&EPA
             United States
             Environmental Protection
             Agency
             Industrial Environmental Research  EPA-600 2 80 .44
             Laboratory          June 1980
             Cincinnati OH 45268
             Research and Development
Calculations of
Painting Wasteloads
Associated  with
Metal  Finishing

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                RESEARCH REPORTING SERIES

Research reports of the Office of Research and Development, U.S. Environmental
Protection Agency, have been grouped into nine series. These nine broad cate-
gories were established to facilitate further development and application of en-
vironmental technology.  Elimination of traditional grouping was consciously
planned to foster technology transfer and a maximum interface in related fields.
The nine series are:

      1.  Environmental  Health Effects Research
      2.  Environmental  Protection Technology
      3.  Ecological Research
      4.  Environmental  Monitoring
      5.  Socioeconomic Environmental Studies
      6.  Scientific and Technical Assessment Reports (STAR)
      7.  Interagency Energy-Environment Research and Development
      8.  "Special" Reports
      9.  Miscellaneous Reports

This report has been assigned to the ENVIRONMENTAL PROTECTION TECH-
NOLOGY series. This series describes research performed to develop and dem-
onstrate instrumentation, equipment, and methodology to repair or prevent en-
vironmental degradation from point and non-point sources of pollution. This work
provides the new or improved technology required for the control and treatment
of pollution-sources to meet environmental quality standards.
This document is available to the public through the National Technical Informa-
tion Service, Springfield, Virginia 22161.

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                                           EPA-600/2-80-144
                                           June 1980
CALCULATIONS OF PAINTING WASTELOADS
   ASSOCIATED WITH METAL FINISHING
                   by
           GEORGE E. F. BREWER
           Coating Consultants
         Brighton, Michigan 48116
            Grant  No. R 803467
             Project Officer
              HUGH B. DURHAM
   Industrial  Pollution Control Division
Industrial  Environmental Research Laboratory
         Cincinnati, Ohio 45268
INDUSTRIAL ENVIRONMENTAL RESEARCH LABORATORY
     OFFICE OF RESEARCH AND DEVELOPMENT
    U.S.  ENVIRONMENTAL PROTECTION AGENCY
           CINCINNATI, OHIO 45268

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                                 DISCLAIMER

     This report has been reviewed by the Industrial Environmental Research
Laboratory - Cincinnati, U. S. Environmental Protection Agency, and approved
for publication.  Approval does not signify that the contents necessarily re-
flect the views and policies of the U. S. Environmental Protection Agency,
nor does mention of trade names or commercial products constitute endorsement
or recommendation for use.
                                     ii

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                                  FOREWORD

     When energy and material resources are extracted, processed, converted,
and used, the related pollutional impacts on our environment and even on our
health often require that new and increasingly more efficient pollution con-
trol methods be used.  The Industrial Environmental Research Laboratory-Cin-
cinnati (lEKL-Ci) assists in developing and demonstrating new and improved
methodologies that will meet these needs both efficiently and economically.

     The subject of the present study is the tabulation of the relative sizes
of the waste loads generated by commonly used industrial paints and painting
processes.  A system of mathematical equations has been developed for the com-
putation of the waste loads expected for any size and for almost any kind of
industrial painting operation.  All parties concerned with the selection of
less wasteful methods of industrial painting will find this report to be a
ready tool for their work.  For further information regarding this study the
Industrial Pollution Control Division should be contacted.
                                               David G. Stephan
                                                   Director
                                Industrial Environmental Research Laboratory
                                                  Cincinnati
                                     iii

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            Bake Curing	   41
            Radiation Curing 	   41
            Formation of Coreactants 	   43
   7 -   Sanding and Stripping	   45
            Sanding	   45
            Stripping	   46
   8.   Calculation of Waste Loads  	   48
            General	   48
            Prediction of Waste Loads  	   48
            Determination of Waste Loads 	   49
            Predicted vs Determined Waste Loads  	   53
   9.   Commercial Paint Compositions Surveyed  	   55
            General	   55
            Classification of Paint Compositions 	   56
            Waste Load Computation Data	   57
            Computations Using Manufacturer's Literature 	   57

Glossary	   68
                                   vi

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                                CONTENTS
Foreword	iii
Abstract	   iv
Figures	vii
Tables	   ix
Abbreviations and Symbols	    x
Conversion Factors 	   xi
Acknowledgments	xii

   1.  Introduction  	    1
            General  	    1
            Scope	    2
            Purpose  	    2
            Theoretical Approach 	 .  	    3
            Phases 	    3
   2.  Conclusions 	    5
   3.  Recommendations	    6
   4.  Survey Processes and Development of Calculations  	    7
            General  	    7
            Objectives 	    8
            Sources of Information 	    8
            Paint Compositions 	    8
            Selection of Paints	   11
            Buying and Using Paints  	   12
            Units of Measurement	   13
            Volume Calculations  	   14
            Organic Volatiles in Paints  	   17
            Organic Volatile Calculations  	   19
   5.  Painting Methods and Equipment  	   23
            General	   23
            Spray Painting	   23
            Dip Coating	   27
            Flow Coating	   28
            Curtain Coating	'	   28
            Roll Coating	   29
            Electrocoating 	   30
            Powder Coatings  	   31
            Paint Losses vs Transfer Efficiency  	   34
            Waste Loads vs Transfer Efficiency 	   35
            Transfer Efficiency Calculations 	   36
            Summary	   38
   6.  Paint Curing Methods	   40
            Ambient Temperature Curing 	   40

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                                 ABSTRACT

     This study presents methods for predicting the waste loads that will be
generated in planned painting operations, and for determination of the actual
waste loads in current operations.

     Nine major classes of industrial paints and the most widely used indus-
trial painting processes were surveyed and have been described.  The upper
and lower limits of frequently encountered waste loads have been tabulated.

     Twelve mathematical equations have been developed for the prediction of
waste loads or for determination of actual waste loads.

     This study indicated that the waste loads generated in most painting
operations can be significantly reduced through the use of better paint
materials and more efficient painting processes.  Such technologies are
currently in various stages of development, but their wide-spread adoption
will require years of field testing so that environmental demands and con-
sumer quality expectations can be"fully assured.

     This report is submitted in fulfillment of Grant No. R 803467 by
Coating Consultants, Brighton, Michigan under the sponsorship of the U. S.
Environmental Protection Agency.
                                     iv

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                                   FIGURES

Number                                                                   Page

  1   Film coating using an ideal nonvolatile filmforming solid.  ....    9

  2   Film coating using organic volatile solvent based liquid
        paint compositions	10

  3   Film coating using water based liquid paint compositions	10

  4   Film coating using organic volatile solvent and water based
        liquid paint compositions	11

  5   Calculations Schematic	14

  6   Maximum coverage equals mininum consumption	17

  7   Volume relationship of paint components	18

  8   Volume relationship of paint components "as used"	19

  9   Vol% ratio of 0V to NV components	20

 10   Air atomized spray	23

 11   Pressure atomized spray	24

 12   Electrostatic field assisted spray painting	25

 13   Centrifugal atomized spray	25

 14   Water bath spray paint booth	26

 15   Dip coating rigid, profiled merchandise	27

 16   Dip coating flexible, unprofiled merchandise	27

 17   Flow coating	28

 18   Curtain coating	28

 19   Roll coating	29

 20   Electrocoating	30


                                    vii

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21   Fluidized bed dip tank	32




22   Electrostatic fluidized bed	32




23   Fluidized electrostatic powder spraying	33




24   Waste loads vs percent expected transfer efficiency	39




25   Electron beam curing	41




26   Ultra-violet ray curing	42




27   Sanding painted surfaces	45
                                    viii

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                                   TABLES




Number                                                                   Page




  1   Commonly Used Paint Measurement Units 	 15




  2   Expected Transfer Efficiency  	 35




  3   Waste Loads vs Percent Expected Transfer Efficiency 	 38




  4   Classification and Composition of Paints Surveyed 	 60




  5   Range of 0V and NV Within Paint Classes Surveyed  	 67
                                     ix

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                           ABBREVIATIONS  AND SYMBOLS



             area                      W
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CONVERSION FACTORS
From: Metric
cm
cm
cm3
kg
kg /I
1
m
m2
ym
To: U. S.
in
in2
in3
Ib
Ib/gal
gal
ft
ft2
mil
Multiply by
0.3937
0.155
0.061
2.203
8.338
0.264
3.281
10.753
0.0394

From: U. S.
ft
ft2
gal
in
in2
in3
Ib
Ib/gal
mil
To: Metric
m
m2
1
cm
cm2
cm3
kg
kg/1
ym
Multiply by
0.3048
0.093
3.785
2.54
6.452
16.393
0.454
0.12
25.4
        xi

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                               ACKNOWLEDGMENTS

     Special thanks are due to Mr. James R. Blegen, Ashland Chemical Company,
Columbus, Ohio, for making typical paint formulations and advice available.

     Thanks for advice and assistance are extended to Dr. Hugh B. Durham,  Pro-
ject Officer, and to Mr. George F. Weesner and Mr. Gordon Haller of the Metals
& Inorganic Chemicals Branch, Industrial Environmental Research Laboratory,
U. S. Environmental Protection Agency, Cincinnati, Ohio.
                                     xii

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                                  SECTION 1

                                 INTRODUCTION
GENERAL

     Large quantities of contaminants are emitted into the environment as a
result of painting operations in the metal fabricating and finishing indus-
tries.

     Prior to 1960, typical industrial paint formulations contained approxi-
mately 40 wt% of paint solids dispersed in volatile organic solvents.   Thus,
60% of the total weight of all paints sold in the United States resulted in
organic volatile waste.  In addition, an estimated 20% of the total paint
solids weight became waste due to overspray, drip-off, and spillage.

     Painting operations result in the generation of three classes of  con-
taminant wastes:

     1)  Vapors of organic volatile solvents which are emitted into the at-
         mosphere unless they are captured and incinerated.  (Incineration
         may cause secondary pollutional waste loads which were not consid-
         ered in this study.)

     2)  Solid or  semisolid nonorganic materials (resins or pigments)  com-
         bined with some adhering organic volatile solvents which must be
         buried in the ground, either directly or after partial incineration.
         (In certain cases, some paint solids waste may be economically re-
         claimed.)

     3)  Minor quantities of nonvolatile waste (water soluble solvents, salts,
         surfactants, and other additives) which may find their way into
         clearing lagoons, sewers, or waterways.

     Since 1960, an increased awareness of environmental factors has resulted
in replacement of many particularly detrimental liquid paint components with
less objectionable materials.  Numerous new ecologically desirable improve-
ments in paint technology have been reported; in particular there have been
waterborne paints, high solids paints, paint powders, and radiation cured
paints introduced on the market.

     In 1970, it was estimated that the annual waste load generated by indus-
trial painting operations was more than 200 million kilograms  (220 thousand
tons) of organic volatile waste plus an additional 100 million kilograms

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(110 thousand tons) of semisolid waste that contained some organic volatiles.-1
At that time, approximately 60% of all industrial painting was done by conven-
tional spraying processes.  By use of this method, 40 to 60% of the paint
solids which enter the plant are not transferred onto the merchandise, but are
lost as unavoidable overspray.  Paint transfer methods other than conventional
air atomized spraying were variously reported as operating with much higher
transfer efficiencies, some as high as 98%.

     In 1973, inquiries which were addressed to the two largest organizations
in the field —the Federation of Societies for Paint Technology, Philadelphia,
Pa., and the National Paint and Coatings Association, Washington, D.C.— did
not produce any comprehensive surveys or statistics.  At that time, no tabu-
lations existed as to the quantities of waste generated by various types of
paints or by the use of different painting processes.

     A literature search produced a number of articles dealing with narrow
facets of the problem of painting wastes, but the literature did not reveal
a generally accepted method that would allow the determination of the waste
load generated by any given industrial painting operation.  No method was
found in the literature for th*e mathematical prediction of the waste load
that would be generated by a given size and kind of painting operation.  The
literature did not contain a method to predict the change in waste load that
would result from replacing one kind of paint or painting process with another.
SCOPE

     This study presents data which allows the calculation of predicted waste
loads generated during  the application of widely used paints by various com-
mon painting processes.  The reported data were compiled from the reviewed
scientific and trade literature and through direct communications with experts
in the painting field.

     Liquid or vaporized wastes and semisolid wastes are reported in weight
and volume units for a  specific size of painting operation and allow, there-
fore, the computation of the waste load for any size of painting operation.

PURPOSE

     This study is  intended to be a useful tool for the prediction of waste
loads that will be  generated by an industrial painting operation when a given
quantity of merchandise is to be painted using common paints and painting
techniques.

     This study can also be used for the determination of the actual waste
loads generated by  a specific industrial painting operation and for pinpoint-
ing unnecessary costly  and pollutional losses.  It should also be an aid to
those engaged in the selection of the best available paint and painting pro-
cess for a particular job.
1 Wapora,  Inc.:   EPA Contract  No.  68-01-2656

                                      2

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THEORETICAL APPROACH

Premises

     1)  Paint formulations are varied somewhat from user to user and batch
         to batch to adjust to changes in the market, color, processing equip-
         ment, etc.

     2)  Paints are invoiced either by weight or by volume.

     3)  The user buys most paints in liquid form,  but actually uses only the
         paint solids on the finished product.  The total volume of the organ-
         ic volatiles in the liquid constitutes a waste load.

     4)  Loss of some portion of the paint solids is inherent in all painting
         processes.  Accidental losses will also occur and contribute addi-
         tional organic volatiles plus nonvolatile  paint solids to the waste
         loads.

     5)  Industrial painting operations vary in size, and production output
         fluctuates with the market.

Method

     In consideration of the above premises, the waste load for an industrial
painting operation can be predicted and/or determined when the following data
are known:

     1)  The weight and volume of paint solids and  organic volatiles that
         enter the plant.

     2)  The surface area of the merchandise painted and the film thickness
         of the applied paint solids.  In other words, the volume of paint
         solids that are actually utilized and that leave the plant on the
         merchandise.

     The difference between the volume of paint solids that enter the plant
and the volume that leave the plant on the merchandise represents the solid
and most of the semisolid waste generated by the painting operation.

     The total volume of organic volatile material   (paint components, solvents,
thinners, additives, cleaning fluids, etc.) that enter the plant represents the
organic volatile waste load generated by the painting operation.


PHASES

     The scientific and trade literature was surveyed for the weights and
volumes of the nonvolatile components (resins, pigments, etc.) of typical,
widely used paints, and also for the weights and volumes of their organic
volatile components (solvents, etc., exclusive of water).

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     The surveyed paint compositions were arranged into nine paint classes
according to the application techniques (spray, dip, etc.) for which the
paints had been formulated.

     The paint application techniques were surveyed and studied for their ex-
pected transfer efficiency;  i.e. their inherent unavoidable paint losses.

     Mathematical equations were then developed by which the expected waste
load for any planned painting operation can be predicted from the composition
of the paint and the equipment and painting process to be used.

     All these data were compiled into a preliminary 25 page report that was
sent to about 30 experts in the field who were requested to provide their
criticisms, suggestions, comments, etc.  Where appropriate, the replies from
these experts have been incorporated into this final report.

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                                  SECTION 2

                                 CONCLUSIONS
     The waste loads generated in painting processes for metal products are
governed by four factors:  1)  paint composition, 2)  painting equipment,
3)  curing method, and 4)  miscellaneous unavoidable losses.

     Solvents (water or organic volatiles) are an essential part of paint  com-
positions .  The more recently developed paint compositions —sometimes called
"low polluting"— are remarkably efficient in reducing the need for evapora-
tion of water or organic volatile solvents, and they also reduce the quantity
of semisolid waste generated.

     The efficiency of the equipment for transferring the paint from the pot
onto the surface of the merchandise varies from about 50% to almost 99%.  The
waste loads are, therefore, very much influenced by the type of painting equip-
ment used.

     Organic volatiles or water are emitted into the air by an evaporative
process during the curing cycle.  Comparatively small quantities of coreact-
ants are also liberated during the cure of some commercial paints.

     Most unavoidable losses are inherent with the method of applying the  paint
to the product.  Additional unavoidable losses occur during normal handling of
the equipment, cleaning of the equipment, and repair of defective paint coats
(sanding, stripping, etc.).

     A series of mathematical equations has been developed that allows the pre-
diction of the waste loads for almost any kind and size of industrial painting
operation or planned alternate, and for the determination of the actual waste
loads calculated from production data.

     In theory, the waste loads in painting operations could be significantly
reduced by the judicious choice of paint, equipment, and curing method, and
by the skill and techniques of operating personnel.

     In practice, many efforts toward waste reduction in paint operations is
currently underway, both for reasons of pollution law enforcement and for the
economic savings possible.  However, in order to ensure the quality of new
coatings, it may take years of field testing before currently used paints and
processes can be completely replaced by other more efficient ones.

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                             SECTION 3

                          RECOMMENDATIONS
1)  An effort should be made to familiarize government and industry per-
    sonnel with the use of the mathematical prediction and actual deter-
    mination of painting waste loads.  Half or 1 day conferences should,
    therefore, be arranged for the presentation of the plaint waste load
    computations.

