Environmental Protection
              OHic« o<
              Solid W«»te «nd
     &EPA
DIRECTIVE NUMBER:  9480.00-13
TITLE: Supplementary Guidaoce on Determining Liner/Leachate
Collection System Compatibility

APPROVAL DATE:  8/7/86
EFFECTIVE DATE:  8/7/86
ORIGINATING OFFICE:  OSW
QD FINAL
D DRAFT
  STATUS:
                              [ I
                              [ ]
                              f J
                 A- Pending OMB approval
                 B- Pending AA-OSWER approval
             t  j  C- For review &/or comment
             [  ]  D- In development or circulating
REFERENCE (other document*):       headquarters
 n.Q i/i/P/?       n Q WPB        n ^ \I\ICD
'E    DIRECTIVE   DIRECTIVE   D

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  AEPA
                                        . .            .  .
                                       Wasnmgton. uC 20460 -
                       OSWER Directive Initiation Reauest
                                                                                     u,l, ,:..e .•,„/'.;
                                                                9480.0013
                                          Ofginator Informat'On
 Name of Contact Person
 Chris W. Rhyne
                                 Mail Code  -
                                 WH-
                              Branch
                                                  Teleonone Numoer
                                                  382-4695
Lead Office
   D OERR
   00 OSW
D OUST
D OWPE
LJ AA-OSWER
                                                           Approved for Review
                                 Signature ol Office Director
                                                                                Date
Title
     Supplementary Guidance on  Determining  Liner/Leachate
     Collection System Compatibility
Summary of Directive                                             . .     .         i     j       T   i     ""
     This memorandum  addresses  several questions  regarding the owner's  and operator s
     responsibility to  demonstrate the chemical resistance of liner and leachate
     collection and removal system components to  the waste or leachate  to which  they
     are exposed.  Outlined is  the Agency's current position on High Density Polyethylene
     testing of liner and leachate collection system components (other  than the  liner),
     environmental stress cracking, and  changing  leachate during the liner immersion
     test  (Method 9090).
Key Words:
     Policy Directive
Type of Directive (Manual. Policy Directive. Announcement, etc.I
                                                                 ' Status
                                                                 \   D Draft
                                                                 \   0 Final
                                                                 i   D New
                                                                 I   I _ I Revision
                             )X| No   Does U Supplement Previous Directive^!?   [ \ Yes   fc"
Ooesin.s Directive Supersede Previous Directive!*;?   | | Yes"
f "Yes" to Either Question. What Directive (number, title)
                                                                                                NO
Review Plan
   d AA-OSWER  D OUST
   D OERR       D OWP6
   D OSW      . D Regions
                                 D OECM
                                 D OGC
                                 D OPPE
                                    Other {Specify!  ORD
This Bequest Meets OSWER Directives System Format
    Iture of Lead Office Directives Officer
                                                                              : Date
Signature of OSWER Directives Officer
                                                                               Date

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                                                   tftfttti
                                                 9480V00=1   3
           UNITED STATES ENVIRONMENTAL PROTECTION AGENCY

                       WASHINGTON, D.C. 20460      *
                          AUG -7 1986
                                               SOLID WASTE AND EMERGENCY RESPONSE
MEMORANDUM
SUBJECT:  Supplementary Guidance on Determining Liner/
          Leachate Collection System Compatibility
FROM:     Bruce R. Weddle, Director1
          Permits and State Programs Division

TO:       Hazardous Waste Management Division Directors
          Regions I-X


     A number of questions have arisen regarding the owners' and
operators' responsibility to demonstrate the chemical resistance
of liner and leachate collection and removal system components
to the waste or leachate to which they are exposed (see especially
40 CFR 264.301, 264.251, and 264.221).  This memorandum answers
some of these questions and further clarifies existing guidance
(See especially the draft Minimum Technology Guidance on Double
Liner Systems for Landfills and Surface Impoundments - Design,
Construction, and Operation, May 1985. )

Is HOPE* a universal material for liner and leachate collection
system components that needs no additional waste/leachate
immersion testing?

     No.  HOPE is a relatively inert synthetic material that can
chemically withstand a wide variety of substances; however,
there are chemicals that can seriously affect the performance of
HOPE (e.g., .many aromatic and halogenated hydrocarbon compounds).
Many of these chemicals are found in measurable concentrations
in leachates generated at hazardous waste facilities.
   HOPE (High Density Polyethylene) is one type of polyethylene
   liner material.  Polyethylene materials are the most popular
   synthetic liner material being proposed for new units.

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                                                      OSWER POLICY _pi.»i'-u«t .m

                               -2-                  '9'48 0*00-1   3
     Long-term immersion test results from low level exposure to
chemicals of concern showed measurable deterioration of HOPE
properties.  Therefore, low concentrations of chemicals of
concern must be tested for liner compatibility if they will be
present in the waste.

     EPA has been asked by the Institute of Chemical Waste
Management (ICWM) to consider approving HDPE liners as being
chemically resistant to certain classes of wastes without
chemical resistance testing.  EPA is investigating this
possibility by reviewing the available data and by discussing
this issue with technical experts in the polymer chemistry
field.  At this time we have not completed our review of the
technical issues or received enough data to grant blanket
approvals for HDPE.  In addition, preliminary conclusions
from an EPA meeting with polymer chemistry experts indicate
that in the case of a typical land disposal unit, they do not
have the ability at this time to establish classes of chemicals
that specific flexible membrane liner materials are universally
chemically resistant to, primarily because of the complexity
of the wastes, liner stresses posed by the typical land disposal
environment (e.g., temperature ranges and differential loading),
and variations in liner properties [See also response to next
question].

     Therefore, in general, EPA is unable at this time to approve
HDPE (or any other liner material) for use at any hazardous waste
unit without unit-specific verification of chemical resistance
based on the specific liner material and waste for that unit.
(Method 9090 or equivalent).

Does the generic term HDPE imply that all HDPE's are alike?

     No.  Polyethylene plastics, as defined by ASTM D 1248
(Polyethylene Plastics Molding and Extrusion Materials), are
plastics or resins prepared by the polymerization of no less
than 85% ethylene and no less than 95% of total olefins, by
weight.  Within this category HDPE is defined as having a density
of greater than 0.940g/cm->.  This higher density is an indication
of increased crystallinity that, with all other things being
equal, produces a material that is harder, stiffer, more chemical
and heat res-istant, and stronger than less crystalline material.
As density increases, the properties of elongation, resistance
to environmental stress cracking, impact strength and permeability
decrease.   In addition, comonomers are added during resin manufacture
that affect the degree of crystallinity and other material properties
(depending on the processing technique and the type and amount
of coraonomer).  Process type and process additives, such as
carbon black,  thermal/ultraviolet stabilizers and antiblocks,
will also affect material properties.

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                                                    OSWER POLICY
     When the sheet: extruder gets the resin he will, in turn,
extrude the material into a sheet using his own proprietary
additives.  The physical and chemical properties of the finished
product will again be affected by the additives and type of
extrusion process.  (Even the handling of the material immediately
after extrusion can affect material properties.)

     As can be seen from the above description, individual
HOPE liner properties can vary, depending on chemical com-
position and a number of processing factors.

     EPA also notes that the ASTM designation for HDPE is not
as meaningful as when originally proposed.  Advances in resin
manufacturing (such as the addition of new comonoraers) have
blurred the characteristic distinction between high density
and medium density and even low density polyethylenes.'
Materials are being marketed that are technically medium
density polyethylenes, but are labelled high density poly-
ethylene, and, in fact, may exhibit some of the physical
characteristics of high density polyethylene.  Therefore,
the density of the polyethylene is not necessarily as key to
overall chemical performance as it once was.  Since the
designation HDPE is no longer as relevant as when first
published by ASTM, EPA prefers to designate the various
polyethylenes as "polyethylene" and distinquish one from
another by their other properties, including resistance to
environmental stress cracking, chemical resistance, yield
strength, impact strength, seamability, etc.  Density is but
one of the factors affecting overall field performance.

     For these reasons EPA is continuing to insist that
owners and operators verify liner/leachate compatibility on
the specific waste and liner material that will be used in
each disposal unit.  Verifying the compatibility of  waste/
leachate with a particular polyethylene does not guarantee
in itself compatibility with other polyethylenes.

     Therefore, permit writers should require owners and
operators to demonstrate the chemical resistance (immersion
testing) of the specific liner material(s) they expect to
use in the actual construction.  When the owner or operator
has already performed the -immersion test, and proposes to
install a different manufacturer's polyethylene or a different
"batch" or formulation of polyethylene, he must demonstrate
that the alternate polyethylene is compatible by either
running Method 9090 (or equivalent) on the material selected
for installation or demonstrate material equivalence through
a "fingerprinting" process (see attachment).

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-4-
                                                   9480^00*1  3
     The attached guidance for "fingerprinting" is very general
If the owner or operator selects this option, agreeing on the
nature of the testing program and interpreting test results
will present difficulties.  The effect of a change in any given
"fingerprinting" characteristic (e.g. ,  percent ash) is poorly
understood.
What other liper and leachate collection system components
are required by current regulations to be compatible with
wastes?

     Landfill design and operating requirements state that the
leachate collection and removal system, as well as the liner,
must be constructed of materials that are chemically resistant
to the waste managed at the landfill and the leachate 'expected
to be generated (§264. 301 (a) (2) ).  Landfill, waste pile,  and
surface impoundment design and operating requirements also
state that liners and leachate collection systems must protect
human health and the environment.  It is, therefore, incumbent
upon owners and operators  to assure EPA that each component of
the liner(s) and leachate  collection system(s) is compatible
with the leachate or waste to which it is subjected.  Suggested
general procedures for various components are as follows;

     1 .  Piping - Piping should be prepared for strength
         testing per ASTM D 2412 or equivalent.  At least
         one prepared sample should be subjected to the
         same immersion test as performed on the liner
         material (e.g., the immersion test outlined in
         Method 9090).  After the immersion test, the pipe
         sample should be  dried (per Method 9090) and
         subjected to a strength test (see especially ASTM
         D 2412 paragraphs 6-9).  Testing of a control
         specimen (a sample not subjected to the immersion
         test) should be performed.  A report should be
         prepared similar  to that outlined in ASTM D 2412
         paragraph 11 (including 11.1.7 and 11.1.9) comparing
         the test results  of the immersed and control
         samples.

     2.  Geotextiles - Geotextiles can be used to perform
         any of three major functions in the land disposal
         unit:  1) protection of the flexible membrane
         liner, 2) use as  filtering media, or 3) use in
         the transmission  of liquid (water or leachate).
         Testing procedures for a given geotextile depend
         on its function.   When the geotextile is used
         either as a filter or as a protective media for
         the flexible membrane liner, immersion testing
         like that for flexible membrane liners should be
         performed.  After drying the immersed specimen(s) ,

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                                                     QSWEfl POLICY DIRECTIVE

                               -5-                 9^80.00*1   $
         both the immersed specimen(s) and identical control
         specimen(s) should be subjected to the ASTM D
         1682 Grab Strength Test and the ASTM D 751 Puncture
         Strength Test to determine if a significant loss
         of strength has occurred.

              Synthetic fabrics used for drainage, such
         as nets, should also be immersed in the expected
         waste/leachate.  Following immersion, both a
         control specimen and the immersed specimen should
         be tested for in plane transraissivity.  At this
         time no ASTM method exists to evaluate in-plane
         transraissivity; however, the Federal Highway
         Administration's Geotextile Engineering Manual
         references a technique by Koerner and Bove.l "

              This method (or another method to determine
         in-plane transmissivity) can be used to compare the
         in-plane transmissivity of the immersed specimen to a
         control specimen.

              Two specific recommendations need to be made
         to implement the test.

              (1) The final pressure exerted on the geotextile
              should be at least 1.5 times the maximum expected
              pressure to be experienced during the active
              life and post-closure period of the unit.

              (2) The geotextile should be placed in the
              apparatus under expected field conditions;
              i.e., both sides of the geotextile should be
              placed against the materials experienced in
              the field (e.g., soil, sand/gravel, flexible
              membrane liner, or other geotextile).

         Earthen Materials - When rock or gravel are used in
         the leachate collection system, the owner or operator
         should verify that the mineral content of the rock is
         compatible with the waste/leachate mixture.  The
         owner or operator will need to demonstrate that the
         rock will not be dissolved or form a precipitant that
         would clog the leachate collection system.
1.   Koerner,  R.M.  and Bove,  J.A.,  "In-Plane Hydraulic
    Properties of  Geotextiles,"  Geotextile Testing Journal,
    GTJODJ,  Vol.  6,  No.  4,  Dec.  1983,  pp.  190-195.

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                      -6-                 9'48-C v 00-1  3
     For soil used as a liner or a component of a liner
the material should be subjected to EPA Method 9100,
using the expected leachate to determine its effect
on the hydraulic conductivity of the compacted low
permeability soil.  The owner or operator may use the
fixed-wall or triaxial test.  (Note: Method 9100 is
currently under revision.)

Should environmental stress cracking be considered
as a modification to Method 9090?

     Although environmental stress cracking (ESC)
is not currently included in Method 9090, recently
reviewed data and discussions with technical
experts, including polymer manufacturers, ha\re
reemphasized the need to require an ESC test for
crystalline and seraicrystalline polymeric membrane
liners.  We are currently making revisions to Method
9090 that will outline available that ESC testing
be methods.

     Until specific test procedures for ESC can be
developed that represent land disposal facility
conditions, we suggest that permit writers discuss
the need for ESC data on these materials and suggest
that the owner or operator conduct ESC testing.
The type of test and initial interpretation of
the data would be the responsibility of the
applicant.

Should the leachate be changed during the immersion
test?

     Some of the constituents of greatest concern
in the chemical resistance immersion test are those
that are volatile or that enter into the material
being tested.  The owner or operator must assure that
the chemical composition of the leachate remains
relatively constant during the test to provide a
representative atmosphere for samples being immersed.

    The owner or operator must attempt to seal the
immersion vessel as tightly as possible to prevent
loss of volatiles.  In addition, the concentration
of chemicals in the leachate that are suspected to
affect the samples (such as aliphatic and halogenated
hydrocarbons) must be determined prior to immersion
testing, and should be checked when samples are
removed at the first 30-day testing period (for
Method 9090).  If the composition of the leachate

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                                                     OSWER peuey m^m we.

                                                   9480.00--1   3

                               -7-
         has changed  significantly,  the owner or operator
         should change  the  leachate  in the  immersion vessels
         and continue to change  the  leachate on a frequent
         basis  (frequency to  be  negotiated  with the permit
         writer)  to assure  that  the  liner samples are experi-
         encing exposure conditions  similar to those in
         the field.

Attachment

cc:  RCRA Branch  Chiefs,  Regions  I-X
     RCRA Permits Section Chiefs, Regions I-X
     Paul Ingrisano,  Region II
     Frank Langone, Region  II
     Greg Uetrecht, Region  VI
     Harvey King, State of  New York,  DEC
     Bob Tonetti
     Ken Shuster
     Terry Grogan
     Les Otte
     Robert Landreth
     Chris Rhyne
     Peter Guerrero
     Ana Aviles
     Agnes Ortiz
     Dave Friedman

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                  ANALYSIS AND FINGERPRINTING OF  UNEXPOSED AND EXPOSED
                              POLYMERIC MEMBRANE LINERS
                                  Henry E.  Haxo,  Jr.
                                   Matrecon,  Inc.
                              Oakland,  California  94623
                                       ABSTRACT
     A plan  is  presented  for analyzing polymeric mer,,brane  liners  for waste storage and
disposal  impoundments  before and after laboratory or ^ilot-scale exposure and  field ser-
vice.  These analyses  can  be used  to fingerprint a    material and to  follow the changes
that take place in a polymeric membrane liner during  exposure  to'waste.   They can also be
used to  determine  components  of a  waste  liquid  that are absorbed and are  aggressive to
polymeric liners.

     This analysis plan includes  determination of.volatiles,  extractables, specific
gravity,  ash and crystallinity  of  polymeric  liners.   The plan also includes gas chroma-
tography  and infrared  analysis of the extractables (and possibly of the organic  volatiles)
and thermogravimetric  analysis of the liner.   Also suggested  is the use  of  pyrolysls gas
chromatography,  which  can  be performed  directly  on unexposed and  exposed  liner  materials.
Typical  analytical  results for unexposed and exposed liners are presented.
INTRODUCTION

     Because of the wide  range  of composi-
tions and  constructions  of  flexible  poly-
meric membrane liners that are currently
available  and being developed for lining
waste impoundments, analysis and finger-
printing of  the  membranes is needed  for  a
number  of  purposes.   For example, a  liner
manufacturer needs to test  his  sheeting  as
new polymers are  used and as new compounds
and constructions are  developed.   He  also
needs tests  to control  the  composition  of
the liner being manufactured.

     The analysis of  a polymeric  membrane
liner at the  time of  placement  can  be used
for three  purposes: first, as a means  of
characterizing and identifying the specific
sheeting; second, as  a  baseline  for  moni-
toring the  effects of exposure on the liner;
and third,  to assess the aggresive ingredi-
ents  in  the  waste  liquid  to determine
chemical compatibility.
     During  exposure • to  waste   liquids,
polymeric liners  may change in  composi-
tion in  various ways  that  may affect their
performance and result  in  actual  failures.
Polymeric materials  may  absorb  water,
organic  solvents  and chemicals, organo-
metallic materials, and  possibly some Inor-
ganics if the  liners become highly swollen.
On the other  hand,  the extractable materials
in  the  original  liner  compound may  be
leacneu  out  and result  in stiffening  and
even brittleness on  the part of  the liner
membrane.   The solid  constituents of  a
polymeric compound  (which Include  carbon
black, inorganic fillers,  and some  of  the
curing agents)  will be retained in the liner
compound, as will  the polymer of  which  the
liner  is  made  (particularly  If  the polymer
is  crosslinked).   If organic materials  are
similar  to  the liner  in  solubility  and
hydrogen  bonding characteristics,  the liner
may swell  excessively.   Some thermoplastic
                                           157

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lining materials  may even dissolve,  when  in
contact with some solvents.

