EPA-450/4-84-013
                                                June 1984
An Update On The Use Of Paniculate Ratios
To Assess Likely  PM<|Q  Attainment Status
                            BY
                          A.D Thrall
                            And
                       A.B Hudischewskyj

                      Systems Applications, Inc.
                       San Rafael, CA 94903

                   EPA Project Officer Edwin L Meyer, Jr

                     EPA Contract No 68-02-3848
                   ENVIRONMENTAL PROTECTION AGENCY
                      Office Of Air And Radiation
                  'ce Of Air Quality Planning And Standards
                    Research Triangle Park. IMC 27711

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This report has been reviewed by the Office Of Air Quality Planning And Standards, U.S.
Environmental Protection Agency, and approved for publication as received from the contractor.
Approval does not signify that the contents necessarily reflect the views and policies of the
Agency, neither does mention of trade names or commercial products constitute endorsement
or recommendation for use.
                                  EPA-450/4-84-013

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Technical Memorandum

 AN UPDATE ON THE USE OF  PARTICULATE  RATIOS
  TO ASSESS LIKELY PM 10  ATTAINMENT STATUS

               13 January 1984

            (Revised  4 June 1984)

                SYSAPP-84/100
                Prepared for

    U.S. Environmental Protection Agency
Office of Air Quality Planning and Standards
   Monitoring and  Data  Analysis  Division
      Research Triangle  Park,  NC   27711
         EPA  Contract  No.  68-02-3848
                 Prepared by

                A. D. Thrall
            A. B.  Hudischewskyj

         Systems  Applications, Inc,
            101 Lucas Valley Road
            San Rafael, CA  94903
                    iv

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Table of Contents
                                                                    Page
Introduction 	     1
Differences In Concentration Ratios When Grouped By Time,
  Location, Or Total Concentration 	      1
Pooling National Data To Estimate The Statistical  Distribution
  Of Concentration Ratios 	     6
Discussion Of Specific Issues 	    11
References 	    16
Supplementary Figures 	    17
Appendix A.  Sites Used In The Analysis 	    51
Appendix B.  Site Classifications According To Climate  	    55
Appendix C.  24-hour Site Cases Omitted Because At Least One
               Of The Following Ratios Was Greater Than 1.05:
               PMio/DS, PMiQ/TSP, DS/TSP 	    56
Appendix D.  Annual  Site Cases Omitted Because At  Least One
               Of The Following Annual  Ratios  Was  Greater Than
               1.05:  PMio/DS, PMio/TSP, DS/TSP 	    57

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INTRODUCTION

In this memorandum the results obtained by Thrall and Burton  (1983a)  based
on 1980-1981 data are compared to results based on 1982 data  and  revised
1980-1981 data.  To facilitate the comparison, the new results are
presented in the same way as in the earlier report.  In addition, illus-
trations in this memo are numbered to correspond to illustrations in  the
earlier report, e.g., Figure 5' here corresponds to Figure 5  in the
earlier report.  For a description of the PM-10 attainment status problem
and the development of a method of solution see Pace and Frank (1982).

There are several differences between the data set analyzed here and  that
used previously:  (1) 1982 data, including PM 10 measurements, are now
available; (2) the first quarter of 1980 has been deleted from the 1980-
1981 data, since a change in filters nominally scheduled for the beginning
of 1980 appears not to have been implemented at a number of sites; and  (3)
24-hour or annual ratios of PM 10/DS, PM 10/TSP, or DS/TSP*exceeding  1.05
have been deleted.  Items 2 and 3 were suggested by EPA technical staff as
a means of improving the reliability and consistency of the data used in
the analysis.
DIFFERENCES IN CONCENTRATION RATIOS WHEN GROUPED
BY TIME, LOCATION, OR TOTAL CONCENTRATION

24-Hour Ratios Undifferentiated by TSP Concentration

The distribution of 24-hour DS/TSP ratios over time, beginning with the
second quarter of 1980 and ending with the last quarter of 1982, is shown
in Figure 5'. Jhe accompanying analysis of variance shows that differ-
ences among the average ratios for the 11 individual quarters are sta-
tistically significant.
* DS is an abbreviation for PM15 measured using a dichotomous sampler.
81003 2                          1

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Figures 6'  and 7'  show the results of grouping ratios  by  climate  and  by
EPA region, respectively.  Group differences are somewhat more  pronounced
between regions (e.g., an average ratio of 0.49 for Region  10 versus  0.59
for Region 8) than between climates (0.52 for West Coast,  0.53 for arid,
and 0.56 for other locations).

Figures 8,1 9,' and 10' show the results of grouping ratios by  state,
city, and site, respectively.   In each of the figures  we  display  the  two
groups whose histograms indicate the range of ratio distributions among
all the groups.  Note, however, that the analysis of variance in  each
figure refers  to all  groups having  at least two observations, and not
merely the two groups  displayed.  As expected, we see  larger differences
between cities than between states.  Since there are typically  only one  or
two sites  per  city in  our  sample, the variability of ratios between sites
is  similar to  that between cities.
 24-Hour  Ratios  Corresponding to High  TSP  Concentration

 Figure  11'  shows  the  effect  of grouping  ratios by TSP concentration (TSP <
         o                       O
 150  pg/m  versus  TSP  > 150 pg/m ).  In most of the remainder of the report
 we  restrict our attention to the latter group of ratios, corresponding to
 high TSP concentrations, since, as Pace and Frank point out, it is this
 group of observations that would most likely produce the high PM 10
 concentrations  of interest.   Indeed,  taking the TSP measurements at face
                                                                •j
 value,  one can  argue  that high PM 10  concentrations (> 150 yg/m )  can
 occur only on days of high TSP concentration.  We see from the results
 presented  in Figure 11*  that screening out observations corresponding to
 low TSP concentrations (< 150 ug/m3)  has  little effect on the average and
 standard deviation of the ratios.  Restricting attention to site-days
                                           o
 having high TSP concentrations (> 150 ug/m ), Figures 12' through 17' show
 distributional  changes in 24-hour DS/TSP  ratios over time and location, in
 parallel with Figures 51 through 10'.
 31*003 2

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Comparing Figures 5' and 12', we see that one result of screening  out  low
TSP concentrations is that the differences among mean ratios  for quarterly
periods are no longer statistically significant  (the quarterly  averages
are 0.50, 0.54, 0.56, and 0.56).

Comparing the results in Figures 6' through 10' with the corresponding
results in Figures 13' through 17', we see that screening 24-hour  DS/TSP
ratios based on TSP concentration reduces the differences in  ratios that
are associated with different site locations.  The analysis of  variance
given in Figure 13' shows that there is no statistically significant
difference (at the 0.01 level) between ratios measured in different
climates.  Figure 14' shows that the differences between EPA  regions
remain statistically significant, although the differences are  reduced.
The differences among states, among cities, or among sites remain  sta-
tistically significant, as shown by Figures 15', 16', and 17',  respec-
tively.  Nevertheless, these geographical differences are less  pronounced
for high TSP concentration, as evidenced by the diminished F-statistics in
the analysis of variance tests.
Annual Ratios Undifferentiated by TSP Concentration

Following the same format for ratios of annual average DS and TSP concen-
trations as for 24-hour concentrations, we see from Figure 18' that the
differences between the 1980, 1981, and 1982 average ratios (0.57, 0.55,
and 0.54, respectively) are not statistically significant.

The analyses of variance presented in Figures 19' through 23'  show that
the annual ratios are geographically more homogeneous than are the 24-hour
ratios.  Partitioning site-years by climate or EPA region does not reveal
geographic differences in average ratios beyond what one might find for a
sample drawn from a geographically homogeneous population.  Only the finer
partitions based on states, cities, and sites show geographic location to
have a statistically significant effect on average annual ratios.
84003 2

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To give an indication of the range of geographic variation  in the distri-
bution of annual ratios, Figures 21', 22', and 23' contrast  results  for
two states, cities, and sites, respectively.  Figure 21' compares the
ratios for the state of Washington (having an average of 0.44) with  those
for North Carolina (having an average of 0.63).  Similarly,  Figure 22'
contrasts the average annual ratio for New York City (0.52,  an average of
0.55 and 0.49 at two sites) with the ratio for Buffalo, New  York  (0.57,  an
average of 0.68 and 0.49 at two sites).  The case of Buffalo illustrates
that wide site  variation can exist within one city.  (Figure 22'  also
shows that the minimum  and maximum city ratios were 0.197 and 1.020,
respectively.)  Finally, Figure 23' demonstrates an even wider variation
between the site-specific  ratios in Will County, Illinois (with an average
of 0.36) and those in Rubidoux, California  (with an average  of 0.72).
 Annual  Ratios Corresponding to  High  TSP  Concentration

 Figure  24'  shows the  effect of  grouping  annual  ratios  into  low  and  high
 annual  average  TSP  concentrations, with  low and high TSP  concentrations
 defined as  being below  and above  55  yg/m ,  respectively.  We  see  that  the
 average and standard  deviation  of the ratios are lower for  the  high TSP
 concentrations  (0.59  ±  0.14 versus 0.55  ± 0.11).  Figures 25' through  30'
 show the effect of  time (year)  and location for annual  ratios
 corresponding to high TSP  concentration, in parallel with Figures 18'
 through 23', which  show ratio distributions undifferentiated  by TSP
 concentration.

 In general, the result  of  screening  out  low TSP concentration has only a
 slight  effect on annual ratios.  Statistically  significant  differences
 between cities  and  sites remain,  whereas the difference between states is
 marginally  statistically significant. The other grouping factors—year,
 climate, and region—do not  reveal statistically significant  differences.
                                  4
 8^003 2

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The Use of Grouping Factors

Screening occurrences of high ratios (greater than  1.05)  from  the  data
produces an effect similar to the one reported by Thrall  and Burton
                                                       o
(1983a) when low TSP concentrations (less than 150 iig/m  ) were excluded.
The effect is to reduce the differences between geographic regions, years,
and so on.  This is not surprising; since the higher ratios correspond to
the lower TSP concentrations, the screening out of high  ratios and the
exclusion of low TSP concentrations produce nearly the same set of data.
As a consequence, the TSP level  (low or high) no longer appears to be a
statistically significant factor.

Thus the case for using group-specific distributions*of ratios to estimate
the probability of PM 10 attainment status, which was not strongly
supported by the previous data,  has even less support in the more recent
and revised data.

Of course, some group differences, e.g., between quarters, are statisti-
cally significant.  Nevertheless, the case against the use of group-
specific ratios, even in the face of statistically significant differ-
ences, is fairly strong:  when group differences are great enough to be of
practical significance, e.g., for differences between sites, the sample
sizes for individual  groups are  too small  to permit reliable estimation
and application of the group-specific distribution of ratios.

Since PM 10 measurements are now available, it is possible to examine this
issue in a more quantitative fashion, i.e., we could evaluate the efficacy
of group-specific predictions of PM 10  measurements (or predictions of
whether the PM 10 concentrations are above or below some level) using
statistical cross-validation techniques.  The cross-validation analysis is
beyond the scope of the present  effort,  however.
  By a  "group-specific  distribution," we mean a distribution of  PM10/TSP  or
  DS/TSP ratio  derived  specifically  from sites of a  particular type  (i.e.,
  within a  particular group).   For example,  if we only considered  ratios
  observed  in a given city,  this  group  of ratios would be  specific for  that
  city  and  the  distribution  of  values would  be a group-specific  distribution,
84003 2

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POOLING NATIONAL DATA TO ESTIMATE THE STATISTICAL
DISTRIBUTION OF CONCENTRATION RATIOS
Table 5' shows the sample distribution of the 24-hour  ratios of  PM  10/DS,
PM 10/TSP, and DS/TSP for those site-days having high  TSP concentrations
(> 150 pg/m ).  Because the effect of high TSP is not  statistically
significant for the current data set, we include Table 5" to show the  same
ratios for all site-days (undifferentiated with respect to high  or  low
TSP).  Tables 7' and 7" give the corresponding distributions of  annual
ratios.  These results may be compared to the unweighted percent!les
previously reported  (Tables 5 and 7 of Thrall and Burton, 1983a).   Because
the use of weighting factors was previously  found to have little effect on
the distribution, this procedure was not followed in the analysis  reported
here.
The  recently available 24-hour  PM  10 measurements  allow  us  to  examine
PM 10/DS  ratios that, of necessity, were  previously  assumed to have the
constant  value 0.83.  Tables  51 and 5"  show that the sample median  (50th
percent!le) ratio  is 0.89  for high TSP  concentrations and 0.85 for  overall
TSP  concentrations.  Figures  31 and 32  display  scatter diagrams of  24-hour
and  annual concentrations,  respectively.   From  the information included in
Figure  31a, we see that the coefficient (a)  minimizing the  sum of squared
residuals

                              (PM 10 -  a-DS)2

is 0.82.   Scatter  diagrams of PM  10/TSP ratios  versus 0.83  times corre-
sponding  DS/TSP  ratios are shown  in Figures 33  and 34 for 24-hour and
annual  data,  respectively.

On the  choice  of  ratio distribution to  be used  to  estimate  PM  10 attain-
ment status,  our judgment  is  that the 24-hour PM  10/TSP  ratios are
sufficiently  numerous to  be of  use for  the short-term standard, but that
the  annual DS/TSP  distribution  multiplied by an appropriate factor  (in the
 84003  2

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TABLE 5'.  24-Hour high  TSP  (>  150 yg/m3), all ratios < 1.05, April 1, 1980 - December 31, 1982.
Ratio =
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
Standard devi
PM 10/DS
Percentile
0.40
0.40
0.68
0.73
0.77
0.83
0.85
0.89
0.91
0.93
0.95
0.98
1.02
1.04
1.05
0.86
ation 0.11
Number of cases 116
Ratio 2 = PM
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
Standard deviation
Number of cases
10/TSP
Percentile
0.19
-
0.30
0.36
0.40
0.43
0.46
0.50
0.51
0.54
0.55
0.57
0.58
0.63
0.64
0.48
0.09
34
Ratio 3 =
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
Standard deviati
Number of cases
DS/TSP
Percentile
0.16
0.18
0.26
0.36
0.44
0.48
0.51
0.55
0.58
0.61
0.66
0.71
0.77
0.88
0.98
0.54
on 0.14
283

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          TABLE  5".  ^differentiated 24-hour TSP,  all  ratios  <  1.05, April 1, 1980 - December 31, 1982.
00
Ratio = PM
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
10/DS
Percentile
0.40
0.50
0.62
0.68
0.75
0.79
0.83
0.85
0.88
0.91
0.93
0.96
1.00
1.04
1.05
0.84
Standard deviation 0.11
Number of cases
287
Ratio 2 = PM
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
Standard deviation
Number of cases
10/TSP
Percentile
0.19
0.20
0.29
0.34
0.39
0.42
0.45
0.48
0.50
0.54
0.57
0.65
0.70
0.79
0.91
0.48
0.12
265
Ratio 3 =
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
DS/TSP
Percentile
0.02
0.21
0.33
0.38
0.44
0.48
0.51
0.54
0.57
0.60
0.65
0.71
0.78
0.92
1.05
0.55
Standard deviation 0.13
Number of cases
5733

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TABLE 7'.  Annual  high  TSP  (>  55 pg/m3), all ratios < 1.05,  April  1,  1980  -  December  31,  1982.
Ratio = PM
Percentage
Minimum
1
. 5
10
20
30
40
50
60
70
80
90
, 95
99
Maximum
Average
10/DS
Percentile
0.52
-
0.52
0.55
0.60
0.61
0.80
0.81
0.83
0.86
0.86
0.91
0.93
-
0.94
0.77
Standard deviation 0.14
Number of cases
18
Ratio 2 = PM
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
Standard deviation
Number of cases
10/TSP
Percentile
0.25
-
-
-
0.38
0.40
0.45
0.48
0.49
0.51
0.53
0.61
-
-
0.64
0.47
0.11
13
Ratio 3 =
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
Standard deviati
Number of cases
DS/TSP
Percentile
0.30
0.31
0.36
0.41
0.46
0.50
0.51
0.54
0.57
0.59
0.63
0.67
0.73
0.84
0.90
0.55
on 0.11
205

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TABLE 7".  Undifferentlated annual  TSP,  all  ratios  <  1.05,  April  1,  1980  -  December  31.  1982.
Ratio = PM
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
10/DS
Percentile
0.52
_
0.52
0.55
0.60
0.73
0.81
0.82
0.83
0.84
0.86
0.91
0.93
-
0.94
0.77
Standard deviation 0.13
Number of cases
19
Ratio 2 = PM
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
Standard deviation
Number of cases
10/TSP
Percentile
0.25
-
0.25
0.36
0.38
0.40
0.46
0.48
0.49
0.53
0.56
0.61
-
-
0.64
0.48
0.11
14
Ratio 3 =
Percentage
Minimum
1
5
10
20
30
40
50
60
70
80
90
95
99
Maximum
Average
DI/TSP
Percentile
0.20
0.29
0.36
0.42
0.47
0.50
0.52
0.55
0.58
0.61
0.63
0.69
0.74
0.90
1.02
0.55
Standard deviation 0.12
Number of cases
254

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range of 0.75 to 0.85, depending  on  the  criterion  used  to guide the
choice) should be used for  the  long-term  standard.
DISCUSSION OF SPECIFIC  ISSUES

Using the above results we address  the  following  issues  raised  by  EPA
staff at the beginning of this updating study.

