EPA-AA-EOD-84/1
CATALYST ACTIVITY TEST SEQUENCE (CATS)
             January 1984
                  by
           Donald D.  Danyko
           William W.  VJatson
 U.S. Environmental Protection Agency
      Office of Air and Radiation
       Office  of Mobile Sources
    Engineering Operations Division
        Testing Services  Group
          2565 Plymouth Road
      Ann Arbor, Michigan 48105

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              CATALYST  ACTIVITY TEST  SEQUENCE  (CATS)
Abstract
The primary  objective  of this program  was  to establish vehicle
operating  modes  during  which  a  temperature  rise  across  the
catalytic  converter  could  be measured  and  used for  determining
the catalyst activity.   The  results  of  twenty-five (25) vehicle
tests   are  reported.   Seventeen   (17)   vehicle   tests   were
conducted  using  known  good converters,  six   (6)  using  dead
converters  and two  (2)  using partially-active (lead-poisoned)
converters.  The  test sequence  consisted of  a series  of  five
engine  operating  modes.   In general, with  careful thermocouple
attachment to  the exhaust  pipe  surface at the  inlet and output
of  the   converter,   active   converters  show  a  large  enough
temperature  rise  that  they can  be   distinguished  from  dead
converters.

Introduction

    The  primary  objective  of  this  program  was  to  establish
vehicle  operating modes  during which a temperature  rise across
the   catalytic  converter   could  be   measured and  used  for
determining   the   catalyst   activity.    In   theory,   unburned
hydrocarbons,   carbon  monoxide  and  nitric  oxides  (three-way
converters)  from  the  engine  will  react  in  an  active converter
and  produce heat.   The  procedure  was  intended  to be  quick,
simple  and cheap, and the equipment used,  easy to  install and
durable.   The  potential application of  the  procedure  would be
as  a  secondary or  referee  test  in cases  where  tampering  or
misfueling  had been  established by  other  means.    This report
details  a procedure which has been  developed  emphasizing these
objectives.  Temperature data for seventeen  (17)  vehicles with
good  or active catalysts  and  eight  (8)  vehicles  with  inactive
or  partially-inactive catalysts  is  presented.  The discussion
also   includes  details  on  the  general  applicability of  the
hardware  and instrumentation employed during the course of this
effort.

Background

    We  were  directed by Field Operations and  Support  Division,
the  sponsors of  this  project,  to develop  a non-idle  procedure
for  assessing  catalyst   activity  by  measuring exhaust system
skin  temperatures.   Procedure development was  divided  into two
phases.    Both   phases   included   extensive  collection   of
temperature   data  from   vehicles   being  run on   a  chassis
dynamometer.   During  the  initial  data  collection  period,  the
temperatures on  the  exhaust  system  skin  near  the  inlet  and
outlet of the  converter were  measured  during  exhaust  emissions

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                               -3-
tests.   The  vehicles being  tested  represented  a  sample  of
in-use  cars procured  from  the public.   Attempts  were made  to
gather temperature data from as many  different  vehicle  types  as
possible   (Table   1).   No  attempt   was  made  to  create   a
statistical  or  weighted  sample  of  any  kind.   The  exhaust
emissions  tests being  performed  included the  FTP,  KWFET  and
various other  short  cycle tests  encompassing  several  different
vehicle operating modes.

    Following  analysis  of  the  temperature data from  ten  (10)
vehicles,  a procedure was designed to yield a  temperature  rise
across  the converter  in  as  short a  time as  possible without
operating  the  vehicle in an  unusual manner.   Temperature  data
was   then  gathered   on   vehicles   using  this   test  cycle.
Throughout  this  second   phase  of  testing,   variations of  the
procedure  were  examined  in order  to  resolve  ambiguities  in the
temperature data.

