EPA 660/3-74-004b
March 1974
                                     Ecological  Research -San:;:
    Turbulent Diffusion In
    Liquid  Jets:   Final Report

                                  Office of Research and Development
                                  U.S. Environmental Protection Agency
                                  Washington, D.C. 20460


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            RESEARCH REPORTING SERIES
Research reports of the  Office  of  Research  and
Monitoring,  Environmental Protection Agency, have
been grouped into five series.  These  five  broad
categories  were established to facilitate further
development  and  application   of   environmental
technology.   Elimination  of traditional grouping
was  consciously  planned  to  foster   technology
transfer   and  a  maximum  interface  in  related
fields.  The five series are:

   1.  Environmental Health Effects Research
   2.  Environmental Protection Technology
   3.  Ecological Research
   4.  Environmental Monitoring
   5.  Socioeconomic Environmental Studies

This report has been assigned  to  the  ECOLOGICAL
RESEARCH  series.   This series describes research
on the effects of pollution on humans,  plant  and
animal   species,  and  materials.   Problems  are
assessed   for   their   long-   and    short-term
influences.    Investigations  include  formation,
transport, and pathway studies  to  determine  the
fate  of  pollutants and their effects.  This work
provides the technical basis for setting standards
to  minimize   undesirable   changes   in   living
organisms   in   the   aquatic,   terrestrial  and
atmospheric environments.

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                                                   EPA 660/3-74-004b
                                                   March 1974
      TURBULENT  DIFFUSION IN LIQUID JETS:   FINAL REPORT
          Strong C.  Chaung and Victor W.  Goldschmidt
                 Engineering Experiment  Station
                School  of Mechanical  Engineering
                        Purdue University
                       Lafayette, Indiana  47907
                     Project No. 16070 DEP
                     Program Element  1BA025
                        Project Officer

                      George R. Ditsworth
      Pacific  Northwest Environmental Research  Laboratory
            National  Environmental Research  Center
                     Cbrvallis, Oregon  97330
                         Prepared for
             OFFICE  OF RESEARCH AND DEVELOPMENT
            U.S.  ENVIRONMENTAL PROTECTION AGENCY
                   WASHINGTON, D.C.  20460
For sale by the Superintendent of Documents, U.S. Government Printing Office Washington, D.C. 20402 - Price $1.70

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                   EPA Review Notice

This report has been reviewed by the Environmental Protection
Agency, and approved for publication.  Approval does not
signify that the contents necessarily reflect the views and
policies of The Environmental Protection Agency, nor does
mention of trade names or commercial products constitute
endorsement or recommendation for use.
                            ii

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                             ABSTRACT
Laboratory studies were conducted on the dispersion of gas  droplets
of different sizes in turbulent water jets.  The main purpose  was
to determine the turbulent transport coefficient of contaminants
suspended in turbulent flows.

The experimental results were compared to measurements of diffusion
of liquid droplets in air jets as well as to a numerical  analysis
based on the equations of motion of the particles themselves.

The results confirm that small particles in turbulent flows have  an
increasing turbulent transport coefficient with size.  The collated
experimental results exhibit when Reynolds analogy (in the transport
of mass and momentum) can be validly employed.

This report was submitted in (partial) fulfillment of Contract 16070
DEP under the (partial) sponsorship of the U.S. Environmental  Protection
Agency.
                            iii

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                         CONTENTS


 Section                                                 Page

   I           Conclusions                                1

  II           Recommendations                            3

 III           Introduction                               5

  IV           Statement of The Problem                   7

   V           Literature Review                          9

  VI           Theoretical Background                    15

 VII           Experimental Set-up and Measurement       21
               Principles

VIII           Experimental Results                      35

  IX           Turbulent Diffusivities                   71

   X           Turbulent Diffusion Characteristics       87

  XI           Significance of Results                   95

 XII           Acknowledgements                          97

XIII           References                                99

 XIV           Publications                             107

  XV           Glossary of Symbols                      109

 XVI           Appendices                               115
                             v

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                         FIGURES


