RESEARCH    T R  1  A  N  G  L E    IN  S T  I 'T  U T:E
                      DEVELOPMENT OF ANALYTICAL TECHNIQUES FOR

                 MEASURING AMBIENT ATMOSPHERIC CARCINOGENIC VAPORS



         EPA Contract No. 68-02-1228

         RTI Project No. 31U-885
                           Monthly Technical Progress Report

                                        No. 6

                       Period:  December 1 - December 31, 1975
                          E. D. Pellizzari, Project^JLgader
                               Date:  January 23, 1976^
          Prepared  for  the Environmental Protection Agency, Research Triangle Park,
          North  Carolina  27711
RESEARCH  TRIANGLE  PARK,   NORTH  CAROLINA   27709

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                         TABLE OF CONTENTS





                                                                 !£-£



Introduction and Rationale 	    1




Methods of Procedure 	    2




     Sampling Methods	    2




     Gas-Liquid Chromatography/Mass Spectrcinetry Computer




     Analysis of Ambient Air Samples  	    6




     Artifact Experiments	  .   10




Results and Discussion  	   12




References	31

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INTRODUCTION AND RATIONALE




     On October 3, 1975,  personnel from the Chemistry and Life Sciences




group at RTI attended a meeting held by Dr. A.  P.  Altschuller at ESRL,




Environmental Protection Agency, Research Triangle Park.  In response




to an OAQPS request,  RTI was asked to participate  in assessing the




nitrosamine' problem in the Baltimore, MD area.   The effort consisted of




obtaining and comparing data on any ambient nitrosamines as measured by




gc/ms methods (RTI) and by thermal energy analysis (Thermal Electron




Corp.).  Samples were to be collected primarily in parallel between




these two contractors.  The Research Triangle Institute proceeded to




undertake a sampling program during the week of October 13-17 and during




the period of November 19-25,  1975 in the Baltimore area, specifically




near and on the FMC property.




     During this sampling period,  the Environmental Protection Agency pro-




vided a meterologist to assist the RTI sampling team in obtaining favorable




locations with respect to downwind locations from  the FMC property.




     The primary objectives were to identify unequivocally the presence of




N-nitrosodimethylamine in ambient air and estimate the levels in this area.

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METHODS OF PROCEDURE


Sampling Methods


     The sampling procedure employed for this study has been previously


described (1,2) which consisted of concentrating nitrosamines and other


organic vapors on a 1.5 x 6.0 cm bed of Tenax GC (35/60) in a glass


cartridge.  All sampling cartridges were preconditioned by heating to


275°C for a period of 20 min under a helium purge of 20-30 ml/min.


After cooling in precleaned Corex centrifuge tubes, the containers were


sealed to prevent contamination of the cartridge.  Sampling cartridges
                                                      I
prepared in this .manner were carried by automobile or air freight to


the sampling site; 2-3 cartridges were designated as blanks to determine


whether any of the cartridges might have been contaminated by the pack-

                                                      I/
ing and transportation procedure.  Cartridges containing known quantities
                                                          /

(100 and 300 ng) of N-nitrosodimethylamine (DMN) were prepared and carried


to and from the field, stored and the percent recoveries were determined.


     Ambient air samples were collected with Nutech Model 221-A AC/DC


portable samplers (2).  In general, a sampling rate of 1 £/min/cartridge


was used throughout this study.


     The sampling locations are shown in Figures 1 and 2 and the sampling


protocol used in this study is given in Table 1.


     Breakthrough volumes for DMN were determined as previously described


(2).  This consisted of injecting DMN vapor onto a gas chromatographic


column packed with the sorbent Tenax GC and determining the elution volume


at a series of decreasing temperatures.  By plotting the log of the elu-


tion volume vs temperature, and extrapolating to ambient temperatures,


(50-90°F) the breakthrough volumes for DMN were determined.  These values

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Figure l.         EAST BROOKLYN,
              BALTIMORE, MARYLAND
        CHESSIE
     COAL PIERS
                            CURTIS BAY
                                 SCALE: ONE INCH =0.5 miles

