oEPA United States Environmental Protection Agency Industrial Environmental Research EPA 600 2-79-210g Laboratory December 1979 Cincinnati OH 45268 Research and Development Status Assessment of Toxic Chemicals Hexachlorobenzene ------- RESEARCH REPORTING SERIES Research reports of the Office of Research and Development, U.S. Environmental Protection Agency, have been grouped into nine series These nine broad cate- gories were established to facilitate further development and application of en- vironmental technology Elimination of traditional grouping was consciously planned to foster technology transfer and a maximum interface in related fields. The nine series are: 1. Environmental Health Effects Research 2 Environmental Protection Technology 3 Ecological Research 4. Environmental Monitoring 5 Socioeconomic Environmental Studies 6. Scientific and Technical Assessment Reports (STAR) 7. Interagency Energy-Environment Research and Development 8, "Special" Reports 9. Miscellaneous Reports This report has been assigned to the ENVIRONMENTAL PROTECTION TECH- NOLOGY series. This series describes research performed to develop and dem- onstrate instrumentation, equipment, and methodology to repair or prevent en- vironmental degradation from point and non-point sources of pollution. This work provides the new or improved technology required for the control and treatment of pollution sources to meet environmental quality standards. This document is available to the public through the National Technical Informa- tion Service. Springfield, Virginia 22161. ------- EPA-600/2-79-210g December 1979 STATUS ASSESSMENT OF TOXIC CHEMICALS: HEXACHLOROBEN Z ENE by T. R. Blackwood Monsanto Research Corporation Dayton, Ohio 45407 and T. G. Sipes Radian Corporation Austin, Texas 78766 Contract No. 68-03-2550 Project Officer David L. Becker Industrial Pollution Control Division Industrial Environmental Research Laboratory Cincinnati, Ohio 45268 INDUSTRIAL ENVIRONMENTAL RESEARCH LABORATORY OFFICE OF RESEARCH AND DEVELOPMENT U.S. ENVIRONMENTAL PROTECTION AGENCY CINCINNATI, OHIO 45268 ------- DISCLAIMER This report has been reviewed by the Industrial Environmental Research Laboratory - Cincinnati, U.S. Environmental Protection Agency, and approved for publication. Approval does not signify that the contents necessarily reflect the views and policies of the U.S. Environmental Protection Agency, nor does mention of trade names or commercial products constitute endorsement or recommendation for use. 11 ------- FOREWORD When energy and material resources are extracted, processed, converted, and used, the related pollutional impacts on our environment and even on our health often require that new and increasingly more efficient pollution control methods be used. The Industrial Environmental Research Laboratory - Cincinnati (lERL-Ci) assists in developing and demonstrating new and improved methodologies that will meet these needs both effi- ciently and economically. This report contains a status assessment of the air emissions, water pollution, health effects, and environmental significance of hexachlorobenzene. This study was conducted to provide a better understanding of the distribution and characteristics of this pollutant. Further information on this subject may be obtained from the Organic Chemicals and Products Branch, Industrial Pollution Control Division. Status assessment reports are used by lERL-Ci to communi- cate the readily available information on selected substances to government, industry, and persons having specific^needs and interests. These reports are based primarily on data from open literature sources, including government reports. They are indicative rather than exhaustive. David G. Stephan Director Industrial Environmental Research Laboratory Cincinnati 111 ------- ABSTRACT Hexachlorobenzene (HCB) can be produced as either a waste or a byproduct from fourteen types of industrial processes. Although 1,450 metric tons were produced in 1975, present HCB production and use quantities are unknown. Emissions from manufacture are unknown. Residues from the manufacture of chlorinated solvents and pes- ticides represent the most prominent source of HCB, and the emissions are estimated at 1,000 to 3,900 metric tons/yr. Air and water, near waste-containing-HCB disposal sites have been observed to contain up to 24 yg/m3 and 90 mg/m3 of HCB, respec- tively. Soil samples near these same sites contain from 11 yg/g to 3,000 yg/g. Due to the persistence of HCB, levels do not decline rapidly. Present control methods consist of incineration, deep-well injec- tion, and landfill. Incineration is most effective at 1,300°C and 0.25 s. While these control methods could be applied to current waste streams, environmental pollution from past HCB waste holding areas may represent a continuing problem because HCB is stable and sublimes in air. The only existing