CD A
Cl f\
U. S. Environmental Protection Agency Industrial Environmental Research
Office of Research and Development  Laboratory
                Research Triangle Park, North Carolina 27711
                            EPA~600/7~78~008
                                  4O7Q
                            JSnUarV 151/0
DEVELOPMENT AND LABORATORY
EVALUATION OF A FIVE-STAGE
CYCLONE SYSTEM
Interagency
Energy-Environment
Research and Development
Program Report

-------
                  RESEARCH REPORTING SERIES


Research reports of the Office of Research and Development, U.S. Environmental
Protection Agency, have been grouped into nine series. These nine broad cate-
gories were established to facilitate further development and application of en-
vironmental technology. Elimination of traditional  grouping  was consciously
planned to foster technology transfer and a maximum interface in related fields.
The nine series are:

    1. Environmental Health Effects Research

    2. Environmental Protection Technology

    3. Ecological Research

    4. Environmental Monitoring

    5. Socioeconomic Environmental Studies

    6. Scientific and Technical Assessment Reports (STAR)

    7. Interagency Energy-Environment Research and Development

    8. "Special" Reports

    9. Miscellaneous Reports

This report has been assigned to the INTERAGENCY ENERGY-ENVIRONMENT
RESEARCH AND DEVELOPMENT series. Reports in this series result from the
effort funded  under the 17-agency Federal Energy/Environment Research  and
Development Program. These studies relate to EPA's mission to protect the public
health and welfare from adverse effects of pollutants associated with energy sys-
tems. The goal of the Program is to assure the rapid development of domestic
energy supplies in an environmentally-compatible manner by providing the nec-
essary environmental data and control technology. Investigations include analy-
ses of the transport of energy-related pollutants and their health and ecological
effects;  assessments of, and development of,  control technologies for energy
systems; and integrated assessments of a wide range of energy-related environ-
mental issues.
                        EPA REVIEW NOTICE
This report has been reviewed by the participating Federal Agencies, and approved
for  publication. Approval does not signify that the contents necessarily reflect
the  views and policies of the Government, nor does mention of trade names or
commercial products  constitute endorsement or recommendation  for use.

This document is available to the public through the National Technical Informa-
tion Service, Springfield, Virginia 22161.

-------
                                        EPA-600/7-78-008
                                             January 1978
DEVELOPMENT AND LABORATORY
   EVALUATION OF A FIVE-STAGE
            CYCLONE  SYSTEM
                         by

                Wallace B. Smith and Rufus Ray Wilson, Jr.

                   Southern Research Institute
                    2000 Ninth Avenue, South
                   Birmingham, Alabama 35205
                 Contract No. 68-02-2131, T.D. 10602
                   Program Element No. EHE624
                 EPA Project Officer: D. Bruce Harris

               Industrial Environmental Research Laboratory
                Office of Energy, Minerals, and Industry
                 Research Triangle Park, N.C. 27711
                       Prepared for

               U.S. ENVIRONMENTAL PROTECTION AGENCY
                 Office of Research and Development
                    Washington, D.C. 20460

-------
                            ABSTRACT
     This report describes the development and calibration of
a Five-Stage Cyclone System designed and fabricated by Southern
Research Institute under EPA Contract Number 68-02-2131.  The
cyclone system was calibrated using a vibrating orifice aerosol
generator to generate monodisperse particles of dye of large
diameter for use at ambient and higher temperatures, and a pres-
surized Collison nebulizer to disperse monodisperse latex par-
ticles of small diameter for use at ambient temperature.  Re-
sults from calibrating the cyclones at several conditions of
flow, temperature, and particle density suggest that the D50
cut points are proportional to the flow rate of the gas raised
to a negative exponent which is between -0.63 and -1.11, lin-
early proportional to the viscosity of the gas, and proportional
to the reciprocal of the square root of the particle density.
At 25°C  (77°F), 28.3 £/min  (1.0 ft3/min) and for a particle
density of 1.0 gm/cm3, the D50 cut points of the cyclone
system were 5.4 ym, 2.1 ym, 1.4 ym, 0.65 ym, and 0.32 ym
for Cyclones I-V, respectively.
                                 11

-------
                        TABLE OF CONTENTS
                                                           Page
Abstract                                                     ii
List of Figures                                               iv
List of Tables                                                vi
Acknowledgment                                              vii

SECTIONS
      I     -  Introduction.	  1
      II    -  Background. .	  3
      III  -  Technical Discussion	 11
             A.   Cyclone  Design.	 11
             B.   Experimental Procedures	 11
      IV    -  Experimental  Results	 19
      V     -  Summary	 35
References	 40
APPENDIX - Shop Drawings  For The EPA-S.R.I. Cyclone System. 42
                               ill

-------
                        LIST OF FIGURES
 1.  Comparison of cascade  impactor stage with cyclone collection
     efficiency curve.

     Cyclone:  S.R.I.-l Cyclone
               28.3 Jl/min,  22°C, 752 mm Hg
               After Smith, et. al.7

     Impactor:  Modified Brink BMS-11 Cascade Impactor
                Greased Collection Plate, Stage 4
                Corrected for wall losses
                0.85 Jl/min, 22°C, 749 mm Hg
                After Gushing, et. al.8                       5

 2.  Collection Efficiency-Particle Density Relationship
     SASS Middle Cyclone
     Ammonium Fluorescein Particle Density = 1.35 gm/cm3
     Turguoise Dye Particle Density = 2.04 gm/cm3
     From Gushing, et. al.9                                   6

 3.  Dso-Viscosity Relationship
     SASS Middle Cyclone
     Ammonium Fluorescein
     Particle Density = 1.35 gm/cm3
     From Gushing, et. al.9                                   7

 4.  Dependence of particle cut size on flow rate for  four  cyclones.
     After Chan and Lippmann.6                                9

 5.  Dependence of particle cut size on flow rate for  a 10  mm
     nylon cyclone.  After Blachman and Lippmann.10           10

 6.  Environmental Protection Agency-Southern Research Institute
     Five-Stage Cyclone.                                     12

 7.  Hypothetical flow through a cyclone of conventional design.
                                                             13
 8.  Hypothetical flow through a cyclone of modified design
     (Cyclone I) .                                            14

 9.  Vibrating orifice aerosol generating system.            15

10.  Calibration system for heated aerosols.                 17.
                                 IV

-------
11

12



13,
14,
15
16
17,
18
19
                    Figures  (Cont'd.

Collison aerosol generator system.
                                                         18
Collection Efficiency of EPA-S.R.I. Cyclone I at a flow
of 28.3 £/min, temperatures of 25, 93, and 204°C, and for
a particle density of 2.04 gm/cm3.                       21

Collection Efficiency of EPA-S.R.I. Cyclones II and III
at a flow of 28.3 £/min, temperatures of 25, 93, and
204°C, and for a particle density of 2.04 gm/cm3.
Solid Symbols:  Derived from data taken at a particle
density of 1.05 gm/cm3.                                  22
Collection Efficiency of EPA-S.R.I. Cyclones I, II, and
at a flowrate of 14.2 &/min, a temperature of 25°C, and
a particle density of 2.04 gm/cm3.
Solid Symbols:  Derived from data taken at a particle
density of 1.35 gm/cm3.

Collection Efficiency of EPA-S.R.I. Cyclones IV and V at
flowrates of 7.1, 14.2, and 28.3 &/min, a temperature of
25°C, and for a particle density of 1.05 gm/cm3.
Solid Symbols:  Derived from data taken at a particle
density of 2.04 gm/cm3.

