EPA-600/2-77-056
February 1977
Environmental Protection Technology Series
       EVALUATION OF CERAMIC  FILTERS FOR  HIGH-
                 TEMPERATURE/HIGH-PRESSURE  FINE
                                 PARTICIPATE  CONTROL

                                  Industrial Environmental Research Laboratory
                                       Office of Research and Development
                                      U.S. Environmental Protection Agency
                                 Research Triangle Park, North Carolina 27711

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               RESEARCH REPORTING SERIES

Research reports of the Office of Research and Development, U.S. Environmental
Protection Agency, have been grouped into five series. These five broad
categories were established to facilitate further development and application of
environmental technology. Elimination of traditional grouping was consciously
planned to foster technology transfer and a maximum interface in related fields.
The five series are:

     1.    Environmental Health Effects Research
     2.    Environmental Protection Technology
     3.    Ecological Research
     4.    Environmental Monitoring
     5.    Socioeconomic Environmental Studies

This report has been  assigned  to the ENVIRONMENTAL PROTECTION
TECHNOLOGY series. This series describes research performed to develop and
demonstrate instrumentation, equipment, and methodology to repair or prevent
environmental degradation from point and non-point sources of.pollution. This
work provides the new  or improved technology required for the control and
treatment of pollution sources to meet environmental quality standards.
                    EPA REVIEW NOTICE

This report has been reviewed by  the U.S.  Environmental
Protection Agency, and approved for publication.  Approval
does not signify that the contents necessarily reflect the
views and policy of the Agency, nor does mention of trade
names or commercial products constitute endorsement or
recommendation for use.
This document is available to the public through the National Technical Informa-
tion Service, Springfield, Virginia 22161.

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                                       EPA-600/2-77-056

                                       February 1977
    EVALUATION OF  CERAMIC FILTERS

FOR  HIGH-TEMPERATURE/HIGH-PRESSURE

        FINE PARTICULATE CONTROL
                         by

               G. G. Poe, R. M. Evans,
          W.S.  Bonnett, andL.R. Waterland

                Aerotherm Corporation
                  485 Clyde Avenue
              Mt. View, California 94042
           Contract No. 68-02-1319, Task 25
                ROAPNo.  21ADL-029
             Program Element No. 1AB012
          EPA Task Officer:  B.C. Drehmel

      Industrial Environmental Research Laboratory
       Office of Energy, Minerals, and Industry
          Research Triangle Park, NC 27711
                    Prepared for

    U.S. ENVIRONMENTAL PROTECTION AGENCY
          Office of Research and Development
                Washington, DC 20460

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                                              FOREWORD





       This document contains a review and evaluation of ceramic membrane filtration as a  novel  con-



cept for the control of fine particulate.  Several  materials are identified as candidates  for testing



as high temperature, fine particulate filters and a test matrix is proposed.




       The study was performed for the Environmental Protection Agency,  Research Triangle  Park,  North



Carolina.  Dr. D. C. Drehmel was the EPA Task Officer.  The Aerotherm Program Manager was  Mr. Fred



Moreno.  Acting as Technical Advisor for the task was Dr. C. B. Moyer.  The study was performed



during the period December 1975 through June 1976.
                                                 n

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                                     TABLE OF CONTENTS
                                                                                           Page
        SUMMARY 	     1
        INTRODUCTION  	     3
        THEORETICAL DISCUSSION  	     4
        3.1  Filter Efficiency  	     5
        3.2  Pressure Drop	     7
        3.3  Actual Filtration  	    10
4       CURRENT RESEARCH  	    13
5       LITERATURE AND MANUFACTURERS SURVEYS  	    14
        5.1  Thick Walled Elements	    17
        5.2  Thin Walled Elements -Catalyst Monolith Supports	    20
        5.3  Potential Cleaning Methods 	    20
6       PROPOSED TEST PROGRAM 	    31
7       PROCESS ECONOMICS 	    36
8       CONCLUSIONS AND RECOMMENDATIONS 	  	    38
        REFERENCES	    39
        APPENDIX A - FILTER TEST PLAN 	    40

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                                       LIST  OF  ILLUSTRATIONS

Figure                                                                                        Page
   1       Collection efficiency versus particle size  	    8
   2       Collection efficiency versus particle size  	    9
   3       Pressure response in constant rate gas filtration 	   11
   4       Multiple element filter assembly  	   18
   5       Flow rate of air at standard conditions for a typical ceramic cylindrical .
           element, wall thickness - 6.0 mm	   19
   6       Examples of 3M Company's ThermaComb corrugated ceramic  	   21
   7       Structural shapes for 3M ThermaComb 	   22
   8       Examples of Coming's Celcor cordierite monoliths 	   23
'  , 9       Examples of Dupont's Turvex honeycomb	   24
  10       Example of General Refractory Company's Versagrid ceramic honeycomb 	   25
  11       Examples of Norton Company's silicon carbide Spectramic honeycomb	 .  .   26
  12       Pore size distribution for 3M Company's ThermaComb AlSiMag 795	   27
  13       Pressure drop across an 0.2 mm (0.008 in) AlSiMag 795 flat ceramic piece  ....   28
  14       Air flow through 0.2 mm (0.008 in) AlSiMag 795 flat ceramic piece	   29
  15       3M Crossflow Ceramic Monolith	   32
  16       3M Element Low Temperature Holder	   33
  17       3M Element and Holder Mounted Inside Pipe	   34
                                          LIST OF TABLES

Table                                                                                         Page
  1         Filter Operating Conditions 	   15
  2         Survey Results  	   16
  3         Comparison of Filter Element Costs for the Conditions in Table 1  	   37

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                                             SECTION 1
                                              SUMMARY

       The purpose of this study was to analyze and  evaluate ceramic membrane filters as a new, fine
(<3um) particulate control concept for high temperature  (~900°C), high pressure (HTHP) processes.
The results of this effort are summarized  in the following paragraphs.
       The concept of membrane filters is  not a new  one.  A review of the theory of operation, from
the standpoint of both particle collection efficiency and fluid flow behavior, is presented here.
The theory is the same as that for fiber filter operation.  The complexity of the problem necessi-
tates that many  simplifying assumptions be made; consequently, theoretical calculations are not
very reliable for predicting actual filter operation.  However, these calculations can be very use-
ful in explaining the quantitative behavior of a filter and in investigating the sensitivity of
filter operation to changes in fluid parameters and  filter material characteristics.  Actual filter
operation can be predicted only with the aid of sufficient experimental data at similar operating
conditions.
       Current research to develop ceramic membrane  filters for use in HTHP processes is limited to
an EPA sponsored project with Westinghouse and Horizon Research Inc.  The purpose of this project
is to develop a thin-walled (-0.6 mm) ceramic material with a pore size of approximately 0.5 urn.
Success in producing a sample suitable for laboratory testing as a filter material has been limited.
       Several ceramic filters were identified in this study as potential candidates for fine parti-
culate removal.  There does not seem to be any inherent material limitation to high temperature
operation; however, no evidence of high temperature  filter application was found.   These filters are
typically 2 to 6 mnTthick, cylindrical in  shape, and available with various pore size increasing up-
wards from 0.5 \m.  It appears that these  elements may be suitable for fine particulate control in
hot gas streams.
       The most promising, although undeveloped, idea for a ceramic filter is to use ceramic honey-
comb monoliths similar to those available  for catalyst supports and heat exchangers.  The walls of
the monoliths are approximately 0.2 to 0.4 mm thick  and of varying pore size and porosity.  Geomet-
ric configurations are available which would force the gas to flow through the membrane walls.

