is»&*& effect was significant at
                                                 A.
  2   0,06 and 0.10 ppm but not at 0,13 ppm.  Considering the 0.02-

  3   ppm 0  treatment (CF) as the control, the mean weight loss for

  4   all potted plants was 4, 25, and 65% at 0.06, 0.10, and 0.13

  5   ppm, respectively.  For plants grown in the ground, the.comparative

  5   losses were 18, 37 and 69%, respectively.  For potted plants,

  1   shoot weight of all cultivars except Viroflay was significantly

  3   affected at 0.10 ppm (Table 4).  For plants in the ground, shoot

  g   weight of Viroflay was significantly affected at 0.06 ppm while

ng   that of other cultivars was not.

11         The shoot weights of potted Winter Bloomsdale in AA (0,05 ppm

12   ®i) was 33.6 o as compared to 36.6 g for those grown in the NF-1

*^    cnanber treatment (0.06 ppm 0,).  However, Hybrid 7 plants growing

. ,.    ir. at^bietxt air were significantly smaller (47.1 g) than those

      proving- in tha NF-1 chambers (60.4 g).
15

           There were statistically significant quadrant and quadrant x
      cultivar effects for shoot weight i
17                                     A                           _

      no significant quadrant y. 0_ treatment nor quadrant x 0  treatment
13                               -^          f                3

      x cultivar effects-^vv wi-^-A^., +w*-1~-*-'-*~t •
19

                                   DISCUSSION
20

           The reason for greater decrease in shoot weights for plants

      grown in the ground than in pots at some 0  doses may be ralaced
22                                              -*

      to growth media differences in fertility, physical characteristics,
23
      water relations, or combinations of these or other edaphic factors.
24
      The reported effects of fertilizer rates and physical factors o£
25

-------
                                        10
  1    growth media on plant sensitivity to  0  have been reviewed (9,  11).

  2    Braver _et_ al.  (1)  have shown the importance  of nutrition on foliar

  3    injury caused  by 0-  on Viroflay spinach but  the cause and effect

  4    relationships  for  the main fertilizer elements have  not been

  5    determined.  Oxidants injured Bel W  tobacco less in open-top

  g    field  chanbers when  plants were grown in pots in a nix of peat-

  7    perlite-soil than  when they were grown in  the ground (5).   However,

  £    potted tobacco and pinto  bean plants  were  niora sensitive vhen grown

  n    in growth  oedia containing veraiculite,  perlite,  or  peat than in

 -Q    pots containing field soil (10).   In  our study,  roots of plants in

 ..     pots ware  zot  pot-bound and moisture  vas adequate to prevent

 -2    wilting.   While plants grown in tha ground were the  sane age as "hose

  ,     in pots, they  ware slower growing after  transplanting than those

       in the  pots.   These  results show a need  for  further  work to  determine
 1^

       relative responses to 0.  of plants grown in  different growth aedia.

           Foliar  injury causes decreased photosynthesis and,  therefore,
 16

       decreased  availability of aetafaolites required for growth.   Chang

       and Eeggestad  (2)  have shown a  direct ispairzrant  by  0  of  the

       photochemical  activity of photosystea II,  and  a decrease in  the
19
      amount  of  E-carotene  in the chloroplasts when  spinach'was  exposed
20
       to 0.35 pom 0-  for 60  to  80 ninutes.   In our dose-response  study,
21             '    3
       the correlation coefficient between foliar injury and frash  weight
22
      of shoots was  -0.186  for  plants  in pots and -0.147 for  plants in
23
       the ground.  The reason for lack of significant correlations between
24
      foliar  injury  and  fresh weight of  shoots is not clear.   Possibly
25

-------
                                        11
  1 large plant-to-plant variability in both injury and shoot weight

  2 within cultivars is a cause.  It is possible that better correlations

  3 would occur if injury and weight measures were taken on the same

  4 day.  However, apparently some cultivars can sustain more foliar

  5 injury than others with comparatively less decrease in shoot

  g growth.  For example, Viroflay was injured significantly more than

  7 was America but there was no difference in the effects of 0., on

  g weight of shoots (Table 2).   There were no significant differences

  n  in foliar injury between America and Seven-R but Seven-R weight

,-  loss was significantly greater than that for America (Table 2).

..       In a previous report (15) foliage of America was found to

  0  be more sensitive than foliage of Winter Bloomsdale, when they were
JM»

    exposed once for 4 hr to 0.10, 0.15, 0.20 or 0.25 ppm 0 .  In our
JL«3                                      •                   J
    study with chronic exposures, foliar sensitivity of these two cul-
14
    tivars was similar (Table 3).  The different results may be related

    to different cultural methods, doses of 0,, or growth conditions
16                                           3
    that differentially affected the sensitivity of the two cultivars.

         For the four cultivars common-to both of the present studies,
13
    foliar injury and loss of shoot weight for potted plants was greater
19
    at 0.13 ppm for the dose-response study than for the cultivar
20
    sensitivity study, probably because of the differences in duration
21
    of exposure.  However, the relative sensitivity of the four cultivars
22
    was the same in both studies (Tables 2-4).
23
         The threshold 0, concentration (7-hr/day mean) for significantly
24                      3
    (P - 0.01) decreased shoot weight of most of the spinach cultivars
25

-------
                                       12
  1  tested was between 0.06 and 0.10  ppm.   The  0.06 ppa  concentration

  2  is probably lower than levels  found in  some spinach  growing areas

  2  of the East (14)  and the 0.10  ppm concentration is probably exceeded

  ^  in some spinach growing areas  of  California (18).  Using the results

  2  reported in Table 4 with values at 0.02 ppta considered  as controls,

  g  we can roughly predict, with some extrapolation, probable weight

  -  losses at higher  0, concentrations.  Assuming  that ambient oxidant

  _  levels fluctuate  diumally like those at our field site,  with 7-hr/
  o

     day mean 0, concentrations of  0.07,  0.09, 0.11 and 0.13 ppa during

     37 days of growth,  the predicted  shoot  weight  decreases of a spinach
 •0

     cultivar with  average  resistance  would  be approximately 20,  30, 50,

     and 65Z respectively.   We have not  attempted to assign  spinach

     crop loss valuss  that  slight result  from various accounts of foliar

     injury.   With,  present  mechanical  harvesting  methods and the  prohibitive
 14
     ccszs  of  separating injured from  non-injured leaves, even small

     amcumcs  af injury could greatly decrease the value of a spinach
 16
     crop,  Hora foliar  injury would probably be  allowable on  spinach  to
 17
     be  canned than on spinach for  use as fresh market produce.
 13
         Our  study did  not  consider effects of Q   at different stages
 19                                               3
     of  growth.  Ambient fluctuations  in oxidant  concentrations (Figure 1)
 20
     were used  in determining  the dose.  The seasonal oxidanc  dose  ovar
21
     the past  several  years  near Raleigh, North Carolina has been  relatively
22
     constant;  the  7-hr/day  mean concentration has  usually been between
23
     0.05 and  0.07  ppra during  the summer months.   Loss  figures  might
 2A
     differ from year  to year  with  the same  total 0. dose but with
25
     different  levels  of 0_  occurring at various  growth stages.

-------
                                     13
  1                             LITERATURE CITED

  2 1.  Brewer, R. F., F. B. Guillemet,  and R.  K.  Graveling.   1961.