2)  Though an effort has been made to include typical paints and painting
    processes, a continuing effort should be made towards the detection
    of wasteful practices and encouragement of cheaper, more protective,
    and less wasteful practices.

3)  Current literature does not refer to the nature of the malodorous
    fumes that are sometimes observed during painting operations.  Lab-
    oratory devices should be developed for the study and generation of
    data towards the elimination of the fume-causing substances and/or
    practices.

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                                  SECTION 4

              SURVEY PROCESSES AND DEVELOPMENT OF CALCULATIONS
GENERAL

     Paint is a general term that is given to compositions that can be applied
in comparatively thin, even layers onto solid surfaces where they convert into
solid, adhesive, wear-resistant film coatings.  Conventional filmforming ma-
terials are organic polymeric compounds;  that is, materials containing carbon,
hydrogen, oxygen, and sometimes minor quantities of other elements.  Typical
nonvolatile filmformer solids are known as acrylics, epoxies, urethanes, al-
kyds, etc.  These generic names refer to the atomic arrangement of the elements
which constitute the filmformer solid.

     Filmformers, often called "resins", must be soluble in a liquid vehicle
or meltable at reasonable temperatures so that they can be applied in thin,
even layers onto the desired surface.  Furthermore, filmformers must convert
into solid film coatings through a "curing" process (drying, baking, etc.).

     Most conventional filmformer solids, when they are used as the only non-
volatile component of a paint composition, will result in transparent film
coatings.  However, to meet the needs and desires of users, most paints are
designed to hide the substrate of the material coated and to impart color to
the finished merchandise.  This is accomplished by the incorporation of pig-
ments into the paint compositions.  Pigments are usually nonvolatile solids
intimately mixed or ground into the filmforming solids.  Most pigments also
increase the durability of the film coating.

     Various other additives of volatile and/or nonvolatile nature may be in-
corporated in small quantities to paint compositions.  These additives may
facilitate the deposition and adhesion of the filmforming solids on the sur-
face to be coated, enhance the curing process, effect a gloss or matte finish
to the coating, etc.

     Water is used in many paint compositions as most or part of the liquid
component.  Water is volatile and though the moisture emitted during painting
operations may cause serious operational problems, water vapor is generally
considered nonpollutional in nature.  For the purpose of this study, attention
has been directed specifically to the two classes of paint components that
generate pollutional waste loads:

     1)  Organic Volatiles (0V)  (solvents, thinners, plasticizers, and other
         liquid additives).

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     2)  Nonvolatiles  (NV)  (resins, pigments, and other solid additives).


OBJECTIVES

     The objectives  of  this  study were  to develop methods for:

     1)  The prediction of pollutional  waste loads that will be generated by
         any size  or type of planned  industrial painting operation.

     2)  The determination of  actual  pollutional waste loads generated by any
         size  or type  of existing industrial painting operation.

     3)  A basis to  be used  for  the selection of alternate paints or painting
         processes to  reduce the predicted  and/or actual pollutional waste
         loads in  industrial painting operations.


SOURCES OF INFORMATION

     The commercial  paint manufacturing industry is highly competitive, there-
fore,  the actual formulation of  commercial  paints is considered proprietary
and, in most cases,  will be  released  only as confidential information that
may not be used in a study of  this nature.

     However,  the  resin manufacturers who supply basic materials to the paint
manufacturers  demonstrate the  quality of their products by means of prototype
formulations which are provided  freely  to the public.  As a result, portions
of this study  have been based  on the  use of such detailed prototype formula-
tions .

     Where actual  commercial paints have been used in calculation  examples and
tabulations, the organic volatile and nonvolatile components  of the formula-
tion have been lumped  into  single figures;  that is, without  consideration of
the proportion of  solvent,  thinner, additives, resins, pigments, etc.

     To insure the validity  of the data developed using this approach and the
relationship of prototype formulations  to actual formulations of commercial
paints on the  market,  the basic  findings of the study were circulated to about
30 experts in  the  paint industry who  were requested to provide their correc-
tions, comments, and suggestions.  The  cooperation of these experts is greatly
appreciated, and their  replies have been incorporated in this final report as
appropriate.


PAINT COMPOSITIONS

     The ideal paint would be  simply  a  nonvolatile filmforming substance that
could be applied directly and  evenly  to any solid surface.  Ideally, by use
of this principle, no material would  be lost in the transfer process, and no
waste load would be  generated  (Figure 1).

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            NONVOLATILE
             FILMFORMER
               (SOLID)
TRANSFER
            IDEAL  PAINT
NONVOLATILE
    FILM
  COATING
                MERCHANDISE
             Figure 1.   Film coating using an ideal nonvolatile
                        filmformer  solid.

     There are certain newer classes of paints which aim at the use of this
principle presently under  development and a few are currently in use in lim-
ited applications.   However,  due  to the time necessary to perfect and produce
the required transfer  equipment and the extensive field testing necessary to
insure the quality  of  the  new coatings, it will be a number of years before
these new classes of paints  widely replace the more conventional paints cur-
rently on the market.

     These newer classes of  paints present some minor pollutional problems in
that a small organic volatile waste load is generated by the liberation of a
small quantity of coreactants during the transfer and curing processes.

     The vast majority of  conventional paints currently on the market consist
of compositions of  nonvolatile filmformer solids mixed with a liquid vehicle
(organic volatile solvents,  water, or in some cases both) and are handled and
applied in this liquid form.   The use of paint compositions in liquid form
provides two major  advantages:

     1)  They allow for the  use of a wide variety of transfer equipment and
         curing processes  (spray, dip, roll, air drying, baking, etc.).

     2)  The viscosity of  the paint composition as bought can be adjusted by
         increasing the ratio of  liquids to solids.  This allows for both an
         adaptation to the equipment and process used for the transfer opera-
         tion and for  control of  the film coating layer applied to the mer-
         chandise.

     The major disadvantage  in using conventional liquid paint compositions
is that the entire  quantity  of liquids is emitted into the air as waste loads
during the transfer and curing processes.  Only the nonvolatile solids depos-
ited on the surface of the merchandise actually leave the plant as part of the
finished product.

     The greatest pollutional problems are encountered in the use of liquid
paint compositions  mixed with organic volatile solvents.  The entire quantity
of solvents in these paint compositions becomes organic volatile waste loads
during the transfer and curing processes  (Figure 2).

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         ORGANIC  VOLATILE
              SOLVENT
              (LIQUID)
            NONVOLATILE
             FILMFORMER
               (SOLID)
                                     ORGANIC  VOLATILE  WASTE  LOAD
TRANSFER
        SOLVENT  BORNE  PAINT
NONVOLATILE
    FILM
  COATING
                MERCHANDISE
           Figure 2.   Film coating using organic volatile solvent
                      based liquid paint compositions.

     The generation of the organic volatile waste load from these paint com-
positions is through an evaporative process that occurs during the entire
transfer and curing cycles of the painting operation.  Emission of the waste
load begins as soon as the paint composition is exposed to the air and con-
tinues until the film coating is fully cured.

     Paint compositions mixed with water as the liquid component function in
much the same manner  as the organic volatile solvent based compositions.  The
entire quantity of water in the composition is emitted as a water vapor waste
load during the transfer and curing processes  (Figure 3).
               WATER
              (LIQUID)
            NONVOLATILE
             FILMFORMER
              (SOLID)
                                     WATER VAPOR  WASTE  LOAD
TRANSFER
        WATER BORNE PAINT
NONVOLATILE
    FILM
  COATING
               MERCHANDISE
    Figure 3.  Film coating using water based  liquid paint compositions.

     Water vapor waste loads are generally considered nonpollutional in nature,
therefore, little further consideration or discussion has been devoted to this
factor in the remainder of this study.  However, it should be noted that due
to the corrosive nature of water vapor, this waste load may cause serious
operational problems.

     Paint compositions mixed with a combination of organic volatile solvents
and water as liquid components generate both the organic volatile and water
vapor waste loads described above (Figure 4).
                                    10

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                 WATER
               (LIQUID)
          ORGANIC  VOLATILE
                SOLVENT
               (LIQUID)
             NONVOLATILE
              FILMFORMER
                (SOLID)
                                       WATER  VAPOR  WASTE  LOAD
                                       ORGANIC VOLATILE  WASTE  LOAD
TRANSFER
       WATER &  SOLVENT BORNE
NONVOLATILE
    FILM
  COATING
                MERCHANDISE
           Figure 4.   Film coating using organic volatile solvent
                      and  water based liquid paint compositions.
SELECTION OF PAINTS

     Until quite recently,  industrial paint users selected paint compositions
and painting processes on the primary basis of the quality of  the film coating
and the basic cost of  the paint materials.  Today, environmental factors and
the energy consumed by the transfer and curing processes must  also be given
weighted consideration in the selection process.  As a result,  the paint man-
ufacturing industry is currently engaged in extensive efforts  to develop more
desirable paint compounds and more efficient painting processes.

     The quality and durability of the film coating remains the primary con-
sideration of the ultimate paint consumer.  It generally takes  about five years
of product experimentation and extensive laboratory and field  testing before an
industrial paint user  can have reasonable assurance that a new paint will meet
quality, cost,  environmental, and energy requirements. Therefore, an indus-
trial switch to newer  classes of paints and painting processes  is expected to
be a slow and cautious process.

     The reason for the long periods of laboratory, field,  and  sometimes out-
door exposure testing  is  to subject the film coatings to the same conditions
they will meet when used  for the actual purpose for which  they  are designed.2

     Obviously, if a paint manufacturer is expected to guarantee a film coat-
ing for a service life of two years, laboratory and field  testing will require
a minimum of two years.   In most cases, a film coating is  applied to hundreds
or even thousands of pieces of material to be used in the  tests.  If the film
  Gardner,  H.  A.,  and  Sward, G. G.  ASTM Paint Testing Manual,  13th Edition,
  American Society for Testing and Materials, Philadelphia, Pa.  1972, pg 251-
  494.
                                    11

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coating fails on an unacceptable number of pieces during the tests and the
paint composition or painting process is changed for improvement, a new series
of tests must be initiated.

     In the case of paints made for use on merchandise designed for outdoor
use extensive exposure tests to a wide range of climatic conditions is fre-
quently required.

     Even after a new paint has been developed in the laboratory or pilot
plant and has met all requirements of quality, cost, environment, and energy,
still further delays may be expected before it is widely adopted.  It may be
several years before the raw materials are available or can be produced in
sufficiently large quantities.  It may also require time for the development,
planning, capital investment, manufacture, and installation of the required
equipment for the new painting process.


BUYING AND USING PAINTS

     The industrial user normally buys paint as a composition consisting of
nonvolatile filmforming solids and sacrificial liquids.  During the painting
operation the nonvolatile solids are applied to the surface of the mechandise
and the liquids are emitted as waste loads.  The film coating on the merchan-
dise must meet certain specifications, such as, durability, color, hardness,
gloss, corrosion resistance, etc., and in many cases film thickness.

     The^re are a number of factors which must be determined before an indus-
trial paint user can figure the cost of a painting operation and make a de-
cision as to what quantity of what paint to buy.

     First, the volume of nonvolatile solids required to coat the surface
area of the merchandise to the specified thickness must be determined.  This
can be found by multiplying the total surface area by the thickness of the
film coating.

     Next, the volume of nonvolatile solids contained in a purchased unit of
paint composition must be known.  Commercial paint compositions are usually
sold by weight, and the quantity of nonvolatile solids in the composition is
also often given by weight.  If this is the case, the weight of the nonvola-
tile solids must be converted to volume.

     From the above factors the quantity and cost of the paint composition
for a specific operation can be calculated.  Suppose several paint manufac-
turers offer paint compositions which meet all the requirements of the film
coating but vary in formulation and cost.  Obviously the most economical com-
position to buy is that which contains the most nonvolatile solids at the low-
est cost.  However, this is only one of the factors in the over-all cost of
the painting operation.

     Since all liquids in paint compositions are emitted as waste loads during
painting operations, the costs for controlling these waste loads is a factor
in the over-all cost of the painting operation.  The most serious pollutional


                                     12

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waste loads are those generated by organic volatile solvents.   From an envir-
onmental standpoint it might appear that the least pollutional paint composi-
tion to buy would be that which contains the least volume of organic volatile
solvent.  However, most paint compositions are sold with nonvolatile concen-
trations too high to be used in most painting processes and must be "thinned"
by the addition of more liquids before they are used.   Waste loads must be
calculated by the volume of liquids in the composition "as used" rather than
"as bought".  The cost of the additional liquids must  also be figured into the
over-all cost of the painting operation.

     The use of paint compositions that use water as part or all of the liquid
content may reduce or eliminate pollutional waste loads.  However, the cost of
overcoming the operational problems, such as corrosion, caused by the water
vapor waste load, and the cost of energy to evaporate  the water may exceed the
costs of controlling environmentally pollutional waste loads.

     Energy consumption required for transfer and curing processes is becoming
an ever greater factor in the over-all cost of a painting operation.  If the
present energy shortage trend continues, it may become more than a matter of
cost and become a matter of availability.

     Another major factor in the calculations of the quantity and cost of ma-
terials and the generation of waste loads is the transfer efficiency of the
equipment and process used in the painting operation.   Unavoidable losses of
part of the total volume of nonvolatile solids occurs  in all painting process-
es.  For example, if the transfer efficiency of a painting process is only 50%
it means that only half of the nonvolatile solids in the paint composition "as
used" is actually deposited on the surface of the merchandise; the other half
becomes nonvolatile waste.

     The final factors which must be considered are other minor unavoidable
losses such as cleaning and repair of equipment, sanding or stripping to re-
pair or remove defective coatings, and accidental spillage or wastage,


UNITS OF MEASUREMENT

     Metric system units of measurement have been used as the primary standard
throughout this study.  In most cases examples have also been shown using U.S.
standard units of measurement for better understanding.

     As stated previously, paint compositions may be bought in either metric
or U.S. units of weight (kilograms or pounds) or volume (liters or gallons).
The quantity of nonvolatile solids and liquids in the composition may also be
provided in units of weight or volume, or may be expressed in percentages of
the total units.

     In order to use the equations developed in this study the industrial
paint user must convert the known units of weight or volume to the other fac-
tor for specific calculations.  The quantity of nonvolatile solids required
to form the film coating on the surface of the merchandise must be calculated
in units of volume (area coated x thickness of film = volume).  The volume


                                     13

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of volatile waste loads,  particularly those generated by organic volatile sol-
vents, does not represent meaningful data due to large variances in density
possible from the range and variety of liquids used in paint compositions.
Normally, all waste loads are  calculated in weight units,  though the volume
of semisolid waste loads may be desired in some cases.  The method for devel-
oping calculations is shown schematically in Figure 5.
       VOLATILE LIQUID
           THINNERS
             PAINT
         COMPOSITION
         (as  bought)
                                   VOLATILE
                                 WASTE LOADS
  (WEIGHT)


      TRANSFER
      (WEIGHT  & VOLUME)
   SOLIDS
WASTE  LOADS
NONVOLATILE
    FILM
  COATING
  (VOLUME)
                              (WEIGHT  OR VOLUME)

                      Figure 5.   Calculation Schematic
VOLUME CALCULATIONS
     A constant (K) factor can be developed to represent the maximum area that
can be film coated to a specified thickness by a standard metric or U.S. unit
of volume of nonvolatile (NV) paint solids.  This K factor  is developed on the
assumption that the entire volume of NV solids are transferred to the surface
of the merchandise, that is,  100% transfer efficiency.

     Since there are some unavoidable NV losses in all  painting processes, the
maximum area coverage will never be achieved in actual  operation.  However, by
using maximum data, computations may be developed for the following three pur-
poses:

     1) Cost comparison between available paint compositions by direct compar-
        ison of costs per unit volume of NV.

     2) The maximum area that may be coated to a specified  thickness in any
        painting operation by a given volume of NV.  (Shown in Equation 1.)