    Vehicle   exhaust  system   configurations   presented   many
challenges   in  attachment   of    the   temperature   measurement
instrumentation.   Hose   clamps   were  used   to  fasten  K-type
thermocouples  to  the exhaust pipe  as close  as  possible  to the
converter  inlet and  outlet.  Special attention  was paid  to the
location   on    the   pipe   (top,    bottom   or   side)   for   each
thermocouple.   Visual estimates  of the heat transfer properties
of the  pipe at the inlet and outlet  to  the  converter  were made
in order  to best yield comparable temperatures.  A strip chart
recorder  was   used  to record  the  temperatures throughout  the
test cycle.

Discussion

    The  CATS   procedure  was  designed  to meet the   following
criteria:

    1.    incorporate  vehicle  operating modes  which create high
          converter loading;

    2.    minimize time to identify an active converter;

    3.    minimize operating stress  on the vehicle;  and

    4.    make  no alterations to vehicle hardware.

    High    converter   loading   results   from  rich   fuel/air
mixtures.   Analysis   of  typical  engine dynamics indicates rich
mixtures  are  likely  during start-up  idle and  high power modes.
Consequently,  the  test segments  of  the  cycle  were designed  so
the vehicle would be  operating at  a rich  fuel/air ratio.

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                               -4-
    Figure 1  (attached)  shows  the test cycle that  was  employed
in . the  second  phase  of  the data   collection  to  achieve  a
temperature rise across  the converter.  All driving is  done  at
FTP  dyno settings  for  each  vehicle.   The  cycle  is  initiated
with  a  30  mph  steady state  to  warm up  the  engine,  exhaust
system  and catalytic converter.   As   the temperature  at  'the
inlet  to the  converter reaches 400CF,  the vehicle is  ready  to
begin  the  actual testing  segment  of  the procedure.  The  first
two modes are  "crowds",  that  is,  accelerations  under  conditions
of   constant   manifold   vacuum.    Crowds  are   a  means   of
automatically  adjusting  engine loading for each  engine/vehicle
combination.   The  7"  crowd will give  a  temperature rise across
the converter  for  most vehicles with  active catalysts.   The  4"
crowds,  in  general,  will supply a  rich  enough  fuel/air mixture
to assure catalyst  activity in vehicles where  the  catalyst  may
be partially  deactivated.   The next mode,  a 10-minute  idle,  is
representative of. another  rich mixture mode of  operation.   Some
vehicles  which  do  not  show  catalyst  activity  during  crowd
conditions  will   demonstrate  activity   during  this   mode.
Finally,  a  misfire  condition  is  initiated   at   2500  rpm  by
removal  of a  spark  plug  wire.   This final  test, by supplying an
unburned charge  to  the converter,  should yield  good evidence of
catalytic activity.

    There  are vast  differences in the  thousands  of  converter
emission calibrations  on the  road today.  A high  percentage of
good  converters  will  likely show  negative  results in  any one of
the  modes.   Fewer  will show  negative results in  two  or  more
modes,   and  so  on.   Although  the entire  procedure  requires
twenty-five (25)  minutes on  the  dyno, most vehicles  with good
converters  will  pass  within   the  first  three   modes.   Only  the
dead  converter vehicles  will have  to  run  through the entire
cycle.   Although  this procedure is not  likely  to identify 100%
of  the  active converters  correctly,  the  passing  criteria  for
each  mode can be  adjusted to  minimize errors  of commission,
omission or both.

    Disadvantages of  the procedure are:

    1.   Temperature   measurements  'are  highly  influenced  by
         thermocouple  placement.

    2.   Many   exhaust   system   configurations  do   not   have
          'equivalent1     inlet    and     outlet    thermocouple
         installation  points.

    3.   Many  exhaust  system configurations make  thermocouple
         installation  difficult.

    4.   Each  unique exhaust/converter system  has  its  own heat
         capacity,   heat   transfer  properties   and    catalyst
         loading design.