  3        Influence of N-P-K fertilization on  incidence and  severity

  4        of oxidant injury to mangels  and spinach.  Soil Sci.  92:298-301.
                                      ^ *
  5 2.  Chang, C. W., and H. E. Heggestad.  1974.   Effects of ozone on

  6        photosystem II in Spinacia oleracea  chloroplasts.
                                                    %
  7        Phytochemistry 13:871-873.

  g 3.  Daines, R. H., I. A. Leone, and  E. Brennan.  1960.  Air pollution

  o        as it affects agriculture in  New Jersey.  New Jersey Agr.

JQ        Exp. Sta. Bull. 794.

«,  4.  Daines, R. H., I. A. Leone, E. Brennan, and J. T. Middlaton.

,2        1960.  Damage to spinach and  other vegetation in New Jersey

, .         fron ozona and other airborne oxidants.  Phytopathology 50:

.t         570 (Abstr.).

    5.  Haagle, A. S., D. E. Body, and W. W. Heck.  1973.  An open-top

           field chamber to assess the impact of air pollution on plants.
16
           J. Environ. Qual. 2:365-368.

    6.  Heagle, A. S., D. E. Body, and G. E. Neely.  1974.  Injury and
13
           yield responses of soybean to chronic doses of ozone and sulfur
19
           dioxide in the field.  Phytopathology 64:132-136.
20
    7.  Heagle, A. S., D. E. Body, and E. K. Pounds.  1972.  Effect of
21
           ozone on yield of sweet corn.  Phytopathology 62:683-687.
22
    8.  Heagle, A. S., R. B. Philbeck, H. H. Rogers, and M. 3. Letchworth.
23
           1978.  Dispensing and monitoring ozone in open-top field
24
           chambers for plant-effects studies.  (Phytopathology, In Press).
25

-------
                                      14
  1   9.   Heck,  W.  W.   1968.   Factors.influencing expression of oxidant

  2          damage to plants.   Annu. Rav.  Phytopathol. 6:135-188.

  3  10.   Heck,  W.  W., and J.  A. Dunning.   1967.   The effects of ozone

  4          on  tobacco and pinto bean as  conditioned by several ecological

  5          factors.   J.  Air  Politic. Control Assoc.  17:112-114.

  6  11.   Heck,  W.  W., J.  B. Mudd,  and P.  R.  Miller.   1977.   Plants and

  7          microorganisms.   p. 437-585.   In:   "Ozone and Other Phoco-

  g          chenical  Oxidants."  Chap.  11, Vol.  2, National Acad.  Sci.,

  9          Washington, D. C.   1977.

 ,    12.   Heggestad, H.  E., A.  S.  Heagle,  and J.  P. Heiners.   1973.

 .            Effects of oxidant air pollution on  yields of green beans.

             Proc.  Inc.  Congr.  of Plant  Pathol.,  2nd,  Minneapolis,  Minnesota,

             1973.   (Abscr.).

     13.   Hill,  A.  C.,  H.  R. Pack,  M.  Tresfaow, R.  J.  Downs,  and L.  G.

             Transeras.  1961.   Plant injury  induced  by ozone.   Phyto-

             aachology 51:356-363.
16
     14.   Jacobson, J.  3.,  and  G. 0.  SalotColo,   1975.   Photochemical

             oxidants  in the Mew York-New Jersey  netrooolitan area.
13
             Ataos. Environ. 9:321-332.
19
     15.  Manning, W.  J., W. A.  Feder, and I. Perkins.   1972.   Sensitivity
20
             of  spinach cultivars to  ozone.   Plant Disease Reporter  56:
21
             832-833.
22
     16.  MacLean, D.  C., and R.  E. Schneider.  1976.   Photocheoical
23
             oxidants  in Yonkers, Sew York: Effects on  Yield  of Bean and
24
            Tomato.  J. Environ. Qual.  5:75-73.
23

-------
                                     15
 1  17.   Oshima, R.  J.,  R.  K.  Braegelmann,  D.  W.  Baldwin,  V.  Van Way,



 2          and 0.  C.  Taylor.   1977.   Reduction of  tomato  fruit size



 3          and yield by ozone.  J.  Amer. Soc. Hort.  Sci.  102:289-293.



 4  18.   Pitts, J.  N.,  J. L. Sprung,  M.  Poe,  M. C.  Carpelan,  and



 5          A.  C. Lloyd.  1976.  Corrected  South  Coast air basin



 6          oxidant data:  Some conclusions and implications.  Environ.



 7          Sci. and Technol.  10:794-801.



 g  19.   Rich,  S.  1964.  Ozone damage to plants.  Annu.  Rev. Phytopathol.



 g          2:253-266.                                    	



JQ  20.   Thompson,  C.  R., E. Hensel,  and G. Kats.  1969.   Effects of



*7          photochemical air pollutants on Zinfandel grapes.  Hort.



j^          Sci. 4:222-224.



,,  21.   Thompson,  C.  R., G. Kats,  and J. W.  Cameron.  1976.   Effects



.,          of  ambient photochemical air pollutants on growth, yield



-_          and ear characters of two sweet corn  hybrids.   J. Environ.



.,          Qual. 5:410-412.
lo



17



13



19



20



21



22



23



24



25

-------
 Table 1.   Mean ozone (0 ) concentrations for  7 hr/day  (0920  to  1620  hr  EDT)
           and standard deviations in two experiments to  determine the effects
           of 0- on spinach.
a/
treatment—
Asbiant Air (AA)
Carbon Filtered Air
Cultivar Sensitivity Study—
O.-ppm Standard &—
deviation
0.047 0.018 330
0.024 0.012 330
Dose-Response Study—
0,-ppa Standard
deviation
0.046 0.019
0.024 0.012
*&
380
380
    (CF)
                     c/
Nonfiltered Air -r 0 — '
                        0.056    0.019
                                                                              1520
Nonfiltered Air 4- 0
   (NF-2)

Nonfiltered Air +• 0
   (NF-3)

Nonfiltersd Air +• 0
   (NF-4)
                         0.125
0.027
1320
                                                          0.096    0.027      1520
                                                          0.129    0.027      1520
a/
    Ozone "-a.3  iddad  to asbier." concentrations in nonfilterad-air  (NF) chambers
    for  7 hr/ds-  (G920 to 1520 hr ZDT).
—   Heatis  for  15  September through 17 October, 1976.

—   Means  for  10  September through 17 October, 1976.

—   The AA and CF means were calculated from N number of 2-oinuta readings
    (10 readings/7 hr/day)  froia one sampling location/mean.  The 117 aeans were
    calculated from N number of 2-sinuta readings (10 readings/7 hr/day) from
    four chasibers/mean.