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Pressure losses would be very small relative to those of standard ceramic filter elements.  The
application of ceramic monoliths to high temperature fine particulate control appears very promising,
and it is strongly recommended that this concept be further  investigated.
       Three ceramic materials were selected for testing and were delivered  to Westinghouse.  The
materials were a standard ceramic  filter material  (Selas), a ceramic monolith  (3M) and a  new ma-
terial called ceramic FiberForm  (FMI).  A test matrix was prepared and  is  included as Appendix A.
       A combined-cycle power plant using ceramic membrane filters appears  to  be  cost competitive
with  other combined-cycle fine particulate removal systems.  The ceramic monolith concept offers
a  substantial cost savings  (perhaps a factor of 10) over other ceramic  filter  elements.
       Ceramic filters appear to be both technically and economically feasible as fine particulate
control  devices  in high temperature gas flows; however, suitable experimental  data must be obtained
 in order to  adequately evaluate  them.  Each type of filter should be tested  under conditions sub-
stantially similar to the expected operating conditions.  Data concerning  the  collection  efficiency,
pressure  loss, duty  cycle,  filter  life, and methods of cleaning should  be  obtained.

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                                             SECTION  2
                                           INTRODUCTION

       High temperature gas turbines used to generate electric power require gas streams virtually
free of particulate matter.  Gas streams from high temperature, high pressure coal processes, such
as low Btu gasification and pressurized fluidized bed combustion, require considerable particulate
removal.  In order to maintain high thermal efficiency the particulate clean-up must be done at the
high temperatures of the process.  Coarse particles  (>10ym) can be successfully removed by high
temperature cyclones.  Many new concepts for fine particulate control at elevated temperatures are
presently being proposed.  One such concept utilizes ceramic membrane filters.
       Ceramic materials have been used extensively  in high temperature environments.  High melting
temperature and mechanical strength, low thermal expansion, and resistance to chemical attack are
some of their attractive features.  These materials  have found application as filters in medicine,
biology, aerospace, and electronics where extremely  clean gas and liquid streams are required.
There are no obvious reasons why ceramic filters would not also be suitable for the high tempera-
ture, fine particulate control applications described here.
       This report presents a review and evaluation  of current, proposed and potential ceramic mem-
brane particulate control  technology.  The theory of membrane filters is reviewed in Section 3.
Section 4 is a brief summary of the current EPA-Westinghouse ceramic membrane filter program, which
is currently the only developmental research program concerning ceramic filters for high temperature
applications.  Section 5 presents the results of the literature and manufacturers surveys.  Three
materials, proposed for testing at Westinghouse, and a test plan are discussed in Section 6.  The
economics of ceramic filters are briefly discussed in Section 7, and the conclusion and recommenda-
tions presented in Section 8.

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                                             SECTION 3
                                      THEORETICAL  DISCUSSION

        Filter  materials  are  usually  classified  as  one of  two  types, membrane  filters  or  fiber  fil-
 ters.   In  a  two  dimensional  representation, membrane  filters  may  be thought of  as  a  uniform solid
 phase  interrupted  by  a fluid phase  (holes), and are generally characterized by  low porosity (void
 fraction).   A  fiber filter may  be thought  of as a  uniform fluid phase  (holes) interrupted  by a
 solid  phase  (fibers)  and is  characterized  by high  porosity.   In an oversimplified  view,  membrane
 filters work because  the membrane pore  diameter is  smaller than that of the particles to be col-
 lected; the  particles are thus  prevented from passina through the membrane.   On the  other  hand,
 fiber  filters  operate most effectively  after an initial "cake" (layer) of  particles  has  been de-
 posited; thus, the cake  serves  as the filter.   In  either  case the theoretical analysis of  the  fil-
 ter operation  is the  same and follows directly  from the theory of flow through  porous media.   The
 analysis results in the  development  of  two measures of filter performance  - particle  collection ef-
 ficiency and fluid pressure  drop across the filter.
        Usually,  the theoretical development of  filter collection  efficiency has been  approached
 microscopically  from  a very  detailed analysis of small scale  events inside the  filter.  Important
 parameters are the particle  size, filter pore size, fluid Reynolds number, and  diffusivity.  Each
 collection mechanism  is  studied separately and  an  expression  for  the collection efficiency derived.
 The individual expressions are  then  combined to yield an  estimate of the total  collection  efficiency
 of the filter.  These expressions are usually derived for a single size particle and  well-defined
 flow conditions.   Unfortunately, the procedure  is  quite complicated, necessitating the use of  many
 simplifying  assumptions  which can lead  to  considerable inaccuracy.
        The analysis of fluid pressure drop, on  the other  hand, is approached  macroscopically.   The
 system is treated  as  a continuum and the suitably modified equations of motion  are applied. A fil-
 ter  porosity (e) is introduced  in the continuity equation and a filter permeability  (K)  modifies
 the momentum conservation equation.  Porosity is a straightforward measure of filter void  fraction
 and may be easily calculated  from density  measurements.   The  permeability, however,  is a measure  of
the fluid drag introduced by  the filter and cannot be accurately  predicted at present.  It thus
becomes an empirical  constant.

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       Expressions for the efficiency and the pressure drop (from Darcy's law) of a filter are
developed for highly idealized systems in the following sections.  This is followed by a discussion
of the possible effects of some real system complications.

3.1    FILTER EFFICIENCY
       Particle collection by filtration results from the action of three basic mechanisms:
       •   Diffusion of particles to solid surfaces
       •   Impaction of particles on solid surfaces due to deviation of the particle motion from the
           streamlines of fluid motion
       •   Interception of particles by solid surfaces due to particle motion along streamlines.
Clearly, the last two mechanisms depend on the details of the fluid flow adjacent to the pore sur-
faces.  Some authors describe a fourth mechanism - sieving, in which a particle with a radius greater
than the largest pore radius is "strained" out of the fluid.  However, this is just a special case
of impaction.
       A detailed analysis of each collection mechanism is quite tedious and complicated, and will
not be presented here.  The resulting equations, as given by Davies (Reference 1), are presented in-
stead.  The analysis assumes that particles are chemically inert, uncharged, solid spheres of iden-
tical size (mono-disperse).  In addition, particles are assumed to be at infinite dilution so that
particle — particle interactions and pore clogging may be neglected.  Thus the porosity and permea-
bility can be considered constants.  The resulting expressions for filter efficiency include the
pore radius (R), the mean fluid velocity in each pore (v) and the average length of the pore (h) as
parameters.  These quantities are determined from measurements of the porosity, the average number
of pores per unit area, and the fluid flowrate.
       The efficiency due to diffusion (ED) has been given by Spurny & Pich (References 2,3,4) as:

                  ED = 1 - 0.81904 exp (-3.6568 NQ) - 0.09752 exp (-22.3045 ND)
                                                                                                (1)
                       - 0.03248 exp (-56.95 ND) - 0.0157 exp (-107.6 ND),

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        where  ND  =  h  V/R2v
               V  =  kTF/6iray  =  Diffusion  coefficient
               F  =  Cunningham  slip  factor
               k  =  Boltzman's  constant
               a  =  particle  radius
               y  =  fluid viscosity.
 The expression is  valid for pore radii  smaller  than  10  percent of  the  filter  thickness.
        The efficiency due  to  inertia! deposition  (Ej) is  given by  Pich (References  5,6)  as

                                    Ej = 1  -  (a  +  B)2/(a + I)2,                                   (2)

        where  a = l/(\Ar/2,/3~e  -  l)
              e = porosity
              B = 1  - 2S Sa  +  2S2 a {1 - exp  (-1/S^a)}
              S = mFv/6irayR  =  Stokes number of particle
              m = mass of particle.
 This is an unproven  expression  in  that  many  unsupported approximations were used  in its  derivation;
 however, it is possibly the most accurate  expression presently available.
        The efficiency due to  interception  (ER)  is determined  geometrically as the ratio  of  the inter-
 ception area  of  the  pore (irR2 -  ir(R - a)2) to the total area  of  the  pore  (irR2).   Thus,

                                           c  _  i  /?   a\                                         ,  ,
                                           fcR "  R  r  " R)  •                                       (i}

