EPA-AA-TEB 66-1
      THE EFFECTS  OF  WATER INJECTION



                     ON



NITROGEN OXIDES  IN AUTOMOTIVE EXHAUST GAS
                    1966




             PROJECT  B-l-7-2



             (In-House Report.)
             D.  M.  Hollabaugh

-------
                       INTRODUCTION


 Use  of water injection in engines dates back as  far as the

 year 1880.   During World War II,  its  use in aircraft engines

 was  quite extensive.   In all these past situations, its use

 has  been exclusively  to prevent knock.   It had a secondary

 advantage on wartime  aircraft and that  was its cooling effect

 on the cylinder valves and the piston,  which prolonged their

 service life at high  performance  levels.  The present investi-

 gation of its use was undertaken  to confirm its  effect on

 reducing the NOX emissions in automotive exhaust gases.


 In a paper (1)  given  before the 53rd  Annual Meeting of the APCA

 in 1960, the theory was discussed on  the way in  which injection

 can  limit NOX.   Briefly, since NOX formation is  basically a

 function of the peak  combustion temperature and  fuel-air mixture

 ratio (availability of oxygen), any means which  affect either

 of these will have a  corresponding effect on the NOX emissions.

 Reduction of NOX by use of rich fuel  mixtures are not desirable

 since this results in marked increase in hydrocarbons and carbon

 monoxide.  With water, .combustion temperatures are lowered

 by the heat used to vaporize, superheat, and finally dissociate

 the  water, which limits the NOX without significantly affecting

 the  other emissions.
(1)''Exhaust Gas Recirculation as a Method of Nitrogen Oxides
    Control in an Internal Combustion Engine" by R.  D.  Kopa
    and Kiroshi (Univ.  of Calif.), APCA Paper 69-72, May,  1960.

-------
This earlier work showed that at water to fuel ratios, on a
weight basis, approaching unity, an 80 percent decrease in NOX
could be effected with only modest fuel consumption increases
and power losses, usually in the order of 10 to 12 percent.
Part throttle power losses, such as occurs at roadload conditions,
are always recoverable with either a throttle adjustment and/or
an ignition timing adjustment.  In either of these.cases,
however, theoretically, changes will occur in the other compo-
nents of the exhaust gas emissions, as previously shown by other
investigators.  For example, increasing either the fuel mixture
ratio or advancing timing should cause an increase in the hydro- .
carbon concentration, with the latter having the more pronounced
effect.

The objective in this project was to confirm previous findings
for roadload conditions and to test an intermediate load value
somewhat representative of a modest acceleration.  Also, it
was considered advisable to examine the effect of an alcohol-
water mixture, at two different ratios, to observe the effects
on emission, since alcohol would be used in cold months to pre-
vent the water from freezing.

Conclusions
1.  For part throttle operation with the engine tested, water
injection ratios of 0.9'lbs. of water per Ib. of fuel gave
NOX reductions of 75 to 80 percent without appreciable power
losses or effects on hydrocarbon or carbon monoxide emissions.

-------
2.  Air-fuel mixture ratios are essentially constant over the



range of injection ratios investigated.





3.  Exhaust gas temperatures increase with increases in the



injection ratio for part throttle operations and conversely,



under wide open throttle conditions, they decrease.   Although



there is no precise explanation currently available, it does



appear to be an enleanment phenomena for the former.





4.  Power loss1 was a minimum with water-alcohol injection.





5.  As part throttle operation approaches higher loads, the




range of injection ratios that can be used becomes less



due to their effect on power and hydrocarbon emissions.





                      TEST EQUIPMENT





Testing was conducted with a 1963 Chevrolet 283 cubic inch



displacement engine and an Eaton Model 1519 DC dynamometer.



Hydrocarbon emissions, CO, and C02 were monitored with Beckman



NDIR equipment, Model type ISA.  The NOX concentrations were



measured by the modified Saltzman technique; and oxygen by



polarographic means with a Beckman #777 analyzer.





Fuel weight consumed was measured with a Cox weighing system,



Model 402A, and the air used with a Meriam 6" laminar flow element.



Engine ignition timing was determined with a Sun distributor



advance meter, Model 214, and a timing light.

-------
An explanation of the ivater injection equipment can best be



accomplished by referring to the photograph in the appendix



section.  Basically, this is a commercial system sold for detona-



tion control under the trade name "Octa-gane" and is made by



the Engine Accessories Manufacturing Company of Los Angeles,



California.  Water is introduced through a plate sandwiched



between the carburetor and intake manifold.  Through incorporation



of several toggle valves, the system could be made to operate



whenever it was desired, as contrasted to its former use only



at higher power conditions at wide open throttle.  Air was



introduced with the water at the large control valve to help atomize



the water on discharge into the engine.





Test Procedure






Tests were conducted under the following conditions:



    1.  Roadloads equivalent to vehicle speeds from 30 to 70 mph,



    in 10 mph increments.



	2.  Intermediate loads (22" Hg. manifold pressure) for the



    same speed range as in step 1.