Deposition of particulate mass in EPA-S.R.I. Cyclones I,
II, and III.
a.  Deposition of mass in
    A.  Cylinder and inlet
    B.  Cone and top of cup
    C.  Cup and outside of exit tube

b.  Deposition of mass in
    A.  Cylinder and inlet
    B.  Cone and top of cup
    C.  Collection cup
    D.  Cap and outside of gas
                                                        III
                                                        for
                                                             24
                                                             25
                               exit tube
                                                             28
Collection Efficiency of EPA-S.R.I. Cyclones I, II, and
the Cyclone I gas exit control cup at a flowrate of 28.3
Jl/min, temperatures of 25, 93, and 204°C, and for a par-
ticle density of 2.04 gm/cm3.                           29

D5o cut point versus viscosity for EPA-S.R.I. Cyclones I,
II, and III at a flowrate of 28.3 £/min, temperatures of
25, 93, and 204°C, and for a particle density of
2.04 gm/cm3.                                            31

DSo cut point versus viscosity for EPA-S.R.I. Cyclones I,
II, and III at a flowrate of 28.3 &/min, temperatures of
25, 93, and 204°C, and for a particle density of 1.00 gm/cm3

-------
                         Figures  (Cont'd.)
                                                               Page
20.   Dso cut point versus flowrate  for  EPA-S.R.I.  Cyclones
     IV and V at flowrates of 7.1,  14.2,  and 28.3  £/min, a tem-
     perature of 25°C, and for a particle density  of 1.05 gm/cm3.
                                                                33

21.   Collection Efficiency of the EPA-S.R.I. Cyclones at a
     flowrate of 28.3 &/min, a temperature  of 25°C, and for
     a particle density of 1.00 gm/cm3.                         37

22.   Collection Efficiency of the EPA-S.R.I. Cyclones at a
     flowrate of 14.2 &/min, a temperature  of 25°C, and for
     a particle density of 1.00 gm/cm3.                         38


                          LIST OF TABLES

1    Laboratory Calibration of EPA-S.R.I. Cyclones,
       Planned Procedure                                          19

2    Deposition Study                                             27

3    Laboratory Calibration of EPA-S. R. I. Cyclones ,
          Cut Points                                             36
                               VI

-------
                         ACKNOWLEDGMENT
     The concept of the cyclone system was formed during dis-
cussions with Bruce Harris of EPA and Kenneth Gushing and J. D,
McCain of Southern Research Institute.  The mechanical design
was done by David Hussey and part of the experimental data
was taken by Don Johnson.
                                vn

-------
                            SECTION 1

                          INTRODUCTION
     The majority of measurements to determine the particle-
size distribution in process streams are made with cascade impac-
tors.  Impactors, however, have several limitations:

        There is not enough mass collected for chemical analysis
        of the particles in each size fraction.

        Frequently there is not enough mass collected on some
        stages to be weighed accurately.

        Particle bounce and reentrainment cause an unpredic-
        table, but significant, error in the stage and backup
        filter catches.*

        When the mass concentration is high, the sampling time
        may be undesirably short.

        Impactors are used with lightweight collection substrates
        which are often unstable in mass when exposed to the
        process stream.2

     A series of cyclones with progressively decreasing cut
points will perform similarly to impactors, but without many
of the associated problems.

     Cyclones, however, also have limitations to their applica-
bility:

        There is no general theory to describe the performance
        of small cyclones under field test conditions.

        Sampling times may be undesirably long at sources where
        the mass concentration is low.

     An experimental study is described in this report that
was undertaken to develop and evaluate a system containing five
cyclones and a backup filter in series.  The cyclones were cali-
brated, using monodisperse aerosols, over a range in temperature,
flow rate, and particle density similar to that expected for
field sampling.  In addition to demonstrating the utility of

-------
cyclones for in-situ particle-size analysis, it is intended that
the experimental data obtained will supplement that already avail
able to serve as the basis for the development of a more accurate
theory of cyclone performance.

     Section 2 contains a brief summary of previous work related
to this study.  Section 3 describes the design and evaluation
of the Environmental Protection Agency-Southern Research Insti-
tute cyclone system.  Section 4 is a summary of the important
experimental results and Section 5 contains shop drawings for
the new system.

-------
                            SECTION 2

                           BACKGROUND
     Several theories have been suggested that attempt to pre-
dict cyclone behavior.  Typically, the theories are based on the
classical equation for centripetal force  (mv2/r) and include
additional terms to describe effects such as viscosity drag
and turbulent flow of the gas in the cyclone.  The final equa-
tion usually gives the cyclone's collection efficiency in terms
of the cyclone's dimensions and various parameters of the test
aerosol.  The dimensions of the cyclone are frequently expressed
as ratios.  For example, the height  (h) of a cyclone, the inlet
diameter  (d. ), and the exit tube diameter (d  ), might be ex-
           JL 11                                " A
pressed as fractions of the diameter of the cyclone body, D;
h/D, d. /D, and d  /D, respectively.  Cyclone performance also
      1 fl         G X
depends upon the particle diameter, the particle density, the
gas flowrate, and the gas viscosity-

     Cyclone behavior may conveniently be expressed in terms
of a "Dso" cut point, which is the diameter of the particle
which is collected with 50 percent efficiency.  The conventional
theory of Lapple gives the cyclone D5o cut point as a square
root function of several parameters:3
where
                             H B  2y
                              c c
                            2irN  p Q
                                                          (D
        D50 is the diameter of particles which will be collec-
               ted with 50 percent efficiency,
         NS is the "effective" number of turns made by the gas
               stream in the cyclone,
          Q is the flowrate of the gas through the cyclone,
         B  is the width of the cyclone inlet,
          \^r
         H  is the height of the cyclone inlet,
          p is the density of the particles,
          y is the gas viscosity.
                                             and
For most conditions of cyclone experimentation, the gas  viscosity
is solely a function of temperature and gas composition,  so
that Lapple' s theory gives the D5 0 cut point  in terms of  easily

-------
measured variables:  gas temperature, cyclone  inlet  dimensions/
gas flowrate, and particle density-  Unfortunately,  because
of the complicated flow patterns in cyclones,  N   is  difficult
to predict.

     Leith and Licht4 proposed a somewhat different, semiempiri-
cal, equation for cyclone DSD'S:
      D5o =
             / 18DBrH
'CnC
             \C(n+l)
                                         (2)
where  C  is a cyclone geometry coefficient dependent on  the
            cyclone's dimension ratios only,
       D  is the diameter of the cyclone body, and
       n  is a parameter that depends on the cyclone diameter  and
            the gas temperature.
     This equation  includes the same  /U/Qp   term  as  did  Lapple's
 equation, but  it  also contains the variable n which  is  dependent
 on  the gas  temperature.  Thus, as the gas  temperature changes,
 the Ds o will not  be a simple square root function  of  the  gas
 viscosity.

     The theories of Lapple, and Leith and Licht provide  a  basis
 for comparison of recent experimental data.   Other cyclone  theo-
 ries are discussed  by Leith and Mehta5 and by Chan and  Lippmann.6

     Previous experimental work by Smith, e_t  al7 on'  small cy~
 clones has  shown  that small cyclones perform  comparably to  im-
 pactors.  Figure  1 compares data from the  study of Smith, e_t
 al,7 with impactor calibration data reported  by Gushing,  et
 al-

     Work reported by Gushing, Felix, and Smith9 on  the cali-
 bration of  the middle cyclone of the EPA Source Assessment  Sam-
pling System (SASS)  included data taken at two particle den-
 sities and  three values of gas viscosities.   The cyclone  is
approximately four inches in diameter and ten inches  in height,
 including the collection cup.  Figure 2 shows collection  effi-
ciency versus particle diameter curves for particle densities
of 1.35 gm/cm3 and 2.04 gm/cm3.  These data support the hypo-
 thesis that a cyclone D50 is inversely proportional to  the
square root of the particle density.  Figure  3 shows  that the
experimental relationship between D50 and gas viscosity (or
 temperature) is not a square root, but a linear relationship.
An earlier  calibration by Gushing e_t al 9   also indicated  the
D5o vs. flowrate relationship is not a square root relationship.