regulations on HCB are prohibition of ocean dumping and limiting HCB in animal carcasses to 0.5 ppm. Future studies should include confirmation of production quanti- ties and use along with emissions estimates, concentrations in pesticides and chlorinated solvents, and methods for removing HCB from wastes such as sludges and wastewater. HCB has been used as a fungicide in the United States with more than 6.9 metric tons used in 1971. Concern over the safety of HCB use, in late 1972, may have eliminated continued use of HCB in grain or food chain products. This report was submitted in partial fulfillment of Contract 68-03-2550 by Monsanto Research Corporation under the sponsorship of the U.S. Environmental Protection Agency. This report covers the period November 1, 1977 to December 31, 1977. The work was completed as of January 20, 1978. IV ------- CONTENTS Foreword iii Abstract iv Conversion Factors and Metric Prefixes vi Acknowledgement vii 1. Introduction 1 2. Summary 2 3. Source Description 5 Chemical and physical properties 5 Production 5 Process description 6 Uses 8 Transportation 8 4. Environmental Significance and Health Effects .... 9 Environmental significance 9 Health effects 13 5. Control Technologies 15 6. Regulatory Action in Progress 17 References 18 ------- CONVERSION FACTORS AND METRIC PREFIXES1 CONVERSION FACTORS To convert from Degree Celsius (°C) Kilogram (kg) Kilometer2 (km2) Meter3 (m3) Meter3 (m3) Metric ton Pascal (Pa) to Degree Fahrenheit (°F) Pound-mass (pound-mass avoirdupois) Mile2 Foot3 Gallon (U.S. liquid) Pound-mass Pound-force/inch2 (psi) Multiply by t« = 1.8 t° + 32 2.204 3.860 x 10"1 3.531 x 101 2.642 x 102 2.205 x 103 1.450 x IQ-1* METRIC PREFIXES Prefix Symbol Multiplication factor Centi Kilo Milli c k m io-2 103 io-3 Example 1 1 1 cm = kg = mm = 1 1 1 x x X 10- 103 10" 2 3 meter grams meter Standard for Metric Practice. ANSI/ASTM Designation: E 380-76e, IEEE Std 268-19,76, American Society for Testing and Materials, Philadelphia, Pennsylvania, February 1976. 37 pp. VI ------- ACKNOWLEDGEMENT This report was assembled for EPA by Radian Corporation, Austin, TX, and Monsanto Research Corporation, Dayton, OH. Mr. D. L. Becker served as EPA Project Officer, and Dr. C. E. Frank, EPA Consultant, was principal advisor and reviewer. VII ------- SECTION 1 INTRODUCTION Hexachlorobenzene (HCB) is toxic to man and has been shown to cause liver tumors and dysfunction in hamsters. It is only marginally produced in the United States and generally as a byproduct of other chlorinated hydrocarbons manufacture. Con- cern over HCB in the environment was heightened by high levels found in beef cattle in 1972. The purpose of this report is to summarize existing information on the production, uses, emis- sions, health effects, control technology, and regulatory action with respect to HCB. The fate and route of HCB in the environ- ment is also summarized. ------- SECTION 2 SUMMARY Serious incidents of environmental contamination have been observed involving hexachlorobenzene (HCB) wastes and products. Despite steps to reduce environmental discharges of hexachloro- benzene, environmental contamination persists. HCB is toxic to man and presents a hazard in the environment. It is highly resistant to chemical, biological, and physical degradation and is persistent throughout the environment. It is apparently accumulated in food chains. There are recent reports of the occurrence of hexachlorobenzene in human adipose tissues (95% of those sampled), the food supply, industrial effluents, and drinking water. Hexachlorobenzene has recently been shown to be a carcinogen in hamsters. Its chronic toxic effects are exhi- bited by liver dysfunction in these animals. Hexachlorobenzene is not a significant item of commerce and is not produced as a direct product of a commercial process. It is a specialty chemical which may be recovered as a byproduct. Whether there are any current uses of HCB or whether byproduct HCB is currently recovered for commercial use or distribution is unknown. In 1975, 1,450 metric tons3 were reported to be pro- duced in the United States. It has been observed that HCB may transport through the environ- ment due to sublimation from wastes containing HCB. For this reason, waste disposal practices are under scrutiny. Industrial wastes from manufacture of chlorinated hydrocarbons in the solvents and pesticides industries are the major source of HCB emissions. Emissions estimates range from 1,000 to 3,900 metric tons/yr. These emissions could be reduced by incineration of wastes. Adequate disposal methods appear to be available. A management plan to define regulatory action for control of HCB emissions would have to be directed toward waste streams from organic solvent and pesticide manufacture. Table 1 summarizes important findings of this assessment on emission sources, extent of the problem, control methods, and regulatory action. al metric ton = 106 grams; conversion factors and metric system prefixes are presented in the prefatory pages of this report. 