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                               -5-
    The  first  three  disadvantages  concern  the  thermocouple
measurement technique  and  will be discussed  later.   The  fourth
addresses  the high  degree of  variation  observed  between  the
individual  temperature traces  of  the data  fleet.   This  item
identifies  some  factors   responsible  for  the  differences  in
temperature traces  from  vehicle to vehicle.   These  factors and
the relatively different exhaust  flow  rates  and temperatures of
each mode  have  been used  in the  refinement  of mode selections,
their order and time length.

Data Analysis

    Figure  2  (attached)  is a  typical  trace  of  exhaust  system
skin  temperature  versus  time.   The outlet  temperature  of the
active converters  is shown higher than the  inlet  for each mode
and the outlet of  the  inactive converters  is shown lower.  This
representation  reflects  the   results  of  the  test   fleet  data
summarized  in Table 1.  For example,  on  the  average,  the good
converters  on the   seventeen  (17)  vehicles  tested  show about
60°F  higher  outlet temperature  at the  end  of  the  7"  crowd
mode.   The range  for  the good  converters   is  from -150°F to
+320°F.  Each mode has a similar high degree of variation.
    Using  the  pass/fail criteria of Figure  1,  all  the good and
both  lead poisoned  converters  .(about  half-active)  passed  and
the  dead  converters   all  failed.   However,  several  of  the
vehicles   were  re-run   due   to   non-equivalent  thermocouple
placement.   Incorrect   thermocouple  installation   caused  the
temperature  rise measured  across the converter to  shift  to the
extent  that  the results  were  contrary to  the  actual converter
condition    (available   FTP   results).     Results    from   the
correctly-placed thermocouple  trace were  included  in the table
and the other  results omitted.

    Examining  Table 1,  we find, the majority  of the seventeen
(17)  good converter  test  vehicles  demonstrating higher  outlet
temperatures  during  the  crowd  modes.   This  is  the clearest
demonstration  of  converter activity considering that both the
inlet  and outlet  temperatures  are rising (Figure 3).  Figures 3
and 4  are temperature traces  taken  from  the same vehicle.  The
difference   is  that  the  converter  beads  were  removed  (no
activity)  for   the  test trace  of  Figure  4.   There   is  a 70°F
crossover  at the end  of the  4" crowds  for the  good  converter
and no  temperature  crossover for the dead one.

    Analysis   of  the   idle  portion  of  these  traces is  more
complicated  than the simple crowd analysis.  Note that there is
a  temperature  crossover  for   the  dead  converter  (Figure  4)
during  the  idle mode.   During the  crowd  modes   (high  power
output)  the converter  interior and shell  are being heated by
the  high temperature  exhaust.   The engine exhaust  temperature
during  the following idle is  much cooler, so both the inlet and

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                               -6-
outlet  skin  temperatures  fall during  this  mode.   The  outlet
skin  temperature  is  partially maintained  during  this time  by
convective heat  transfer  from the  converter  interior  to  the
cooler  idle  exhaust  gas.    Note  also   that   in  both  figures
neither   temperature  has   reached   an   equilibrium   (steady)
condition after  10  minutes.   This behavior is a result  of  (1)
the  heat  capacity  (retained heat  from   crowd  modes),  (2)  the
heat transfer  (heat  loss  of the converter to its surroundings),
and  (3) the amount of  heat  being generated during  the  idle (HC,
CO and NOx loading from the engine).

    Early  in   the  development  of  this   procedure,  equilibrium
idle   temperature   comparisons  were   sought  but   cycle-time
requirements limited  this possibility.   Reviewing  the  idle data
in  Table  1  indicates there  are  distinguishable  temperature
differences in  the  good and  dead  converter groups  in  spite  of
the  complicated  factors at work during  this mode.   Therefore a
100°F  temperature difference at the five-minute idle  point  was
chosen  as  a  pass/fail  criteria.   It  is  important  to  recognize
that   the  temperature  condition   of   the  converter   at  the
beginning of  the idle  period shown  in  Figures 3  and 4  has  an
integral part  in determining  the  five-minute  point  temperature
difference.  That is to say,  each  mode is a preconditioning for
the  following  mode.   The  outlet pipe  temperature  is lower than
the  inlet  for  the dead converter  (Figure 4)  at the  instant the
idle  mode  begins,  and higher  for  the  good  (Figure  3).   At  the
end   of   the   idle   mode   (beginning   misfire)    the   outlet
temperatures  are  very  different  in  the  two  figures.   The
misfire  portion  of  Figure  3  (good  converter)  may look  very
different if the  vehicle  were operated in a manner to bring the
inlet  and  outlet   temperatures  together  before  the  misfire
begins.