        The overall collection efficiency  (E) is then given by:

                                     E ' Ei + 0 - EI)(ED  + **)>                                 <«>

        where  y = 0.6 ^  " a/R\
When this  number exceeds unity the  efficiency is  assumed  to be 100 percent.   The  overall collection
efficiency  is  seen to  be a  function  of  particle size, pore size,  porosity,  and particle density.
Fluid properties of  importance are  the  viscosity, the Cunningham slip  factor, the flowrate and the
fluid mean velocity  in the  pore.  The effects of  pore size distribution on  collection efficiency
have been found to be quite significant (Reference 7);  however,  these  effects are not included here.
                                                 6

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       Figure 1 shows the- predicted overall collection efficiency as a function of particle size
with superficial fluid velocity as a parameter.  These results are for a membrane filter 0.25 mm
thick with an e of 0.3 and uniform pore radius of 5 microns.  As expected, for larger particles
(>0.5vim radius) collection efficiency increases with increasing particle size.  However, note that
for very small particles the predicted collection efficiency increases with decreasing particle
radius.  This results from enhanced diffusion of these particles to the collector surface.  Figure
2 shows overall collection efficiency as a function of particle size with filter pore radius as a
parameter.

3.2    PRESSURE DROP
       The flow of a continuum fluid through a porous medium is described by the continuity and con-
servation of momentum equations.  For a chemically inert, electrically neutral, homogeneous Newtonian
fluid these equations are:
                                                 ->•     ->
                                                 V  - p V0                                      (5)

                                                                                               (6)
where V   is the superficial velocity of the fluid at the surface of the porous medium, e is the
porosity, K is the permeability and y is the gas viscosity.  Equation (6) is commonly called Darcy's
law.  For steady flow of a clean, ideal gas of constant viscosity these equations may be solved for
a variety of geometries.  The most common form of Darcy's law for flow through a planar filter of
thickness L is:

                                           Vo = A = Hi?                                       ^

where Q is the volumetric flowrate and A is the surface area and AP has been assumed to be small
compared to P.  This equation is often used to calculate the permeability of a material, since
permeability is not derivable from other basic considerations.  For a system of two planar filters
of thickness L-, and I?
                                       AP = AP, + AP2 =                                        (8)
       where L = 1^ + L2 and

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                                     1.0
oo
                                                            Superficial  velocity
                                                        V =  Q/A =  10 cm/secQ
                                                                   7 cm/secA
                                                                   4 cni/secQ
                                                                   2 cm/sec<>
                                                                   1  cm/sec>
                                                                                                          h = 0.25 mm
                                                                                                          y = 0.035 cp
                                                                                                          E = 0.3
                                                                                                          R = Sum
                                       0.05
0.1
              0.5         1.0

Particle radius (a) in microns
                                                                                                        2.0
5.0
                                                       Figure 1.  Collection efficiency versus particle  size.

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                                                                   h = 0.25 mm
                                                             V = Q/A = 10 cm/sec
                                                                   u = 0.035 cp
                                                                   e = 0.3
0.05
                          Particle radius  (a)  in microns
             Figure 2.  Collection efficiency versus  particle  size.

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                                     K = lK^K2/(l2!^ + L^).                                   (9)

This form of Darcy's law is useful for determining the permeability of a cake-filter system with
clean air.  Similar results can be obtained for a cylindrical  system.
       If particles are contained in the fluid the pressure drop is affected in two ways.  First
the permeability of the filter changes with time as the smaller particles plug the pores.  Second,
a dust cake builds up on the surface and forms a new porous medium.  These effects can be quantified
by appropriate use of Equation (0) or (9).   The dust cake is considered to be one of the filters
and its thickness (l_2) and permeability (ic2) are taken as functions of time.  After a short initial
transient period the permeability and rate of growth (k) of the dust cake are approximately constant;
thus the pressure drop of the combination of filter and dust cake is given by:
                                         AP = AP  +     ,                                      do)
where
                                                  QuL,
This linear time dependence of the pressure drop is illustrated in Figure 3 which shows data for a
fiber filter.

3.3    ACTUAL FILTRATION
       The development described above is based on a number of simplifying assumptions.  Few, if
any, of these assumptions are true in actual  practice.   Real effects not considered in the above
theoretical development include:
       •   Filter pores are not uniformly sized, right circular cylinders
       •   Particles are not spheres of uniform radii
       •   Chemical  reactions may become important at high temperatures and pressures
       •   Corrosion of filter material  may be important at high temperatures or in adverse environ-
           ments
       •   Pressure  fluctuations may cause changes in dust cake properties
      •   The effects  of reentrainment  may be significant.
                                                 10

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    A - Establishment of cake
    B — Homogeneous dust deposit
      Total filtering cycle
                      16   20    24   28
                       Time, minutes
32  36   40   44
Figure 3.   Pressure response in constant  rate  gas  filtration.
                              11

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Consequently, the expressions for efficiency and pressure drop should be taken as approximations,
useful only to illustrate functional  relationships of important system parameters.
       The effects of temperature and pressure on filter operation are introduced largely through
changes in the fluid viscosity.   The  viscosity of air, for example, is relatively unaffected by
pressure, but is (to a good approximation)  directly proportional  to temperature.  Consequently, as
temperature increases, both viscosity and filter pressure drop increase (cf. Equation (10)).  In
addition, thermal expansion can  decrease the porosity and permeability.  These effects also give
rise to increased filter pressure drop.
       The effects of temperature on  filter collection efficiency are similarly adverse.  Strauss
and Lancaster (Reference 8) have shown that collection efficiency (through the mechanisms of impac-
tion and interception) decreases as the gas viscosity increases.   Conversely, collection efficiency
due to particle diffusion may increase slightly with increasing temperature.  Therefore lower col-
lection efficiencies are expected at  increased temperatures for particles larger than 0.2 microns
in diameter.   The converse is true for particles smaller than 0.2 microns.
                                                 12

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                                             SECTION 4
                                         CURRENT RESEARCH

       Westinghouse Research Laboratories is currently performing the only large scale effort
directed toward applying ceramic membrane filters to  particulate removal from hot gas streams.
This study has potential application to cleaning high temperature fuel gas from coal gasifiers,
and is being funded by the EPA  (Reference 9).  The Westinghouse effort seeks to develop thin
(0.25 mm) cylindrical membrane  filter elements with small, uniform pore size (0.5ym).  These fil-
ter elements are then to be tested and evaluated as a technique for collecting sub-micron particu-
late from a high temperature (>1500°F) fuel gas stream.
       To date progress in obtaining appropriate planar samples of the filter material for perfor-
mance testing has been limited.  Fabrication problems have included:
       •   Difficulty in laying down a planar membrane free of oxide irregularities, which can
           become large holes when the membrane is etched
       •   Difficulty in converting the initially deposited yalumina to a-alumina without warping
           the filter disk (warped disks break when installed in filter holders for performance
           testing)
       •   Difficulty in uniformly enlarging the pores throughout the membrane to produce a filter
           with acceptable pore size.
As a result of these problems,  few data for either clean gas flow characteristics of particulate
removal performance are available.  Recently Horizon Research has fabricated a  suitable ceramic mem-
brane and support structure, and has performed several successful  preliminary performance tests.
However, it appears that development of this material will be curtailed due to  continued difficulties
in preparation of suitable samples.
                                                 13

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                                             SECTION 5
                               LITERATURE AND MANUFACTURERS SURVEYS