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                        Figure 2.  Map of  FMC plant.
  1.
;  2.
  3.
  4.
'  6.
  7.
  9.
 10.
 11.
 11A
 12.
 13A
 13B
 13C
 14A
 14 B
                        ^ E"T!-!fP%  "£ -  ••'•(  Ir11^,. A-rr-<-<
                        L^^^Lnr^l?^5^  HnSfe^ /
                                                                                                           =^D  a t
                                                                                                           *-""^"^
                                                           .	5T5.# -Vr=^^//,.3
                                                           I"0  LW  e 'S'«/^7O
                                                           ZwkVL  !'  A  ///_//
                                                                              X= INCINERATOR STACK
                                                                              SS= SAMPLING SITE
Power House
Stack
Dcpon Bldg.
Refined Chemicals Bldg.
Ethion & Butoxide Bldg.
P2S8 Conveyor & Storage Bldg
Diallyl Phthalate Bldg.
Packaging Bldg.
General Shop & Storeroom
 Maintenance Office Trailer
Fire Pump House
 Warehouse
           Shop
           & Shipping Dept.
Carpenter
Warehouse
Storage
Storage
.14C.  Drum Recovery
    Dapon Manufacturing
    Warehouse
16. Warehouse
18. Lab
19. Main Office Bldg.
20. Gate House
25. Booster Pump House
26. Anhydrous Ammonia
28. Dinazinc Control Rm
29. Lab
30. CO Compressor Shed
31. Production Office
34. Pyrethrum Refining
38. Hydrcgenators
39. Nitroso
40. Purification & Reco
    very
41.
43.
A4.
44.
47.
48.
49.

51.
52.
53.
54.
55.
59.
61.
62.
63.
Valve House
PuT.p House
Storage
Storage
Pump House
Chloroformates
Scdiuir. Condensa-
tions
Sodium Storage
Tedion Bldg.
Lockers
Lockers
Cafeteria
Paint Storage
Maint. & Prod.
Central Eng.
J. F. Wilson
Trailer
69.
70.
71.
72.
73.
74,
75.

76,

77,
73.
79,
30.
31.
Hydrogenation
7-OH Production
Control Lab
Incinerator Area
Elec . Control Rin.
7-OK Warehouse
Effluent Control
Rr.;.
>'otor Control &
Locker Km.
7-OH Shop
Cl2 Control Rm.
Fire Pur.-.p House
Locker Km.
Compressor Bldg.
82.
86.
37.
83.

89.
91.

92.
93.
95.
98.
CT.
TF.
£3.
Locker P.TJ.
Inert Gas Generator
Locker Rn.
Calgon Carbon Treat-
ment Bldg.
Shop
Resin Seai-Works
Plant
Pilot Plant
Elec. Control Ra.
Orvis Pilot Plant
Compressor Eldg.
Cooling Tower
Tank Farm
Sub Station

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                        Table 1.   SAMPLING  PROTOCOL FOR BALTIMORE STUDY
Site Cartridge Replicates
FMCS
FMC
FMC
FMC
FMC
FMC
FMC
PS
PS
CP
CP
1
5
9
13
17
1
5
1
5
1
5
_
-
-
-
-
_
-
	
-
	
-
T

a
i.
6
10
14
IS
2
6
2
6
2
6

- 3 -
- 7 —
- 11
- 15
- 19
- 3 -
— 7 —
- 3 -
- 7 -
- 3 -
- 7 -
-m/e
4
8
- 12
- 16
- 20
4
8
4
8
4
8
74
11
3
7
11
3
11
3
10
2
9
p

Time Period
:00
:00
:00
:00
:00
:00
:00
:00
:00
:56
:10

AM
PM
PM
PM
AM
AM
PM
AM
PM
AM
PM

- 2:50
- 6:50
- 10:50
-2:50
- 6:50
- 2:50
- 6:50
- 1:50
- 5:50
- 1:46
- 6:00

PM
PM
PM
AM
AM
PM
PM
PM
PM
PM
PM

Date
10/14/75
10/14/75
10/14/75
10/14 - 15/75
10/15/75
10/15/75
10/15/75
10/16/75
10/16/75
10/17/75
10/17/75

(Quant.)
GC-MS-COMP (Qual
FMC (W of Dimazine Destructor)
Town of Fairfield
Near Memirac Corp .
FMC (SW of Dimazine Destructor)
ir
II
it
Northbridge and Convery St.
"