     It  is  possible  to  divide this  procedure  into  discrete
segments  for   special  purposes, however  the  existing  analysis
criteria  would no longer  apply,  and  the  diagnostic ability of
any  section  will be  less than the whole.   Further  development
and  analysis   could  also  be  directed  into  any  given mode  to
determine its  single maximum  usefulness.

Hardware Applicability

    Application  of  the temperature measurement hardware  to the
different   exhaust    system   configurations    created    many
complicated installations.

    The equipment used  for  this measurement process was:

         K-Type Thermocouples,  1/16" Diameter  (Calibrated)
         Vacuum Gauge  (Calibrated)
     -    Worm-gear type hose  Clamps
         Temperature  Recorder,  able  to  read from  0-2000°F.
          (Calibrated)

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                               -7-
The primary  problem areas were  shields (attached  to  converter
and  exhaust  pipes),   converter  location  and  exhaust  system
routing.

    Shields protecting  the exhaust pipes  and  converter created
major  complications.   The  imported vehicles  appeared  to  have
the most  occurences of shields, whereas most  domestic vehicles
avoid  the  use of  shields.   For example,  Subaru  vehicles  which
posed  the  worst  case,  have shields  welded  on the entire exhaust
system  except for  the  converter.   The  converter  has  a bolted
shield, where the removal of six bolts  will  expose the surface
areas  necessary   for  proper  temperature  measurement.    In  most
cases  however,   the exhaust  shields  are  bolted  on,   such  as,
Mazda  GLC  and Toyota  Tercel.  Once  the nuts and the shields are
removed,  the  inlet and  outlet  areas  necessary for temperature
measurement are  adequately  exposed.  Problems  that arose during
installation  on  domestic  vehicles  were  also  with  catalyst
shields,  and  shields  on  mechanical components.   Ford Escorts,
for  example,  have  a  two  piece   shield  welded  around  the
catalyst.   However,  adequate  space  is  allowed  to  properly
attach  the  thermocouples  if  care   is  used  during attachment.
Chrysler Omni and Horizon models generally have  a two catalyst
system,  with the  first  catalyst located  six  inches  after the
exhaust manifold along the  fire  wall.  To properly  expose the
catalyst   inlet  pipe,  removal  of   a   shield   above   the  right
transaxle  shaft  is  required.

    Exhaust  system routing  and converte'r  location created the
second   problem   area.    In  most  cases  this   problem  was
non-existent,  but  where  it  did  exist,  major obstacles  were
created.    Some   specific  cases   are  Chrysler   K   cars  and
Omni-Horizon  models,  late   model  Hondas,  all  Subarus,  Ford
Escort-Lynx,  Ford Mustang-Capri, and Ford  Fairmont  models.

    The  Chrysler K cars  and Omni-Horizon   models are  equipped
with a two-catalyst system.   A splash  shield  blocks  the access
and  one of the  converters is located up  and  behind  the engine
against the fire  wall, six  inches below  the exhaust manifold.

    Late  model  Hondas,   although   none  were  tested,   have the
converter  mounted to  the outlet of  the  exhaust manifold.  This
will  create a special  problem,  in  that no inlet  pipe  mounting
area exists.

    All  Subaru  models  have  two  seperate  inlet pipes into the
converter,  with  only  one   outlet  pipe.   And   as   mentioned
earlier,  welded   shields  encompass  the  inlet  and   outlet pipes,
with a two piece  shield bolted  around  the  entire converter.