     (1)  What options are available  to regulatory agencies  in  making
          initial  PM 10 attainment  determinations based  on scant or
          indirect measures of PM 10?

The options considered to date consist  of variations on  the  application  of
the methodology developed by Pace and Frank (1982).  Also, see  Thrall and
Burton (1983b).  The primary issue  is the choice  of ratio distribution to
be used, e.g., whether to apply a national or local sample distribution.
     (2)  Does the use of a single national distribution, estimated  from
          currently available data, still appear to be the most appropri-
          ate option?  If not, how should this recommendation be revised?

The use of a single national distribution still appears to be more
reliable than the use of local distributions, because of (i) the small
numbers of observations in most localities and (ii) the difficulty of
applying a geographic-specific distribution to anything other than the
identical geographical unit from which it was derived.
     (3)  Are the TSP cutpoints of 55 ug/nr for annual average concentra-
          tions and 150 pg/m3 for 24-hour average concentrations still
          appropriate thresholds for potential PM 10 nonattainment?
8^03 2
                                    11

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Having screened out high DS/TSP ratios  (which  are  almost  always  concurrent
with low TSP concentrations), the difference between  the  average ratios
for low and high TSP concentrations is  no  longer statistically  significant,
The preferable procedure still appears  to  be to differentiate  ratios  on
the basis of the TSP (denominator) concentration rather than  simply
screening out high ratios.
     (4)  Are the data provided by EMSL  sufficient  to  reliably estimate
          PM 10/DS and PM 10/TSP distributions?   Is the  0.83  conversion
          factor between DS and PM 10  still  appropriate?

 Sample  sizes of 24-hour ratios appear  to be  sufficient for  reliable
 estimation, but few  annual  ratios are  available.  The  0.83  conversion
 factor  appears to be appropriate, although more precise  criteria and
 probably  more data would be required to  estimate  (with two-digit accuracy)
 the  "best" conversion  factor.
      (5)   Recommend  a  procedure  to be used by regulatory agencies for
           initial  determination  of attainment of annual  and 24-hour PM 10
           standards.  Discuss  the reliability of the procedure.  Provide
           all  results  necessary  to the implementation of the procedure and
           the  evaluation of its  reliability.  These results may include
           estimated  distributions of DS/TSP, PM 10/TSP,  and PM 10/DS as
           appropriate.

 We recommend that the  national 24-hour PM 10/TSP distribution be used to
 estimate  24-hour PM  10 attainment status and that attainment of the annual
 PM 10 standard be estimated using the national DS/TSP distribution
 multiplied by  0.83.   For the current data, in which high ratios have been
 screened  out,  no differentiation between low and high TSP ratios is
 needed.  These distributions are given in Tables 5" and  7".  As indicated
 by Figures 31  and 32 these procedures should yield predicted PM 10
                                        q
 concentrations typically within  10 pg/m  of the measured concentration.

 8*1003 2                           12

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As discussed in the previous section, and by Thrall and  Burton  (1983b),
there are further methods for gauging the reliability of these  procedures.

After circulation of an initial draft of this memorandum, we  received
several comments from EPA reviewers to which we now respond.

    (A)  The exclusion of ratios greater than 1.05 causes the previously
         reported relationship between DS/TSP ratios and TSP concentra-
         tions to disappear.  The deletion of high ratios may also induce
         a bias in the estimated distribution of ratios.  Two alternatives
         to the deletion of high ratios are: (1) to eliminate from the
         analysis those sites tending to produce high ratios (or other
         anomalies) or (2) to remove extremely low ratios in addition to
         the  removal of extremely high ratios.

The high concentrations were deleted at the request of EPA project staff
since these ratios are regarded as not physically meaningful.  At issue is
whether we wish to use the ratios to estimate the results of PM-10
monitoring, even though monitoring results may be occasionally erroneous,
or whether we wish to use the definition of PM-10, PM-15, and TSP (concen-
trations of particulate having aerodynamic diameters  less than 10, 15,  and
20 urn, respectively) to rule out ratios greater than  unity.   The latter
course was taken at the direction of EPA staff.

The deletion of high ratios does of course alter the  empirical  cumulative
distribution.  The number of site-days or site-years  in  which ratios  are
less than a specified value, x, with x between zero and  unity, is
unaltered but the total  number of site-days  or site-years is reduced.  The
result is that the proportion of site-days or site-years having  ratios
less than x is increased.  This has the effect of increasing the estimated
probability that the PM-10 concentration corresponding to a  given TSP
concentration is below the PM-10 standard.  That is,  the effect  of
deleting high ratios is to increase (or possibly leave unaltered) the
                    .»
number of sites deemed to be in attainment of the PM-10  standard, and to
84003 2                            13

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reduce (or possibly leave unaltered) the number of sites deemed to have
failed to attain the standard.

The suggested alterations to the deletion of high ratios are worth
pursuing in future work.  As more PM-10 measurements become available it
will be possible to compare the performance of various procedures for
estimating either PM-10 concentrations or PM-10 attainment status.

    (B)  Please clarify the reasoning leading to your recommendation that
         a national distribution of ratios be used rather than separate
         distributions for different geographic regions.  Also comment on
         the use of the analysis of variance to test the similarity of
         distributions as opposed to a Kolmogorov-Smirnov test, for
         example.

The use of computer program BMDP7D, entitled "Description of Groups
(Strata) with Histograms and Analysis of Variance," proved to be an
efficient way to make the many comparisons in which we were interested.
As noted in our previous report of 4 May 1983, an analysis of variance
finding that group differences are not statistically significant does not
imply that the distributions are identical, since the finding pertains not
to group distributions in their entirety but only to group means (and
variance in the case of BNMDP7D).  In general, the "significant" factors
such  as "site"  remained significant under a more robust  (but less power-
ful)  analysis, included in BMDP7D, that used separate rather than pooled
estimates of variance.  As the reviewer suggests, we did conduct nonpara-
metric  (Kolmogorov-Smirnov) tests in a few instances, but these did not
alter our findings.  We did not use nonparametric tests more extensively
because they require much more computation and programming time, and, more
importantly these tests are much less powerful, particularly for the
screening of approximately 100 groups with an average of about 50 observa-
tions per group.

Regarding the use  of a national distribution, our judgment is that if the
choice  is to apply to each group of sites either a national distribution

8i*003 2                           14

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or the distribution obtained from that group, then the national distribu-
tion appears preferable.  Our preference is based on considerations of
both practicality and statistical reliability.  Comparing the magnitude  of
sampling variability to the magnitude of group differences, it appears
that the use of one large-sample distribution, that admittedly represents
individual  sites imperfectly, will  do a better job in limiting the number
of PM-10 misclassifications.  We fully agree, however, that this recom-
mendation should be further examined by comparing the performance of
various methods of classifying PM-10 attainment status.

    (C)  Why has the analysis focused on ratios of particulates as a means
         of assessing PM-10 attainment status rather than some other means
         of assessment?  More specifically, the PM-10 assessments might
         well be improved by taking the logarithm of particulate concen-
         trations and using log TSP as a covariate of log PM-15 or log
         PM-10.

EPA project staff requested that we focus our analysis on particulate
ratios, since our task was to refine the work of Pace and Frank.   We did
examine the covariation of log OS and log TSP in previous work.   These
results along with those of other workers indicate that a linear  model
fits the log-transformed data slightly better than the untransformed data,
homogeneity of variance being an important  benefit of the transforma-
tion.   Our  work also suggests, however,  that TSP cutpoints,  to be used to
classify the status of sites, derived from  either particulate  ratios or
logged particulates would be much the same.  Again,  it would be  useful  to
use the recently available PM-10 data to compare the  rate of correct
classification of these different methods.

    (D)  Consideration should be given to the grouping of data into  the
         four quarters of the year,  i.e., by season,  rather  than  grouping
         data into the quarters  spanning the period  under study.
         Additionally, the analysis  might he improved  by  removing  sites
         having an insufficient  number of observations  during  a quarter  or
         year.

81*003  2                          15

-------
In our previous report we did find differences between DS/TSP ratios  for
the four quarters of the year.  Using those pairs of 24-hour DS and TSP
concentrations reported during 1980-1981 for which the TSP concentration
exceeded 150 pg/m , the quarterly averages were 0.48, 0.54, 0.57, and
0.56, respectively.  A similar analysis for the current data set was
hampered (although still possible) by the exclusion of the first quarter
of 1980.  The suggestion to remove sites having an insufficient number of
observations is worth pursuing in future analyses.
REFERENCES

Pace, T. G., and N. H. Frank.  1982.  "Procedure for Estimating Probabil-
    ity of Nonattainment of a PM^g NAAQS using Total Suspended Particulate
    or  Inhalable Particulate Data."  U.S. Environmental  Protection Agency,
    Research Triangle Park, NC.

Thrall, A. D., and C. S. Burton.  1983a.  "Characterizing  Ratios  of
    Particulate Concentrations:  A Preliminary Step in  Assessing  Likely
    Attainment Status Under a PM 10 National Ambient Air Quality  Stan-
    dard."  Systems Applications, Inc., San  Rafael, CA.  (SYSAPP-83/078).

Thrall, A. D., and C. S. Burton.  1983b.  "Considerations  in  Assessing
    PM  10 Attainment Status Using TSP Data."  Systems Applications, Inc.,
    San Rafael, CA.  (SYSAPP-83/079).
 8«t003 2                            16

-------
        1980
        01
1980
02
1980
03
1980
04
1981
Ql
1901
02
1931
03
1981
04
1982
Ql
1982
02
1982
03
1982
04
VAR 14
XCLUOED
VAL UE S
                       ........... ..49S  ..•.....•••••785 •"•••••••••"1036 "••••"••••"•1143 ••••••
         TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES  LISTED ABOVE
                                                                                                •1343
                                                                                                      ******* it •* ik *
                                                                                                                 1447 *«*•«
                                                                                                                             **"*1254  *"«*»»*«»«**«97|  ** ********MMMQgg •*••••••***M*7g3 ••••••••••••*7g|
IDPOINTS 	 	
1.085) — — ~~"^
1.060)
1.0151
0.9UJ)
0.945)
0.910)
0.875)
0.8401
0.805)
0.770)
0.*7«0>
0.666)
0.630)
' 0.695)
0.62S)
0.490)
0.455)
0.420)
D.3d5)
0.350)
0.316)
0.280)
0.245)
0.210)
0.175)
0.140)
0.105)
0.070)
0.035)
ROUP MEANS ARE DENOTED
EAN 0.000
TD.OEV. 0.000
.E.S.D. ».itJ
. E. M. 0.000
AX I MUM 0.044
INIMUM 0.000
AMPLE SIZE 0
•
..
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••• ••..**•••• ••• .••*• •.• ••••••••
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• • .. • ••••• ...... ••
••• •••«•• • • •••
• ••
•
BY M'S IF THEY COINCIDE WITH "S. N'S OTHERWISE
0.638 0.663 0.670 0.647 .527 0.666
0.153 0.154 0.138 0.140 .128 0.137
0.160 0.161 0.1J2 0.132 .124 0.131
0.008 0.007 0.006 0.006 .006 0.006
1.049 1.019 1.027 1.042 .988 1.016
0.160 0.163 0.086 0.171 .131 0.136
406 606 516 600 463 669
•
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• *• *•** ***
***** *** * *
* • ••*• **•
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It
0.532 .636 0.520 0.662
0.118 .123 0.126 0.129
0.H2 .117 0.121 0.123
0 . 045 . 006 0 . .C*5 0 . 005
1.010 .942 1.001 1.036
0.U9 .154 0.173 0.166
669 499 637 609
•
•
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0.566
0.127
0.122
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370



                                THE NUMBER OF GROUPS IS  NOT CONSISTENT WITH THE TWO-WAV SPECIFICATION. ONE-WAY ANALYSIS OF VARIANCE  IS COMPUTED

                                                                   .............................  ANALYSIS OF VARIANCE TABLE  ••••••«••••••••••••••••••••••••

                                                                     SOURCE             SUM OF  SQUARES      UK     MEAN ROUARE   F VALUr   TAIL PROBABILITY
                ALL  CROUPS COMBINED
          (EXCEPT CASES WITH UNUSED VALUES
           FOR VE1R.     AND
                                MEAN
                                STD.DEV.
                                R.E.S.D.
                                S. E. N.
                                MAXIMUM
                                MINIMUM
                                SAMPLE SIZE
                         0.647
                         0.134
                         0.129
                         0.002
                         1.049
                         0.022
                          6733
                               BETWEEN GROUPS
                               WITHIN  CROUPS
                               TOfAL
                                       1.7284
                                     101.9364
                                                    103.£638
                                     10
                                   5722
                                                                  5732
                              0.1728
                              «.1/170
                                                                                                                                 9.70
                                                                                                                                             0.0000
                          •    U.VtNfS TEST FUK  EQUAL VAIUANCLS     l0,i>VZ2                  6.71         0.0000
                                                                     ONE-WAY ANALYSIS OF VAhlAIICt
                                                                     UST STATISTICS FOR Wl I'llltl-UftOUP
                                                                     VARIANCES NOT ASSUMED TO UE EQUAL
                                                                        WELCH
                                                                        BROWH-FORSVTHE
                                                                                  10.2200
                                                                                  10.5249
                                                                                          10.11
                                                                                           9.68
                                                                                       0.0000
                                                                                       0.0000
                                                                  NOTE - ONLY THOSE GROUPS WITH NON-ZERO VARIANCE ARE USED IN THE  COMPUTATIONS.
                                 FIGURE  5'.   Distribution  of  24-hour  DS/TSP ratios  by  year  (1980.  1981.  1982)
                                 and  quarter.
      84003

-------
00
         W.COAST                       ARID                          OTHER
         	+	+	»
 VAR 14
EXCLUDED
 VALUES
         •••*..•**••****••**••****!424 «******•*******•***•**.*•i70e  •««•*••••*****«****«**«*«7765
           TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE  VALUES LISTED ABOVE
MIDPOINTS

   1.050)*
   1.0IS)*
   0.980)**                             *«•                          •*•«•••••«
   0.945>*«*                            *•••                         •*.*•••««*••»•••
   0.910)******                         ****                         ******************

   0.840)«********                     •««.*••*«*«••*                .......................... «34
   0.805)********"*                    ***************                *********•***********>»«**>gi
   0770 )••**•*.*««•••••               A****************              •*****************«****.»..g7
   0,7 351******************.**          **********************        *»*********«***********.**]2l
    .700j***************************34 *******«*******************g2  *****************».»*»»***J90
    .666)***************************4Z ***********************»***5a  **»****«**«***********«*»*247
    .630>***************************70 •**«*****************«**«**66  *******««**«***"«****«"***3Z6
    .595).**.».***..*****.**.**.*.».B2 ***..*.....*.***..*....*..*94  ..*.**........**.....*..**44a
    .560)****«*********«****«*******96 ••**•*«*««•«****«•*•*««««*104  H"*********«***"«*****"»**467
    .625)M***••****•*•••*••*•*******9s M**************************96  *«»•«•....•«••««»»«...«**.474
    .490}**************************100 *****************«***«*****8g  **************«********«**390
    .455 I**************************102 *«*•***»**•«***•********•••83  •*«•**•«**••«««*«**«***«««339
    .420)******«********«***********79 ••••««....*....*...........74  *****.«...**....*......*.*206
    .385 )*•««"••«"«*«*•«*•«•«•«.«••.63 ««*******««««**«•*.........64  ..........................137
    .350)***«**«*****************«**43 ...........................45  .......................****8S
    .315 I******************* *..«....3) *******..*•«*..**...**.**•     .................... ........45
    .200)****************              *****************              *******n*******************30

    .210)*******                       **********                     A******.********.**
    .175)**                            *********                      ********..***
    .140)***                           *«                             *•*
    .105)                                                             *
    .070)                                                             *
   0.035)                                                             •
GROUP MEANS ARE DENOTED BV'M'S  IF THEV COINCIDE WITH  "S, N'S OTHERWISE
                  MEAN
                  STD.DEV.
                  R.E.S.D.
                  S.  E.  M.
                  MAXIMUM
                  MINIMUM
                  SAMPLE SIZE
             0.522
             0.137
             0.133
             0.004
             1.036
             0.131
               946
   0.633
   0.150
   0.147
   0.005
   1.042
   0.150
     992
              0.557
              0.128
              0.122
              0.002
              1.049
              0.022
               3795
                         ALL GROUPS COMBINED
                  (EXCEPT CASES WITH UNUSED VALUES
                    FOR CLIMATE  )
                                   ******
                                   •
                  MEAN
                  STD.DEV.
                  R.E.S.D.
                  S.  E.  M.