No.                                                          Page

 1    Schematic Diagram of Experimental Equipment 	 22

 2    Constant Head Tank, Water Filter, Deionizer 	 23

 3    Photograph of Jet Tank	24

 4    Energy Distribution of Bubble Signal	28

 5    Filtered vs. Unfiltered Peak Voltage	30

 6    Filtered and Unfiltered Signals 	 31

 7    Block Diagram of Electronic Instrumentation 	 32

 8    Electronic Instrumentation	33

 9    Normalized Velocity Profile (With Syringe Tube)  .... 36

10    Velocity Half Width (With Syringe Tube)  	 38

11    Velocity Distribution Along Jet Axis (With
      Syringe Tube) 	 39

12    Normalized Velocity Profile (Without Syringe Tube)... 42

13    Velocity Half Width (Without Syringe Tube)	43

14    Velocity Distribution Along Jet Axis (Without
      Syringe Tube)	 44

15    Distribution of Eddy Viscosity Based on Different
      Models	 46

16    Sensor Calibration Curve	47

17    Sensor Sensitivity Curve	48

18    Transverse Distribution of Turbulence Intensities ... 49

19    Energy Spectrum Along Center Line of the Jet	'51
                            VI

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No.                                                       Page

20    Longitudinal Macro Scale Along the Turbulent
      Jet Axis	53

21    Variation of the Integrated Concentration Flux
      Along the Axial Direction	56

22    Concentration Flux Profile	57

23    Concentration Flux Profile	58

24    Concentration Flux Profile	59

25    Concentration Flux Profile	60

26    Half Width Spreading of the Concentration Flux ... 62

27    Center Line Concentration Flux Decay	63

28    Normalized Velocity Profile  (With & Without
      Contamination)  	 66

29    Velocity Half Width  (With and Without Bubble
      Contamination)  	 67

30    Velocity Distribution Along Jet Axis (With & Without
      Bubble Contamination)	68

31    Transverse Fluctuation Level  (With and Without
      Bubble Contamination 	 69

32    Concentration Profile	74

33    Concentration Profile	75

34    Concentration Profile	76

35    Concentration Profile	77

36    Concentration Profile	79

37    Concentration Profile	80
                           VI1

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No.                                                         Page



38    Concentration Profile  (With Bubble Rising Vel. Corr.)   81



39    Concentration Profile  (With Bubble Rising Vel. Corr.)   82



40    Concentration Profile  (With Bubble Rising Vel. Corr.)   83



41    Concentration Profile -(With Bubble Rising Vel. Corr.)   84



42    Concentration Profile  (With Bubble Rising Vel. Corr.)   85



43    Concentration Profile  (With Bubble Rising Vel. Corr.)   86



44    Dependence of S   on Particle Paramenter ty	89



45    Dependence of S   on Particle Parameter \l>'	94
                           Vlll

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                         TABLES


No.                                                        Paqe
1    Comparison of Various Axi-symmetric Turbulent Jet      41
     Measurements


2    Total Bubble Concentration of the Experiments          55


3    Rising Bubble Velocity                                 71


4    Turbulent Schmidt Number                               72

                     _1         >
5    Calculation of S   versus ^T                           93
                            IX

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                        SECTION I

                       CONCLUSIONS
1.  Turbulent diffusion measurements of four different bubble
sizes i.e., 343, 527, 780, and 970 microns were made.  The
measured concentration profiles of the bubbles in the axi-
symmetric water jet revealed that similarity at successive
sections was preserved and that the profiles had the same
virtual origin as the momentum diffusion.  This result
supported the original postualte that the contaminant is
diffused in a manner similar to that of momentum.

2.  The particle diffusivities and the corresponding turbulent
Schmidt numbers were obtained by matching the measured data
with different models.  Three models based on phenomenological
theories of turbulence were used to analyze the diffusion.
The first one, which assumed constant eddy viscosity and
constant particle eddy diffusivity, gave the best agreement
with the measured data.  The results showed that in general
the contaminant diffuses faster than the momentum and that
the rate of diffusion increases with an increase of particle
size.

3.  In order to compare the measured results with others, a
particle parameter, ^m, originally presented by Householder and
Goldschmidt (1968) and later modified by Ahmadi  (1970), was
adopted as a characterizing parameter.  The present data suggest
that the particle parameter ^T is suitable for describing the
particle motion only within the Stokesian range.  When the
particle Reynolds number is outside this range another modified
parameter ^.j is defined in which the particle response time is
correctly predicted from the simplified B.B.O. Equation in the
corresponding Reynolds number range.

4.  The relationship between the turbulent Schmidt number and
the characteristic parameter, ty^>, is constant at low I|JT values.
When t|>T is large, there seem to be different trends according
to the geometry of the flow fields.

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                      SECTION II

                     RECOMMENDATIONS
This study was limited to the measure of the turbulent transport
coefficient of small contaminants of spherical shape in free
turbulent jet flows.  The results give a direct measure of the
eddy diffusivity coefficient necessary to predict the dispersion
of contaminants when released in such conditions.