     The  objective  of  this  paper  is  to
present an  analytical  methodology that can
be used  to fingerprint and identify  liner
materials  and to give a baseline for
assessing the changes in composition  of
these materials when they are  under  test  or
in service.  Also  presented are  the  analy-
tical procedures  for testing  exposed  liner
materials  to determine  these changes.   Data
on  representative  liner materials,   before
and  after waste  exposure, are  presented.


POLYMERS USED IN MEMBRANE LINER MANUFACTURE

     Polymers used in the manufacture  of
lining materials include  rubbers  and
plastics  differing in polarity, chemical
resistance,  basic composition,   etc.,
and  can  be  classified  into  four  types:

     - Rubbers  (elastomers)  that  are  gen-
       erally  crosslinked  (vulcanized),
     - Plastics  that  a'-e  generally  unvul-
       canized (such as PVC),

     - Plastics that  have  a  Relatively
       hign crystalline content  (such as
       the  polyolefins), and

     - Thermoplastic elastomers that  do not
       reed to be vulcanized.

     Table  1  lists the various  types of
polymers  that are used and indicates whether
they are  used in vulcanized or nonvulcanized
form  and whether  they  are reinforced  with
fabric.   The polymeric  materials most  fre-
quently  used in liners  are polyvinyl chlo-
ride  (PVC),  chlorosulfonated  polyethylene
(CSPE),  chlorinated  polyethylene  (CPE),
butyl  rubber  (IIR), -.ethylene  propylene
rubber (EPDM),  neoprene  (CR^-,  and  high-den-
sity polyethylene  (HOPE).  The  thickness of
polymeric membranes  for liners ranges  from
20 to 120 mils, with most in the 20  to 60-
mi 1  range.
                     TABLE 1.POLYMERIC MATERIALS USED IN LINERS
Polymer
Butyl rubber
Chlorinated polyethylene
Chlorosulfonated polyethylene
Elasticized polyolefin
Use
Thermo-
plastic
No
Yes
Yes
Yes
in liners
Vulcanized
Yes
Yes
Yes
No
Fabric
reinforcement
With
Yes
Yes
Yes
No
W/0
Yes
Yes
Yes
Yes
      (partially crystalline)

     Elasticized polyvinyl chloride        Yes

     Epichlorohydrin rubber               Yes

     Ethylene  propylene rubber            Yes

     Neoprene  (chloroprene rubber)          No

     Nitrile rubber                       Yes

     Polyethylene  (partially crystal-
      line)                               Yes

     Polyvinyl  chloride                   Yes
        No

        Yes

        Yes

        Yes




         No

         No
Yes

Yes

Yes

Yes

Yes


 No

Yes
 No

Yes

Yes

Yes





Yes

Yes
                                          158

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     Most  polymeric  lining materials are
based on single polymers, but blends of two
or  more  polymers  (e.g.,  plastic-rubber
alloys)  are being developed  and  used in
liners.   Consequently,  it  is  difficult to
make   generic   classifications  based  on
individual polymers  in  the  liners,  even
though one polymer may  predominate.  Blend-
ing  of  polymers  introduces  tne long-range
possibility  of  the  need for  performance
specifications,  but  long-term  liner  per-
formance in  the  field  cannot  presently be
completely defined by  current  laboratory
tests.

     The basic  compositions  of the different
types  of  compounds are shown  in  Table 2.
The  crosslinked  rubber  compositions  are
usually the most  complex  because they  con-
tain  a  crosslinking  system that  requires
more ingredients  (e.g.,  the sulfur system).
Thermoplastics,  except  for  CSPE compounds,
contain no curatives.   Although  supplied as
thermoplastic  membranes,  CSPE  liners  con-
tain  inorganic  crosslinking  chemicals  that
allow the  compound to crosslink  slowly over
time during service.  Crystalline materials
have the simplest composition and generally
consist of  polymer,  a  small  amount of carbon
black  for  ultra-violet  protection,  and
antidegradants.

     Of the various'liner  components (except
for  the  polymer),  the following are poten-
tial extractables:
            - Small  amounts in the original  polymer
              (i.e.,  .stabilizers  and  antidegrad-
              ants)

            - Oils  and plasticizers

            - Antidegradants added to the compound.

            - Organic  constituents  of  the  sulfur
              crosslinking system (e.g., vulcaniza-
              tion   accelerators  and  activators).

       These ingredients  are  extracted in the de-
       termination  of extractables.

            Most  of the polymeric membrane  liners
       currently  manufactured  are based on  unvul-
       canized  or uncrosslirvked  compounds and thus
       are thermoplastic.   Even T-f  the  polymer in
       the  vulcanized  form   is more  chemically
       resistant  (such as CPE and  CSPE), it is
       generally  supplied  unvulcanized because it
       is easier to  obtain  reliable seams  and to
       make  repairs in the field.    Thermoplastic
       polymers  can be heat-sealed or  seamed with
       a solvent  or bodied solvent (a solvent con-
       taining  dissolved  polymer  to increase the
       viscosity  and reduce the rate of  evapora-
       tion).  Crystalline sheetings, which are
       also  thermoplastic, are  seamed  by  thermal
       welding  or  fusion methods.   Information on
       individual  polymers and  liners  is  presented
       in the  EPA  Technical  Resource Document on
       liners (Matrecon, 1982).
            TABLE  2.BASIC COMPOSITIONS OF POLYMERIC MEMBRANE  LINER COMPOUNDS
                                               Type of polymeric compound
                Component
Crosslinked   Thermoplastic   Crystalline
         Polymer  or  blends  (alloys)

         Oil  or plasticizer

         Fillers:
           Carbon  black
           Inorganics

         Antidegradants

         Crosslinking system:
           Inorganic system
           Sulfur  system
    100

   5-40
   5-40
   5-40

    1-2
    5-9
    5-9
 100

5-40


5-40
5-40

 1-2


 (*)
 100

0-10


 2-5


   1
         *An  inorganic curing system that crosslinks over  time is Incorporated
          in  CSPE  liner compounds.
                                           159

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ANALYSIS AND FINGERPRINTING OF UNEXPOSED
   POLYMERIC LINING  MATERIALS

     Analyses of liners  run before and after
exposure to  different environments  include:

    -  Volatlles

    -  Ash

    -  Extractables

    -  Gas chromatography

    -  Thermogravimetric analysis

    -  Differential  scanning  calorimetry
       if  Hner material  is  crystalline

    -  Specific  gravity

The  following  subsections  describe  the
tests  performed on  unexposed  polymeric
linings.

Volatiles

     The volatile fraction is represented by
the weight lost by an unexposed specimen of
the liner  on heating in a  circulating  air
oven at  105°C  for  2 hr.   Polymeric  compo-
sitions generally contain  a  small amount of
volatiles  (<1.0%), usually  moisture.    The
recommended specimen  is  a  disk  cut  from  the
membrane.

     The volatiles  test  can  also  be used to
determine the direction of  the grain  that
has been  introduced  in  the  membrane  during
manufacture.   By identifying the orientation
of the  2-in.  disk  specimen with  respect to
the sheeting  at the  time  the  specimen  was
died out, the grain  direction  can  be  iden-
tified.  The  grain direction must  be  known
so that  tensile  and  tear  properties  can be
determined  in machine (grain) and transverse
directions.   Upon heating  in  the oven at
105°C,  sheeting with a grain  will shrink
more  in the grain  direction  than in  the
transverse  direction  (Figure 1).

     Volatiles  need  to be  removed before
determining  ash, extractables,  and spec-
ific  gravity.   Ash  and extractables  are
reported on  a dry basis  (db).  Volatiles
contents of  representative membrane  liners
are presented in Table  3.   Monomeric  plas-
ticizers that  are generally  used in  PVC
compositions  have a  limited  volatility  and
can slowly  volatilize at  105°C.    Thus  the
air oven test  must  be  limited to  2  hr.
                As received
             After air oven heating
             2hr. at 105°C

Figure 1.Machine   direction  determinations.
     A standard test  for  the  volatility of
plasticizers in PVC  compounds  is  performed
in accordance with  ASTM D1203.   In this
test, activated charcoal  is used  to  absorb
volatilized plasticizer.
Ash
     The ash content of a liner material  is
the inorganic fraction that  remains  after a
devolatiiized sample is thoroughly burned  at
550°±2bJC.   The  ash  consists  of (1) the
inorganic materials that have been  used  as
fillers  and  curatives  in  the  polymeric
coating compound,  and  (2)  ash  residues  in
tne polymer.  Different liner manufacturers
formulate their compounds  differently,  and
determining  the ash content  can  be a  way  to
"fingerprint" a  polymeric  liner  compound.
The  residue  obtained  by  ashinq  can  be
retained for other analyses  (such as metals
content) needed  for  further identification
and  for providing a  reference  point  to
determine trace  metals  that may have  been
absorbed  by the  liner.   The test method
                                           160

-------
described  in  ASTM  0297,  Section  34,  is
generally   followed   in  performing  this
analysis.   Ash  contents  of  representative
membrane liners  are  presented  in  Table  3.

Extractables

     The extractable  content of a polymeric
sheeting is  the  fraction of the  compound
that can be  extracted  from a devolati 1 ized
sample  of  the  liner  with  a solvent that
neither  decomposes nor dissolves  the poly-
mer.  Extractables consist of plasticizers,
oils, or other  solvent-soluble  constituents
that  impart  or help maintain  specific
properties  such  as  flexibility  and proces-
sability.   A  measurement  of  extractable
content  and  an  analytical  study  of  the
extract can be  used  as part of the finger-
printing of a  sheeting.

     During exposure  to  a  waste,  the  ex-
tractable  constituents in a liner may be
               removeu  and  resu]t in property changes.   At
               the same  time during exposure, the  liner
               might  absorb  nonvolatiIizable  constituents
               from a waste.  Measuring  the extractable
               content of  unexposed lining materials  is
               therefore  useful  for  monitoring the effects
               of  exposure.   The extract and the extracted
               liner  obtained by  this procedure can be used
               for further  analytical  testing  (e.g.,  gas
               chromatography,  infrared  spectroscopy,  ash,
               tnermogravimetry,  etc.)   and  fingerprinting
               of  the liner.

                   The  procedure for extraction generally
               follows ASTM  03421, "Extraction and Analysis
               of  Plasticizer Mixtures  from  Vinyl  Chloride
               Plastics".   Also  see ASTM  D297,  "Rubber
               Products-Chemical Analysis",  paragraphs
               16-18.

                   Because  of the  wide  differences  among
               the polymers  used  in liner  manufacture,  a
               variety  of extracting media  must  be  used.
                      TABLE 3. ANALYSIS OF UNEXPOSED POLrMERIC MEMBRANE LINERS*.*
Base polymer,
Polymer specific gravity
Butyl rubber
Chlorinated polyetnylene
Chlorosulfonated poly-
ethylene
Elasticized polyolefin
Epichloronydrin rubber
Etnylene propylene rubber
Neoprene
Polybutylene
Polyester elastomer
Polyethylene (low density)
Polyethylene (nigh density)
Polyethylene (high density)
al loy
Polyvinyl chloride
0.92
1.16-1.26
1.11
0.92
1.27-1.36
0.86
1.25
0.91
1.17-1.25
0.92
0.96
0.95
1.40
Compound
Specific
gravity •
1.206
1.176
1.360
1.362
1.377
1.433
1.343
0.938
1.490
1.173
1.122
1.199
1.503
1.480
1.390
0.915
1.236
0.921
0.961
0.949
1.275
1.264
1.231
1.280
1.308
Volatiles,
X
0.45
0.46
0.10
0.00
0.05
0.84
0.51
0.15
0.63
0.38
0.50
0.31
0.76
0.19
0.37
0.12
0.26
0.18
0.12
0.11
0.11
0.09
0.05
0.31
0.03
Extractables
X
10.96
11.79
7.47
9.13
1.49
3.77
5.50
7.27
23.41
31.77
18.16
10.15
13.43
21.46
...
2.74
2.07
0.49
2.09
33.90
37.25
38.91
35.86
25.17
. Asn,
I
5.25
4.28
14.40
12.56
17.37
33.95
3.28
0.90
4.49
6.78
5.42
0.32
12.98
13.43
4.67
0.08
0.38
0.13
0.46
0.32
6.20
5.81
3.6S
6.94
5.67
            •Source of some of the data
            ^Multiple figures represent
: Haxo et a). (1982).
materials from different manufacturers.
                                            161

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Table 4  lists the recommended solvents  for
extraction  of  membrane  liners  of  each
polymer type.

     Typical values for the extractables in
polymeric  membranes  are given in  Table 3.

Gas Chromatography

     Gas Chromatography can be used to  find
the level of the plasticizer  (e.g., diethyl-
hexyl phthalate (DEHP), a  dioctyl phthalate)
compounded into a  PVC  liner material.   Fig-
ure  2, shows  the  quantification  of  DEHP in
the solvent extract of  a PVC  liner material.
The weight percent of  the DEHP in the liner
can then be calculated, assuming  the extrac-
tion  to  be  100% efficient.   A  typical
procedure is summarized below.

     A weighed sample  of  liner is extracted
with an  appropriate solvent. The extract is
evaporated to dryness over a steam bath.
The  dry  residue  is  redissolved  irr solvent
and  brought  to an accurately known volume.
Following the development of appropriate
chromatographic  conditions, injection of
this  solution into  the  instrument  will
separate it  Into  chemically pure components
characterized by  different retention times.
An  injection of  a DEHP standard  solution
will identify the retention time  of the  DEHP
component.   Comparison of the  peak height
 I  0.4
 >-
 I
    0.2
O Standards
+ Sample
     0123456789  10  11
                 PEAK HEIGHT IN CM

Figure 2.Gas  chromatograph determination
         of  the di ethyl he'x'yl  phthalate
         content  in an  extract  of  a  PVC
         membrane.    Column:  6'xl/8"  3% 0V
         101 on  Chromosorb WHP.    Tempera-
         ture:  200°-3QO°C  at  8°C/min.   He
         carrier gas: at  30cc/min.

(area) data  obtained from  the injection of
equal volumes  of the  extract  solution  and
from  quantitatively   prepared   standard
solutions  allows  the  interpolation  of  the
DEHP concentration  in  the  extract  solution
(Figure  2).
                TABLE 4.  SOLVENTS  FOR  EXTRACTION OF HULYintRIC MEMBRANES*
                    Polymer type
       Extraction  solvent
        Butyl  rubber (IIR)
        Chlorinated polyethylene  (CPE)
        Chlorosulfonated polyethylene  (CSPE)
        Elasticized polyolefin
        Epichlorhydrin rubber  (CO and  ECO)
        Ethylene propylene  rubber (EPDM)
        Neoprene
        Nitrile rubber (vulcanized)
        Nitrile-modified polyvinyl chloride

        Polyester elastomer
        High-density polyethylene (HOPE)
        Polyvinyl chloride  (PVC)

        Thermoplastic olefinic  elastomer
    Methyl  ethyl  ketone
    n-Heptane
    Acetone
    Methyl  ethyl  ketone
    Methyl  ethyl  ketone  or  acetone
    Methyl  ethyl  ketone
    Acetone
    Acetone
    2:1 blend of  carbon  tetrachlo-
     ride and methyl  alcohol
    Methyl  ethyl  ketone
    Methyl  ethyl  ketone
    2:1 blend of  carbon  tetrachlo-
     ride and methyl  alcohol
    Methyl  ethyl  ketone
        *Because lining  materials can be sheetings based on polymeric aloys mar-
         keted under a  trade  name or under the name of only one of polymers, this
         list can only  be  taken as a guideline for choosing a suitable solvent for
         determining the extractables.  Once a suitable solvent has been found, it
         is important that the same solvent be used for determining the extract-
         ables across the  range of exposure periods.
                                           162

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Pyrolysis gas  chromatography

     Pyrolysis  gas  chromatography  is  an
alternative method  for measuring a plas-
ticizer in  liner materials.   In  this  tech-
nique, a  small, weighed sample of  liner  is
heated very  rapidly  to a  temperature  suf-
ficient  to volatilize all  of its organic
components.   The  plasticizer  and  other
lower-molecular weight  organics  will  be
driven off  as  chemically  unchanged  vapors.
The polymer will undergo  pyrolysis, or  high
temperature decomposition,  and  will   vola-
tilize as lower-molecular-weight organic
compounds.  The resulting  volatiles may  be
separated and  quantified  by  gas chroma-
tography   as  previously  described,  and the
plasticizer content  of  the  liner  may  be
calculated.

     This method has the strong advantage  of
not  requiring  extraction  of   the  liner
sample,  but it may  not  be  as  reliable a
means of  quantification because of the  very
small sample  size  and the  large  number  of
components that  must be separated  by the gas
chromatograph.

Thermogravimetric analysis (TGA)

     TGA   is a  thermal  technique  for asses-
sing the  composition  of  a material  by its
loss  in  weight  on  heating at a  controlled
rate  in  an inert  or  oxidizing  atmosphere.
For example, when a material is heated  in  an
inert atmosphere from room  temperature  to
600°C at  a controlled rate, it will  vola-
tilize at different  temperatures  until  only
carbon,  char  and  ash remain.   The intro-
duction  of oxygen  into the system will  burn
off  the  char  and  carbon  black.    Thus  from
the weight-time curve which  can  be  related
to weight  and  temperature,  the amounts  of
volatiles,  plasticizer,  polymer,  carbon
black, and ash can  be calculated.    In  some
cases,   thermogravimetric   analysis  can
replace  measurements  of the  volatiles,  ash,
and  extractables contents discussed above.
The TGA curve and  the derivative  of the TGA
curve can thus be  used as  part of a finger-
print of a polymeric composition.    This
technique 1s  described by  Reich and  Levi
(1971).

     A  Perkin-Elmer  TGS-2  thermogravi-
metric system, consisting  of an analyzer
unit, balance control unit,  heater control
unit, and first  derivative computer, is  used
in our laboratory.   Temperature  control  is
supplied   by  the temperature controller  on
the  Perkin-Elmer  DSC-2  (Differential  Scan-
ning Calorimeter).  A  double  side-arm  fur-
nace tube was  used  to  allow  rapid  changing
of  the  atmosphere  from inert  (N2)  to  oxi-
dative  (N2/02 mixture).   For  the oxida-
tive  atmosphere,  N2  purge  is  maintained
through  the  analyzer  unit  head,  and 02
is  introduced  at  the  upper side arm  where
it  mixes  with the  N2 to  burn  the carbon
black  and any carbonaceous  residue that
forms during  the  pyrolysis of the  polymer.
Use  of  the double  side-arm  furnace tube
shortens  the  turnaround  time  because it
eliminates the need to flush  the  analyzer
head completely to  remove  0?  between  runs,
as  would  be  necessary if &2 were intro-
duced through  the head.  A dual pen  recorder
Perkin-Elmer  Model  56  allows a simultaneous
display of thermocouple temperature in the
furnace  and  the  change in weight of the
specimen  or  the  first derivative of the
change in  weight.