       There is a paucity of data available on the use of ceramic filters to collect particulate from
 hot gas streams.  A limited survey of filtration literature and of ceramic manufacturers/suppliers was
 therefore undertaken to determine:
       •   The available types of ceramic filter materials
       •   The use of ceramic filters in current filtering applications
       •   The types of ceramic filter materials which may be suitable for collecting sub-micron
           particulate from a high temperature gas stream.
 The survey was accomplished in four steps:
       •   Review of existing filtration literature
       •   Telephone contact with ceramic filter suppliers
       •   Telephone contact with ceramic manufacturers
       0   Telephone contact with monolithic catalyst support manufacturers.
       The literature survey revealed that sub-micron particle ceramic filters are in use  in medical
 aerospace, electronic and biological applications for both gases and liquids.  However, no discussion
 of the operation of these filters at high temperatures was found.  This appeared to be more a case of
 lack  of present applications rather than ceramic material limitations.
       These findings prompted the telephone survey discussed below.  The purpose of the survey was
 to contact a representative sample of ceramic manufacturers and suppliers, and to determine if capabil-
 ities exist to develop a suitable rigid ceramic filter for application to hot gas clean-up.  As a guide,
 a  representative  set of operating conditions was established (see Table 1).  The conditions in Table 1
 approximate those from a low BTU coal gasifier downstream of the cyclones.  The key parameters are  the
 temperature and the particle size limits.  A summary of the relevant telephone contacts  is given  in
Table 2.
                                                  14

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TABLE 1.   FILTER OPERATING CONDITIONS
Temperature
Pressure
Gas Flow Rate
Gas Composition (% Vol)









Molecular Weight
Density
Heat Capacity
Viscosity
Particulate Loading
(upstream of filter)
Distribution (by weight)



Particulate Loading
(downstream of filter)
Distribution (by weight)



1100 to 1400°K
2000 kPa
200 mVmin
H2
CO
H20
co2
N2
CH4
H2S
COS
NH3
tars, heavy HC,
23
4.8 kg/m3
2510 J/kg°C
3.5 x 10-5 N-s/m
1.144 x 10'3 £f
100% < 30ym
80% < lOym
50% < 4ym
15% < lum
1.144 x 10-5 |jjf
100% < 6ym
98% < 4ym
95% < 2ym
80% < lym
(1500 to 2000°F)
(300 psia)
(7000 SCFM)
21
14
13
n
38
2.5
0.5
30 ppm
600 ppm
others trace

(0.3 Ibm/ACF)
(0.6 Btu/lbm°F)
2 (0.035 centipoise)
(0.5 grain/SCF)




(0.005 grain/SCF)




                  15

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                         TABLE 2.  SURVEY RESULTS
Company
1. Babcock & Mil cox Co. ,
Refractories Div.
Augusta, Georgia
2. Coors Porcelain Co.
Golden, Colorado
3. Corning Glass Co.
4. Do! linger Corp.
Rochester, New York
5. General Refractories
Bala Cynwyd, Pa.
6. Horizons, Inc.
Cleveland, Ohio
7. 3-H Company
Saint Paul , Minn.
8. Norton Company
Worcester, Mass.
9. Selas Flotronics
Springhouse, Pa.
10. Wisconsin Porcelain Co.
Sun Prairie, Wisconsin
Code*
c
c,f
f,s
f
c.s
c
c,s
c,s
f
c,f
Comments
Did not think they had any materials
that would work for the application.
Several small scale filters for this
particle size. No high temperature
filter experience. Samples sent to
Aerotherm. Nominal wall thickness
~6 mm (1/4").
Nothing for this application. Celcor
cordierite monoliths a possibility.
Some filter elements that would work
for this application. Relatively
thick wall, large pressure drop
(-100 kPa (1 atm)). Elements
available for testing.
Nothing for this application. Ver-
sagrid cordierite honeycomb is a
possibility; however geometrical
constraints a problem.
This membrane (-0.25 mm thick) being
developed for testing in this applica-
tion under Westinghouse — EPA program.
AlSiMag 795 (cordierite) honeycomb
structure should work for this appli-
cation. Elements available for test-
ing. Low pressure drop. High sur-
face area to volume ratio. Good
process control over pore size,
porosity and membrane thickness.
Samples sent to Aerotherm.
Two materials suitable for thick
walled filters. Also Spectramic
honeycomb is a possibility.
Micro-porous porcelain element
would be suitable. Pressure drop
~50 kPa. Sample sent to Aerotherm.
Thick walled filter elements
similar to 4 and 9. No membranes.
c - ceramic manufacturer
f - filter supplier
s - catalyst support manufacturer
                                       16

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       All  contacts were asked to supply information pertaining to:
       •   High temperature operation
       •   High flowrate operation
       •   Cleaning procedures
       •   Cost
       t   Novel applications and design ideas.
In addition, all contacts were asked if they were supplying anyone with ceramic elements suitable
for hot gas cleaning, if they were developing any materials suitable for this application, and what
if any, material limitations should be considered for this application.
       In general,  two  types of ceramic materials suitable for this application were identified.
These  are discussed separately in the following sections, and a brief discussion of possible filter
element cleaning methods is also given.

5.1    THICK WALLED ELEMENTS
       The type of  filter element generally available from ceramic manufacturers and filter suppliers
is referred to as a  "thick walled element".  It is usually cylindrical and has a wall  thickness  of
4 to 6 mm which is  "thick" in comparison to the Westinghouse/Horizons membrane and ceramic monoliths
(wall  thickness ~0.25 mm).  For large flowrate applications, the elements (typically 50-100 mm in
diameter and 250-300  mm in length) would be grouped in an assembly similar to the one shown in Figure
4.  The wall thickness  of the element is somewhat limited by the ceramic forming process; however,
a more significant  limitation is mechanical strength.  The structural strength of the wall decreases
with decreasing wall  thickness; hence, thin walls in the cyclindrical geometry would probably be  too
fragile for heavy duty  use.
       Thick walled elements have several  inherent disadvantages.  First, the pressure drop across
an element increases  directly with the wall thickness (see Equation (11)).  Typical pressure losses
for a  6 mm thick filter of this type are shown in Figure 5 with pore size as a parameter.  Values on
the order of 35 to  70 kPa (5 to 10 psi) may be expected for filters of this type.  A second problem
with thick walled elements is the possible occurrence of thermal stress and spelling when the element
is subjected to temperature cycling.  This requires considerable care in start-up and shut-down pro-
cedures.  Finally,  material costs for thick walled elements are greater than for thin walled elements.
This is discussed in  more detail in Section 6.
                                                 17

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Figure 4.  -Multiple element filter assembly.


-------

   200
   150-
3.
Q.

   TOO.
3
CO
to
S-
o.
    50-,
                                     10                            100
                                         Flow rate — 'cm3/sec-cm2
                                                                                                    psi
                                                                                                   t-25
  -20
  -15
  -10
                                                                                                   -5
1000
               Figure 5.   Flow rate  of  air at standard conditions for a typical ceramic
                          cylindrical element, wall thickness ~ 6.0 mm.

-------
       The  impact of the disadvantages described  above  will  have to be assessed in ngnt or outer
ceramic devices  and participate  removal methods.   An  adequate assessment can be made on-ly if opera-
tional performance data at  the conditions of  interest are available.

5.2    THIN WALLED ELEMENTS - CATALYST MONOLITH SUPPORTS
       The  ceramic monoliths  used  as  catalyst supports  for combustion processes were considered as
potential filters, since the  desired  characteristics  of a ceramic membrane filter are very similar
to those  of a  monolith, i.e.,
       •    High  temperature capability
       t    Structural  integrity
       t    Large surface area to volume ratio
       •    Moderate porosity  (25-30 percent)
       •    Small  pore  diameter  (less  than 10pm).
       These ceramic monoliths are manufactured by several  companies (see Table 2) in a variety of
configurations.   Typically  they  have  a honeycomb  appearance with a wall  thickness of approximately
0.25 mm.  The  honeycomb construction  provides excellent structural strength.  Figures 6 through 11
illustrate  some  of the various structural configurations.   Those monoliths manufactured by an extru-
sion process have rather limited geometric  flexibility.   However, some processes (e.g., 3M Company
as shown  in Figure 7)  allow very flexible geometries.  The 3M process is similar to that used in
making corregated paper products.  3M reports that the  process allows independent control over wall
thickness,  pore  size and porosity.  A typical  pore size distribution for one of 3M's products is shown
in Figure 12.  Preliminary  flowrate/pressure  drop relationships for the 3M material are shown in
Figures 13  and 14.  It should be noted that pressure  drop is in the 1 to 10 kPa range which  is a fac-
tor  of 10 to 100 less  than  that  for thick walled  ceramic  elements.  The decrease in flowrate with in-
creasing temperature shown  in Figure  14 is  primarily  due  to increases in gas viscosity.  The advantages
discussed above  strongly suggest that this  type of material  be tested for use as a fine particulate
filter.