-------
      100
o
z
LU
o
LLI
O
O
                                                Dp/D50
                Figure 1.  Comparison of cascade impactor stage with cyclone collection
                          efficiency curve.
                          Cyclone:   S.R.I.   1 Cyclone
                                     28.3 K/min, 22° C, 752 mm Hg
                                     From Smith, et. al7
                          Impactor:   Modified Brink BMS-11 Cascade Impactor
                                     Greased  Collection Plate, Stage 4
                                     Corrected for wall losses
                                     0.85 1/min, 22° C, 749 mm Hg
                                     From Gushing, et. al.&
                                              5

-------
    100
>
o
o
HI
O
o
     80
     60
     40
     20
                          DENSITY COMPARISON
O  AMMONIUM FLUORESCEIN
   21°C, 154 Wmin
D  TURQUOISE DYE
   21°C, 153C/min
                              I     I    I    I   I   I  I
                                        5  6   7 8  910
                PARTICLE DIAMETER, micrometers
Figure 2. Collection efficiency-particle density relationship
         SASS Middle Cyclone
         Ammonium fluorescein particle density = 1.35 gm/cm^
         Turquoise dye particle density = 2.04 gm/cm^
         From Cashing, et. al.9

-------
                                     177°C
CD

o
                          93°C
 LO
Q
                21°C
      140
180
                                   220
260
                   VISCOSITY, poise x 10'6
         Figure 3. DpjQ-viscosity relationship
                  SASS Middle Cyclone
                  Ammonium  fluorescein
                  Particle density = 1.35 gm/cm^
                  From Gushing, et. al.9

-------
     Chan and Lippmann,6 in their development of an empirical
theory, also observed that the D50 of cyclones does not have
an inverse square root dependence on the sample flowrate.

In fitting an equation of the form, D5o = KQ , to their experi-
mental data, n was found to be between -0.636 and -2.13 for cali
bration data from several cyclones.  Figure 4 is the data of
Chan and Lippmann showing the experimental Dso vs. flowrate
relationship for several cyclones.  Notice that one set of
data has two lines fitted to it>  presumably due to an abrupt
change in the gas flow pattern in the cyclone at higher flow-
rates.  Figure 5 shows additional data from a study by Blachman
and Lippmann that also suggests a discontinuity in the D50 vs.
flowrate relationship.10

     In summary, there does not yet seem to be a theory which
can accurately predict small cyclone Ds o cut points for vary-
ing aerosol flowrates and viscosities.  Nevertheless, conven-
tional theories, semi-empirical theory, and experimental data
agree that the Dso's of small cyclones are inversely propor-
tional to the square root of the particle density.  However,
experimental data indicate that the Dso's of small cyclones
are not inversely proportional to the square root of the flow-
rate nor directly proportional to the square root of the gas
viscosity, as some theories predict.

-------
o
o

E
 in
G
                                                                   AEROTEC 2
                               AEROTEC 3/4
                      10mm NYLON
                                                               UNICO 240
                                 10                  50      100

                                          FLOWRATE, liters/min
500
1000
                 Figure 4. Dependence of particle cut size on flow rate for four cyclones.
                          After Chan and  Lippmann.®

-------
(D
4->
CD
E
o
u

E

a
in
0
           .6   .8
                                  FLOWRATE, liters/min




            Figure 5.  Dependence of particle cut size on  flow rate for a 10 mm*

                     nylon cyclone.  After Blachman and Lippmann. "
                                           10

-------
                            SECTION 3

                      TECHNICAL DISCUSSION

                       A.  Cyclone Design


     Figure 6 shows the EPA-Southern Research Institute cyclone
system.  One prototype system is made of aluminum, with silicone
rubber o-rings, and a second prototype system is made of  titanium,
with metal o-rings.  The system is designed to operate  instack,
at a sample flowrate of 28.3 £/min, and is compact enough to  fit
through a 10 cm diameter port.  The objective was to obtain five
cut points equally spaced on a logarithmic scale within the range
of 0.1-10 urn.  Since there is no theory that is sufficiently  accu-
rate to serve as a basis for small cyclone design, the  individual
cyclones of the system were designed empirically-  The  dimensions
were selected to be identical or related to those of cyclones
that had been previously evaluated in our laboratories.7  Lapple's
equation was used to obtain extrapolated cyclone dimensions
for cutpoints between those observed previously, and some rede-
sign based upon trial and error was required to achieve the
final designs.

     The cyclones are numbered sequentially as I through V,
starting with the largest.  Cyclones II-V are of conventional
design, as shown in Figure 7.  Cyclone I is somewhat different,
with the gas exit tube passing through the collection cup as
shown in Figure 8.

                   B.  Experimental Procedures

     Two aerosol generator systems were used to calibrate the
cyclones.  A vibrating orifice aerosol generator was used to
produce dye particles 1.2-8 ym in diameter.  A Collison nebuli-
zer system was employed to disperse latex .spheres of 0.3-2.0  ym
diameter.

     The vibrating orifice aerosol generator (VOAG) is  shown
in Figure 9.  This system is similar to that developed  by
Berglund and Liu11  and has been described previously by Gushing
et al.6 The two types of dye particles were ammonium fluores-
cein~(density 1.35 gm/cm3) and du Pont Pontamine Fast Turquoise
8GLP dye  (density 2.04 gm/cm3).  The VOAG system was used to
calibrate Cyclones I, II, and III at flowrates of 14.2  and
28.3 £/min  (0.50 and 1.00 ft3/min) and temperatures of  25,
                               11

-------
                                   CYCLONE 1
             CYCLONE 4
CYCLONE 5
                                              CYCLONE 2
                                                                   CYCLONE 3
OUTLET
                                                                  INLET NOZZLE
                                                                            3630-056
         Figure 6. Environmental Protection Agency-Southern Research Institute
                  Five-Stage Cyclone.
                                         12

-------
                                                    GAS EXIT TUBE
                                                          CAP
SAMPLE AIR FLOW
                                                             CYLINDER
                                                     CONE
                                                            •COLLECTION CUP
      Figure,?.  Hypothetical flow through a cyclone of conventional design.
                                  13

-------
SAMPLE AIR FLOW
-CAP

GAS EXIT CONTROL CUP

     CYLINDER
                                                      COLLECTION CUP
                                                      GAS EXIT TUBE
         Figure 8. Hypothetical flow through a cyclone of modified
                 design (Cyclone I).
                                   14

-------
CHAMBER
                                      CHARGE IMEUTRALIZER
y
VSS DRYING
—
VIBRATING
ORIFICE 	








FLOW J
METERS'^— f
|!

h
CONTROL /^-^
VALVES *^

' \ 	
\
\
J_
•— »







n
[ i

M
1 I

	 i \
' /
//
//
!/

i
1
L
v^





H



SIGNAL GENERATOR

^^




^
\/^ 	 MEMBRANE
/\ FILTER

*— SYRINGE
PUMP

ABSOLUTE
.S' FILTER
^ t
/\i DRY AIR
            Figure 9.  Vibrating orifice aerosol generating system.
                                  15

-------
93, and 204°C (77, 200 and 400°P) ;  and Cyclone IV at 7.1 JL/min
(0.25 ft3/min) and 25°C (77°F).   All of the internal surfaces
of the cyclones were washed after sampling, and the mass col-
lected on each surface was determined by absorption spectroscopy.

     The apparatus  used to heat the  turquoise dye aerosol  to
the  desired  temperatures  is  shown  in Figure  10.   A pump was
used to obtain the  desired air flow  through .the  cyclones.   In
general the  cyclones  were calibrated individually with a 47 mm
Gelman Filter holder  connected to  the cyclone gas exit*"tube 8
cm from the  cap.  For tests  in which the  flowrate of  the aerosol
stream from  the VOAG  was  greater than the  desired flowrate through
the  cyclone,  the  bleed valve was opened to allow the  excess air
to escape.   For tests in  which the flowrate  from the  VOAG was
less than  the desired flow through the cyclone,  makeup air was
supplied through  the  absolute filter. The aerosol stream to the
cyclone passed through a  heated  copper tube  and  the temperature
was  measured at the inlet of the cyclone.  The sampling port was
used to collect and examine  heated particles  for correct size,
color, shape,  and general integrity.  The  cyclone to  be tested,
and  a glass  fiber back-up filter,  were kept*heated in an oven at
the'same temperature  as the  aerosol  stream.   The air  exiting the
filter entered a  heat exchanger  which allowed the air to come to
room temperature.  The flowrate  was  measured with a calibrated
orifice  located just  upstream from the pump.   A valving arrange-
ment on  the  pump  was  used to adjust  the air  flow to the desired
rate.