    Finally,  the aforementioned Ford models have  catalysts with
sharp  angled  inlets and  outlets.   The  Fairmont models  also have
heavy  steel  flanges at the converter inlet and  outlet  areas.

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                               -8-
    During development of the procedure, differences  as  high as
70°F  were  measured  simply  by  locating  the  thermocouples  on
different   sides   of   the  exhaust  pipe.    Therefore   certain
precautions must  be  observed when  attaching  the thermocouples.
During   tightening  of   the   hose  clamp,   the  tip   of.   the
thermocouple  must be  covered  by  the  band.   The  axes  of  the
thermocouple and  the exhaust pipe  must  be  parallel  or the  clamp
will  not  apply adequate  pressure.   The worm gear  on the  clamp
should be  opposite the  thermocouple.   Otherwise,  the metal in
the  worm  gear  creates  ,a  heat  sink,  giving  an  inaccurate
temperature reading.   The thermocouple wires must  be kept  away
from moving parts and  the hot  exhaust system.  All thermocouple
mounting   surfaces  should  be   sanded   to   remove   excessive
corrosion,  allowing  for  good contact and  proper heat transfer.
The  hose clamps  should  be  as  tight  as possible, holding  the
thermocouple  firmly  against  the  pipe.   There should  be  no
exhaust  leaks  near  the thermocouples,  or  there  will  be  an
impact  on  measured   temperatures.    Thermocouples  should  be
mounted as  close  as possible to the converter inlet and  outlet,
the  farther away  from the  converter inlet and  outlet  the  more
heat  that  will  be lost through radiation.  If a bend exists in
the  inlet  and outlet pipes, thermocouples should  be  mounted on
the  outside of  the  bend, allowing  measurement  at the  hottest
point  on  the pipe.   Lastly,   the thermocouples  should be at
least  one  to two  inches  away from  overlapping  pipe  joints,
inlet  and  outlet  connection  flanges,   mounting  brackets  or
hangers,  and   shields.   All of these  are heat  sinks  and  can
radiate  heat  away  from   the thermocouples.   Note  that  in   some
cases  one  to  two  inches  will  not apply because of  interfering
brackets,  etc.   In these special cases, a brief analysis of the
mounting problem  and  engineering  judgement  will  allow  for the
proper thermocouple location.

Conclusion

    Measurement  of  exhaust  system  skin  temperatures,  if   done
carefully,  may indicate  whether  a catalytic  converter  is   good
or bad.   Temperature measurement across the converter indicates
thermal  activity "but  it  does  not  establish whether  it   is  a
result   of  hydrocarbon,  carbon'   monoxide  and  nitric  oxide
conversion  or of any combination  of  those  three conversions.
Assessment  of temperature  data taken  from  the  exhaust system
skin  at  the outlet and inlet of the converter is complicated by
the  variety  of   exhaust  system  configurations  and  the unique
properties  of each converter.   The CATS procedure, by operating
the  vehicle  in  rich  fuel/air  mode, provides  a test  that was
successful  in identifying  active  and  inactive  catalysts.   The
procedure  does 'require a  large  amount  of equipment  including a
chassis   dynamometer.     Extensive  engineering   judgment   was
employed  in  interpretation  of  the  data  generated  during   this
program,  but  with proper  training the use of  the procedure is
clearly  feasible.

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                               -9-
Recommendatlons

    The  procedure  should  be  performed  as  designed,  since  the
differing exhaust  system  configurations  and their corresponding
heat transfer  and  heat capacity characteristics  will  alter  the
temperature data if a  different  sequence is used.  The simplest
and most  effective means of thermocouple attachment is  by hose
clamp.   Strip  charts  should be  used to  record  the temperature
data  to allow  analysis.  A  relatively  small  sample fleet  of
screened tampering/misfueled vehicles  should  be  CATS tested  and
then FTP  tested to determine real-world CATS accuracy prior to
full scale implementation.