1-2
1-2
1 - 2
1~* - 2
1° - 2
1-2
1^-2
1. - 2
1-2









m/e 74 (Quant
•)









•)

2
3
8
11
1
6
6
1
3


:00
:45
:20
:50
:55
:35
:35
:4S
:59


PM
PM
PM
AM
PM
PM
PM
PM
PM


- 4:00
- 5:45

PM
PM
- 10:20 PM
- 1:50
- 3:55
- 8:35
- 8:35
- 3:48
- 5:59

PM
PM
PM
PM
PM
PM


11/19/75
11/20/75
11/20/75
11/24/75
11/24/75
11/24/75
11/24/75
11/25/75
11/25/75

Parking lot
Part of Artifact Experiment

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wer-:  used for quantitative collection of DMN, if present, during field




sampling.  The breakthrough volumes are shown in Table 2.




Gas-L-iquid Chromatography/Mass Spectrometry Computer Analysis of Ambient




Air Samples




     The instrumental system (glc-ms-comp) used for the qualitative and




quantitative analyses of nitrosamines and other ambient air pollutants




and the inlet manifold used for recovering vapors trapped on Tenax GC




cartridge samplers were as described elsewhere (1,2).  The descrbed




vapors were resolved by capillar}7 gas-liquid chromatography and mass




cracking patterns were automatically and continuously obtained through-




out the glc run with a Varian CH-7 gas chromatograph/irsass spectrometer.




The cracking patterns and retention time data were accumulated on a




magnetic tape deck and further processed by an on-line Varian 620i com-




puter.  Computer programs (KOSB) were employed which converted the




acquired spectra into a sequential series of mass spectra and uere cor-




related to peak retention time on a total ion current plot.  Data output




from the 6201 computer was provided in two forms:  (1) a teletype listing




which contained the mass spectrum number, number of peaks in the cracking




pattern, total maximum and minimum m/e peak intensity and standard devia-




tion from calibration m/e and (2) an electrostatic plot of total ion




current plots and/or normalized mass spectral.  Single ion plots (e^.g_.




m/e 74) were obtained as an analog output.




     The operating parameters for the glc-ms-comp system for analysis




of samples collected on glass cartridges from the Baltimore, MD area are




shown in Table 3.  Ambient air samples were analyzed en 55, 80 or 100




meter glass SCOT columns coated with either OV-101, OV-225 or DECS sta-




tionary phase, respectively.  The desorption of ambient air pollutants

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Table 2.   BREAKTHROUGH VOL FOR DMN
?F
50
55
60
65
70
75
80
85
90
95
100
105
110
2.2 g /cartridge
(1.5 x 6.0)
liters
385
332
280
242
204
224
163
156
148
127
107
93
79
2.93 g/cartridge
(1.5 x 8.0)
liters
513
493
373
322
272
244
217
207
197
170
143
123
103

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       Table  3.   OPERATING  PARAMETERS FOR GLC-MS-COMP SYSTEM
  Parameter
 Setting
Inlet-manifold
  desorption chamber
  valve
  capillary trap - minimum
                   maximum
  thermal desorption time       ""
GLC
  OV-101 glass SCOT (100M)
  OV-225 glass (80M)
  DECS glass SCOT (55M)
  carrier (He) flow
MS
  single stage glass jet separator
  ion source vacuum
  filament current
  multiplier
  scan rate, automatic-cyclic
  scan range
 265°-270°
 175°
-195°C
4175°C
~4 min

 30-225°C, 4°C/min
 80-2106C, 4°C/min
 70-205°C, 4°C/min
 1.5 ml/min

 200° C
~2 x 10~  torr
 300 yA
 5.5
 1 sec/decade
 m/e 20 -»• 300

-------
including nitrosamines from the Tenax cartridge samplers x^as achieved




at 265-270°C.  A single stage glass jet separator interfaced the SCOT




capillary columns to the mass spectrometer and was maintained at 200°C.