2 ------- TABLE 1. HEXACHLOROBENZENE Emission source Extent of problem Control methods Regulatory action u> Production of hexachloro- benzene Waste disposal at chlorine, carbon tetrachloride, per- chloroethylene, trichloro- ethylene, Dacthal, atrazine, propazine, simazine, vinyl chloride, pentachloronitro- benzene, hexachloroethane, diethyl tetrachlorotere- phthalate, mirex, and other chlorinated hydrocarbon pro- ducing plants. Uses include: grain fungi- cide, pyrotechnic compound chemical intermediate, wood preservative, feedstock for pentachlorophenol, and pep- tizing agent in rubber manufacture. Over 100 sites across U.S. may have produced HCB as a by-product or waste. Airconcentrations of 1 yg/m3 to 24 yg/m3, observed waste disposal sites. Water concentrations of 1 mg/m3 to 90 mg/m3 observed in wastewaters leaving these plants. Soil samples taken beyond plant boundaries varied from 11 yg/g to 3,000 yg/g. From 1,000 to 3,900 metric tons of HCB are estimated to be emitted per year (1972 to 1977). 6.9 metric tons used as grain fungicide in 1971. Incineration at high tempera- ture (l,300°c and 0.25 s). Deep-well injection. Landfill using barriers and 1 m to 2 m of cover. In 1973, an interim tolerance of 0.5 ppm was set for HCB con- tent in animal car- casses by the EPA. The state of Louisiana required better solid waste disposal practices. Dacthal and other pes- ticides containing HCB are under review by EPA. Ocean dumping of HCB- laden wastes is prohibited. Designated a priority pollutant under the Federal Water Pollu- tion Control Act. ------- Based upon information presented in this report, the following items need to be considered in future studies: • Determination of the concentration of HCB in various pesticide products such as atrazine, propazine, simazine, Dacthal, pentachloronitrobenzene, or mirex. • Methods for removing HCB from wastes such as sludges and process wastewater. • Identification of the amount of HCB used in dye manufac- ture, organic synthesis, and rubber manufacture as well as its use as a grain fungicide and wood preservative. • Identification and production quantity of locations, if any, which presently manufacture HCB. • The potential for chronic effects at low-level exposure of hexachlorobenzene. • Methods to contain or treat existing HCB which has been disposed as waste in landfill from chlorinated solvents manufacture. ------- SECTION 3 SOURCE DESCRIPTION CHEMICAL AND PHYSICAL PROPERTIES Hexachlorobenzene or perchlorobenzene (Cede) is a white powder that is soluble in benzene, ethyl ether, and chloroform; spar- ingly soluble in cold alcohol; and insoluble in water. It has a molecular weight of 284.80, a melting point of 227°C, boiling point of 325°C, and flash point of 243°C. It sublimes rapidly at ambient temperatures, 0 to 30°C (1, 2). PRODUCTION Hexachlorobenzene (HCB) is a specialty chemical recovered as a byproduct from proprietary chlorinated hydrocarbon processes (3). Two companies produced HCB in 1976 (4). These were Hummel Chemical Co., Inc., in South Plainfield, New Jersey and Dover Chemical Corp. in Dover, Ohio. Stauffer Chemical Company has also produced HCB in recent years. Recent information indicates that HCB is no longer produced at these sites (5); however, the 1977 Buyers Guide issue of "Chemical Week" lists three producers (1) Stecher, P. G., M. Windholy, D. S. Leathy, D. M. Bolton, and L. G. Eaton. The Merck Index, Eighth Edition. Merck and Company, Inc., Rahway, New Jersey, 1968. (2) Hawley, G. G. Condensed Chemical Dictionary. Eighth Edition. Van Nostrand Reinhold Co., New York, New York, 1971. (3) Mumma, C. E., and E. W. Lawless. Survey of Industrial Processing Data. Task 1 - Hexachlorobenzene and Hexa- chlorobutadiene Pollution from Chlorocarbon Processing. EPA-560/3-75-003, U.S. Environmental Protection Agency, Washington, D.C., June 1976. 187 pp. (4) 1977 Directory of Chemical Producers United States of America. Stanford Research Institute, Menlo Park, Cali- fornia, 1977. 1059 pp. (5) 1977 Directory of Chemical Producers United States of America. January to September Supplement. Stanford Research Institute, Menlo Park, California, 1977. 