5.3    POTENTIAL"CLEANING METHODS
       During  the course of the  survey several methods  were proposed for cleaning the filter elements.
These fell  into three  general categories:
       •   Ultrasonic  treatment
       •   Washing
       •    Back flow
                                                  20

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                   a.   8x  enlargment
b.  Rolled structures
c.  Rolled and stacked structures
 Figure  6.   Examples  of  3M  Company's ThermaComb
            corrugated ceramic.
                       21

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                SC SPIH CELL  (Note Separator)
           XFSC
        CROSS-FLOW,
         SPLIT CELL
       Note separators
       and corrugations
           at 90°
    XXSC
 CRISS-CROSS,
  SPLIT CELL
Note separators
and corrugations
    at 45°
    XXHC
 CRISS-CROSS,
 HONEYCOMB
with corrugations
   at 45°
 Note there is no
   separator.
Figure 7.    Structural  shapes  for  3M  ThermaComb.
                             22

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ej
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oo

5
        Figure 8.  Examples of Coming's Celcor  cordierite monoliths,
                                 23

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                      a.   Straight honeycomb
b.  Slant cell honeycomb
c.  Cross-flow honeycomb
         Figure 9.   Examples of  Dupont's  Turvex  honeycomb.
                                  24

-------
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 Figure 10.   Example of General Refractory Company's
            Versagrid ceramic  honeycomb.
                          25

-------
Figure 11.   Examples of Norton Company's  silicon
            carbide Spectramic honeycomb.
                      26

-------
c
(0
-C
re
O)
en
OJ
S-
o
CL
      IOC
       80-
       50.
40-
       20-
                                                                                                  (0
                                                                                                   I
                                                                                                  ^_

         100               10                 1.0              0.1               0.01


                                       Pore diameter (microns)


              Figure 12.  Pore size distribution for  3M  Company's  ThermaComb AISiMag 795.

-------
 100-i
                                  AP (in of H20)
                   0.5
       1.0
        I
            1.5
            2.0
             i
  80-

  60-
o

01
  40 -
o
  20-
                 r
                0.1
 r
0.2
   0.3
AP (kPa)
 r
0.4
 I
0.5
                                                                           0.6
              Figure 13.   Pressure drop across  an  0.2  mm (0.008 in)
                          AlSiMag 795 flat ceramic piece.
                                        28

-------
    560-
   480
   400
320
E
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c
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-------
No specific information was obtained concerning either possible implementation methods or possible
treatment efficiencies of sonic cleaning although it was  generally thought that the application of
ultrasonic energy would aid and speed a washing cycle.  Washing of a filter would necessarily'be done
off-line due to time and temperature requirements.   Thick walled elements  would require slow cooling
to prevent thermal stress, cracking and spalling.   Thin walled elements  probably would not require as
lengthy a cool-down period.
       Back flow appears to be the most promising cleaning method at this  time.  There are numerous
ways this can be accomplished.  One is to briefly take  a  filter element  off-line and use the pressure
in the filter assembly to blow down the element in  a reverse  flow pulse.   Alternatively, part of the
clean gas could be used to reverse flow one element of  a  multi-element assembly.   Gravity would carry
the particles to the bottom of the assembly and possibly  out  of the vessel.   Another possibility
is the use of a pressure pulse similar to baghouse  cleaning methods.   Cleaning methods and duty cycles
still require considerable experimental investigation.
                                                 30

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                                             SECTION 6.
                                       PROPOSED TEST  PROGRAM

       At the conclusion of the work described in Sections 4 and 5 it was evident that the only way
to realistically evaluate high temperature,  high pressure ceramic filters would be to test the
available materials at the conditions  of  interest.   Three materials were identified for testing,
and a test matrix was prepared.  The materials and the test matrix are discussed below.
       A standard ceramic filter manufactured by Selas Flotronics was selected as representative
of the "thick walled" elements described  in  Section  5.1.  This material has been tested and used in
low temperature environments; however,  there are no  data available on the high temperature (T  > 200°C)
performance of this material.  There is a relatively large pressure drop (50 - 100 kPa) across the
element.  It is expected that the  pressure drop will increase at higher temperatures.
       A cross-flow ceramic monolith manufactured by 3M was selected to represent the ceramic  mono-
lith elements described in Section 5.2.  The primary reason for this  choice  was  that  this was the
only monolith available in a cross-flow geometry.  Preliminary data for the pressure drop-flowrate-
temperature relationships were available  from 3M (Figures 13 and 14).  However,  there are no data  on
the filtration characteristics of  this  material.  Several samples of this material  were provided by
3M.  These samples and a low temperature  element holder were delivered to Westinghouse for testing.
The split cell cross-flow construction  is shown in Figure 3.  Sketches of the material and holder
are shown in Figures 15, 16 and 17.
       A third material, which is  significantly different from the two described above, was also
identified.  This material, called alumina FiberForm, is manufactured by Fiber Materials, Inc.  It
is made of alumina-silica fibers bonded with a high  purity alumina binder and produced using vacuum
slurry molding techniques.  FiberForm  has a  useful temperature limit of about 1450°C (2600°F).  It
is a very high porosity, low density material and has a texture somewhat like styrofoam.  This ma-
terial has never been tested as a  filter; however, its pore size, porosity and temperature limits
make it an attractive candidate.  Samples of FiberForm have been delivered to Westinghouse.
                                                31

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Figure 15.  3M crossflow ceramic monolith.

-------
CO
oo
                                                                                                                              -j-
                                                          Figure 16.  3M  element  low  temperature holder.

-------
Figure 17.  3M element and holder mounted inside pipe.

-------
       A test plan for the evaluation of potential filter materials was prepared and is included
as Appendix A.  The major test objectives for both low and high temperature testing are:
       •   Establish pressure drop-flowrate relationships for clean air flow
       •   Determine fine particle collection efficiency
       •   Measure pressure drop as a function of time for dirty air
       •   Investigate various cleaning methods
       The testing would be done in two phases.  The first phase is for low temperature testing and
screening of materials.  Only those materials that perform satisfactory will  be tested at high
temperatures.
                                                 35

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                                             SECTION 7
                                         PROCESS ECONOMICS