     Identification of resolved components was achieved by comparing




the mass cracking pattern of the unknown mass spectra to an 8 major peak




index of mass spectra (1,2).  In several cases the identification was




confirmed by comparison with authentic compounds of the mass spectrum




and the elution temperature on two different columns.  Particular note




was made of the relationship of the boiling point of the identified




compound to its elution temperature and to its order of elution of cons-




tituent in homologous series since the OV-101 SCOT capillary column




separates primarily on the basis of boiling point.




     For quantitative analysis, the mass spectrometer was set in the




single ion plotting mode whereby the selected master charge ratio was




recorded on analog output.  Quantitation of K-nitrosodimethylamine (by




monitoring only m/e 74) was conducted on a 55 meter glass SCOT capillary




coated with DECS.




     A standard curve for the response of the mass spectrometer set at




m/e 74 vs the concentration of DMN was prepared by introducing known




quantities of DMN vapor.  Synthetic air-DMN vapor was synthesized and




specified quantities collected on Tenax GC cartridges.  By thermally




desorbing the cartridge and monitoring the m/e 74, responses vs concen-




tration were obtained.  Cartridge samplers containing unknown concentra-




tions of DMN were analyzed by monitoring the m/e 74 ion and obtaining the




quantity/cartridge from the standard curve.  Based on the volume of air




sampled and the breakthrough volume for DMN, the concentration of N-




nitrosodimethylamine was calculated in yg/m  of ambient air.

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                                                                    10
Artifact Experiments



     The possibility of formation of DMN on the Tenax sampling cartridge



was investigated.  Since the Tenax cartridge sampler would concentrate



the dimethylamine if present in ambient air (breakthrough volume approxi-



mately 35 H at 25°C), it is conceivable that in the presence of NO > the



dimethylamine could become nitrosated to form DMN.  Two types of experi-



ments were conducted to either support or refute this possibility.  The



first set of experiments were conducted under laboratory conditions.



Synthetic mixtures of NO, water vapor, and air were prepared at known con-



centrations of 1, 10 and 250 parts-per-billion (in NO) in 7 £ glass bulbs,



Tenax cartridges were loaded with approximately 5 parts-per-million of



dimethylamine and the NO __ air vapor mixture was drax-m through the cart-
                        A


ridge.  Cartridges were subsequently analyzed by single ion monitoring



of the in/e 74.  In another set of experiments, NO (~2 x 10   mole/min,



1 ppm) was introduced into a stream of laboratory air which was pulled



across a permeation tube containing dimethylamine at 1 £/min and into



the Tenax cartridge.  The sampling period was approximately 30 min.  The



dimethylamine permeation tube permeated at a rate of ~9 x 1C   mole/min



(~4.5 ppm).  Thus, the amine to NO ratio was ~45:1.



     Experiments were also conducted during field sampling to demonstrate



whether an enhancement in the collection of N-nitrosodimethylamine could



occur above background when Tenax cartridges were either pre-loaded with



dimethylamine or when field air was drawn across a permeation tube con-



taining dimethylamine and into the Tenax cartridge.  The permeation tube



containing dimethylamine (~2.4 x 10   g/min) was placed in front of the



glass fiber filter on the Tenax cartridge.  Therefore in these experi-



ments, the dimethylamine was introduced prior and after the glass fiber

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                                                                    11
filter.   All experiments were conducted in at least triplicate.  A total



of ~120  £ of ambient air was sampled in all cases.



     Further experiments were conducted to also demonstrate whether sto-



rage of  cartridges which had been exposed to dimethylamine and NO  might
                                                                 J^


gradually produce DMN.   Replicate cartridges were stored at room tempera-



ture and at -15°C for periods of 1,  2 and 3 weeks.

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                                                                   12
RESULTS AND DISCUSSION




     As shown in Figure 1,  the sampling sites selected were (1) on the




Fl-IC property, (2) at the Patapsco Sewage Treatment Plant, and  (3) the




Chessie Coal Piers.   During the ambient air sampling on the F>!C pro-




perty, the samplers were located either in the parking lot area or near




the dimazine thermal destructor as shown in Figure 2.




     The sampling protocol  for the Baltimore study was depicted in




Table 1.  During the week of October 14, the sampling protocol included




the collection of quadruplicate cartridges during each time period.