                  MAXIMUM
                  MINIMUM
                  SAMPLE SIZE
                 0.647
                 0.134
                 0.129
                 0.002

                 1.049
                 0.022
                  6733
SOURCE

BETWEEN GROUPS
WITHIN  GROUPS

TOTAL
*******  ANALYSIS  OF  VARIANCE  TABLE   **«

 SUM OF SQUARES       OF      MEAN  SQUARE
      1.1900
    102.4737

    103.6630
   2
6730
0.5950
0.0179
                       f  VALUE   TAIL PROBABILITY

                         33.27         0.0000
LtVENE'S TEST FOR EQUAL VARIANCES
                   5732


                    2.67J0
                                                               22.34
                                                                             0.0000
                                                         ONE-WAY ANALYSIS OF VARIANCE
                                                         TEST STATISTICS FOR WITIIIN-GROUP
                                                         VARIANCES NOT ASSUMED TO BE EQUAL
                                                            WELCH
                                                            BROWN-FORSYTHE
                                                                              2.1742
                                                                              2,2572
                                                               32.02
                                                               29.90
                                                          0.001/0
                                                          0.0000
                                           FIGURE  6'.    Distribution  of 24-hour  DS/TSP by climate.

-------
                         REGION  1   REGION 2   REGION 3   REGION 4   REGION 6   REGION  6    REGION  7    REGION 8   REGION 9   REGION10
                                  +   ...,... +	+	+	....*.	+	+	*	...»	*
                 VAR 14
                EXCLUDED
                 VALUES
                MIDPOINTS
                         *..*...557 *.*****779 *«****230s •««***1304 **««»*i68l  »**«**«587  *«****«768  •••«**«623
                          TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE  VALUES  LISTED  ABOVE
                                                                                                                                 •625
                   1.0501
                   1.015)*
                   0.9B0)*
                   0.945>««
                   0.910)**
                   0.875)*
                   0.840)**
                   0.805)**
                   0.770)**
                   0.735)**
                   0'.700)**
                   0.665)**
                   0.630)**
                   0.595)**
                   0.560)*
                   0.525)H
                   0.490)**
                   0.455)**
                   0.420)**
                   0.385)**
                   0.3S0)**
                   0.315)**
                   0.280)**
                   0.245)*
                   0.210)**
                   0.175)**
                   0.140)**
                   0.105)*
                   0.070)
                   0.035)
                GROUP MEANS

                MEAN
                STD.DEV.
                R.E.S.O.
                S.  E. M.
                MAXIMUM
                MINIMUM
                SAMPLE SIZE
                    ********** ***
                                         ****
                                         ** *•
                                        *•
                                        **
                                        *****
                  •****•

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                                                               **«•
                                                               *****
                                                             ***
                                                             *•
           ***       ********|g **«****«|4 ****«***}3
           *         ........28 «**««««*15 .«...«««.*
      It  ********    ********34 ********24 ********30
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 ****«I9  .«.*•*..32  ********9Q *««•>.**7g ***«****5|
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******33  ********g4  *******|2g n***««**95 ********gg
......38  H...***«66  *«*..**i3| ...*»***74 H*****«i)B
******37  ******«*g9  ********9g ........54 ********95
         ********54  ********78 *«******4g ********72
         ..***...40  ********29 ********37 •«•««..ngf
         **.****.24  ****«***24 ********|8 ..«««...39
         ********I4  ****«***jg ********   ***«****27
         ******      *****      *******    ****.***|4
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                                                                          **********
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                                                                                   ****.
                                                                                   *****
                                                                                   *****
                                                              *****
                                                              *****
                                                              *****
                                                              *****
                                                              *****
                                                              *****
                                                           13
                                                        *«*15
                                                        ***30
                                                        *«*36
                                                        •**39
                                                        •••43
                                                           40
                                                        •••62
                                                        «**50
                                                        *"*37
                                                        *"*38
                                                        ***17
                                                        «**20
 ARE DENOTED BV M'S  IF  THEV COINCIDE WITH "S, N'S OTHERWISE
  0.529
  0.146
  a. 135
  0.008
  1.001
  0.119
    309
0.529
0.1)6
0.104
0.005
1.027
0.209
  468
0.683
0.122
0.115
0.004
1.017
0.192
 1014
0.577
0.120
0.114
0.005
0.986
0.086
  698
0.534
0.130
0.124
0.004
1.049
0.022
  862
                                                        0.542
                                                        0.139
                                                        0.139
                                                        0.006
                                                        0.967
                                                        0.150
                                                          494
         0.572
         0.133
         0.129
         0.007
         1.026
         0.226
           343
0.590
0.117
0.116
0.010
0.961
0.208
  149
0.530
0.146
0.137
0.006
1.042
0.154
  920
                                                                                                ********
                                                                                                •
0.489
0. 143
0.141
0.007
0.974
0.131
  476
                       ALL  GROUPS  COMBINED
                (EXCEPT CASES  WITH UNUSED VALUES
                  FOR RE6ION   )
                MEAN
                STD.DEV.
                R.E.S.D.
                S.  E.  M.
                MAXIMUM
                MINIMUM
                SAMPLE SIZE
      0.547
      0.134
      0.129
      0.002
      1.049
      0.022
       6733
                SOURCE

                BETWEEN GROUPS
                WITHIN  GROUPS

                TOTAL
                                                •««*"**  ANALYSIS OF VARIANCE TABLE  •*'

                                                SUM OF SQUARES      OF     MEAN SQUARE
                              4.7168
                             98.9469

                            103.6637
                                   9
                                5723

                                5732
                                 0.6241
                                 0.0173
                                                                                         F VALUE   TAIL PROBABILITY

                                                                                           30.31         0.0000
                LEVENE-S TEST FOR EQUAL VARIANCES
                                            9.5723
                                                                                6.85
                                                                                             0.0000
                                                       ONE-WAV ANALYSIS OF VARIANCE
                                                       TEST STATISTICS FOR WITHIN-GROUP
                                                       VARIANCES NOT ASSUMED TO BE EQUAL
                                                          WELCH
                                                          BROWN-FORSVTHE
                                                                    9.1606
                                                                    9,4048
                                                                               30.83
                                                                               30.32
                                                                                  0.0000
                                                                                  0.0000
84003
                                    FIGURE  7'.   Distribution  of  24-hour  DS/TSP  ratios by  EPA  region.

-------
                          NE
                                               ID
                  VAR 14
                 EXCLUDED
                  VALUES
                                                        43
ro
o
          TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED ABOVE
MIDPOINTS
   1.085)
   1.050)
   I. 015)
   0.980)
   0.945)"
   0.910)
   0.875)
   0.640)*
   0.805)*"                   ••
   0.770)"
   0.735)*
   0.700)*
   0.665)M
   0.630)" •
   0.596)* *
   0.660)* «"                 *****
   0.52S)*                    •••«•••
   0.490)**                   ******
   0.455)                     **
   0.4Z0)                     H******
   0.386)                     *.*««*••••
   0.360)                     *«**«*««J3
   0.316)                     «•*«••
   0.280)                     • «**«*«•«
   0.245)                     *«
   0.210)                     •*
   0.176)
   0.140)
   0.105)
   0.070)
   0.035)
CROUP  MEANS ARE DENOTED BY H'S IF THEV COINCIDE WITH *'S,  N'S OTHERWISE
                            **
                 MEAN
                 STD.DEV.
                 R.E.S.D.
                 S. E.  M.
                 MAXIMUM
                 MINIMUM
                 SAMPLE SIZE
            0.668
            0.111
            0.115
            0.021
            0.942
            0.602
               27
.418
.126
.128
.014
.803
.194
  77
            ALL GROUPS COMBINED
     (EXCEPT CASES WITH UNUSED VALUES
       FOR STATE   )

     MEAN            0.647
     STD.DEV.         0.134
     R.E.S.D.         0.129
     S. E. M.         0.032
     MAXIMUM         1.049
     MINIMUM         0.022
     SAMPLE SIZE       6733
    ••••••••A**********************  ANALYSIS OF VARIANCE TABLE  **•••*•••*••••••*•**
        SOURCE

        BETWEEN GROUPS
        WITHIN  GROUPS
SUM OF  SQUARES      DF

    11.0502         37
    92.6136       5695
MEAN SQUARE

   0.2987
   0.0163
F VALUE    TAIL

  18.36
                                                                                                                                   !*.*•*••***.


                                                                                                                                   PROBABILITY

                                                                                                                                     0.0000
*
*
TOTAL 103.6637
LEVENE'S TEST FOR EQUAL VARIANCES
5732
37,5695

4.03

0.0000
                                                            ONE-WAV ANALYSIS OF VARIANCE
                                                            TEST STATISTICS FOR WITIIIH-GROUP
                                                            VARIANCES NOT ASSUMED TO BE EQUAL
                                                              WELCH
                                                              BROWN-FORSVTHE
                                                                              37, 750
                                                                              37,1109
                                                                    19.61
                                                                    18.23
                                                      0.0000
                                                      0.0000
                                                        NOTE  - ONLY THOSE GROUPS WITH NON-ZERO VARIANCE ARE USED IN  THE COMPUTATIONS.
                         FIGURE  8'.   Distribution  of  24-hour  DS/TSP  ratios  by  state.   The  states  of  Nebraska
                         and  Idaho are  contrasted.   Other  states  are not shown  but  are included  in the  analysis
                         of  variance.

-------
St. Paul, t M1,nn.
                                                     " Pa-
             VAR 14
            EXCLUDED
             VALUES
            MIDPOINTS
                      TABULATIONS AND COMPUTATIONS WHICH HM.LUW EXCLUDE VALUES LtSfED ABOVE
               I .050)
               1.015)
               0.980)
               0.94S)
               0.910)
               0.675)
               0.0401
               0.805)
               0.770)                              ••••••••••
               0.7351                              ........12
               0.700)                              •••••••»i2
               0.665)           «                   ••••••••13
               0.6301                              H..»....20
               0.595)                              ••••••••22
               0.560)                              ••••••••23
               0.525)           •                   •••.••••|7
               0.490)                              ••••••••
               0.4SSI           ••••                .........
               0.420)           •                   •••
               0.305)           ••                  ....
               0.350)           •••                 «*
               0.315)           M
               0.280)           •••••••
               0.246)           •••••
               0.210)           •••
               0.175)
               0.1401
               0.105)
               0.070)
               0.0351
            CROUP MEANS ARE DENOTED BY  M'S  IF THEV COINCIDE WITH *'S. N'S OTHERWISE
            MEAN
            STD.DEV.
            R.E.S.D.
            S.  E. M.
            MAXIMUM
            MINIMUM
            SAMPLE SIZE
      0.320
      0.115
      0.115
      0.021
      0.680
      0.173
         31
0.628
0.129
0. 127
0.010
1.002
0.341
  174
                 ALL GROUPS COMBINED
           (EXCEPT CASES WITH UNUSED VALUES
             FOR CITV    )

           MEAN            0.547
           S1D.DEV.        0.134
           R.E.S.D.        0.129

           S. E. M.        0.002
           MAXIMUM         1.049
           MINIMUM         0.022
           SAMPLE SIZE      6733
                  SOURCE

                  BETWEEN GROUPS
                  WITHIN  CROUPS
          .......  ANALYSIS  OF VARIANCE TABLE  •"•

           SUM OF SQUARES     OF     MEAN  SQUARE
               23.0828
               80.5000
  96
5636
0.2404
0.0143
VALUE   TAIL PROBABILITY

16.82         0.0000
•
*
TOTAL 103.6b37
LEVENE'S TEST FOR EQUAL VARIANCES
5732
96,5636

6.80

0.0000
                                                ONE-WAV ANALYSIS OF VARIANCE
                                                TEST STATISTICS FOR WITHIM-GROUP
                                                VARIANCES NOT ASSUMED TO DE EQUAL
                                                  WELCH
                                                  BROUN-FORSVTHE
                                                     96, 800
                                                     96,1428
                                                   17.74
                                                   15.69
                                    0.0000
                                    0.0000
                                            NOTE  - ONLY THOSE  GROUPS WITH NON-ZERO VARIANCE ARE USED IN  THE COMPUTATIONS.
                      FIGURE 9'.    Distribution  of  24-hour  DS/TSP by city.   The  cities  of  St.  Paul, Minnesota
                      (ratios obtained  at one site)  and Philadelphia,  Pennsylvania  (four  sites) are  contrast-
                      ed.   Other cities are not shown,  but are  included in'the  analysis of variance.
84003

-------
                            St.Paul.Mn.
                            Phil., Pa.
                    VAR 14
                   EXCLUDED
                    VALUES
                                  .84
                                                  ••"•II
rv>
ro
          TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES  LISTED ABOVE
MIDPOINTS
   i.aasi
   I. 0501
   1.015)                     .
    .980)
    .945)
    .9101
    .B75I
    .840)
    .045)
    .770)
    .735)
    .700)
    .665) •
    .630)
    .595)
    .660)
    .526) •
    .490)
    .455)
    .420)
    .385)
    .350)
    .315)
    .280)
    .245)
    .210)
    .175)
    .140)
    .105)
    .070)
    .035)
GROUP MEANS ARE DENOTED  8V M'S IF THEY COINCIDE WITH ••$. N'S OTHERWISE
                  MEAN
                  STD.OEV.
                  R.E.S.D.
                  S. E. H.
                  MAXIMUM
                  MINIMUM
                  SAMPLE SIZE
              0.320
              0.116
              0.116
              0.021
              0.680
              0.173
                31
0.670
0.128
0.125
0.015
I .002
0.341
   69
                               ALL CROUPS COMBINED
                         (EXCEPT CASES WITH UNUSED VALUES
                           FOR
MEAN
STD.DEV.
R.E.S.D.
S. E. M.
MAXIMUM
MINIMUM
SAMPLE SIZE
0.547
a. 134
a. 129
0.002
1.049
15.822
S7J3
* SOURCE SUM OF SQUARES
• BETWEEN GROUPS 25.9093
• WITHIN GROUPS 77.7543
*
. TOTAL I03.0U3G
• LEVENE'S TEST FOR EQUAL VARIANCES
• ONE -WAV ANALYSIS OF VARIANCE
• TEST STATISTICS FOR WITIIIN-GROUP
• VARIANCES NOT ASSUMED TO BE EQUAL
* WELCH
• BROWN-FORSVTHE
DF MEAN SQUARE
118 0.2196
5614 0.0139
{.732
110.1,6)4
118. 840
118. 835
F VALUE
15.85
6.68
17.49
14.60
TAIL PROBABILITY
0.0000
0.0000
0.0000
0.0000
                                                         NOTE - ONLV THOSE  GROUPS WITH  NON-ZERO VARIANCE ARE USED IN THE COMPUTATIONS.

                   FIGURE  10'.   Distribution ;of  24-hour  DS/TSP ratios by site.   Sites  in  St.  Paul,  Minnesota and
                   Philadelphia,  Pennsylvania  are contrasted.   Other sites are  not shown,  but  are  included  in
                   the analysis of  variance.