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                           TABLE 1.  Converter Activity Test Sequence Fleet Data
VEH
# MANUFACTURER/^DEL
ENGINE
CLASS/TYPE
GOOD
10
14
4
16
5
6
17
1
2
9
CONVERTERS
GM Camaro
GM Cutlass
GM Regal
GM Grand Prix
GM Skylark
GM Citation
GM Citation
Ford Escort
Ford Escort
Chrysler Horizon

^
A106
A110
A110
A69
A69
-
A3
A3
A86
(Two Converters
15
3
7
8
11
12
13
DEAD
10
14
16
17
1
9

LEAD
16
17
Chrysler Champ
Nissan Datsun 210
Toyota Tergel
Honda Accord
Toyota Mazda
Isuzu Subaru'
Isuzu Subaru
CONVERTERS
A109
A73
A125
A83
Alll
A105
A105


v-e
V-8
V-6
V-6
1-4
1-4
1-4
1-4
1-4
1-4
FTP (GM/MI)
HC CO

0.2 3
0.2 3
0.8 8
0.4 7
0.6 14
0.3 3
0.2 4
0.2 3
0.6 9
0.5 8
NOx

0.9
0.8
2.9
0.6
0.5
1.1
0.4
0.3
0.7
1.0
in Series)
1-4
1-4
1-4
1-4
1-4
H-4
H-4

SAME VEHICLES AS ABOVE






POISONED CONVERTERS














SAME VEHICLES AS ABOVE



0.6 6
0.4 8
0.3 5
0.5 7
0.8 10
0.3 6
0.2 3

2.5 24
2.2 22
2.3 18
- -
2.5 31
2.9 42
2.9 42

1.0 7
- -
1.0
1.2
0.5
0.4
0.6
0.7
0.8

3.4
2.1
2.5
-
0.9
1.0
1.0

1.3
-
TEST MODE/TEMPERATURE RISE ACROSS CONVERTER °F
CROWDS
7" 4"

10 -10
50 70*
80* 150
-30 70*
50* 130
-20 20
-150 -110
85* 260
320* 275
80* -220
-65 -110
80* 110
100* 130
120* 180
60* 110
170* 270
-20 -15
30 90*

-115 -145
-100 -45
-80 -65
-190 -135
-50
-340 -300
-100 -45

-30 -30
-80 -80

IDLE
START 5 MIN

-10
70
150
70,
130
-20
-110
130
320
-220
-110
110
190
60
115
440
-15
90

-145
-45
-65
-135
-150
-300
-45

-30
-80

185*
170
170
200
85
80
50
210
85
160
-160
240
270
115
140
430
60
170

-30
15
60
-30
-50
5
55

140*
130*
MISFIRE
END

215
155
160
230
0
0
0
80
20
45
-70
220
280
90
-
480
-20
140

-30
-20
35
-65
-40
-90
45

165
50
START END

150
145
-
200
-
115
0
40
-
0
-60
200
-
-.
-
400
-15
70

-60
-20
20
-55
-
-60
0

95
55

65
175
-
130
-
330*
50*
190
-
-20
-60
330
-
- -
-
540
85*
150

-150
-20
-95
-70
-
-230
-20

-10
70
Refers to 'pass' point according to Figure 1 criteria.

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                               Figure 1
                                                           11
           Converter  Activity Test Sequence (CATS) Flowchart
           'FAIL'
           END OF
            TEST
                             START 30 MPH
                           3 MINUTE WARM-UP
                                             Yes
                                        No
                             RUN 7  CROWDS
                         20/40 MPH - 4 MIN MAX
                                             Yes
                                        No
                             RUN 4" CROWDS
                         20/50 MPH - 4 MIN MAX
                                             Yes
                                        No
                               RUN IDLE
                              10 MINUTES
                                             Yes
                                        No
                               RUN MISFIRE
                          2500 RPM-2 MIN MAX
.*   AT  is  the  temperature  rise  across  the  converter  (outlet-inlet),

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