One cartridge from the series of replicates were committed to gas chroraa-




tography/mass spectrometer  computer for qualitative analyses.  Another




series of cartridges were designated for quantitation.  The remaining




cartridges served either as duplicates for qualitative or quantitative




analysis.  During the period from November 19 to November 25, the samp-




ling protocol was slightly  modified to allow only the collection of




duplicate cartridges as well as inclusion of the field artifact studies




(see Table 1).  For quantitative analysis in all cases the calculation




of the amount of N-nitrosodimethylamine in ambient air was based on the




breakthrough volume and the ambient air temperature at the time of field




sampling.




     Figure 3 depicts the profile of ambient air pollutants in a sample




taken during the day in the FMC parking lot area.  The volume of air col-




lected represents 75 I.  A 100 meter glass SCOT column containing OV-101




stationary phase was used to effect this separation.  The remaining




conditions for glc-ms-comp  analysis is shown in Table 3.  In contrast to




Figure 3, Figure 4 represents a profile of ambient air pollutants in a




sample taken during the subsequent evening at the same location in the

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20
68
                              I    »\"  I
                              l\    tz\\   '420
                            4jyd
         116
                                          TEMPERATURE (°c)
                          164
                                        212
                  12
     15
18
21
                  24
         27
30   33


TIME (min)
36
     39
43
51
                                                                               54
57
60
            Figure 3.  Profile of ambient air pollutants in a sample ts.ken during the day on FtfC parking lot.


                     A 100M glass SCOT column containing OV-101 was used, see Table 3 for GLC/MS/COMP conditions.
                                                                                              u>

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                                  23
20

0~
                                     28  32
         68
                         16
                            20
                                            36
                                            n
                                          54
                                         i
                                                                      50
                                                                    49  33     64  69
                                                    48
                                                 '.2
                                                                {43

                                                                f. ^
                                                                «45
                                                                 US
                                                                              ;i
                                                           %°stt
                                                                            85

                                                                            ••':! v\n
                                                                          \ r-ir   i  w
                                 115
                                           TEMPERATURE.(°c)
                                                         164
                                                         _i_
                                                                   'S5

                                                                                   3-;: 102

                                                                                  '^•';i-!C%.^
                                                                                          10'
                                                                  212
                                                                 	L_
                                                                              IOS
                                                            2:0
                                                                                                      111  112
         12
15     18
                            21
•&	2T
TO	33

 TIME (min)
                                                          3S     39
                                                                            45
                                                                                                    57
                                                                                                                         SO    63
Figure 4.  Profile of ambient air pollutants  in a sample-taken during the night on FMC parking  lot,

            A 100M OV-101  glass SCOT  column was used, see Table 3  for GLC/MS/COMP conditions.

-------
                                                                    15
FMC parking lot.  Of particular interest here is the comparison of the




overall quantity of ambient air pollutants which are significantly




greater during the night sampling period as compared to the day.  This




phenomenon is frequently observed in our other studies where day and




night sampling have been compared in geographical areac such as Los




Angeles, CA, Houston,  TX,  St.  Louis, MO, Denver, CO and the Kanawha




Valley in W. VA.




     Figure 5 depicts  a profile of ambient air pollutants in a sample




taken during the daylight hours near the Patapsco Sewage Treatment Plant.




This sampling location is upwind from the FMC Corporation plant but down-




wind from the Sewage Treatment plant.  The profile depicted in Figures 3




and 4 were taken downwind from the FMC Corporation.




     Many of the pollutants resolved in Figures 3-5 have been identified,




however only a partial listing will be discussed later.




     A profile of ambient air  pollutants in a sample taken during the




daylight hours on the  FMC parking lot which is identical to the samples.




taken as shown in Figure 3, is given in Figure 6.  The chromatographic




separation of constituents was achieved in this case on a semi-polar




stationary phase, OV-225,  coated in a 80M glass SCOT column.  Semi-polar




and polar phases are not well  suited for resolution of non-polar pollu-




tants.  However, the resolution of semi-polar and polar constituents are




significantly better.   Figure.  7 depicts the profile of ambient air pol-




lutants in a sample taken again during the daylight in the FMC parking




lot.  In this case, the chromatographic column consisted of a 55M DECS




glass SCOT column.