To make the study complete it should be extended to consider
the following cases:

1.  Dispersion  in  stratified and disturbed  (crossed, deflected,
etc) flows.

2.  Dispersion of non-spherical contaminants.

3.  Optimization of dispersion by control of particle size
and shape.

4.  Dispersion in flow fields of different geometries.

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                       SECTION III

                      INTRODUCTION
A prediction of the concentration distribution of scalar
contaminants  (such as heat, dye, particles or bubbles) introduced
in a turbulent flow field requires a knowledge of the corres-
ponding turbulent transport coefficients.  This work concerns
itself with the transport of discrete contaminants suspended
in turbulent flows.  The specific questions being answered are:
Is the coefficient describing the turbulent transport of sus-
pended particles equal to that of momentum?  And if it is not,
how does it depend on the size of the particle-contaminant?

The specific set of experiments reported herein are for the
dispersion of gas bubbles in a turbulent water jet.  They were
performed simultaneously with a separately funded study on
the dispersion of liquid droplets in air jets.  In sections IX
and X the results are compared and generalized.  It is shown
that for contaminants with a certain size and specific gravity
range it is not possible to assume equality of the turbulent
fluid and particle transport coefficients.  The results correlate
sufficiently well to permint an estimate of the actual turbulent
transport coefficient for a given contaminant to carrier stream
density ratio, contaminant size, and characteristics of the
turbulent flow.

The stated objectives of this work were twofold.  One to
establish an effective method of tracking contaminants in a
liquid jet, including the use of a laser system.  Two to
determine the diffusion due to turbulence of contaminants of
different size and density.  The second objective was fully
met.  This report deals directly with it.  On the other hand
the first objective was only partly met.  It will be reported
on in a separate report.  The second objective was met through
the research of Dr. Strong C. Chuang.  His doctoral thesis was
completed on August 1970.  The research into the use of a laser
as a sampling device was conducted by Mr. Charles H. Tinsley as
part of his M. S. studies at Purdue University.  His Master's
Thesis is currently (May 1971) in the final write-up stages.
Mr. -Tinsley's research and study program is presently being
financed through university funds.

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                         SECTION IV

                  STATEMENT OF THE PROBLEM
It is well known that a turbulent flow field will not only
transport but also rapidly disperse any material injected in
it.  This is of basic importance in problems related to pollu-
tion and dispersion of contaminants in oceans, lakes, and
rivers as well as the atmosphere and in the transport of
slurries and sediments.

Success of attempts at predicting the extent of dispersion of
injected contaminants so far has been very limited due to the
lack of a simple and yet all-encompassing mathematical model.
Consequently most of the research to date has consisted of
experimental measurement and empirical formulation.  Among
these, Householder (1968)  (references are alphabetically listed
in Section XIII) measured the diffusion of liquid particles in
a two dimensional air jet.  In his experiment the contaminant
particles were much heavier than the carrier stream.  The pre-
sent study is essentially a continuation of Householder's work
where now the diffusion characteristics of gas bubbles in an
axi-symmetric water jet are treated.  In this case the conta-
minants are much lighter than the carrier stream.  The major
purpose is to determine the effect of contaminant particle
size on the diffusion characteristics, be they heavier or
lighter than the carrier stream.

The extension of Householder's measurements was in part sug-
gested by Ahmadi (1970).  In his thesis Ahmadi considered
Householder's data and proposed different methods of predicting
the dependence of the turbulent transport on particle size, as
well as on particle specific gravity.  The measurements reported
in this work will then fill a lack of information on the dis-
persion of particles whose specific gravity is less than one.
The work is then not only a needed extension to Householder's
review but also an added input to a bank of data to substanti-
ate analytical predictions such as Ahmadi's.
                        i
In this work a series of constant size Nitrogen bubbles were
generated at the center of a submerged turbulent axi-symmetric
water jet.  A hot film anemometer sensor was modified to measure
the concentration flux of the bubbles by counting the number of
impactions on the sensor per unit time.  The corresponding con-
centration distributions were compared to predictions of three
different analytical models, based on the phenomenological theo-
ries describing the turbulent flow.  The three models are re-
spectively based on Prandtl's mixing length theory, Taylor's
vorticity transport theory and Reichardt's Inductive theory.
Finally the corresponding eddy viscosity, eddy diffusivity and
turbulent Schmidt number of the bubbles are obtained.

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                        SECTION V

                   LITERATURE REVIEW


The turbulent diffusion of a marked fluid particle   (a particle
of infinitesimal volume) in a homogeneous turbulent flow field
was first described by Taylor (1921) and then by Batchelor
(1949) , Frenkiel (1953) , Roberts  (1957) , Lin  (1960a) and Corrsin
(1962).  The relative dispersion of two marked fluid particles
was studied by Batchelor (1952)  , Roberts (1960) , Corrsin (1962)
and Kraichnan (1966) .