       Lack of sufficient data at present precludes accurate calculations of process costs for a
 high temperature particulate cleaning device utilizing ceramic membrane filters.  However, suffi-
 cient  preliminary data do exist to obtain an order of magnitude estimate of the capital require-
 ments  and operating costs for a ceramic filter, gas cleaning plant.
       Westinghouse Research Laboratories has compiled extensive cost data on ceramic filtration
 for cleaning  fuel gas from a coal gasifier for use in a combined cycle power plant.  These data
 appear in Reference 9 and will only be briefly summarized here.
       Westinghouse compared the costs of a ceramic membrane filtration system to those of a com-
 bined  granular bed/conventional baghouse filtration system.  For purposes of illustration, the
 initial  capital investment and the annual operating expenses were estimated for each particulate
 cleanup  system which treats approximately 30 mVsec (63,600 ACFM) of fuel gas at 870°C and 1620 kPa
 (235 psia).   This is equivalent to the output of a coal gasifier which supplies fuel to a 250 MW
 combined cycle plant.  An installed capital cost of $8.25 million and total annual operating ex-
 penses of $1.8 million were estimated for the granular bed/conventional baghouse system.  Esti-
 mated  costs for the ceramic membrane filter system were made for various filter characteristics —
 pore diameter, membrane thickness, gas velocity, free cross section, etc.  For a filter with 1
 micron diameter pores, the estimated capital investment ranged from about $0.7 to $7.0 million,
 and total annual operating expenses ranged from $0.7 to $2.3 million.  For example, for a case
 requiring 800 m2* of 0.25 mm thick ceramic membrane filter, the capital investment is $2.1 million
 and the annual costs are $0.9 million, which is easily competitive with the above alternative.
       Several ceramic materials currently produced by ceramic and catalyst monolith suppliers
were described in a previous section.   Many of these materials have the potential to meet the re-
quirements of a hot gas filtration system.  A cost comparison of various filter systems operating
at the conditions shown in Table 1 is given in Table 3.  These results are for a single
*
 Pore size = lym, superficial gas velocity = 4.5 cm/sec, pressure loss = 60  kPa.
                                              36

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filter system and do not include any duplication which may be required for on-line/off-line opera-
tion.  The costs shown are for the filter materials only; no pressure vessel or tube sheet costs
are included.  It is interesting to note that the pressure drop required for either the thick- or
thin-walled membranes is significantly lower than the 50 to 80 kPa estimated for reasonable flows
through the Westinghouse/Horizons material.  This is primarily due to the different pore size  and
permeability of these materials.

            TABLE 3.  COMPARISON OF' FILTER ELEMENT COSTS FOR THE CONDITIONS IN TABLE  1

Wall Thickness - mm
Flow Area - m2(ft2)
Superficial Velocity - cm/sec
(in/sec)
Approximate Pressure Drop, Clean -
kPa (psi)
Size of Elements - mm (in)
Number of Elements
Approximate Cost of Elements
Thick-Wall
4.76
8.17
(88)
9.1
(3.57)
34.5
(5)
66.7 dia x 254 x 4.8
(2-5/8 dia x 10 x 3/16)
153
$4600
($560/m2)
Thin-Wall
0.25
24.00
(258)
2.54
(1.0)
3.732
(0.54)
152 x 152 x 152
(6x6x6)
17
$850
($35.50/m2)
Westinghouse
0.25
17.0
(177)
4.5
(1.77)
60.0
(8.7)
-
-
$4080
($240/m2)
       The most interesting aspect of the cost comparison is the projected cost for  thin-wall ce-
ramic material in monolith form.  Currently available material at $35.50/m2 for 4  cells/cm is
roughly 10 times less expensive than the projected cost of the Westinghouse ceramic  material.   If,
for either material, the costs associated with plant construction are approximately  equivalent, and
if the element cost is a significant portion of total cost of the system,  then the use of ceramic
monoliths offers a great potential cost savings.
       It appears that the economics of ceramic membrane filters, in particular the  ceramic  monoliths,
compare quite favorably with other gas cleanup schemes for particulate removal from  high temperature
gas streams.
                                                  37

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                                             SECTION 8
                                  CONCLUSIONS AND RECOMMENDATIONS

       This  investigation resulted in the following conclusions:
       •   The theory for the operation of membrane filters is not adequate to predict the opera-
           tion of  real filters.
       •   The Westinghouse project has had  only  limited success thus far in developing and testing
           a ceramic membrane filter.
       0   Current  available ceramic filters
           —  appear promising for high temperature fine particulate control
           —  appear to be economically feasible
           -  need to be experimentally tested for high temperature operation.
       •   Ceramic  honeycomb monoliths
               offer excellent possibilities for use in high temperature particulate control
           -  are  economically superior to  present ceramic filter elements
           -  need to be experimentally tested in particulate control applications.
       Before adequate assessment of these control methods can be made, several important questions
must be answered.   These are:
       •   What is  the relationship of collection efficiency to pore size and pore size distribu-
           tion and to particulate size and  size distribution?
       t   What is the relationship of pressure loss to pore size, porosity, and permeability?
       •   How susceptible to clogging are the ceramic elements?
       •   How can the elements be cleaned?
       An experimental program that will provide answers to the above  questions  is recommended.
This program utilizes currently available ceramic filter elements and  ceramic monoliths,  and  thus,
requires  no material development.
                                                38

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                                            REFERENCES


1.  Oavies, C. N., Air Filtration, Academic Press, London,  1973.

2.  Spumy, K. and Pich, J., "Analytical Methods for  Determination of Aerosols by*Means of Membrane
    Filters:  VI, On the Mechanisms of Membrane Ultrafilter Action.  VII, Diffusion and Impaction
    Precipitation of Aerosol Particles by Membrane Ultrafliters," Collect. Czech. Chem. Commun.,
    Vol. 28, 1963, pp. 2886-2894; Vol. 30, 1965, pp.  2276-2287.

3.  Spurny, K. and Pich, 0., "Zur frage der Filtrationmechanismen bei Membranfiltern," Staub, Vol.
    24(7), 1964, pp. 250-256.

4.  Spurny, K. and Pich, J., "Auffangen von Aerosolteilchen mittels Membranfilter unter Wirkung der
    Diffusion und Impaction," Zent. Biolog. Aerosol Forsch., Vol. 11(6), 1964, pp. 508-511.

5.  Pich, J., "Abscheidung von Aerosolteilchen durch  Ausschleuderung in der Umgeburg einer kreis-
    formigen Offnung," Staub. Vol. 24(2), 1964, pp. 60-62.

6.  Pich, J., "Impaction of Aerosol Particles in the  Neighborhood of a Circular Hole,"  Collect.
    Czech. Chem. Commun., Vol. 29, 1964, pp. 2223-2227.

7.  Caroff, M., Choudhary, K. R., and Gentry, J. W.,  "Effect of Pore and Particle Size Distribution
    on Efficiencies of Membrane  Filters," J. Aerosol  Sci.,  Vol. 4(2), 1973, pp. 93-102.

8.  Strauss, W. and Lancaster, 8. W., "Prediction of  Effectiveness of Gas Cleaning Methods at High
    Temperatures and Pressures," Atmospheric Environment, Vol. 2, 1968, pp. 135-144.

9.  Westinghouse Research Laboratories, Monthly Progress Reports, "Fine Particle Collection," EPA
    Contract 68-02-1887.
                                                 39

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                                            APPENDIX A
                                         FILTER TEST PLAN

1.     NOMENCLATURE
       A   -   Surface area available for filtration (cm2)
       B   -   Inlet gas particle loading (g/cm3)
       P   -   Pressure (kPa)
       AP  -   Pressure drop across a filter element (kPa)
       Q   -   Gas flowrate (cmVsec)
       t   -   Time (sec)
       T   -   Temperature (°K)
       V   -   Superficial gas velocity, Q/A (cm/sec)
       TI   —   Particle collection efficiency
2.     AVAILABLE TEST FACILITIES
       Several  of Westinghouse Research Laboratories'  filter test facilities are available for use.
The flow conditions for three of them, which are to be used in the initial phase of the testing, are
given below.
2.1    10 Liter/min Facility
       •   Q from 15 to 150 cmVsec (1 to 10 £/min)
       •   Maximum AP of 50 kPa  (7 psi)
       •   T to 1150°K (1600°F)
       •   Atmospheric pressure
       •   Polydisperse particles,  sub-10 ym diameter
       •    Particle loading limits  unspecified  (but nominally 0.1 to 0.5 grain/SCF)
                                                40