-------
                                                       0 -  150
                                                                                       150
ro
CO
 VAR 14
EXCLUDED
 VALUES
                                      ***••••..................5294  *••••••••*•••••••••••••*«.335
           TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED ABOVE
MIDPOINTS
   1.085)
   I.0S0)                              ••••
   1.015)                              ...........
   0.980)                              •••••••••••••••
   0.9<6)                              •••••••••••••••••••••••
    .910)                              ••••••••••••••••••••••••••••
    .876)                              ...........................38   .*
    .840)                              *••••••••••••••••••••••••••56
    .80S)                              •••••••••••••••••••••••••••79  •••••••
    .770)                              •••«•••••••••••••..........97  ..
    .735)                              ••••••••••••••••••••••••••153  ..........
    .700)                              ••••••••••••••••••••••••••250  ..*.........*«..
    .665)                              •••••••	.324  .......................
    .630)                              ••••••••••••••••••••••••••444  .................
    .595)                              ••*••*•*••*•**•••..•••••••SB/  ...........................37
    .560)                              (!••••••••• ................635  H..........................32
   0.525)                              •.•••••••...••••.•......«.64I  .........................
   0.490)                              ••••••••••••••••*•••••••**54B  •••••••	••	
   0.455)                              ••••*••••••«•••«•.*«•.•••.502	
   0.42*)                              ..........................34,  ..................
   0.385)                              ••••••••..••••••••••••••••254  ••*•••.•••
   0.360)                              ••••••••••••••••••••••••••|64  .........
   0.315)                              ••••..•••.••••••••••••••.••gg  ...
    .200)                              ...........................60  •••
    .245)                              ...........................36  ....
    .210)                              .............................  .......
    .176)                              «••••••••••••••	        .*
    .140)                              •••••••                       •
    .105)                              •
   0.070)                              «
   0.035)                              •
CROUP MEANS ARE  DENOTED 6V M'S IF THEV COINCIDE WITH *"S, N'S OTHERWISE
                 MEAN
                 STD.DEV.
                 R.E.S.D.
                 S. E. H.
                 MAXIMUM
                 MINIMUM
                 SAMPLE SIZE

                        ALL GROUPS COMBINED
                 (EXCEPT CASES WITH UNUSED VALUES
                   FOR
                                          0.547
                                          0.134
                                          0.128
                                          0.002
                                          1.049
                                          0.022
                                           6450
                                 .544
                                 .144
                                 . 139
                                 .009
                                 .984
                                 .I5S
                                  283
                                  •••••••••••••••••••••••*•••••••  ANALYSIS OF  VARIANCE TABLE
                                  •
                                  •    SOURCE              SUM OF SQUARES      OF     MEAN SQUARE
                                                                                             ••••••••••••••••*••••
MEAN
STD.DEV.
R.E.S.D.
S. E. M.
MAXIMUM
MINIMUM
SAMPLE SIZE
                                  0.547
                                  0.134
                                  0.129
                                  0.002
                                  I. 049
                                  0.022
                                   6733
BETWEEN GROUPS
WITHIN  GROUPS
  0.0033
103.6605
   I
S73I
0.0033
0.01BI
F VALUE

   0.18
                                                                                                                             TAIL
PROBABILITY

 0.6702
TOTAL                  103.6630       5732

LEVENE'S TEST FOR  EQUAL VARIANCES      1,5731                   2.60"
                                                                           0.1071
                                                        ONE-WAV ANALVSIS  OF VARIANCE
                                                        TEST STATISTICS FOR WITHIN-UROUP
                                                        VARIANCES NOT ASSUMED TO BE EQUAL
                                                           WE1CH
                                                           BROWN-FORSVTHE
                                                                             1.  308
                                                                             I .  308
                                                              0.16
                                                              0.16
                                                    0.6899
                                                    0.6899
                                                    NOTE - ONLV THOSE  GROUPS WITH NON-ZERO VARIANCE ARE  USED  IN  THE  COMPUTATIONS.
                    FIGURE  11!.   Distribution  of  24-hour DS/TSP  ratios  by  24-hour TSP concentration  (low  versus
                    high TSP,  with  high  TSP defined  as  concentrations greater  than  150
   84003

-------
         1980
         01
1980
02
1980
03
1980
04
1981
01
1981
03
1981
04
                                                                                                                                          1982
                                                                                                                                          01
                                                                                                             1902
                                                                                                             02
                                                                             1902
                                                                             UJ
                                                            1982
                                                            04
 VAR 14
EXCLUDED
 VALUES
MIDPOINTS
   1. 1120)
   U.99J)
                         • ••••••••••••IB7  •••(•••••••••*207  ••••••••••••*29B ****
          TABULATIONS AND COMPUTATIONS  WHICH FOLLOW EXCLUDE VALUtS LISTED ABOVE
                                                                                                    "626
                                                                                 *ft«tt*****ft**MQ?g •«*«*»**««**«7qg •••••••••••**cge •••«***•***• *KfiQ

                                                                                  TABULATIONS AND COMPUTATIONS WHICH FOLLOW CXCLUOC VALUCS LICTCD ABOUC
                                                                                                                                                                          .............56tr
   0.93d I
   0.84ti)
   0.813)
   a.xe?)
   0.7t0>
   0.72«>
   it. 690 I
   U.fi6!J)
   0.63J)
   a.t,aa>
   U.S7S)
   u.B4u)
   U.SIJ)
   0.41)1)!
   0.4!iin
   0.391H
   0.360)
   U.33J)
   a . 30 J )
   0.270)
   0.240)
   U.21J)
   U.ID8)
   0.12*1
GROUP MEANS

MEAN
STD.OEV.
R.E.S.D.
S. E. H.
MAXIMUM
MINIMUM
SAMPLE SIZE
           ARE DENOTED BY M'S IF THEY COINCIDE WITH "'S. N'S OTHERWISE
                                                                                                         NS ARE DENOTED BV M'S IF  THEV COINCIDE WITH *'S,  N'S OTHERWISE
             .lag
             ,000
             .000
             .000
             .000
             .0»0
     .6S9
     .147
     .1S6
     .034
     .791
     .23)
      19
.672
.142
.128
.024
.87*
.177
  34
                     .671
                     .171
                     .166
                     .031
                     .984
                     .194
                      30
                     .497
                     .145
                     .136
                     .027
                     .893
                     .171
                       28
.622
.147
.144
.031
.739
.214
  23
                                     .644
                                     .120
                                     .115
                                     .024
                                     .827
                                     .269
                                       25
.648
.132
.128
.023
.020
.166
  32
                                    0.496
                                    0.130
                                    0.138
                                    0.024
                                    0.747
                                    0.208
                                       29
.646
.153
.144
.029
.957
.208
  28
                                                      .572
                                                      .152
                                                      .161
                                                      .031
                                                      .800
                                                      .204
                                                       24
.574
.118
.17?
.H:>,
.80S
.473
  II
                THE NUMBER OF GROUPS  IS NOT CONSISTENT WITH THE TWO-WAY  SPECIFICATION.  ONE-WAV ANALYSIS OF VARIANCE  IS COMPUTED

                      AIL GROUPS  COMBINED
                (EXCePT CASES WITH UNUSED VALUES
                  FOR YiAR

                MEAN
                SIII.DEV.
                R.E.S.D.
                S.  E. H.
                KAX1WUII
                HI III HUM
                SAMPLE SIZE
                              AND
       0.644
       0.144
       0.139
       0.009
       0.984
       0.I6S
         283



SOURCE
BETWEEN GROUPS
WITHIN GROUPS
TOTAL
SUM OF SQUARES
0.2218
S.6146
5.11364
OF MEAN SnUARC
10 0.0222
272 tt.HtUti
282
F VALUE TAIL PROBABILITY
1.07 0.3020

             LEVEHE-S TEST FOR EQUAL VARIANCES
                                                 10.  272                  0.44
                                                                                      a. 9,MO
                                                     ONE-WAY ANALYSIS OF VARIANCE
                                                     TEST STATISTICS FOR WUIIIN-GROUP
                                                     VARIANCES NOT AiUUHED TO iff EOUAL
                                                        WELCH
                                                        OROWN-FORSYTHE
                                                                 10.  97
                                                                 10. 26*
                                                                                                                  I.I*

                                                 NOTE - ONLY THOSE GROUPS WITH NON-ZERO VARIANCE ARE  USED  IN THE COMPUTATIONS.
                                                                                                      3.40ft,
                       FIGURE  12'.    Distribution  of  24-hour  DS/high-TSP  ratios  by  year  (1980,   1981,  1*982)  and  quarter
     84003

-------
                          V. COAST
                                                       ARID
                                                                                    OTHER
ro
01
                   VAR  14
                  EXCLUDED
                   VALUES
                                                  **gB3
                                                                                                            •3948
                  MIDPOINTS
                     1.020)
                            TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED ABOVE
                     0.960)
                     0.930)
                    .0.900)
                     #.840)
                     0.810)"*
tf.760)**
I/. 720)*****
H.600)**1"'**
0.660)***»*
0.630)*   •
0.6/90)**
0.570)M******
0.640)***
J/.SU)*****
tf.4au)*«****«
                                                       M****
i».420)«*»"*
JJ.390)*
tf.360)
0. 33*)
                                                          *•
                                                          4*
                     0.240)
                     0.210)*
                     0.100)
                     0.160)                                                           *
                     0.120)
                  GROUP MEANS ARE DENOTED 0V N'S IF THEV  COINCIDE WITH *'S, N'S OTHERWISE
                  KEAN
                  STC.DEV.
                  R.E.S.I).
                  S. K. M.
                  MAXIMUM
                  MINIMUM
                  SAMPLE SIZE
          0.581
          0.149
          0.1S4
          0.018
          0.984
          0.214
             72
                         ALL CROUPS COHBINED
                  (EXCEPT CASES  WITH UNUSED VALUES
                    FOR CLIMATE  >
MEAN
STD.PEV.
R.E.S.D.
S. E. M.
MAXIMUM
MINIMUM
SAMPLE SIZE
0.S44
0.144
0.139
0.009
0.984
0.155
203












0.543
0.158
0.153
0.016
0.957
0.171
94
SOURCE

BETWEEN GROUPS
WITHIN GROUPS
TOTAL







0.S22
0.124
0.122
0.012
0.747
0.155
117
SUM OF SQUARES

0. 1563
5.6802
5.8364











DF MEAN SQUARE

2 0.0781
200 0.0203
282







F VALUE TAIL PROBABILITY

3.85 0.0224


LEVENE'S TEST  FOR  EQUAL VARIANCES      2,  200                  2.74

ONE-WAV ANALYSIS OF VARIANCE
TEST STATISTICS FOR WITHIH-GROUP
VAH I AHCF.S NOT  ASSUMED TO BE EQUAL
   WELCH                         .     2,  162
   BROWN-FORSVTHE                      2.  237
                                                                                                                       3.98
                                                                                                                       3.70
                                                                                                                                    0.0661
                                                                                                               0.0205
                                                                                                               0.0261
                   FIGURE 13'.   Distribution of 24-hour  DS/high-TSP ratios  by  climate.

-------
                              REGION  1   REGION 2   REGION  3   REGION 4   REGION 5   REGION 6   REGION 7   REGION 0   REGION  9   REGION10
                      VAR 14
                     EXCLUDED
                      VALUES
                     MIDPOINTS
                        I .i'Z0>
                        0.090)
                        0.360)
                        «.93'J>
                        0.90JO)
                        0.H70)
                        0.84U)
                        0.819)
                        0.730)
                        0.7501
                        0./2J)
                        0.69)))
                              •••••**40| •••••••428  ******I264 *******820 •••••••739  •••••••209 *••*•'
                               TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE  VALUES LISTED ABOVE
                                                                                                   •231
   0.600>M
   0.070)
   4.040)
                       0.40.0)
                       a.'
                       I'.J
                       U.;
                       J9.3JU)
                       0.31'.))
                       fl.;
                                        •
                                        M«
                                                              *•*
                                                              • •*
                                                                                               * •••
                                                                                               i *
                                                                                               • •
                                                                                                                   H«
                                                                                                                   A * * * *
                                                                                  H-"
                                                                                    * • *
                         • *•
                         •*•
                     >n  •*•
                         |.|« •**•
                                                                                                                              * **
ro
cr>
   K.2I4I           •          •                    ••
   U.l&fl)                                                      •
   u.it.n                                 •
   i».i z>j >
GROUP MEANS  ARE DENOTED Bf H'S IF THEV COINCIDE WITH *'S. N'S OTHERWISE
MEAN
SIU.OEV.
K.F..S.D.
S. E. H.
HAKfNl'il
14 1 Mil IUII
SAMPLE SIZE
ALL
(EXCEPT CAS
P«JA KEUIQ
MEAN
STO.DEV.
P..E.S.D.
S. E. N.
IJ n 'J riJIll 1
"•l\ * t llvrl
SAMPLE SIZE
0.603
0.000
0.000
0.000
0.603
0.60J
1
.477
.141
.134
.042
.690
.2*9
11
0.535 0.549
0.152 0.119
0.148 0.109
0.042 0.022
0.681 0.747
0.Z08 0.155
13 28
0.516
0.121
0.1 18
0.016
0.747
0 . 2iM
55
IS WITH UIIUSEO VALUFS •
it )
0.544
B. 144
9 . i .n
a. an'}
0 . 904
283






* SOURCE
UETUEEN GROUPS
* WIIIIIN CROUPS
*
TOTAL
• LEVLNE'S TESI FOR
SUM




LOUAL
0.538
0.147
0.142
0.020
0.9b7
0.171
54

OF SQUARES
0.8462
4.9902

G.B3M
VARIANCES
0.556
0.046
0.055
0.H20
0.593
0.497
5
OF VARIANCE
0.354
H . ?Bb
Il.?!i8
«.M5
W.49U
II.ZUU
2

Uf MEAM nilUARE
0
274

202
(I. 2/4
0.1058
0.01U2



0
a
u
if
H
a


F





.616
.146
. 14U
.016
. !>(M
.177
80

VALUE
5.HI



1 .t.6
0.457
£.110
0.0'J9
u. a; H
£'.Uf,'J
It. 1P4
3/1









TAIL PROBAffLITY
0


•
a
eeiia



1358
                                                           ONE-WAV  ANALYSIS UK V.U.'IAHCE
                                                           iLsr siArisrits FOR ui IIIIH-GHOUP
                                                           VARIAHCLS  NOT ASSUMED  10 HE EQUAL
                                                              WE 1C II
                                                              URUWN-FORSYTIIE
                                                                             0.
                                                                             U,
I!)
13
4.55
5.47
0.0032
0.0U36
                                                       NOTE - ONLY  THOSE GROUPS WITH NON-ZERO VARIANCE  ARC  USED  IN THE COMPUTATIONS.
                   FIGURE  14'.   Distribution  of  24-hour DS/high-TSP  ratios  by EPA region.
  84003

-------
                                                                CA
                  VAR 14
                 EXCLUDED
                  VALUES
                 MIDPOINTS
                    I .020)
                    a.'JlO)
                    U.-.K.O)
                    D.'JJfl)
                    H . 9»IO )
                    M.U71O
                    1I.B4.Q)
                    U.81U)
                    0 . 7U.-J )
                    0. /.M)
                    fl.L'JJ)
                    (3T.CCO)
                    U.C3I)
                    1) . 1,10 )
                           TABULATIONS AHO COMPUTATIONS WHICH FOLLOW EXCLUUE VALUE!,  L1SUO ABOVE
ro
                    0.4QJU)
                    H.4'.ifl)
                    fl.4?3)
                    fl.39.9)
                    0.3G.C)
                    D.JJOt
                    V.Z10)
                    0.249)
                    tf.104)
                      .
                  GROUI- n.-X.HS ARE DENOTED BV H'S IF THEY COINCIDE WITH «'S. N'S OTHERWISE
STD.IUV.
R.E.S.D.
S. t. M.
MAX IMUH
M Jill MUM
0.408 0.619
0.069 if. 155
0.082 1). 159
0.035 M.019
0.479 JI.984
0.326 0.177
SAN.UE SIZE 4 66
(EXCEPT CASES WITH UNUSED VALUES
FUR STATE )
MS AH
STli.DLV.
R . 1 . 6 . 0 .
S. E. M.
M J vii Iiini
f lAA I rlUFl
MINlMUII
Q * Mb I L~ PI *JC
a APlrl. L i*l £L




0.S44
0.144
0.139
0.009
0. 934
0.155
on i
Zu J



SOURCE SUM
BETWEEN GROUPS
WITHIN GROUPS

TOTAL
Li:vLNE'S TEST FOR EQUAL
ONE-WAY ANALYSIS <;f VAIS


OF SQUARES
1.2675
4.S689

5.0364
VARIANCES
IAIII:E


OF MEAN SUUARE
17 0.0746
265 0.4172

282
17, i-1,5



F VALUE TAIL PROBABILITY
4.32 B. Bit fa



2.31 il.audl

Ttsr S.TATIS1ICS FUK VM Til I II CROUP
VARIANCES NOT ASSUMEU TO UE EQUAL
\IELCil
OROWN-FOaSVTME


17. 29
17, 66
4 . 68 .0 . 001/2
4.116 .0.00U0
                  FIGURE  15'.
                  contrasted.
                     NOTE -  ONLY THOSE GROUPS WITH NON-ZERO VARIANCE ARE USLD IN TKE  COMMIT/*! ION?.