      The second  aerosol  generator, shown  in  Figure 11, was
 a pressurized Collison nebulizer which was used to disperse
 polystyrene  latex  (PSL)  particles,with diameters from 0.312 ym
 to 1.099  ym  and  with a density  of  1.05 gm/cm3 and polyvinyl-
 toluene  particles with diameters of 2.01  ym  with a density of
 1.027  gm/cm3.  A general  description of  the  system was given
 by Calvert,12 and a more  specific description by Gushing, et
 al.9  The  Gollison  system was  used to calibrate Cyclones IV
 and V at three flowrates:  7.1,  14.2, and 28.3 i/min  (0.25,
 0.50,  and  1.00 ft3/min).   Due  to the low  melting point of the
 latex spheres,  cyclones  IV and  V were calibrated at 25°C  (77°F)
 only.
                                16

-------
AEROSOL STREAM
FROM VOAG
                        -ABSOLUTE FILTER
                                                   OVEN
                                                   KEPT AT
                                                   AEROSOL TEMPERATURE
BLEED

     HEATED

   COPPER TUBE

          INSULATION
                          SAMPLING
                          PORT
                                                                          MERCURY    WATER
                                                                          MANOMETER  MANOMETER
                        Figure 10.  Calibration system for heated aerosols.
                                                      17

-------
              PRESSURE GAUGE
                                                                     DIFFUSIONAL DRYER
DEVICE TO BE
CALIBRATED
     AP,
                   o
MASS FLOWMETER


THREE-WAY VALVE
    MASS FLOWMETER I
             CLIMET PARTICLE
             ANALYZER
              AUXILIARY PUMP
                                                       BLEED VALVE
                                1VALVE A
                                  VALVE B
                                    jG-tf	-v  ABSOLUTE
                                    ~V$<	->~ FILTER
                                     VALVE C
                                                               Po210
                                                             MIXING
                                                             CHAMBER
 PRESSURE
'GAUGE
                                                                       DILUTION        _
                                                                      AIR ROTAMETER -^* COLLISON ROTAMETER
                                                                                                        VALVE
                                                         DRYER
                                                                                         VALVE
                    COMPRESSED AIR LINE
                                               REGULATOR "	   ABSOLUTE FILTER
                                                        DRYER
                                              REGULATOR
                                                   O  E3   c=>
                                        ABSOLUTE FILTER
                                    Figure 11.  Collison aerosol generator system.

-------
                           SECTION 4

                      EXPERIMENTAL RESULTS
     Table 1 lists the experimental parameters for the labora-
tory calibration study.  As previously stated, three values
each of flowrate, particle density, and gas temperature were
used to simulate a range of conditions that might be expected
in field use.  The object of the experiments was to accu-
rately determine the D5o cut points of the cyclones by measuring
the collection efficiency of the cyclones for particle diameters
near the Ds o.
                             Table 1

          Laboratory Calibration  of  Five Stage Cyclone System
                        Test Conditions
      Cyclone
                           II
           III
            IV
             V
Flowrate
  5,/min •

   7.1
  14.2
  28.3
  28.3
  28.3
Temperature
 degrees C

    25
    25
    25
    93
   204
T
T
T
T
T
T
T
T
T/A
T/P
 T
 T
T/P
 P
 P
P
P
P
         T is turquoise dye particles
         A is ammonium fluorescein particles
         P is polystyrene latex or polyvinyltoluene particles
     In tests conducted with particles generated by the VOAG,
each point on the collection efficiency graphs represents the
entrance of a very large number  (over 10 ) monodisperse particles
into the cyclone inlet.  Thus, each data point was found to be
reproducible to within one or two percent of the initial value
of the collection efficiency, except for particle diameters very
close to the Dso cut point where the efficiency curve is almost
vertical.
                               19

-------
      The sample flowrate, as measured by the metering orifice,
 was accurate to within 1 k/min.  The temperature of the dye
 aerosol was accurate to within 3°C of the true value.  The den-
 sity of the dye particles was accurate to within 0.05 gm/cm3
 and the reported size is estimated to be within 1% of the true
 size.

      For tests conducted with the Collison system, the aero-
 sol concentration was approximately 10-40 particles/cm3.  One
 minute samples were run alternately through the cyclone and
 the bypass line.  At least five sets of inlet/bypass data were
 averaged to calculate each point shown in the graphs of collec-
 tion efficiency vs. particle diameter.  The flowrate was mea-
 sured by an electronic mass flowmeter that is accurate to within
 ±1 &/min of the true value.  The temperature was stable to with-
 in 1°C.  The density of the latex particles is reported to be
 accurate to three significant digits.  Particle size standard
 deviations were less than 0.0082 micrometers for sizes smaller
 than 2 micrometers in diameter and 0*0135 micrometers for the
 2.020 micrometer diameter particles.13  The average standard
 deviation of the collection efficiency was 5% except for par-
 ticle diameters very close to the Dso cut point.

      The collection efficiency curves for Cyclones I, II,
 and III, calibrated at 28.3 2,/min with turquoise dye par-
 ticles  (particle density 2.04 gm/cm3) at temperatures of 25,
 93, and 204°C  (77, 200, and 400°F), are shown in Figures 12
 and 13.  The steepness of the curves indicate the extent to
 which the cyclones will have ideal behavior at these conditions.
 In Figure 13,  the solid symbols represent collection efficien-
 cies measured  using latex particles and the Collison system
 and are called derived data.  Derived data are values of col-
 lection efficiency and Dso which were measured using particles
__of a different density than that listed on the graph and were
 then transposed to particle diameters of equivalent aerodynamic
 behavior and the same density as those listed, by means of Stokes
 law.  Application of Stokes law yields:


                          /   Pid \ h
                    --  -'   plLl •   Dl
 where D! and D2 are the diameters of particles of densities
       pi and p2, respectively, which have the same aerodynamic
                 behavior, and
       Ci and C2 are the slip correction factors for particles
                 of diameters DI and D2 , respectively.

 Equation (3) must be solved by iteration, to yield D2 and C2
 from an initial value of Di and d.
                                  20

-------
     100
c
u
o
LU
O
H
O
LU
O
O
      80
o     60
      40
      20
                                  O
                          25°C
                                                     1    TT
                                                    93°C
                                                                                              100
204°C
                    2.0     3.0   4.0  5.0 6.0    3.0    4.0  5.0 6.0
                                                                                             80
                                                                                              60
                                                                                             40
                                                                                              20
                                                                            I    I   I  I
                                                                      3.0  4.0 5.0 6.0 7.0
                                    PARTICLE DIAMETER, micrometers
                 Figure 12.   Collection efficiency of EPA-S.R.I. Cyclone I at a flow
                             of 28.3 %/min, temperatures of 25, 93, and 204°C, and
                             for a particle density of 2.04 gm/cm3.
                                             21

-------
                 CYCLONE II
CYCLONE III
      100
c
o
u
^

-------
     As an example, in Figure 13, the collection  efficiency
of Cyclone III was 23% for PSL particles,  1.099 ym  in  dia-
meter and with a density of 1.05 gm/cm3.   Using these  values
in equation  (3), we find an equivalent  diameter for  particles
of density 2.04 gm/cm3.
                       f (1.05) (1.152) ~]
                    =  |_(2.04)(C2)	J
Therefore, in Figure 13, the 23% collection efficiency  for  Cy-
clone III is plotted at  .75 ym.  Similarly, the  99%  collection
efficiency is plotted at 1.4 ym for a particle density  of  2.04
gm/cm3 instead of the actual 2.0 ym diameter for the polyvinyl-
toluene particle density of 1.027 gm/cm3.

     Figure 14 shows the collection efficiency curves for
Cyclones I, II, and III, calibrated at a flowrate of 14.2
S,/min and temperature of 25°C with turquoise dye particles
(particle density 2.04 gm/cm3).  The two derived data points
were obtained using ammonium fluorescein (particle density
1.35 gm/cm3).  Again the steepness of the collection efficiency
curves indicates that the cyclones have nearly ideal col-
lection characteristics  at the reduced flowrate  of 14.2 £,pm.