73 pp. ------- of HCB: Dover Chemical Corporation; Rhodia, Incorporated, Chemi- cal Division; and Stauffer Chemical Company, Industrial Chemicals Division (6). Only occasional and fragmentary production statistics are pub- lished for higher chlorobenzenes, such as hexachlorobenzene. A data base prepared by Radian Corporation listed HCB production as 1,450 metric tons in 1975 (7). PROCESS DESCRIPTION Methods for production of HCB are proprietary and limited infor- mation is available. At Stauffer Chemical in Louisville, Ken- tucky, HCB has been recovered from a byproduct that contains 80% HCB. The remainder of the tar is recycled to the process. Processes for direct production of HCB use either benzene or hexachlorocyclohexane (C6H6Cl6) as the raw materials. In one of the basic processes, benzene is reacted with excess chlorine in the presence of ferric chloride at 150°C to 200°C as shown in Figure 1. The reaction products are scrubbed with water to remove hydrogen chloride. The gaseous chlorobenzenes are recycled to the initial reactor. The reaction products are cooled to 100°C to allow the HCB to crystallize (3). A contin- uous process for HCB production by this method has been patented by Olin Mathieson Corporation (8). In another major process, isomers of hexachlorocyclohexane are refluxed with sulfuryl chloride (S02C12) or chlorosulfonic acid (HC1S03). A ferric chloride or an aluminum chloride catalyst is employed. Reaction temperatures are 130°C to 200°C. The reaction mixture is cooled to crystallize the HCB, which is fil- tered, centrifuged, and washed. A schematic for this process is given in Figure 2 (3). Hexachlorobenzene is formed as a byproduct of hexachloroethane production and is also produced as one of a group of coproducts formed when ethylene is substituted for methane in the Huls process for carbon tetrachloride production (8). In addition, HCB can be produced as a byproduct, waste, or impurity with the following chemicals: chlorine, perchloroethylene, trichloro- ethylene, Dacthal, atrazine, propazine, simazine, vinyl chlo- ride, pentachloronitrobenzene, and Mirex (3). (6) 1977 Buyers Guide. Chemical Week, 119(17), 1976. (7) Garner, D. N. and P. S. Dzierlenga. Organic Chemical Pro- ducers' Data Base Program. Radian Corporation, Austin, Texas, 1976. (8) Kirk-Othmer Encyclopedia of Chemical Technology, Second Edi- tion, Vol. 5. John Wiley & Sons, Inc., New York, New York, 1964. 884 pp. 6 ------- BYPRODUCT HCI CI2 PRIMARY REACTOR WITH FeCI3 AS CATALYST CRYSTALLIZER PARTIALLY CHLORINATED BENZENES SEPARATION DRYING PACKAGING SHIPMENT OF SHIPMENT OF LESS CHLORINATED HEXACHLOROBENZENE BENZENES PENTACHLOROBENZENE, ETC. Figure 1. Production schematic for hexachlorobenzene by chlorination of benzene and chlorobenzenes (3). W<6 ISOMERS * CHLOROSULFONIC ACID OR SULFURYL CHLORIDE "~ REFLUX- CONDENSER - REACTOR WITH FeCI3 AS CATALYST COOLER FILTER DRYING PACKAGING - SHIPMENT HEXACHLOROBENZENE Figure 2. Production schematic for hexachlorobenzene from hexachlorocyclohexane (3). ------- USES Hexachlorobenzene has been used in the past as a fungicide to control wheat bunt and smut fungi of grains. The U.S. Department of Agriculture estimated that about 6.9 metric tons of HCB was used in 1971 as a grain fungicide, principally in Washington, Oregon, and California (9). It is not clear whether HCB is still used as a grain fungicide. Several other uses for HCB have been reported, but may not be current. These applications include the use of HCB as an addi- tive for pyrotechnic compounds, a porosity controller, a chemical intermediate in dye manufacture and organic synthesis, and a wood preservative. Hexachlorobenzene is also reportedly used as a peptizing agent in nitroso and styrene type rubber manufactur- ing. It has been used as a feedstock in the production of pen- tachlorophenol, but this process is no longer in use in the United States. Current estimates of the amounts of HCB used are unavailable (3, 8, 10, 11, 12). TRANSPORTATION HCB wastes are transported by forklift truck, pipeline, heated tank trucks, and railcars. Prior to ultimate disposal they are stored as solid waste cubes under plastic cover and in water- covered lagoons (13). Diamond Shamrock in Deer Park, Texas, transports HCB-containing wastes to off-site disposal facilities. The wastes are packaged in sealed containers before being shipped (3). HCB powder used as a fungicide would have to be transported from its production site to the location where it is used, most likely in small drums. Improper containment during transport can result in HCB emissions into the air via sublimation or dust kickup. HCB emitted during transportation can contaminate soil and water and settle on the surface of vegetation (10). (9) Assessing Potential Ocean Pollutants. National Academy of Sciences, Washington, D.C., 1975. (10) Environmental Contamination from Hexachlorobenzene. EPA-560/6-76-014, U.S. Environmental Protection Agency, Washington, D.C., July 1973. 