     3) The minimum volume of NV required to coat a specified area to a spec-
        ified thickness.  (Shown in Equation 2.)
                                    14

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     The volume calculations which follow have been developed using the metric
and U. S. Standard measurement units commonly used by both the paint manufac-
turing industry and industrial paint users (Table 1).
               TABLE 1.  COMMONLY USED PAINT MEASUREMENT UNITS
MEASUREMENT
Length
Area
Thickness
Volume
METRIC
1m = 100 cm
1m2 = 10,000 cm2
or 1 x 104 cm2
1 ym = .0001 cm
or 1 x lO"4 cm
11 = 1,000 cm3
or 1 x 103 cm3
U. S. STANDARD
1 ft = 12 in
1 ft2 = 144 in2
1 mil = .001 in
or 1 x 10~3 in
1 gal = 231 in3
     Using these units of measurement, the theoretical maximum area that can
be covered by 1 liter of NV 1 ym thick, and by 1 gallon of NV 1 mil thick,
can be established,  (volume / thickness = area)
                METRIC
         11  _  1 x 103
cm"
        1 ym     1 x 10"1* cm

              =  1 x 107 cm2

            convert to m2

              _  1 x 107 cm2
                 1 x
                         cm
              =  1,000 m
                        2
U. S. STANDARD

1 gal  =    231 in3
1 mil     1 x 10~3 in

       =  231 in2 x 103

     convert to ft2

       =  231 in2 x 103
             144 inz

       =  1,604 ft2
Equation 1
     The following equation may be used to calculate the maximum surface area
that may be coated to a specified thickness by a given volume of NV:
                                     15

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                            x v NV

     where  (metric)

          Amax.   =   maximum possible area in m2

          K      =   1,000 m2 x 1 ym/liter

          t      =   film thickness in ym

          v      =   volume in 1

     or, where  (U. S. Standard)

          Amax.   =   maximum possible area in ft2

          K      =   1,604 ft2 x 1 mil/gallon

          t      =   film thickness in mil

          v      =   volume in gal

Example 1

     To calculate the maximum area that can be coated with a film 38.1 ym
(1.5 mil) thick with a quantity of paint containing 64 liters (16.9 gal) of
nonvolatile (NV) solids:

                      1,000   ,.       (1,604)
          Amax.   =   387Tx64        (1.5)  x (16'9)

                      1,680 m2         (18,072 ft2)

Equation 2

     The following equation may be used to calculate the minimum volume of
NV required to coat a given surface area to a specified thickness:

          vNVmin. =   (Ap/K) x t

     where

          vNVm^n  =   minimum volume of nonvolatiles in 1 (gal)

          Ap      =   area to be painted in m2 (ft2)

          K       =   1,000 m2 x 1 ym/1 (1,604 ft2 x 1 mil/gal)

          t       =   film thickness in ym (mil)
                                     16

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Example 2

     To calculate the minimum volume of  nonvolatiles  (NV) necessary to cover
a surface area of 9,295 m2 (100,000 ft2) with a film  19 ym  (.75 mil) thick:
          vNV,
             min.
x 19
(100.000)
 (1,604)  :

(46.8  gal)
(.75)
Summary
     It should be noted that "Maximum Area" and "Minimum Volume" have been
emphasized in computing the consumption of nonvolatile solids (Figure 6)-
                 PAINT
                VOLUME
                   NV
                                    MAXIMUM
                                    COVERAGE
                                    MINIMUM
                                  CONSUMPTION
                            FILM
                           VOLUME
                             NV
                         1  LITER   =  1,000 m2  X 1  ym
                        1 GALLON   =  1,604 ft2 X  1  mil

           Figure 6.   Maximum coverage equals minimum consumption.

     Since there are  some unavoidable losses of NV in all painting processes,
maximum coverage with a minimum volume will never be achieved.  The discussion
of these losses is one of the objectives of this study and is provided in the
following sections of this report.


ORGANIC VOLATILES IN  PAINTS

     All paint compositions  contain  some amount of organic volatile (0V) ma-
terial.  Even, the so-called  "water borne" paint compositions contain a moder-
ate amount of 0V. ' These 0V  materials are necessary to provide compatibility
of components during  the manufacture of the compositions and to facilitate the
application of the nonvolatile (NV)  solids to the desired surface.  Compara-
tively, the largest amount of 0V material is usually found in paint composi-
tions designed for use in spray painting operations, while the least amount
is found in dry paint powder compositions.

As Bought

     Most paint manufacturers list the various components in their paint com-
positions as volume percentages (vol%).  For example, a certain water borne
paint (Code lAw 1) surveyed  during this study is listed by the manufacturer
as containing:
                                     17

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                26.6 vol% NV
                15.1 vol% 0V
                58.3 vol% water

      Since  the  volume  of the NV components is the basis used for buying  and
using paint compositions,  the vol% of NV can be established as a measurement
unit  (liter or  gallon)  of  volume.  The vol% relationship of all components
can then be shown  as units of volume:  (Figure 7)

                1.000 vol (liter or gallon) NV
                0.568 vol (liter or gallon) 0V
                2.192 vol (liter or gallon) water
                3.760 vol  (liter or gallon) paint composition
2
0
1
.192 VOL
WATER
.568 VOL
0V
.000 VOL
NV
                                    EQUALS
 3.750 VOL
    PAINT
COMPOSITION
(as  bought)
                                                     (Code:  lAw 1)
            Figure 7 -  Volume relationship of paint components.

     As shown above, in order to provide one unit volume (liter  or  gallon) of
NV for a painting operation it is necessary to buy and use 3.76  unit volumes
(liters or gallons) of this particular paint composition (Code lAw  1).  The
entire volumes of 0V and water are emitted during the painting operation as
0V and water waste loads as previously shown in Figure 4.

As Used

     Most commercial paint compositions are manufactured and sold for use in
a variety of painting processes.  Many of these compositions contain a  solids
concentration too high to be used by most painting equipment and processes.
Therefore, the user must add an additional volume of liquid (0V  solvent and/or
water) to reduce the viscosity as necessary for his specific painting opera-
tion.

     When "thinners" are added to a paint composition "as  bought" the volume of
NV remains the same, but  the volume of 0V and/or water and the  total volume
is increased proportionally.  In order to calculate waste loads  it  is neces-
sary to correct the vol% and volume relationship to reflect the  actual  "as
                                     18

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used" composition.   For example, a certain solvent borne paint (lAs  6)  survey-
ed is listed as containing:
                As Bought

               36.4 vol% NV
               63.6 vol% 0V
   As Used

 28.6 vol% NV
 71.4 vol% 0V
     The vol% of all components, both as bought and as used,  can then be shown
as units of measure:  (Figure 8)
                   Buy

               1.000 vol
               1.747 vol
               2.747 vol
    Use

 1.000 vol  (1 or gal)  NV
 2.496 vol  (1 or gal)  0V
 3.496 vol  (1 or gal)  paint composition
            0.749  VOL
           0V  THINNER
             (added)
            1.747  VOL
                0V
           (as bought)
            1.000  VOL
                NV
EQUALS
  3.496 VOL
     PAINT
 COMPOSITION
  (as  used)

(Code:  lAs  6)
        Figure 8.   Volume relationship of paint components  "as used".

     The total paint  composition under the "buy" column can be used  to calculate
the quantity of paint that must be bought.  The difference  in the volume of 0V
between the buy and use  columns can be used to calculate the quantity of thin-
ner that must also  be bought.  The total volume of 0V under the  "use" column be-
comes an 0V waste load during painting and curing processes.
ORGANIC VOLATILE CALCULATIONS
     Since the volume of NV is the controlling factor in the quantity of paint
composition required  in a painting operation, the ratio of 0V to  NV  in  the com-
position is required  to determine the 0V waste load.  This ratio  must be estab-
lished for the 0V and NV components in the mixture "as used".  For solvent
borne paint compositions, such as lAs 6 used in the example above, the  total
"as used" volume contains only 0V and NV components.  This example shows a
ratio of 2.496 vol (liter or gallon) of 0V for each vol (liter or gallon) of

-------
NV in the "as used" composition.  For water borne paint compositions,  such as
lAw 1 used in the "as bought" example and shown in Figure 7,  it may be desired
to establish a vol% ratio between just the 0V and NV components and disregard
the water in the composition (Figure 9).
WATER
0

1

.568
0V
.000
NV
VOL

VOL

                                    0.568  VOL 0V  x 100

                                    1.568  VOL 0V  + NV
                       36.3  VOL%  0V
                Figure  9.  Vol% ratio  of 0V to NV components.

     For  0V waste  load  calculations, the vol% ratio of 0V to NV must first be
reduced to the volume  (liter  or gallon) of 0V associated with 1 volume (liter
or gallon) of NV  (Equation 3) and  then the volume (liter or gallon)  converted
to weight (kilogram or  pound) (Equation 4).

EquatioQ  3

     The  following equation may be used to calculate the volume (liter or gal-
lon) of 0V associated with 1  volume  (liter or gallon) of NV:
          vOV
                        vol%  0V
                     (100  - vol%  0V)
 or
vol% 0V
vol% NV
     where
           vOV   =   volume of  0V in liters or gallons

 Example 3

      The volume of 0V associated with 1 volume of NV in paint composition
 lAw 1 can be found by using the vol% ratio established in Figure 9:
           vOV
                        36.3
36.3
63.7
   0.57 (liter or gallon)
                    (100 - 36.3)

      or,  by using the original vol% ratio  of  0V  to NV given on page 18:

                    15.1 vol% 0V
           vOV
                    26.6 vol% NV
 0.57 (liter or gallon)
                                      20

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Equation 4

     The following equation may be used to calculate the weight (kilograms or
pounds) of a given volume (liter or gallon) of 0V:

          wOV   =   vOV x dOV

     where

          wOV   =   weight in kilograms or pounds

          vOV   =   volume in liters or gallons

          dOV   =   density weight for 1 volume unit in kg/1 or Ib/gal

Example 4

     The weight of 0V associated with 1 volume of NV in paint composition
lAw 1 can be found if the density weight of the 0V is known:

          wOV   =   0.57 x 0.91         (0.57 x 7.5)

                    0.52 kg             (4.3 Ib)

     where

          dOV   =   0.91 kg/1           (7.5 Ib/gal)

Variations of Equation 4

     Paint manufacturers may show the ratio of 0V to NV in their compositions
in several different ways.  Frequently the ratio is expressed as "weight (kg
or Ib) of 0V per volume (liter or gal) of paint composition less water"; i.e.
wOV/(vOV + vNV).  In other cases the ratio is expressed as "weight (kg or Ib)
of 0V per volume (liter or gal) of NV"; i.e. wOV/vNV.  These ratios can each be
converted to the other by use of Equations 4a and 4b respectively.

Equation 4a—
     The following equation can be used to find the weight of 0V associated
with 1 volume unit of NV when the wOV/(vOV + vNV) and dOV are known:


          w'OV/v'NV   =    .   W°Iov
                           I     dOV

     where

          w'OV/v'NV   =   weight (kg or Ib) of 0V per 1 volume (1 or gal) of NV
                                      21

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Example 4a—
          w'OV/v'NV   =   	°'348   .                  (2.90)
                           f 1  -  0.348]               L  _ (2.90)
                           I     0.930'               \     (7.75)1

                      =   0.348                     (2.900)
                          0.626                     (0.626)

                          0.556  kg OV/1 NV         (4.63 Ib OV/gal NV)

     where

          wOV         =   0.348  kg/1 (0V + NV)      (2.9 Ib/gal (0V + NV))

          dOV         =   0.93 kg/1                 (7.75 Ib/gal)

Equation 4b—
     The following equation can  be used to find the weight  of  0V associated
with 1 volume unit of (0V + NV)  when the wOV/vNV and dOV are known:


          w'OV/(v'OV + v'NV)  «      W°V
                                    [1+wOV]
                                    1     dOV J
     where
      \
          w'OV/(v'OV + v'NV)    =  weight (kg or Ib)  of 0V per 1  volume of
                                   (0V + NV)
Example 4b—
          w'OV/(v'OV + v'NV)    =      °-556                	£4-^
                                         0.930]              I     (7.75)

                                =  0.556                    (4.63)
                                   1.598                    (1.598)

                                =  0.348 kg/1 (0V + NV)      (2.9 Ib/gal
                                                                 (0V + NV))

     where

          wOV                   =  0.556 kg/1 NV           (4.63 Ib/gal NV)

          dOV                   =  0.93 kg/1               (7.75 Ib/gal)
                                      "22

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                                  SECTION 5

                       PAINTING METHODS AND EQUIPMENT
GENERAL
     It was shown in the previous Section that the first  factor  in paint  cal-
culations is the ratio of organic volatiles to nonvolatile  solids in  the  paint
composition.  The next factor to be considered is  the  "transfer  efficiency" of
the painting method and equipment used to apply the paint composition to  the
surface of the merchandise.

     The most commonly used  methods and equipment  used for  painting operations
by the metal fabricating and finishing industry were surveyed  and are discuss-
ed in this Section.
SPRAY PAINTING

     The principle of spray painting is to break up  the liquid  paint  composi-
tion into tiny droplets and propel them through  the air onto the  surface  of
the merchandise to be coated.   There are several methods for atomizing the
paint composition and there is a variety of spray painting equipment  current-
ly in use.

Air Atomization

     In this method a j et of compressed air impinges on a stream of liquid
paint which emerges from an orifice in the tip of the spray gun.  The air  jet
atomizes the paint and propels (transfers) the droplets onto the surface of
the merchandise (Figure 10).
            COMPRESSED
               AIR
                                                       OVERSPRAY
                       Figure 10.
Air atomized spray.

   23

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     Conventional spray painting using the air atomized method has  the lowest
 expected  transfer efficiency" (about 50%) of all the methods  surveyed.  This
low  transfer efficiency is due in part to the unavoidable overspray necessary
to achieve full coverage of the film coating on the merchandise and in part to
a factor called "air back bounce" which prevents many of the paint  droplets
from reaching  the surface of the merchandise.

Pressure Atomization

     In this method the liquid paint is forced through a small diverging ori-
fice at a  relatively high pressure of about 600 psi.  The paint emerges from
the  orifice as a fine spray with sufficiently high kinetic energy to propel
(transfer) it  through the intervening air onto the surface of  the merchandise
(Figure 11).
                        <£n
              VENT
                                                  OVERSPRAY
                                  PRESSURE
                                  PUMP
                    Figure 11.  Pressure atomized spray.

     The pressure atomized method has a higher "expected  transfer efficiency"
 (about 65%) than the air atomized method.  Though relatively  the same amount
 of unavoidable overspray is necessary to achieve full coverage, the "air back
 bounce" factor is considerably reduced due to the smaller mass volume of air
movement.

 Electrostatic Field Assisted Spray Painting

     In this method the atomized paint is given a polarized high voltage elec-
 trical charge (usually about 100,000 volts) at or near the point where it
 emerges from the paint gun and the merchandise is electrically grounded to
 the opposite polarity of the power source.  Thus, the charged paint particles
 are electrically attracted to the surface of the merchandise  (Figure 12).

     By using electrostatic field assistance in either the air atomized or
pressure atomized method, the "expected transfer efficiency"  can be increased
 to approximately 85%.  Both the necessary unavoidable overspray and "air back
bounce" factors are appreciably overcome by the electrical attraction of the
paint particles to the surface of the merchandise.
                                     24

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                                                        •x
         HIGH
       VOLTAGE
          DC
          Figure 12.   Electrostatic  field assisted spray painting.

Centrifugal Atomization

     In the most commonly used  centrifugal atomization method, liquid paint is
oozed onto the center inside  surface of a rapidly rotating bell.  The centri-
fugal force of the rotating bell moves the paint to the open end where it pass-
es through an electrostatic field  and emerges as a charged, atomized spray.
As the spray emerges, the electrostatic field directs (transfers) it to the
surface of the merchandise (Figure 13).
      HIGH
     VOLTAGE
        DC
ROTATING
BELL
   COMPRESSED
       AIR 	
                   Figure 13.   Centrifugal atomized spray.

     The centrifugal atomization has  the highest "expected transfer efficiency"
of all spray painting methods  surveyed  (about  93%).

     A common variation of the centrifugal atomization method uses a horizon-
tally rotating disk instead of the bell described  above.  This variation has
about the same transfer efficiency and  provides a  wider coverage area.  In
this method the merchandise is usually  carried by  a conveyor in a horse shoe
shaped loop around the disk.
                                      25

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Associated Equipment

     Due to the airborne solid and semisolid wastes generated  by  spray paint-
ing operations they must be performed in a confined area.   A paint  spray booth
may simply be an area enclosed on three sides with an exhaust  fan and filter
in an overhead hood, or it may be a much more elaborate arrangement.

Strippable Coatings—
     There are several products on the market that can be  applied to the inner
surfaces of spray booths.  When a layer of waste has accumulated  on these coat-
ings, they can be peeled off along with the waste and a new coating applied.

Water Bath Spray Booth—
     In this type of booth, the sides consist of a series  of baffles over which
a curtain of water cascades (Figure 14).
                        WATER
                                           EXHAUST  AIR
                                                                 _ WASTE
                                                                    WATER
                  Figure  14.  Water bath spray paint booth.

     The airborne solids  are absorbed by the water curtain so that the exhaust
air contains only volatile wastes.  The solids form a sludge in an associated
tank or reservoir and  in  some limited circumstances may be reclaimed.   Waste
water from such methods   may contain both organic liquids and solid contamin-
ants and require additional treatment.

Hot Melt Spray Paints

     There are a number of spray paint compositions manufactured that are de-
signed to be preheated before use.  These paints have such high concentrations
of solids that the viscosity at ambient temperatures is too high to be handled
by spray devices, but  when preheated thin sufficiently for normal application.

     These paint compositions are satisfactory for use in any of the spray
methods described above and have approximately the same "expected transfer
efficiency" as other paints used by the same method.