     The mass cracking pattern for N-nitrosodimethylamine as reported




in the literature is shown in  Figure 8.  Upon electron impact, the

-------
20
6-
                                               26  30
68
JL
                                    40
                                    11
                                    39,.
                                    • n
                                                                  58
                                                                         74
                                                          44
                                                          43-
                                                         V
                                                                K
                                                                r.
                                                    70
                                                    G3
                                                a   68
                                                •9  67
                                                  63
                                                                          75
                                                                           70
                                                                           77
                                                                            70
                                             U   62\'S   TO   6C
                                          -,fe  S;i*j'&  ,V'
                                         4?f  Jiffli'1'™/^
                                        .giMyuy   ^^".v
                                        JJ1
                                               TEMPERATURE (°c)
                                       116
                                                          164
                                                          212
                                                          i
                                                                                       98
                                                                    73
                                                                    100
                                                                     ICI
                                                                      i02
                                                                                       230
                                                                                              103
                                                                                                    106
12    15    18   21    24    27
                             30   33
                             TIME (min)
                                       36
                                                 42   45
                                                               5!
                                                                    54    57
                                                                              6O
                                                                                  	l
                                                                                   63
         Figure 5.  Profile of ambient air pollutants in a sample  taken during the day near  Patapsco Sewage Plant.

                  A 100M OV-101 glass SCOT column was used, see  Table 3  for GLC/MS/COMP conditions.

-------
lOOp




 90-




 80-
UJ


g  TO
0.
 J
o
_)

-------
UJ
lOOp

 90-


 80-
o:

5   TO

H   60
ui
!r   50
O
z   40h
O

_l   30"

P   20

    10
                 air
                                                                   DMN
           Figure  7.   Profile of ambient air pollutants in a sample taken during  the day on FMC

                       parking lot.   A 55M DEGS glass SCOT column was used,  see  Table 3  for CLC/MS/COMP

                       conditions.
                                                                                                         00

-------
                                                                19
Figure 8.  Mass cracking pattern for N-nitrosodimethylamine
         CH
         CH
           3X         	b
            xK-NO    	
            /
4
                   'N-N=0
                                            m/e 74
                                              -H,  UNO
                                           CH2 = N = CH2
                                              m/e 42

-------
                                                                    20
N-nitroscdimethylamine forms a radical ion with an m/e of 74.  This ion


represents the most intense ion in the mass spectrum.  Furthermore, the


formation of the ion m/e of 42 is observed which represents ~68% of the


base peak.


     Figure 9 depicts the mass spectra of an authentic sample of N-nitroso-


dimethylaniine which was chromatographed on the 100M glass SCOT coated with


OV-225.  Also shown in. Figure 9 is an ambient air sample taken at the FMC


parking lot which represents a mass spectrum from Figure 6.  Comparison


of this mass spectrum with the one for the. authentic N-nitrosodirnethyl-


ainine indicates that the unknown peak in Figure 6 is indeed N-nitro.^o-


dimethylarair.e.  The mass spectra are essentially superimposablc.  The


retention time of the authentic N-nitrosodimethylamine was identical to


that of the unknown peak in Figure 6.                 ^

                                                          /
     Likewise, Figure 10 depicts the mass spectrum of a peak in Figure 7


which subsequently has been identified as K-nitrosodimethylamine.  This


mass spectra was obtained on the 55M glass SCOT DECS column.  Furthermore,


the retention times of the authentic N-nitrosodimethylanine standard was


identical to that of the unknown peak in Figure 7.


     A partial listing of the ambient air pollutants which have been ten-


tatively identified in samples of ambient air taken in the FMC parking lot


is given in Table 4.  As it can be readily seen, many chlorinated hydro-


carbons have been detected.  The compounds which have been marked with an


asterick represents air pollutants which have been identified for the


first time.  The remaining constituents have been observed fequently in


other ambient air samples taken in areas such as Los Angeles, CA, Hous-


ton, TX, St. Louis, MO, Denver, CO and the Kanawha Valley, W VA.  Of


particular interest in this listing are the dimethylvinylchloride.  The

-------
JDMN
IOOMGSCOT  OV225
    70-225 ec
AFMC4
IOOMGSCOT  OV225
   70-225°c
too
90
(PERCENT)
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0 0
£ 6°
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UJ
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CC 2°
10



-
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1


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• M.' . M .