     An example of the TGA procedure for the
analysis  of a  polymeric liner is described
below.

     A 5-mg specimen of the liner was  placed
in the balance pan and weighed  in a  nitrogen
flow  of   40  cc/min.   The instrument was
adjusted  to give  a  100% full-scale  deflec-
tion for  the  weight of the sample, so the
percent   of  weight change  can   be  read
directly  from  the chart.

     The   specimen  was  heated  to 110°C and
held there for  5  min  to  determine  whether
measurable volatiles were  present;  it was
then heated from  110°  to 650°C at a rate of
20°C/min  in  a nitrogen atmosphere.   The
specimen  was  held at 650°C until  no more
weight loss occurred,   usually 2 to 3 min,
after which it was  cooled to  500°C and Q£
was introduced at a rate of 10  cc/min with
an N2 flow rate of 30 cc/m1n.

     Typical  thermograms  for  HOPE  and EPDM
appear in Figures 3 and  4, respectively.
Analyses  of a variety  of polymeric  membrane
liners are presented in Table  5.

Differential Scanning Calorimetry (DSC)

     DSC  is  a thermal  technique  for measur-
ing  the  melting  point  and the  amount
of  crystallinity  in partially  crystalline
polymers  such as  the  polyolefins polyethy-
lene,  polypropylene,   and polybutylene.
This technique measures  the heat of fu-
sion of  a crystalline structure;  it can
also give an indication of the modification
of crystalline sheeting  with other  polymers
                                          163

-------
                                   12   16   20  24   28   32  36   40
                                          TIME. MINUTES

Figure 3.TGA of an unexposed black  HOPE liner.   The plots of sample weight and temperature
         as a function  of  time are shown.   Under an N2  atmosphere,  the black HOPE  sample
         lost approximately  95.5% of  its mass as  hydrocarbons were evolved.   The  carbon
         black added  as an ultraviolet  light  absorber remained  as a carbonaceous  residue
         and was  not  volatilized until  it was oxidized  when oxygen was  allowed into the
         system.
llftJU
900
900


700

°. 600
UJ
3
K
< 500
or
UJ
^
£
lu 400
K

300

200


100

0
^"^^^
,- COMPOSITION FROM TGA.
Volatilei 0
Oil 33.0
Polymer 3 1 .0
Carbon Black 31.0
Ash 5.0
Total 100.0
\ 3
\
\
\

'
3\0it




^\
j-A /"
% Original Wei^it of Specimen 	 — H /
\X
/i
' '




/'
k X
\ /
^


> \ 31% Polymer
.' 1
s \
~ s \
/ \
S
Temperature — _ _ *
/
S
S


^_ _f* ^
i i i i i i i i t i




'








3



.
. l«
*^*
1 f 1
I
-
-

,-\
\
\
\
\
\
\
\
\
\
\
\
\
N
% Carbon Black
-


f 5
-------
           TABLE  5.THERMOGRAVIMETRIC ANALYSIS OF POLYMERIC MEMBRANE LINERS
                           Volatiles,   Polymer,   uiI or plas-  Carbon      Ash,
         Polymer type          %           %       ticizer, %    black,  %     %
         Butyl  rubber

         Chlorinated
           polyethylene
         Chlorosulfonated
           polyethylene
         Elasticized
           polyolefin

         Epichlorhydrin
           rubber

         Ethylene propylene
           rubber
         Neoprene
         Polyethylene (high
  0


  0
  0
0.4
1.0
0.9
0.1
0.1
0.2

1.0
  0
45.0


72.2
71.3
53.9


49.3
47.7
58.1


93.1


49.3
30.8
33.5

42.3
44.0
12.2


 7.6
 9.1
13.9


 1.5
 3.2
 5.5


 1.7


 8.2
32.9
23.2

10.7
10.7
37.1


 5.3
 6.5
21.0


45.6
45.2
 9.8


 4.0


37.7


30.9
35.5

34.9
33.8
 5.7


14.9
13.1
10.8


 2.6
 3.0
26.5


 1.2


 4.8
 5.3
 7.6

11.1
11.5
density)


Polyvinyl chloride


0
0
0
0
0
0
97.9
95.6
97.0
48.7
46.0
51.0
U
0
0
38.2
42.1
35.0
2.1
4.2
1.8
6.2
7.8
7.0
• • •
0.2
1.2
6.9
4.1
7.0
by alloying.   Thus this type of analysis  can
be used as  a  means  of fingerprinting  crys-
talline polymeric liner  materials  (partic-
ularly   high-density  polyethylene)   and
assessing  the effects of  aging and exposure
to wastes.   This  technique  is  described by
Boyer (1977)  and  Ke  (1966).

     The  differential  scanning  calorimeter
used  in  this work  was   the  Perkin-Elmer
Model DSC-2C,  equipped with an Intracooler I
subambient temperature accessory  to provide
an operating temperature range of -40 to
725°C.

     The  equipment  is used  to characterize
the  thermal  transitions  of materials
such  as melting, boiling,  and changes in
crystal structure.   A  sample  and  reference
cell  are  provided.  A  weighed sample is
placed  in  the sample holder;  the  reference
cell   is  generally  run empty to provide an
                absence of thermal  transitions.   The two
                cells are simultaneously heated or  cooled so
                that  the  average  cell  temperature  follows a
                preset  program.   When the  sample  undergoes
                a  thermal  transition,  an endotherraic or
                exothermic  reaction will   occur.   The
                change in power  required  to  maintain the
                sample  cell  at the same temperature as the
                reference cell  1s recorded as  a deflection
                of the  recorder pen.   The recorder  plots the
                temperature  (°C) versus the  differential
                energy  flow  (meal/sec)  required to maintain
                the sample cell temperature.  An endothermic
                transition such  as  melting  1s shown as a
                positive  peak;  an exothermic  reaction such
                as  crystallization  1s  shown  as a  negative
                peak.   The magnitudes of these peaks and the
                temperatures at which they occur are charac-
                teristic of the material analyzed.

                    An example  of  the use  of the DSC to
                determine the  polyethylene  crystal Unity 1n
                an HOPE Uner 1s  shown 1n Figure 5.
                                           163

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     2
     <
     
-------
                   2    —> ~


PLASTICIZER
FILLER
POLYMER
XL OR TP
ORIGINAL
LINER
T
•s

. WASTE . .
. ' LIQUID
PLASTICIZER
FILLER
POLYMER
I

EXPOSED
LINER
i, WEIGHT INCREASE
• A'ASTE •
' LIQUID .
PLASTICIZER
FILLER
POLYMER
VOLATILES
REMOVED
_ VOLATILES
\
i
PLASTICIZER
FILLER
POLYMER
VOLATILES
AND
EXTRACTABLES
<, VOLATILES \EXTRACTABLE
• Momure • Nonvolatile organic
• Organics
                                                                              EXTRACTABLES
Figure 6.Schematic presentation of changes  in composition  of  a polymeric  liner  compound on
           exposure  to  a  waste  liquid,  on  removal   of  volatiles,. and  on  extraction  with
           an appropriate solvent.
                                                        H20 * volatile orgamcs
                                                        Plasticizer
                                                        Polymer
                                                        Carbon black
                                                        Ash
                   TGA " Ihermogravimetric analysis
                   GC - gw chromitograpny
                   IR - infrared soeclroscopv
                   AAS * atomic absorption spectroscopy
                   CHONS * Carbon. hydrog«n, nitrogen, oxygen, and suMur determination
            Figure  7.Plan  for the analysis  of exposed polymeric  lining materials.
                                                   167

-------
Volatiles

     The initial  analytical  test generally
performed  is a  determination  of  the vola-
tiles content,  which  gives an  indication of
the amount of wast* liquid that has been ab-
sorbed by the Hner.   As  an approximation,
the  weight  Increase can be calculated by
dividing the  percent of volatiles  by  the
percent of  nonvolatiles.   For example,  if
the volatiles  are  15%,  and the nonvolatiles
are  85%,  the percent  Increase  in  weight
based on the original  Hner would be 17.6%.

     Inasmuch  as  the volatiles  contain
both  water  and  organic components,  it
1s  desirable to  separate these two.   A
study  was  made  to  dehydrate the  speci-
mens  of the exposed  Hner  to  remove  the
water.  A series of desiccants  was stud-
led  at  room temperature and  50°C.    Four
days  of exposure of the exposed liner at
50°C  in  a  small  Individual  desiccator
containing  calcium  chloride   removed  the
moisture  from  the  2-1n.  disk  specimen
without  removing  organic  constituents.
After removal  of the water,  a   2-hr heating
of the  specimen 1n a circulat-ing air oven
removed the remaining organic  volatiles.
Collection  of the organic  volatiles  and
determination  of  composition  by  gas
chromatography   would  be  desirable  but
has  not been attempted  to  date.   The
water  and  the  organic  volatiles  equal
the  volatiles obtained  in  bypassing  the
desiccator exposure.   Such a bypass  removes
the moisture by exposure at room temperature
for 1 week 1n moving air followed  by heating
in a circulating  air  oven  for  20  hr at 50°C
and 2 hr at  105°C.   We have  found, however,
that the highly swollen CPE  liner may take
up to  6 days  at  50°C to come to constant
weight.  The time  required  to  remove
volatiles  depends  on the  thickness  and
permeability of the liner and the  care taken
to  avoid  the  "skin"  that  forms   on  the
surface of  the specimen when using too high
an  initial  temperature  to devolatilize.
After the  volatiles are  removed,  the
exposed  materials  can  be  subjected  to
the other tests, Including specific gravity,
extractables, ashing, etc.

     Total  volatiles  can  also  be  determined
through the  use  of  TGA which  is discussed
below.

Extractables

     Extractables  of  exposed  materials
will  probably differ from  the  original
values  because of the  loss to the waste
liquid and  absorption  of nonvolatile
organics  (e.g.,  oils).   After  the  vol-
atiles  have  been  removed from the  liner,
the extractables are determined  by the  same
method used on the unexposed liner materi-
als.  Examples of extractable contents after
exposure are given in  Table 6.   If the liner
has been  in contact with wastes containing
nonvolatile  constituents,  the  extractables
recovered  may  be greater than  the original
values. Analysis of the  extractables by gas
chromatography  and infrared analysis  may
give  an  indication  of  the  nonvolatile
organics that were absorbed.  The analysis of
the extractables will  give an indication of
the  constituents  of  the waste  that  are
aggressive to  the liner, as they are  the
constituents that  have been absorbed.  They
may  show  up  in minor amounts  in a waste
analysis,  but  because  of  their  chemical
characteristics  such  as  solubility parame-
ters  and  hydrogen  bonding, they may  be
scavenged  by the polymeric liner.

Ash

     Thp ash  content of  an exposed membrane
liner is determined after the volatiles  have
been  removed  from the  specimen.   As  in the
case of the unexposed  membrane,  the exposed
liner  is  ashed  in a muffle  furnace  at
550°C. The ash  value  usually differs  from
that of the unexposed material, depending on
how many  nonvolatile  organics were lost or
gained during the exposure period.  If plas-
ticizer is lost,  the  value will  increase
because of the nonash  content of the plasti-
cizer.  Also, if any organic  metal compounds
are absorbed by the liner, they will show as
an  increased  ash content.   A comparison of
the elemental analysis of the ash with  that
of the original liner will  determine whether
any absorption of metal species  occurred
during the exposure.  No  such absorption has
been observed,  but  metal organics might be
absorbed by a  liner.    In general,  the in-
organics that  make up  the ash  are retained
in the  liner and maintain a constant ratio
with  respect  to the  polymer  content,  as
polymer is generally   not dissolved  by  the
waste liquid.

Thermogravimetric analysis

     The TGA  analysis  can be used to give a
quick  analysis of the  composition of an
exposed polymeric membrane liner.   The  test
is  run  similarly  to that  of the unexposed
material,  except that  care must  be taken in
handling  the  small specimens  of exposed
                                          168

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               TABLE 6.EXTRACTABLES  OF DIFFERENT POLYMERIC MEMBRANE LINERS
                             BEFORE  AND AFTER VARIOUS EXPOSURES
Polymer
Butyl rubber
Unexposed
11.79
Type of exposure
by waste
Aromatic oil
Spent caustic
Oil 104
Extractables
after exposure
27.23
10.87
40.34
          Chlorinated
            polyetnylene       9.13
          Chlorosulfonated
            polyethylene        4.08
          Elasticized
            polyolefin          5.50
          Ethylene  prop-
            ylene rubber       23.64
          Neoprene             21.46
          Polyvinyl
            chloride           33.90
Oil 104
Roof exposure
Aromatic oil
Oil 104
Slop water
Oil 104
Aromatic oil
Slop water


Aromatic oil
Oil 104
Spent caustic

Aromatic oil
Oil 104
Slop water
Aromatic oil
Roof exposure
Pesticide
Oil 104
17.00
 5.99
59.81
15.92
 3.70
20.74
23.37
 2.96
38.35
43.45
22.89

58.47
23.85
17.63
40.55
26.27
35.38
17.95
liners that  contain  the volatiles.   These
volatiles can be easily  lost.  Figure 8 is a
thermogram of an exposed PVC membrane liner
that had absorbed more than 7% of the waste
liquid, which was predominantly water.  The
results are  shown  on the  figure,   but the
losses show the effect of the char formation
of the PVC  when It  is  heated in a nitrogen
atmosphere.    Chlorinated polymers  lose HC1
and leave a  char for which correction must
be made  in  the calculations of the polymer
content.   These  calculations have been made
on the figure,  and  the  results compare fa-
vorably with those obtained by direct analy-
sis of the volatiles, extractables, and ash.

Specific  gravity

     The  specific  gravity   of  exposed  mem-
brane  liners  is also determined  after the
  membrane  specimen  has been  thoroughly de-
  volatilized.   Three  steps  must  be taken to
  avoid the formation  of bubbles 1n the  Uner
  mass during a direct  devolatilizlng process
  (which  would affect the specific  gravity
  results).  First,  the  specimens must be
  allowed to "dry"  at  room temperature  1n an
  air stream in  a hood until constant weight
  is achieved, which could take several  days.
  Second, they must  be placed  in  an  oven at
  70°C  for 16 hr;  and third, they must be
  heated at 105°C for  2 hr.

       The  specific  gravity  of an  exposed
  membrane can differ from that  before ex-
  posure, depending on how much of  the origi-
  nal extractable  material  was  lost  and how
  much material  from  the  waste was absorbed
  during exposure.  The procedure followed was
  ASTM  D297 using the hydrostatic  method.
                                           169

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        iooo
                                                                             100
                                    60       80

                                       TIME. MINUTES
                                                    100
                                                            120
                                                                  140
                                                                         160
                   Figure 8. TGA of an exposed polymeric  PVC liner.
        Weight  loss A
        Weight  loss B
        Weight  loss C
        Weight  loss D
        Residue weight E
 7.0% volatiles  = moisture + possible organics.
60.2% = plasticizer + HC1 from the polymer (PVC).
16.0% = residual polymer.
10.0% = carbonaceous polymer residue + carbon black,
 6.8% = ash.
        Composition of the exposed liner as received  calculated from above data.
        Values  by direct analysis are shown in parentheses.

        Volatiles       7.0% (7.9)a
        Polymer (PVC)  44.7%
        Plasticizer    34.1% (32.2% as extractables)3
        Carbon  black    7.4%
        Ash            6.8% (6.4)a

        aBy direct analysis.
SUMMARY AND CONCLUSIONS

     A protocol  is  presented for the analysis
of  polymeric  membrane lining  materials
before and  after exposure  to  waste liquid.

     The results of the  analysis can be used
as a fingerprint of the unexposed liner and
as a baseline for assessing the changes that
occurred during exposure to a waste liquid.

     The  analysis of  an  exposed liner
furnishes information regarding  the change
in the composition  of the  membrane and the
chemical  materials  that  are actually absorb-
ed during exposure.  This latter information
indicates the constituents of the waste that
are  aggressive to  the lining  material.

     Thermal  analysis and gas chromatography
are  particularly  useful  in  the  analysis
and  fingerprinting   of  polymeric  membranes.
                   The  use   of  gas  chromatography  coupled
                   with  mass  spectroscopy  needs  to  be  investi-
                   gated  to   determine  the specific  chemicals
                   that  are  absorbed by  a polymeric liner.

                       The  use  of this  analysis  may lead to
                   techniques which  will better  predict the
                   service life  of a flexible membrane  liner.

                   ACKNOWLEDGEMENTS

                       Tho  work reported in this  paper was
                   performed under  Contracts  68-03-2134
                   ("Evaluation  of  Liner Materials Exposed to
                   Leachate"), 68-03-2173 ("Evaluation  of Liner
                   Materials Exposed to Hazardous and Toxic
                   Wastes"),  and 68-03-2969 ("Long-term Testing
                   of  Liner  Materials")  with  the Municipal En-
                   vironmental Research Laboratory  of the U. S.
                   Environmental  Protection Agency,  Cincinnati,
                   Ohio.
                                           170

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     The  author wishes to  thank  Robert  E.
Landreth,  Project  Officer,  for his support
and guidance in these projects.

REFERENCES

ASTM Standards, American Society for Testing
and Materials, Philadelphia,  PA.

     D297-81,  Rubber  Products -  Chemical
       Analyses: Section  15,  Density (Hydro-
       static Method); Section 34, Fillers,
       Referee Ash Method

     D792-66, Specific  Gravity  and Density of
       Plastics by Displacement; Method A-l
       for Testing Solid  Plastics in Water,
       Sections 6-12.

     D1203-67,  Volatile Loss  from  Plastics
       Using  Activated  Carbon  Methods.