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 2-2    100 Liter/min  Facility
        •   Q  from 500 cmVsec to 5000 cmVsec  (30  fc/min.  to  300  fc/min)
        •   Maximum AP of 6 kPa  (1 psi)
        •   Ambient temperature
        •   Atmospheric pressure
        •   Polydisperse particles, sub-10 pm diameter
        •   Particle loading limits unspecified (but nominally 0.1 to 0.5  grain/SCF)
 2.3    High Flowrate Facility
        •   Q  up to 2.36 x 105cm3/sec (14,158 tjm, 500 acfm at 1500°F)
        •   Maximum AP of 7.5 kPa (7.1 psi)
        •   Temperatures up to 1150°K (1500°F)
        •   Atmospheric pressure
        •   Polydisperse particles, sub-10 ym diameter
        •   Particle loading limits unspecified (but nominally 0.1  to 0.5  grain/scf)
 3.     FILTER TEST MATERIALS
        Three  types of ceramic filter materials will  be tested.   If other materials become available
 they will  be  included in the Phase 1  testing.
 3.1     Thick  Walled  (1/8"  to 3/8")  Ceramic Filter Disks
        Several disks  will  be tested  in  the 1  to 10 £/min.  facility.  Filter properties to be varied
 include pore  size  and disk  thickness.
 3.2     Thin Walled  (-0.010")  Ceramic  Catalyst  Monoliths
        Several  monoliths will be tested  in the  30 to 300 ft/mln. facility.  The cell size and wall
 thickness may  be varied.
3.3    Alumina  FiberForm
       Alumina  FiberForm, manufactured by  Fiber Materials, Inc., is a new material made of alumina-
silica fibers  bonded with a high purity alumina binder  and produced using vacuum slurry molding
techniques.   This material is significantly different from the ceramic filter materials and the
                                                41

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ceramic monoliths.   It has a useful  temperature unit of about 1450°C (2600°F)  and a very high
porosity.

4.     PRETEST ACTIVITY
       •   Westinghouse will procure suitable ceramic filter disks and disk holders
       •   Aerotherm will  procure catalyst monolith materials and FiberForm, and deliver them to
           Westinghouse

5.     FILTER TEST MATRIX
       Filter testing will proceed in two phases - Phase 1  for ambient temperature tests and Phase
2 for high temperature tests.  The Phase 1 testing is intended to screen out materials which are
not suitable for use as fine particulate filters.

5.1    Phase 1 - Ambient Temperature Testing (~80°F)
       This test phase has the following general objectives:
       •   Obtain AP versus V  relationships for clean gas flow at ambient temperature
       •   Evaluate n as a function of t, V , and particle size at ambient temperature
       •   Evaluate the effectiveness of various backflow filter cleaning methods
       •   Evaluate various filter cycle possibilities
Testing to fulfill these objectives will be accomplished in four test series.

5.1.1   Test Series 1 - Clean Flow Characterization
       •   Objective:
           - Establish the AP versus VQ relationships as functions of filter pore size and thickness
             for clean gas flow at ambient temperature
       •    Test Variables:
           -Q  - vary over appropriate  facility test range
           - Pore size  - vary  by  testing several  elements of each type
           - Thickness  - vary  by  testing several  elements of each type
      •    Measure:
           - AP  as a  function  of  Q
                                                 42

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 Results  from this series Will  consist of plots of AP vs VQ, with filter pore size and  thickness as
 possible parameters.

 5.1.2  Test Series 2  -Participate Removal Efficiency Characterization
       •   Objectives:
            - Determine  AP versus t as a function of C, VQ, and filter pore  size at ambient tempera-
              ture.
            - Determine  filter  collection efficiency (n) versus particle  size as a function of C, V ,
              and filter pore size.
            — Investigate the effects of cake buildup and compression  on  n-
       •   Test Variables:
            - Q - vary over appropriate facility test range
            -C - vary in the range 0.2 to 1.0 x 10~5 g/cm3 (0.1  to 0.5 grain/SCF) for each flowrate
            — Pore size  - vary  by testing several  elements  of each type
       t   Measure:
            - AP vs t
            — Inlet particle loading and size distribution
            — Outlet particle loading and size distribution as  a  function of time
       Inlet gas particulate load will  consist of a polydisperse sub-lOpm particle mixture.   Each
 filter element is to  be tested at several  gas flowrates  and several inlet particle loadings.   Mea-
 surements of AP versus  t will  give the  rate  of dust cake accumulation on the filter.   The influences
 of gas superficial  velocity, inlet particle  loading,  and filter pore  size on this rate of accumula-
 tion will be  investigated.   Comparison  of outlet  particle  load and size distribution  with inlet load
 and distribution  will allow calculation of particle collection efficiency versus particle size.  The
 influence of V ,  C, and filter pore size on  n will  also be investigated.  Measurement of n versus t
 will allow  assessment of the relative contributions to particle  collection  from filter collection
 and dust cake  collection  mechanisms.  Obviously,  the filter element should  be thoroughly cleaned be-
 tween individual  experiments.   Results  from  this  series  will include  plots  of AP  versus t, and n as
a function  of  particle  size versus  t, with C,  VQ,  and pore size  as parameters.  The possibility of
combining this  series with  test  series  3 should be  considered.
                                                  43

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5.1.3  Test Series 3 -Cleaning  Method  Study
       •   Objective:
           - Investigate various backflow filter  cleaning methods  including  steady backflow and
             pulsed backflow
       t   Test Variables:
           - Backflow Q and duration  of backflow  for  steady  backflow methods
           - Pulse pressure and  duration for  pulsed backflow methods
       •   Measure:
           - Initial AP after the cleaning operation
       The primary purpose  of this study is to  observe  dust  cake removal  and pore  cleaning.   Two
types of backflow cleaning  experiments  should be  performed:  steady backflow, in which  the  rate and
duration of backflow are varied, and  pulsed backflow, where  the backflow  pressure  pulse magnitude
and duration are varied. Measurement of the  initial, clean  gas AP (forward  flow)  will serve as a
reference point to define the degree  of dust  cake removal achieved.  Assessment of the degree of
short term (one cycle) pore clogging  and the  effect of  V  on pore  clogging will also be possible.
This series will result in  the determination  of the "best" backflow cleaning methods for each fil-
ter element type.  The possibility of combining experiments  in this series with those  in Series 2
should be considered.

5.1.4  Test Series 4 -Cleaning  Cycle Study
       •   Objectives:
           -Determine feasible, long-term filter cycles, including filter times and cleaning times
             for the "best"  cleaning  methods  from Series 3
           - Investigate the  effects  of  filter  pore clogging on long term filter operations, includ-
             ing an  estimate  of  filter  lifetime at ambient temperature
          —  Investigate the effects of  flow channel  clogging in monolith elements on  long-term
             filter operation
      •   Test Variables:
          - Filter time and cleaning time in  a  complete filter cycle
          -Q
          -C
                                                44

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       •   Measure
           — AP versus t during filtering operation
           — TI as a function of particle size
       This test series will extend the work of Series 3 by investigating feasible filtering cycles,
using the "best" backflow filter cleaning method(s) defined in Series 3.  A "best" combination of
filtering time, followed by cleaning time, over many filter cycles will be described for long-term
filter operations.  Since the rate of dust cake accumulation is dependent on filtering flowrate and
inlet particulate loading, these variables will be parameters in the cleaning cycle description.   As
such, Q and C will be varied during this test series.  Measurements of AP versus t and initial  filter
cycle AP will be used to evaluate candidate filter cycles.  Occasional measurements of particulate
collection efficiency should also be performed to monitor filter performance.   It is expected that
initial cycle AP will increase with time as filter pores clog; therefore, the length of the filter-
ing portion of a cycle will have to decrease as number of cycles performed increases.  The rate of
this increase in initial AP with time will serve to define the useful life of a filter element.  An
additional concern relates to flow channel clogging in monolith elements.  Backflow alone may not
completely clear these channels.  The effects of this clogging on element usable lifetime may also
be assessed by noting the time rate of increase in initial cycle AP.  Results from this series will
consist of time specifications for "best" feasible filter-clean cycles, together with estimates of
filter element usable life.