60 70
0
/Li.
n/e 74







i

i iji I i 'Mi
SO SO CO 120 IZO 140
100
J*5. '
 Figure 9.  Mass spectra  of  N-nitrosodimethylamine.  AFKC4  represents mass spectrs. from  Figure 6.

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  100




   90




   80




co  70


LU

t  60
      AFMC5
LU
u
cc
   50








   30




   20



   10
                              m/e 74
                                        60MGSCOT DECS
                             I .P.. I.;.. I,
Illijilll 111111111 Hil IIII Illllllii lllli.il!
II II
10 20 30 40
D 5
m
'"T"|""i""|""l""|""!""|""!""
GO 70 80 90
0 l(
/o . , 	 It*

X!

!

0

1
!
£> \:
"T
50 1^

K)

i;
1 |
ISO 170
30
  Figure 10.  Mass  spectrum of N--nitrcsodimethylamine, see  Figure 7


               for chromatographic profile.

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                                                                     23
         Table 4.   PARTIAL LISTING OF AMBIENT AIR POLLUTANTS
                  TENTATIVELY IDENTIFIED IN SAMPLES
                        FROM FMC PARKING LOT
         Compound                            Chromatographic Peak No.a
*methylene chloride                                     2
*chloroform                                             5
 l-chloro-2-methylpropene                               6
 3-chloro-2-methylpropene                               7
*l,l,l-trichloroethane                                  9
*carbon tetrachloride                                  11
 methylene dibromide                                   15
*trichloroethyler.e                                     15B
 l-chloro-2-brorr.opropane                               19
 2,3-dichlorobutane                                    21
 chlorobutens isomer                                   2,2
*tetrachloroethylene                                   27
 dichlorobutene isomer                                 28
 2-chloro-l,3-butadiene                                29
*chlorobenzene                                         30
 dibromochlorofluoromethane                            33
 1,1-dichloropropene + trichlorobutane                 40
*in-dichlorobenzene                                     46
*^-dichlorobenzene                                     52
 a
  See Fig. 3 for corresponding profile.
  These pollutants have been also found in many other  areas  of  the  country,

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                                                                    24
unequivocal identification of many of these compounds awaits the com-




parison of the mass spectra and the retention time of authentic com-




pounds to those listed in Table 4.




     The standard curve for N-nitrosocliinethylamine generated on the gas




chromatograph/mass spectrometer during single ion monitoring of m/e Ik




is given in Figure 11.  Because of the concentrations anticipated as a




result of the qualitative analysis, the standard curve was constructed




from 10-3,000 ng.  This would represent the linear concentration range




which is present on a cartridge sampler.  The detection limit observed




for the m/e 74 ion is ~.5 parts-per-trillion when the ambient air




temperature during field sampling is 85°F.  Thus, the minimum amount




which can be quantitated is 5 parts-per-trillion.




     Single ion plots for N-nitrosodimethylamine of replicate cartridges




are shown in Figure 12 and 13.  It is evident from these two figures that




the replicate cartridge sampling technique is highly reproducible.  All




single ion monitoring for quantitative analysis was conducted on the




55M glass SCOT capillary coated with DECS.




     Using the described procedures for quantiting N-nitrosodircethylamine,




the concentration of the nitrosodimethylamine in ambient air was deter-




mined in the immediate area of the FMC plant in Baltimore, MD.  Table 5




depicts these results.  During the week of October 14, the highest values




observed were ~13.4 ug/m  in the late afternoon.  Only trace quantities




were observed upwind from the FMC plant at the Patapsco Sewage Treatment




Plant.  Significant quantities were also measured at ~l/2 mile downwind




from the FMC Corporation at the Chessie Coal Piers.

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                                                                                25
3OOr-
200-
                                     20O      400   600 600 IOOO
                                     "9
                                                                2000  3OOO
       Figure 11.   Standard cruve  for N-nitrosodimethylamine

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  10.0
  9.0
   ao
   7.0
o
cc
LJ
   5.0
   4.0
   3.0
   2.C
                                                                                 xl
         x3
                                                                                           2S min
       Figure 12.   Single ion plot  (m/e  74) for N-nitrosodimethylamine,  see Table 3  for GLC/MS/CCMP
                    conditions.