                                      26

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DIP COATING

     In the dip coating method the merchandise is actually submerged  in a  con-
tainer of liquid paint and then lifted back out.   The excess  paint drips off
the merchandise either directly back into the paint container or  into a drip
recovery tray.  Dip coating of rigid,  profiled merchandise requires that each
piece be submerged individually (Figure 15).
                                                                PAN
             Figure 15.  Dip coating rigid, profiled merchandise.

     The drip off process is sometimes aided by the use of a high  voltage elec-
trostatic field which is effective in eliminating drops of paint that might
otherwise form on the bottom of the merchandise.

     Flexible, essentially unprofiled merchandise such as coil stock or wire
is dip coated by a continuous process (Figure 16).
                                                               BLADE
                                                               OR DIE
           Figure  16.  Dip  coating flexible, unprofiled merchandise.

      The drip off process  from continuous material  is usually aided by passing
 the merchandise through a  blade or  die  that serves  to wipe off excess paint.

      The "expected transfer  efficiency" for both  the dip  coating methods cited
 above is in the range of 75  to 90%.
                                      27

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FLOW COATING

     In the flow coating method liquid paint is poured over the top of the
merchandise and allowed to drip off the bottom.  The merchandise is position-
ed over a container of paint, part of the paint is pumped to a dispensing
head over the merchandise, the paint flows over the merchandise forming a
coating, and the excess drips back into the container (Figure 17).
                              CONVEYOR
                                                   o    o
                          Figure 17.  Flow coating.

     Drip off is sometimes aided by use of a high voltage electrostatic field.
The "expected transfer efficiency" for the flow coating method is  about the
same asxfor the dip coating method (75 to 90%).
CURTAIN COATING
     The curtain coating method is similar in principle to the flow coating
method.  Curtain coating is usually used to paint flat, relatively  thin pieces
of merchandise.  The merchandise is passed beneath a paint trough that has a
slit in the bottom that is perpendicular to the direction of movement of the
merchandise (Figure 18).
                               TROUGH  WITH SLIT IN  BOTTOM

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     Liquid paint in the paint trough flows  through  the  slit by gravity onto
the merchandise as it passes below.   Excess  paint  flow and drip off is caught
in a container positioned below the  merchandise.   The system usually contains
a circulating pump which recycles the paint  from the container below the mer-
chandise back up into the trough and maintains  the paint level in the trough.

     The "expected transfer efficiency" for  the curtain  coating method is a-
bout the same as for the dip and flow coating methods (75 to 90%).
ROLL COATING

     In this method liquid paint is applied by  a  transfer roll directly to the
surface of the merchandise.  This method can be used  to  paint any flat mater-
rial, rigid or flexible, individual pieces or continuous sheets, to one side
or to both sides simultaneously.  The principle of  roll  coating is to cover
the surface of the transfer roll with liquid paint, control  the amount of paint
on the surface of the transfer roll by means of a metering roll, and then to
transfer the paint from the transfer roll directly  to the surface of the mer-
chandise by direct contact (Figure 19).
                              CROTCH  FED PAINT
                                                   MERCHANDISE
                               PAN FED  PAINT

                          Figure 19.  Roll coating.

     The above illustration shows basically a typical arrangement for roll
coating both sides of a continuous sheet of material simultaneously.  In a
typical arrangement for coating only one side, the transfer  and metering
rolls on the opposite side would be replaced by a single "nip" roll for the
purpose of maintaining pressure between the transfer roll and the material.

                                      29

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     There are a number of variations to the typical method  of  roll coating
shown in Figure 19.  For example, a better application of the paint to the
surface of the merchandise is sometimes achieved by "reverse roll  coating".
In other words, at the point of contact between the transfer roll  and the ma-
terial the transfer roll is rotating in the opposite direction  from the direc-
tion of travel of the material.  This causes a "wiping" action  at  the point of
transfer.

     The "expected transfer efficiency" for the roll coating method is in the
range of 90 to 98%.  Another advantage of this method is that roll coating
paints are used at relatively high viscosity and, therefore, contain a compar-
atively low ratio of organic volatile solvents to nonvolatile solids.
ELECTROCOATING

     In this method the merchandise is submerged into a dilute (low viscosity)
dispersion of specially formulated nonvolatile paint solids mixed with water.
A low voltage (50 to 500 volt), direct current electrostatic field is applied,
which attracts the nonvolatile paint particles to the surface  of the merchan-
dise, -where they form a highly viscous deposit.  The merchandise is then lift-
ed out of the electrocoating bath and subjected to several ultrafiltrate rinse
stages.  Any droplets of paint lifted out of the bath on the newly painted sur-
face are rinsed back into the dip tank (Figure 20).
                                  frnl
                    CONVEYOR
               ELECTROCOATING
                     BATH
                ULTRAFILTER
                                         3 RINSE STAGES
                         Figure 20.  Electrocoating.

     Theoretically, the electrocoating method should create no waste  loads.
In practice, however, some waste is unavoidable.  It has been reported  that
the freshly deposited film contains from 0.07 to 2.0 wt% organic volatiles.d
  Phillips, G. Electrocoat 71, paper No. 5, National Paint and Coating Asso-
  ciation, Washington, D.C.
                                      30

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Using these weight percentages, and assuming a nonvolatile density of 1.44 kg/1
(12 Ib/gal), for each liter (gallon) of film coating 0.01 to 0.03 kg (0.08 to
.12 Ib) of organic volatile waste will be generated during the bake curing
process.  There is also a very minor amount of organic volatile waste caused
by evaporation from the electrocoating tank, and a very small quantity of both
organic volatiles and nonvolatile solids in ultrafiltrate waste water that may
sometimes be discarded.

     The electrocoat (Code 4Bw) paint compositions surveyed during this study
and reported in Section 9 of this report list the weight 0V associated with
1 unit volume of NV ranging from 0.31 to 0.47 kg/1 (2.6 to 3.9 Ib/gal).  This
is given as the ratio for the original fill of the electrocoating tank, and
there are indications that replenishment paint, which must be continuously
added to the tank, contains less 0V, but detailed information is lacking.

     The "expected transfer efficiency" of the electrocoating method is better
than 90% and is thought by some to be as high as 99%.  Compared with the other
methods discussed previously, the electrocoating method generates markedly
less organic volatile and nonvolatile semisolid waste loads.  There may also
be a cost advantage in using the electrocoating method.  In one case the cost
has been described as "...equal to or even less than conventional dip coating
methods...".5


POWDER COATINGS

     The principle of the powder coating method is to apply a layer of fusible
powdered plastics (powder paint) to the surface of the merchandise where it is
melted and heat cured into a nonvolatile solid film coating.  There are sever-
al techniques for applying the powder paint composition to the merchandise,
each requiring a different arrangement of equipment.

Characteristics

     Powder paint compositions have characteristic differences from liquid
paint compositions.  A bulk volume of liquid paint composition contains a
specific volume percentage of nonvolatile solids, with the balance being vol-
atile liquids.  A bulk volume of powder paint composition contains only about
50 volume percent of nonvolatile solids, with the balance being air.  Powder
paint compositions "as bought" have a bulk volume density weight in the range
of 0.6 to 0.84 kg/1 (5 to 7 Ib/gal), however, when the powder is melted into
a nonvolatile solid, the solid density is in the range of 1.2 to 1.8 kg/1
(10 to 15 Ib/gal).

Fluidized Bed Technique

     A "fluidized bed" is achieved by installing a false bottom made from a
4 Burnside, G. L., Brewer, G. E. F., Strosberg, G. G.  Journal of Painting
  Technology, Vol. 41, No. 534, pp 431-437, July 1969.

5 Levinson, S. B.  Journal of Painting Technology, pp 41-49, June 1972.

                                     31

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porous material inside the paint tank.  A thin layer of powder paint is placed
on top of the porous material.   A controlled flow of air or an inert gas  such
as nitrogen is pumped into the  tank chamber below the porous material.  The
turbulence caused as the air or gas passes through the porous material and out
the top of the tank causes the  particles of paint powder to rise and remain
suspended much as dust particles in the air.  The flow rate is controlled at
a point where none of the particles are raised as high as the top of the  tank
(Figure 21).
   =Tl
            VERY  FINE  SCREEN
                                                     "FLUIDIZED"
                                                       POWDER   .
                                                        PAINT   :
COMPRESSED  AIR
 OR  INERT  GAS
                     Figure 21.  Fluidized bed dip  tank.

      The merchandise is preheated to a temperature  above the melting point of
 the paint powder and then is dipped into the fluidized bed.  The paint powder
 particles that contact the surface of the merchandise melt and form a film
 coating.

 Fluidized Bed Plus Electrostatic Field Technique

      A shallow ''fluidized bed" is formed as described above, then the paint
 powder particles are charged by a high voltage electrostatic field (Figure 22)
            AIR



VM*^*
.»••«•«
i ' : ; ' , I
' ' ' "' ''/' ,4p f""' ' ' '• , n'n " /'
, ' ', ' >t,/tys* ' * / ' ' ' ' ^>
,./'%/$/"$}'"'" ' ' " *'
"""^"^k^'- •"---'' •'< ' ''^*fsfci;$
	
1







IGH
VOLTAGE
DC

                   Figure  22.  Electrostatic fluidized bed,
                                      32

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     In this technique, the merchandise is not preheated  but  is  electrically
grounded to the power source that supplies the electrostatic  field.  The mer-
chandise does not actually enter the fluidized bed,  but when  it  passes above'
the surface the charged paint powder particles are attracted  to  it and form a
coating of powder.  The particles are retained on the surface of  the merchan-
dise by the residual electrostatic charge.  The merchandise is then processed
into a heating chamber where the paint powder particles melt  and  form a film
coating.

Fluidized Spray Technique

     The powder paint is fluidized by mixture with air or an  inert gas such as
nitrogen and sprayed from a paint gun under a very small  pressure.  The paint
particles are charged by an electrostatic field at or near the point at which
they leave the spray gun and the merchandise is grounded  electrically to the
power source that provides the field.  The paint powder particles are attract-
ed to the surface of the merchandise where they form a powder coating  (Fig-
ure 23).
       FLUIDIZED
      POWDER  PAINT
                             HIGH
                           VOLTAGE
                              DC
ELECTROSTATIC
  ATTRACTION
  ELECTROSTATIC
    REPELLENCY
            Figure 23.  Fluidized  electrostatic  powder  spraying.

     The thickness of the powder coating on the merchandise can be predeter-
mined and controlled by the strength of the electrostatic  field.  Due to the
weight of the paint particles and the low pressure of  the  operation, without
the electrostatic charge they would settle as they emerged from the paint gun.
Even if they contacted the surface of the merchandise  they would not be re-
tained.  When the powder coating has reached the  desired thickness, the at-
traction is counteracted by the residual charge in the particles already at-
tached and no more particles will be retained.  This residual charge in the
particles attached to the merchandise will also cause them to be retained on
the surface while the merchandise is processed  to  a heat chamber where they
melt and form a film coating.
     Unlike liquid paint spraying,  all the
erations is collected in a filter chamber and reused.
            "overspray"
in powder spraying op-
                                     33

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Summary

     The "expected  transfer efficiency" for powder paints using any of the
techniques described above is very good, possibly as high as 98%.

     The powder paints  surveyed  in this study and reported in Section 9 show
a very favorably  low generation  of organic volatile waste loads.  The weight
of organic volatiles per unit volume of final nonvolatile film is in the range
of 0.001 to 0.12  kg OV/1 NV (0.05 to 1.0 Ib OV/gal NV) .  This is the result of
coreactants in the  paint powders.

     There may also be  a material cost savings in using powder paints.  The
coat has been described as "...equal to conventional films at equal film thick-
       ti C                                                    	^	
ness.  "
PAINT LOSSES VS TRANSFER EFFICIENCY

     It has been  shown  in  the discussion of the various painting methods that
some paint loss must be expected in  the process of transferring a paint com-
position from  the container  to  the surface of the merchandise.  Losses will
occur whether  the most  primitive or most sophisticated methods and equipment
are used.  These  are called  "unavoidable losses" in that they are inherent to
the method and equipment used for the painting operation.

     There are many factors  which must be considered when determining the meth-
od and equipment  to be  used  for a specific painting operation.  Some factors,
such as the quality of  the finished  film coating, may automatically eliminate
the use of some classes of paint compositions and, therefore, some painting
methods.  The  nature of the  merchandise may also be a determining factor.  For
example, the roll coating  method is  obviously unsuited to merchandise with a
highly irregular  surface configuration.

     When two  or  more painting methods are equally acceptable for a specific
painting operation, the "unavoidable losses" associated with each method may
become the deciding factor in the method selected.

     The total amount of "unavoidable losses" represents the difference of the
volume of nonvolatile solids in the paint used in the operation and the volume
of nonvolatile solids in the film coating on the finished merchandise.  For
planning and calculation purposes this is usually expressed as "percent ex-
pected transfer efficiency"  (%  exp.t.e.).

     However,  a single  distinct % exp.t.e. cannot be established for each
painting method.  "Unavoidable  losses" for each method will vary with the pe-
culiarities of the specific  operation.  For example, there are more overspray
losses when painting small irregular pieces of merchandise than when painting
large flat surfaces; there are more clean-up losses if the operation requires
frequent changeover or  shutdown; etc.  Table 2 shows the range of % exp.t.e.
found through  the review of  literature and/or received by direct communica-

b Levinson, S. B., Journal of Painting Technology, pp 39-56, July 1972.

                                      34

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tion during the period of this study.

                   TABLE 2.  EXPECTED TRANSFER EFFICIENCY
            PAINTING METHOD
PERCENT EXPECTED TRANSFER EFFICIENCY
  Air Atomized, Conventional

  Air Atomized, Electrostatic

  Pressure Atomized, Conventional

  Pressure Atomized, Electrostatic

  Centrifugally Atomized, Electrostat.

  Dip, Flow, and Curtain Coating

  Roll Coating

  Electrocoating

  Powder Coatings
  43%*;  50%2;  30-60%3

  87%*;  68-87%^

  65-70%5

  85-90%6

  93%J;  85-95%"*

  75-90%6

  90-98%6;  96-98%7

  90-96%6;  99%2

  50-80%8;  98%2;  90-99%9
  1 E. P. Miller, Ransburg Co.;  SME Paper, FC73-553.
  2 J. A. Antonelli, duPont Co.;  SME Paper, FC74-654.
  3 J. A. Antonelli, duPont Co.;  "depending upon equipment and shape of
          merchandise" (direct communication)
  4 E. P. Miller, Ransburg Co.;  "depending upon object being coated"
          (direct communication)
  5 W. H. Cobbs, Jr., Nordson Corp.;  (direct communication)
  6 F. Scofield, Wapora, Inc.;  EPA Contract 68-01-2656
  7 M. Wismer, PPG Industries;  (direct communication)
  8 S. B. Levinson, D. Litter Lab.;  Journal of Painting Technology
          pp 35-56, July 1972
  9 T. W. Seitz, Sherwin-Williams Co.;  "newer reuse methods" (direct com-
          munication)
WASTE LOADS VS TRANSFER EFFICIENCY

     The following factors were established in Section 4:

     1)  All volatile components in paint compositions are sacrificed during
         the transfer and curing operations.

     2)  The quantity of paint composition required for a painting operation
         is determined by the volume of nonvolatile solids required in the
         film coating on the finished merchandise.
                                      35

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     3)  The greatest pollutional waste loads generated by painting operations
         are the organic volatile vapors emitted during transfer and curing.

     4)  The volume of waste loads does not provide meaningful data and must
         be converted to weight.

     Assuming that a 100% transfer efficiency could be achieved, only volatile
waste loads would be generated, and these would be in direct proportion to the
ratio  of the components in the "as used" paint composition.  However, since
100% transfer efficiency is never realized, not only are volatile waste loads
increased in proportion to the actual percentage of transfer efficiency, but
nonvolatile waste loads are also generated.

     A certain water borne spray paint  (Code lAw 1) was shown in Section 4 to
have a volume relationship of:

               1.000 vol (liter or gallon) NV
               0.568 vol (liter or gallon) 0V
               2.192 vol (liter or gallon) water
               3.760 vol  (liter  or  gallon) paint composition

      If  this paint  composition is used  in an operation with only a 50% trans-
fer efficiency, only half  the volume  of NV would actually become film coating
on the merchandise; the other half  would become an NV waste load.  The entire
volume of 0V would  become  an 0V  waste load.
TRANSFER EFFICIENCY  CALCULATIONS

     The weight  of NV,  0V,  and  total waste  loads can be calculated by use of
the following  three  equations.