5.2    Phase II - High Temperature Testing
       High temperature testing will be performed for those materials identified in the Phase 1 test-
ing as potential filters.  General objectives for this phase of testing include:
       •   Obtain AP versus V  relationships for clean gas as a function of temperature
       •   Assess potential filter porosity decreases, due to material  phase  change  or material  sin-
           tering, on AP vs VQ relationships
       •   Evaluate n as a function of particle size and  temperature  at constant  VQ  and  C
       •   Evaluate candidate filter-cleaning cycles at high temperatures
Testing to fulfill these objectives at temperatures up to 1100°K  (1500°F)  will  be accomplished in
four additional test series.
                                                 45

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 5.2.1   Test Series 5 — High  Temperature  Clean  Flow  Characterization
        •   Objectives:
            — Determine  AP vs V  for clean  gas  flow  as  a  function of  temperature
            — Determine  if changes  in the AP, V  curves can  be  accounted  for  solely  by  gas  viscosity
              changes or are  material  pore  structure changes also important
        i   Test Variables:
            -T - vary temperature  to 1100°K  (1500°F)
            — Q - vary flowrate over appropriate  facility test  range
            — Pore size  -  vary by testing several elements of each type
        •   Measure:
            — AP as a function of Q at each T
        AP is expected to  increase  with increasing temperatures, at constant  V  , due to
        t   Increasing gas viscosity with increasing T
        •   Potential  porosity decreases  due to phase change, or material sintering
        Results of this  series will  consist of  plots of AP versus V  with temperature as a  parameter
 for each pore size tested, and a determination of the  relative effects of gas  viscosity and decreases
 in porosity on AP-V  curves.
 5.2.2   Test Series 6 —High  Temperature  Particulate Removal Efficiency Characterization
        •   Objectives:
            — Investigate  AP  versus  t  as  a function of  filter pore size and temperature
            — Investigate  n as  a function of filter pore size and temperature
        •   Test Variables:
            - T -  vary to  1100°K (1500°F)
            — Pore size -  vary  by testing several elements of each type
        •   Measure:
           — AP versus t
           — Inlet particle size distribution
           - Outlet particle  loading  and size distribution  as  a function of  time
       The test series is essentially a  repeat of Series 2  with the  introduction  of temperature as
a primary test variable.  The  theory  of  filter particle  collection mechanisms  predicts that n should
decrease with  increasing  temperature.  This would imply  that  the  rate of dust  cake accumulation

                                                 46

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(and the slope of a AP versus  t  plot)  should  be  smaller at  high  temperatures.  However, these effects
may be offset by potential porosity  decreases as discussed  in  Section  5.2.1.  The findings of this
test series, taken with those  of Series  5,  will  serve  to define  the  relative magnitude of the effects
of possible decreased porosity versus  decreased  collection  efficiency  on overall filter collection at
high temperature.  Results from  this series will  consist of plots of AP versus t, with T as a param-
eter, at varying pore size, and  n as a function  of  particle size versus T at varying filter pore size.
5.2.3  Test Series 7 - High Temperature  Cleaning Cycle  Study
       •   Objective:
           — Determine feasible  high temperature cleaning cycles
       §   Test Variables:                                                                   ,
           — Filter time, cleaning time
       •   Measure:
           — AP versus t during  filtering operation
           — n as a function of  particle size
       This series is essentially a  high temperature repeat of Test Series 4.  In this series,  test-
ing at one flowrate, one particle loading,  and one  temperature should  suffice.  Test temperature
should be the highest temperature expected  in eventual  ceramic filtration applications (~1500°F).
The purpose of this test series  is to  refine  and extend the conclusions derived in Test Series 4 to
high temperature.  Results from  this test series will  consist of the time specifications for "best"
feasible high temperature filter-clean cycles, together with estimates of filter element usable life
at high temperature.
5.2.4  Test Series 8 - High temperature, High Flow  Tests
       This test series will be  conducted only with those materials that perform satisfactorily in
Test Series 5 through 7.  The  objective  of  this  test is to  simulate as close as possible "real world
conditions.  These tests will  be done  in the  high flow facility  described in Section  2.3.  The test
will encompass the activities  described  in  Test  Series  6 and 7.
                                                  47

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                                 TECHNICAL REPORT DATA
                          (Please read Instructions on the reverse before cornpleting)
  . REPORT NO.
  EPA- 600/2 -77 -056
                                                       3. RECIPIENT'S ACCESSION-NO.
 4. T.TLE AND SUBTITLE Evaluation of Ceramic Filters for High-
 Temperature/High-Pressure Fine Particulate Control
                                                      5. REPORT DATE
                                                       February 1977
                                                      6. PERFORMING ORGANIZATION CODE
 7. AUTHOR(S)
 G.G. Poe, R. M. Evans, W. S.  Bonnett, and
    L.R. Water land
                                                       8. PERFORMING ORGANIZATION REPORT NO.
9. PERFORMING ORGANIZATION NAME AND ADDRESS
Aer other m Corp.
485 Clyde Avenue
Mt. View, California  94042
                                                       10. PROGRAM ELEMENT NO.
                                                        1AB012; ROAP 21ADL-029
                                                       11. CONTRACT/GRANT NO.

                                                        68-02-1318, Task 25
 12. SPONSORING AGENCY NAME AND ADDRESS
  EPA, Office'of Research and Development
  Industrial Environmental Research Laboratory
  Research Triangle Park, NC 27711
                                                      13. TYPE OF REPORT AND PERIOD COVERED
                                                       Task Final;  12/75-6/76
                                                      14. SPONSORING AGENCY CODE
                                                       EPA/600/13
 is. SUPPLEMENTARY NOTES  j£RL-RTP Task Officer for this report is D.C.  Drehmel,  Mail
 Drop 61, 919/549-8411 Ext 2925.
 is. ABSTRACT
               repOrt gives results of a study to analyze and evaluate ceramic mem-
  brane filters as a new, fine particulate «3 micrometers) control concept for high-
  temperature (approx. 900 C), high-pressure processes. Several ceramic filters
  were identified as potential candidates for fine particulate removal.  There does not
  seem to be any inherent material limitation to high-temperature operation;  however,
  no evidence of high-temperature filter application was found. The filters typically are
  2-6  mm thick, cylindrical,  and available with various pore sizes, increasing upward
  from 0. 5 micrometer.  These elements may be suitable for fine particulate control in
  hot gas streams. The most promising, although undeveloped, idea for a ceramic fil-
  ter is to use ceramic honeycomb monoliths similar to those available for catalyst
  supports and heat exchangers.  The walls o.f the monoliths  are  about 0. 2-0. 4 mm
  thick and of varying pore size and porosity. Geometric configurations are available
  which would force the gas to flow through the membrane walls. Pressure losses
  would be very small relative to those of standard ceramic filter elements..  The
  application of ceramic monoliths to high-temperature fine particulate control appears
  very promising.  It is strongly recommended that this concept be investigated further.
 7.
                              KEY WORDS AND DOCUMENT ANALYSIS
                 DESCRIPTORS
                                          b.lDENTIFIERS/OPEN ENDED TERMS
                                                                    c. COSATI Field/Group
 Air Pollution
 Flue Gases
 Particles
  eramics
 Fluid Filters
 Membranes
                     Filtration
Air Pollution Control
Stationary Sources
Particulate  Control
High Temperature
High Pressure
13B
21B

11B
13K
11G,06C
07D
 3. DISTRIBUTION STATEMENT
 Unlimited
                                            9^ SECURITY CLASS (This Report)'
                                            Unclassified
                                                                   21. NO. OF PAGES
                                                                        52
                                          20. SECURITY CLASS (Thispage)
                                          Unclassified
                         22. PRICE
EPA Form 2220-1 (9-73)
                                        48

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