-------
Table 2.  Injury and growth response of 11 spinach cultivars exposed in open-top field chambers to carbon-
          filtered air (0.02 ppjn 0„) or non-filtered air with 0  added for 7 hr/day  (0.13 ppm 0 }.-
                                  J                            _y                               J
Cultivar


America
Winter Bloomsdale
Seven-R
Hybrid-424
Hybrid 7
Viking
Dark Green Bloomsdale
Viroflay
Chesapeake
Hybrid-612
Dixie Market
LSD 0.05
— 0_ concentrations
i / J
Foliar
Injury

49 h
52 hi
52 hi
54 hij
56 hijk.
58 hijk
58 hljk
6Q ijk
63 jk
65 k
65 . k
9.95
are means for

0.02j
(>0
4,'i.O
-.17.5
67.6
65. 'J
61,'J
48.4
51.2
68.0
61.5
62.6
58.2

7 hr/day
SUoot FresU Weight
put 0.13 f
(r.) (
20.8
20.6
30.4
30.2
35,3
27 . 1
21.5
45.6
3$. 7
24.4
26.2

(0920 to 1620 hr


% lo!Jti}->
36 hi
45 ij
55 jlc
42 111
43 hi
44 hij
58 k
33 h
42 hi
61 Y
55 jk
11.00
EOT) for
Shoot
0.02 ppm

-------
 Table 3.   Percentage foliar injury per leaf of four spinach cultivars grown
           in pocs or in Che ground and exposed to different concentrations of
           ozone.5.'


Treatment


NF-1
NF-2
NF-3
7 hr/day-
meaa 0.
cone.
(ppa)

0.06
0.10
0.13
./


America


3
41
65
Hean Foliar Injury - %—

Winter
Bloomsdale

Plants in
7
37
62


Hybrid

Pots - Z
9
44
63
Plants in Ground - %
NF-1
N?F-2
NF-3
0.06
0.10
0.13
3
36
60
3
33
65
9
39
69


7 Viraflay

Injury
6
37
59
In j ury
0
36
70


Jra*,
"
—
8*
40**
64**

5*
36**
66**
a/
    Concentrations shown  are  the neans  for 7 hr/day  (0920  co 162Q hr SOT)  for
    33 days  (10 Septaaber through  17  October).
b/  „ .
—   m 1
c/
 Joliar is/jury is cafined as (Injury of NF-treatad plants - Injury of CF-
 treated pleats).  Isch cultivar value for pottsd plants is the sean of
 96 leaves (3 leaves aa 3 plants in 4 blocks).   Each cultivar value for
 plants in the ground is the niean of 72 leaves  (3 leaves on 3 plants in-. 3
 blocks).  Theresa percentage foliar injury (chlorosis and necrosis) for •^.-^/••^
'CF-treated-CO.02 ppc) cgasrSS of America, Winter Bloomsdala, Hybrid 7,
"and Viroflay plants in pots was 3, 5, 10, and  13, respectively;  the
 comparative values for plants in the ground were 1, 2, 3, and S, respectively.

 The ? tests for  treatment and cultivar ware highly significant but the
 treatment x cultivar interaction was not significant for either  growth
 aedia.  * and ** = significantly different fron the controls at  the 0.01
 and 0.05 level of confidence according to the  treatment LSDs.

-------
                                         19
  Table 4.  Percentage  loss  of shoot  fresh veight  of  four  spinach cultivars
            grown in  pots  or in the,ground and  exposed  to  different  con-
            centrations of  ozone.—
Treatment
NF-1
NF-2
NF-3
NF-1
NF-2
NF-3
7 hr/day^
mean 0_
cone.
(ppm)
0.06
0.10
0.13
0.06
0.10
0.13
Fresh Weight of Shoots - Percentage Loss-
America
11
33**
60**
23
39**
70**
Winter
Bloomsdale
Plants
8
35**
70**
Plants
19
44**
73**
Hybrid 7
in Pots
.6
29**
71**
in Ground
4
35**
61**
Viroflay
•_c/
11 ^
59** ^
26* / !
35** *
72** £
—   Concentrations  shown,  are the neans for 7 hr/day (0920  to  1620 hr EDI)  for
    38 cays  (10  September through 17  October).

b/  _          ,        ,  ..   ,     , nn   .weight  of  NF-treated plants%  irt_
—   Percentage less  is  d2-^r.ad  as 100 - (—r=r	r-r^	fc j f\	)  100.
             0                            weight  or  CF-treated plants
    Each value for  pottac plants is  the sear. o£  32  plants  (S  plants  in - blocks).
    Each value for  plants in the ground is the mean of 24  plants  (3  plants  in 3
    blocks).  The 2=an  fresh weights  of shoots for  CF-treated controls (0.02 ppm)
    of America,  Winter  Blooi^sdale,  Hybrid  7, and Viroflay  plants  in  pots were
    45.1, 39.4,  64.5, and 69.Og,respectively; comparative  values  for plants in the
    ground were  21.1, 20.6,  35.6, and 40.5 g respectively.  The F tests for treatment,
    cultivar and the trestnent  x cultivar  interaction were highly significant for
    both growth  mediay?X^"anj) ** = significantly different from the  respective
    "contr51s""aT~the 0.01  ariiri 0. 05 level of confidence, respectively  according to
    the LSDs for the cuTtivar x treatment  interaction.

c/
—   The minus sign  indicates a  percentage  gain.

-------
Table 5.  Degrees of freedom and nean squares for foliar injury and shooc
          fresh weight of four spinach culcivars grown in pots or in Che
          ground and exposed to different concentrations of ozone.

Foliar Injury
Source
Block
Treatment (T)
Error A
Cultivar (C
T x C
Error B
Shoot Fresh "eiaht
Source
Block
Treatment (T)
Error A
quadrant C")
T x q
Error 3
Culcivar (C)
T x C
q x c
T x q x C
Error C

df


3
3
9
3
9
36


3
3
9
3
9
36
3
9
9
27
144
Plants in Pots
Mean Square

-
169
41093 **^
245
996 **
40
121


1217
33869 **
336
5229 **
269
211
23016 **
992 **
390 **
211
204
Plants
df


2
3
6
3
9
24


2
3
6
3
9
24
3
9
9
27
96
in the Ground
Mean Square


31
34347 **
26
- 423 -**--
75
46


325
7227 **
430
273
137
93
5363 **
256 **
56
96
80
       The F test vas significant at ?_ » 0.01.

-------
  1                              FIGURE LEGENDS


  2 Figure 1.   Mean 0  concentrations in anbient air (AA) for 7 hr/day


  3        -    (0920 to 1620 hr EDI) and 24 hr/day 4.8 ko south of


  $            Raleigh, N. C. from 10 September through 17 October, 1976.


  5            A •% C « duration of the dose-response study; B •> C =


  g            duration of the cultivar sensitivity study.


  7 Figure 2.   Mean, hourly 0. concentrations in ambient air (AA),


  a            carfaon-filtered-air chambers (CF) and nonfiltered-air


  Q            (NF) chambers to which different: concentrations of 0-


,Q            were added for 7 hr/day (NF-1, 2, 3) froo 10 September


-.             through 17 October, 1976.  The hourly means for the


.,             }i"?-4 treatment are values for 15 September through


               17 October, 1976.


    Fisura 3.   Diagram of spinach cultivar positions in chamber plots;


               o = potted plants, A = plants in Che ground.  1 =• America,


               2 = Winter Bloomsdale, 3 = Viroflay, 4 = Hybrid 7.
15


17


13


19


20


21


22


23


24


25

-------
    O.O8
    O.O7
 a
 a  O.O6
   O.O5
u
Z
O
   O.O-*
   O.O3
Z

O
M

O  O.O2
   O.O I
   o.oo
                                      \
                                      c
             9/1O
                                           I
                                                         I
                           9/2O
             9/3O


          OATE
                                                      IO/IO
    O.IS
    O.I*
  I o.ia
  a
  t

 Z
 O 0.1O
 2  o.aa

 u
 z
 O
 
-------
*
A
*
*
*
ft
*
*
*
A
*
A.
*
*
*
*
A
T
i
•
s
1
>
I
1
*
X
1
4
•
>
4
»
1
>
»
*
1
*
•
4
1
*
1
*
*
>
X
*
*
*
*
*
*
*
A
*
*
*
«
*
*
*
k^

-------
                            Appendix C
  1               Yield Responses of Winter Wheat  Cultivars  to

  2                          Chronic Doses of Ozone

  3          Allen S.  Heagle, Suzanne Spencer, Michael B.  Letchworth

  ^       Plant Pathologist, Southern Region, Science and  Education

  e  Administration, U. S.  Department of Agriculture, Plant  Pathology

  g  Department, North Carolina State University,  Raleigh, N. C.  27650;

  -  and Graduate Research Assistant and Plant Physiologist  respectively,

  _  Plant Pathology Department, North Carolina State University,

     Raleigh, N. C.  27650.