     D3421-75,  Extraction  and Analysis  of
       Plasticizers  from  Vinyl  Chloride
       Plastics

Boyer,  R. F.  1977.  Transitions and Relaxa-
     tions.    In:  Encycl.   Polymer.   Sci.
     Technol.   Supplement,  Vol.  2.  pp
     745-839.
Haxo,  H. E.  1983.   Liner  Materials Exposed
     to Hazardous and  Toxic  Wastes.  Final
     Report.   Contract 68-02-2173.   U.  S.
     Environmental  Protection  Agency,
     Cincinnati, OH.   In preparation.

Haxo,  H. E., R. M. White,  P. D. Haxo, and M.
     H. Fong.    1982.   Liner  Materials
     Exposed  to Municipal  Solid Waste
     Leachate.    Final Report.   Contract
     68-03-2134.   U. S.  Environmental
     Protection Agency, Cincinnati, OH.  In
     press.

Ke, B.  1971.  Differential Thermal Analy-
     sis.    In:  Encycl.  Polymer.  Sci.
     Technol. Vol  5,  pp 37-65.

Matrecon,  Inc.   1982...  Lining of Waste
     Impoundment  and  Disposal  Facilities.
     SW-870, Second Edition.  U.S.  Environ-
    mental  Protection  Agency,  Washington,
     DC.   In press.

Reich, L., and  D. W. Levi.   1971.   Thermo-
    gravimetric Analysis.   In:   Encycl.
    Polymer Sci.  Technol.  Vol  14.    pp
     Ir41.
                                         171

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                                      - 5 -
                   Figure  1.  Outline of  EIR Review Process
                         | Appl leant subm.11=3 SIR|
    Public
 submissions
      V
 To ATSDR and
  forwarded
 to EPA/State
                                                (1)
     EPA/State does initial screen

     Completeness review of EIR
     based on Permit Applicants'
           Guidance Manual
   (coordinated with Part B review)
                                                    incomplete
                             revision
                 Additional data
                 froro applicant
                                   complete
                       Technical review of EIR
                    to address steps 2 through 6
                    (using other data as needed)
Gather further
 data/ using
permit process,
3004(u) RFA,
 enforcement
 orders, etc.
  unknown
new data.
                                         [2]
Is there evidence
 of significant
    prior or
   continuing
    release?
Gather further
 data, using
permit process,
 3004(u) RFI,
 enforcement
 orders, etc.
  Use of ORD,
 ATSDR, or PAT
 for technical
  assistance
  unknown
new
                                  \/
                                    [5]
  Could future
 release result
in significant
public exposure?
                                   yes
                                  V
                               [3]
   Is there known or
 suspected exposure to
    the public at
 significant levels?
                                   no
  Usual
permitting
 process
                                               yes
                                                            [6]
               Consider permit
                conditions to
              mitigate potential
                  exposure
              (or permit denial)
              Consider
         corrective action
             as needed
                      yes
                                       A
                                                    V
              Consider interim
             remedial action and
             public involvement
                 as needed
                             Consider Health
                           Assessment by ATSDR,
                             with HO (OSWER)
                               concurrence

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                             - 6 -


     This Guidance is organized according to the steps  in Figure 1.
A checklist and'-tables are presented in this Guidance to assist in
summarizing the results of the EIR review.  These checklists and
tables are provided as examples only.  The Regions are welcome to
revise the format and content of these documents in order to conform
to Regional priorities and methods.  Attachments at the end of the
Guidance include a completeness checklist (Attachment II), and
the types of health evaluations ATSDR may perform when  requested
(Attachment.Ill).

E.  Relationship to Existing RCRA Programs

     This Guidance describes the overall §3019 review process, and
how this review should be integrated into existing RCRA activities.
RCRA programs are already in place to identify, investigate, and
clean up prior/continuing releases to ground water (Subpart F
regulations) and other pathways (RFA/RFI process).  Therefore,
the two primary goals in implementing §3019 are to: (1) identify
human exposures to past releases that may require ATSDR involvement;
and, (2) to identify potential exposures from future releases that
may be mitigated by specific permit conditions.

     The RFA/RFI and permitting programs should provide the infor-
mation needed to determine if a release has occurred and if human
exposure is likely.  These activities should also generate most of
the documentation the EIR reviewer needs for the §3019 review
process.  The EIR reviewer is required to prepare a separate report
for §3019 when the Regional Administrator (or his designee) believes
that a site is a candidate for referral to ATSDR for a health
assessment.  This requires the submittal of a summary report to
EPA Headquarters for concurrence prior to referral to ATSDR (see
Section III.C.2).  The EIR reviewer should also produce a brief
memorandum for the administrative record at other important
decision points, i.e., the results of the completeness check/initial
screen (Step 1), and the examination of potential exposures to
future releases (Step 5).  In addition, the reviewer should write
a short memorandum for the record documenting a decision not to
refer a site to ATSDRj "and summarizing why the site does not meet
the necessary criterii^for referral (see Section III.B.I).
Documentation of these-decisions may be more important for sites
where public concerns exist.

     The prevention of releases and subsequent human exposure
should already be ah-integral part of the permitting process.
However, Step 5 of thei-.EIR review process provides the permit
writer with the opportunity to identify sites that require
special permit conditions to mitigate possible risks from
future releases.  Section III.D provides a qualitative approach
that may be used in completing Step 5.

     The exposure information review process outlined in Figure 1
illustrates the need to integrate this review with ongoing and
planned permitting and enforcement activities.  Which of the
Steps are completed prior to permit issuance depends, to some
extent, on Regional priorities for a particular site.  Normally,

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Steps 1, 2, 5, and 6 will be completed at most sites prior to
issuing the permit.  In addition, the permit writer should make
at least an initial decision whether the potential for significant
public exposure  (Step  3) warrants action via enforcement orders
(e.g., 3008(h))  before permitting.  Recommendations on the
appropriate use  of the investigation/corrective measure authorities
for the EIR review are described in Section III.B.

F.  State Roles  in EIR Reviews

     States with final authorization are required under 40 CFR
271.21(e) to adopt requirements equivalent to any new Federal
requirements.  Pursuant to Section 3006(g) of RCRA, the require-
ments of Section 3019 will be implemented by EPA until each
State receives authorization for this provision.  Until States
receive such authorization, the Regions may amend existing
grant Memoranda  of Agreement (MOA) with States to> allow them
to assist in reviewing the EIRs.  This may be especially helpful
where the State  is already reviewing the Part B application.
The State's role in implementing Section 3019 should be clearly
defined in the MOA or other agreements with EPA.  The Region
will need to oversee State reviews and follow up if more infor- "
mation is needed under Section 3019, if referral to the Agency
for Toxic Substances and Diseases Registry (ATSDR) is deemed
necessary,  or if new permit conditions are needed under 3005(c).
Section 3005(c)  (the "omnibus" provision) is discussed in
Section III.E. of this guidance.


II.  EIR INITIAL SCREEN AND COMPLETENESS REVIEW (STEP 1)

A.  Setting Priorities for EIR Reviews/Identifying Imminent
    Hazards

    Since the EIR is based in large part on information from the
Part B application, it makes sense in most cases to perform the
Part B and  EIR reviews concurrently.  Accordingly, the order
in which EIRs are reviewed depends largely on the order in
which the Part B applications-are reviewed.  (Since Part B
reviews should generally be conducted in order of environmental
significance, as reflected in .the-annual Agency Guidance and
the National Permits Strategy,: the-priorities for EIR reviews
will therefore have an environmental basis as well.)  Never-
theless, the permit writer should conduct an initial screen
of all EIRs upon receipt.  If the initial screen indicates
that the EIR provides- new evidence of a release and/or potential
exposure, the permit writer should reevaluate the environmental
significance of  the facility and consider raising the technical
review of the Part B and EIR to a higher priority.  If the EIR
reviewer suspects an imminent hazard, program and enforcement
personnel should be consulted immediately to formulate an
appropriate course of action.  Section III.C describes interim
remedial measures and corrective action responses that may be
necessary in these cases.

-------
     There will -be situations where the Part B and the EIR will
not be reviewe.d concurrently.  For instance, when an EIR is
submitted for a facility whose draft permit has been prepared,
it will usually be appropriate to conduct a full EIR review as
soon as possible even though the Part B review has already been
completed.  The EIR reviewer in this case must be particularly
careful to ensure that the data provided in the EIR and in the
Part B are consistent and that no new information is provided in
the EIR which affects the draft permit conditions.  Unless the
draft permit has already been issued, the EIR reviewer is advised
to review the EIR before the draft permit goes to public notice.

B.  Performing the EIR Completeness Review

1.  EIR Completeness Review Format

     The EIR should be reviewed for completeness "based on the
Permit Applicants' Guidance Manual for Exposure Information
Under RCRA 3019 (PAGM).  The EIR completeness review may be
conducted in a fashion similar to that used for a Part B
application completeness review.  The EIR reviewer may fill out
a completeness checklist and develop corresponding comments
to summarize any important omissions in the EIR.  A completeness
checklist has been provided in Attachment II and may be used
as a guide by the EIR reviewer during a completeness check.
This checklist is based on the permit applicants' checklist
found in the PAGM; however, it has been expanded and revised
to include a section on the "potential for human exposure"
narrative required of the owner/operator.

     Although the Part B and EIR reviews should be conducted
concurrently whenever possible, any requests to the owner/operator
for missing information required under 3019 should remain separate
from a Part B Notice of Deficiency (NOD) because the EIR is not
legally a part of the permit application.  The regulations in
40 CFR 270.10(c) were amended on July 15, 1985 to provide'that
a Part B which is not accompanied by an EIR will not be deemed
incomplete on that basis alone.  The permit writer may find
deficiencies in the Part B which impact-'the EIR.  In this
case, a warning letter or enforcement order containing the EIR
completeness comments should note these deficiencies by referencing
the deficiency comments in the Part B Notice of Deficiency (NOD).
For example, if the Part B inadequately described overtopping
control at the surface impoundment, then"the EIR checklist and
comments may simply instruct the applicant to: "See Part B NOD
Comment # 	 regarding overtopping control."  Any comments
generated from an EIR review should be simply entitled "EIR
Completeness Review Comments" rather than "Notice of Deficiency
Comments", to further distinguish the EIR review from the Part
B review.

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                             - 9 -. .

2.  Other Information Sources

   a.  Permit Writer .and Compliance/Enforcement Personnel

     In addition to the Part B application, several other infor-
mation sources may be useful in a completeness review of the
EIR.  Both the permit writer and the enforcement official may
have knowledge of the facility's history which will be helpful
in determining whether there are significant omissions in the
applicant's submittal or in pursuing any EIR reference to
other RCRA documents, such as 3004(u) SWMU response letters or
previous facility inspection, compliance, or enforcement reports.

   b.  Other Federal/State Agencies

     The EIR reviewer may consider contacting other Federal or
State environmental agencies during the completeness review if
an applicant's EIR refers to relevant information which is
contained in documents located at these agencies.  For example,
the EIR may reference or summarize NPDES permit information or
air monitoring reports which may be located in the Regional
EPA offices or State Water/Air Offices.  If the information
appears to be important (e.g., if a release is indicated) the
reviewer may wish to confirm that the document is accessible
and contains the expected information.   If important documents
are not accessible to the EIR reviewer (s)he may request the
applicant to submit a copy of the relevant information.

   c.  Public Submissions

     The Exposure Information provision of RCRA also allows the
public  to submit information on possible exposures.  Public
submittals may be received by EPA either directly, or via
reports forwarded to EPA trom ATSDR.  Upon receipt of public
submissions relating to a RCRA site, ATSDR should contact the
appropriate EPA Regional staff and forward a copy of the submission.
Regional staff should attempt to coordinate any needed response
to the  public with any response planned by ATSDR, and EPA Public
Involvement staff should be consulted in these situations.  In
addition to providing important information to the reviewer, a
report  of suspected human exposure from the public may create
a rather sensitive situation in terms of public fears and
expectations.  The Revised National Permits Strategy (July,
1985) encourages early publicinvolvementin permitting facilities
and directs Che Region or authorized State to prepare public
participation plans for "environmentally significant" facilities.
Furthermore, the Permits Strategy recommends that the exposure
information be included early in the public participation
process for these environmentally significant facilities.

3.  Determining the Adequacy of Submitted Information

     RCRA Section 3019 requires the applicant to provide all
"reasonably ascertainable information."  Although much of the
information in the EIR can be cross-referenced to the Part B
application, the PAGM does require the applicant to submit

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                            - 10 -

addicional information.  The legislative history of Section 3019
indicates thac Congress did not expect applicants to develop
major pieces of new information; however, if applicants do have
access to already existing data, they should submit or cite the
data, or provide an explanation as to why they could not obtain
the data.  See the PAGM for additional discussion of this topic.

     Unlike the requirements for the Part B, there is no regula- •
tory requirement for a "complete" EIR beyond the 40 CFR 270.10(j)
requirement to submit exposure information.   The PAGM states
that applicants who fully provide the information outlined in
that document will be considered to have satisfied the infor-
mation requirements of Section 3019.   From a practical viewpoint,
EIR reviewers should focus on missing information that will be
important in defining one of the three components of exposure,
i.e., data on releases, pathway characteristics,  -and target
populations.  Therefore, a reviewer need not literally apply
the PAGM information requirements and request that the applicant
submit missing information just for the sake of completeness.
Additional or missing information should only be requested
when it would be useful in determining human exposure.  For
example,  if an applicant discussed surface water use within a
two-mile  radius of the facility, rather than the three-mile
radius requested in the PAGM,  the permit writer should decide
whether the additional one-mile radius would really be helpful
in determining human exposure potential.

     An important question the EIR reviewer needs to consider
is the best way to collect the further information he/she feels
is necessary to complete the EIR review.  If the EIR submission
is obviously incomplete and information missing is deemed impor-
tant, the EIR reviewer may request through a warning letter or
an enforcement order issued under the authority of Section
3008, that the owner/operator submit the information.   If a
Part B Notice of Deficiency (NOD) is issued for the facility, the
EIR warning letter should accompany the NOD, if possible.
Additionally, the EIR information request may be included in
an enforcement order that is issued to require additional Part
B information.

     However, the needed information might also be gathered by
the reviewer directly from other sources (e.g., State files)
either during the. EIR review or, perhaps, as part of the initial
data gathering efforts for any RCRA Facility Assessment activities
planned under Section.3004(u).  The EIR reviewer must determine
which approach makes the most efficient use of resources while
also allowing important information to be gathered in a timely
and complete fashion.

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                             - 11 -

III.  EIR TECHNICAL REVIEW  (Steps 2 through 6)

A.  Evidence of Significant Prior or Continuing Release (Step 2)

     Once the EIR is determined to be complete, the reviewer
should review existing data for evidence of significant prior
or continuing releases from the subject landfill or surface
impoundment..  As noted previously, existing RCRA permitting and
corrective action programs should provide the information to
answer this question.

1.  Definition of "Significant Release"

     In the case of ground-water releases, Subparts F to
40 CFR Parts 264 and 265 provide regulatory definitions of a
"release".  Detection of any parameter above background usually
forces the owner/operator to undertake an extensfve monitoring
program to characterize the extent of the contamination.
Therefore, essentially all releases to ground water from units
subject to §3019 will be examined through the permitting process.

     Definitions of "release" for the corrective action authorities
(3004(u) and 3008(h)) are given in the RFA Guidance and in the
Preamble to the Codification Rule (50 FR 28713, July 15, 1985).
These documents define "release" as any spilling, leaking,
pumping, pouring, emitting, emptying, discharging, injecting,
escaping, leaching, dumping, or disposing into the environment.
Furthermore, the "environment" includes all media, i.e., air,
surface water, ground water, and unsaturated soils.  The RFA
process attempts to identify releases that threaten human
health and the environment.  Although Section 3019 is concerned
with only human exposure, these definitions used by the RFA
process are generally applicable to the 3019 process.

     A "significant" release can be further analyzed in terms of
the three exposure criteria, i.e., the type and amount of material
released, possible pathways for migration, and the presence of
nearby populations.  However, in this initial stage of identifying
releases, the primary concern is gathering enough data to confirm
that a release of potential significance has occurred.  The
extent and seriousness of a release will usually require further
investigation by the owner/operator.


2.  Useful Information Sources

    If the EIR does not contain conclusive evidence of prior or
continuing releases at the facility, or if the data concerning
the release are not complete, then the EIR reviewer can obtain
additional data via a number of information sources.  These
sources are described in more detail in the RFA Guidance/ and
relevant information should be gathered and assessed during
the initial stage of the RFA process.

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                            - 12 -

   a.  RCRA Part .B Permit Application

     One of the best sources of information is the Part B permit
application.  Most importantly, information concerning releases
to ground water is a required element of the application.  If
the facility has an adequate well system, the ground-water
monitoring data developed under Part 265 and § 270.14(c) should
reveal if releases to ground water have occurred.  Owners/operators
that have submitted inadequate ground-water data in their Part
Bs must upgrade their monitoring systems or conduct additional
sampling as needed.  See the Draft RCRA Ground-Water Monitoring
Technical Enforcement Guidance Document (August, 1985) for details
in addressing inadequate ground-water data.

     In addition, required Part B information concerning
contingency plans, unit designs, and other features of the
facility can provide useful background on any releases indicated.
The completeness checklist for the EIR given in Attachment II
lists portions of the Part B that may be relevant for assessing
releases .

   b.  RCRA Sections -3004(u) and 3008(h)
     Information concerning releases to surface water, air,
soil, and via subsurface gas may be obtained under the authority
of RCRA Sections 3004(u) and 3008(h), which authorize corrective
action for continuing releases.  Data can be gathered from the
SWMU letter responses, from the RFA process, and through 3008(h)
Interim Status Compliance Orders.  As described previously,
these authorities will perhaps provide the most effective means
of obtaining additional information.  The EIR reviewer should
consult the RFA Guidance for implementing 3004(u) and the
Porter/Price memo (December 16, 1985) on the use of 3008(h).

   c.  Compliance and Enforcement Records

     Information pertaining to the general compliance and
enforcement status of the facility should be evaluated with the
EIR.  In addition to the records of the operator's compliance
with the 40 CFR 265 requirements for ground-water monitoring, any
problems in compliance with other RCRA Standards may also be
indicative of potential releases.  Both the permitting and
enforcement files should be examined for evidence of improper
management of waste that may have led to releases to any other
pathways.