The complications encountered when considering diffusion in a
nonuniform turbulent shear flow have been partly overcome by
Batchelor and Townsend  (1956) , Lin  (1960b)  and Cermak  (1963) .

A general description of turbulent diffusion of a marked fluid
particle requires a knowledge of the Lagrangian correlation
coefficient of such a marked fluid particle.  When the particles
under consideration are distinguishable in their dimensions or
density from the main stream, the analysis will then depend on
the Lagrangian velocity correlations for these particles (Fried-
lander  (1957)).   So far, such a velocity correlation has only
been either qualitatively discussed or quantitatively calcu-
lated.  Such calculations have been through very simplified
models with questionable applicability  (see for instance Tchen
(1947), Shirazi et al  (1967) and Ahmadi (1970)).


                   ANALYTICAL STUDIES

Tchen (1947)  first studied the motion of a spherical particle
in a homogeneous turbulent flow field.  He extended the B.B.O.
equation (Basset, Boussinesq and Oseen Equation, see Hinze
(1959) for the general equation and the significance of each
one of its terms) to the case of a particle in a fluid with
variable velocity.  Corrsin and Lumley  (1956) made further
modifications in order to make the equation applicable to the
motion of a small spherical particle in a turbulent fluid.

Hinze (1959) assumed that the particle is very small so that
the non-linear term in the B.B.O. equation and the viscous drag
due to the pressure gradient are negligible.  Thus, it was
possible to relate the power spectrum of the particle to the
power spectrum of the Lagrangian velocity field.  Levich and
Kuchanov (1967)  made a similar approximation.  In addition they
neglected the unsteady Basset term  (which accounts for the
effect of the previous history of the particle motion from some
original time) and solved the equation for the relative velocity
between the particle and the carrier fluid.  They concluded
that the mean square of the relative velocity is always much
smaller than the mean square velocity of the fluid.

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Shirazi et al  (1967) applied a conditional averaging to reduce
the B.B.O. equation to a stochastic integro-differential
equation with  zero mean.  By assuming that the particle velocity
and the turbulent velocity vectors are uncorrelated, they obtained
specific relationships between the statistical properties of
the particle velocity and the fluid velocity.  Their published
results include relationships for the Lagrangian micro scale,
autocorrelation function, and diffusivity of the particles.

Ahmadi  (1970)  studied the dynamic behavior of a small spherical
particle in a numerically generated two dimensional turbulent
flow field and calculated the particle diffusivity as a function
of particle size and density.  He found that the particle
diffusivity increases with particle size and decreases with
particle density.

                   EXPERIMENTAL STUDIES

Rouse  (1938) performed a basic study in particle diffusion by
measuring the concentration in the vertical direction of sand
particles in which the turbulence was generated in repeating
patterns by mechanical agitation in a cylindrical tank.  He
found that for any particle size, the particle diffusivity
e  is directly proportional to the frequency of agitation;
at low frequencies, Gy is independent of the particle size;
and at high frequencies EY increases with an increase in particle
size.

Kampe de Feriet  (1938) reported diffusion experiments by Dupuit
in a wind tunnel, where soap bubbles about 3 mm in diameter were
used and introduced at a point in the wind tunnel stream.
The concentration of the bubbles passing a plane perpendicular
to the mean flow showed a Gaussian distribution.

Kalinske and Pien  (1944) performed diffusion experiments in
water flowing through a channel at a certain distance from
the bottom and side walls, the turbulent flow there being nearly
isotropic.  Small drops were formed by injecting a mixture
of carbon tetrachloride and benzene of the same density as
the water.  The value of the variance of the displacement
was determined from photographic records.  The concentration
distribution of the droplets passing a plane perpendicular to
the flow at a distance from the point of injection was found
to be very close to Gaussian.  The rough shape of the Lagrangian
correlation coefficient could be well approximated by an empirical
function.

Vanoni  (1946) used sand of geometric mean sieve sizes of
0.147 mm, 0.12 mm and 0.091 mm and found that for coarse sediment
e  is less than the momentum diffusivity em and for fine
sediment e  is greater than em.  The difference in the two eddy

                            10

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diffusivities is due to differences in the possible combinations
of u and v as compared to the combinations of v and Y  , thus
leading to a difference between momentum transfer and  sediment
transfer ( u and v are respectively the longitudinal and lateral
velocity fluctuations and Y is the fluctuation of the  sediment
concentration).  Vanoni argued that during acceleration the
relative velocity between the sediment and the fluid must be
greater than the fall velocity in the quiescent fluid  and thus
the sediment is carried a shorter distance than assumed.  This
tends to make ey less than em.