10                          ~
                                    Abstract

          The relative sensitivity of 11 cultivars of soft red  winter

     wheat, Triticm aestivum L., exposed as young plants  to ambient

     levels of oxidant air pollution was determined.   On the basis of the
14
     shoot weight response, the cultivars Holly and Blueboy  II  were

     significantly more sensitive than Oasis or Coker 47-27. Plants of
16
     these four cultivars,  grown in pots or in the ground, were exposed

     for 54 days in open-top field chambers to different concentrations
18
     of 0_ added for 7-hr/day to existing levels of ambient  oxidants.
19       3
     The effects of 0  on injury, growth, and yield were determined.
20                   3
     For the four cultivars combined, in both growth medias, the
21
22
        Cooperative investigations of the U. S.  Department of Agriculture
23
     and the North Carolina State University.   Paper No.      of the Journal
24
     Series of the North Carolina Agricultural Research..Service,    Raleigh.
25

-------
  1  threshold 0_ concentration (7-hr/day mean) for significant injury

  2  and decreased yield was between 0.06 and 0.10 ppm.   For potted

  3  plants, exposed to 0.10 and 0.13 ppm of 0_, seed weight yields were

  4  10 and 27% less, respectively, than seed yield of plants in charcoal-

  5  filtered-air chambers (0.03 ppm).  For plants in the ground at 0.10

  g  and 0.13 ppm, the yields were 16 and 34% less, respectively, than

  7  at 0.03 ppm.  The relative sensitivity of cultivars to growth effects

  a  as young plants was not a good predictor of relative sensitivity of

  a  cultivars to yield effects.

 .-       Additional key words:  air pollution, photochemical oxidants


 11
                                   Introduction

          Present estimates of economic losses to agricultural crops

     from exposure to air pollutants are based primarily on visual
 14
     estiaates of foliar injury (1, 2, 8,  9,  10, 11,  12, 13).   However,

     except for foliage crops, little is known of the relationships
 16
     between injury of leaves and  loss of  yield (1).   Experimental

     effects of ambient oxidants on yield  of  crops have  been reported for
13
     only a few species and recent reviews have emphasized the need for
19
     further research (6,  14,  17).   There  are no reports of the effect
20
     of long-term exposure to ambient oxidants on yield  of wheat,
21
     Triticum sp.
22
          In greenhouse tests (7,  15)  wheat was relatively sensitive to
23
     ozone (0_),  the principle phytotoxic  component of ambient photochem-
24           3
     ical oxidants.   In a  field test,  ozone at 0.20 ppm  for 4-hr/day on
25

-------
  1  7 days during anthesis significantly decreased  yield  of winter


  2  wheat, T^  aestivum L., Arthur 71 and Blueboy (16).  In another


  3  field test,  the biomass of T^ aestivum was decreased  by exposure


  4  to 0.08 - 0.10 ppm of  0  for 5-hr/day but effects  of  0  on yield


  5  were not reported (14).


  $       Our objectives were to determine threshold concentrations of


  7  0_ in long-term (chronic) exposures, required to cause significant


  g  injury and decrease growth and yield of T_. aestivum cultivars under


  9  field conditions.  The relative sensitivity of  11  cultivars was


JQ  determined and four cultivars with varying degrees of sensitivity


i^  were selected for dose-response studies.


12

,«                            Materials and Methods


. ,        Cultivar sensitivity - Eleven cultivars of soft  red  winter


._   wheat, Triticua aestivum L., (Table 1) were tested.  Seeds were


  ,   planted in 3.8-liter pots containing a 1:1:1 mixture  of sand:
lo

     Metro-Mix 200 :soil (Appling, Typic Hapludults; clayey, Icaolinitic


     thermic) on 6 August 1976.  Metro-Mix 200 is a  mixture of perlite,
13

     peat moss, vermiculite, and sand with added nutrients (W. R. Grace
20   	

        Mention of a trademark, proprietary product,  or vendor does not


     constitute a guarantee or warranty by the U.  S.  Department of Agricul-


     ture or the North Carolina Agricultural Research .Service,  and does
23

     not imply approval of it to the exclusion of  other products or vendors
24

     that also may be suitable.                       •  -
23

-------
  1  and Co., Cambridge, MA..)-  Seedlings were thinned to three/pot on


  2  16 August.  Plants were watered as needed to prevent wilting.


  3  Insects were controlled with one application of Malathion and


  4  Carbaryl.


  5       Plants in five pots/cultivar were placed randomly in each of


  5  two open-top field chambers (3^). Plants in one chamber were


  7  exposed continuously to charcoal filtered air (CF);  those in the


  g  other chamber were exposed continuously to nonfiltered air (NF).


  9  Ozone (0.10 ppm = 196 yg/m )  was added to existing  oxidant concen-


 10  trations in the air of the NF chamber for 7-hr/day  (0930 to 1630 hr


 11   EDT) for 27 days starting on 17 August.  Ozone was  dispensed to  the


 12  inlet air stream of the NF chamber and was monitored at plant-canopy


 ,.   height in both chambers using an automatic dispensing and monitoring


 .,   sjste^ described previously (4).


 1         Fresh and dry (70° C - 5 days) weights of plant shoots were


     treasured on 15 September.  Analyses of variance were performed and
 16

     significant differences between cultivars were identified using  the


     LSD test when the F test was  significant (P = 0.05).
 13

          Dose-response - Four cultivars were selected on the basis of
 19	

     their sensitivity to 0  as seedlings;  Holly and Blueboy II were
20                         3

     sensitive and Oasis and Coker 47-27 were resistant  (Table 1).


          An  0.8 ha field was fertilized with 8-8-8 (N-P-K)  fertilizer
22

     at  the rate of 113 kg/ha prior to  planting.   Seeds were planted  at


     the rate of 70 kg/ha on 2 November, 1976,  using a 12-row grain


     planter  with a 17.5 cm row spacing. The hopper of  the  planter was
25

-------
  1  partitioned to allow a separate cultivar to  be  planted  in  each


  2  of three rows (three four-row strips  containing one  row of each


  3  cultivar in the same sequence).   On 3 November,  seeds of each


  4  cultivar were planted in 3.8-liter  pots containing a 1:1:1 mixture


  5  of sand:Metro-Mix:sandy-loam soil (Appling).  Potted plants were


  6  watered as needed and left outdoors for the  duration of the winter.