     Additional data gathered from other EPA programs, especially
CERCLA and NPDES, may also provide data on possible releases.
Superfund sources that may be useful include CERCLA PA/SI and
RI/FS reports and Reportable Quantity notifications.  Information  '
from Federal/State air and water agencies, OSHA, and transportation
related agencies may provide further evidence of release via

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                              -  13 -
the air, water, worker  management,  and  transportation  pathways,
resnectively.  Especially  useful  are  records  of  chronic violations
indicative of releases.  Although the owner/operator should
have  summarized much  of  this data in  the  EIR,  the  reviewer may
have  to oather referenced  documents or  incomplete/missing  data
from  these sources.


3.  Deciding Future Course of Action


      After considering  the data  initially  available the EIR
reviewer must decide  whether or not (s)he  needs  additional data
to rule out or confirm  the occurrence of  a prior (or continuing)
release.  If the available information  is  adequate, the  reviewer
may decide that no evidence for a significant  release  exists; in
this  case, the only Steps  remaining in  the EIR review  process are
5 and 6, i.e., the consideration of any impacts  of  future  releases
and oossible permit conditions needed to  address these  concerns.
On the other hand, if releases of potential significance are
known (or suspected)  to have occurred,  then a  more  detailed
examination of the exposure potential is  required as described
in the following section (Step 3).

      In some cases additional information  will be needed to address
possible releases to one or more of the exposure pathways.  As
noted above, these questions may be answered through the RFA
or normal oermittinq  processes.  Alternatively,  the EIR reviewer
may be able to qather enouqh information  from  existing  records
or other Reqional, State, or local officials to  satisfy lingering
doubts or conerns about particular leaks,  accidents, etc.

     Figure 2 provides an example of how evidence of releases
and possible follow-up actions for each pathway  were summarized,
followinq review of an actual EIR and other information  regarding
a RCRA site.   While this example was derived from a review of
data  from an actual facility/ the case was simplified  somewhat
for il lustratative purposes.   In order to  put  this  example in
perspective,  Figure 2 also contains background information on
the site.

      Figure 2 describes the follow up actions  that might be
undertaken during Step 2 to determine if a release has  in  fact
occurred, and whether the release warrants  further  investigation.
The EIR reviewer may wish to write up a short  summary  of the
results of his/her analysis at this stage  in the process.
However, other reports or records produced as  part  of  the
nermittinq or RFA process should be adequate to  document this
staqe of EIR review.

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                                       -  14  -

                  Figure  2.   Example of Summary Sheet Following  Initial Review
                             of Release Data:  Release Evidence and Suggested
                             Follow UD.
 Ooerations:
 Units of Concern:
 Location:
               Background Summary of Example Site

    A small off-site cororercial facility treats and stores hazardous
    waste; operations  include waste oil/gasoline recycling, cyanide
    waste treatment, solvent recovery, other treatrtent.

    Surface impoundments are used to store and treat wastes before
    discharge to waste water treatnent plant on site.

    The  facility is located in an industrialized area, also bounded
    by residential areas.
   Pathway


Ground Water
Surface
Water
Air
Soil
 Summary of Release Evidence
Existing Part B data not adeguate;
monitoring Plan in developnent.
Possible releases via contaminated
run-off fron area around unit which
enters v«ter through municipal sewer
systan; subseguent treatment by POIW
unclear.

Definite release based on odor.
State monitoring program in
development.  Sane corrective
action also taken.
Likely releases from spills,
leaks, and accidents.  Extent
of clean up of these past
releases unclear.
  Possible Follow Up Action
Follow peEmitting/enforcement
procedures to obtain necessary
monitoring data.

Determine if run-off should be
managed as hazardous waste.
Collect available analytical
data on run-off and determine
if discharge goes to POTW.

Obtain data fron air monitoring
program whe:. available, then
consider need for futher inves-
tigation to study extent of
potential exposure and adequacy
of corrective action taken.

Examine any existing soil
analysis undertaken and assess
need for RFA or RFI follow up.

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                                      - 15 -
                                 Figure 2.    (contirued)
   Pathway
     Release  Evidence
 Possible Follow UD Action
Subsurface
Gas
No evidence;  unlikely  for
surface  impoundment.
     None necessary.
Trans DO rt at ion
Management
Practices
Facility, sweeps  nearby streets
to remove dirt,  perhaps due to  •
track-out problem;  may not be
related  to operation of surface
impoundments.  No  record of
releases  from spills off-site.

Occupational records submitted do
not indicate significant illnesses
due to unsafe cperating conditions.
No other  serious enforcement problems
found for facility operation, beyond
those already noted.
Review existing soil analysis
as noted above.  Consider
requiring o/o to analyze dirt
found on nearby residential
street for likely hazardous
constituents via RFA or RFI.

     None necessary

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                             -  16  -

3.  Determination of  Known/Suspected  Public  Exposures  at
    Significant 'Levels   ( S t ep  3 )

     Once a prior or  continuinq release  from the  surface
impoundment or landfill  has  been  documented,  the  EIR reviewer
"lust determine whether the public  has been exposed  to  the
release, and if so, whether  there  is  "substantial potential  risk"
due to that exoosure  (see  §3019(b)).

     The three human  exposure  elements noted  earlier must  be
addressed in order to determine whether  the  public  has been
exnosed to a hazardous release and the significance of this
exposure.  Listed below  are  the three  exposure elements and  the
information needed by the  reviewer to  assess  the  presence  of
these components.  When  a release  of  concern  from a unit is
identified, then the  reviewer must assess the adequacy of  the
supportinq evidence to confirm that all  three  elements for
public exposure are documented.


1.  Human Exposure Components

   a.   Evidence that  the  release from  the landfill  or  surface
impoundment contains hazardous wastes  or constituents.
Documentation would include:

 o   Monitorinq data  confirming a  release from the  unit; and

 o   Data indicating that the hazardous  materials or constituents
     of concern are present  in the release from the unit.


   b.   Evidence that the release containing hazardous  materials
or constituents of concern has m iqrated  off-site  (or to on-site human
exposure point).   Evidence includes:

 o   Monitorinq data confirming off-site contamination; and

 o   Monitoring/modeling data indicating the  extent of release
     and migration via a plausible  pathway.


  _c._ .Evidence showing a likelihood  that a nearby  population
has been, or is being, exposed to  toxic  constituents from  the
release at levels constituting a substantial  risk to human health.
Information needed would include:

 o   Monitoring/modeling data suggesting that  the public is being,
     or has been,  exposed (e.g., contaminated drinking water
     wells );  and

 o   Data showing levels of  constituents at the exposure point
     indicative of a health  threat  (e.g., levels  exceed existing
     Agency standards  or criteria).

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                             - 17 -

2.  Gathering Da'ta to Document Exposure

    a. Use of the Permitting Process

     The permit writer should use the permit process and the
3UU4(u) program to gather information concerning possible releases
and human exposure.  The first exposure element, the existence of
a documented release, should have largely been satisfied by a
positive determination for Step 2.  Any release should be documented
through the usual permitting process (for ground water) or through
30U4(u)/3008(h) RFA studies (for other pathways).  The second
element, documented off-site migration, will normally require the
owner/operator to investigate the extent of migration, both in
terms of the constituents released and the area contaminated.

     In the case of ground water contamination, the existing RCRA
Subpart F regulations require the owner/operator to characterize
the plume of contamination in some detail, and devise a corrective
action program.  The contaminated ground water must be cleaned up
to Ground Water Protection Standards set at background levels or
existing drinking water standards, unless an Alternate Concen-
tration Limit (ACL) is approved.  An ACL demonstration is
essentially an exposure/risk assessment for a ground water
contaminant, and a successful demonstration should be sufficient
evidence that no potential for significant human exposure
exists for that constituent.  An unsuccessful ACL demonstration
may still provide information useful to the EIR reviewer in
deciding if human exposure is likely.

      However, the existing Subpart F regulations only require
the owner/operator to clean up contamination to the facility
boundary.  Section 3UU4(v) of HWSA requires corrective measures
(tor releases to all pathways) beyond the facility boundary, but
§3UU4(v) has not yet been codified in the regulations. (Pending
promulgation of these regulations, EPA may issue 3008(h) orders
to implement the directives of 3004(v).)

     In some cases of suspected off-site migration of unit
releases, the owner/operator may elect to gather off-site data
to establish.-the'presence and extent of any contamination.  In
the past, cooperative owner/operators have been willing to
monitor off-site.ground water for plume movement in order to
devise adequate^corrective action plans, or to support ACL
demonstrations.; Permit writers are encouraged to try to obtain
data on oft-site releases from willing owners/operators.

     for releases to pathways other than ground water, the
owner/operator may be required to gather data on the extent of
contamination under either 3004(u) or 3008(h) authorities.  The
permit writer must realize, however, that an investigation under
3(J04(u) on the-extent of the contamination may not be initiated
until after the permit is issued.  Generally, compliance schedules
will be used in the permit to require the owner/operator to

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                               -  13  - '

conduct  a RCRA  Facility  Investigation (RFI)  under 3004(u).   Some
information  on  the  level  of  contamination may be  gathered from
the owner/operator's  response  to  the  initial  SWMU letter  and
from the RFA investigation  performed  under 3004(u).   However,  in
most cases,  monitoring results at this  stage  will probably  be
focused  on detecting  a release  from  a SWMU,  not  on determining
the extent of contamination.

     Because  RFIs reguired under  3004(u)  will not generally be used
to aather data  prior  to  oermit issuance,  the  permit  writer  (in
conjunction with appropriate enforcement  staff)  should  consider
whether enforcement orders are needed to  ensure an  investigation
of releases  and the likely human  exposure potential  before  permit
issuance.  The  following  section  describe  the  enforcement
authorities  that might be used and the  situations  that  may  warrant
their use.

   b. Use of  Enforcement  Orders

     An enforcement order may be  issued to reguire  the
owner/operator  (o/o)  to  aather information (on-site  or  off-site)
under 3013 or 3008(h) authorities for releases to any pathway.
The issuance  of a 3013 order reouires evidence showing  that the
presence or release of hazardous  waste  from a  facility  may  present
a substantial hazard  to human health  or the  environment.  Note
that 3013 oives EPA the authority to  perform  any  needed investi-
aations and  recover the costs later  if  the o/o is incapable of
(or refuses to) gather the reguired  information.  The use of a
3008(h) order reouires evidence that  a  release (to  any  medium)
has occurred.  See the RCRA Ground-Water  Monitoring  Complicance
Order Guidance  (August,  1985) for a  description of  these  two
types of orders, and  the  recent Porter/Price  Memo on the  use of
3008(h), "Interpretation  of Section  3008(h) of the Solid  Waste
Disposal Act" (December 16,  1985).

     Whether  to undertake the investigation of a  release  from  a
facility through the  permitting process or an  enforcement order
will depend on Regional1 priori ties, resources, and  various  site
soecific factors.  Thrirs decision will encompass considerations
that qo beyond the ffumarn  exposure concerns of  the  3019  EIR  review
process.  For example,1 "3008(h ) orders may be  used  when  a  release
is miaratinq  rap id IY^ ~and;  may move off-site.   In addition, the
corrective action programs will be used to investigate  releases
from all suspect SWMUs:-at a  facility, not  just regulated  landfills
and surface impoundments'.

     Another  important factor to  consider is  how  close  the
facility is to receiving a permit.  If permit  issuance  appears
likely within the near future, the permit  writer  might  decide  to
incorporate a compliance  schedule for a RFI in the permit,  rather
than hold up  the permit while awaiting the issuance  of  an order
to gather more information.  A related concern is  the level of
cooperation exhibited by  the owner/operator  in the past,  and the
likelihood that he will meet the compliance schedule for  RFI in
the permit.

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                              - 19 -

     Situations'- which mighc prorapc che permit wricer to seek more
immediate exposure information than could be provided through
the 3004(u) process include cases in which the existing data
indicate a high potential for human exposure.  The EIR reviewer
should undertake a preliminary analysis of available information to
estimate the potential impact of a known release.  For example,
if evidence of a release and movement off-site to surface water
exists (e.g- ,  fish kill, complaints of tainted water), the EIR
reviewer should consider the likelihood of releases from the
unit reaching  surface water (distance to river, characteristics
of intervening terrain), potential transport and dilution
(river flow and size vs. potential release, the properties of
likely constituents in a release) , and the likelihood of human
exposure (distance to downstream intakes, other uses of surface
wa t e r).

     After such a preliminary analysis, the EIR reviewer may
determine that the release requires attention prior to permit
issuance.  In  such cases, the EIR reviewer should consult with
enforcement and permitting personnel to map out an appropriate
strategy (which may include the use of 3008(h) or 3013 orders)
to obtain the  needed data and initiate corrective action.

     Even in cases of suspected human exposure, the RFI may be
implemented through the use of 3004(u) compliance schedules if
there is no current (or imminent)  exposure potential.  For example,
a case of past human exposure (e.g., eating of contaminated
fish)  due to a prior (but not continuing) release to surface
water, might be addressed after permit issuance if no current or
imminent human exposure is expected. [Note, that if the elements
of exposure can be adequately documented, these situations may
still be candidates for referral to ATSDR as described in
Section III.C.2.J

   c.   Other Sources of Information

     Many of the additional information sources used in determining
evidence of a  release may also:provide data on migration of the
waste off-site and possible human exposure.  Particularly important
at this stage  in Che review^is-any evidence of health complaints
related to Che sice.  Pub lie..submissions may provide indications
of exposure.  For sices with•„ suspected human exposure, local or
State health departments sho.uXd also be contacted by the EIR
reviewer co check for any reporcs of health concerns in the
immediate vicinity of che facility.  It is important for Regional
and State pennitcing -scaff Co escablish concaccs wich che local
healch departments for sites at which real problems may exist.
For sites thac are evencually referred co ATSDR for healch asses-
sments,  one of Che firsc seeps caken by ATSDR would be co concact
chese local deparcmencs for healch complaincs in che area.

3.  Technical  Assiscance

     The EIR reviewer is encouraged co use all of che above infor-
macion sources and rouces for gachering che daca necessary co

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                            - 20 -

confirm the existence (or absence) of all chree exposure com-
ponents (release, migration, receptor location).  After examining
the data gathered under the permitting and enforcement processes,
the EIR reviewer may have some questions concerning the potential
health impacts of documented/suspected human exposures. . The primary
contact for technical assistance will be the Permit Assistance
Team (PAT) at Headquarters as described below.   The capabilities
and possible uses of ORD and ATSDR are also discussed.  Finally,
existing EPA manuals which could provide the EIR reviewer with
possible approaches for interpreting the assembled data are
noted.

   a.   Permit Assistance Team (PAT)

     The EPA Permit Assistance Team (PAT) at Headquarters
(FTS/382-4740) stands ready to provide technical assistance.
to coordinate assistance from ORD and ATSDR, and^ to provide help
in deciding when referral to ATSDR is warranted.  ORD and ATSDR
may, to a limited extent, be accessed directly by the EIR reviewer
on a consultative basis by telephoning the appropriate individuals
(see below).  Such informal consultations could provide quick
response to questions on possible health effects raised by infor-
mation available at that point.   However, if- the EIR reviewer
needs more extensive technical assistance (e.g., detailed review
of written reports, monitoring data, models, etc.), (s)he should
contact the PAT at Headquarters.  The PAT will draw on the
expertise available within OSW,  other EPA Offices, and ATSDR
as needed to respond to the Regional request for assistance.
If warranted, health assessments may be recommended for some
facilities, as described in Step 4 of EIR review process.

   b.   Office of Research and Development (ORD)

     The office within ORD which may be useful to the EIR
reviewer is the Office of Health and Environmental Assessment
(OHEA).  Within OHEA, the two groups which can provide the most
assistance in evaluating EIRs are the Exposure Assessment Group
(EAG),  located in Washington, D.C., and the Environmental Criteria
and Assessment Office located in Cincinnati, Ohio (ECAO-Cin).

     ECAO-Cin can provide assistanee~in determining whether any
constituents found at off-site exposure points constitute a
public  health threat at measured or projected exposure levels.
ECAO-Cin has developed a Rapid Response Toxicity Program to aid
Regional and State offices in quickly (i.e., 48 hrs.) evaluating
potential human health hazards posed by chemical releases.
These responses may include: rough estimates of cancer risk or
toxic potential; identification of key chemicals tor further
monitoring; a rough description of possible exposure situations
and their potential health hazards; and some recommendations for
future assessment efforts.

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                              - 21 -

     Most recommendations will require the involvement of EAG to
evaluate monitoring data/methods and for a discussion of likely
exposure scenarios and their uncertainties.  While this program
is designed to provide only preliminary estimates of health
hazards, more detailed site assessments can also be provided.
Requests for rapid technical response from ECAO-Cin may be
forwarded directly to Chris DeRosa (FTS/684-7534).  Requests for
more detailed assessments should be sent to the PAT, which will
coordinate ECAO/EAG assistance.

     Through the PAT, OHEA may be able to help the EIR reviewer
complete an exposure/risk analysis to project the likely effects
from past or ongoing exposure to hazardous constituents.  With
the expertise available in OSW and ORD, the PAT can recommend a
variety of models for use at a particular site, and may be able
to assist in using this type of analysis in determining the
extent of constituent transport via the usual pathways and the
likely levels of contamination at projected exposure points.
The PAT may also provide assistance in reviewing any analyses or
projections submitted by the owner/operator.

   b.  The Agency for Toxic Substances and Disease Registry
       (ATSDR)

     RCRA §3019 specifically identifies ATSDR as a potential
participant in the evaluation of exposure information.  ATSDR is
an agency within the Public Health Service, Department of Health
and Human Services.  Its overall function is to carry out
health-related responsibilities under CERCLA and RCRA.  An Inter-
agency Agreement (IAG) has been established to define RCRA-ATSDR
interactions, and a Memorandum of Understanding  (MOU) is currently
under development.

     Sites will be referred to ATSDR when a health assessment is
warranted, as described in Step 4(b).   ATSDR has the ability to
perform several different levels of health assessment (see
Attachment III), and the more extensive studies will usually be
preceded by more limited investigations..  ATSDR's major task in
any level of health assessment will be to evaluate populations
with known (or suspected) exposure to hazardous.constituents
as a result of a release from a regulated surface impoundment or
landfill.                                  ..,-" "".