34 pp. (11) Wilkins, G. E. End Use Patterns for Significant Organic Chemicals. Radian Corporation, Austin, Texas, July 21, 1976. (12) Chemical Origins and Markets. G. M. Lawler, ed. Stanford Research Institute, Menlo Park, California, 1967. (13) Journal of Hazardous Materials, 1 (4):343-359, March 1977. ------- SECTION 4 ENVIRONMENTAL SIGNIFICANCE AND HEALTH EFFECTS ENVIRONMENTAL SIGNIFICANCE Sources of Emissions Fourteen types of industrial processes produce HCB as a waste or byproduct (13). In processes where hexachlorobenzene is re- covered as a byproduct, HCB is recovered or recycled to the process. The majority of HCB containing wastes is produced in pesticide and chlorinated solvent manufacture, Processes for the production of perchloroethylene, trichloroethylene, carbon tetrachloride, other chlorinated hydrocarbons, and pesticides produce HCB containing wastes. This waste is in the form of a heavy, tarry residue which contains chlorinated hydrocarbons including HCB. The wastes from perchloroethylene and carbon tetrachloride production reportedly contain 10% to 15% HCB and are disposed in waste dumps. The dumps are then sources of HCB which may be leached or sublimed into the environment. Production of chlorine gas by electrolysis of NaCl with a graph- ite anode and mercury cathode may also release HCB. In addition, HCB is contained as a significant contaminant in the pesticides diethyl tetrachloroterephthalate and pentachloronitrobenzene (3, 9, 10). It may also be present in other pesticides. Since HCB sublimes, the use of pesticides may be an important source of HCB. No confirmatory data are available. Estimated production of HCB wastes is given in Tables 2 and 3. According to one estimate, production of perchloroethylene accounts for about 72% of all HCB formed in the United States and production of carbon tetrachloride, perchloroethylene and trichloroethylene accounts for 89% (3). Results published in 1977 (Table 3) indicate that chlorinated solvent production accounts for about 60% of HCB wastes (13). Hexachlorobenzene can also be emitted directly into the air from production processes for HCB (10); however, one study shows waste holding areas were often the most significant emission source within the plant area (3). ------- TABLE 2. ESTIMATED TOTAL QUANTITY OF HEXACHLOROBENZENE CONTAINED IN U.S. INDUSTRIAL WASTES, BYPRODUCTS, AND PRODUCTS IN 1972 (3) Estimated HCB U.S. production, produced, metric tons Product 1,000 metric tons High Low Perchloroethylene 334 1,590 794 Trichloroethylene 194 204 104 Carbon tetrachloride 453 182 90 Chlorine 8,660 177 73 Dacthal 0.9 45 36 Vinyl chloride 2,040 12 0 Atrazine, propazine, simazine 51 42 Pentachloronitrobenzene 1.4 3 1 Mirex 0.4 0.9 0.4 TOTAL -a 2,200 1,010 Not applicable. TABLE 3. ANNUAL VOLUME OF HCB WASTES FROM PESTICIDES AND CHLORINATED SOLVENT INDUSTRIES IN 1977 (13) Annual production of HCB wastes, Industry Products metric tons Pesticide Dacthal, pentachloronitrobenzene, 1,500 mirex, simazine, atrazine, propazine. Industrial Chlorinated solvents. 2,400 organic chemicals Environmental Levels The concentration of HCB in various media is primarily due to solid- or semi-liquid wastes containing HCB. Although contami- nated soil has been observed, it is believed to be caused by particulate or vapor HCB in the air (14). In 1975, 46% of the (14) Li, R. T., J. L. Spigarelli, and J. E. Going. Sampling and Analysis of Selected Toxic Substances. Task 1A - Hexachlo- robenzene. EPA-560/6-76-001, U.S. Environmental Protection Agency, Washington, D.C., June 1976. 166 pp. 10 ------- soil samples collected at 26 locations along a 240 km transect in Louisiana were contaminated with HCB at levels from 20 ppb (parts per billion) to 440 ppb. Although water samples generally con- tained less than 3 ppb, one sample downstream of an industrial discharge contained 90 ppb. Air immediately adjacent to waste dumps has shown concentrations from 1.0 yg/m3 to 24 yg/m3. Most of the hexachlorobenzene appeared to be associated with particu- late matter although some was found in the gas phase. This may have resulted from volatilization of solid material. Samples collected from pastureland near a known production site revealed concentrations in the vegetation from 0.01 ppm (parts per mil- lion) to 630 ppm and in the soil from 0.01 ppb to 300 ppb (10). In 1974 and 1975, soil, water, and organism samples were col- lected periodically from sites in southeastern Louisiana, with emphasis along the Mississippi River and an industrial region of known contamination near Geismar, Louisiana. Maximum HCB con- centrations in water from the two areas were 90 mg/m3 and 75 mg/m3 (ppb). Maximum concentrations in soil were 874 yg/kg and 53,130 yg/kg (ppb) (15). Sampling tests at nine industrial plants representing six indus- tries (perchloroethylene, trichloroethylene, carbon tetrachloride, chlorine, triazine herbicides, and pentachloronitrobenzene) showed HCB levels as high as 24 yg/m3 in the air and 306 mg/m3 in open wastewater treatment ponds. Levels of HCB in the soil within plant boundaries were greater than 1,000 yg/g at three of the plants sampled. The maximum concentration found in air beyond these plant sites was 0.36 yg/m3; however, 3 yg/m3 was detected at the boundary of another plant. Soil in a cornfield adjacent to another plant site showed a concentration of 11 yg/g and more than 3,000 