     In the collection efficiency curves for Cyclone III  in
Figure 14, the transposed data taken using the ammonium
fluorescein dye and the  turquoise dye lie close  to a single
smooth curve as would be expected according to Stokes'  law-


     Figure 15 shows the collection efficiency curves for
Cyclones IV and V for a  temperature of 25°C and  flowrates
of 7.1, 14.2, and 28.3 Jl/min.  The open symbols  indicate
data taken using either  polystyrene latex particles  (density
1.05 gm/cm3) or polyvinyltoluene particles (density  1.027
gm/cm ).  The darkened symbols represent data taken  using
turquoise dye particles  (density 2.04 gm/cm3) and trans-
lated to a density of 1.05 gm/cm3 using Stokes'  law.  The  limita-
tion in the particle sizes available in the range 1.0 ym  to 2.8
ym is quite evident and  the uncertainty in the values of  the  D50
cut point that are in this size range is greater than for  those
cut points that lie outside this size range.


     The data cited above were for each of the cyclones
sampling at the same actual inlet flows.  However, when
operating the cyclones as a series train,  the  inlet  flowrate
to each cyclone will be  slightly different due to the pres-
sure drops across the cyclones preceding it.   In order  to
allow more accurate calculations of the cyclone  D50  cut
points in field operation, the pressure drop was measured
across each cyclone at the same mass flow with the inlet
of the large cyclone operating at ambient pressure and  tem-
perature and at 28.3 2,/min.  The results of this measurement
are listed below:

                                23

-------
        100
         80
 o
 o
 u.
 LL,
 o
 l-
 o
 o
 o
         60
         40
         20
                                            O Cyclone I
                                           A Cyclone 11
                                           D Cyclone III
                                 Solid Symbols — Derived Data
                                                      8    10
                   PARTICLE DIAMETER, micrometers
Figure 14.   Collection efficiency of EPA-S.R.I.  Cyclones I, II, and III
            at a flow rate of 14.2 S./min, a temperature of 25°C, and
            for a particle density of 2.04 gm/cm^.  Solid symbols:
            Derived from data  taken at a particle density of 1.35 gm/cm^
                                24

-------
                                        Cyclone IV
                                                      Cyclone V
                 100
Ln
            c
            O)
            o
           >
           O
           O

           LL

           LL

           LLJ


           2

           O
            o
            UJ
            O
            O
                                         I      I    IJJJI
                  40
                  20
            O28.3 fe/min

            A 14.2 C/min

            D 7.1
                                                     I.I.I
                              O 28.3 Wmin

                              A 14.2 C/min

                              D 7.1
                                                I	[
                       0.6  0.8 1.0
2.0
4.0
6.0  8.0
                                                                                         0.3  0.4
                                                          0.6  0.8  1.0
                                                                   2.0
                                                         PARTICLE DIAMETER ,  micrometers
                                    Figure 75.  Collection efficiency of EPA-S.R.I.  Cyclones IV and V at flow

                                               rates of 7. 1,  14.2, and 28.3 ^/min, a temperature of 25°C, and

                                               for a particle density of  1.05 gm/cm3   So/id symbols:  Derived

                                               from data taken at a particle density of 2.04 gm/cm3

-------
Barometric Pressure = 747 mm Hg
                         Ambient Temperature = 25°C
Cyclone
I
II
III
IV
V
Total
Pressure Drop Across
      Cyclone
     5
    40
    71
   332
   137
,1  mm H20
,6  mm H20
.1  mm H20
,7  mm H20
,2  mm Hg
   170.2 mm Hg
of Total Pressure
      Drop.

       0.22
       1.76
       3.07
      14.37
      80.58
     100.00
                                         Inlet Flow
28.3
28.8
28.9
29.1
30.1
     These pressure drops were measured without a backup  fiber
downstream of Cyclone V-  If a back-up filter  is used,  its
pressure drop should be measured separately and subtracted
from the total pressure drop to yield just the pressure
drop across the cyclones.  Then the above percentages can
be used to determine the flow at the inlet of  each cyclone.

     A study of particulate deposition in a cyclone during
its operation yielded some interesting results.  Deposition
data were taken from tests on three cyclones at two flow-
rates and two particle densities.  The aerosol particles collec-
ted were turquoise dye and ammonium fluorescein.  The par-
ticulate concentrations were low and thus no data were  ob-
tained under conditions where there was a large amount  of
material on the surfaces.  The analysis was performed by
rinsing the various parts of the cyclone separately after
each test and measuring the absorbance of each wash with  a
spectrophotometer.  The data on deposition are listed in
Table 2, with a short explanation, and plotted in a bar graph
format in Figure  16.  In each cyclone, the largest deposition
occurred in tne cone.  The next largest depositions occurred
in the cup.

     For each of  the cyclones, the material collected inside
the exit tube was considered part of the catch of the next
stage.  It was questioned whether a similar procedure should
be used for the gas exit control cup of Cyclone I.  During
the calibration procedure, particulate matter  collected in
the gas exit control cup was measured separately from that
collected in the  rest of the cyclone.  Figure  17 shows  the
results of these  measurements.  Since the cup's collection
efficiency is zero for particles slightly larger than the
D50 of Cyclone II, for data reduction the catch of the  con-
trol cup was considered to be part of the Cyclone II catch,
and not part of the Cyclone I catch.

-------
                             TABLE 2

                        DEPOSITION STUDY


Cyclone I at 14.2 £/min, ambient temperature, 6 urn dye particles

   Collection Efficiency - Cyclone        53.3%

   Deposition - Cylinder and inlet        21.3%
               Cone and top of cup        55.6
      Cup and outside of exit tube        23.1
                  Total in cyclone       100.0%

Cyclone II at 28.3 5,/min,  ambient temperature, 2 ym dye particles

   Collection Efficiency                  93.3%

   Deposition - Cylinder and inlet         2.4%
               Cone and top of cup        51.0
                    Collection cup        46.0
     Top of cyclone and outside of
        gas exit tube                      0.6
                                         100.0%

Cyclone III at 14.2 S,/min, ambient temperature, 2 ym ammonium
                                          fluorescein particles

   Collection Efficiency                  32.5%

   Deposition - Cylinder and inlet         0.0
    Cone and top of collection cup        72.1
                    Collection cup        27.9
    Top of cyclone and outside of
     gas exit tube                         0.0
                                         100.0%
Note:  Inside of gas exit tube was not considered part of
       the cyclone catch.

-------
       60
Q
LU
h-
O
LU
O
CJ
co
CO
O

LL
h-
2
LU
O
IT
LU
0.
o
LU
O
O
CO
CO
<

O
I-
LU
O
LU

<
O
IT
      40
              A
                     B
                  CYCLONE I
              14.2 %Jm\n  6 p.m dye
       60
       40
       20
              ABC

                    CYCLONE II
                28.3 C/min 2 /urn dye
                                           Depositon of mass in
                                           A.   Cylinder and inlet
                                           B.   Cone and  top of cup
                                           C.   Cup and outside of exit tube
                                             Deposition of mass in
                                             A.   Cylinder and inlet
                                             B.   Cone and top of cup
                                             C.   Collection cup
                                             D.   Cap  and outside of gas exit tube
                                                  A
                                                          B
D
                                                         CYCLONE III
                                                   14.2 g/min  2 /jm amm. fl.
     Figure  16.   Deposition of paniculate mass in  EPA-S.R.I. Cyclones I, II, and III.