     As noted in the Attachment III, ATSDR may also provide
informal "health consultations" to provide health advice and/or
health effects information regarding a specific site.  The Regions
should limit their consultative use of ATSDR before referral
to situations that require relatively short-term assistance,
e.g., assistance available through a telephone call.  Requests
for more extensive work should be sent to the PAT (ATSDR will
also have a representative on the PAT), and the PAT.will coordinate
ATSDR assistance.  The EIR reviewer may contact Ralph Touch at
ATSDR (FTS/236-4551) directly for short-term technical assistance.

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                              - 22 -

   c.  Technical Documents

     The EIR reviewer may consult a number of EPA manuals
which provide a variety of approaches in assessing the exposure
potential and health impact of releases from hazardous waste
sites.  As mentioned previously, the RFA Guidance may prove
useful in the early stages of release investigation.   Perhaps
most helpful in cases when the EIR reviewer feels a more extensive
analysis of exposure potential is waranted is the Superfund
Public Health Evaluation Manual (December, 1985)  and  the companion
Superfund Assessment Manual (January, 1986).  Copies  of these
manuals have been distributed to Regional Division Directors and
Branch Chiefs; current information on the availability of these
documents may be obtained by contacting OERR (382-2182).

     Elements of the Public Health Evaluation Manual  that may be
useful in cases where seriousexposureproblems are suspected
include: procedures for selecting indicator chemicals;
physical/chemical and toxicity data for chemicals; and a summary
of existing EPA standards and criteria for hazardous  substances.

     The Exposure Assessment Manual is a complex and  highly
technical compendium of approaches and models to use  in assessing
exposure potential.  The data requirements of the various models
discussed are provided.   The extensive data needs illustrate
the major problem in undertaking such a detailed analysis,
i.e., much of the information needed to use quantitative modeling
will not be available at many RCRA sites, and expensive and
lengthy data gathering efforts would be required.  Therefore, the
EIR reviewer is urged to limit the use of complex models unless
the data are available,  and may seek assistance in the use of
these manuals from the PAT.

C.  Possible Actions in Cases of Human Exposure
    (Steps 4(a),  4(b) , and 4(c))

     If the EIR reviewer believes that more information is required
to decide if a release has resulted in known or suspected exposure
to the public at significant levels, (s)he should obtain the
necessary data as outlined above.  If (s)he decides, that the
criteria for human exposure (see Section III.8.1) are not met,
and that significant human exposure is unlikely, then the EIR
reviewer muse still consider whether corrective action is needed
to clean up che release (Step 4(c)).  After this, the reviewer
should also consider the impact of future releases (Step 5) and
possible permit changes, if needed (Step 6).  These steps are
discussed in later sections of this guidance.  The EIR reviewer
may wish to prepare a short report for the administrative record
summarizing decisions not to refer facilities for health assessments.
Such reports may be useful documents tor explaining the decision
during public hearings.

     If the components for human exposure given in Section III.B.I
are present, there are several actions the EIR reviewer should

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                            - 23 -

consider.  These actions include implementing interim remedial
actions with appropriate public involvement (Step 4(a)), referral
to ATSDR for a health assessment (Step 4(b)), and final corrective
action (Step 4(c).  Which actions are completed and the order
in which these activities are pursued will depend on the situation;
normally, however, the need for interim measures should be
assessed first to insure that continuing public exposure is
minimized.  Furthermore, while a completed health assessment
could be useful in designing a final corrective action plan,
corrective action should not be significantly delayed.

1. Interim Remedial Action (Step 4(a))

     Interim remedial measures may be necessary to prevent
further human exposure.  These may be pursued through the various
enforcement and program authorities available to EPA, such as
RCRA Sections 3008 and 7003, and CERCLA Sections ^104 and 106.
Examples of interim remedial action would include off-site and
source control measures, such as:

   o  evacuation of the public from the area if the problem is
      so serious as to pose an imminent and substantial
      endangerment;

   o  requiring the owner/operator to provide bottled water
      and/or drinking water treatment when public drinking
      water is the pathway of exposure;

   o  temporary suspension of facility operations that may cause
      or exacerbate the problem;

   o  temporary removal/storage of wastes of concern, and
      other interim measures to contain or prevent releases (e.g.,
      berm stabilization).

The EIR reviewer should consult with appropriate permittin-g and
enforcement staff to map out a plan for needed remedial actions.
A review of response actions available under §3008(h) may be found
in the draft guidance, "RCRA §3008(h) Corrective Action Interim
Measures", issued by OWPE (latest draft, May 13, 1986).  The reviewer
should also contact public participation staff in order to design
and implement a public information program to inform the public of
the health concerns associated with the facility and the immediate
and long-term actions planned to address the problems.


2. Referral to ATSDR for Health Assessment  (Step 4(b))

   a.  Referral Authority and Concurrence

     If there is sufficient evidence that a release from a
regulated surface impoundment or landfill has resulted in
significant human exposure (i.e., if the three necessary components
of exposure have been established for any of the exposure pathways),
then EPA (or authorized States) may refer the facility to ATSDR
for a health assessment (Step 4(b)).  While the statute originally

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                              - 24 - .

assigned the authority to refer a facility to ATSDR to the EPA
Administrator, this authority has been delegated to the Regional
Administrators.   The Regional Administrator, if (s)he so chooses,
may redelegate the authority to the Division Director level.

     However, the Delegation provides that, before seeking a
health assessment from ATSDR under §3019, the Region must obtain
the concurrence of the Assistant Administrator for Solid Waste and
Emergency Response.This concurrence requirement is designedto
ensure tnatimportant sites are assessed first, and to encourage
national consistency in the types of sites that are referred  to
ATSDR.  Regions seeking concurrence for referrals to ATSDR should
contact the Permit Assistance Team (PAT) at EPA Headquarters
(contact Terry Grogan or Bob Kayser, FTS/382-4740).   The PAT  will
coordinate the review of the information by OSW, OWPE, ATSDR,  and
other EPA offices (e.g., ORD) as needed, and make recommendations
to the Assistant Administrator concerning the referral.

   b.  Documentation of Referral Request

     When a Region believes that a health assessment by ATSDR  is
necessary, the EIR reviewer must prepare a written report for  submission
to Headquarters which summarizes the exposure analysis completed
to date, and identifies the pathways of concern.  This report  will
serve several functions, including: (1) forcing the EIR reviewer
to formally consider the adequacy of the assembled evidence prior
to referral; (2) allowing the Headquarters concurrence group  to
review the data in a timely manner; and, (3) providing a useful
summary document for initial review by ATSDR, if a health assessment
is required.

     This report must summarize the evidence that the three elements
for human exposure are present at the site.  Section III.B.I
describes the kinds of evidence needed to document human exposure.
The report should follow a logical format and should include:

0   background information on the facility (location, types of
   wastes handled, brief description of all units on site, nearby
   land use, map of facility);

0   evidence confirming a significant release from the regulated
   surface impoundment or landfill (monitoring data and the level
   of confidence in data, all hazardous constituents detected,
   approximate quantitity of wastes released, identification  of
   major constituents in waste);

0   evidence indicating extent of contamination and migration  path-
   way of released constituents (monitoring data or modeling  results
   showing movement off-site, the ranges of substances detected
   throughout contaminated area);

0   evidence indicating a likelihood of human exposure via ingestion,
   inhalation, or direct contact at levels suggesting a potential
   health threat (location of nearby populations, monitoring

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                              - 25 -

   data at exposure point, health complaints from public, records
   of local health departments, constituents measured or projected
   at levels exceeding Agency standards or other health-based
   criteria);

0  on-going or planned activities to collect more data and institute
   remedial action at the site (including public participation
   plans ) ;

0  results of any preliminary evaluations or assessments of site
   data undertaken by the State, Region, ORD, ATSDR, the o/o, or
   others;

0  level of health assessment sought (if possible, include specific
   questions ); and,

0  name and phone number of Regional/State contacts most familiar with
   details of the site.

     The report should summarize pertinent monitoring data in
tabular form with clear indications (i.e., on a map) of the sampling
locations.  Any analysis of the data (e.g., by the owner/operator,
contractors, Regional/State staff) should be succinctly described,
and any references used must be cited.  While the level of effort
required to prepare the referral report will vary with the complexity
of the site, the report should be a summary document, not a lengthy
treatise on the facility.  Source documents (Part B, EIR, etc.)
should be referenced for details, and copies of important pages
from these documents may be provided.

3.  Corrective Action  (Step 4(c))

     Corrective action will be considered whether or not the EIR
reviewer determines that significant exposure to the public has
occurred.   If exposure routes have been documented and a health
assessment is initiated, appropriate permitting and enforcement
staff should be kept informed.  Permit and/or enforcement staff
developing the corrective action plan should coordinate the plan
with the health assessment, if necessary.  The level of clean-up
may be affected by the results of the assessment, if for example,
the health assessment uncovers a causal link between the level
of the hazardous constituent at the exposure point and the parti-
cular health effects in the exposed population.  In most cases,
however, the permit writer is urged to proceed with permit issuance
to begin initial clean up activities if the available data on
the extent of contamination are adequate.  The permit may be
modified to incorporate any useful information arising out of
health assessment activities.  As described in section III.B,
§3008(h) orders may be used to institute corrective action prior
to permit issuance.

     The EIR reviewer may decide that the evidence does not
indicate that significant public exposure due to prior/continuing
releases has occurred, and therefore, that referral to ATSDR is not
warranted.  However, the permit writer should still examine the need

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                              - 26 -

for corrective measures to lessen the possibility of f ut u r e
exposures to past releases.  In the case of ground-water
contamination, of course, the Subpart F regulations (§264.100)
require clean up to levels set by Ground-Water Protection Standards.
There are other corrective action measures to take and several
vehicles for requiring these measures.  Guidance is being developed
to assist the permit writer in instituting corrective measures
under 3004(u), 3004(v), and 3008(h).  These authorities are the
primary vehicles available to the permit writer for clean up of
releases from regulated units to media other than ground water.

     In those situations involving an imminent and substantial
endangerment to public health, EPA may take action under 7003 of
RCRA or 106(a) of CERCLA to institute remedial action.  The
"Endangerment Assessment Memorandum" issued by J. Winston Porter
(November 22, 1985) provides guidance on the preparation of
endangerment assessments to support all administrative and judicial
enforcement actions under CERCLA Section 106 and RCRA Section
7003.  An endangerment assessment must be developed in order to
document and justify that an imminent and substantial endangerment
to public health or welfare exists.  A supplement to the Guidance
has also been prepared by the Office of Waste Programs Enforcement,
in draft form, entitled the Endangerment Assessment Handbook
(August, 1985).

     These authorities described above allow EPA to force clean
up of releases prior to actual human exposure.  Therefore, the
EIR reviewer and/or permit writer should consult with enforcement
staff in cases that warrant corrective measures prior to permit
issuance.  Section III.E. of this guidance should also be consulted
for possible use of the new "omnibus" provision (3005(c)(3)) in
establishing additional permit conditions to address potential
exposure concerns.


D. Determining the Potential for Significant Public Exposure From
   Future Releases (Step 5)

     In addition to evaluating prior/continuing releases from all
regulated surface impoundments or landfills (steps 2 through 4 in
Figure 1), the EIR reviewer must also address the potential for
human exposure in the case of future releasest (step 5).  As such,
Step 5 is the most conjectural part of the EIR review.  When
reviewing EIRs for new landfills and surface impoundments, the
EIR review will consist only of this Step and Step 6, consider-
ation of permit conditions necessary to prevent human exposure.
The timing of Step 5 may vary depending on the need to investigate
prior releases.    In addition, the EIR reviewer and/or permit writer
may wish to use this analysis of the impact of future releases
as a tool in focusing attention on human exposure potential
throughout the permitting and RFA/RFI processes.
f'Future releases" also include releases that may have already
 occurred; but are not yet detected.

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                              - 27 -

1. General Approach

     The reason for examining the impact of future releases is
to highlight pathways of concern and allow permit conditions to
be modified or strengthened to mitigate site-specific potential
problems (Step 6).  Of course, the occurrence of prior releases
to a particular pathway, and any evidence of subsequent migration
and human exposure,.should be used as the primary indicator of
the potential impact of future releases.  This is why the flow
chart in Figure 1 also leads the EIR reviewer to consider the
impacts of future releases (Step 5) after the process for prior
releases (Steps 2-4) is followed.

     In the absence of a history of past releases, however, the
EIR reviewer should consider the potential exposure rf a release
should occur.  The EIR reviewer is encouraged to,use a qualitative
approach for screening facilities for possible exposure concerns
from future releases.  In a limited number of cases a more detailed
evaluation may be warranted if the initial qualitative screen
indicates that a future release from the unit is likely to result
in significant human exposure.  In these cases,  the permit writer
may wish to quantify possible exposure scenarios in order to
justify the imposition of permit conditions that go beyond the
existing Part 264 standards (see next section for a discussion
of the new "omnibus" provision).  Future guidance will provide
information on applying a more quantitative approach.

     The EIR reviewer may follow the general approach outlined
below to qualitatively screen units.  This approach examines the
same elements for exposure as defined for past releases (i.e.,
release, migration, and receptor location).  Due to the prospective
nature of the evaluation, however, the approach  first examines
the route characteristics and receptor information assuming a
release occurs.  If a potential concern is identified, the design
and operating features of the unit should be critically examined
for their adequacy to prevent or detect releases.  The infomation
needed to evaluate the major pathways should be  available from
the EIR, the Part B, or the other information sources mentioned
in Section I.

     The requirement under 3019 to consider the  impact of future
releases (i.e., Step 5) has many features in common with the RCRA
RFA process designed to implement 3004(u) and 3008(h).  The
potential for future releases becomes an important factor if the EIR
reviewer decides that a particular pathway is of concern.  There-
fore, the EIR reviewer (and permit writer) should use the results
of a RFA investigation as a valuable source of information in
deciding if the location, design,  and operating  features of the unit
are adequate to prevent (or render less likely)  future releases
to pathways of concern.

     Because the RFA and EIR review processes share many similar
concerns relating to the potential for a release and subsequent
migration off-site, many elements of the methods given in the RFA
guidance have been incorporated into the following qualitative

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                              -  23  -

approach.  The followi.no sections describe  important  factors  for
each pathway that should by considered  in an  initial qualitative
screen .


2.  Pathway-Specific Factors

   a.  Ground Water

     The EIR reviewer should examine the pertinent hydrogeological
and geoloqical factors of the site, as well as the location of
possible taraet populations, in order to assess  the potential
impact if a future release to the ground-water pathway occurred.
The important route characteristics and receptor  information  to
examine are described below.

Route Characteristics Affecting Exposure Potentia.l

     An evaluation of the ground water pathway should indicate
the potential for contaminant movement through the unsaturated
zone to the aguifer and subsequent off-site migration in the  ground
water to human receptors.  Therefore, the important characteristics
to examine should include the soil characteristics (i.e., per-
meability) of the unsaturated zone, the depth of  the aquifer, and the
flow rate and direction of the ground water.  If  the hydrogeology
of the site is properly defined in the Part B (including at least
the oermeablity of the saturated zone and the hydraulic head),
the EIR reviewer should be able to estimate the  time-of-travel  (TOT)
for the around water to the facility boundary, and perhaps to
the nearest off-site downgradient well.  Other factors which may
be important at some sites include the local climate (e.g., net
precipitation,  which would effect the generation  of leachate),
the existence of confined aquifers, the discharge of ground
water to surface water, and seasonal variations  in the water
table.

     Receptor information of prime importance include the location
of the  nearest down gradient wells, the uses of the ground water
in the area, and magnitude of the population served by nearby wells.
While drinking ground water is an obvious exposure route, other
ground  water uses may lead to human exposure through contamination
of food crops (irrigation uses) or other food products (milk).  In
addition, nearby populations may be impacted if  the site character-
istics  promote basement seepage into nearby buildings.

     An example of a site of obvious concern would be one at which
the unit overlies a highly permeable unsaturated  zone (sand,  silt,
permeability > 10~4 cm/sec), the aauifer is shallow, the ground-
water flow is moderately fast, perhaps due  to faults, joints, or
solution channels (TOT to facility boundary < 5   yrs.), and
nearby  drinkinq water wells lie down gradient (TOT to nearest
well <  10 yrs.).   Conversely, if the aquifer were situated
below an extensive impermeable layer (clay; permeability < 10~°
cm/sec), the ground water flow was slow (TOT to  facility boundary
> 50 yrs.), and the aguifer was not presently used by nearby

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                              - 29 -

populacions, then the EIR reviewer could decide chac exposures
via chis rouce are unlikely if a release occurred.

     Sicuacions which are noc so clear-cut may scill be of only
limited concern if either a reasonable migration route (i.e.,
moderately fast ground water flow to off-site wells),  or likely
target receptors (i.e., nearby populations using the ground
water) are not present.  For these intermediate cases, however,
the EIR reviewer may require more information on the hydrogeology,
receptor locations, or aquifer uses.   More definitive guidance
on evaluating ground-water vunerability may be found in the manual
Criteria for Identifying Areas of Vunerable Hydrogeology Under
the Resource Conservation and Recovery Act (OSWER7 July,1986).
The EIR reviewer should refer to this guidance if a more complete
analysis of ground water location characteristics is warranted.

Unit Design and Operating Features

     If the EIR reviewer has some concerns about the possible
exposure to the public from releases to the ground water, then
(s)he should undertake a review of the relevant design and
operating features of the unit.   The relevant features of landfills
and surface impoundments are related to the containment of
leachate and the leak detection/monitoring systems.  The adequacy
of the liner and leachate collection systems, leak detection
procedures (e.g., routine leachate analysis), and the ground-water
monitoring systems around the units should be reexamined.  During
this examination, the EIR reviewer should decide if any modifications
to the existing systems are necessary to reduce the likelihood
of releases (or increase the probability of detecting releases)
to the ground water.  Any special waste characteristics, or pre-
treatment process that might affect the amount of liquid waste
managed should also be considered.

   b.  Surface Water and Drainage

     Assuming a release might occur, the EIR reviewer should first
evaluate the potential for human exposure.  Releases that occur
to surface water and off-site surface drainage areas may arise
from leaks, surface run-off, spills, or floods.  The effectiveness
of pertinent'design/operating features should be examined if the
EIR reviewer concludes that this pathway is of concern.