yg/g was detected along the boundary road of yet another plant. The observed HCB concentration in water beyond plant property was more than 1 mg/m3 at two plants (14). Hexachlorobenzene has been detected in rivers and chemical efflu- ents at various locations (16). Hexachlorobenzene residues have been found in soil, wildlife, fish, and food samples collected from all over the world. In the United States, residues have been reported in birds and bird eggs collected from Maine to Florida, duck tissues collected from across the country, and fish (15) Laseter, J. L., C. K. Bentell, A. L. Lacka, D. G. Holmquist, D. B. Condie, J. W. Brown, and R. L. Evans. An Ecological Study of Hexachlorobenzene (HCB). EPA-560/6-76-009, U.S. Environmental Protection Agency, Washington, D.C., April 1976. 74 pp. (16) Shackelford, W. M. and L. H. Keith. Frequency of Organic Compounds Identified in Water. EPA-600/4-76-062, U.S. Environmental Protection Agency, Athens, Georgia, December 1976. 629 pp. 11 ------- and fish eggs from the East Coast and Oregon. Animal foods, including chicken feed, fish food, and general laboratory feeds, have been found to contain residues. The frequency of detection of residues in domestic meats has been steadily increasing since 1972, in part because of closer scrutiny. In 1972, beef cattle carcasses in Louisiana were found to contain concentrations as high as 1.5 ppm. The chemical has been detected in trace amounts in only two drinking water supplies. EPA's monitoring of human adipose tissues collected from across the United States reveals that about 95% of the population has trace residues (10). More information on levels of HCB residues found in aquatic organizms and man is available in reports by the National Academy of Sciences (9) and the Midwest Research Institute (3). Reactions in the Environment Hexachlorobenzene is a very stable, unreactive, and mobile com- pound. It apparently does not undergo photochemical reactions in the atmosphere, and it is not hydrolyzed in aqueous solutions. There is no evidence that it is broken down by physical or chemi- cal processes in the environment. It also appears to be largely immune to the biological degradation process. Studies indicate that it is not metabolized to any significant extent, but penta- chlorobenzene is a possible metabolic derivative (9). Since hexachlorobenzene is volatile over water, even at low temperatures, codistillation is a method of dispersal. HCB also sublimes readily and will evaporate if exposed to air under adequate ventilation (9). It readily vaporizes from soil into the air; emissions to the air can in turn contaminate more soil (10). Aerial dispersal may be the major pathway for HCB entering the marine environment (9). Population Exposed Hexachlorobenzene has been produced at Dover, Ohio, (estimated population 11,200) South Plainfield, New Jersey, (population 21,300); Louisville, Kentucky (population 706,000) and possibly at other locations. Because of the persistence of HCB, resi- dents of these areas could be exposed to HCB residues resulting from emissions from the plants even if the plants are not cur- rently producing HCB. Plants that produce HCB as a byproduct or waste are located at over 100 sites throughout the country. Locations and production capacities of these plants are given in a study by Midwest Research Institute (3). (Most of these sites are located in highly industrialized complexes in the South and eastern United States.) Residents of areas near plants that produce HCB as a byproduct or waste may be exposed to HCB emitted into the air or contained in soil. Occupational exposure to HCB could affect 12 ------- workers at these plants as well as at the plants that directly produce HCB. HCB has been used as a grain fungicide, especially in Washington, Oregon, and California (9). Because of the persistence of HCB, residues of HCB could exist in soil where treated seed has been planted. The population may also be exposed to HCB from the use of pesticides such as Dacthal and pentachloronitrobenzene that contain HCB as an impurity (9). HEALTH EFFECTS Effects on Humans Evidence of the toxic effects of HCB for humans exists. The death of breast-fed infants and an epidemic of skin sores and skin discoloration were associated with accidental consumption of hexachlorobenzene-contaminated seed grain in Turkey in the mid-1950's. Doses were estimated at 50 to 200 ing/day for several months to two years. Clinical manifestations included weight loss, enlargement of the thyroid and lymph nodes, skin photo- sensitization, and abnormal growth of body hair. Hexachloro- benzene levels of up to 23 ppb in blood are believed to have contributed to enzyme disruptions in the population of a small community in southern Louisiana in 1973 (10). Effects on Animals Long-term (up to 3 years) animal ingestion studies show a detectable increase in deaths