Carstens (1952) solved the equation of motion of a sphere in
an oscillating fluid, omitting the gravitational force.  For
a motion of the oscillating fluid specified by x=x0 sin cot,
he showed that the motion of the sphere may be described by
xs=xSp sin  (o)t+<|>) , in which  is a phase difference.   By
assuming such an oscillation to be prevailing in a sediment-
laden flow field, he concluded that for sediment particles in
water £y/em can never be greater than 1.  He developed a mathe-
matical expression for the ratio £y/em for an oscillating
spherical particle in a liquid flow field.  It reads:
     fY _  (1+3N/2)2 +  [(3N/2)(1+N)3	
     e_    ~ P_    ,    9ia  2                 2
           (l p  +  I +  T^  +  K3N/2) (1+N)]                  (II-l)


where N =  /8v/(co/d)  ,  an  oscillation  parameter  and w  is  circular
frequency.

Ismail  (1952) performed experiments with  suspended sediment  in
a closed channel.  He  obtained  ey/em=1.5  for  0.1 mm sand and
1.3 for 0.16 mm sand.  Brush  et al  (1965)  applied  corrections
to the fall velocity term and showed  that the values  would be
reduced to 1 and 0.6,  respectively.

Longwell and Weiss (1953) assumed the velocity  fluctuations  to
be sinusoidal functions of time, and  by solving the equation
of motion with certain simplifications they showed that  the
eddy diffusivity of liquid drops in a turbulent gas stream
should be  less than the eddy  diffusivity  of the marked gas
particles.

Laursen (1958) measured the velocity  distribution  and the
sediment concentration distribution for 0.04  mm and 0.1  mm sands.
Without correcting the concentration  by accounting for the actual
fall velocity, and assuming Karman's  K to be  a  constant  and
that the turbulence characteristics were  unchanged by the
particles, he concluded that  £y/em>l.

Smith (1959) investigated the expansion of a  falling  cluster of
particles  in an isotropic homogeneous turbulent flow  field.  He

                            11

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showed that the rate of expansion of the cluster decreases as
the terminal fall velocity increases.

Brush  (1962) studied the diffusion of glass beads in a submerged
axi-symmetric jet in order to compare the characteristics of the
diffusion of sediment with those of momentum in free turbulent
shear flow.  The efflux velocity was maintained at 20 feet per
second to lessen the relative importance of the fall velocity
of the individual particles.  He obtained the corresponding
particle turbulent Schmidt number for different particle sizes.
The following results were obtained:

Particle mean diameter (mm)                 ey/ein

             0.55                           0.15
             0.32                           0.50
             0.19                           1.00
Ho  (1964) found that the fall velocity in an oscillating fluid
was significantly lower than in a still fluid.  Reasonable
values of the settling velocity in an oscillating fluid were
found to be predictable from numerical solutions of the equation
of motion.

Goldschmidt and Eskinazi (1966) measured the concentration
distribution of aerosol droplets in a plane jet of air by
means of a hot wire anemometer.  It was found that the turbulent
diffusivity of the contaminant particles e  varies with the
location in the flow field and that an average value for the
turbulent diffusivity of the droplets (with an average size of
3.3 microns) in a plane jet of air is 0.03U bu, where Um is the
maximum velocity and bu is the half width o? the two dimensional
jet.  A comparison of the velocity and concentration profiles at
various sections of the flow field shows that although the
concentration profiles have spread more than the velocity
profiles, their rate of diffusion is lower.  The average ratio
of ev/Ejn  (inverse of the particle turbulent Schmidt number)
was found to be 0.91.

Baker and Chao (1965) measured the relative velocity of bubbles
in a vertical turbulent conduit.  The size of the bubbles used
ranged from 760 to 7,000 microns.  They concluded that the
bubble relative velocity in a turbulent water stream is similar
to the rise velocity of single bubbles through a quiescent
liquid.