  7       On 15 March 1977, 20 3 x 2 m field plots  (five  in  each of


  3  four blocks)  were selected on the basis of uniform plant appearance


  g  and physical  soil characteristics within each block.  Two  blocks


J_Q  were located  on sandy-loam soil (Appling) and  two blocks were  on


jj^  clay-loam soil (Cecil, Typic Hapludults). On 21-23  March, plants


»2  in field plots were thinned to one  plant/5-8 cm and  plants in  pots


.,  were thinned  to two/pot.   Fertilizer  (10-10-10,  N-P-K)  was applied


.,   on 29 }£arch at the rate of 320 kg/ha  in field plots  and 5  g/pot.


^ _   Plants in the ground and in pots were watered as needed to provide


  ,   uniform soil  moisture and prevent wilting.   Aphids were controlled
lo

     with an application of Malathion on 21 April.


          Open-top field chambers, 3 m diameter by 2.4 m  tall,  (3,  4)
13

     were placed on 16 field plots (four plots in each of four  blocks)


     on 28 March;  the fifth plot in each block remained in ambient  air
20

     (AA)  with no  chamber.   Plants in one  chamber per block  were exposed
21

     continuously  to charcoal-filtered air (CF).  Plants  in  the remaining
22

     three chambers were exposed continuously to  nonfiltered (NF) air
23

     (particulate  filter only).  However,  from 9  April to 31 May 1977,
24

     small constant concentrations of 0  were added  to -the existing

-------
  1  ambient oxidant concentrations in the NF chambers for 7-hr/day

  2  (0930 to 1630 hr EDT).   Ozone addition of 0.02 ppm (NF-1)  resulted

  3  in 7-hr oxidant curves  that resembled ambient curves by making up

  ^  for the 0_ lost in the  chamber air handling system.   Ozone addition

  5  of 0.06 ppm (NF-2) or 0.09 ppm (NF-3) resulted in 7-hr oxidant

  g  curves with 0  concentrations averaging 0.04 and 0.07 ppm, respectively,

  •j  above ambient concentrations.

  .       The design for potted plants was similar to that for  plants in

  _  the ground.   Eight pots per cultivar  were randomly placed  in each of

 ,ft  12 open-top chambers and in three ambient air (AA) plots (two pots

 .    in each of four chamber quadrants)  on 29 March.   This provided for

     three replicates of the five treatments as described for plants

     grown in the ground.

          When exposures began,  plants in  the ground  had  five to six
 14
     leaves with a mean height of 28,  34,  45,  and 41  cm in blocks 1-4,

     respectively.   Plants in pots also  had five  to six leaves  with a
 16
     mean height  of 28  cm.   Plant height,  growth  stage, and foliar injury

     were recorded once each week for  6  weeks  starting on 19 April.
13
     Injury (chlorosis  and necrosis) was visually estimated in  5% incre-
19
     ments (0-100%)  on  the four  uppermost  leaves  of three plants per
20
     cultivar for each  treatment in two  blocks.
21
          Plants  were harvested  on 8-10  June.   For plants in the ground,
22
     yield measures  were taken for two rows  per cultivar  (one row in each
23
     half  of  the  chamber).   Each of the  eight  rows were subdivided into
24
     six 40-cm sections  from which a sample  of  four plants  were randomly
23

-------
  1 chosen for yield measure.   Plants in Che two outer and  two  center

  2 rows of each plot and those in the 20-30 cm at the ends of  rows

  3 were used only as borders.  All potted plants were harvested and

  4 the two plants/pot were treated as one sample.  The total shoot

  5 weight (stems, leaves, and heads), and number and weight of heads

  £ were determined at harvest.  The heads were threshed by hand and

  7 seed weight per sample, weight of 100 seeds, and seed moisture content

  g were measured.

  o       Separate statistical analyses were performed on data  from

JQ plants in the ground and for potted plants.  Analyses of variance

•«  were performed and LSD (P = 0.05) tests were used when  warranted by

-»  significant F tests.  Regression analyses were performed to determine

...  relationships between percentage foliar injury and seed yield for

, ,  Dlants in each medium separately using the block x treatment x
14

    cultivar means.


16

                                     Results

         Cultivar sensitivity - Foliar symptoms of 0  injury included
18                                                  j

    chlorosis and small white necrotic areas (flecking), as previously

    described (7).  Bifacial necrosis occurred on young leaves  of
20
    Ruler, Holly, and Blueboy II, but not on other cultivars.  A significant
21
    interaction between 0_ treatment and cultivars occurred for shoot
22                       3

    dry weight but not for shoot fresh weight, although the cultivar
23
    trends for both measures were similar (Table 1).  Ozone caused dry
24
    weight decreases ranging from 42% (Ruler) to 8% (Coker  47-27).
25

-------
  1       Dose-response — ozone concentrations  -  The daily  7-hr  (0930  to


  2  1630 hr  EDT)  and 24-hr mean 0_  concentrations  in the ambient air at


  3  our field  site near Raleigh,  N.  C.,  are  shown in Figure 1.  The


  4  mean diurnal  fluctuation in 0  concentrations  for the AA, CF, NF-1,


  5  NF-2 and NF-3 treatments are shown in Figure  2.  The mean 7-hr/day


  6  0.  concentration exceeded 0.08  ppm on each  day from 12  May through


  7  20  May,  the period when wheat plants were in  the watery-ripe to


  9  milky-ripe stage of development.  The highest  hourly mean 0. concen-


  9  tration  (0.14 ppm)  occurred on  18 May.


 £0       For the  period 9  April through  31 May, the mean 7-hr/day 0


 jj_  concentrations  for the AA,  CF, NF-1, NF-2 and  NF-3 treatments were


 j£  0.06, 0.03, 0.06,  0.10 and  0.13 ppm, respectively.  Differences in


 •*  mean 7-hr  0   concentrations between replicates of a given treatment


 ,,   for potted plants  and  for plants in the  ground x^ere less than 0.01


 15   ?pn-

 ,.      - growth and  injury - Ozone did not affect  the date  of flowering
 10        	——

     or  rate  of maturity.   Plant height was not  significantly affected  by


     0_  in either media  except at  the last measurement date when plants in
 13   J

    pots at  0.13  ppm were  6  cm  shorter than plants at 0.03 ppm.


         The overall trends  for injury were similar whether plants were


    grown in pots or in  the  ground (Table 2).  Foliar injury increased


    rapidly  in all treatments during the period when estimates were made,
22

    one week before  flowering to when kernels were in the mealy-ripe
23

    stage (Figure 3).  Injury at 0.10 (NF-2) and 0.13 ppm (NF-3) was
24

    significantly greater  than at 0.03 ppm (CF)  on all but  the last
25

-------
  1 date of estimate when plants were starting to mature in all treatments.

  2 In both growth medias, the mean injury was slightly greater in the

  3 NF-1 and AA treatments than in the CF treatment but the differences

  4 were not significant (Table 2).

  5     For plants in pots, the cultivar x treatment interaction for

  g injury was not significant except on the fourth estimate date.  At

  7 this time, more injury was present at 0.10 ppm of 0, on Coker 47-27

  Q and Blueboy II than for Holly and Oasis.  There were no significant

  g cultivar differences in the overall amount of injury (mean of first

5« 5 estimate dates) for potted plants, although Holly showed somewhat

., more injury than other cultivars at 0.06 ppm (NF-1) (Table 3).