Distribution  of 24-hour DS/high-TSP  ratios  by state.   Minnesota and California  are
Other states  are  not shown,  but  are  included in  the  analysis  of variance.
  84003

-------
                             Minn., Minn.
Rubldoux, Ca.
              VAR 14
              EXCLUDED
              V,UlttS
             MIDPOINTS
                i .
                       TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISltO ABOVE
                i| . Ql'.O >
                0.8/0)
                0.843)
                U.01UI
                0.700)
                «.7S'J>
                0.72JJ)
                0 . 690 1
                O.G07)
                C.639)
                fl.COtfl
                9.570)
                0 . S4.U I
                0.5191
                0.481)
    »»
    • *
                fl.li'J)
                U.399I
                o.36*>
                0.33*)
PO U.ZI4)
CO 0. 1801
0!l24> '
GROUP MCANS ARE DENOTED BY M'S IF THEY
MEAN 0.418
SrO.DEV. 0.081
R.E.S.D. 0.094
S. t. H. 0.047
MAXIMUM 0.4/9
MINIMUM 0.326
COINCIDE WITH *'S. N'S OTHERWISE
0.693
0.036
0.085
0.0IS
0.878
SAMPLE SIZE 3
Al 1 £Di*lllQC t?*nU&tllFfl **•
AL L GKUUr S CUff D I HE 0
(EXCEPT CASES WITH UNUSED VALUES
FOR CITY )
MEAN
STD.DEV.
R.E.S.D.
S. E. M.
MAX I MUM
MINIMUM
SAtll'LE SIZE

0.S44
0.144
0.139
0.009
0.984
0.ISS
283

•
•
Q
•
•
•
•
3)
SOURCE
BETWEEN CROUPS
WITHIN CROUPS

TOTAL

SUM OF SQUARES
2.6215
3.3149

3.8364
* LEVENE'S TEST FOR EQUAL VARIANCES
*
•
ONE-WAV ANALYSIS OF
TEST STATISTICS FOR
VARIANCE
WITH 114 -GROUP

OF MEAN SQUARE
31 0.0813
251 0.0132

Z8Z
31, 2S1



F VALUE TAIL PROBABILITY
6.16 . 0.0000



2.84 0.0000


* VARIANCES NOT ASSUMED TO BE EQUAL




*
*
WELCH
BROUit-FORSVTHE


31 , 31
31 . 65
11.04 0.0000
6.lb 0.0000
                                                NOTE - ONLY THOSE GROUPS WITH NON-ZERO VARIANCE ARE USCO IN THE COMPUTATIONS.
               FIGURE  16'.  Distribution of  24-hour  DS/high-TSP  ratios  by city.   Minneapolis and  Rubidoux are
               contrasted.  High TSP  ratios  were recorded  at a single site for  both  cities.   Other cities are
               not shown, but  are included in  the analysis  of variance.
8U003

-------
                    VAR 14
                    EX.LUDCO
                    VALUES
                   MIDPOINTS
                      1.020)
                                    Rubldoux
                                     Boise,  Idaho
                                      ....«-...64           • ••••«-*.19
                             TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISILl) ABOVE
ro
vo
                      0. UP1))
                      U.U7J)
                      i). 84tf)
                      0 010)
                      H.70W)
                      a.720}

                      (I.60JV)
                      !'.(
                      U.(
                      «*.:
                      «.!
                   • * ••
                   *«•«
   U. 39.1/1                              ***
   IJ.36iJ)                              H
   £.130)
   0. JOJ)
   0.270)                              •

i  a.210)
   u.ieoi                              *
   0. !!.#>
   0.12^1               i
GRO.ii' II ANS ARE DENOTED BV M'S IF THEV COINCIDE WITH *'S. N'S OTHERWISE
                    ME AH
                    STIi.DEV.
                    K. F . S. D .
                    S.  I.'. H.
                    MAXlMUi-t
                    Ml III HUH
                    SAI'.PLt SIZE
                      0.693
                      C.PUb
                             ALL GROUPS COMBINED
                            T CAStS WITH UNUSED VALUES
MtAII
i'ri>. DCV.
i! . L' . S . I) .
r, . L . M .
II/.X.IIUH
MINU'IUM
SAMPLE SIZE
0.544
0.144
0.139
0.009
0.904
0. 155
283



ri
*
*
M
*
*
•
M
«
*
*
*
H
Jff.077
B.077
v.an
0.421
0.104
0
SOURCE

OUVtEEN CROUPS
WITHIN GROUPS

TOTAL
LCVINE'S TEST FOR
OHf -WAY ANALYSIS
IKbT STATISVICS F
VAP.lAIILtS NOT ASS
WELCH
UROWH-FOUSVTIIE



SUM OF SQUARES

2.06/S
J. Ib9t)

G.Q364
EQUAL VARIANCES
OF VARIAMCb
OR Wl YHIN-GROUP
•HMO 10 BE EQUAL





OF IHEAH !>OUARc

33 «.i)H9U
249 U. 1/127

282
33. 249



33. 33
33. 66



F VALUE TAIL PilOBAllILIT/

6.35 0.00911

i

2.
-------
                         198*
                                                      1981
                                                                                    1982
00
O
 VAR 14
EXCLUDED
 VALUES
         a***********.********«****H4 ****************«**********73  **»*****«**«
           TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE  VALUES LISTED ABOVE
MIDPOINTS
   1.085)
   1.050)
   1.016)                             •*
    .980)
    .946)
    .9)0)                             *
    .875)
    .8401*                            *
    .80S)
    .770)***                           .                             ••
    .736)**                           •                             *•
    .700)*****                         ******                        *
    .666)*******                       **                            •«•
    .630)***«"*«                       ••*.«••«•••                   .*•**•***••
    ,696)*******                       *•*******•****••****           **********
    .6601M*******                      M**•**«*•«                    .«.*.*«..
    .625)*********                     •****•*****•*•                H********
    .490)**.**.**                      *«****..**.****                ............
    .465)***                           ..***•***                      **
    .420)***                            ******                        ***
    .386)**                            •*
    .360)**
    .316)
    .280>*
    .246)
    .210)                             «
    .175)
    .140)
CROUP MEANS ARE DENOTED BV H'S IF THEV COINCIDE WITH *'S.  N'S OTHERWISE
                                                                                                             •105
                MEAN
                STD.DEV.
                R.E.S.O.
                S. E.  M.
                MAXIMUM
                MINIMUM
                SAMPLE SIZE
             0.673
             0.112
             0.111
             0.014
             0.841
             0.277
                60
                       ALL  GROUPS COMBINED
                (EXCEPT CASES  WITH UNUSED VALUES
                  FOR VEAR     >
                MEAN
                STD.OEV.
                R.E.S.D.
                S. E.  M.
                MAXIMUM
                MINIMUM
                SAMPLE SIZE
                0.664
                0.116
                0.110
                0.007
                1.020
                0.197
                  264
0.661
0.127
0.115
0.012
1.020
0.197
109
SOURCE
BETWEEN GROUPS
WITHIN GROUPS
TOTAL
• LEVENE-S TEST FOR
0.541
0.101
0.102
0.012
0.768
0.316
77
SUM Of SQUARES
0.0380
3.3614
3.3994
EQUAL VARIANCES

OF MEAN SQUARE F VALUE
2 0.0190 1.42
261 0.0134
263
2, 251 0.48

TAIL PROBABILITY
0.2437

B.6210
                                                       ONE-WAV ANALYSIS  OF  VARIANCE
                                                       TEST STATISTICS FOR  WITHIN-GROUP
                                                       VARIANCES NOT ASSUMED  TO  BE EQUAL
                                                          WELCH
                                                          BROWN-FORSVTHE
                                                                             2, 168
                                                                             2, 240
1.60
1.49
0.2049
0.2279
                   FIGURE 18'.   Distribution of annual  DS/TSP  ratios by year.

-------
                       V. COAST
                                                    ARID
                                                                                 OTHER
                VAR  14
               EXCLUDED
                VALUES
                                                                              •44
                                                                                                          •223
                         TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE  VALUES LISTED ABOVE
              MIDPOINTS
                  1.0BS)
                  1.060)
                  1.015)                             *                            "
                  0.980)
                  0.945)
                  0.910)*
                  0.875)
                  0.840)*                                                         "
                  0.805)
                  0.770)"                            "••"                         *
                  0.735)*                                                         «•••
                  0.700)*
                  0.665)*
                  0.630)*
                  0.596)*
                  0.5601M
                  0.S25)*
                  0.490)*
                  0.466)*                              *                          **********
                  0.420)*****
                  0.386)"*
                  0.350)
                  0.316)*
                  0.280)*                                                         «
                  0.246)
                  0.210)                                                          *
                  0.176)
                  0.140)
              CROUP MEANS ARE DENOTED BV M'S  IF THEV COINCIDE WITH *'S,  N'S OTHERWISE
               MEAN
               STD.OEV.
               R.E.S.D.
               S.  E. M.
               MAXIMUM
               MINIMUM
               SAMPLE SIZE
.645
.134
.129
.022
.896
.293
  38
   0.647
   0.140
   0.135
   0.022
   1.020
   0.333
      40
        0.SS7
        0.106
        0.I0I
        0.008
        1.010
        0.197
          176
                     ALL GROUPS COMBINED
               (EXCEPT CASES WITH UNUSED VALUES
                FOR CLIMATE )
               MEAN
               STD.DEV.
               R.E.S.D.
               S.  E. M.
               MAXIMUM
               MINIMUM
               SAMPLE SIZE
   0.654
   0.116
   0.110
   0.007
   1.020
   0.197
     264
SOURCE

BETWEEN GROUPS
WITHIN  GROUPS

TOTAL
                                            .......  ANALYSIS OF VARIANCE  TABLE   «*•

                                            SUM OF SQUARES      OF     MEAN SQUARE
0.0062
3.3932

3.3994
  2
261

263
0.0031
0.0135
F VALUE   TAIL  PROBABILITY

   0.23         0.7949
LEVENE'S TEST FOR EQUAL VARIANCES      2, 251                   2.78         0.0640
                                                     ONE-WAV ANALYSIS OF VARIANCE
                                                     TEST STATISTICS FOR WITHIN GROUP
                                                     VARIANCES NOT ASSUMED TO BE EQUAL
                                                        WELCH
                                                        BROWN-FORSVTHE
                                                               2,  63
                                                               2,  93
                                                               0.19
                                                               0.18
                                                   0.8287
                                                   0.8383
                  FIGURE  19'.    Distribution  of  annual  DS/TSP ratio by climata.
64003

-------
U)
ro
         REGION I    REGION 2    REGION 3   REGION 4   REGION 5   REGION 6
         	»	»	+	*	+	H
 VAR 14
EXCLUDED
 VALUES
         ••••••••21  ••••••••jg  ••••••••gg ••••••••45 ••••••••4g  •*•••••••
           TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED
MIDPOINTS
   1.086)
   1.060)
   1.016)                                                      •
   0.980)
   0.946)
   0.910)
   0.876)
   0.840)
   0.806)
   0.770)
   0.736)
   0.700)*          •
   0.666)*                     •••
   0.630)*          •           ••••••••]
   0.696)***        ••«•        •••••*••
   0.660)M*         **         M***
   0.626)"**        M"         "*"
   0.490)           •»••        •••••••
   0.466)           •           •••
   0.420)           "           *••
   0.386)           *           *•
   0.360)           •                     ••         •           •
   0.315)                      •                     ••
   0.280)                                                      *
   0.246)
   0.210)*
   0.176)
   0.140)
GROUP MEANS ARE  DENOTED BV M'S  IF THEV COINCIDE WITH *'S.  N'S OTHERWISE
                                                                                            REGION
                                                                                                   7   REGION
                                                                                                   . . . +	
                                                                              8   REGION
                                                                              . . . +	
                                                                                                                             REGIONI0
                                                                                            •••••*»
                                                                                            ABOVE
                                                                                                    16
                                                                                                              •30
                                                                       *•
                                                                       *•*•
                                                             *•
                                                             **•
                                                                            •••13
                                                                                 *•**

                                                                                 H
                                                                                 • *•
                                                                                 • *•
                                        • ••

                                        M*


                                        • ••
                                                                                    *•
                                                                                    *••
                                                                                            H
                                                                                            *••
                   MEAN
                   STD.DEV.
                   R.E.S.D.
                   S.  E. M.
                   MAN IMUM
                   MINIMUM
                   SAMPLE SIZE
.660
.124
.098
.036
.684
.197
  12
                         ,6)6
                         ,093
                         094
                         022
                         ,709
                         ,356
                           18
0.660
0.096
0.102
0.014
0.707
0.311
   49
.686
.110
,100
,020
,841
,333
  30
0.646
0.094
0.090
0.014
0.749
0.312
   46
0.666
0.164
0.146
0.031
1.010
0.277
   24
.674
,088
,090
,024
,733
,448
  14
0.496
0.109
0.119
0.046
0.617
0.352
    6
0.671
0.148
0.139
0.024
1.020
0.369
   38
.600
.123
.13S
.029
.700
.293
  18
                         ALL CROUPS COMBINED
                   (EXCEPT CASES WITH UNUSED VALUES
                     FOR REGION  )
                                                     *•••••**•*•••
                   MEAN
                   STD.DEV.
                   R.E.S.D.
                   S.  E. M.
                   MAXIMUM
                   MINIMUM
                   SAMPLE SIZE
   0.654
   0.116
   0.110
   0.007
   1.020
   0.197
     264
                                       SOURCE

                                       BETWEEN GROUPS
                                       WITHIN  GROUPS

                                       TOTAL
                         SUM OF SQUARES

                             0.1356
                             3.2638

                             3.3994
                                                     ANALYSIS OF VARIANCE TABLE  •*•

                                                                       MEAN SQUARE
                                OF

                                 9
                               244

                               263
                                0.0161
                                0.0134
                                  VALUE   TAIL PROBABILITY

                                    I.13         0.3446
                                       LEVENE'S TEST FOR  EQUAL VARIANCES
                                           9. 244
                                                                                                      1.40
                                                                                                                   0.1893
                                                          ONE-WAV ANALYSIS OF VARIANCE
                                                          TEST  STATISTICS FOR WITHIN-GROUP
                                                          VARIANCES NOT ASSUMED TO BE EQUAL
                                                            WELCH
                                                            BROWN-FORSVTHE
                                                               9.
                                                               9.
                                                                                 69
                                                                                144
                                                                    1.10
                                                                    1.12
                                                                    0.3779
                                                                    6.3529
                    FIGURE  20'.   Distribution  of  annual  DS/TSP  ratios  by  EPA region.
   84003

-------
                                     WA
                                                         NC
CO
                   VAR 14
                  EXCLUDED
                   VALUES
                  MIDPOINTS
                                     • •••                 ««•..«•«>«
                            TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED ABOVE
                     1.060)
                     1.015)
                     0.980)
                     0.945)
                     0.910)
                     0.875)
                     0.840)
                     0.805)
                     •.770)
                     0.736)
                     0.700)
                     0.666)
                     0.630)
                     0.696)
                     0.560)
                     0.626)
                     0.490)
                     0.465)
                     0.420)
                     0.385)
                     0.360)
                     0.315)
                     0.280)           •
                     0.246)
                     0.210)
                     0.176)
                     0.140)
                  GROUP MEANS ARE DENOTED  BV M1
                  MEAN
                  STD.DEV.
                  R.E.S.D.
                  S. E. M.
                  MAXIMUM
                  MINIMUM
                  SAMPLE SIZE
                            S  IF THEY COINCIDE WITH *'S.  N'S OTHERWISE

                       0.443               0.629
                       0.087               0.0B8
                       0.090               0.093
                       0.031               0.027
                       0.664               0.770
                       0.293               0.469
                           8                  II
                        ALL GROUPS COMBINED
                  (EXCEPT CASES WITH UNUSED VALUES
                    FOR STATE   >
MEAN
STO.DEV.
R.E.S.O.
S. E.  M.
MAXIMUM
MINIMUM
SAMPLE SIZE
0.664
0.116
0.110
0.007
I .020
0.197
  264
SOURCE

BETWEEN GROUPS
WITHIN  GROUPS

TOTAL
                                                       .......  ANALYSIS OF VARIANCE TABLE   •••

                                                        SUM OF SQUARES     OF     MEAN SQUARE
                                                                              F VALUE   TAIL  PROBABILITY
                                                                              0.B2I0
                                                                              2.6784