Route Characteristics Affecting Exposure Potential

     The primary considerations in evaluating the potential
for human exposure for this pathway are the proximity of the
unit to surface water, the likelihood that a release would
migrate overland, and the current uses of the surface water.
Therefore, the requirements for a realistic surface water pathway
for human exposure generally would include all of the following:

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                              -  30 -
 0 surface water  located  close  to  the  unit;

 0 the  characteristics  (slope,  soil  type,  vegetation, paved areas)
  of the likely  oaths  for  run-off  from  the  unit are sufficient
  for  a  relase to  reach  the water;  and
o
  use of the surface  water  for drinking  water, commercial fishing,
  shellfish harvesting, or  extensive  agricultural  (irrigation of '
  food croos ) or recreational uses.

     For example, releases  from units  located  in topographically
depressed areas are unlikely to leave  the site as  run-off.  Also,
facilities located close  to surface water may  still be unlikely
to contaminate this medium  if the  intervening  terrain is
characterized by sandy soil and heavy  vegetation; .in this case
run-off is likelv to  migrate into  the  unsaturated-or saturated
zone.  On the other hand, a pathway characterized  by clayey
soils, little vegetation, and/or the  presence  of natural or
man-made run-off routes (e.g., ditches,  paved  areas, storm sewer
systems, etc.) may indicate a potential  problem if the usage of
the surface water makes human exposure likely  (e.g., drinking
water intake or commercial  fishing areas are a short distance
downstream).  The permit writer should also consider possible
discharge of contaminated groundwater  into surface water.

     In the case of a likely route to  the surface water, the EIR
reviewer may examine  the  features  of the surface water itself
to estimate the impact of a release.   For example, a release
from a relatively small surface impoundment or a limited amount
of run-off from a nearby  landfill  may  not have a significant
impact on a large, fast flowing river  due to dilution.  However,
the validity of this  type of assumption  depends to a great
degree on the characteristics of the chemical constituents
which might be released,  i.e., the toxicity and fate/transport
properties of the substances.  If  the  EIR reviewer feels that a
more detailed evaluation  of the potential for  significant exposure
due to future releases to surface  water  is required, (s)he may
refer to the procedures: contained  in  the RFA Guidance which
discuss how to assess such  releases.

Design and Operating-Features

     If a significant., potent ial for exposure due to. a future
release to nearby surface water exists,  the EIR reviewer should
examine the pertinent design features.   The effectiveness of
landfill and surface  impoundment run-off and erosion controls,
the adequacy of collection  and secondary containment systems,
overflow alarms, automatic  cut-off systems, and dike design
should be considered  for  surface impoundments.  (The EIR reviewer
should also consult* an. OSW  policy  memorandum from  John Skinner
to the Regions dated:  November 14,  1985 for details on the manage-
ment of precipitation run-off at landfills).   In addition, if the
unit is within the 100-year foodplain,  procedures  to ensure

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                               -  31  -

 protection  from* wash-out  during  flooding should  be  reviewed.
 The  EIR  reviewer and/or  the  permit  writer should decide  if  changes
 or additions  to  the  unit  design/operating features  in  the  permit
 are  needed  to address  ootential  exposure from  releases to  a
 surface-water pathway  identified  as  a  concern.

   c.  Air

      In  general,  the  two  types of air  releases of concern  are
 continuous, chronic  releases, and releases  that  are  intermittent
 and sudden  in nature.  Continuous air  releases associated with
 surface  impoundments usually arise  from the volatilization  of
 organic  constituents of.  the  waste handled.   For  landfills,  air
 releases may  occur by  volatilization through inadequate  daily
 covers, or  by narticulate releases  generated by  filling  operations
 or wind erosion.   (Subsurface gas is a  uni-gue  ty.pe  of  air  problem
 treated seoarately in  the next section).   Intermittent air  releases
 may result  from  accidents (fires, explosions) occuring during
 the mishandling  of incompatible,  reactive,  or  ignitable  wastes.

 Route Characteristics  Affecting  Exposure Potential

     Population  density and  distance from the unit-are the  primary
 factors in the potential  for exposure  to an air  release.  Another
 factor to consider is  if  people  are  located along the  line  of
 the predominant  wind direction at the  site.  While  wind  velocity
 and direction  are variable at most  locations, people  located
 along this vector are  more likely to receive increased exposures
 to air releases  (especially  chronic  releases).   In  general,
 however, releases to the  atmosphere may be  rapidly  dispersed
 throughout the area around the facility,  and some exposure  to
any of the nearby populations may occur.

 Design and Operating Features

     Because  route characteristics  are  of  limited use  in
determining if a release  from .a.  unit would  pose  an  exposure
problem, the  EIR reviewer may Zins tead  focus on the  potential for
air releases.   This aonroacK! ..is essentially identical  to the
approach incorporated  in,  the RFA Guidance and the EIR  reviewer
should refer  to  this manual -for details.   In general,  this  approach
 relies heavily on the  characteristics  of  the wastes  handled and
 unit design/operating  features to uncover potential  releases.
 For example, an  impoundment  .with  a  large surface area  containing
 fairly concentrated solutions of  volatile organics  may warrant
examination if people  are immediately downwind from  the  unit.
Conversely, surface impoundments handling wastewaters  containing
only non-volatile metals  should  not  pose a  significant exposure
 problem.  If  volatile  wastes are handled at the  unit,  and  population
 centers are nearby, the EIR  reviewer should examine  (and consider
 permit changes to correct) unit characteristics  that may promote
air releases,  such as: large.., uncovered surface  impoundments,
 treatment methods using aeration, inadequate daily/permanent
 landfill covers, and trench  fill  operations.

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                               -  32  -

      Potential "release and  exposures  to  nearby  oopulations  due
 to  accidents  such  as  fires  and explosions  also  will "depend  on
 waste  characteristics.   If  siqnificant amounts  of  iqnitable,
 reactive, or  incompatible wastes  are  handled, the  EIR  reviewer
 shouM examine the  Part  B submission  to  ensure  that  the  relevant
 264  standards  (264.17, 264.312-314,  264.229-230) are adequately
 addressed.  Waste  analysis/management plans,  including procedures
 to  identify such wa-stes  when  received and  special  handling,
 treatment, or mixing  procedures employed,  should be  scrutinized
 to  ensure that additional permit  conditions  are not  needed  to
 orevent violent reactions,  fire,  or explosions.

   d.  Subsurface  Gas

      Routine  subsurface  qas releases  are most likely from sites
 where  biodegradable wastes  are managed.  Landfills used  for
 codisoosal of nutrescible refuse  with hazardous waste  pose  the
 most serious  nroblem  because  of the potential for  other  volatile
 hazardous constituents to become  mixed with  the methane  generated
 from the decomposable material.   If codisposal  has not occurred
 (and will not occur in the  future), the  EIR  reviewer may generally
 disregard this exposure  oathway.  However, if codisposal is
 known or suspected, the  factors that  affect migration  of subsurface
 gas should be examined.

     If an analysis is warranted  by codisposal  practices, the
 RFA Guidance should he consulted  for details on procedures  to
 assess the potential  for release  and off-site migration  of  sub-
 surface aas.  Subsurface gas  migration may be facilitated by
 man-made underground  conduits used for power  lines, drainage/sewer
 pipes, and telephone  cables.  The presence of natural  or engineered
 barriers or controls  (surface water, ground water, synthetic
 liners, slurry walls, gas venting systems) will  impede or prevent
 lateral migration  of gas produced.  The  geological setting  and
 climate will have a large impact  on gas  movement,  e.g.,  soils
with high permeability and  effective porosity tend to  allow
upward (rather than lateral)  gas  migration,  while  relatively
 impermeable (or frozen)  soils may promote  lateral  movement.
 Nearby buildings must also  be present in order  for subsurface
gas to consitute a potential  threat via  explosion  of methane
 gas, or through human exposure to toxic  gases (e.g., vinyl  chloride)

     If codisposal at a  landfill  is known  or  suspected,  and if
 the site characteristics promote  the "lateral migration of gas
 to nearby buildings,  then a potential for  human exposure exists.
Any existing monitoring or control systems for  subsurface gas
 should be examined, including any passive  venting  designs (gravel
walls, vents to surface), any active recovery system/  and treatment
 procedures used for recovered or  vented  gas.  Normally,  the
usual path to assess the significance of this pathway  would be
as part of a RFA investigation.   Probably  only  after completion
 of the RFA (and RFI,  if necessary) would the  permit  writer  consider
 additions to the permit  that would address these concerns,  e.g,
 installation of gas venting systems.
i« ,

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                             -  33  -
     Potential  exposures due  to  direct  contact with  contaminated
soils should be neqliqible  if the site  at  which  the  unit  is  located
has the  reauired security  (see  relevant  section  of  Part 3).
Therefore, the  orime concern  should be  intermedia  transfer of  con-
taminated soil  to another  pathway and subsequent  off-site  transport.
For example', any potential  for  transport off-site  by run-off  to
surface water or through wind dispersion to  air  should be  examined
under the appropriate pathway evaluations  described  in the preceding
sections.  The  potential for  food chain  contamination should also
be considered if any food  crops  are grown  near contaminated  soils.

     Design and operating  features relevant  to contaminated soil
intermedia transfer have been previously described.  The SIR
reviewer should review these  procedures, as  well  as  the
security procedures . and equipment used  to  limit 'public access  to
active portions of the units, and spill  clean-up, procedures
for routine spills, accidents, and leaks.  An additional concern
related to the  transportation of waste  (see  next  section)  is the
adequacy of current operating procedures in  preventing the "track
out" of contaminated soils  by transportation vehicles from active
portions of the site.


3 . Transportation Factors

     Routine transportation releases are associated  with  leaks or
unloadinq/loadinq practices.  The EIR reviewer should examine  the
type,  capacity, and adequacy of  vehicles and other conveyances
(e.q., pipelines) used, and the  procedures taken  to  minimize
releases.  The  traffic pattern  information should  be examined
to determine if the routes  traveled through  nearby  populated
areas pose potential exposure concerns.  For example, the  potential
for exposure is increased  if  large quantities of  waste (especially
acutely toxic, highly volatile,  ignitable, or explos ive wastes )
are transported through highly populated areas.  Transportation
routes through  thinly populated  area, or on-site waste disposal,
are less likely to lead to  significant human exposure.

     If the permit writer  has concerns  about the  potential exposure
arising from transportation of waste, ( s ).he  should  examine the
past compliance records of  the  facility, noting  any  accidents  and
transportation  violations.  The  permit writer should also  consider
requiring improved emergency  spill/clean-up  procedures used  for
transportation accidents,  special contingency plans  with nearby
localities, or other ways  of dealing with  the problem.


4.  History of Management  Practices

     Proper management practices are necessary to  ensure  the
operation of the unit is adequate to render  releases unlikely
or to detect and correct problems.  Obviously, the most definitive

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                               -  34 -
 indicator of  problems  is a  past  release,  and  the  EIR reviewer
 •nust  examine  the  desicjn  and operation  of  the  unit to see  if
 chanaes  in permit conditions  are warranted  to address  these
 nast  nroblems.  Other  less  definitive  types of  information  that
 are indicative of the  adequacy of  the  operation/design  of the
 unit  include  insurance claims and  settlements,  and  the  compliance
 history  of 'the unit with Federal,  State,  and  local  regulations,
 especially inspection  records and  any  violation citations.
 The EIR  reviewer should consider the history  of complicance  with
 RCRA  reaulations, as well as  other records  th'at the owner/operator
 submitted or  identified  in  the EIR, such  as:

 0 occupational health  and safety records;

 0 NPDES  compliance records;

 0 compliance  records for applicable air  regulations;  and

 0 spills reported under CERCLA.

      For example, worker data on injuries, accidents, and illnesses
 related  to operation of the  unit may be used  to help  identify  those
 facilities with guestionable  management practices,  and  hence,  with
 potential for releases.  The  EIR reviewer should  focus  on the
 nature and freouency of these and  other chronic violations
 to assess the likelihood that a  future release  to any pathway
might occur.

      If  a chronic compliance  problem exists,  the  EIR reviewer
 should examine relevant permit conditions (e.g.,  worker training
problems, contingency plans,  inspection schedules/  proposed
compliance schedules) to ensure  that the  unit  is  operated in
 an adeguate manner.  The EIR  reviewer  should  also discuss compliance
 problems and  possible remedies with appropriate RCRA enforcement
staff.


 5.  Example of Exposure Potential  Determination -


     Figure 3 summarizes an  example of the results  of a qualitative
 screen of the potential for exposure from future  releases (Step  5).
This example examines the same site that  was  reviewed in Figure  2
 (for prior releases, Step 2)  and the same background  information
applies.  Figure 3 illustrates the  types  of decisions that can be
made concerning:  the potential impact  of  future releases to  each
pathway; when release potential  should be considered; and, possible
 follow up action to address  potential  problems.   Note  that  the
existence of   prior releases  is given important  consideration in
assessing release potential,  and the outcome  of investigations
 of past releases will greatly affect possible  follow up actions.

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                                   - 35 -
       Figure 3.  Example of Summary Sheet Following Qualitative Screen for
                  Future Releases
                                 Background Summary

 See Figure 2 for general background.  Concerning Management Practices, no chronic
 RCRA compliance problems documented; occupational and CERCIA records do not
 indicate problems. (Odor violation being examined through prior release analysis;
 see air pathway)
 Pathway
 Potential for Exposure
  Release Potential and
Possible Follow-Up Action
Ground Water
Very low.  Aquifer not used for
drinking water;  ground-water
flow very slow (K < ICT^cm/sec,
minimal hydraulic head).
 Not required due to low
 exposure potential.
Surface
Water
Very low.  Use of nearest surface
water severely limited due to
existing pollution.  No overland
route; run-off goes to POTW before
discharge.
 Not required due to low
 exposure potrential.
Air
Subsurface
Gas
Soil
Transportation
Possible due to population areas
adjacent to site and the handling
of some volatile wastes.  Level
of concern raised due to odor
violation.

Very low.  While underground con-
duits exist, unlikely route for
surface impoundment.

Possible concern due to record of
facility sweeping nearby resi-
dential street.  Direct exposure
of nearby population could result
from track-out of contaminated
soil.
No indication of potential problems
beyond track-out concern raised under
soil pathway.
 Based on past releases,
 future release likely.
 Await results of monitoring
 to decide if new permit
 conditions warranted.

 Not required due to low
 exposure potential.
 Potential for track-out
 exists; if subsequent
 RFA or RFI shows soil
 contamination, consider
 permit conditions (e.g.,
 cleaning trucks prior to
 off-site transport).

 Not required due to low
 exposure potential.

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                              - 36 -


E.  Considering Permic Conditions to Mitigate Potential
    Exposure (Seep 6)


     If che analysis oucLined for Seep 5 indicates che potential
for significant public exposure due to future releases, then the
EIR reviewer should examine the design and operating features of
the unit as described in the preceding section to decide if
additional permit conditions are necessary to decrease the potential
for releases.  If this examination suggests that the existing
design and operating features are adequate to address any potential
exposure pathways, then the EIR reviewer may end the EIR review
process.

     Alternatively, if the EIR reviewer feels that additional
permit conditions are required, (s)he must consider what conditions
are warranted and how these can be required in the permit.  In
some cases, strengthening permit conditions already required under
existing 264 standards may be adequate.  In the case of concerns
over releases to ground water, for example, the owner/operator.
might be required to undertake more frequent monitoring of existing
wells, or sink new wells, in order to insure that a release will  be
detected in a timely manner.  Because the existing regulations
were designed to address primarily ground-water contamination, the
permit writer may find a variety of ways to decrease exposure
potential for this pathway under the existing regulations.

     Concerns about releases to other media may also be addressed,
to a limited degree, under existing 264 standards.  For example,
release potential to the air might be reduced through a strengthening
of conditions related to waste analysis (to ensure that accidental
releases through explosion, fire, or productions of toxic gases do
not occur through mismanagement).  Exposure potential via air
releases may be decreased by insisting on well designed contingency
plans and other agreements with the surrounding communities.  In
some cases, however, the permit writer may have to go beyond the
standards contained in Part 264.  Permit denial (the "ultimate"
permit condition) is the final option in extreme cases of serious
exposure potential.

     The Hazardous and Solid Waste Amendments of 1984 (HWSA)
provided EPA with a new "omnibus" authority in Section 3005(c)(3),
and this provision has been codified in the RCRA regulations in
40 CFR Part 270.32(b)(2).  This provision enables the permit
writer to require the owner/operator to comply with permit
conditions "necessary to protect public health and the environment".
The accompanying legislative history indicates that Congress
intended EPA to add permit conditions beyond those specified in
the exisiting regulations (see the codification rule, 50 FR
28722, July 15, 1985).

     Therefore, EPA may require permit conditions that go beyond
existing 264 standards if an examination of the exposure potential
of the facility warrants such action.  In these cases, the  EIR

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                              -  37  -

reviewer/permit- writer may  wish  to perform  a  more  extensive
analysis of future  release/exposure  potential  to  justify  additional
oermit conditions.  However,  for sites at which past  releases  and
exposures have been documented for a  particular pathway  (e.q./
via the process beqinnina with Step  2  in the  EIR review- process),
further documentation of future  release potential  via  this  route
may not be needed.

     Examples of additional permit conditions  that  could  be  added
under 3005(c) include:

0   new desiqn/operatinq features to  rapidly detect  releases  (e.g.,
   require routine air monitorinq  for  indicator parameters at  or
   near the s ite) ;

0   additional release control desiqn  features  (e.g., covers  or
   wind screens to decrease air  emissions from surface  impoundments;
   increased dike stability requirements and/or secondary containment
   systems to prevent release to surface water); and,

0   limitations on the operations of  the unit/site  (e.g.,  limit
   the handling of wastes with volatile constituents  to  mitigate
   air releases; limit the  acceptance  and treatment of  ignitable
   or reactive wastes to prevent possible explosions or  intermittent
   air releases; limit the  acceptance  of certain acutely  toxic
   wa s t e s ) .