Kennedy  (1965)  measured the dispersion of 1,250 micron soap
bubbles, and 700 and 900 micron polystyrene beads in a grid
generated turbulent air flow.  The following results were
obtained:
                            12

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       Particles

1250.y soap bubbles
70Oy polystyrene beads
900y polystyrene beads
eY/e

1.52
1.42
1.10
m
  Particle-carrier
stream density ratio
        1.41
          39
          39
Singamsetti  (1966) used sand with a geometric mean sieve diameter
of 0.068, 0.115, 0.23, 0.32 and 0.46 mm for measurement of
diffusion in a circular jet of water and obtained the following:
     Particle diameter  (mm)
          0.068
          0.115
          0.23
          0. 32
          0.46
   Particle Reynolds number
               0.4
               1.2
               7.2
                          £Y/£m
                           1.23
                           1.20
                           1.24
              18.0
              33.0
                      1. 35-1.39
                      1.43-1.45
The particle Reynolds number is based on the fall velocity of
the particle in a quiescent infinite fluid.  Singamsetti
concluded from his measurements that  (1) the linear oscillation
model for simulating the turbulent flow field is invalid  for
three dimensional turbulence,  (2) £y/ey0approaches unity  within
the Stokes range. £yo ^s "the diffusivity of the marked fluid parti-
cle and the Stokes range is understood to be that for which
the viscous drag on the spherical particle is given by Stokes
law.  (3) £y/£yO is greater than unity for particle Reynolds
number beyond the Stokes range provided that the fall velocity
is less than the rms value of the turbulent fluctuation in
the direction of fall.

Jones et al (1966) developed a linearized theory based on
the particle displacement rather than the particle velocity
to describe the motion of small particles in a turbulent  flow.
They found that most of the energy of the particle fluctuation
was contained at  lower frequencies  (less than 3 cps) than
that of the carrier fluid (less than 10 cps).  Moreover,
the heavier particles contained more tubulent energy than
the lighter one.

Majumdar and Carstens (1967) used nearly neutrally buoyant
particles in an apparatus restricting the particle motion to
a horizontal plane in a supposedly homogeneous isotropic
turbulent flow field.  The particle diffusion occurs without
mean motion.  The motion of individual particles was recorded
on motion picture film, which was subsequently projected  for
displacement measurements.  The particle displacement data
were analyzed, using the diffusion theory of continuous
movement.  The values of the particle diffusivity, £y, and
particle mixing length, &c, were plotted as a function of
particle diameter, d.  They concluded that
     (1)  if d < &c,eY=eYO:
     (2)  if d >34,c,  EY=O; and
     (3)  ev/ev  continuously decreases in the range l
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Sayre and Chang  (1968) investigated the dispersion process
in a turbulent open channel  flow.  They found that the  longi-
tudinal dispersion process for suspended silt-size sediment
particles differs from the process for a'dissolved dispersant
in that the particles tend to settle toward the slower  moving
flow near the bed and eventually deposit on the bed.  The
lateral dispersion of floating particles  (released from an
intermittent point source at the water surface) can be
represented as a Fickian diffusion process.  However, the
dispersion pattern is somewhat distorted by the effects  of
secondary circulation.

Householder (1968) performed an experiment similar to that of
Goldschmidt and Eskinazi, and found the following dependence
of the particle turbulent Schmidt number on the particle size

     Particle size (microns)                eY/em
           6.4                              2.38
          13.1                              7.70
          16.7                              3.33

Householder and Goldschmidt  (1969) made an extensive review
and unified the available data on dispersion of contaminants
in open channels and circular pipes.  They related the  turbu-
lent Schmidt number to a particle parameter, ip, proportional
to the Stokesian particle response and defined as

            A 2
     * = Re(l)   (

where Re is the Reynolds number,(based on the mean flow  velocity
and a characteristic width of the conduit),d is the particle
diameter, a is the characteristic dimension of the flow  field
and pp and Pf are the density of the particle and carrier
fluid respectively.   They concluded that there is a general
trend towards an increase of particle diffusion with  ty, and
hence particle size.
                            14

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                       SECTION VI

                 THEORETICAL BACKGROUND


MOMENTUM TRANSPORT IN AN AXI-SYMMETRIC JET

Based on the assumptions that  (1) the mean motion is steady,
(2) the flow field is axi- symmetric, and  (3) the turbulent
region is narrow in the radial direction when compared with
the axial direction, the equation of motion of an axi-symme-
tric turbulent jet in the axial direction,  (Appendix I) ,
reads :
where x and r are respectively the coordinates in the axial and
radial directions, U and V are respectively the mean values of
the x and r components of velocity, a   is the Reynolds stress,
and p is the fluid density.  The corresponding boundary condi-
tions are:

                                   \
         r = O:  V = 0;  ^ = 0

         r = oo  :  u = 0            '                    (VI-2)

         conservation of momentum

Equation  (VI-1) together with the equation of mass conservation
and the boundary conditions  (VI-2) can be integrated to give
(Appendix II)
                             n „   _
           pU      n   m Jo        m
             m

where n = r/(x+a).  With n so defined the immediate consequences
of the similarity of the flow field will give  (Appendix II)


          ^5 ' kb 
           m

where a is the distance from the virtual origin to the jet nozzle
plane, U  is the jet efflux velocity, Um is the maximum velocity
at the section of consideration, b  and kb are respectively the
values of r and n where the velocity is half the maximum at the
section of consideration, and k  is the slope of the linear


                           15

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relationship as given in Equation  (VI- 5) .  The Reynolds stress
a   i' expressed as a   = -puv, where u and v are respectively
the fluctaation velocity components in the x and r directions.
In this derivation the "kinematic" and "dynamic" virtual ori-
gins have been assumed to be equivalent.  The experimental
results for the particular jet will confirm this.  In general
(see Flora & Goldschmidt (1969) )  this need not be true.  In
analogy with the coefficient of viscosity in Stokes ' law for
laminar flows, Boussinesq introduced the kinematic eddy vis-
cosity, e , for the Reynolds stress in turbulent flows by
putting
Note that e  accounts only for the turbulent transport.  The
molecular transport is neglected since it is approximately three
orders of magnitude smaller than the transport due to turbulence,
Substituting Equation (VI- 6) into Equation  (VI-3) , the relation
between e  and U/U  reads:
                       -       - <
              m                   __                  (VI-7)
          Vx+a)        n |_ (U_,


An assumption concerning e  has to be made in order to calculate
the velocity distribution.

          First Model:  (Constant Eddy Viscosity)

Prandtl's mixing length hypothesis leads to a simplified expres-
sion for the eddy viscosity (Schlichting (I960)) as follows:

                                  SU
                            = J6
                          'm

In the above & is the mixing length, a length scale related to
the size of the fluid lump in the turbulent flow field.  If it
is further assumed that the dimensions of the lumps of fluid
which move in a transverse direction during turbulent mixing are
of the same order of magnitude as the width of the mixing zone
and that the mixing length is proportional to the half width,
bu/ of the mixing zone then


                   em

Here x denotes a dimensionless constant to be determined exper-
imentally.  From conversation of momentum, Schlichting  (I960)
showed that for a turbulent circular jet
and
                      U
                       m

                           16

-------
Thus from Equations  (VI-8) ,  (VI-9) and  (VI-10) , the kinematic
eddy viscosity  (employing Prandtl's mixing length hypothesis)
becomes a constant value over the whole flow field of a turbulent
jet.  Consequently Equation  (VI-7) can be solved for U/U  .  One
useful form of the solution  (Appendix III) reads:
                                                        m
              U
                         U(x+a)
                                   2
                                   2
                                      ~2
        Second Model :   (Taylor ' s Vorticity Transport Theory)

Equation  (VI-7) states  that if  U  (x+a)  is constant  then  e
would be a function of  n -  Another  form of the  solution, without
adopting the intuitive  assumption given in Equation (VI-8) ,  is
obtained using Taylor's vorticity transport  theory  (Schlichting
(I960)).  Introducing an eddy viscosity based on  the mixing
length of the vorticity transport,  &  ,  such  that
               'm
and
                    U)
                        3U
                        3r
                                                       (VI-12)
                 = Cu
-------
        Third Model:   (Reichardt's Inductive Theory)
Another solution is obtained by applying Reichardt's inductive
theory and transforming Equation  (VI-1) into a diffusion type of
equation  (Hinze  (1959)).  The theory yields an exponential solution:


          §- = e-V2                                   (VI-17)
           m

Substituting Equation  (VI-17) into Equation  (VI-7) the corresponding
eddy viscosity becomes

            em    _ l-e"Kun
          Vx+a)   4K2 n2
                      u

It is worthy to note that the above three models have all been
used in the literature, together with other solutions not reported
herein.  Equations  (VI-11),  (VI-14) and  (VI-17) result from
different models used to obtain an expression relating the Reynolds
stress to the mean flow properties.  Which one of the listed models
is more suitable can only be determined by a comparison with
accurate measurements of the mean velocity and the Reynolds stress
or by an up to now unavailable rigorous formulation for the eddy
viscosity itself.  For comparison purposes all of the models
described will be used in the discussion that follows.