                                                                              3.3994
 36
218

263
0.0235
0.0118
                                                                                                                   1.98
                                                                                                                               0.0017
                                                       LEVENE'S TEST FOR  EQUAL VARIANCES
                                                                                          35, 218
                                                                                                                   1.61
                                                                                                                               0.0400
                                                       ONE-WAV ANALYSIS OF VARIANCE
                                                       TEST  STATISTICS FOR UITHIN-UROUP
                                                       VARIANCES NOT ASSUMED TO BE EQUAL
                                                         WELCH
                                                         BROWN-FORSVTHE
                                                                         36.
                                                                         36.
                                                              36
                                                              78
                                                           11.34
                                                            2.63
                                    0.0000
                                    0.0002
                                                   NOTE  -  ONLY THOSE GROUPS WITH NON-ZERO VARIANCE ARE  USED  IN THE COMPUTATIONS.
                   FIGURE  21'.   Distribution  of annual  DS/TSP ratios  by  state.   The  states  of  Washington  and
                   North Carolina  are  contrasted.   Other  states  are  not  shown,  but  are  included  in the analysis
                   of  variance.
  84003

-------
                                  Buffalo,  M.Y.
                                     14.Y., N.Y.
                   VAR 14
                  EXCLUDED
                   VALUES
U)
MIDPOINTS
   1.085)
   1.050)
   1.015)
    .980)
    .945)
    .91*)
    .075)
    .840)
    .805*
    .770)
    .735)
    .700)
    .665)
    .630)
    .695)
    .560)
    .625)
    .490)
    .455)
    .420)
    .385)
    .350)
    .315)
    .280)
    .245)
    .210)
    . m>
    .140)
CROUP MEANS ARE

MEAN
STO.OEV.
R.E.S.O.
S. E. H.
MAX IHUH
H1NIHUN
SAMPLE SIZE
                            TABULATIONS AND COMPUTATIONS WHICH  FOLLOW EXCLUDE VALUtS LISTED  ABOVE
                                 DENOTED BV M'S IF THEY COINCIDE WITH *'S. N'S OTHERWISE
                                        0.567
                                        0.113
                                        M.I49
                                        0.0M
                                        0.781
                                        0.376
                                           S
                         ALL CROUPS COMBINED
                   (EXCEPT CASES WITH UNUSED VALUES
                    FOR CITV    I
                   MFAN
                   STD.DEV.
                   R.E.S.O.
                   S. E. H.
                   MAXIMUM
                   MINIMUM
                   SAMPLE SIZE
               0.S54
               0.116
               0.110
               0.007
               1.020
               0.197
                 254
0.S21
0.037
0.044
0.019
0.562
0.479
4
SOURCE
BETWEEN GROUPS
WITHIN GROUPS
TOTAL

SUM OF SQUARES OF MEAN SQUARE
1.6453 79 0.0208
1.7S4I 174 0.0101
3.3994 253
LEVCHE'S TEST FOR EQUAL VARIANCES 79. 174
ONE -WAV ANAL VS IS OF VARIANCE
TEST STATISTICS FOR WITHIN -UROUH
VARIANCES NOT ASSUMED TO BE EQUAL
WELCH 79, 37
BROWN-FORSVTHE 79. 13

F VALUE TAIL PROBABILITY
2.07 0.0000

5.86 0.0000
27.48 0.0000
1.64 0.1600
                                                   NOTE - ONLY THOSE GROUPS WITH NON-ZERO VARIANCE  ARE USED IN THE COMPUTATIONS.
                   FIGURE  22'.   Distribution  of annual  DS/TSP ratios  by city.   Buffalo,  New  York  and  New  York  City,
                   New York are contrasted.   Ratios were recorded at  two  sites  in  each  city.   Other cities are not
                   shown,  but  are  included  in the  analysis  of variance.
   81*003

-------
                                      gubldpux,  C/i.
              ₯111.Co., IJ1.
CO
en
                      VAR 14
                     EXCLUDED
                      VALUES
                                                           •
                               TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES  LISTED ABOVE
                     MIDPOINTS
                        !.*••>
                        1.050)
                        1.015)
                         .980)
                         .945)
                         .9101
                         .875)
                         .640)          •
                         .80S)
                         .770)
                         .735)          N
                         .700)
                         .665)
                         .630)
                         .595)
                         .560)          *
                         .525)
                         .490)
                         .455)
                         .420)                              •
                         .385)
                         .350)                              N
                         .315)                              •
                         .280)
                         .245)
                         .210)
                         .175)
                         .140)
                     WOUP MEANS ARE DENOTED BV H'S IF THEV COINCIDE WITH *'S.  N'S OTHERWISE
                     MEAN
                     STO.DEV.
                     R.E.S.D.
                     S. E.  M.
                     MAXIMUM
                     MINIMUM
                     SAMPLE SIZE
.719
.139
.149
.080
.849
.673
   3
0.359
0.066
0.082
0.046
0.405
0.312
    2
                          ALL  GROUPS COMBINED
                    (EXCEPT CASES WITH UNUSED VALUES
                     FOR SITt.   )

                    MEAN            0.SS4
                    STU.DEV.        0.116
                    R.E.S.O.        0.110
                    S. E. M.        0.007
                    MAXIMUM         1.020
                    MINIMUM         0.197
                    SAMPLE SIZE        254
SOURCE SUM OF SQUARES
BETWEEN GROUPS 1.8332
WITHIN CROUPS 1.5662
TOTAL 3.3994
LEVENE'S TEST FOR EQUAL VARIANCES
ONE-WAV ANALYSIS OF VARIANCE
TEST STATISTICS FOR WITHIN-GROUP
VARIANCES NOT ASSUMED TO BE EQUAL
WELCH
BROWN-FORSVTHE
DF MEAN SQUARE
94 0.0195
159 0.0099
253
94. 159
94. 39
94. 17
F VALUE
1.98

9.27
22.09
I.b2
TAIL PROBABILITY
0.0001

0 . 0000
0.0000
0.1626
                                                    NOTE  - ONLV THOSE GROUPS WITH NON-ZERO VARIANCE ARE USED IN THE COMPUTATIONS.
                   FIGURE 23'.   Distribution  of annual  DS/TSP ratios  by  site.   Sites  in Rubidoux,  California and
                   Will  County,  Illinois  are  contrasted.  Other  sites are not  shown,  but  are  included  in the
                   analysis  of variance.
   84003

-------
                                                      0-56
CO
CT>
                   VAR 14
                  EXCLUDED
                   VALUES
                  MIDPOINTS
                     l.0dS)
                     1.PG0)
                     I.015)
                      .980)
                      .945)
                      .910)
                      .875)
                      .040)
                            TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES  LISftD ABOVE
                                                                                                           •79
    .770)
    .735)
    .700)
    .665)
    .630)
    .595)
    .660)
    .525)
    .490)
    .465)
    .420)
    .385)
    .350)
    .315)                                                         ••'
    .280)                             •                            •
    .246)
    .210)                             *
    .1751
    .140)
GROUP  MEANS ARE DENOTED BV M'S IF THEV  COINCIDE WITH ••$. N'S OTHERWISE
                                                                                      • ••*<
                                                                          •30
                                                                          •34
                 MEAN
                 STD.DEV.   <
                 R.E.S.D.
                 S. E. M.
                 MAXIMUM
                 MINIMUM
                 SAMPLE SIZE

                        ALL GROUPS COMBINED
                 (EXCEPT CASES WITH UNUSED VALUES
                   FOR MHIVOL  )
                        0.587
                        0.144
                        0.124
                        0.021
                        1.020
                        0.197
                           49
                                                                    0.546
                                                                    a. in?
                                                                    0. 104
                                                                    a.BUI
                                                                    0,896
                                                                    0.293
                                                                      205
                 MEAN
                 STD.DEV.
                 R.E.S.D.
                 S. E. M.
                 MAXIMUM
                 MINIMUM
                 SAMPLE SIZE
0.664
0.116
0.110
                                     SOURCE

                                     BETWEEN GROUPS
                                     WITHIN  GROUPS

                                     TOTAL
                                        •••••••  ANALYSIS OF VARIANCE TABLE   «•«

                                         SUM OF SQUARES     OF     MEAN SQUARE
O.J688
3.3306

3.3994
  I
252

253
0.0688
0.0132
           F VALUE   TAIL PROBABILITY

             6.21         0.0233
1.020
0.197
  254
                                     LEVENE'S TEST  FOR EQUAL VARIANCES
             I. 2S2
                                                                                                  1.66
                                                                                                              0.1985
                                                       ONE-WAV ANALYSIS  OF VARIANCE
                                                       TEST STATISTICS FOR W1THIH-GROUP
                                                       VARIANCES NOT ASSUMED TO BE EQUAL
                                                         WELCH
                                                         BROWN-FORSVTHE
                                                           I.  61
                                                           I.  61
                                                                                                  3.62
                                                                                                  3.62
                                                 0.0619
                                                 0.0619
                                                   NOTE  - ONLV THOSE GROUPS WITH NON-ZERO VARIANCE ARE USED  IN THE COMPUTATIONS.
                   FIGURE 24'.   Distribution of annual  DS/TSP  ratios  by  annual  TSP  concentrations  (low versus
                   high  TSP,  with high  TSP  defined  as  concentrations  greater than 55 yg/m-3).
  84003

-------
                           1980
                                                        1981
                                                                                     1982
                   VAR 14
                  EXCLUDED
                   VALUES
                  MIDPOINTS
                      .925)
                           it.....*.........*.*.*.*....95 »»»»»»»•»»»«»»»»«•««••««»»»56 •»»• »*»»»»••*»*•*»»»•*»»•»«94
                             TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED ABOVE
    .876)
    .8601*
    .825)
    .800)
    .775)"
    .750)*
    .725)
    .700)"
    .675)"
    .650)*
                                                         ••
                                                         **
    .625)*
    .600)*
    .676 )H
    .550)*
    .525)*
    ,600)***«****                      ••••••«•*•••
    ,475).                             • «•«•
    .460)*•                            .*««•••
    .425)                              ••••••
    .400)***                           ***
    .376)*                             *
    .360)"                             ••
    .326)*
    .300)                              ***
    .275)
CROUP MEANS ARE DENOTED BY M'S IF THEY COINCIDE WITH
                                                                                     M****
                                                                                      **
                                                                                      **
                                                                      '•S, N'S OTHERWISE
                  MEAN
                  STD.DEV.
                  R.E.S.D.
                  S. E. M.
                  MAXIMUM
                  MINIMUM
                  SAMPLE SIZE
             0.664
             0.106
             0.103
             0.014
             0.841
             0.333
                63
,539
,111
,107
,012
,896
,293
  90
0.539
0.102
a.me
0.013
0.768
0.315
   62
                         ALL CROUPS COMBINED
                  (EXCEPT CASES WITH UNUSED VALUES
                    FOR VEAR    )

                  MEAN             0.546
                  STD.DEV.         0.107
                  R.E.S.D.         0.104
                  S. E. M.         0.007
                  MAXIMUM          0.896
                  MINIMUM          0.293
                  SAMPLE SIZE        20S
                                       SOURCE
              .......  ANALVSIS OF  VARIANCE TABLE  **•

               SUM OF SQUARES      OF     MEAN SQUARE
                                                                                                  F VALUE   TAIL PROBABILITY
*
*
*
*
BETWEEN GROUPS
WITHIN GROUPS
TOTAL
LEVEME'S TEST FOR
0.0230
2.3071
2.3301
EQUAL VARIANCES
2
202
204
2, 202
0.0116
0.0114


1.01

0.12
0.3675

0.8B93
                                                         ONE-WAY ANALVSIS  OF  VARIANCE
                                                         TEST STATISTICS FOR  WiTHIN-GROUP
                                                         VARIANCES NOT ASSUMED TO BE  EQUAL
                                                            WELCH
                                                            BROWN-FORSVTHE
                                                                             2, 123
                                                                             2, 185
                                                           1.02
                                                           1.03
                                            0.3643
                                            0.3606
                 FIGURE 25'.   Distribution of annual  DS/high-TSP ratios by year.
8U003

-------
                             W.COAST
                                                          ARID
                                                                                       OTHER
                     VAR 14
                    EXCLUDED
                     VALUES
                                                                                   •36
                                                                                                                •190
CO
00
           TABULATIONS AND COMPUTATIONS WHICH FOLLOW  EXCLUDE VALUES LISTED ABOVE
MIDPOINTS
    .925)
    .900)*
    .875)
    .850)"                                                         "
    .826)
    .800)
    .776)"                            """
    .750)                             •                            **
    .726)*                                                         ••
    .700)                                                          ••••••
    .676)                             *»                           *•
    .660)"                            *                            «••••••••
    .626)*"*                           *"                           ••»*••«««•
    .600,                             •••                          .........to.
    .575)**«
    .550)M*"                           M                            M*
    .626)                             * «**                         ••
    .500)*"*                           •
    .476)*"
    .460)""                           «
    .426)"**                           «
    .400)**                           •
    .376)
    .350)                             **
    .326)"                            •
    .300)*
    .276)
GROUP  MEANS ARE DENOTED BY M'S IF THEV COINCIDE WITH  *'S, N'S OTHERWISE
                                                                                         ***•«
                                                                                         *•
                    MEAN
                    STD.DEV.
                    R.E.S.D.
                    S.  E.  M.
                    MAXIMUM
                    MINIMUM
                    SAMPLE SIZE
              .646
              .143
              .137
              .027
              .896
              .293
                29
.642
.120
.121
.020
.769
.333
  36
.647
.095
.093
. ana
.841
.311
.141
                          ALL GROUPS COMBINED
                    (EXCEPT CASES WITH UNUSED VALUES
                      FOR  CLIMATE )
                                                          SOURCE
                                                         ...*.««  ANALYSIS  OF VARIANCE TABLE  *•••*••••••••«•••"•••*««•••••••

                                                          SUM OF SQUARES      OF     MEAN SQUARE   F VALUE   TAIL  PROBABILITY
                    MEAN
                    STD.DEV.
                    R.E.S.O.
                    S.  E.  H.
                    MAXIMUM
                    MINIMUM
                    SAMPLE SIZE
                  .646
                  .107
                  .104
                  .007
                  .896
                  .293
                  206
BETWEEN GROUPS
WITHIN GROUPS
TOTAL
LEVENE'S TEST FOR EQUAL
0.0005
2.3296
2.3301
VARIANCES
2
202
204
2, 202
0.0003
0.0116

0.02
3.77
0.9768
0.0248
                                                          ONE-WAV ANALYSIS OF VARIANCE

                                                          TEST STATISTICS FOR W1THIN-GROUP
                                                          VARIANCES NOT ASSUMED TO BE  EQUAL
                                                             WELCH
                                                             BROWN-FORSVTHE
                                                                             2.  50
                                                                             2.  68
                                                          0.02
                                                          0.02
                                          0.9800
                                          0.9834
                     FIGURE  26'.   Distribution of annual  DS/high-TSP ratios  by climate.
          84003

-------
CO
UD
                                                                                                                         ••**«***
         REGION 1   REGION 2   REGION 3   REGION 4   REGION 5   REGION 6   REGION  7    REGION 8   REGION 9   REGION10
         	»...	»	»	*	*	*	*	*	*	
 VAR 14
EXCLUDED
 VALUES
         ********I7 ********j7  *******«49 ••••••»*42  ********40 •»****«    ««*«»«
           TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED ABOVE
MIDPOINTS
   0.925)
   0.900)
   0.875)
   0.850)                               *
   0.426)
   0.800)
   0.775)
   0.760)
   0.725)
   0.700)          *
   0.676)
   0.650)          *
   0.626)
   0.600)          •
   0.576)"
   0.560)H*        **
   0.525>"        •
                                 *
                                    H*
                                                  «•*
                                                  **
                                                           **
                                                           *****
                                                                               M
                                                                               **«
                                                                               ***
   0.500)
   0.476)
   0.460)
   0.425)
   0.400)
   0.375)
   0,350)
   0.325)
   0.300)                     *                    *
   0.276)
CROUP MEANS ARE  DENOTED BV H'S IF  THEV COINCIDE WITH "'S,  N'S  OTHERWISE
                                                                                                                         N
                                                                                                                         • *•
                                                                                                                         *
                                                                                                                         *•
                 MEAN
                 STD.DEV.
                 R.E.S.D.
                 S. E. M.
                 MAXIMUM
                 MINIMUM
                 SAMPLE SIZE
             0.546
             0.024
             0.026
             0.011
             0.681
             0.621
,511
,100
,099
,027
,709
,366
  14
                        ALL CROUPS COMBINED
                  (EXCEPT CASES WITH UNUSED VALUES
                   FOR REGION  )
                 MEAN
                 STD.DEV.
                 R.E.S.D.
                 S. E. M.
                 MAXIMUM
                 MINIMUM
                 SAMPLE SIZE
                  ,546
                   107
                  ,104
                  .007
                  ,896
                  ,293
                   206
0.548 .671 0.545 0.547
0.099 .106 0.097 0.111
0.100 .090 0.092 0.115
0.016 .021 0.016 0.024
0.707 .841 0.749 0.768
0.311 .333 0.312 0.333
41 26 40 22
H
* SOURCE SUM OF SQUARES
*
* BETWEEN GROUPS 0.1326
* WITHIN GROUPS 2.1976
*
* TOTAL 2.3301
* LEVENE'S TEST FOR EQUAL VARIANCES
* ONE-WAV ANALYSIS OF VARIANCE
• TEST STATISTICS FOR WITHIN-GROUP
* VARIANCES NOT ASSUMED TO BE EQUAL
* WELCH
* BROWN-FORSVTHE
0.562
0.090
0.090
0.028
0.733
0.448
0.518
0.104
0.098
0.046
0.617
0.362
10 6
DF MEAN SQUARE