.«     For plants in the ground, the cultivar x treatment interaction

   was significant on the second, fourth and fifth estimate dates.  On

   these dates, Coker 47-27 generally showed significantly more injury
14
   caused by 0.10 ppn of 0  than did Blueboy II.  This difference is also

   reflected in the overall (5 week) injury means for plants in the
16
   ground (Table 3).

      - weight and yield - The 0  treatment and cultivar effects were
13                              3

   highly significant for all weight measures taken.  For plants in
19
   chambers, the threshold 0_ concentration (7 hr/day mean) was the
20                          J
   same for all weight measures in both growth medias (between 0.06 and

   0.10 ppm) (Table 2).  Weight decreases were slightly greater for
22
   plants in the ground than for plants in pots.  Seed weight per plant
23
   (yield) for plants in the ground at 0.10 and 0.13 ppm was 16 and 33%
24
   less, respectively, than yield at 0.03 ppm; the comparative values
25

-------
                                        10
  1 for potted plants were 10 and 27%, respectively (Table 2).  Similar

  2 trends occurred for the other weight measures.  The percentage

  3 decrease in seed weight per plant was slightly higher than the

  4 percentage decrease in weight of shoots (heads, leaves, and stalks)

  5 or weight of heads per plant.

  g      The data show that the decrease in yield was caused by decreased

  7 seed numbers as well as by decreased weight per seed (Table 2).   For

  a example, at 0.13 ppm, the mean weight of 100 seeds was decreased by

  o 17% but the yield was decreased by 30%.

 3Q      The cultivar response to 0  was different in both medias (Table

 «,  3).  For plants in pots, the yield of Holly was decreased more than

 ., that of most other cultivars at 0.10 and 0.13 ppm.   For plants in the

 ,_  ground, yield of Coker 42-27 was decreased more than that of other

 , .  cultivars at all 0. concentrations (Table 3).
 IQ                    J
         Significant chamber position effects occurred for yield of

    plants grown in both medias.   For potted plants,  yields were 4%  less
 Id
    in the two northern chamber quadrants than in the two southern quadrants.

    However,  there were no significant quadrant x 0_  treatment interactions
 13                                                 -*
    for any of the weight measures taken.   For plants in the ground,
 19
    yield was 7% less  in the sampling position closest  to the northern
20
    edge of the chambers than yield in other sampling positions.   At  0.10
21
    and 0.13  ppm,  yield at the northern-most sampling position was
22
    decreased by 20 and 45%,  respectively compared to mean yield decreases
23
    of 16  and 33%  respectively at  the other  positions.   However,  there

    were no significant treatment  x position x cultivar interactions.
25

-------
                                       11
  1   - correlations between injury and yield - A linear regression


  2 analysis was performed using the block x cultivar x treatment means


  3 for seed weight per plant (yield), weekly mean foliar injury and


  4 6-week mean foliar injury.  In both medias, the correlations were


  5 highly significant for each weekly period and for the 6-week mean.


  g For plants in pots, the correlation coefficients were -0.82, -0.74,


  7 -0.71, -0.67, -0.68, and -0.56 for the consecutive individual weekly


  g injury means respectively, and was -0.75 for the overall (6-week mean)


  a injury values.  The regression equation between seed weight (y) and


,Q overall injury (x) was y = 6.50 - 0.367x.  For plants in the ground,


., the correlation coefficients were -0.59, -0.59, -0.55, -0.53, -0.46


.- and -0.33 for the consecutive weekly means respectively, and was -0.51


... for the overall injury values.  The regression equation between seed


  , weight (y) and overall injury (x) was y = 5.78 - 0.311x.


15

                                  Discussion
16

        In the present study, plants were treated by adding constant


   amounts of 0. to nonfiltered air rather than to filtered air.  Thus,
13             3

   the daily dose of 0_ was determined partly by daily and hourly changes
19                    ->

   in ambient 0, concentrations.  We chose this approach because of the
20             J

   complex nature of photochemical oxidant air pollution.  Plant response
21

   to. 0_ might be affected by other components in the photochemical



23
22
   oxidant complex but there is little information on the subject. The
   use of filtered air would interfere with any possible interactions
24
   of this type.  In most areas, oxidant concentrations "follow a diurnal
25

-------
                                        12
  1  pattern similar  to  that  shown  in Figure 2, although concentrations

  2  are different  from  day to  day  (Fig. 1) depending on local and

  3  regional weather.   Relationships between the effects of 0, at

  4  constant levels  and the  effects of 0, at changing levels have not

  5  been shown.  Therefore,  we chose to add small constant amounts of 0_

  6  to  the  existing  oxidant  complex during the daily period when concen-

  7  trations of 0  are  normally the highest (0930 - 1630 hr EDT).

  g       Previous methods of describing ambient pollutant doses include

  9  seasonal means, weekly means,  24-hr means, ppm hrs, peak hourly

 20  means,  and number of hours above a set concentration.  None of these

 jj^  methods  adequately  describe the dose from a biological standpoint

 *2  because  pollutant dose - plant response curves are not linear and

 «3  plants may respond  differently to pollutants at different times during

 -,   growth.  Doses have also been described in terms of percentage of

 . -   tic=  or  number of hours  above set concentration intervals, but

 , -   neither  of these methods consider the timing of exposure to given
 io
     concentrations in relation to plant growth stage or time of day.  In

    our experience, the 7-hr/day (0930 to 1630 hr EDT)  and 24-hr/day
 18
    means, adequately characterize the dose from a biological standpoint.

    At our field site, the 7-hr/day mean 0., concentration rarely varied

    by more than ^0.02 ppm from the daily minimum or maximum concen-

    tration from 0930 to 1630 hr EDT.
 22
         The mechanism for decreased yield from exposure to 00 appeared
23                                                           J
    to be through foliar injury which decreased photosynthesis,  causing
mi^9
    slower growth and a decrease in the number and size of seeds.
23

-------
                                        13
  1 Injury was progressive,  beginning  on  lower leaves and advancing, with


  2 continuing exposure,  to  younger  leaves.   It is possible  that


  3 environmental alterations  caused by the  open-top chambers  affected


  4 the sensitivity of  leaves  to  0_.   However, there are no  reports


  5 showing significant changes in sensitivity caused by environmental


  g variations of the magnitude caused by the chambers  (4, 6).  Light,


  7 measured in the photosynthetically active region of wavelengths


  9 (PAR), averaged 12% less and  temperature 0.7 C higher in the  chambers


  g than in ambient air (4).  The chambers did not affect relative


20 humidity (3)  but the air velocity  in  chambers was constant  at  about


H 2.5 km/hr (4) compared to  variable velocities in ambient air.  Foliar


j2  injury of plants in ambient air  (7 hr/day mean of 0.06 ppm of 0_)


»3  was not significantly different  from  that in the NF-1 chambers at


,i  the sane relative dose of  0_  (Table 3).   However, Holly  and Oasis


, -  grown in the ground were more injured in ambient air than  in  chambers.


, -       The cause for  greater yield decrease for plants grown in the
1&

    ground at the northern sampling  position (about 25-65 cm from the


    chamber frame)  is not known.  The  cause  may be related to  small
18

    differences in air  velocity,  light intensity, soil  moisture,  or  a


_^  combination of these factors.
20

         Drought stress is known  to  decrease the sensitivity of plants


    to gaseous pollutants (6). The  present  results were obtained in-a


    relatively normal growing  season although plants were watered to
23

    prevent wilting. While different  results might occur during  seasons
24

    with extreme weather conditions, we feel that similar effects
23

-------
  1 would occur during most  seasons with similar oxidant concentrations


  2 and adequate soil moisture.