Equation 5

     The following equation may be used  to  calculate the weight of NV waste
at any  given "percent expected  transfer  efficiency":

          wNV  Wet    =   [(100/et)  - 1] x (Ap/K) x  t x dNV

     where

                 W    =   waste

               et    =   percent expected transfer  efficiency

               A    =   area  to be painted  in m2  (ft2)

                 JC    =   1,000 m2 x 1 ym/1  (1,604  ft2 x 1 mil/gal)

                 t    =   thickness  of coating in ym (mil)
                                      36

-------
                d   =   density in kg/1 (Ib/gal)

Example 5

     To calculate the weight of the NV waste load generated by painting a sur-
face area of 149 m2 (1,604 ft2) with a film coating 25.4 ym (1 mil) thick at
an expected transfer efficiency of 85% using a paint with an NV density of
1.75 kg/1 (14.6 Ib/gal):

          wNV Wet   =   [(100/85) - 1] x 149/1,000 x 25.4 x 1.75

                        (1.176    - 1) x 0.149     x 44.45

                        0.176          x 6.62

                    =   1.17 kg NV waste expected

     or, using U.S. standards

          wNV Wet   =   [(100/85) - 1] x 1,604/1,604 x 1 x 14.6

                        0.176          x 14.6

                        2.57 Ib NV waste expected

Equation 6

     The following equation may be used to calculate the weight of 0V waste
at any given "percent expected transfer efficiency":

          wOV Wet   =   (100/et) x (A^/K) x t x wOV/vNV

     where

          wOV/vNV   =   weigh  (kg or Ib) of 0V per volume (1 or gal) of NV

Example 6

     To calculate the weight of the 0V waste load generated by the same paint-
ing operation used in example  5:  (wOV/vNV =0.50 kg/1  (4.3 Ib/gal))

          wOV Wet   =   (100/85) x (149/1,000) x 25.4 x 0.52

                        1.176    x 0.149       x 13.21

                        2.31 kg 0V waste expected   or    (5.06 Ib)

Equation 7

     The following equation may be used to calculate the weight of Total
waste at any given "percent expected  transfer efficiency":
                                      37

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          wT Wet
     where
Example 7
wNV Wet + wOV Wet
                        total
     To calculate  the weight of  total waste loads generated by the operation
described in Examples 5 and 6:
          wT W
              et
1.17 kg NV + 2.31 kg 0V

3.48 kg total waste   (7.6.7 Ib)
SUMMARY

     Transfer efficiency has a direct relationship to all the waste loads gen-
erated by any painting operation.  0V waste loads are generated by;all painting
operations and are directly proportional to the amount of 0V in the total quan-
tity of paint composition used in the painting operation.  NV waste loads are
the direct result of transfer efficiency;  ideally, if a 100% transfer effi-
ciency could be achieved, no NV waste loads would be generated, however,  since
this is nearly impossible, some NV waste loads are generated by all painting
operations.  NV waste loads rise at an accelerated rate with decreasing trans-
fer efficiency.

     Table 3 has been prepared to show the waste loads generated at various
"percent expected transfer efficiency" for the specific painting operation
        TABLE 3.  WASTE LOADS VS PERCENT EXPECTED TRANSFER EFFICIENCY
%
exp . e . t .
100
95
90
85
80
75
70
65
60
55
50
*33
wOV Wet
kg
1.97
2.07
2.19
2.31
2.46
2.63
2.81
3.03
3.28
3.58
3.94
5.91
(Ib)
(4.34)
(4.56)
(4.83)
(5.09)
(5.42)
(5.79)
(6.19)
(6.68)
(7.23)
(7.89)
(8.68)
(13.02)
wNV Wet
kg
0.00
0.35
0.74
1.17
1.66
2.21
2.84
3.56
4.41
5.47
6.62
13.28
(Ib)
(0.00)
(0.77)
(1.63)
(2.57)
(3.66)
(4.87)
(6.26)
(7.84)
(9.72)
(12.05)
(14.58)
(29.16)
wT Wet
kg.
1.97
2.42
2.93
3.48
4.12
4.84
5.65
6.59
7.69
9.05
10.56
19.19
(Ib)
(4.34)
(5.33)
(6.46)
(7.67)
(9.08)
(10.66)
(12.45)
(14.52)
(16.95)
(19.95)
(23.26)
(42.18)
vOV + vNV
liter
5.90
6.24
6.54
6.96
7.37
7.86
8.43
9.07
9.83
10.77
11.80
17.70
(gal)
(1.56)
(1.65)
(1.73)
(1.84)
(1.95)
(2.08)
(2.23)
(2.40)
(2.60)
(2.85)
(3.12)
(4.68)
   *  Used  for the purpose of illustration only.
                                     38

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used in Examples 5, 6, and 7; i.e. to paint a surface area of 149 m  (1,604
ft ) with a film coating 25.4  m (1 mil) thick using paint composition Code
lAw 1.

     The information contained in Table 3 is shown graphically in Figure 24.

         kg

       11.0—1

       10.0-
                      90        80        70        60
                    •*• "% expected  transfer efficiency" -»•

      Figure 24.   Waste loads vs percent expected transfer efficiency

     The two most important factors to remember are:

     1)   0V waste loads are the result of both the ratio of 0V to NV in the
         paint composition (wOV/vNV) and the expected  transfer efficiency.
         Minimum waste loads are generated at maximum  transfer efficiency and
         increase in direct proportion to the total volume of paint used.

     2)   NV waste loads are generated only as the result of transfer efficien-
         cy.  Minimum waste loads are generated at maximum transfer efficiency
         and increase at an-accelerating rate as percent of transfer efficien-
         cy decreases.
                                     39

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                                   SECTION 6

                            PAINT  CURING METHODS


     The process by which  the paint composition "as used" is transformed into
a solid, wear-resistant nonvolatile film coating on the merchandise is known
as "curing".  Most paint compositions are formulated to function best when a
specific curing method is  used.  However, some compositions may be used under
several curing methods, or even with a combination of methods.  Curing methods
fall in the three general  principles described below.


AMBIENT TEMPERATURE CURING

     The simplest method of curing is provided by those paint compositions that
"dry" in an atmosphere at  or near  the ambient temperature of the work area.
There are three general classes of paint compositions that are normally cured
at ambient temperature:  1) solvent and/or water borne paints that cure through
evaporation of the liquid  components;  2) paints which cure through the absorp-
tion of moisture from the  atmosphere; and 3) two component paint compositions
which, when mixed, solidify within a few minutes.

Evaporation

     Air drying through evaporation was, historically, the earliest used method
of paint curing.  Paint compositions may undergo a strictly physical change as
the solvents are evaporated, or they may undergo a combination of physical and
chemical changes.  Some paints, such as lacquers used for nail polish, cure by
physical evaporation only.  This is a reversible, process, and the nonvolatile
solid film can be redissolved into a liquid state by use of the same solvents.

     Paint compositions with oils, such as linseed, as part of the liquid com-
ponents cure by a combination of physical evaporation and chemical reaction.
During the evaporation of  the solvents, other components undergo a chemical
combination with oxygen from the air.  This is an irreversible process and the
film cannot be redissolved.

Moisture Curing

     Some paint compositions contain liquid components which when exppsed to
the air react with the moisture in the air to form solids.  This is actually
a combination of physical  evaporation and chemical reaction during the curing
process, and as such is irreversible.  These paint compositions require special
handling and must be kept  sealed until they are used.


                                     40

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Two Component Paints

     A comparatively new family of paints form polymerized films at ambient
temperatures when two liquid components are mixed together.  When the two com-
ponents are mixed, they react chemically with each other to form a solid poly-
mer.  Since only a limited time is available to apply the paint after the two
components are mixed, they are usually used in spray operations where they are
mixed in the spray gun chamber.


BAKE CURING

     The application of heat to accelerate the evaporation process is the most
widely used curing method by industry.  There are a number of ways to achieve
"bake" curing, but they all function on the principle of subjecting the paint-
ed merchandise to temperature in the range of 120 to 175°C ( 250 to 350°F)  for
a period usually about 8 to 30 minutes.  Continuous air circulation through the
baking chamber is essential to remove the organic volatile waste and to dilute
the vapors to below the explosive level.


RADIATION CURING

     There are several classes of liquid paint compositions that will solidify
quite rapidly when exposed to radiant energy.  The two classes surveyed in this
study were the electron beam activated and the ultra-violet ray activated.

Electronic Beam Curing

     Electronic beam radiation curable paint compositions are identified as
Code 6eb in Section 9.  These paints may be applied to the merchandise by a
variety of methods such as spray, roll, flow, dip, etc.   After the paint is
applied the merchandise is placed in a chamber containing a relatively oxygen
free atmosphere (usually less than 500 ppm)  and exposed to high energy elec-
tron beams (g-rays).   When the beta-rays impinge on the liquid paint compon-
ents,  a chemical reaction is initiated which causes them to solidify into a
solid film coating (Figure 25).
           ELECTRONIC
              BEAM
           GENERATOR
BEAM
TAINTED
 SURFACED
                      Figure 25.   Electron beam curing.

                                     41

-------
     Paints in this class are used where a comparatively thick film  coating is
required on either flat or profiled merchandise.  The composition may be either
pigmented or clear.  The weight of organic volatiles associated with a unit vol-
ume of final solid nonvolatile film is approximately 0.048 kg OV/1 NV (0.40 Ib
OV/gal NV).

     In comparison with other classes of paints, electron beam curing paints
have been reported as competitive:  "...cost of liquid coating mil x ft2 may
be less than that of solvent thinned coatings...".7

Ultra-Violet Ray Curing

     Ultra-violet ray curable paint compositions are identified as Code 6uv in
Section 9.  These paint compositions are used where a comparatively  thin film
coating is required on virtually flat surfaces, therefore, they are  generally
applied to the merchandise by the roll coating method.  The freshly  coated mer-
chandise is then passed within a few inches of one or more ultra-violet lamps
(usually mercury vapor tubes) which emit 315 to 400 millimicron waves (Figure
26).

                     REFLECTOR
               ULTRA-VIOLET
               LAMP
                   r^f ?"   /'"'' ''i"  i   V' " "v-v '  v  "v  ^ '-\
                   £?&-,    /   /         >     *  \  v   \  \  \
                          ~. ;    *    ^     \  s  \  \  v
                          ^^-/     i     \      .   .   <  \
                          "^ ^.-'   -'fc-'^ -'^	 ,,VA ,.,*.;
                    Figure 26.  Ultra-violet ray curing

     The weight of organic volatiles associated with a unit volume of  final
solid nonvolatile film ranges from 0.024 to 0.060 kg OV/1 NV (0.20 to  0.50 Ib
OV/gal NV).

     Ultra-violet ray curing paint compositions have been described as having:
"...limited applicability:  thin films and special pigments...low capital
cost...less floor space...".7
7 Levinson, S. B.  Journal of Painting Technology, pp 29-40,  August 1972.

                                      42

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FORMATION OF COREACTANTS

     In addition to the organic volatile wastes previously discussed,  there
are certain organic volatiles generated by chemical reaction during the curing
process of some paint compounds.  These organic volatiles are called "coreact-
ants (COR).  The coreactants most frequently encountered are water, methanol,
etc.  The weight of coreactants has been reported as usually less than 5 wt%
of the nonvolatile solids portion of the paint compositions.8

     The weight of vaporized, organic volatile coreactants has not been in-
cluded in the previous calculations of weight 0V/volume NV.  (An exception has
been made for the powder paints surveyed in Section 9.   The weight of  coreact-
tants has been included in the tables in Section 9 for  powder paints (Code 5B)
as these are the only organic volatile wastes for these compositions.)

     Prior to the chemical reaction that causes them to vaporize, coreactants
are actually a part of the nonvolatile solids in the paint composition.

Equation 8

     The following equation may be used to calculate the weight of coreactants
generated during the curing process.  The weight of organic volatile coreact-
ant waste must then be added to the organic volatile waste calculated  by other
considerations.

          wCOR  =  (Ap/K) x t x dNV x (wt% COR/100)

     where

            A^  =  area painted

             K  =  1,000 m2 x 1 ym   (1,604 ft2 x 1 mil)

             t  =  thickness of nonvolatile film coating

           dNV  =  density of nonvolatiles

       wt% COR  =  weight percentage of coreactants in nonvolatiles

Example 8

     To calculate the wCOR generated during the curing of a painted surface
area of 149 m2 (1,604 ft2) with a film thickness of 25.4 ym (1 mil) assuming
a dNV of 1.98 kg/1 NV (16.5 Ib/gal NV) and a wt% COR of 4.5:

          wCOR  =  (149/1,000) x 25.4 x 1.98 x (4.5/100)

                =  0.34 kg    (0.74 Ib)
8 Greer, S. T.; and Anderson, C.;  Industrial Finishing, April 1973.  (and
  direct communications with the authors and others)

                                      43

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Odors
     Heavy malodorous fumes have been detected at times during the curing pro-
cess of some paint compositions.  These fumes are currently the subject of
odor analysis and further study.9
  Schuetzle, D.;  Prater, T. J.; and Ruddell, S. R.;  "Sampling and Analysis
  of Emissions from Stationary Sources:  I.  Odor and Total Hydrocarbons",
  Journal of the Air Pollution Control Association, Volume 25, Page 925,  (1975)
                                     44

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                                  SECTION  7

                            SANDING AND STRIPPING
     There are certain unavoidable losses  of  paint solids that are caused by
the nature of the painting operation and in some  cases by mistakes made in
the operation.  Primary among these are the losses caused by sanding opera-
tions between coats and stripping necessary to remove defective coats.


SANDING

     Sanding may be necessary to achieve the  desired smoothness to the surface
of the film coating on the merchandise.  Cured film coatings may show some im-
perfections due to defects in the original surface of the  merchandise, by the
settling of dust or lint on the paint before  it dries, and some roughness or
"orange peel" effect inherent in the paint or painting technique.  These im-
perfections are removed by either a wet or dry sanding process, which removes
part of the film coating and  generates a small amount of nonvolatile waste
(Figure 27).
   ORANGE  PEEL
LINT  OR DUST
                                PRIMER PAINT
                    SANDED  SURFACE
                                 PRIMER  PAINT
                    Figure 27.   Sanding painted  surfaces.

     Merchandise with a highly uneven or porous  surface  is often painted first
with a primer coat and sanded smooth before the  application of the finished
coatings.  Calculation of the waste loads generated by sanding operations is
extremely difficult.  Actually, the waste should include the weight of the dis-
carded disks or belts of sandpaper, and in the case of a wet sanding process,
                                     45

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the total weight of the detergents, oils, or organic solvents used.


STRIPPING

     Occasionally the film coating applied to some pieces of merchandise may
be defective or may be damaged to a point where it must be removed.  In many
painting processes, paint may also accumulate on equipment used in the process
that must be stripped.

     A paint "stripping" operation usually consists of a stripping bath into
which the parts to be stripped are submerged.  The stripping  bath is composed
of water and paint-lifting chemicals, usually caustic soda, surfacants, melted
salts, etc.  The bath is usually heated to near the boiling point.  The pro-
cess may include scraping or wire brushing and two or more emersions may be
necessary.

     The weight of paint stripped is usually relatively small in comparison to
the total paint consumption in the overall operation, except in refinishing
shops where it may be a normal part of the operation.

Equation 9

     The following equation may be used to calculate the weight of stripped
paint :
          wWs  =   (dNV/K) xtCAjn x 1^) +  (Ah x th)]

     where

          wWs  =  weight of stripped off waste

           Am  =  area of merchandise stripped

           1^  =  thickness of film on merchandise

           Ah  =  area of hangers stripped

           t^  =  thickness of film on hangers

Example 9

     To calculate the wWs generated by a stripping operation consisting of a
merchandise area of  12.9 m2 (138.9 ft2) with a film thickness of 50.8 ym (2
mil) and a hanger area of 1.35 m2 (14.5 ft2) with a film thickness of 557.2
(18 mil) assuming a  dNV of 2.02 kg/1 (16.83 Ib/gal):

          wW   =   (2.02/1.0) x [(166.4 x 0.0000508) +  (1.82 x 0.0005572)]
            s

               =  2.02 x (0.0085 + 0.001)

               =  0.019 kg   (.158 Ibs)


                                     46

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Summary

     It should be noted that the thickness of the film coating on the merchan-
dise is usually only about 25.4 to 76.2 pm (1 to 3 mils), while the thickness
of the film on the hangers may be 500 ym (20 mils) or more.  It should also be
noted that the nonvolatile paint solids:
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                                  SECTION 8

                         CALCULATION OF WASTE LOADS
GENERAL
     It has been shown in the preceding Sections of this report that both or-
ganic volatile  (0V) and nonvolatile  (NV) waste loads are generated by all paint-
ing operations.  Procedures and equations have been given for the prediction
of waste loads based on known factors.

     The actual waste loads generated can be determined based on these same
known factors plus production and inventory data developed during the period
of operation.


PREDICTION OF WASTE LOADS

     Equations  1 through 9 were developed and have been presented as tools to
be used for the calculation of predicted waste loads from a specific, planned
painting operation.  Actually, equations 1 through 4 are used for basic paint-
ing calculations and equations 5 through 9 are used for waste load calculations.

     Each calculation requires the use of known or estimated factors.  For ex-
ample:

     1)  The surface area of the merchandise to be painted.

     2)  The thickness of the film coating to be applied.

     3)  Percent of expected transfer efficiency of the painting method and
         equipment to be used.