at 32 ppm, cellular alteration at 1 ppm, and behavioral alteration between 0.5 ppm and 5 ppm. Apparently, the effective dosage to offspring is increased by exposure to the parent. A 12% reduction in offspring survival results when exposure to very low levels had been continuous for three generations. Teratogenic effects appear minimal (10). A recent feeding study in hamsters showed that hexachlorobenzene causes hepatomas (liver tumors) and hemangioendotheliomas (capil- lary tumors). Doses of 50 ppm, 100 ppm, and 200 ppm of hexa- chlorobenzene mixed with feed were used. Hepatomas were observed at all dose levels, at rates and latencies appearing to be dose related. Hemangioendotheliomas appeared only in the high dose group (9% in females, 34% in males), and three of these tumors in males metastacized (10). Additional toxicological information on HCB is given in Table 4 (17). (17) Registry of Toxic Effects of Chemical Substances, 1976 Edition. H. E. Christensen, E. J. Fairchild, eds. U.S. Department of Health, Education, and Welfare, Rockville, Maryland, June 1976. 1245 pp. 13 ------- TABLE 4. TOXIC EFFECTS OF HEXACHLOROBENZENE (17) Oral lethal dose (50 percent kill) mg/kg body weight Animal 3,500 Rat 4,000 Mouse 1,700 Cat 2,600 Rabbit Bioaccumulation in catfish has been observed to be extremely high, and the half-life in cattle and sheep is almost 90 days (10). 14 ------- SECTION 5 CONTROL TECHNOLOGIES The major source of environmental contamination from HCB is wastes from plants producing other chemicals. Some work has been done on the development of environmentally sound disposal methods for waste containing HCB. A study by Midwest Research Institute includes a survey of waste disposal techniques practiced by industries that produce wastes containing HCB (3). Three methods are currently being used for disposal of these wastes: landfill, deep-well injection, and incineration. High temperature incineration appears to be the best alternative. Deep-well injection may create geological fractures resulting in contamination of aquifers (3). Landfill disposal of wastes con- taining HCB can lead to migration of HCB via water and sublima- tion of HCB into the air (10). Virtually all the HCB can be destroyed in high temperature incineration systems (3). Incin- eration of chlorinated hydrocarbons such as HCB is generally carried out at temperatures around 1,300°C with a retention time of about 0.25 s. Several types of incinerators are available. Most hexachlorobenzene waste is a viscous liquid at ambient temperature and can be incinerated in rotary kiln incinerators or in fluidized sand bed incinerators. Exhaust gases from in- cineration must be scrubbed in high energy scrubbers with caus- tic soda or lime solution to neutralize HC1 and other acids evolved (3). Dow Chemicals uses a proprietary "thermal oxidizer" (steam-oxygen fed incinerator) to incinerate wastes containing HCB. Products of the incineration are hydrogen chloride, carbon dioxide, and water. More than 99% of the HCB is reportedly destroyed (10). Plastic sheets are reportedly effective in reducing particulate emissions of HCB from waste storage areas, but vapor emissions of HCB from such areas may still be high. Hexachlorobenzene content in water was reportedly reduced about 50% at two plants sampled by detaining wastes in holding ponds or treatment canals (14). A discussion and evaluation of methods used for treatment 15 ------- and disposal of wastes containing HCB is given in a report done by TRW Corporation for EPA (18). A recent report indicates that land disposal is the most preva- lent disposal method. Land disposal was characterized as environmentally acceptable if soil covers of 1 m to 2 m and intermediate plastic layers were employed to reduce the sublima- tion rate. Selection of a site with geological characteristics that would provide for leachate containment is also necessary (13). (18) Quinlivan, S., M. Ghassemi, and M. Sontry. Survey of Methods Used to Control Wastes Containing Hexachlorobenzene, EPA-530/SW-120C, U.S. Environmental Protection Agency, Washington, D.C., November 1975. 92 pp. 16 ------- SECTION 6 REGULATORY ACTION IN PROGRESS In the wake of widespread hexachlorobenzene contamination of cattle in Louisiana in 1973 and concern over possible contamina- tion of sheep in California, EPA established an interim toler- ance level of 0.5 ppm. Concurrently, the State of Louisiana and several companies took immediate steps to improve solid waste disposal practices from manufacturing. Also, supplies of Dacthal containing 10% HCB were voluntarily withdrawn from the Cali- fornia market. As soon as the needed toxicological data are available, a food tolerance will be established. Also, all pesticidal uses will be reviewed, including pesticides which contain hexachloro- benzene as a contaminant. Studies of land and other disposal methods have been completed. Ocean dumping of hexachlorobenzene- laden tars is prohibited (10). It has also been designated a priority pollutant under the Federal Water Pollution Control Act. 17 ------- REFERENCES 1. Stecher, P. G., M. Windholy, D. S. Leathy, D. M. Bolton, and L. G. Eaton. The Merck Index, Eighth Edition. Merck and Company, Inc., Rahway, New Jersey, 1968. 