  3      Further refinements are needed in protocols for screening


  ^ winter wheat cultivars for sensitivity to 0.,.  Neither  the cultivar


  e sensitivity test, performed on seedlings, nor foliar sensitivity of


  * older plants, adequately predicted the relative sensitivity of


  - cultivars to loss of yield caused by 0 .  These results may be


  a related to changes with  age in relative foliar sensitivity of
  o

    cultivars, to cultivar differences in relative tolerance to foliar


  ft injury, or to a combination of these factors.  We do not understand


    why the relative sensitivity of cultivars to yield loss was


    different in the two medias; Holly was the most sensitive cultivar


    in pots and Coker 47-27 was the most sensitive cultivar in the
13

    grcua-d.  Much reoains to be discovered about the ways that methods
14

    of culture and exposure affect the response of plants to air pollu-


    tants.
16


17

                       Acknowledgements
18

         The authors thank Hans Hamann for statistical analyses and
19
    Cindy A. Mitchell and Robert P. Philbeck for technical assistance.
20


21


22


23


24


25

-------
                                 15
                         LITERATURE CITED

  1   1.  BENEDICT, H.M., C.S. MILLER, and R.E. OLSON.  1971.  Economic

  2           impact of  air pollutants on plants in the United States.

  3           Stanford Research Inst.  SRI Project LSD-1056, Menlo Park,

  4           Calif.  77 p.

  5   2.  FELICIANO, A.  1971.  1971 survey and assessment of air pollu-

  g           tion damage to vegetation in New Jersey.  Cooperative Exten-

  7           sion Service, Rutgers - The State University, New Brunswick,

  g           N.J.  43 p.

  «   3.  HEAGLE, A.S.,. D.E. BODY, and W.W. HECK.  1973.  An open-top

,-           field chamber to assess the impact of air pollution on

..            plants.  J. Environmental Quality.  2:365-368.

-.   4.  HEAGLE, A.S., R.B. PHILBECK, H.H. ROGERS, AND M.B. LETCHWORTH.

              1978.  Dispensing and monitoring ozone in open-top field

              chambers for plant-effects studies.  Phytopathology (in press).
1*
      5.  HECK, W.W., AND C.S. BRANDT.  1975.  Impact of air pollutants

              on vegetation:  crops, forests, native.  In:  "Air Pollution"
16
              (A.C. Stern, ed.), 3rd ed., Vol. 2, Chap. 14.  Academic Press,

              New York.  (in press).
18
      6.  HECK, W.W., J.B. MUDD, AND P.R. MILLER.  1977.  Effects on
19
              plants and microorganisms.  In:  "Ozone and Other Photo-
20
              chemical Oxidants."  pp.  437-585.  National Acad. Sci.,
21
              Washington, D.C.
22
      7.  HILL, A.C., M.R. PACK, M. TRESHOW, R.V. DOWNS, and L.G. TRANSTRUM.
23
              1961.  Plant injury induced by ozone.  Phytopathology   51:
24
              356-363.
23

-------
                                  16
  1    8.  LACASSE, N.L.  1971.  Assessment of air pollution damage  to

  2           vegetation in Pennsylvania.   Center Air Environ.  Studies.

  3           Pa. State Univ. CAES Pub.  No. 209-71.   61  p.

  4    9.  LACASSE, N.L., AND T.C. WEIDENSAUL.   1971.  A cooperative

  5           extension-based system of  assessing air pollution damage

  5           to vegetation:   organization, results,  and recommendations

  •j           for future surveys.   "Proc.  Second International  Clean

  g           Air Congress"  (H.M. England and  W.T. Berry,  eds.) Acad-

  o           emic Press, N.Y. pp. 132-136.

 ,Q   10.  MILLECAN,  A.A.  1971.   A survey and  assessment of air pollu-

 ..            tion damage to  California  vegetation in  1970.   California

 ._            Dept. Agric., Sacramento,  California.  48  p.

      11.  NAEGELE, J.A., W.A. FEDER, AND  C.J.  BRANDT.   1972.  Assessment

              of air  pollution damage to vegetation in New  England:  July,
 14
              1971-July,  1972. Final Report, Suburban Experiment Station,

              University of Mass., Amberst, Mass.  Contract No.  68-02-0084.
 16
      12.   PELL,  E.J.  1973.   1972 survey  and assessment  of air pollution

              damage  to  vegetation in New  Jersey.  The State University
 13
              Department  of Plant Biology,  Rutgers, N.J.  Publication No.
 19
              EPA-R5-73-022.   44 p.
 20
      13.   PELL,  E.J., and  E.  BRENNAN.   1975.  Economic impact of air
 21
              pollution on  vegetation in New Jersey and an interpretation
 22
              of  its  annual variability.   Environ. Poll. 8:23-33.
 23
      14.  PHILLIPS,  S.F.,  and V.C. RUNECKLES.  1974.   Field response of
24
              a wheat-pea mixture to ozone and ambient oxidant.   Proc.
23
              Can. Phytopathological Soc. 41:28 (Abstr.).

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                                 17
  1  15.   SECHLER, DALE, and D.R. DAVIS.  1964.  Ozone toxicity in




  2          small grain.  Plant Disease Reptr.  48:919-922.




  3  16.   SHANNON, J.G., and C.L. MULCHI.  1974.  Ozone damage to




  4          wheat varieties to anthesis.  Crop Science  14:335-337.




  5  17.   U.S. Environmental Protection Agecny.  1978.  Air quality




  f          criteria for photochemical oxidants and oxidant precursors.




  -          Volume II.
 3




 9




10




11




12




13




14




15




16




17




IS




19




20




21




22




23




24




25

-------
Table 1.  Shoot weight response of 11 soft red winter wheat cultivars exposed in open-top field .chambers to
          carbon-filtered air (CF) or to nonfiltered air with 0  added for 7-hr/day  (NF + O.J .—
Shoot Dry Wt.—
Cultivar
Name
Ruler
Holly
McNair 4823
Blueboy 11
Funk W-540
McNair 3001
Coker 68-15
Oasis
McNair 1813
Arthur 71
Coker 47-27
C.I. No.
17314
14579
15290
15281
-
-
15291
15929
15289
15282
12563
li/plant
0.83
0.64
0.59
0.72
0.62
0.61
0.60
0.66
0.56
0.64
0.61
LSD (P = 0.05) =
NF -1- 00
J
{•/plant
0.48
0.41
0.39
0.52
0.45
0.46
0.52
0.58
0.49
0.58
0.56
0.13
% loss from
c/
exposure—
42
36
34
28
27
25
13
12
12
9
8
23%
Fresh Weight
% loss from
exposure
30
24
27
20
21
19
11
10
2
7
0
                                                                                                                  co
        —   Plants were exposed for 27 days (11-38 days after planting).  The mean 7-hr/day and 24-hr 0.,
            concentrations in the CF treatment were 0.02 and 0.01 ppm respectively.  The comparative values
            for the NF 4- 0_ treatment were 0.15 and 0.06 ppm, respectively.  At standard temperature and pres-
            sure, 1.0 ppm of 0- = 1960 pg/m .
        b/
            Each  value  is  the  mean  of  15  plants  (3 plants  in  each  of  5  pots).