                                   28

-------
                                      O Cyclone I

                                      A Gas Exit Control Cup

                                      D Cyclone II
      100
                Temperature = 77 F
Temperature = 200° F
>
O
LU

O
2
O
CJ
LU
O
O
Temperature = 400°F
                        3   4  5678910  2     3    4   56789 10   2     3    4  5678910
                                         PARTICLE DIAMETER, micrometers
              Figure 17.   Collection efficiency of EPA-S.R.I.  Cyclones I, II, and the
                          Cyclone I gas exit control cup at a  flow rate of 28.3 9./m/n,
                          temperatures of 25, 93, and 204°C, and for a particle density
                          of 2.04 gm/cm^.
                                                  29

-------
     Figure 18 shows the change in Dso cut point due to the
change in gas viscosity for Cyclones I, II, and III.  Vis-
cosity is dependent only on temperature for our calibration
conditions, and the viscosity values 183, 214, and 259 mi-
cropoise correspond to 25°C, 93°C, and 204°C respectively.
These values of viscosity were calculated from the equation

                               T3/2
                            .068T + 7.8


where  u is the viscosity in micropoise and T is the tempera-
ture in degrees Kelvin.  Equation 4 is a curve fit to data
given.. in the Chemical Rubber Handbook for the viscosity of
air.''14  For each cyclone, a linear regression has been per-
formed on the three data points to give the best straight
line.  Although a search of the literature has not revealed
a theory which suggests a linear dependence of Dso on vis-
cosity, a straight line was suggested by the lack of a con-
sistent trend in curvature of the data and by the linear fit
made on earlier data shown in Figure 3.9  The coefficient of
determination is near to unity for each set of data.  The
curves have been extrapolated to 316°C for each cyclone and
replotted for a particle density of 1.00 gm/cm3 in Figure
19.  This facilitates the determination of the D5 o cut points
at actual test conditions.

     Figure 20 indicates the change in Dso cut point due to
the change in gas flow for Cyclones IV and V.  A power curve
was fitted to both sets of data points to yield the follow-
ing equations:

             For Cyclone IV:  D5 0 = 17.6 Q~°-98       (5)
                              where r2 = 0.981


             For Cyclone V:   Dso = 14.0 Q"1'11       (6)
                              where r2 = 0.974


            and r2 is the coefficient of determination.

     In their April 1977 work as discussed above, Chan and
Lippmann suggested that the relationship between Dso  cut point
and gas flowrate  (Q) was Dso = KQ  where K and n are  experi-
mentally determined constants.6  From our data, the values
of n and K for Cyclones I-V are:
                               30

-------
                     TEMPERATURE, degrees C
             25
               204
316
     CD
     +-•
     CD

     O
     O
     £

     6
     in
    Q
           180
 220           260

VISCOSITY, micropoise
 300
Figure 18,   D§Q cut point versus viscosity for EPA-S.R.I.  Cyclones I, II,
            and III at a flow rate of 28.3 S./m/n,  temperatures of 25, 93,
            and 204°C, and for a particle density of 2.04 gm/cm^
                              31

-------
                      TEMPERATURE, degrees C
                                        204
             316
     E
     o
     i_
     u
     E
     6
     in
     Q
                          220
260
300
                         VISCOSITY, micropoise
Figure  19.  D$Q cut point versus viscosity for EPA-S.R.I. Cyclones I, II
           and III at a flow rate of 28.3 Q./min, temperatures of 25, 93,
           and 204°C, and for a particle density of 1.00 gm/cm^

                                 32

-------
         10
   OJ

   o
   o

   E
  O
  Q,

  D
  O
   O
   in
  Q
         1.0
         0.1
                       Temperature = 25°C
                       Density = 1.05 gm/cm^
                    Cyclone IV
                                          Cyclone V
                                       L 1  1  I
          2.83
5.7
14.2
28.3
                     GAS FLOW (Q)   liters per minute
Figure 20.   D$Q cut point versus flow rate for EPA-S.R.I. Cyclones IV and V
            at flow rates of 7.1, 14.2, and 28.3 Q./min  a temperature of 25°C,
            and for a particle density of 1.05 gm/cm^.
                                       33

-------
Cyclone           I        II        III        iv        V

  n              -.63     -.70       -.84      -.98     -1.11

  K             44.6     22.2       22.7      17.6       14.0
Note that only two data points were available to determine the
constants n and K for Cyclones I, II, and III.  The range in
values for n reported by Chan and Lippmann was -0.636 to -2.13,
the reported magnitudes of K were from 6.17 to 4591, and the
diameters of the cyclones range from 10 to 152 mm.  Also, the
geometries and relative dimensions of the cyclones used by Chan
and Lippmann may not have been identical to each other, or to
the ones used in this study.15
                               34

-------
                            SECTION 5

                             SUMMARY
     The EPA-S.R.I. cyclone system is an inertial particle
sizing device that is designed for in-situ  sampling  of  indus-
trial process streams.  It will fit through a 10 cm  diameter
port and is equipped with nozzles of different diameters
to allow isokinetic sampling at the nominal sample flowrate
of 28.3 2,/min.

     In this study, the individual cyclones of the system
were tested and calibrated in the laboratory under conditions
similar to those frequently encountered in  field tests:  gas
temperatures of 25, 93, and 204°C, flowrates of 7.1,  14.2,
and 28.3 A/min, and particle densities of 1.05, 1.35, and
2.04 gm/cm3.

     The Dso cut points for the cyclone system at various
operating conditions are given in Table 3.  For laboratory
test conditions (25°C, 28.3 &/min, particle density  1.0 gm/cm3)
the cut points are 5.4, 2.1,  1.4, 0.65, and 0.32 ym.  Figures
21 and 22'show some of the calibration curves that were ob-
tained.  Figure 21 has efficiency vs. aerodynamic  (particle
density =1.0 gm/cm3) particle diameter plots at a sampling
rate of 28.3 il/min and Figure 22 shows similar data  where
the flowrate is 14 H/min.  These two figures illustrate that
the small cyclones have "sharp" efficiency  curves and indicate
that the system should function adequately  as a particle siz-
ing device.  At the test conditions for Figure 21, the pres-
sure drop across the cyclone  system was 170 mm Hg.

     Data from this study wherein dif f erent^par tide densities
(p) were used tend to support the D50 vs. p2 relationship sug-
gested by several  theories3.'17'18  On the other hand, the experi
mental results indicated that the cut points were directly
proportional to the gas viscosity which is  in opposition to most
theories. 3 ' **'16 ' 17  Also, it  was found in this study and by Chan
and Lippmann6 that the D50's  of small cyclones are not  inversely
proportional to the square root of the flowrate as some  theories
predict.
                               35

-------
                                                    TABLE 3

                                    LABORATORY CALIBRATION OF THE FIVE-STAGE CYCLONES
                                                 DSQ Cut Points
Cyclone

Particle Density (gm/cm3
OJ
CTN





Flow
d/min
7.1
14.2
28.3
28.3
28.3
Temperature
°C
25
25
25
93
204
2.04   1.00
                     II
2.04   1.00
         III

  2.04   1.35   1.00

Cyclone DSQ cut points
      micrometers
                                           IV
1.05
1.00
                     V
1.05   1.00

5.9
3.8
4.4
6.4

(8.4)
(5.4)
(6.3)
(9.1)

2.4
1.5
2.3
2.9

(3.5)
(2.1)
(3.3)
(4.1)

(1.7) 2.1
.95
1.2
1.9

(2.4)
(1.4)
(1.8)
(2.8)
2.5
1.5
.64


(2.5)
(1.5)
(.65)


1.5
.85
.32


(1.5)
(.87)
(.32)


      cut points enclosed in parentheses are derived from the experimental data using Stoke1s law.

-------
      100
c
o>
o
O
2
UJ
o
LL
U-
LU
0
o
o
CYCLONE
CYCLONE II
CYCLONE III
CYCLONE!V
CYCLONE V
                               PARTICLE DIAMETER, micrometer*
          Figure 21.   Collection efficiency of the EPA-S.R.I. Cyclones at a flow rate
                      of 28.3 C//??//?, a temperature of 25°C, and for a particle
                      density of 1.00 gm/cm^.
                                           37

-------
0)
Q.
o
o
z
o
o
LU
o
o
     100
      80
      60
40
      20
              CYCLONE I
              CYCLONE II
              CYCLONE III
              CYCLONE IV
              CYCLONE V
                  J	1	I	I  I   1  I 1
        0.1
                                   1.0
                                                                             10
                            PARTICLE DIAMETER, micrometers
          Figure 22.   Collection efficiency of the EPA-S.R.I. Cyclones at a flow rate
                     of 14.2 Si/min, a temperature of 25°C, and for a particle
                     density of 1.00 gm/cm^.
                                         38

-------
     Work is continuing in an effort to identify or develop
an adequate theory for the prediction of cyclone performance
   er a ranae of test conditions.
under a range of test conditions
                                39

-------
                           REFERENCES


1.    McCain,  J.  D.,  J.  E.  McCormack,  and D.  B.  Harris.
     Non-Ideal Behavior in Cascade Impactors.  70th Annual
     Meeting, APCA,  Toronto,  Ontario, Canada, 1977.  Paper
     77-35.3.