2. Hawley, G. G. Condensed Chemical Dictionary. Eighth Edition. Van Nostrand Reinhold Co., New York, New York, 1971. 3. Mumma, C. E., and E. W. Lawless. Survey of Industrial Processing Data. Task 1 - Hexachlorobenzene and Hexa- chlorobutadiene Pollution from Chlorocarbon Processing. EPA-560/3-75-003, U.S. Environmental Protection Agency, Washington, D.C., June 1975. 187 pp. 4. 1977 Directory of Chemical Producers United States of America. Stanford Research Institute, Menlo Park, Cali- fornia, 1977. 1059 pp. 5. 1977 Directory of Chemical Producers United States of America. January to September Supplement. Stanford Research Institute, Menlo Park, California, 1977. 73 pp. 6. 1977 Buyers Guide. Chemical Week, 119(17), 1976. 7. Garner, D. N., and P. S. Dzierlenga. Organic Chemical Producers' Data Base Program. Radian Corporation, Austin, Texas, 1976. 8. Kirk-Othmer Encyclopedia of Chemical Technology, Second Edition, Vol. 18. John Wiley & Sons, Inc., New York, New York, 1964. 884 pp. 9. Assessing Potential Ocean Pollutants. National Academy of Sciences, Washington, D.C., 1975. 10. Environmental Contamination from Hexachlorobenzene. EPA-560/6-76-014, U.S. Environmental Protection Agency, Washington, D.C., July 1973. 34 pp. 11. Wilkins, G. E. End Use Patterns for Significant Organic Chemicals. Radian Corporation, Austin, Texas, July 21, 1976. 18 ------- 12. Chemical Origins and Markets. G. M. Lawler, ed. Stanford Research Institute, Menlo Park, California, 1967. 13. Journal of Hazardous Materials, 1(4) :343-359, March 1977. 14. Li, R. T., J. L. Spigarelli, and J. E. Going. Sampling and Analysis of Selected Toxic Substances. Task 1A - Hexachlo- robenzene. EPA-560/6-76-001, U.S. Environmental Protection Agency, Washington, B.C., June 1976. 166 pp. 15. Laseter, J. L., C. K. Bentell, A. L. Lacka, D. G. Holmquist, D. B. Condie, J. W. Brown, and R. L. Evans. An Ecological Study of Hexachlorobenzene (HCB). EPA-560/6-76-009, U.S. Environmental Protection Agency, Washington, D.C., April 1976. 74 pp. 16. Shackelford, W. M., and L. H. Keith. Frequency of Organic Compounds Identified in Water. EPA-600/4-76-062, U.S. Environmental Protection Agency, Athens, Georgia, December 1976. 629 pp. 17. Registry of Toxic Effects of Chemical Substances, 1976 Edition. H. E. Christensen, E. J. Fairchild, eds. U.S. Department of Health, Education, and Welfare, Rockville, Maryland, June 1976. 1245 pp. 18. Quinlivan, S., M. Ghassemi, and M. Sontry. Survey of Methods Used to Control Wastes Containing Hexachlorobenzene, EPA-530/SW-120C, U.S. Environmental Protection Agency, Washington, D.C., November 1975. 92 pp. 19 ------- TECHNICAL REPORT DATA (Please read Instructions on the reverse before completing) 1. REPORT NO. EPA-600/2-79-210g 2. 3. RECIPIENT'S ACCESSION NO. 4. TITLE AND SUBTITLE Status Assessment of Toxic Chemicals 5. REPORT DATE December 1979 Hexachloro- benzene issuing date 6. PERFORMING ORGANIZATION CODE 7. AUTHOR(S) T.R. Blackwood, T.G. Sipes 8. PERFORMING ORGANIZATION REPORT NO. 9. PERFORMING ORGANIZATION NAME AND ADDRESS Monsanto Research Corp Radian Corp 1515 Nichols Road 8500 Shoal Creek Blvd Dayton, Ohio U5H07 P.O. Box 99U8 Austin, Texas 78766 1O. PROGRAM ELEMENT NO. 11. CONTRACT/GRANT NO. 68-03-2550 12. SPONSORING AGENCY NAME AND ADDRESS Industrial Environmental Research Lab Office of Research and Development U.S. Environmental Protection Agency Cincinnati, Ohio ^5268 - Cinn, OH 13. TYPE OF REPORT AND PERIOD COVERED Task Final 11/77 - 12/77 14. SPONSORING AGENCY CODE EPA/600/12 15. SUPPLEMENTARY NOTES IERL-Ci project leader for this report is Dr. Charles Frank, 513-6Qk-kkQl 16. ABSTRACT The properties, production processes, uses, and emission sources for hexachlorbenzene are explained in this report. The environmental effects, health hazards, and current control technologies are discussed. The problems of the longevity of the hexachlorobenzene molecule and past hexachlorobenzene contamination are discussed and areas requiring further study are pointed out. 7. KEY WORDS AND DOCUMENT ANALYSIS DESCRIPTORS b.lDENTIFIERS/OPEN ENDED TERMS c. cos AT I Field/Group Benzene, Aromatic Hydrocarbons, Aromatic Monocyclic Hydrocarbons, Hydrocarbons, Unsaturated Hydrocarbons, Chlorobenzenes Solvents, Pesticides, Fungicides 68A 68D 68G 8. DISTRIBUTION STATEMENT Release to Public 19. SECURITY CLASS (ThisReport) Unclassified 21. NO. OF PAGES 28 20. SECURITY CLASS (Thispage) Unclassified 22. PRICE EPA Form 2220-1 (Rev. 4-77) PREVIOUS EDITION IS OBSOLETE 20 •i US GOVERNMENT PfllNTPNC OFFICE 1980-657-146/5512 ------- |