     4)  The nature of the components of the paint composition to be used.
         (Specifically the density weight of the nonvolatile components per
         volume unit and the weight of organic volatile components per volume
         unit of nonvolatiles.)

     5)  If applicable, the weight percent of coreactants in the nonvolatiles.

     Using the above factors and equations 5, 6, and 8, the predicted NV, 0V,
and COR waste loads can be calculated.

     Additional waste loads are occasionally generated by paint losses result-


                                     48

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ing from accidental spills and leaks, cleaning and repairing of equipment, the
use of organic volatile cleaning materials, and paint sanding and stripping op-
erations.  Though these waste generations usually evade prediction, it is esti-
mated that in most painting operations they actually add less than 5 percent to
the predictable waste loads.                            '


DETERMINATION OF WASTE LOADS

     The actual waste loads generated during a painting operation include all
organic volatile and nonvolatile solids which are consumed during the opera-
tion except the weight of the nonvolatile solids that actually leave the plant
in the form of the finished film coating on the merchandise.

     In addition to the five basic factors required to calculate the predicted
waste loads, the following factors are required to calculate the determined
waste loads:

     1)  The total consumption of paint compositions, thinners, cleaning fluids,
         etc. during a specific production or inventory period.

     2)  The total area and thickness of the nonvolatile film coating on the
         merchandise that actually leaves the facility.

     Using all this data, the weight of nonvolatile waste (wNV W),  the weight
of organic volatile waste (wOV W), and the weight of total waste (wT W) can be
determined by calculations using Equations 10, 11, and 12.

Equation 10

     The following equation may be used to calculate the determined nonvolatile
waste load generated by a specific painting operation:

          wNV Wd£t  =  wNVcons  -  [(Ap/K) x t x dNV]

     where

              Wj t  =  determined waste load

           wNV      =  weight of the nonvolatile components of all paint com-
                       position consumed during the painting operation

     As you can see, this equation is quite similar to equation 5 except that
actual consumption data is used in place of an "expected transfer efficiency"
factor.  The determined NV waste load will include all losses of nonvolatile
solids caused by transfer efficiencies, sanding and stripping processes, clean-
up, spillage, etc.  However, NV wastes from sources other than the paint com-
position, such as discarded sand paper or abrasives used in sanding operations
are not included.  It is estimated that NV waste from such sources will add
only a very small percentage to the plant waste load, and in many cases may be
entirely insignificant.  If such wastes are considered significant, they must
be added separately.

                                     49

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Example 10

     To calculate the weight of the determined NV waste load generated by an
operation in which 9,290 m2 of essentially flat merchandise has been painted
with a nonvolatile film coating 30.5 ym thick.  Assume that inventory records
show that 863 liters (228.4 gallons) of paint composition Code IBs 2 contain-
ing 412 kilograms (908 pounds) of NV with a density of 1.15 kg/1 (9.6 Ib/gal)
were consumed during the operation:

          wNV Wdet  =  412 -  [(9,290/1,000) x 30.5 x 1.15]

                    =  412 -  (9.29 x 35.08)

                    =  412 - 325.89

                    =  86.11 kg   (189.7 Ibs)

     The above example shows only the determined waste load generated by the
NV solids in the paint composition used.  If significant additional waste is
generated by other sources such as discarded sand paper or abrasives used in
sanding or stripping operations, that weight must be added to the above total

Equation 11

     The following equation may be used to calculate the determined organic
volatile waste load generated by a specific painting operation:
          wOV wdet  =  vNVcons x

     where

              W(jet  =  determined waste load

           vNVcons  =  volume of the nonvolatile components of all paint com-
                       position consumed during the painting operation

           wOV/vNV  =  weight of 0V per unit volume of NV

     This equation produces a result similar to equation 6 by using actual con-
sumption data rather than "expected transfer efficiency" and finished film coat-
ing data.  The determined 0V waste load will include all wastes generated by
the organic volatiles in the paint composition as used.  However, 0V wastes
from sources other than the paint composition, such as organic volatile clean-
ing fluids, chemicals used for paint stripping, etc., are not included.  This
additional 0V waste in most painting operations represents only a small per-
centage of the plant waste load, but in some cases may be quite significant.
If such wastes are considered significant, they must be added separately.

Example 11

     To calculate the weight of the determined 0V waste load generated by the
same painting operation used in Example 11:  (The weight ration of 0V to unit

                                     50

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volume of NV for paint composition Code IBs 2 as used is 1.28 kg/liter (10.7
Ib/gal.)

          wOV Wdet  =  863 x 1.28

                    =  1104.6 kg   (2444 Ibs)

     The above example shows only the determined waste load generated  by the
organic volatile solvents in the paint composition used.  If significant ad-
ditional waste is generated by other sources such as cleaning fluids or  strip-
ping compounds, that weight must be added to the above total.

Equation 12

     The following equation may be used to calculate the determined total waste
loads generated by a specific painting operation:
          wT Wdet  =  wNV Wdet = wOV wdet x wCOR

     where

                   =  weight of the total determined waste loads
         wNV Wdet  =  result of equation 10 with any other significant  NV
                      waste added

         wOV Wj t  =  result of equation 11 with any other significant  0V
                      waste added

             wCOR  =  result of equation 8

     The weight of coreactant waste as calculated by use of equation 8  is
based on the volume of NV applied as a film coating on the merchandise.  This
factor is used for two primary reasons:   1) Coreactants are most often  found
in paint compositions designed for bake or radiation curing; and 2)  the re-
lease of coreactant waste is stimulated by the curing process.

     Actually, since coreactant waste is the result of chemical reaction which
transform a percentage of the nonvolatile paint solids into volatile coreact-
ants, for a finite calculation of waste loads the weight of coreactant  waste
should be subtracted from the weight of NV waste as determined.  In fact, co-
reactant waste may be generated by the entire weight of NV consumed, though
coreactants released from NV waste may be much slower than that released from
the NV film on the merchandise during the curing operation.

Example 12

     To calculate the weight of the determined total waste loads generated by
a painting operation in which 9,290 m2 of essentially flat merchandise  has been
prime coated with a film coating 20.3 iam thick and top coated with a film coat-
ing 35.6 um thick.  Assume that inventory records show that 277 liters  (73.4
gallons) of paint composition Code 4Bw 4 containing 295 kilograms (650  pounds)

                                      51

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of NV with a density of 1.43 kg/1 (11.9 Ig/gal) were consumed during the prime
coating operation and that 969 liters (256.4 gallons) of paint composition Code
IBs 3 containing 704 kilograms (1,551 pounds) of NV with a density of 1.58 kg/1
(13.2 Ib/gal) were consumed during the top coating operation:  (Primer paint
composition Code 4Bw 4 contains no coreactants;  top coat paint composition
Code IBs 3 contains approximately 4 wt%.)

Prime Coat—

          wNV Wdet  =  295 -  [(9,290/1,000) x 20.3 x 1.43]

                    =  295 -  (9.29 x 29.03)

                    =  295 -  270

                    =  25 kg  NV waste determined    (56 Ib)

          wOV Wdet  =  0.31 x 206

                    =  64 kg  0V waste determined    (142 Ib)

           wT wdet  =  25+64+0

                    =  89 kg  Total waste  determined    (198 Ib)

Top Coat—

          wNV Wdet  =  704 -  [(9,290/1,000) x  35.6 x 1.58]

                    =  704 -  (9.29 x 56.25)

                    =  704 -  523

                    =  181 kg NV waste  determined    (399  Ib)

          wOV Wdet  =  1*06 x 446

                    =  473 kg NV waste  determined    (1,042 Ib)

              wCOR  =   (9,290/1,000) x  35.6  x  1.58  x  (4/100)

                    =  9.29 x 56.25 x 0.04

                    =  21 kg  COR waste  determined    (46  Ib)

           wT Wdet  =   181 +  473 + 21

                    =  675 kg Total waste determined    (1,487 Ib)

Total Plant  Waste—
     The  total  plant waste  for this  specific painting  operation can be found
by adding the  sum of  the prime coat total waste to  the sum of the top coat

                                      52

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waste:

     Total Plant Waste  =  89 + 675

                        =  764 kg Total Plant waste determined   (1,683 Ib)


PREDICTED VS DETERMINED WASTE LOADS

     For a comparison of the predicted and determined waste loads for the oper-
ation described in example 12, first calculate the predicted loads using the
highest "expected transfer efficiency" for the painting method used in accord-
ance with equations 5 and 6:

Prime Coat  (Electrocoating method at 96% expected transfer efficiency)

          wNV Wefc  =  [(100/96) - 1] x (9,290/1,000) x 20.3 x 1.43

                   =  0.042 x 9.29 x 29.03

                   =  11.33 kg NV waste predicted   (25 Ib)

          wOV Wet  =  (100/96) x (9,290/1,000) x 20.3 x 0.31

                   =  1.042 x 9.29 x 6.3

                   =  61 kg 0V waste predicted   (134.4 Ib)

Top Coat  (Air atomized spray method at 87% expected transfer efficiency)

          wNV Wet  =  [(100/87) - 1] x (9,290/1,000) x 35.6 x 1.58

                   =  0.149 x 9.29 x 56.25

                   =  77.8 kg NV waste predicted   (171.4 Ib)

          wOV Wet  =  (100/87) x (9,290/1,000) x 35.6 x 1.06

                   =  1.149 x 9.29 x 37.74

                   =  402.85 kg 0V waste predicted    (887.5 Ib)

     As you can see, the predicted loads at these transfer efficiencies are
less than the determined loads calculated in  example  12.  Next, calculate the
predicted loads using the lowest "expected transfer efficiency":

Prime Coat  (At 90% expected transfer efficiency)

          wNV Wet  =  [(100/90) - 1] x (9,290/1,000) x 20.3 x 1.43

                   =  0.111 x 9.29 x 29.03
                                      53

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                   =  29.94 kg NV waste predicted    (66 Ib)

          wOV Wet  =  (10.0/90) x (9,290/1,000) x 20.3 x 0.31

                   =  1.111 x 9.29 x  6.3

                   =  65 kg 0V waste  predicted   (143.2 Ib)

Top Coat  (At 68% expected transfer efficiency)

          wNV Wet  =  [(100/68) - 1]  x  (9,290/1,000) x 35.6 x  1.58

                   =  .47 x 9.29 x 56.25

                   =  245.6 kg NV waste predicted    (541  Ib)

          wOV Wet  =  (100/68) x (9,290/1,000) x 35.6 x 1.06

                   =  1.47 x 9.29 x 37.74

                   =  515.4 kg 0V waste predicted    (1,135.4 Ib)

     Using the lower  transfer efficiencies,  the predicted waste loads are
greater than the determined loads calculated in example 12.  Therefore,  the
determined waste loads  are within the acceptable percentage of transfer  ef-
ficiency range.
                                      54

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                                  SECTION 9

                   COMMERCIAL PAINT COMPOSITIONS SURVEYED
GENERAL

     During the course of this study, a number of commercial paint compositions
currently available on the market were surveyed.   Such paint compositions are
usually classified generically according to the filmformer content.  The film-
formers contained in the surveyed paints included: acrylic, alkyd, epoxy, phen-
olic, cellulose acetate butyrate, polyester, polythioester, urethane, and vinyl.

     The filmformers constitute the majority of the nonvolatile solids in most
paint compositions, with pigments and other additives constituting the rest.

     The greatest and most troublesome waste loads are generated by the organic
volatile solvents used in the paint compositions.  Most paint compositions are
carefully formulated for compatibility with specific painting methods and equip-
ment and curing processes.  For example, compositions containing acrylic film-
formers may be designed for application by spray, dip, roll, etc. methods. Dip
coating requires less organic volatile solvents than spray coating, and roll
coating requires still less.  Also, solvent borne paint compositions are more
suitable for air drying, and water borne more suitable for bake drying.

     It is obvious from the above that the organic volatile solvent content of
paint compositions is influenced by the paint method and equipment and curing
process for which it was designed.  Furthermore,  it has been established in the
earlier Sections of this report that the normal unavoidable losses of nonvola-
tile paint solids during painting operations are also directly related to these
two factors.

     This study has identified the following causes for waste generation and
paint losses during industrial painting operations:

     1)  All volatile components of paint compositions are sacrificed during
         the transfer and curing processes and result in waste load generation.

     2)  Some loss of nonvolatile solids are inherent in all painting methods
         and equipment which result in nonvolatile waste load generation.

     3)  Sanding and stripping operations cause paint losses and contribute to
         nonvolatile waste load generation.

     4)  Cleaning and repair of equipment cause paint losses and contribute to
         both organic volatile and nonvolatile waste load generation.

                                      55

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      5)   Coreactants  generated  by  chemical  reaction during the curing process
          of  some  paint  compositions  cause   the  loss of nonvolatile paint solids
          and contributes  to waste  load  generation.

      6)   Some losses  will occur from accidental spillage and leakage.
CLASSIFICATION OF PAINT COMPOSITIONS

      Early  in the survey of  available  commercial paint compositions it was
deemed  advisable  to  classify the surveyed paints in accordance with the paint-
ing method  and curing  process for which  they were designed, and to assign codes
to each class to  facilitate  cross reference.   The first step was to assign each
paint surveyed to one  of the following general numeric classes:

      1   Spray coatings
      2   Dip,  Flow and  Curtain coatings
      3   Coil  and  Roll  coatings
      4   Electro coatings
      5   Powder coatings
      6   Radiation Cured coatings
      7   High  Solids  Spray coatings
      8   Low Solvent  Emulsion coatings
      9   Powder Slurry  coatings

      During the survey, attention was  particularly drawn to the last three
classes of  paints identified above  due to their relatively low organic volatile
content and resulting  low generation of  0V waste loads.  These paints are com-
paratively  new and are not presently in  generally wide usage.  These new paint
compositions  have been developed by resin and  paint manufacturers largely to
meet  environmental requirements  for low  0V waste generation.

      It was found that in many of the  paint classes some of the compositions
were  designed for air  drying and others  for bake curing.  The capital letters
A and B were  assigned  to these compositions respectively to identify the curing
process. For class  6, Radiation Cured coatings, it was found that some compo-
sitions were  designed  for electron  beam  curing and others for ultraviolet light
curing.  The  lower case letters  eb  and uv were assigned to these compositions
respectively  to identify the type of radiation that is required.

      Finally,  it  was found that  in  many  of the paint classes, some of the com-
positions contain only organic volatile  solvents as liquid components while
others  contain primarily water.   These compositions are commonly referred to
as solvent  borne  and water borne.   The lowercase letters s and w were assigned
to these compositions  to identify the  primary  liquid component.

      Also,  since  more  than one commercial paint composition was surveyed within
some  of the paint classes and having the same  characteristics, a serial number
was assigned  to each composition surveyed.  Thus, the first surveyed Spray
paint,  designed for  Mr drying,  solvent  borne, was assigned a Code lAsl.
                                      56

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WASTE LOAD COMPUTATION DATA

     The computation of either predicted or determined waste loads requires the
use of basic data related to the paint composition used in the painting oper-
ation.  The two basic factors required to use the equations given in the pre-
vious sections of this report are:  1) the density of the nonvolatile compon-
ents (dNV); and 2) the weight of organic volatiles associated with a volume
unit of nonvolatiles (wOV/vNV).

     These data are usually obtained in one of the following ways:

     1)  Directly from the manufacturer of the paint composition.  This is by
         far the easiest course, and will be provided by most manufacturers in
         immediately usable form in response to communications if they under-
         stand the purpose for which it is requested.

     2)  By using formulation data provided in the manufacturer's literature.
         This process requires the mathematical computations necessary to de-
         velop the desired information.

     3)  By laboratory determination of a quantity of the paint composition.
         Such analysis should be conducted in accordance with the ASTM Paint
         Testing Manual, Philadelphia, Pa.


COMPUTATIONS USING MANUFACTURER'S LITERATURE

     The following illustrates the computations necessary to develop the den-
sity of NV components (dNV)  and  weight of 0V associated with a volume of NV
(wOV/vNV) from typical information provided in the manufacturer's literature.

Typical Manufacturer's Data

     The following is the data supplied in manufacturer's literature for paint
composition Code lAw 1.  This composition is an air drying, water borne, short
oil alkyd white enamel, designed for use in spray painting operations "as
bought" without the addition of  thinners, based on Arolon 363 resin binder
(Formula 8042-50-29b), ADM Formulary No. P-216.

                          ADM Formulary No. P-216


               Component

     Rutile

     Arolon 363 Resin

     Naptha

     Water
                                     57
Weight
Ib kg*
170.0 77.2
102.0 46.3
3.4 1.5
68.0 30.9
Volume
gal. lit.*
4.86 18.4
11.65 44.0
0.52 2.0
8.35 31.5

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                                         Weight               Volume
               Component              lb         kg*      gal.       lit.*

          Pebble Mill Grind-24h

     Arolon 363 Resin               323.0      146.6      36.87     139.4

     24% Lead Naphthenate Drier       0.4        0.2       0.04       0.15

     6% Cobalt Naphthenate Drier      1.8        0.8       0.22       0.83

     Water                          307.0      139.4      37.49     141.71
                       TOTALS       975.6      442.9     100.00     377.99

     * Weight and volume were given by the manufacturer in U.S. measures;
       metric measures added by the author.