2.    Felix,  L. G.,  G.  I.  Clinard,  G.  E.  Lacey,  and J. D. McCain.
     Inertial Cascade  Impactor Substrate Media for Flue Gas
     Sampling.  EPA-600/7-77-060,  U.S. Environmental Protection
     Agency,  Research  Triangle Park,  North Carolina, 1977, 89 pp.

3.    Lapple,  C.  E.   Processes Use  Many Collector Types.
     Chemical Engineering, 58:  144-151, 1951.

4.    Leith,  D. and W.  Licht.   The  Collection Efficiency of Cyclone
     Type Particle Collectors-A New Theoretical Approach, A.I.Ch.E.
     Symposium Series, New York, New York, 1971, pp. 196-206.

5.    Leith,  D. and D.  Mehta.   Cyclone Performance and Design.
     Atmospheric Environment, 7:  527-549, 1973.

6.    Chan, T. , and M.  Lippmann.  Particle Collection Efficiencies
     of Air Sampling Cyclones:  An Empirical Theory.  Environ-
     mental Science and Technology, 11(4):  377-382, 1977.

7.    Smith,  W. B., K.  M. Gushing,  G.  E.  Lacey, and J. D. McCain.
     Particulate Sizing Techniques for Control Device Evaluation.
     EPA-650/2-74-102-a, U.S. Environmental Protection Agency,
     Research Triangle Park,  North Carolina, 1975.  132 pp.

8.    Gushing, K. M., G. E. Lacey,  J.  D.  McCain and W. B. Smith.
     Particulate Sizing Techniques for Control Device Evaluation:
     Cascade Impactor  Calibrations.  EPA-600/2-76-280, U.S. En-
     vironmental Protection Agency, Research Triangle Park,
     North Carolina, 1976.  94 pp.

9.    Gushing, K. M., W. Farthing,  L.  G.  Felix, J. D. McCain,  and
     W. B. Smith.  Particulate Sampling and Support, Annual Report
     (November 1976-October 1977).  EPA Contract Number 68-02-"
     2131, U.S.  Environmental Protection Agency, Research Triangle
     Park, NC, 1977.
                               40

-------
                     References  (Cont'd.
10.   Blachman,  M.  and M.  Lippmann.  Performance Characteristics
     of the Multicyclone  Aerosol Sampler.  Amer.  Ind. Hyg. Assoc,
     J. 35:  311,  1974.

11.   Berglund,  R.  N.  and  B. Y. H. Liu.  Generation of Monodis-
     perse Aerosol Standards.  Environmental Science and Tech-
     nology, 7(2):  147-153, 1973.

1.2.   Calvert, S. ,  C.  Lake, and R. Parker.  Cascade Impactor
     Calibration Guidelines.  EPA-600/2-76-118, U.S. Environ-
     mental Protection Agency, Research Triangle Park, North
     Carolina,  1976.

13.   Supplied by Dow Diagnostics, The Dow Chemical Company,
     Indianapolis, Indiana.

14.   Weast, R.  C., ed.  Handbook of Chemistry and Physics,
     49th ed.,   The Chemical Rubber Company, Cleveland, OH,
     1968.

15.   Lippmann,  M.  and T.  Chan.  Calibration of Dual Inlet Cy-
     clones for "Respirable" Mass Sampling.  Amer. Ind. Hyg.
     Assoc. J.  35:  189,  1974.

16.   Muschelknautz, E.  Design of Cyclone Separators in the
     Engineering Practice.  Staub-Reinhalt. Luft, 30(5):  1,
     1970.

17.   Sproull, W. T.  Air  Pollution and Its Control.  Exposition
     Press, New York, 1970.
                                41

-------
                    APPENDIX




SHOP DRAWINGS FOR THE EPA-S.R.I. CYCLONE SYSTEM
                        42

-------
GO
                                                                                                                                          SOUTHERN  RESEARCH  INSTITUTE
                                                                                                                                            BIRMINGHAM, ALABAMA 35105

-------
                                                                       T5T
                             TBT"
                                                                                 t> //P ll'OSf C
*=•
jpllPS^
T^\k-j
                                                                 X. W,
                                                                       FACTIONS  \t 1? [ ^


                                                                       OFCIMAI.S  !j


                                                                       ANGLES   I4
                                                                       	p	j.

                                                                       MMSH     I
                                                                                   SOUTHERN RESEARCH INSTITUTE
                                                                                     BIRMINGHAM, ALABAMA 35205
                                                                       APPflOVED


                                                                       CHECKED
                                                                                  C. yc/otf? -Z~ //J-J
-------
                                                                                                                                                                 man
                                             A
                                                                                                                   f /„
£*•
U1
                                                                                                                             TOLERANCtS UNLESS

                                                                                                                              OTHERWISE NOTED
SOUTHERN  RESEARCH INSTITUTE
   BIRMINGHAM, ALABAMA  35205

-------
                                TBT
                                        Je*.
•rar
                                                                irosr
*-''/"
 3^f J-2>
                                                   SOUTHERN RESEARCH INSTITUTE
                                                     BIRMINGHAM, ALABAMA 35205

-------
                                                      USE
                                                           goj
                                                                    -VST
                                                                                            HATttUl
                                                                               J.ti"
. nJ. ;
                   Cc*j.fflf,<,*  C~f>
                  £>
                 r
SOUTHERN RESEARCH  INSTITUTE
   BIRMINGHAM. ALABAMA 352O5

-------
cx»
                                                                                                                                     m	wssm
                  3  .-0.397,
                                      _QL3.5'£'	[_   .
                                                                                                                                           SOUTHERN  RESEARCH INSTITUTE
                                                                                                                                              BIRMINGHAM, ALABAMA 35205

-------
                                                                                                           iw. iita i HUII mil
                                                                                                                                                  -zw
he*
               — -.'WAJi/^v-
          f/^f Jf     £r«/'-re
 4
 3
 C
 xJ
  G-
          -32
        0. 4 ft "3>icL
        '• $93 " Tie/
         O  s -so '
         o- Jfe
         o.
/J7"
                      o.Jlg" S>,4
                                                                                                                    —- -S
                                                                                                            TOUtflAHCES UNLtSS
                                                                                                             OTHEfiWSt HOT£D
                                                                                                          FRACTIONS  * L  +-L,
                                                                                                                  ~ &— ~^tt
                                                                                            SOUTHERN  RESEARCH INSTITUTE
                                                                                           	BIRMINGHAM. ALABAMA 33203
                                                                                                                                  31,

-------
                O  ///


                c. /9i>


                o 3J3


                c. 23S


                O.S77

                £ ..-?/*

                O 3S#
1 V
	  yp	  _     ts, v /~~>      _    cj  o /
                                                                                                               TBT
                                                                                                                -/- C-

-------
                                                                                                                   ^iiSf^^^L  ft.
                                                                                                                              KJ> /n
                                                     I-
                                                                                       TOoTEHREr^ESNu0NTLEE?
                                                                                    ANGLES

                                                                                    FINISH
                                                                                              1 010


                                                                                              + 1"
                                                                                     CHECKED


                                                                                     DRAWN  ', J
SOUTHIIH             INSTITUTE
   BIRMINGHAM,  ALABAMA  35205
BEP8INT CORP  ?-73

-------
                                                                                         TST
TOT
                                                                                                   .0*5-
TJBT
HAIDUAl
Ln
                                                                                                                            REVISIONS
                                                                                                                                                ZONE  NO
                                                                                                                SOUTHERN  RESEARCH  INSTITUTE
                                                                                                                   BIRMINGHAM, ALABAMA  35205
                                                                                                                        DWG. NO.
                                                                                                                                         -B-J3
     REPtlKT COtP.  7-75