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   IQOr


   9.0-


   ao-


   7.0
CO
cc
UJ
p  5.0
<

a;
2  4.0
   3.C
   2.0
    1.0
                                                                                    xl
          x3
                                                                                           26m in.
         Figure 13.  Single ion  plot (m/e 74) for N-nitrosodimethylamine  (replicate cartridge of Fig. 12),

                      see Table 3 for GLC/MS/COMP conditions.
Kl
—I

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Table 5.  SAMPLING CONDITIONS AND CONCENTRATION OF N-NITROSODIMETHYLAMINE IN AMBIENT AIR
Wind Molecular
Date
10/14




10/15

10/15


10/16

10/17
Time
(EOT)
11-2
3-6:

7-10

11-2
3-6:
11-2
3-6:

10-1
2-5:
:50
50

:50

:50
50
:50
50

:50
50
9:56-1:
2:10-6:
PM
PM

PM

AM
AM
PM
PM

PM
PM
46 PM
00 PM
Temperature RH
Location (°F) (%)
FMC (P.
FMC (P.

FMC (P.

FMC (P.
FMC (P.
FMC (P.
FMC (P.

Sewage
Sewage
Chessie
Chessie
Lot)
Lot)

Lot)

Lot)
Lot)
Lot)
Lot)

Plant
Plant
Pier
Pier
83
85

74

65
61
85
83

72
72
55
55
40-50
45-50

65-85

90-97
97
40-50
40-50

45-57
45-50
88-94
94-100
Direc-
tion
WNW
WNW

WSW

Calm .
S
WSW
WSW

NNW
NNW
ENE
E
Speed
(KTS) DECS
10 x
7 x

7 x

_

8-10 x
5-8 x

9-11
5-12
7-9 x
10-14 x
Verification DMN Concentration
OV-225 (ng/m3)
2,133
10,500 ± 1,
(±11%)


167

x 1,375 ± 125
(±9%)
416
571
3,200




x 13,437 i 937
(±7%)
trace
trace
909'
x 84





                                                                                                      NJ
                                                                                                      00

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          Table 6.  SAMPLING CONDITIONS AND CONCENTRATIONS OF N-NITROSODIMETHYLAMT.NE
Date
                Time
Wind/Temperature
Location
JJg/m"
11/19/75    2:00 PM-4:00 PM
11/20/75    3:45 PM-5:45 PM
11/20/75    8:20 PM-10:20 PM
11/24/75

11/24/75

11/24/75

11/25/75
            11:50 PM-1:50 PM

            1:55 PM-3:55 PM

            6:35 PM-8:35 PM

            1:48 PM-3:48 PM
                                   E-SE
                                 6KN-SW,
                                 3KN-SE, 63°
                                 6KN-S, 57'
                    West-Northwest of dimazine
                    thermal destructor on FMC
                    property.

                    Town of Fairfield, 200 yd
                    from residential area,
                    Conoco parking lot.

                    Memirac Corp., north of FMC
                    plant.

                    FMC lot, SV7 of dimazine plant
                    Northbridge & Cannery St,
                    downwind of FMC
                         3"2 ± 1.5



                         1.95 -



                         1.36 ± 0.51


                         20 ± 4

                         14 i 0.2

                         26-'± 0.5

                         7.6
                                                                                                         to

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                                                                    30
     Approximately one month later during the period of November 19-25,




additional values for N-nitrosodimethylamine were obtained.  Again on




the FMC property, high values of this nitrosamine were detected.  How-




ever, the sampling locations were much closer to the general area of




the dimazine thermal destructor.  The concentrations ranged from 14-32




Ug/m •




     Experiments on artifact formation,  i^.e^. production of DMN on the




cartridge sampler during field sampling could not be detected when the




air stream was deliberately spiked with dinethylamine from a permeation




tube.  Laboratory experiments indicated that 10 or more ppm of NO/NO,,




spiked  into an air stream containing DMA can produce DMN; 1 ppm or less




yielded undetectable quantities.  We found it necessary to purify our




DMA by  subambient vacuum distillation prior to any field experiments




since it contained 1 part in 10  DMN.

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