    3.  Wide open throttle at 30 and 50 mph.



For each of these operating conditions, the injection ratios tested



ranged from 0.3 to 1.1 Ibs. of water per Ib. of fuel.  Water-



alcohol injection, was tested •only at 5y mph roadload  on two



different mixture ratios  (80/20 and 60/40 percent, respectively).

-------
Changes in engine torque at constant speed settings were compen-



sated for by throttle adjustments.  Initially, spark timing



changes were tried to correct or hold engine performance, but



this was abandoned early because of its more adverse effect on



hydrocarbon emissions.





Results





Graphical results on the effects of water or water-alcohol



injection on emissions and engine performance are shown by the



curves in the appendix section.  In all cases, the greatest



reduction in NOX was obtained at the highest injection ratio



(1.1).  Through 60 mph, the NOX reduction at this ratio averaged



84.5 percent.  Above 60 mph, the gains in NOx reduction became



less because of the limitation on injection ratios that can be



used with effecting power or the other emissions.  At 70 mph,



roadload, the maximum ratio was 0.5.  For wide open throttle



operation, the only ratio which gave an NOX reduction was 0.3



and this was restricted to .30 mph.  At 50 mph, wide open throttle,



no reduction was made in either NOX or hydrocarbon emissions,



in fact both increased by 22 and 32 percent, respectively.





With respect to alcohol-i^ater injection, the 20/80 percent



solution decreased NOX concentration by 80 percent with only a



marginal increase of 4 percent in hydrocarbons.  The 40/60



percent solution reduced NOX by 84 percent but hydrocarbon



concentration increased to 52$.  Throttle adjustments to hold



power with the alcohol mixtures were very slight as contrasted

-------
with straight water injection.  With the latter, increases in



manifold pressure become evident at about a 0.5 injection ratio.



At the maximum ratio, the manifold pressure has usually increased



between 1.5 to 2.0" Hg. above the baseline setting at any test



condition.





Recommendations





That if interest exists, the following be given consideration:





    1.  Test an injection system on the road and/or under cycling



    conditions on the chassis dynamometer for emission eval-




    uation and driveability.



    2.  Evaluate the continuous effects of water injection on



    engine durability.



    3.  Investigate the design and economic aspects of incorpor-



    ating water on a passenger car to help establish its



    feasibility.



    4.  Determine what effect water injection has on specific



    groups of hydrocarbon under similar test conditions.





Discussion



Under throttled or roadload conditions, the effects of water



injection on combustion are evidenced both by changes in manifold



pressure and exhaust emissions.  In regard to the latter, both



NOX and hydrocarbons are reduced by this injection, except



at the highest ratios.  At the higher ratios (0.9 to 1.1)



hydrocarbons begin to increase rapidly indicating a progressive

-------
deterioration in combustion.  The same effect also occurs at



maximum power with any degree of injection.   The increase in



exhaust gas temperatures in the manifold accompanying injection



at roadload conditions appears to be due to a slower burning



rate it imparts, simulating a lean fuel mixture, and causes



late burning in the exhaust manifold.  This lower energy level



of combustion reduces nitrogen fixation but also allows further



oxidation of the unburned hydrocarbons before leaving the engine.





At higher load conditions above roadload, water injection has



quite pronounced adverse effects on engine power and hydrocarbon




emissions.  Usually where water injection is used for maximum



power conditions, such as in racing engines, its use is predicated



on using leaner fuel mixtures than would be possible without



it.  Under these conditions, water serves not only for detonation



control but also to cool the various combustion chamber parts.





The highest injection ratio which did not seriously affect



performance up to 60 mph, roadload (2500 engine rpm), was 0.9.



At this ratio, usually 75 to 80 percent reduction in NOX was



effected.  Above it, hydrocarbon emissions and power loss increase



too rapidly.  In most cases, something approaching 2" Hg.



increase in manifold pressure was required to maintain specified



torque.  With water-alcohol injection, this effect in power all



but vanished and is probably explained by the energy contribution



of the alcohol.  From the results,"it appears that 80/20 percent

-------
solution would be the more desirable of the two water-alcohol



mixtures tested, because it gave approximately the same NOX



reduction but with very little increase in hydrocarbons.  The



80/20 mixture, however, would probably not be sufficient for



anti-freeze protection.





At part throttle operation, the air-fuel ratio remains essen-



tially constant, although slight changes do occur in brake



specific fuel consumption.  However, from an over-all stand-



point, fuel economy should not be too drastically affected



with this control technique, unless the transient response




of the engine has been somehow affected by it.  Since an auto-



matic arrangement of this system for part throttle operation



does not currently exist, it was not possible to test this



condition.

-------
                              10
                   OTHER REFERENCES
1.  "Detonation and Internal Coolants" by E.  F.  Obert,
    Northwestern University, SAE Quarterly Trans.,  Jan-
    uary, 1948, Vol. 2-1.
2.   "Antidetonation Injection" by C.  H.  Van Hartesveldt,
    Thompson Vitameter Corp., SAE Quarterly Trans., April,
    1949, Vol. 3-2.
3.   "Aviation Fuels and Their Effects on Engine Perfor-
    mance" (Manual of general information for U.S.A.F.
    and Navy), by the Ethyl Corp., 1951.

-------