-------
                                 Addendum
ASSY  ITEM   QUANT,
NAME
DESCRIPTION
MATERIAL
B
B
N/A
B
B
B
B
B
1001A
1001B
1001C
1002A
1002B
1002C
&
1003C
1003A
1003B
1
1
1
1
1
1
1
1
1
Collection Cup
Vortex Tube/Out-
let
Inlet Adapter
Collection Cup
Vortex Tube/Out-
let
Inlet Adapter
(402C & 403C
Identical)
Collection Cup
Vortex Tube/Out-
let
Cyclone II,
6A7-4V
Cyclone II,
6A7-4V
Cyclone II,
6A7-4V
Cyclone III,
6A7-4V
Cyclone III,
6A7-4V
Cyclone III,
6A7-4V
Cyclone IV,
6A7-4V
Cyclone IV,
6A7-4V
1.79" O.D. X 1 5/16" L,
Titanium
1.79" O.D. x 1.6" L,
Titanium
1.1" W x 1.1" H x 3/8" L,
Titanium
1.54" O.D. x 1.6" L,
Titanium
1.54" O.D. x 1.4" L,
Titanium
0.8" W x 0.8" H x 3/8" L,
Titanium
1.35" O.D. x 1.6" L,
Titanium
1.35" O.D. x 1.21" L,
Titanium
                                      53

-------

PETI

rnnn
'go/
/?&;
*0?!
£/
-------
                                   All
                                                                                                   TO:
                                                                                                        TIB
                                                                                                                              TUittUi
/
  o.
                                                                                                              SOUTHERN RESEARCH  INSTITUTE
                                                                                                                 BIRMINGHAM, ALABAMA 3520.5
                                                                                                                                     2Z"
                                                                                                         SI Alf  , K
                                                                                                             ^-A
                                                                                                         OAIF /• / , .

-------
                                         JJ)  r-,))*/s
                                                                                     Tssrrm
m.
TUT
                                   4' /fa.3 f-<-
Ul
O>
                                                                                      TOLERANCES UNLESS
                                                                                       OTHERWISE NOTED
                                                                                            y//
            SOUTHERN RESEARCH INSTITUTE
               BIRMINGHAM, ALABAMA  35205
                          - /
                                                                                                                                 -B-

-------
     ircy IUUL
                       BOOTH
WGLEi.

INISH


arPHOvFO


HETKf Ll
                      SOUTHERN  RESEARCH  INSTITUTE
                        BIRMINGHAM, ALABAMA 35205
                                          : - C - ^\

-------
The following is a listing of seals required for a single set of cyclones:
     Cyclone I:
          1 ea.  #1000-1-7, 1.000" O.D. X 0.035" Dia.,  Inconel X-750 Metal-0-Ring;
          2 ea.  #1875-2-7, 1.875" O.D. X 0.062" Dia.,  Inconel X-750 Metal-0-Ring,
             or #E-C-E-001750-5-7-l, 1.750" I.D. X 0.062" Free Height Metal-C-Ring;
     Cyclone II:
          2 ea.  #1625-2-7, 1.625" O.D. X 0.062" Dia.,  Inconel X-750 Metal-0-Ring,
             or #E-C-E-001500-5-7-l, 1.500" I.D. X 0.062" Free Height Metal-C-Ring;
     Cyclone III:
          2 ea.  #1375-2-7, 1.375" O.D. X 0.062" Dia.,  Inconel X-750 Metal-0-Ring,
             or #E-C-E-001250-5-7-l, 1.250" I.D. X 0.062" Free Height Metal-C-Ring;
     Cyclone IV:
          2 ea.  #1188-2-7, 1.188" O.D. X 0.062" Dia.,  Inconel X-750 Metal-0-Ring,
             or #E-C-E-001062-5-7-l, 1.062" I.D. X 0.062" Free Height Metal-C-Ring;
     Cyclone V:
          2 ea.  #1062-2-7, 1.062" O.D. X 0.062" Dia.,  Inconel X-750 Metal-0-Ring,
             or #E-C-E-000938-5-7-l, 0.938" I.D. X 0.062" Free Height Metal-C-Ring;
          1 ea.  #1938-2-7, 1.938" O.D. X 0.062" Dia.,  Inconel X-750 Metal-0-Ring,
             or #E-C-E-001812-5-7-l, 1.812" I.D. X 0.062" Free Height Metal-C-Ring.
Available from:   Advanced Products Co.
                  Defco Park Road
                  North Haven, Connecticut
                                     06473
BIRMINGHAM, ALABAMA 35205
                                            TITLE                           "~	
                                                 Five stage Series Cyclone & Backup
                                            SCALE          j DWG. NO.
                                            DATE 7y/i4/-77  "1     £63 0- l-A-24

-------
                                 TECHNICAL REPORT DATA
                          (Please read Instructions or ll-e rci'trse before completing!
 . REPORT NO.

  EPA-600/7-78-008
                                 3. RECIPIENT'S ACCESSION NO.
4.TITLE ANDSUBTITLE
Development and Laboratory Evaluation of a
   Five-stage Cyclone System
                                 5. REPORT DATE
                                  January 1978
                                 6. PERFORMING ORGANIZATION CODE
7. AUTHOR(S)
 Wallace B.  Smith and Rufus Ray Wilson, Jr,
                                 8. PERFORMING ORGANIZATION REPORT NO.

                                   SORI-EAS-78-44
9. PERFORMING ORGANIZATION NAME AND ADDRESS
Southern Research Institute
2000 Ninth Avenue, South
Birmingham, Alabama  35205
                                 10. PROGRAM ELEMENT NO.
                                  EHE624
                                 11. CONTRACT/GRANT NO.

                                 68-02-2131,  T.D. 10602
 12. SPONSORING AGENCY NAME AND ADDRESS
 EPA, Office of Research and Development
 Industrial Environmental Research Laboratory
 Research Triangle Park, NC 27711
                                 13. TYPE OF REPORT AND PERIOD COVERED
                                 Final; 4/76-6/77	
                                 14. SPONSORING AGENCY CODE
                                   EPA/600/13
 is. SUPPLEMENTARY NOTES IERL-RTP project officer is D.  Bruce Harris,  Mail Drop 62, 919/
 541-2557.
 is. ABSTRACT
               repOrt describes the development and calibration of a five-stage
 cyclone system, designed and fabricated by Southern Research Institute.  The system
 was calibrated using both a vibrating-orifice aerosol generator (to generate mono-
 disperse, large -diameter dye particles for use at ambient and higher temperatures)
 and a pressurized Collison nebulizer (to disperse monodisperse, small-diameter
 latex particles for use at ambient temperature). Results  from calibrating the cyclone;
 at several conditions of flow,  temperature, and particle density suggest that the D(50)
 cut points are proportional to  the gas flow rate raised to a negative exponent which is
 between -0.63 and -1.11, linearly proportional to the gas viscosity, and proportional
 to the reciprocal of  the square root of the particle density.  At 25 C, 28. 3 liters/min,
 and for a particle density of 1.0 g/cc, the D(50) cut points were 5.4, 2.1, 1.4,  0.65,
 and 0.32 micrometers for cyclones I-V, respectively.
17.
                             KEY WORDS AND DOCUMENT ANALYSIS
                DESCRIPTORS
                                           b. IDENTIFIERS/OPEN ENDED TERMS
                                              c. COSATl Field/Group
 Air Pollution
 Cyclone Separators
 Development
 Evaluation
 Aerosols
 Dust
Calibrating
Air Pollution Control
Stationary Sources
Particulate
13B
07A
14 B

07D
11G
 8. DISTRIBUTION STATEMENT

 Unlimited
                     19. SECURITY CLASS (Thn Report)
                     Unclassified
                         21. NO. OF PAGES
                             66
                     20. SECURITY CLASS (This page)
                     Unclassified
                                              22. PRICE
EPA Form 2220-1 (9-73)
                                        59

-------