                            Formula 8042-50-29b
Density
Ib/gal kg/1
Arolon 363
50 wt% NV
25 wt% 0V
25 wt% H20
8.76
9.89
7.50
8.20
1.052
1.188
0.901
0.985
Computations

     Using the above manufacturer's data, the following computations must be
made before dNV and wOV/vNV can be calculated;

Arolon 363—

          Vol% NV  =  [(density Arolon 363 x 0.5)/dNV] x 100

                   =  [(8.76 x 0.5)/9.89] x 100

                   -  (4.38/9.89) x 100

                   = 44.2

ADM Formulary No. P-216—
                                       Weight 0V             Volume NV
               Component              lb         kg_       gal.       lit.
     Rutile Ti02
                                                          4.86       18.4
                                      58

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                                       Weight 0V             Volume NV
               Component              Ib         _kg_       gal,       lit.

     Arolon 363 Resin                25.5       11.6      5.15       19.5

     Naptha                           3.4        1.5

     Arolon 363 Resin                80.8       36.7     16.30       61.6

     24% Lead Naphthenate Drier       0.399      0.199    0.001       0.001

     6% Cobalt Naphthenate Drier      1.799      0.799    0.001       0.001
                       TOTALS       111.9       50.8     26.3        99.5

     As you can see, all the water component has been dropped from the above
computation.  The driers add an insignificant volume of coreactant solids to
the total volume of NV which is actually even less than the 0.001 shown.  The
estimated wCOR generated by use of this paint composition is less than 0.05%
of total NV weight so is seldom worth the effort to calculate.

Total Weight of NV—

          wNV  =  w Rutile + (w Arolon 363 x wt% NV)

               =  170 + (425 x 0.5)

               =  382.5 Ib   (173.6 kg)

Density of NV—

          dNV  =  wNV/vNV

               =  382.5/26.3   (173.6/99.5)

               =  14.5 Ib/gal   (1.75 kg/1)

Weight of 0V Associated With 1 Unit Volume of NV—

          wOV/vNV  =  111.9 Ib OV/26.3 gal NV  (50.8 kg OV/99.5 1 NV)

                   =  4.26 Ib OV/gal NV   (0.51 kg OV/1 NV)

     Similar computations were performed for each paint composition surveyed
during the study and the resulting dNV and wOV/vNV data has been entered in
the appropriate columns in Table 4.  (In a few cases, manufacturer's data was
not available, hence computations were not possible and Unk has been entered
on the Table.)  Table 5 is a summary showing the range of dNV and wOV/vNV
within each class of paint compositions surveyed.
                                      59

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                             TABLE 4.   CLASSIFICATION AND  COMPOSITION OF PAINTS SURVEYED
PAINT CLASS
lAs - SPRAY, Air drying,
solvent borne







lAw - SPRAY, Air drying,
water borne
IBs - SPRAY, Bake cured,
solvent borne




PAINT DESCRIPTION
(FORMULATION)
1. Medium Oil Alkyd White
Enamel (Ashland P-31)
2. Modified Alkyd Red Primer
(Ashland Q-405a)
3. Modidied Alkyd Brown Primer
(Ashland Q-315a)
4. Modified Alkyd Green Primer
(Ashland P-lll)
5. Ur ethane Lacquer Blue
(Ashland R-501)
6. Short Oil Alkyd White
Enamel (Ashland P-49)
7. Medium Oil Alkyd White Gloss
Enamel (Ashland 1-46)
8. Zinc Rich Primer (Mirasol
601)
1. Short Oil Alkyd White Enamel
(Ashland P-216)
1. Thermoset Acrylic White
Enamel (Ashland P-36)
2. Thermoset Acrylic Black
Enamel (Ashland P-188)
3. Thermoset Acrylic White
Enamel (Ashland P-232)
4. Short Oil Alkyd White Primer
(Ashland P-63)
5. Non-oxidizing Alkyd White
Enamel (Ashland P-122a)
COMPOSITION OF BINDER .
52% Soybean Oil, 34% Phth. Anh.
in Alphatics (Aroplaz 1082M60)
32% Linseed/Tung Oil, 39* Phth.
Anh. in Xylene - Modifier:
Phenolic rosin (Aroplaz X663X50)
32% Linseed/Tung Oil, 39% Phth.
Anh. in Xylene - Modifier:
Phenolic rosin (Aroplaz X663X50)
29% Linseed Oil, 30% Phth. Anh.
in VM & P - Modifier: Rosin
(Aroplaz 1385V50)
25% Urethane in Xylene/MIBK/but .
20/50/30 (Arothane M529)
30% Tall Oil, 40% Phth. Anh. in
Xylene (Aroplaz 6065X50)
51% Soybean Oil, 30% Phth. Anh.
in mineral spirits
Epoxyester Xylene, naphtha/
acetate
Soybean Oil resin in Butoxy
ethanol /water solution
(Arolon 363)
Selfcrosslink acrylic in ethoxy
ethanol/xylene (Aroset 701XA3-50
Acrylic resin in Xylene cross-
link/melamine (Aroset 4110X60)
Acrylic resin in Xylene cross-
link/melaraine (Aroset 4110X60)
32% Tall Oil, 40% Phth. Anh. in
Xylene (Aroplaz 1453X50)
35% Coconut Oil, 41% Phth. Anh.
in Xylene (Aroplaz 2580X60)
SUGGESTED USE
TTR266d - Type IV,
low vis., color fast
TTE515 & TTP664c
fast dry, lift resist.
Rust inhibiting, lacq.
resisting
Fast drying, It. color,
Drums, machinery, etc.
For flexing parts like
bumpers, etc.
Fast drying, economical,
industrial finish
High viscosity, general
purpose, flexible, hard
Industrial weld-through
primer
Industrial coatings
Quality coat, good ad-
hesion
High gloss automotive,
industrial coatings
High gloss automotive,
industrial coatings
Light color industrial
finishes
Ultradurable exterior &
automotive
NV
kg/lit
(Ib/gal)
1.50
(12.5)
1.90
(15.8)
2.21
(18.4)
1.70
(14.2)
1.69
(14.0)
1.73
(H.4)
1.61
(13.4)
3.82
(31.8)
1.75
(14.6)
1.64
(13.7)
1.15
(9.60)
1.58
(13.2)
1.67
(13.9)
1.66
(13.8)
kg OV/lit NV
(Ib OV/gal NV)
buy
2.09
(17.4)
1.09
(9.10)
1.39
(11.6)
1.69
(14.1)
3.37
(28.1)
1.50
(12.5)
1.24
(10.3)
1.10
(9.20)
0.51
(4.26)
1.63
(13.6)
1.03
(8.60)
1.06
(8.80)
1.22
(10.2)
0.90
(7.50)
use
2.09
(17.4)
1.39
(11.6)
1.39
(11.6)
1.69
(14.1)
4.45
(37.1)
2.12
(17.7)
1.78
(14.8)
Unk
Unk
0.51
(4.26)
1.94
(16.2)
1.28
(10.7)
1.06
(8.80)
1.51
(12.6)
1.03
(8.60)
ON
O
         (continued)

-------
                                                   TABLE 4.  (continued)


PAINT CLASS
IBs - (continued)

IBw - SPRAY, Bake cured,
water borne









2As - DIP, FLOW, CURTAIN,
Air drying, solvent
borne









2Aw - DIP, FLOW, CURTAIN,
Air drying, water
borne


2Bs - DIP, FLOW, CURTAIN,
Bake cured, solvent
borne

PAINT DESCRIPTION
(FORMULATION)
6. Non-oxidizing Alkyd Yellow,
Gray, Green (Ashland R-322)
1. Modified Meleinize Gray
Surfacer (Ashland Q-509)

2. Medium Short Alkyd Orange
Enamel (Ashland P-225)

3. Medium Short Alkyd Red
Primer (Ashland Q-514)

4. Medium Short Alkyd Green
Enamel (Ashland P-223c)
1. Medium & Short Alkyd /Modi-
fied Rosin Gray Enamel
(Ashland P-134)



2. Medium & Short Modified
Rosin Black Enamel
(Ashland P-134)



1. Short, Modified Alkyd Orange
Enamel (Ashland P-235a)

2. Short, Modified Alkyd White
Enamel (Ashland P-238)
1. Short Alkyd Yellow Enamel
(Ashland P-140)



COMPOSITION OF BINDER
47% Castor Oil, 37% Phth. Anh.
in Xylene (Aroplaz 2477X65)
Linseed/Castor Oil in Butixy
Ethanol water solution (Arolon
324)
Saf flower Oil Alkyd in water/ t.
but./butoxyl ethanol water
solution (Arolon 376)
Safflower Oil Alkyd in water/t.
but./butoxyl ethanol water
solution (Arolon 376)
Safflower Oil Alkyd in water/t.
but./butoxyl ethanol water
51% Soybean, 30% Phth. Anh.
(Aroplaz 7307M50)

35% Soybean, 37% Phth. Anh.
(Aroplaz 7424X50)
Phenol-Rosin (Arochem 335)
51% Soybean, 30% Phth. Anh.
(Aroplaz 7307M50)

35% Soybean, 37% Phth. Anh.
(Aroplaz 7424X50)
Phenol-Rosin (Arochem 335)
Safflower Oil Rosin - water dis-
persion type (Arolon 585)

Safflower Oil Rosin - water dis-
persion type (Arolon 585)
35% Tall Oil, 38% Phth. in Xy-
lene/Aliphatics (Aroplaz
7435XM50)


SUGGESTED USE
Semi-dry Alkyd lacquer &
baked enamel
Sandable primer


Exterior, durable, bake
or air dry

Exterior, durable, bake
or air dry

Exterior, durable, bake
or air dry
Fast drying, general use,
flexible, hard, tough




Fast drying, general use.
flexible, hard, tough




Fast drying, good adhe-
sion & toughness

Fast drying, good adhe-
sion & toughness
Toys, etc. Excellent for
electrostatic spray

NV
kg/lit
(Ib/gal)
2.35
(19.6)
2.08
(17.3)

1.92
(16.0)

2.35
(19.6)

1.54
(12.8)
1.51
(12.6)




1.10
(9.20)




1.49
(12.4)

1.69
(14.1)
1.27
(10.6)

kg OV/lit NV
(Ib OV/gal NV)
buy
2.65
(22.1)
0.67
(5.60)

0.84
(7.00)

0.76
(6.30)

0.84
(7.00)
1.36
(11.3)




1.45
(12.1)




0.11
(0.90)

0.12
(1.00)
1.73
(14.4)

use
7.27
(60.6)
0.67
(5.60)

0.84
(7.00)

0.76
(6.30)

0.84
(7.00)
1.96
(16.3)




2.09
(17.4)




0.11
(0.90)

0.12
(1.00)
2.09
(17.4)

CT>
         (continued)

-------
                                                  TABLE 4.  (continued)


FAINT CLASS
2Bs - (continued)

2Bw - DIP, FLOW, CURTAIN,
Bake cured, water
borne

















3As - COIL & ROLL, Air or
mild heat drying,
solvent borne





3Bs - COIL & ROLL, Bake
cured, solvent borne


PAINT DESCRIPTION
(FORMULATION)
2. Oil Free Alkyd

1. Short Oil Alkyd Red Enamel
(Ashland P-243)

2. Short Oil Alkyd White Enamel
(Ashland P-233)
3. Short Oil Alkyd Black Enamel
(Ashland P227)
4. Modified Oil Maleinized
Black Primer (Ashland Q-510)

5. Medium Short Alkyd Orange
Primer (Ashland P-234)

6. Modified Alkyd Gray Primer
(Ashland 8635P1154)

7. Maleinized Oil Resin Black
Primer (Ashland Q-519)
8. Maleinized Oil Resin Black
Primer (Ashland Q-515)
1. Medium Oil Alkyd Red Shop
Coat (Ashland Q-14)

2. Medium Oil Alkyd Flat White
Enamel (Ashland H-305a)
3. Short Oil Alkyd White Enamel
(Ashland B-15)

1. Oil Free Polyester White
(Ashland P-87)



COMPOSITION OF BINDER
Polyester in aromatic solvents
(Aroplaz 6025R70)
Saf flower Oil Resin in water
dispersion (Arolon 585)

Safflower Oil Resin in water
dispersion (Arolon 585)
Safflower Oil Resin in water
dispersion (Arolon 585)
Linseed/Castor Oil Resin in eth-
oxy ethanol glycol butyl
(Arolon 324)
Safflower Oil Resin in Butoxy
ethanol/t. butanol water solu-
tion (Arolon 377)
Meleinized Oil Resin in Butoxy
ethanol/mineral spirits water
solution (Arolon 507)
Linseed Oil Resin in water solu-
tion (Arolon 525)
Linseed Oil Resin in water solu-
tion (Arolon 525)
52% High Soya, 34% Phth. Anh. in
Min. Spirits (Aroplaz 1082M50)

52% High Soya, 34% Phth. Anh. in
Min. Spirits (Aroplaz 1082M50)
38% Soyabean Oil, 43% Phth. Anh.
in Xylene/Min. Spirits (Aroplaz
7310X50)
Non-oxidizing Alkyd in Arom./
methyl-heptyl ketone (Aroplaz
6022R65)


SUGGESTED USE
Industrial high flexi-
bility
High gloss, high solids,
industrial use

High gloss, high solids,
Industrial use
High gloss, high solids,
industrial use
Rust inhibitive


High gloss, hard flexible
mar-resistand

Tough resin, outstanding
pigment suspension for
automotive use
Corrosion resistant,
economical
Automotive use

Low viscosity TTR266d-IV,
high color retention

Low viscosity TTR266d-IV,
high color retention
Very flexible, high
weather durability

Exterior coil coat


NV
kg/lit
(Ib/gal)
1.20
(10.0)
1.32
(11.0)

2.04
(17.0)
1.46
(12.2)
2.17
(18.1)

1.52
(12.7)

1.92
(16.0)

1.34
(11.2)
1.46
(12.2)
1.60
(13.3)

2.06
(17.2)
2.24
(18.7)

1.79
(14.9)

kg OV/lit NV
(Ib OV/gal NV)
buy
1.16
(9.70)
0.48
(4.00)

0.28
(2.30)
0.29
(2.40)
0.64
(5.30)

1.01
(8.40)

0.60
(5.00)

0.95
(7.90)
0.76
(6.30)
1.10
(9.20)

1.16
(9.70)
1.27
(10.6)

0.79
(6.60)

use
1.16
(9.70)
0.48
(4.00)

0.28
(2.30)
0.29
(2.40)
0.64
(5.30)

1.01
(8.40)

0.60
(5.00)

0.95
(7.90)
0.76
(6.30)
1.10
(9.20)

1.69
(14.1)
1.57
(13.1)

0.79
(6.60)

ON
         (continued)

-------
                                                  TABLE 4.   (continued)
FAINT CLASS
3Bs - (continued)




3Bw - COIL & ROLL, Bake
cured, water borne


4Bw - ELECTROCOATS, Bake
cured, water borne




PAINT DESCRIPTION
(FORMULATION)
2. Silicone modifier Polyester
White Enamel (Ashland P-77)
3. Oil Free Polyester White
Gloss Enamel (Ashland P-84)
4. Oil Free Polyester White
Gloss Enamel (Ashland P-88)
5. Oil Free Polyester White
Gloss Enamel (Ashland P-89)
6. Oil Free Polyester White
Gloss Enamel (Ashland P-81)
1. Oil Free Polyester White
Gloss Enamel (Ashland P-240)
2. Medium Short Alkyd Red
Primer (Ashland Q-514)
3. Medium Short Alkyd Green
Enamel (Ashland P-223c)
1. Short Oil Alkyd Red Primer
(Ashland Q-602)
2. Short Oil Alkyd Flat Black
(Ashland P-702)
3'. Short Oil Alkyd Gloss Black
(Ashland P-704)
4. Short Oil Alkyd Gray Primer
(Ashland Q-601)
5. Short Oil Alkyd White
Enamel (Ashland P-701)
COMPOSITION OF BINDER
70* Oil Free Alkyd, 30% Silicone
in Aromatic/polyester/butanol
(Aroplaz 1711A960)
85% Oil Free Alkyd, 15% Silicone
in Arom./but. ac. (Aroplaz
6025R70)
Oil Free Alkyd in Aromatics
(Aroplaz 6023R70)
Oil Free Alkyd in Aromatics
(Aroplaz 6029S60)
Oil Free Alkyd in Aromatics
(Aroplaz 6025R70)
Thermoset Alkyd in Butoxy ethan.
water solution (Arolon 465)
Safflower Oil in butanol/butoxy
ethanol water solution
(Arolon 376)
Safflower Oil in butanol/butoxy
ethanol water solution
(Arolon 376)
Soy Oil Resin in n-butanol water
solution (Arolon 369)
Soy Oil Resin in n-butanol water
solution (Arolon 369)
Soy Oil Resin In n-butanol water
solution (Arolon 369)
Soy Oil Resin in n-butanol water
solution (Arolon 369)
Soy Oil Resin in n-butanol water
solution (Arolon 369)
SUGGESTED USE
Good durability, econ-
omical
Good exterior durability,
economical
Low temperature curing,
interior & exterior
Low temperature curing,
interior & exterior
High flexibility, color
retention, adhesion
Excellent color retention
High gloss, adhesion,
corrosion resistant,
flexible
High gloss, adhesion,
corrosion resistant,
flexible
Automotive & other high
quality uses
Automotive & other high
quality uses
Automotive & other high
quality uses
Automotive & other high
quality uses
Automotive & other high
quality uses
NV
kg/Ut
(Ib/gal)
1.82
(15.2)
1.84
(15.3)
2.04
(17.0)
1.81
(15.1)
2.82
(23.5)
1.74
(14.5)
2.35
(19.6)
1.55
(12.9)
1.44
(12.0)
1.50
(12.5)
1.14
(9.50)
1.43
(11.9)
1.33
(11.1)
kg OV/lit NV
(Ib OV/gal NV)
buy
0.70
(5.80)
0.66
(5.50)
0.73
(6.10)
0.85
(7.10)
0.66
(5.50)
0.32
(2.70)
0.76
(6.30)
0.84
(7.00)
0.31
(2.60)
0.30
(2.80)
0.47
(3.90)
0.31
(2.60)
0.34
(2.80)
use
0.70
(5.80)
0.66
(5.50)
0.73
(6.10)
0.85
(7.10)
0.66
(5.50)
0.32
(2.70)
0.76
(6.30)
0.84
(7.00)
0.31
(2.60)
0.30
(2.80)
0.47
(3.90)
0.31
(2.60)
0.34
(2.80)
U)
         (continued)