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                    Attachment I  Section 3019 Statute

 Section 3019.   Exposure  Information  and  Health  Assessments

     •*«:. 3019. (a) EXPOSURE INFORMATIOK.-Beginning on th« date nine months
after the enactment of the Hazardous and  Solid Waste Amendments of 1984,  each
application for a final determination  regarding a  permit under section 3005(e)' for  a
landfill or iurfact  impoundment  shall be  accompanied  by  information reasonably
ascertainable by the owner or operator on  the potential for  the public to be exposed to
hazardous wastes or hazardous constituents through releases related to the unit.  At a
minimum, such information must address:
           "(1)  reasonably  forseeable potential releases from  both normal operations
     and accidents at  the unit, including releases associated with transportation  to or
     from the unit;
           
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                         Attachment I  (Continued)
Registry shall give priority to those facilities  or cites at where  there is documented
evidence of  release of hazardous  constituents, at which the potential risk to human
health appears highest, and for  which in the  Judgment of the Administrator of such
Agency existing  health assessment data is  inadequate to assess  the potential  risk to
human health as provided in subjsection (f).
     "(e) PERIODIC REPORTS.—The Administrator of such Agency shall issue periodic
reports which include  the  results of all the  assessments carried out under this section.
Such assessments or other activities shall be reported after appropriate peer review.
     *(f) DEFINITION.—For the  purposes of this section,  the term "health assessments'
shall  include preliminary assessments of the potential risk to human health  posed by
individual sites and facilities subject to this section, based on such factors as the nature
and extent of contamination, the existence of potential for pathways of human exposure
(including  ground  or  surface water  contamination,  air emissions,  and  food chain
contamination),  the size and potential susceptibility of the community within  the likely
pathways of  exposure, the comparison of expected human exposure levels to the short-
term  and  long-term health  effects associated with  identified contaminants and any
available recommended exposure or tolerance limits  for such contaminants, and the
comparison of existing morbidity and mortality data on diseases that may be associated
with the observed levels of exposure. The assessment shall include an evaluation of the
risks  to the  potentially affected  population from ail sources of such contaminants,
cinluding known point or nonpoint sources other than the site or facility in question.  A
purpose of such preliminary assessments shall  be to help determine whether  full-scale
health or epidemiological studies and medical evaluations of exposed populations shall be
undertaken.
     "(g) COST  RECOVERY.—In  any case in which a health assessment performed under
this  section  discloses the exposure of  a population to  the  release  of a hazardous
substance,  the costs of such health assessment  may be recovered  as a cost of response
under  section 107  of  the  Comprehensive Environmental  Response,  Compensation, and
Liability Act of 1980  from  persons causing or contributing to  such  release of such
hazardous substance or, in the case of multiple releases contributing to such exposure, to
all such release.

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                                                                           TAC
                                                                              HUE NT I I
                                                                                                     Facility Name
                                                                                                     ID No.
                                                   EXfOSUHE  INFORMATION  REPORT (E1H)  REQUIREMENT CHECKLIST
A.  General Information
Numbers
A-l.
A-la
A-lb
A-lc
A-ld
A-le
A-lf
A-lg
A-lh
A-li
A-1J
A-lk
A-ll
A-lm
Information Requirement
Information in Part B Application
General description of facility
Chemical and physical analyse* of wastes
Access control and security
description of active portion
General inspection schedule' and procedures
Preparedness and prevention documentation
Contingency plan
Preventive procedures
Facility location information
Closure plan
Post-closure care plan
Documentation of insurance
Topographic mad .(site plotted on uses
quadrangle maps)
List of wastes placed or to be placed
In each unit
Provided Complete Not
Reg. Cite (i/N) (i/N) Applicable Location In Part B or e lit/Comment
27U.14(b)(l>
270.14
and (J)
270.14(b)(4)
270.14(b)(5),
27(1. 17(6)
270.14(6) (7)
27U.14(b)(U)
27U.14(b)(ll)
(i) and (ii)
27U.14(b)UJ)
27U.14(b)(U)
27U.14(b)(17)
270.14(b)(iy)
270.21(a) and
27U.17(a)

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                                                                         Ill - 2
                                                          IMPOKHATIOM REPORT (EM)  HBflUIREMBIIT CHECKLIST
A. . General Information (continued)
Information Requirement
Numbers	

A-2.     Additional Information

  A-2a   Bxiating riak assessment  reports  and
         information,  including liability  insurance
         analyses,  claims,  and settlements

  A-2b   land use and  toning map(a) for an area of
         4  miles around the unit

  A-2c   Existing aerial photographs of the facility

  A-2d   Identify and  summarize any waste  analysis
         data not already aubmlttedi provide
         additional data as discussed in text

  A-2e   Current estimate of annual amount of waste
         received and  description of any pretreatment
         process used

  A-2f   Identification of  any Federal, State, or
         local Inspection or compliance records
         related to environmental and health programs!
         include descriptions  of any major violations
                                                                             Provided  Complete     Not
                                                               Reg. Cite      (y/M)      IY/H)    Applicable
                                                            270.101))



                                                            270.101))


                                                            270.10()»



                                                            270.10
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                                                                          II - 3
                                                  EXPOSURE INfORMATION REPORT (E1R)  REQUIREMENT CHECKLIST
B.  Ground-Mater Pathway
                      Information Requirement
Number a  	

B-l.     Interaction tn Part B Application

  B-la   Interim atatua ground-water monitoring reaulta

  B-lb   Identification of uppermost aquifer.
         Including flow rate and direction
              '' '••              ' -" IU. I  »«!di toUd '  ' a i » .
  B-lc   Topographic aiapa related to ground-water
         protection (well location,  water  table
         elevation contour*, etc.)      .     ..

  B-ld   Oeacription of eiiating contamination


  B-le   Detailed plans for ground-water •onltoring
         prograa

  B-lf   Deacrlption of detection Monitoring
         program (if applicable)

  B-lg   Oeacription of compliance Monitoring
         program and characterisation of
         contaminated ground water  (If applicable)

  B-lh   ACL deawnatration (if any)

  B-lI   Corrective action program (if applicable)
   Reg. Cite



27u.l4(c)(l)

27U.l«(c)(2)
270.14(c)(J) and
270.14(b)(19)
27U.14(c)(4)
(i) and (11)

270.H(c)(5)
270.14(c)(6)
27U.14(C)(7)
and (c)(7)(il)
270.14(c)(7)(lv)

27U.14(c)(B)
Provided  Complete     Not
 (T/M)     O/H)     Applicable
Location tn Part B of eiR/Cowwnt
  B-l)   Deacrlption of liner and leachate collection        27U.17lb)(l)
         ayateaw (if applicable)                             270.2Kb) (1)

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                                                                          II - 4



                                                  EXPOSURE INFORMATION HBPORT  (Bill) REQUIREMENT CHECKLIST


B.  Ground-Mater Pathway (continued)

                                                                              Provided  Complete     Hot
Humbert  	Information Requirement	     Reg. Clte      (If/M)     (Y/N)    Applicable   	Location  in  fact B or EIR/Comment

B-2.     Additional Information

  B-2a   Bxiating nap showing location of all  known
         well* within three mlleai number and
         location of drinking water wella                    27U.10<))         	     	     	     	.
  B-2b   Diacuaaion of ground-water uaea within
         three aiilea of unit
                                                             27U.1UI])

  B-2c   Regional aap ahowing areaa of  ground-water
         recharge and diacharge                              270.10(1)

  B-2d   Net precipitation uaing net awaaoaal  rainfall
         or other available data  -   ii. .     •<              270.10IJ)

  B-2e   unleaa otherwlae reported to BPA, available
         well data Indicating a release,  and
         information on any affected public  or private
         water auppliea. Including populations aerved         270.10(j)

  B-2f   Any known food chain contamination  due to
         prior releaae from the unit to ground water          27U.10(j)

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                                                                          II - 5
                                                  EXPOSURE mrORH»TIOH  REPORT  (E1R) HeQUlHEHgMT CHECKLIST
C.  Surface Mater Pathway
                      Information Requirement
Numbers  	

C-i.     Information In Part B Application

  C-la   Location information related to 100  yr flood
         plain including variance demonstration*

  C-lb   System for control of run-on fro* each
         peak discharge of 2S yr  ator*

  C-lc   System for control of run-off fro* 24 hr,
         2S yr storm

  C-ld   Procedures/equipment to  prevent overtopping


  C-le   Structural integrity of  dikes
Reg. Cite
                                                             (ill) thru  (v)

                                                             270.21(bl(2)


                                                             270.21(b)(J)
                                                            270.17(b)(2),
                                                            2t«.221(f I

                                                            270.17(bHJ)
Provided  Complete    Not
 (i/M)     (y/M)     Applicable
                                                                                                                   location in Part B or tin/Comment
C-2.     Additional Information

  C-2a   Dlacuaaion of aurface water uaea within
         three allea of the unit. Including a «ap
         •howing the location of all aurface water
         bodlee and downatreaa drinking water intake*        270.101))

  C-2b   velocltlee of atrea>a and rivera paaalng
         through and adjacent to the property               27o.lo())

  C-2c   Oeacrlption of any ayatcB uaed to Monitor
         aurface water quality, and a auavMry of the data    270.10)})

  C-2d   Description of known releaaee to aurface water;
         the eiteot of contaailnationi  reaiedial action.
         If anyi  and if known,  severity of impact            270.101))

  C-2e   Any known food1 chain contamination reaultlng
         from prior release from the unit to aurface
         water                                              270.101)1

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                                                                          II - 6
                                                  BKPOSURg IMPORHATIOH  REPORT  
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                                                                         -II  -  7



                                                 EXPOSURE  1HPOH«ATIOM RBfORT (BIB) REQUIREMENT CHECKLIST


B.  subsurface Caa Pathway

                                                                             Provided  Complete     Not
Number a  	Information Requirement	    Reg. Cite      U/M)     IK/M)     Applicable         Location in Part B or eiR/Comment

B-l.     Information in Part  B Application

             (Note:   None in  addition to General  Information Requirements!


B-2.     Additional  Information

  B-2a   Any paat dlapoaal of municipal-type waatea in the
         unit;  approilmate quantitlea and datee of
         diapoaal, if known                                 270.10(}>         	     	     	      	

  B-2b   Nap location of  any  underground conduit*
         within the  aite  and  known underground
         conduita within  1000 feet of property boundary      270.10IJ)         	     	     	      	

  B-2c   Description* of  any  monitoring  or control
         mechaniama  for aubaurface gaa releases
         aummarlie reaulting  data                           270.lO(j)         	     	     	      	

  B-2d   Description of any known releaaea; extent of
         contaminations remedial  action  taken, if anys
         and the aeverity of  Impact,  If  known                270.10<))         	     	     	      	

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                                                                          II  -  0



                                                 BKP03URB  INrtmmTIOM REPORT (B1R) REgtllHEHEHT CHECKLIST


P.  Contaminated Soli Pathway

                                                                             Provided  Complete     Not
Numbera  	Information Requirement	    Reg. Cite      (Y/H)     (Y/M)    Applicable         location In Pact B or em/Comment

f-1.     Information In Part  • application

             (Mote:   Hone In  addition to General  Information Requirements)


P-2.     Additional  Information

  f-2a   If aoll •aaplin9 haa been done, a map ahowinq
         areaa of aoll contamination,  and  a aumawry of
         analytical  result*                                 270.10(]|         	     	     	     	
  P-2b   Oeacriptlon of  the typea of major  releaaea
         that resulted in aoil contamination, and any
         clean-up action                                    270.10(}J

  P-2c   Any known food-chain contamination resulting from
         the use of contaminated  aoila  for  raising crops     27U.lO(j)

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                                                                          II - 9
                                                  B1TOSUHB INfOBMATIOM REPORT  (BIB) REQUIREMENT CHECKLIST
0.  Tranaportatlon information
C-l.
                      Information Baquirea»nt
         Information In Part 1 aplication
  C-le   Traffic pattern, voluM, aiMI eoatcolai  «cce««
         road character t«tlc«
                                                                   .  Ctt«
270.14(b)(10)
                 Provided  Coaplet*     Not
                            (If/M)    AppllcabU
Location in Part B or tlK/Com»tnt
C-2.     Additional Inforaatlon

  C-2a   Deacrlptlon of th« typea and capacltiaa of
         vehicle* uaed to transport waate                    270.101])

  G-2b   Identification of noraal transport  routea
         for hasardoua Maate Into the alte and within
         one aile of the facility entriea                    27u.lo(j)

  C-2c   Deacriptlon of procedures for clean-up of
         transportation-related spill* or leaka              270.10(j)

  C-2d   Deacrlptlon of any transportation accldenta
         releasing hazardous wastes on-site, or in  the
         lawediate vicinity                                  270.10(j)

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                                                                         'II - 10
                                                          mronmTioM REPORT (BIB)  REUUIREHEHT CH ecu LIST
H.  Management Practices InfonMtlon
                      Information aequlrement
Humbers  	

M-l.     Information in Part  B *gpiic«tioa

  M-l«   Outline of progrM«  to  trala ••ployce* to
         •afely operate and ••iotalo facility,
         including  eaergency  reapooa* actlvitle*
Reg. Cite
                                                            27U.14(b)(12)
                                                            264.16
Provided  Complete     Not
 Qf/M)     
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                                                  B1POSUBB IMfORMATlOM RBPOBT  18III) BBQUIRBIKMT CHECKLIST
I.  Potential tor HuMan Biposure
                      Information BaquireMcnt
MuMbers	

I-I.     Croundwater Pathway

  I-la   Description of hoi* the units'  location
         •fleet* the potential for and  possible
         •agnitude ot huMan exposure fro* releases
         to groundwater
              Provided  Complete     Not
Reg. Cite      Qf/M)      (»/M)    Applicable         Location in Part  B or eiR/Coament
                                                             270.101])
  I-lb   Description of the deaiqn and operating
         features that affect the potential
         for releases to groundwater and the
         •agnltude of these releaaea
                                                            270.101})
1-2.     Surface Mater Pathway

  I-2a   Description of how the units'  location affects
         the potential for and poaaible Magnitude of
         huMan exposure froM releases to surface
         water.                                              270.10(1)

  I-2b   Description of the design snd operating
         featurea that affect the potential  for
         releases to surface water and the
         Magnitude of these releases.                         270.10(1)

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                                                                          II  -  12



                                                  BKPOSUBB IlirORHfcTIOM REPORT (BIR) RBQUIHBIgMT CM ECU LIST


I.  Potential tor Hu»an Ixposure (Continued)

                                                                             Provided  Complete     Not
MiMbers  	information RegutreMent	     Reg.  Cite       (Y/M)     (ir/M)    Applicable         Location in  Part B or BIK/Coaaent

I-J.     Mr

  I-Js   Description of how the uslts*  location affect*
         the potential for and possible Multitude of
         husan eipoaure fro* releases to the air.             270.10(j)         	     	     	      	.
  1-36   Description of the design ana operating
         features that affect the potential for
         releases to the air and the
         Magnitude of these releases.                         270.10()I

  I-Jc   Description of wastes indicative of air
         rslsases and aaoagestent of these waates.             270.101))

  l-Jc(l) Description of any waste characteristics
          (e.g., incoapatlblllty, reactivity, Ignita-
          bllity, volatility) indicative of potential
          for releases to the air.                            270.10IJ)

  I-Jc(2) Description of speclsl handling, treatment,
          or eiiiing procedures used to prevent  violent
          reactions, fires,  explosions,  or extensive
          evaporation of volatile constituents.               270.101))
1-4.      Subsurface Cas Releases

  I-«a   Description of bow the'units'  location affects
         the potential for and possible Magnitude of
         huaan exposure frosi subsurface gas  releases.        270.10())

  I-46   Description of the design and  operating
         featurea that affect the potential  for
         subsurface gas releases and the
         Magnitude of these releases                        270.10())

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                                                                          II  -  u



                                                  UPOSURg IHPORmTlOM BEPORT (BIB) REQUIREMENT CHECKLIST


 I.  Potential for Hu»an Biposure (Continued)

                                                                             Provided  Complete     Not
 Number*  	Information Requirement	     Reg.  Cite       Clf/ll)     (f/Ht    Applicable         location In  Pact B or tin/Comment

 1-5.     Release* to Soil

  1-5*   Description of how th* unit*' location affect*
         the potential for and po*«lble Magnitude of                                                                                         '.
         human eiposure fro* release* to aoll.                270.101)1         	     	     		  	
  I-5b   Description of the design and operating
         feature* that affect th* potential for
         releaaea to *oll and th* Magnitude of
         the** releaae*.                                     270.10(J)
I-t.     Ttan*portatlon-Rel*t«d »*l*a*e*

  I-6a   Description of how Method* and rout** of
         transportation of wa*t* on-*lt* and In th*
         iMwdiat* vicinity of the facility affect
         the potential for hu«*n eipoaure fro*
         transportation-related releases.                   27U.10()>
1-7.     Horfcer-IUnsqeaent Practice*

  I-7a   Analysis of worker data and discussion of  the
         potential for off-alt* Migration and public
         eipoaure resulting fro* any release*
         related to worker-*anage*ent practice*.             27U.10())

  I-7b   Description of training prograa* In place  for
         th* worker* to ensure the safe handling of
         wastes and Minlals* the potential for
         release* fro* normal operation of the unit*.        270.101)1

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          Attachment III.  Levels of ATSDR Assistance*
1.  Health Consultation;   Immediate or-short-term consultation
    by ATSDR to provide health advice and/or health effects
    information regarding a specific site.

2.  Health Assessment;   Initial multi-disciplinary reviews by
    ATSDR of all readily available data to  evaluate the nature
    and magnitude of any threat to human health at a site.
    These evaluations will adapt EPA's risk assessment for the
    characterization of potential health threats at a site or sites,
    and may include literature searches, information summarization,
    and evaluation of existing environmental data, pilot samples,
    testing for food chain contamination,  and similar activities.

3.  Pilot Study;  A preliminary or short-term medical, laboratory,
    or epidemiologic study on a limited human population to
    decide if additional, large-scale studies are warranted.   The
    study populations can include those living at, or near,  a
    site and those not  residing at, or near, a site (control
    or reference population).

4.  Epidemiologic Study;   Long-term study by ATSDR involving  a
    comprehensive protocol designed to add  knowledge of the
    health effects of a specific substance  or substances at  a
    site or sites.

5.  Health Registry;  A site-specific or adverse health effects-
    specific registry established and maintained to track
    specific diseases and illnesses and long-term health effects
    to persons exposed  to toxic substances.


* These levels of assistance are taken from the EPA/ATSDR
  MOU for CERCLA; definitions of these ATSDR activities may
  change in the EPA/ATSDR MOU for RCRA.

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