-------
                                     19
Table 2.  Effect of chronic doses of ozone on foliar injury,  growth,  and
          yield of winter wheat grown in pots or in the ground in open-top
          field chambers.
Treatment
Ozone cone. •
Growth Medium—
7-hr/day mean .
ppm . Pots—
Ground—
Foliar Injury - 5 week mean—
AA
CF
NF-1
NF-2
NF-3


AA
CF
NF-1
NF-2
NF-3


AA
CF
NF-1
NF-2
NF-3


AA
CF
NF-1
NF-2
NF-3


AA
CF
NF-1
NF-2
NF-3

0.06
0.03
0.06
0.10
0.13


0.06
0.03
0.06
0.10
0.13


0.05
0.03
0.06
0.10
0.13


0.06
0.03
0.06
0.10
0.13


0.06
0.03
0.06
0.10
0.13

25 a
22 a
25 a
50 b
64 c
LSD (P=0.05) 10.6
Shoot wt.
13.21 a
: 12.08 b
12.34 ab
11.12
9.96
LSD (P=0.05) 0.95
Head wt.
6.70 ab
6.85 ab
7.08 a
6.18 b
5.33
LSD (P=0.05) 0.75
Seed wt.
33 ab
21 a
26 a
48 be
61 c
15.5
per plant - g
9.83 ab
10.74 a
10.38 a
c 9.18 b
d 7.62 c
1.10
per plant - g
5.59 b
6.52 a
6.32 a
5.65 b
c 4.51 c
0.42
(yield) per plant - s,
4.77 be 4.25 b
5.25 ab
5.34 a
4.72
3.85
LSD (p=0.05) 0.48
100-seed
2.91 b
3.08 a.
3.06 a
3.00 ab
2.62
LSD (P=0.05) 0.10
5.08 a
4.90 a
c 4.28 b
d 3.38 c
0.53
wt. - g —
3.41 b
3.49 ab
3.52 a
3.43 b
c 2.87 c
0.08

-------
                                   20
Table  2  (continued)
 a/
—   Ozone was  added to  the  inlet  duct  of nonfiltered air  (NF) chambers
     for  7-h4/day  (0930  to 1630  hr EDT)  to produce  the 7-hr/day mean
     concentrations  shown.
W
     Data for each growth medium were analyzed separately.  Means followed
     by different  letters are  significantly different according to the
     LSD  (P=0.05)  (Treatment).
£/
     Each value is the mean  of 192 plants (4  cultivars, 2 plants/8 pots,
     3 blocks), except for seed  100-wt.  values.
I/
     Each value  is  the mean of  768  plants (4 cultivars, 4 plants/6 samples,
     2 rows, 4  blocks),  except for seed  100-wt. values.
£/
     Each value is the mean  percentage  chlorosis and necrosis from 576
     estimates  (4  leaves/3 plants, 4 cultivars, 2 blocks, 6 dates).
I/
     Seed 100-wt.  values for plants in pots are the mean of 36 samples
     (3 samples of 4 cultivars from 3 blocks) .  Values for plants in the
     ground are the mean of  48 samples  (3 samples of 4 cultivars from 4
    blocks) .

-------
Table 3.  Effect of chronic doses of ozone on foliar injury and seed yield of four winter wheat cultivars.
Growth
Medium Treatment
Pots AA
CF
NF-1
NF-2
NF-3

Ground AA
CF
NF-1
NF-2
NF-3

Ozone cone. -
7-hr/day mean
ppm
0
0
0
0
0

0
0
0
0
0

.06
.03
.06
.10
.13

.06
.03
.06
.10
.13

Foliar Injury % —
Coker
Blueboy II 47-27
24
19
24
51*
62*
LSI)
33
24
31
41*
59*
LSD
18
16
21
51*
62*
(I1 - 0.05) »
23
16
21
49*
59*
(P = 0.05) -
Holly
29
22
32
46*
68*
12.3
45
26
32
52*
68*
9.2
Oasis
25
20
23
48*
62*

30
20
22
49*
60*

Seed Weight -
Coker
Blueboy II 47-27
4.67
5.12
5.16
4.64*
4.08*
LSD (P
4.79*
5.84
5.74
4.97*
4.02*
LSD (P
5.07
5.14
5.53
4.82*
3.98*
« 0.05) =
4.01*
5.09
4.55*
3.82*
2.91*
- 0.05) =
• ^/plant-
Holly
4.
5.
5.
4.
2.
0.47
4.
4.
4.
4.
3.
0.32
45*
61
32
59*
97*

16*
95
91
43*
30*

Oasis
4.90
5.12
5.34
4.85
4.37*

4.06*
4.45
4.41
3.89*
3.28*

a/
—   Each value is the mean percentage injury  from 120 estimates  (4 youngest leaves on 3 plants/cultivar in 2
    blocks on 5 dates).

—   Each value for potted plants is  the mean  of 48 plants  (2 plants in each of 8 pots in 3 blocks); each value
    for plants in the ground is the  mean of 192 plants  (4  plants  for each of 6 samples in each of 2 rows in
    4 blocks).
Vtf
    = significantly different  from the respective CF values, LSD  =  (P =  0.05) for cultivar x  treatment.

-------
                                  22
                           FIGURE LEGENDS


  1   Figure 1.  Daily 7 (0930 to 1630 hr EDT) and 24-hr mean ozone


  2              concentrations in ambient air 4.8 km south of Raleigh,


  3              N.C.


  *


  5   Figure 2.  Mean ozone concentrations at different hours of the


  g              day in ambient air (AA) , charcoal f iltered-air chambers


  7              (CF) , or in nonf iltered-air chambers with different


  a              concentrations of ozone added (NF-1, NF-2, NF-3)  for


  «              7-hr/day.   Concentrations are the means from 9 April


 ^Q              through 31 May,  1977.



 11

 _9   Figure 3.  Foliar injury on winter wheat at different times  after


                 exposures  began  for plants grown in the ground in ambient


                 air (AA, 0.06 ppm 0_) ,  charcoal f iltered-air chambers
 14                                 J

                 (CF, 0.03  ppm 0,,), or nonfiltered air (NF)  chambers with


                 different  concentrations of ozone added for 7-hr/day
 16

                 [(NF-1,  0.06 ppm),  (NF-2, 0.10 ppm),  (NF-3, 0.13  ppm)].


                 Each point is the mean  injury on 96 leaves (4 cultivars,
 18

                 3  plants,  4 leaves  per  plant,  2 blocks).
 19


 20


21


 22


 23
25

-------
             I       I
                   7  HR (O93O- I63O HR ) MEANS
                  24-  HR  MEANS
.02 -
.Ol
    4VIO
4/2O
 4/3O
DATE - 1977
5/IO
5/2O

-------
    .16
a
a
2
O
    .15 -


    .14


    .13

    .12


    .1 I

    .10
S  -09
h-
2  .08
UJ

y  .o^
O
«->  .06


2  -O5
O
N  .04
O

   .03


   .02

   .01

   .OO
                                                                           AA

                                                                           NF


                                                                           CF
             6OO
                           IOOO         I4OO

                                    HOUR  OF  DAY
I8OO
22OO

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                                                                     .;, 3
u.
4
Ui
   100
    90
    80
    70
tC   6O
Ul
0.
    5O
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2
S   4O
o
u.
Ui
5
    3O
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                I
L
               IO       17     24      3t      38

                 DAYS AFTER EXPOSURES  BEGAN
               45

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