-------
                                         TABLE 4.   (continued)
PAINT CLASS

5B - POWDERS, Bake cured



































PAINT DESCRIPTION
(FORMULATION)

1. Epowy, Conventional



2. Epoxy, low Temperature



3. Thermoset Polyester, Mela-
mine cured






4. Thermoset Polyester, Ure-
thane cured






5. Thermoplastic Polyester



6. Thermoset Acrylic







COMPOSITION OF BINDER





































SUGGESTED USE

Indoor or primer1







Outdoor metal1







Outdoor metal1







Furniture, fencing6



Outdoor metal &
equipment1






NV
kg /lit
(Ib/gal)

1.20-
1.30
(10.0-
15.0)
1.16-
1.79
(9.60-
14.9)
1.16-
1.79
(9.60-
14.9)




1.16-
1.793
(9.60-
14.9)




1.15-
1.31
(9.60-
10.9)
1.20-
1.52
(10.0-
12.7)




kg OV/lit NV
(Ib OV/gal NV)
buy
*
0.012-
0.0182
(0.120-
0.150)2
0.007-
0.0103
(0.060-
0.080)3
0.042-
0.0782
(0.350-
0.640)2
0.030-
0.04811
(0.250-
0.400)1*
0.048-
0.060
(0.400-
0.500)3
0.054-
0.0705
(0.450-
0.580)5
0.001-
0.0046
(0.010-
0.030)6
0.030-
0.0422
(0.250-
0.350)2
0.098-
0.1242
(0.820-
1.030)2
use
*
0.012-
0.0182
(0.120-
0.150)2
0.007
0.0103
(0.060-
0.080)3
0.042-
0.0782
(0.350-
0.640)2
0.030-
0.0481*
(0.250-
0.400)"
0.048-
0.0603
(0.400-
0.500)3
0.054-
0.070s
(0.450-
0.580)5
0.001-
0.0046
(0.010-
0.030)6
0.030-
0.0422
(0.250-
0.350)2
0.098-
0.1242
(0.820-
1.030)2
(continued)

-------
                                          TABLE 4.   (continued)


PAINT CLASS
SB - (continued)











6eb - RADIATION, Electron
beam cured







6uv - RADIATION, Ultra-
violet ray cured




7As - HIGH SOLIDS, Air
drying, solvent borne


PAINT DESCRIPTION
(FORMULATION)
7. Vinyl



g. Cellulose Acetate Butyrate







1. Polyester, US Pat. 3,437,514
(Ford Motor Co.)
2. Clear Acrylic, US Pat.
3,437,514 (Ford Motor Co.)
3. White Acrylic, US Pat.
3,437,513 (Ford Motor Co.)
4. White Silicone Polyester,
US Pat. 3,437,513 (Ford
Motor Co.)
1. Polyester

2. Acrylic

3. Poly-thioether (W.R. Grace
& Co.)
1. Acrylic White Enamel (Rohm
& Haas QR 568)



COMPOSITION OF BINDER












56% Styrene, 3% Maleic Anh.

97% Acrylates

90% Acrylates, 8% Styrene

30% Polyester, 30% Styrene, 10%
Acryclic Siloxane, 30% Methyl
Metacrylate






59% Acrylic oligomer, 41% Des-
modur N in ethoxy ethanol
acetate moist ener


SUGGESTED USE
Outdoor furniture,
bicycles1
Fencing, wires, under-
ground uses7
Furniture1







Wood & metal

Wood & metal

Wood & metal

Wood & metal


Printed decorations

Clear overcoats

Elevated temperature
coats, magnetic wire
Large equipment, heat
sensitive items, shop
refinishing
NV
kg/lit
(Ib/gal)
1.20-
1.68
(10.0-
14.0)
1.14-
1.32
(9. SO-
IL 0)




0.91t
(7.60)t
0.91t
(7.60)t
0.91t
(7.60)t
0.91t
(7.60)t

Unk
(Unk)
Unk
(Unk)
Unk
(Unk)
1.58
(13.2)

kg OV/lit NV
(Ib OV/gal NV)
buy
0.005-
0.0267
(0.050-
0.220)7
0.060-
0.096"
(0.500-
0.800)11
0.030-
0.0426
(0.250-
0.350)6
0.048t
(0.400)t
0.048t
(0.400)t
0.048t
(0.400)t
0.048t
(0.400)t

0.0248
(0.200)6
0.0248
(0.200)8
Unk 9
(Unk) 9
0.68
(5.70)

use
0.005-
0.0267
(0.050-
0.220)7
0.060-
0.096M
(0.500-
O.SOO)11
0.030-
0.0426
(0.250-
0.350)6
0.048t
(0.400)t
0.048t
(0.400)t
0.048t
(0.400)t
0.048t
(0.400)t

0.0608
(0.500)8
0.0608
(0.500)8
Unk 9
(Unk) 9
0.68
(5.70)

(continued)

-------
                                                                 TABLE  4.    (continued)
PAINT CLASS
7Bs - HIGH SOLIDS, Bake
cured, solvent borne
8Bw - LOW SOLVENT, Bake
cured, water borne
9Bw - POWDER SLURRY, Bake
cured, water borne
PAINT DESCRIPTION
(FORMULATION)
1. Acryloid OL 42 White Enamel
(Rohm & Haas)
2. Acrylic White Enamel (Rohm
& Haas)
1. Acrylic White Enamel
(Ashland EF-11)
1. Acrylic White Enamel
COMPOSITION OF BINDER
Hydroxyl acrylic oligoraer in
ethoxy ethanol crosslink with
melomine
40% Carboxyl acrylic oligomer,
60% Epoxy in crosslink with
Methyl-amyl-ketone/ toluene
75/25 wt%
Acrylic emulsion in water
(Arolon X-801)
Acrylic powder in water
SUGGESTED USE
Indoor & outdoor furni-
ture, air conditioners,
etc.
Low energy porcelain
replacements
General industrial or
outdoor over primer
General industrial
NV
kg/tit
(Ib/gal)
1.72
(H-3)
1.69
(14.1)
1.19
(9.90)
1.36
(11.3)
kg OV/lit NV
(Ib OV/gal NV)
buy
0.50
(4.20)
0.59
(4.90)
0.18
(1.50)
0.0180
(0.150)0
use
0.50
(4.20)
0.59
(4.90)
0.18
(1.50)
0.0181?
(0.150)0
ON
1 G. E.
2 R. D.
3 0. J.
it
5 P.
6 R.
7 J. W.
8 S. H.
                  Cole, Jr.;  SME paper, FC 74-560,  and direct  communication.
                  Hardy & T. W. Seitz;  SME paper,  FC 74-589.
            T. W.
               R.
               A.
Stvan, Sherwin-Williams  Co.
Seitz, Sherwin-Williams  Co.
Gribble, SEM-Glidden-Durkee
                                  Newer Formulations, and direct communication.
                                  direct communication.
                                  direct communication.
      Johnston,  Eastman Chemical Products, Inc.; Newer Formulations,  and  direct communication.
      Hagen,  Union Carbide  Corporation; direct communication.
      Schroeter,  General Electric Company;  "The Ultraviolet Cure of  Solventless Resins", Non-polluting Coatings & Coating Processes;
     & Prane, Editors;  Plenum Press, New York, N. Y. 1973.
A. D. Ketley, W.  R.  Grace & Company; SME paper, FC 75-331.
                                                                                                                                                 Gardon
           *  Data given for Paint Class SB only include liberated  organic coreactants.
           t  Data given are estimates.
           t  Data given include liberated organic coreactants.

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TABLE 5.  RANGE OF 0V AND NV WITHIN PAINT CLASSES SURVEYED
PAINT CLASS
SPRAY
DIP, FLOW, CURTAIN
COIL & ROLL
ELECTROCOATS
POWDERS
RADIATION
HIGH SOLIDS
LOW SOLVENT
POWDER SLURRY
CODE
lAs
lAw
IBs
IBw
2As
2Aw
2Bs
2Bw
3 As
3Bs
3Bw
4Bw
5B
6eb
6uv
7As
7Bs
8Bw
9Bw
CURE
Air dry
Air dry
Bake
Bake
Air dry
Air dry
Bake
Bake
Air dry
Bake
Bake
Bake
Bake
Elec. Beam
U' violet Ray
Air dry
Bake
Bake
Bake
CARRIER
Solvent
Water
Solvent
Water
Solvent
Water
Solvent
Water
Solvent
Solvent
Water
Water
None
None
None
Solvent
Water
Water
Water
kg OV/lit NV
1.09 - 4.45
0.52
0.90 - 7.27
0.67 - 0.84
1.36 - 2.09
0.11 - 0.12
1.16 - 2.09
0.28 - 1.01
1.10 - 1.69
0.66 - 0.85
0.32 - 0.84
0.30 - 0.47
0.005- 0.124
0.05
0.024- 0.06
0.68
0.50 - 0.59
0.18
0.018
Ib OV/gal NV
9.1 - 37.1
4.3
7.5 - 60.6
5.6 - 7.0
11.3 - 17.4
0.9 - 1.0
9.7 - 17.4
2.3 - 8.4
9.2 - 14.1
5.5 - 7.1
2.7 - 7.0
2.6 - 3.9
0.005- 1.03
0.4
0.2 - 0.5
5.7
4.2 - 4.9
1.5
0.15
kg OV/lit (OV+NV)
0.54 - 0.69
0.34
0.47 - 0.78
0.40 - 0.45
0.60 - 0.62
0.10 - 0.11
0.50 - 0.62
0.20 - 0.42
0.44 - 0.51
0.38 - 0.44
0.24 - 0.44
0.23 - 0.30
0.01 - 0.11
0.05
0.02 - 0.06
0.39
0.33 - 0.36
0.15
0.016
Ib OV/gal (OV+NV)
4.43 - 5.70
2.76
3.91 - 6.41
3.26 - 3.68
4.98 - 5.07
0.80 - 0.88
4.12 - 5.07
1.65 - 3.47
3.61 - 4.17
3.17 - 3.64
1.99 - 3.62
1.87 - 2.50
0.05 - 0.87
0.38
0.19 - 0.47
3.24
2.69 - 2.97
1.25
0.14

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                                  GLOSSARY


as bought:  A composition as produced by the manufacturer and delivered to the
     user.

as used:  A composition as used by the consumer.  Some compositions may be used
     "as bought" while others may have additional components added to achieve
     the desired characteristics for use.

calculation:  The mathematical operation used to arrive at a numerical answer.

constant (K factor):  A constant factor developed for use in mathematical cal-
     culations designed to provide specific results.

coreactant:  An organic volatile substance liberated from a nonvolatile solid
     as a result of chemical reaction.

curing method:  The method by which the organic volatiles are evaporated from
     the paint liquid to leave a solid nonvolatile film.

density:  the specific weight/volume of a substance.

determined waste:  The actual waste generated as determined after the fact.

electrostatic field:  A field of static electricity that imparts a charge to
     particles which pass through it.

filmformer:  A nonvolatile substance consisting of particles that can be formed
     into a film on a solid surface.

hot melt:  A nonvolatile solid substance that will melt into a liquid state at
     a relatively low temperature.

merchandise:  A manufactured product made from a solid material.

nonvolatile:  A nonevaporative solid substance.

organic volatile:  A substance essentially composed of carbon, hydrogen, and
     oxygen which will evaporate into the atmosphere.

paint composition:  A formulation of materials designed for used in applying
     a nonvolatile film coating to the surface of a solid material.

painting operation:  An operation in which a nonvolatile solid film coating
     is applied to the surface of a solid material.

                                     68

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painting process:  The method used to transfer a paint composition from a con-
     tainer to the surface of a solid material.

predicted waste:  The waste estimated to be produced by a planned painting
     operation using a specific painting process and curing method.

primer coat:  An initial paint coating applied to the surface of the merchan-
     dise to prepare the surface for a final "top" coating.

transfer efficiency:  A factor, usually expressed as a percentage, to repre-
     sent the amount of nonvolatile solids in the paint composition used that
     will actually become the final film coating on the merchandise.

top coat:  The final film coating on the finished merchandise.

viscosity:  The specific gravity of a paint composition.

volume percent:  The relationship of components in a paint composition ex-
     pressed in units of volume.

waste load:  The pollutional waste generated during a painting operation, us-
     ually expressed in units of weight.

weight percent:  The relationship of components in a paint composition ex-
     pressed in units of weight.
                                      69

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                                   TECHNICAL REPORT DATA
                            (Please read Instructions on the reverse before completing)
1. REPORT NO.
  EPA-600/2-80-144
             3. RECIPIENT'S ACCESSIOWNO.
4. TITLE AND SUBTITLE
  Calculations  of Painting Wasteloads  Associated with
  Metal Finishing
             5. REPORT DATE

                 JUNE  1980 ISSUING DATE.
             6. PERFORMING ORGANIZATION CODE
7. AUTHOR(S)

      George  E.  F.  Brewer
             8. PERFORMING ORGANIZATION REPORT NO.
9. PERFORMING ORGANIZATION NAME AND ADDRESS
                                                            10. PROGRAM ELEMENT NO.
  Coating Consultants
  11065 E. Grand River Road
  Brighton,  MI  48116
                 1BB610
             11. CONTRACT/GRANT NO.

                 R803467
 12. SPONSORING AGENCY NAME AND ADDRESS
  Industrial  Environmental Research  Laboratory
  Office of  Research and Development
  U.S. Environmental Protection Agency
  Cincinnati,  OH 45268	
             13. TYPE OF REPORT AND PERIOD COVERED
               Final-Dec 74 to Dec 76	
             14. SPONSORING AGENCY CODE
                   EPA/600712
 15. SUPPLEMENTARY NOTES
 16. ABSTRACT
        Twelve mathematical equations have been developed  which provide a method for
   predicting  the wasteload that  will be generated in planned  painting operations and
   for determining the actual waste load in current operations.
        The waste load generated  during the painting of metal  products is governed
   by four factors: paint composition; painting equipment; curing method; and
   miscellaneous unavoidable  losses.
        The scientific and trade  literature was surveyed for the weights and volumes
   of the nonvolatile components  (resins, pigments, etc.)  of about 70 typical, widely
   used paints, and also for  the  weights and volumes of their  organic volatile
   components.   These have been tabulated.
        Nine paint application and paint curing processes  (spray, dip, coil, flow,
   roll, curtain, electro, power  and powder slurry coating) were surveyed and the
   upper and lower reported limits of the expected transfer efficiencies were
   tabulated.
17.
                                KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
                                               b.lDENTIFIERS/OPEN ENDED TERMS  C.  COSATI Field/Group
   Industrial  Wastes 1302
   Paints 1103
   Calculations
  Pollution
  Nonmetallic coatings
  Painting
  Water pollution
  Wasteloads
                                                                               13B
18. DISTRIBUTION STATEMENT


    Release unlimited

    •^^
EPA Form 2220-1 (9-73)
                                               19. SECURITY CLASS (ThisReport)
   Unclassified
                                 82
20. SECURITY CLASS (Thispage)
   Unclassified
                           22. PRICE
                                              70
             U.S. 80VERNMENT PRINTING OFFICE:  1980--657-165/0015

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