9
195

204
9. 195



9, 44
9, 113

0.0147
0.0113







0.571
0.137
0.133
0.025
0.896
0.369
30
F VALUE

1.31



1.21



1.04
1.45
.470
.113
.117
.031
.654
.293
13
TAIL PROBABILITY

0.2361



0.2899



0.4234
0.1763
                   FIGURE  27'.    Distribution of annual  DS/high-TSP ratios by EPA  region.
  84003

-------
                   OH
                                       WA
 VAR 14
EXCLUDED
 VALUES
          TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED ABOVE
MIDPOINTS
   0.925)
    .900)
    .876)
    .860)
    .826)
    .800)
    .776)
    .750)
    .726)
    .700)
    .676)
    .650)
    .626)
    .600)
    .676)          M«*«
    .650)          •                    •
    .626)          **•
    .500)          »*•••••              *
    .475)          •
    .450)                               *
    .425)                               M
    .400)                               ««
    .376)
    .360)
    .325)
    .300)                               *
    .276)
CROUP  MEANS ARE DENOTED BV M'S  IF THEV COINCIDE WITH *'S, N'S OTHERWISE
MEAN
STD.DEV.
R.E.S.D.
S. E.  M.
MAXIMUM
MINIMUM
SAMPLE SIZE
  .574
  .083
  .089
  .017
  .749
  .481
    23
      ALL CROUPS COMBINED
(EXCEPT CASES WITH UNUSED VALUES
  FOR STATE   )
MEAN
STD.DEV.
R.E.S.D.
S. E. M.
MAXIMUM
MINIMUM
SAMPLE SIZE
.546
.107
.104
.007
.896
.293
 206

0.428
0.080
0.079
0.030
0.642
0.293
7

SOURCE SUM OF SQUARES OF MEAN SQUARE F VALUE TAIL


*"*
BETWEEN CROUPS 0.5846
WITHIN CROUPS 1.7464
TOTAL 2.3301
LEVENE'S TEST FOR EQUAL VARIANCES
ONE-WAV ANALYSIS OF VARIANCE
TEST STATISTICS FOR WiTHIN-GROUP
VARIANCES NOT ASSUMED TO BE EQUAL
WELCH
BROWN-FORSVTHE
NOTE - ONLV THOSE GROUPS WITH NON-ZERO.
Of
annual DS/high-TSP ratios
33 0.0177 1.74
171 0.0102
204
33. 171 1.69
33, 26 11.81
33, 53 2.37
VARIANCE ARE USED IN THE COMPUTATIONS.
by state. The states of Ohio

PROBABILITY
0.0128

0.0313
0.0000
0.0025

and
 FIGURE 28'.   Distributi                                                   .
Washington are contrasted.   Other  states are not shown, but are included  in the analysis
of variance.

-------
                                W11J Co.,  111.
              El Cajon, Ca.
                VAR 14
               EXCLUDED
                VALUES

                         TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED ABOVE
               MIDPOINTS
                  0.02E)
                  a.900)
                  0.87S)
                  0.860)
                  0.826)
                  0.800)
                  0.776>                              •
                  0.750)
                  0.725)
                  0.700)                              H
                  0.675)
                  0.650)
                  0.625)                              *
                  0.600)
                  0.575)
                  0.550)
                  0.525)
                  0.500)
                  0.475)
                  0.450)
                  0.425)
                  0.400)           •
                  0.375)
                  ,0.360)           N
                  0.326)
                  0.300)           •

               GROUPZMEANS ARE DENOTED BV M'S IF THEV COINCIDE WITH ••$. N'S OTHERWISE
                MEAN
                STD.DEV.
                R.E.S.D.
                S. E. M.
                MAXIMUM
                MINIMUM
                SAMPLE SIZE
.359
.066
.082
.046
.405
.312
   2
0.710
0.103
0.129
0.073
0.783
0.637
    2
                      ALL GROUPS COMBINED
                (EXCEPT CASES WITH UNUSED VALUES
                  FOR CITV    >

                MEAN            0.646
                STD.OEV.        0.107
                R.E.S.D.        0.104
                S. E. M.        0.007
                MAXIMUM         0.896
                MINIMUM         0.293
                SAMPLE SIZE       206
                                                 NOTE - ONLV THOSE GROUPS WITH NON-ZERO VARIANCE ARE USED IN THE COMPUTATIONS.


                FIGURE  29'.   Distribution of  annual DS/high-TSP ratios  by  city.   Will  County,  Illinois  and  El
                Cajon,  California are contrasted.   High-TSP ratios  were recorded at one site in each city.
SOURCE SUM OF SQUARES
BETWEEN GROUPS 1.2603
WITHIN GROUPS 1.0698
TOTAL 2.3301
LEVENE'S TEST FOR EQUAL VARIANCES
ONE-WAV ANALYSIS OF VARIANCE
TEST STATISTICS FOR W1THIH-GROUP
VARIANCES NOT ASSUMED TO BE EQUAL
WELCH
BROWN-FORSVTHE
DF MEAN SQUARE
64
140
204
64, 140
64. 29
64, 20
0.0197
0.0076



F VALUE
2.68

3.94
18.77
2.24
TAIL PROBABILITY
0.0000

0.0000
0.0000
0.0234
84003

-------
   VAR 14
  EXCLUDED
   VALUES
  MIDPOINTS
      .926)
      .900)
      .876)
      .860)
      .825)
      .800)
      .776)
      .760)
      .725)
      .700)
      .675)
      .660)
      .625)
      .600)
      .676)
      .560)
      .626)
      .600)
      .475)
      .450)
      .425)
      .400)
      .376)
      .350)
      .326)
      .300)
      .275)
                    KJ.1.1! Co.,,111.
                                            Cajon,
             TABULATIONS AND COMPUTATIONS WHICH FOLLOW EXCLUDE VALUES LISTED ABOVE
  GROUP MEANS ARE DENOTED  BY N'S IF THEY COINCIDE WITH •'S, N'S OTHERWISE
  MEAN
  STD.DEV.
  R.E.S.D.
  S.  E. H.
  MAXIMUM
  MINIMUM
  SAMPLE SIZE
                        0.359
                        0.066
                        0.082
                        0.046
                        0.405
                        0.312
                            2
0.710
0.103
0.129
0.073
0.783
0.637
    2
       ALL  GROUPS COMBINED
(EXCEPT CASES WITH UNUSED VALUES
  FOR SlTC     )

MEAN            0.646
STD.DEV.         0.107
R.E.S.D.         0.104
S. E. M.         0.007
MAXIMUM         0.896
MINIMUM         0.293
SAMPLE SIZE        205
                                 ***************•«**•*•*«*••«*•«
FU
                                     SOURCE

                                     BETWEEN GROUPS
                                     WITHIN  GROUPS
                                                                ANALYSIS  OF VARIANCE TABLE  **'

                                                        SUM OF SQUARES      DF     MEAN SQUARE
                1.4309
                0.8992
 73
131
0.0196
0.0069
                                                   F  VALUE   TAIL PROBABILITY

                                                      2.86         0.0000
                                     TOTAL                   2.3301        204
                                  ••••••••*••••••••••••**••••*••«•••••••••••••••••••*••*•*•»•«*«••••*••«•••••**•*•••*••*•*•••
                                     LEVENE'S TEST FOR EQUAL VARIANCES     73, 131                  8.36         0.0000
                                  •••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••••0«K««»««*«««««*««««««»
                                      ONE-WAY  ANALYSIS OF VARIANCE
                                      TEST STATISTICS FOR WITHIN-GROUP
                                      VARIANCES  NOT ASSUMED TO BE EQUAL
                                         WELCH
                                         BROWN-FORSYTHE
                                                                          73.
                                                                          73.
                                  29
                                  22
                       16.83
                        2.07
                          0.0000
                          0.0287
                                  NOTE - ONLY  THOSE GROUPS WITH NON-ZERO VARIANCE ARE USED  IN THE COMPUTATIONS.
                 D!s*!f!but!on  of  annual  DS/high-TSP ratios by site.   Sites  in  Will  County,  Illinois
                                      C°ntraSted-   «*" '»«  -e not shown  but  are included  in  tne

-------
                   N-  237
                   COR=  .9647

                       MlAN
                   X   54.263
                   Y   44.G32
                                            ST.DEV.     REGRESSION LINE     RES. MS.
                                             32.669   X- 1.1504*Y+ 2.2429   74.319
                                             27.158   Y- . 801 94*X-t- 1.3123   51.359
                                    ZERO INTERCEPT  REGRESSION LINE   RES. MS.
                                    Y = 0.81971*X                     51.6382
          *************
                                     '.***+	X. .Y.+	'
    200
    175
    150
    125
    100
    75
    25
    0.0
                            1
                       2
                     11  111
                    11       1
                   2    1
                  1  22  1
                111  1
              221  2   1
            1  1   1
           11  4
         112321          1
         154 1
        232 1
        7331 1
     23776 1 11
     286313
   17D921
   CF122
  BF934  1
 383
8932
2
*
*
*
*
                                                                                *
                                                                                *
                                                                                *
                                                                                *
Y +

0.0

25.

+

50.

75.

. * .

100

125



150

175



200

225



250
. . •*• . .
275



300
..+....
325
3
                                                                              350
                                          DS
   FIGURE 31a..  Regression analyses for 24-hour concentrations:  PM 10 versus DS
81+003
                                      43

-------
                                    N =   265
                                    COR= .H916

                                        MEAN    ST.DEV.     REGRESSION  LINE     RES. MS.
                                    X    92.468    49.215   X- 1.6673*Y+  18.292    498.56
                                    Y    44.490    26.318   Y- ,47680*X+  .40157    142.58

                                        ZERO INTERCEPT  REGRESSION LINE   RES. MS.
                                        Y = 0.48018*X                    142.0728
           * * xx***x*«*«*w* *** ******XXK *******************    + * *y + * * +   Y + *   +*
           •                                              »«o»~«A~ ••"•••?"•••"



      2ZZ   +                                                                       *
      175
      IStf
      1?5
                                 l   l  l  l   l
      100  +                       111                                          +
                               11        1
                            1       31                                              *
                                   2     1                                         *
                           1  111  1  11  2    1
      75.  +                 2  11   1                                                +
                          1    12  11  1                                              *
                        1    12112  111                                            *
                          112   1   1  1                                              *
                      2   1  12 11     1                                             *
      5-3.  +            42333211                                                    *
                     1114214 211                                                 *
                    13351232 1  1                                                  *
                  133 533411     1      1                                            *
                  1365341113                                                      *
      25.  +      13AD2421  21     1                                                  *
                 14122                                                            *
               14554 21                                                           *
           .   1131                                                                 *
                35.        105       175       245        315        385       455
           0.0       70.        140       210       280       350       420       490

                                          TSP
                              FIGURE 31b.  PM 10 versus TSP.
8*t003
                                         44

-------
 co
 o
      320
      280
      24JET
      2J0
      160
      80.
      40.
     0.0








.
;
*
•
+
•
•

*
,
.
f
.
+
.
.
,
.
+
.
.
.
»
+
.
.
.
.
+
,
,
. 3
. 4*
Y 51
.X

0.0
N= 5733
COR= .SS46
MEAN ST.DEV.
X 72.696 39.553
Y 39.894 24.213
ZERO INTERCEPT
Y = 0.54709*X
***************************************








i
1
i 11
l i i
i i
11 11 l
1 1 21 1
1 1 1
1 212 21313 1 21
2111 1 2112 4421 1 1
21 12221514 11 21
1 121 53221312 1 1
1 12 36 5312 221 11
443328379642341 1 11
112286D79A96235211 1
44488GGEBCA44422 1 11 1
1167GILKPBE836522
46HLV***YCEB634 1 11
3FU*****USI5212131 1 1
7E******OPA45621 2
1CX******QGA1 2 13 1 11 1
50*****«*RD4332 21 11
4U******MB31111111 1
*****OKA42 311 1
**YE7241
21 1
+ + + + + + + +
35. 105 175 245
70. 140 210 280


REGRESSION LINE RES. MS.
X- 1.4453*Y+ 15.036 340.60
Y= .54136*X-f .53966 127.57
REGRESSION LINE RES. MS.
127.6199
* * .+....**. ..+....+*. . . +*
X
*
*
*
Y
*
1 *
*
*
.
1 1
1
*
*
1 *
*
*
1 *
*
*
*
*
1 *
*
*
*
*
*
*
*
*
*
*
*

315 385 455
350 420 490
                                            TSP
                              FIGURE 31c.  DS versus  TSP.
8^003

-------
                                 N-   19
                                 COR= .8985

                                     MEAN    ST.DEV.    REGRESSION LINE    RES.MS.
                                 X   47.6?8   18.444  X» 1.2179*Y+ 3.2985   69.398
                                 Y   36.448   13.607  Y- .66289*X+ 4.8359   37.773

                                       ZERO INTERCEPT REGRESSION  LINE   RES.MS.

                                       Y = 0.75171*X                     38.739


                                         * *+   *  y  **  y     +     +     4.    +   ft +  *
                                          •  ^ • •  • A •   aT****'****^** ••*»•••'»•  • ~ •
         •                                                                        •

   75.J0T  +                                     1                                   +
   67.5
   52.5

0
         .                  1  1
                            1
    37.5  +1                                                     +
                         1 2
                        11
                        1
                      1
    30. J?  +                                                                       +
                            1
         •                                                                       •

         !                i                                                      *
    22.5  +               1                                                       +
    15.0
             12.50     37.50     62.50     87.50     112.5     137.5     162.5
                 25.00     50.00     75.00     100.0     125.0     150.0     175.0


                                          DS
   FIGURE 32a.   Regression analysis for annual concentrations:  PM 10 versus DS.
84003                                   46

-------
                                    N-    14
                                    COR =  .7618

                                        MEAN    ST.DEV.    REGRESSION LINE    RES.MS.
                                    X   85.418   27.227  X=  1.4938*Y+ 25.906    337.00
                                    Y   39.339   13.886  Y-  .38853-X+ 6.6516    87.650

                                         ZERO INTERCEPT  REGRESSION LINE    RES.MS.
                                         Y = 0.45969*X                      85.0163


                                                     •X.*.*	*. . *Y +	+..*.+.«..+*


      75.0  *                                    1                                  +
      57.5
     60.0
     ?2.5

  0
  Q.
     45.0
                                      1    1
                                        1
     37.5  +                             1                                          +
                            11  1
                                1                                                   *
           .                                                                       *
                             1
     30.0  +                                                                       «.
           .                                                                       *




     22.5  +                          1                                             I
     15.0  +                                                                      *
           •"*•*•• •••**«X«*» **• + ••••*•*•**•••«*•,«• + •••• + •••» + »•••^•* *• + •••• + •».• + .
               17.50     52.50     87.50     122.5      157.5      192.5     227.5
          0.000     35.00     70.00     105.0    140.0     175.0     210.0     245.0
                                           TSP
                               FIGURE 32b.  PM 10 versus TSP.
81*003                                    47

-------
   160
   140
   BZ.
   6.7.
   4*.
   23.
.*. .«****.
•
+
•f
+
1
2
"17.50
0.000
N= 25<;
COR* .3*44
MEAN ST.DEV. REGRESSION LINE RES. MS.
X 74.475 27.592 X- 1.3208*/* 20.529 219.29
Y 4,C'.645 17.641 Y= .53991-X+ .63493 89.645
ZERO INTERCEPT REGRESSION LINE RES. MS.
Y = 0.54741*X 89.3398
**w*******************«* * + ** «* + + +. + 4. * +*
X
i
•
+
•
Y
•»•
*
1 1
1
1
1
1 1
1 +
11
1 1
1111
11 1 1
112 11 21 1
1 11 1
12 1 22 1 1 1 *
1 1121211112 2 1 *
1 41355222 121 1
131425233 21 2 *
126A4274122 11 *
1654465 11 1 *
261143112 12 *
11213 311 2 *
1 2 11 11 *
111 *
1 1
1
* « ^ » • **^« • • **• • • •^••••^••« »*••••*••••*••» •*•• ••*• • »•*«•••*••••*•
52.50 87.50 122.5 157.5 192.5 227.5
35.00 70.00 105.0 140.0 175.0 210.0 245.0
TSP
                            FIGURE 32c.  DS versus TSP.
8«f003
                                         48

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*
9
^
.750 +
*
*
*
,
.675 +
m
f
.
^
.600 +
a
»
O.

-------


.65 +
o
.60 +
•
.55 +
.
.50 «•
CO
|HMK »
O
«-« .45 +
S:
«x
.40 +
•
1
.35 +
Y
.30 +
.25 + 1
•A*» • * •*• • • •*• • • •*«
N- 14
COR- .8221
MEAN ST.DEV. REGRESSION LINE RES. MS.
X .49571 .09212 X» .70584-Y+ .15672 .00298
Y .48027 .10729 Y» .95753*X+ .00561 .00404
...-••.... + .... + .... + .... + .... + .... + .... + ....+X... + 	
•
Y
1
1 '.
I
1
+
•
1
*
1
*
1
*
1
I +
*
*
•
1 +
i !
+
•
+
•
•
*
+
           .325      .375      .425      .475      .525      .575       .625
                .350      .400      .450      .500      .550      .600       .650
                                    0.83(DS/TSP)
                 FIGURE 34.  Annual  PM 10/TSP versus 0.83(DS/TSP).
84003
                                       50

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                                   Appendix A
                          SITES USED  IN  THE  ANALYSIS
         Codes are  from  SAROAD (Storage and Retrieval  of Aerometric Data) in
    AEROS Manual Series, Vol.  V:  AEROS Manual  of Codes (1976). EPA-450/2-76-005,
    Research Triangle  Park,  NC.   Asterisks  before names indicate  a county.
           010380003A07
           010380023A07
           010380023A57
           010380026A07
           010570001A07
           012380029A07
           012540001A07
           013200001A07
           020040003A07
           030050110A07
           030440006A07
           030600002A07
           030600002A57
           030600004A07
           030600004A57
           041440001A07
           050500002A07
           050520003A07
           051260002A07
           052220003A07
           052800005A07
           052820002A07
           054020002A07
           054020003A07
           054080002A07
           054180103A07
           055760004A07
           056300003A07
           056535001A07
           056860003A07
           056980004A07
           060080003A07
           060580001A07
           061260001A07
           061260001A57
Birmingham, Alabama
Center Point, Alabama
Mobile, Alabama
Mountian Brook, Alabama
Tarrant City, Alabama
Anchorage, Alaska
Apache Sitegreaves National Forest, Arizona
*Maricopa County, Arizona
Phoenix, Arizona
Little Bock, Arizona
Azusa, California
Bakersfield, California
Chico, California
El Cajon, California
Fresno, California
*Fresno County, California
Livermore, California

Lompoc, California
Los Angeles, California
Pasadena, California
Richmond, California
Rubidoux, California
San Francisco, California
San Jose, California
*Arapahoe County, Colorado
Denver, Colorado
Lakewood, Colorado
84003
                                       51

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81*003
           061820001A07  Pueblo, Colorado
           061820001A57
           062220101A07  *Weld County, Colorado
           070420003A07  Hartford, Connecticut
           070478001A07  *Litchfield County, Connecticut
           080020001A07  Dover, Delaware
           080180001A07  *New Castle County, Delaware
           090020017A07  Washington, District of  Columbia
           090020019A07
           104360035A07  Tampa, Florida
           110200001A07  Atlanta,  Georgia
           110200039A07
           114500017A07  Savannah, Georgia
           120370004A07  Pearl City, Hawaii
           130220003A07  Boise City, Idaho
           141220014A07  Chicago,  Illinois
           141220022A07
           142360010A07  Evahston, Illinois
           148320007A07  *Will County, Illinois
           151520016A07  Gary, Indiana
           152040021A07  Indianapolis, Indiana
           152160002AQ7  Oeffersonville, Indiana
           162500003A07  Harshalltown, Iowa
           162500004A07
           171800011A07  Kansas City, Kansas
           173560007A07  Topeka,  Kansas
           173740012A07  Wichita,  Kansas
           180080002A07  Ashland,  Kentucky
           183090001A07  Okolona,  Kentucky
           191490101A07  Kisatchie National Forest,  Louisiana
           200010001A07  Acadia National Forest,  Maine
           210120001A07  Baltimore,  Maryland
           210120008A07
           210120009A07
           211380002A07  Rockville,  Maryland
           211380007A07
           220240012A07  Boston,  Massachusetts
           220240013A07
           222160011A07  Springfield, Massachusetts
           222160011A57
           222640016A07  Worcester,  Massachusetts
           222640016A57
           231180015A07  Detroit, Michigan
           231180020A07
           241040025A07  Duluth,  Minnesota
           241620007A07   International  Falls, Minnesota
           242260049A07  Minneapolis, Minnesota
           242260051A07
           243300003A07   St. Paul, Minnesota
           251260003A07   Jackson, Mississippi
                                          52

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           260030001A07
           262380002A07
           262950001A07
           264280007A07
           270160005A07
           270310101A07
           271100020A07
           281880028A07
           290480001A07
           290580001A07
           310720005A07
           311380001A07
           312320005A07
           320040001A07
           320090001A07
           330660003A07
           330660010A07
           330660010A57
           332000003A07
           333520001A07
           333520001A57
           334680005A07
           334680011A07
           334680079A07
           340700010A07
           340945101A07
           341160006A07
           341160006A57
           341160101A07
           341160102A07
           341160102A57
           360060014A07
           361220020A07
           361300013A07
           361300021A07
           361300041A07
           361460001A07
           361660014A07
           363080010A07
           364140002A07
           364340005A07
           364340005A57
           366420012A07
           366420012A57
           367760002A07
           372200035A07
           380420111A07
           380500104A07
           380560013A07
           381460D15A07
           390100064A07
           390100068A07
Affton, Missouri
Kansas City, Missouri
Mark  IWain National  Forest,  Missouri
St. Louis,  Missouri
Butte - Silver  Bow,  Montana
Custer National Forest,  Montana
*Missoula  County, Montana
Omaha, Nebraska
Beno, Nevada
Winneroucca, Nevada
Camden, New Jersey
*Essex County,  New Jersey
Jersey City, New Jersey
Albuquerque, New Mexico
Bayard, New Mexico
Buffalo, New York
*Erie County, New York
Lackawanna, New York

New York City, New York
Charlotte, North Carolina
Croatan National Forest, North Carolina
Durham, North Carolina
Akron, Ohio
Cincinnati, Ohio
Cleveland, Ohio
Columbus, Ohio
Dayton, Ohio
Ironton, Ohio
Medina, Ohio
Middletown, Ohio

Steubenville, Ohio

Youngstown, Ohio
Oklahoma City, Oklahoma
*Crook County, Oregon
Deschutes, Oregon
Eugene, Oregon
Portland, Oregon
*Allegheny County, Pennsylvania
84003
                                       53

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390400002A07  Avalon, Pennsylvania
390780725A07  Bethlehem, Pennsylvania
390780725A57
396620001A07  North Braddock, Pennsylvania
397140003A07  Philadelphia, Pennsylvania
397140003A57
397140019A07
397140020A07
397140023A07
397140024A07
397140032A07
397140036A07
397140037A07
397140037A57
397140038A07
397260021A07  Pittsburgh, Pennsylvania
410300012A07  Providence, Rhode Island
420560003A07  *Charleston County, South Carolina
440380006A07  Chattanooga, Tennessee
442540006A07  Hurfreesboro, Tennessee
451310050A07  Dallas, Texas
451700002A07  El Paso,  Texas
451710004A07  *E1 Paso  County, Texas
452330024A07  'Harris County, Texas
452560034A07  Houston,  Texas
454715001A07  Seabrook, Texas
460520001A07  Hagna, Utah
460920001A07  Salt  Lake City, Utah
470265101A07  Green Mountain National Forest, Vermont
480200020A07  'Arlington County, Virginia
481440005A07  'Hampton  County, Virginia
481560002A07  Hopewell, Virginia
482140007A07  Norfolk,  Virginia
482630001A07  Reston, Virginia
482660002A07  Richmond, Virginia
491840057A07  Seattle,  Washington
491840057A57
491840073A07
492040013A07  Spokane,  Washington
500280004A07  Charleston, West Virginia
502000002A07  Weirton,  West Virginia
502120002A07  Wheeling, West Virginia
510240002A07  Beloit, Wisconsin
510490001A07  Chequaroegon National Forest, Wisconsin
511180009A07  Green Bay, Wisconsin
                            54

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                        Appendix B

         SITE CLASSIFICATIONS ACCORDING TO CLIMATE
              ARID

030050110A07  Apache Sitegreaves National  Forest,  Arizona
030600004A07  Phoenix, Arizona
030600004A57
052800005A07  Fresno, California
061820001A07  Pueblo, Colorado
061820001A57
290580001A07  Winnemucca, Nevada
451710004A07  El Paso County, Texas

              WEST COAST

051260002A07  Chico, California
052220003A07  El Cajon, California
054020002A07  Livermore, California
054180103A07  Los Angeles, California
012380029A07
104360035A07
114500017A07
142360010A07
152160002A07
173740012A07
211380007A07
222160011A07
222160011A57
222640016A07
222640016A57
251260003A07
270160005A07
270310101A07
271100020A07
281880028A07
334680079A07
367760002A07
390100064AQ7
410300012A07
420560003A07
500280004A07
502000002A07
510240002A07
OTHER

Mobile, Alabama
Tampa, Florida
Savannah, Georgia
Evanston, Illinois
Jeffersonville, Indiana
Wichita, Kansas
Rockville, Maryland
Springfield, Massachusetts

Worcester, Massachusetts

Jackson, Mississippi
Butte - Silver Bow, Montana
Custer National Forest, Montana
Missoula County, Montana
Omaha, Nebraska
New York City, New York
Youngstown, Ohio
Allegheny County, Pennsylvania
Providence, Rhode Island
Charleston County, South Carolina
Charleston, West Virginia
Weirton, West Virginia
Beloit, Wisconsin
                            55

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                                   Appendix C

   24-HOUR SITE CASES OMITTED  BECAUSE AT LEAST ONE  OF THE FOLLOWING
   RATIOS WAS GREATER THAN  1.05:   PM 10/DS, PM 10/TSP, DS/TSP
010380023A0782 529
010380023A0782 8  3
010570001A0780 5  3
010570001A0780 5  9
010570001A0780 515
010570001A0780 521
010570001A0780 527
010570001A0780 626
010570001A0780 7  8
010570001A0780 714
010570001A0780 720
010570001A07801117
010570001A0781 8  2
030600002A0781 6  3
030600002A0781 621
030600002A0782 312
052220003A0782 926
052820002A0780 527
056535001A0782 411
056860003A0782 821
062220101A0782 6  4
062220101A0782 616
062220101A0782 8  9
062220101A0782 926
062220101A078210U
062220101A07821020
062220101A0782H13
062220101A07821119
062220101A078212  1
062220101A07821213
062220101A07821225
070478001A0782 628
090020017A0781 913
090020017A0781 919
090020017A078110 1
090020017A07811013
090020017A078111  6
090020017A07811118
130220003A07821231
141220022A0782 616
152040021A07821119
162500003A0782 312
162500004A0780 924
162500004A07801111
162500004A07801117
162500004A07801223
200010001A0782 8 3
200010001A0782 827
210120009A07801123
210120009A078110 7
211380007A0782 920
220240012A0780 626
220240013A0780 8 1
220240013A0781 9 7
242260051A078012 5
260030001A0780 831
290580001A0780 7 2
310720005A0782 8 3
311380001A0781 329
311380001A07811230
311380001A0782 228
311380001A0782 4 5
311380001A0782 8 3
320040001A0782 216
320090001A07801217
32.9.99.?.?91A.97Q1 4 4
320090001A0781 8 8
320090001A0781 820
320090001A0781 9 7
330660003A078010 6
330660003A07801111
330660003A078012 5
330660003A0781 1 4
330660003A0781 122
330660003A0781 2 3
330660010A07821231
332000003A0780 8 7
332000003A0780 813
332000003A0780 819
332000003A0780 825
332000003A0780 831
332000003A0780 9 6
332000003A0780 918
332000003A0780 930
332000003A078010  6
332000003A07801012
332000003A07801024
332000003A078011  5
332000003A07801111
332000003A07801117
 332000003A07801123
 332000003A07801211
 3 3 2000003A07 801223
 332000003A0781  221
 333520001A0781  522
 334680005A0781  9  7
 334680079A0781  9  7
 340700010A07821113
 340700010A078212  1
 340700010A078212  7
 340700010A07821213
 340700010A07821219
 340700010A07821231
 341160006A07821231
 341160006A578212  1'
 341160101A0780 7  2
 341160102A0781 919
 341160102A0781 925
 341160102A0782 4  5
361300013A0781 826
361300021A0780 7 8
363080010A07811112
363080010A0782 2 4
366420012A0782 5 5'
366420012A0782 8 3'
366420012A07821219
367760002A078212 7
367760002A07821225
380500104A0780 415
380500104A0780 5 9
380500104A0780 521
380500104A07801129
380560013A0780 9 6
380560013A0780 918
381460015A0780 4 3
381460015A0780 415
381460015A0780 427
381460015A0780 620
390780725A0782 210
396620001A0782 210
396620001A0782 3 6
396620001A0782 5 5
396620001A0782 722
397140003A0782 722
397140003A07821125
397140003A5782 3 6
397140003A5782 716
397260021A0782 7 4
397260021A0782 716
451700002A0780 421
451700002A0780 614
454715001A0781 8 2
460520001A0781 721
460520001A0782 1 5
481S60002A0781 416
491840057A07821231
491840073A0780 4 9
492040013A0782 7 4
510240002A0782 216
511180009A0782 4 5
84003
                                          56

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                                   Appendix D

          ANNUAL  SITE CASES OMITTED BECAUSE AT LEAST ONE OF THE FOLLOWING
          ANNUAL  RATIOS WAS GREATER THAN 1.05:  PM 10/DS, PM 10/TSP, DS/TSP
                                332000003AQ781
                                050520003A0782
                                052800005ft0782
                                061820001A0782
                                062220101A0782
                                130220003A0782
                                290480001A0782
                                381460015A0782
                                460520001A0782
                                460920001A0782
84003
                                       57

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                                    TECHNICAL REPORT DATA
                             (Please read Instructions on the reverse before completing)
1. REPORT NO.
                              2.
                                                             3. RECIPIENT'S ACCESSION NO.
4. TITLE AND SUBTITLE
  An Update On The Use of Particulate Ratios To
  Assess Likely PM^p Attainment  Status
                                                             5. REPORT DATE
                                                                June 1984
                                                             6. PERFORMING ORGANIZATION CODE
7. AUTHOR(S)
  A.  D. Thrall, A.  B. Hudischewskyj
                                                             8. PERFORMING ORGANIZATION REPORT NO.
9. PERFORMING ORGANIZATION NAME AND ADDRESS
  Systems Applications, Incorporated
  101 Lucas Valley  Road
  San Rafael, California  94903
                                                             10. PROGRAM ELEMENT NO.
                                                             11. CONTRACT/GRANT NO.
12. SPONSORING AGENCY NAME AND ADDRESS
  U.S. Environmental Protection  Agency
  Office of Air  Quality Planning and Standards
  Research Triangle Park, North  Carolina  27711
                                                             13. TYPE OF REPORT AND PERIOD COVERED
                                                             14. SPONSORING AGENCY CODE
15. SUPPLEMENTARY NOTES

  EPA Project Officer:  Edwin L. Meyer, Jr.
16. ABSTRACT
       This report describes results of statistical analyses of  PM15',  TSP and PM10
  data collected  during 1980-82  at collocated sites in the National Inhalable
  Particulate Monitoring Network.   Results from  this report have been used to support
  the use of national distributions for PM10/TSP ratios.  Selection of a distribution
  of PMio/TSP ratios is an inherent assumption made in order to  estimate nonattainment
  probabilities for PM10 at sites  collecting only TSP data.
                                KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
                                               b.lDENTIFIERS/OPEN ENDED TERMS
                                                                          c.  COSATI Field/Group
   PM
   TSP
   IP
   Monitoring
   PM1Q/TSP Ratios
   Nonattainment probability
 8. DISTRIBUTION STATEMENT
                                               19. SECURITY CLASS (This Report)
                                                                           21. NO. OF PAGES
                                                                                  63
                                               20. SECURITY CLASS (This page)
                                                                          22. PRICE
EPA Form 2220—1 (Rev. 4-77)   PREVIOUS EDITION is OBSOLETE

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