SCALAR QUANTITY TRANSPORT IN AN AXI-SYMMETRIC JET

The equation of transport for a scalar quantity in an axi-symmetric
jet  (Appendix IV) reads:

           8V    3V _ _ 1 3     	
           3x    3r ~~   r 3r     '
where y is the fluctuation component of the scalar quantity.  The
above is limited, again, to  (1) steady mean motion,  (2) an axi-
symmetric flow field,  (3) a narrow turbulent region in the radial
direction when compared with the axial direction, and  (4) neglect
of molecular transport.
Assuming that the turbulent transport of V can be described by
analogy to Pick's law, using a coefficient of diffusivity £y, the
following expression is postulated:

                                                        (VI-20)


Again, as for em, £y doesn't account for the molecular effects.  By
substituting Equation  (VI-20) into Equation  (VI-19) and invoking
conservation of ^, the distribution of the scalar quantity becomes
(Appendix IV):
                           18

-------
v        /    fn   (x+a)um
          -
 m
                                                       (VI-21)
Again, the above expression  implies  the  similarity of the  v -
distribution.  The immediate consequences of the  similarity give
(Appendix IV)
                 Yv   a
        	 — lr   ^ J_ ci\
        D~ ~ Kh  (D + D'


        IT = kY(5" + ^                                 (VI-23)


Where a is the distance from the virtual  source of  the  concentra-
tion to the jet nozzle plane and is  assumed  to be equal to  that
to the virtual origin of  the velocity distribution.  This need not
be the case, it is now assumed  so  strictly for convenience.   "o
is the efflux concentration at  the jet  nozzle, ^"m is the maximum
concentration at the section of consideration, by and k, are  re-
spectively the values of  r and  n where  the concentration is half
the maximum at the section of consideration,  and ky is  the  slope
of the linear relation between  the inverted  centerline  concentration
and the axial distance as given in Equation  (VI-23).

If e  and e  as well as the velocity distribution are known,  then
the Y distribution can be obtained from Equation  (VI-21).   Con-
versely, in the absence of a proper  model for e  , but provided
E  and U/U  are given and Vv   is  measured,  then e  can be  deter-
mined.  Inmthe first part of this  section different models  relating
the eddy viscosity to the mean  flow  properties were discussed.
These in turn gave relationships for U/U  .   In a very similar man-
ner if different models were defined for  e  ,  then a relationship
for VY  would result.  A basic assumption'is now made.  Irrespec-
tive of how e  or e  might vary through the  jet, it is  now  assumed
that the sameYbasismfor describing e will apply toward a descrip-
tion of e .  Hence the three models  of  section A are now employed
to obtain^alternate formulations for Vv  in terms of e and  em-

First Model:  (Constant Eddy Viscosity  and Eddy Diffusivity)

If the velocity profile is assumed as expressed in Equation  (VI-7),
substituting it into Equation  (VI-21),  the concentration distribu-
tion becomes:

             — = exp   f d n  —  i-   in (n-)           (vi-24)
             r>          I       £   cin      u
             x          J o      Y           m
              m
Assuming as in section A  that e and now  e   are constant across
the whole flow field then Equation (VI-24)Ysimplifies to

         Y         £         U  ,   »  ,.  —£
              /U »  m     i  .  m(XTa/  &  ~£  m           /TTT ^c.\
         	 = (:;—) — =   1 +  Q 	 n     —           (VI-25)
         ^m     m   Y            m          Y

                           19

-------
    Second Model:   (Taylor's Vorticity Transport  Theory)
If the velocity profile is calculated according to- Taylor's
modified vorticity transport theory and the  eddy  diffusivity  is
expressed as
              y
U (x+a)   Cy
           m
Ir
                                                        (VI-26)
     m
then substitution of Equations  (VI-14) and  (VI-26)  into Equation
 (VI-21) yields a solution of V/Vm in the  form:



                              o        ao   7/0   2a_
'    :    f  f* , .  l/2n*1/2 -faln*2 t B2"*   -  -IJ
— = .; exp      dn*  ——!	•	
Vm   l       °           3           3/2   9a3  3
                      - | a1 + 3a2n* 7	2^            (VI-27)


where n* is as defined in Equation  (VI-15).

         Third Model:   (Reichardt's Inductive Theory)

The velocity profile based on Reichardt's inductive  theory  is
given in Equation  (VI-17).  Substituting  now Equation  (VI-17)  into
Equation (VI-21)  and expressing Um(x+a) in  terms of  the eddy vis-
cosity as given in Equation  (VI-7), the final solution for  the
concentration profile reads:



          — = exp I - -H K n2 'v                          (VI-28)
          Y            v

Hereafter,  Equations  (VI-25), (VI-27) and (VI-28) will be referred
to as the first,  second and third proposed  models respectively.
To obtain the dependence of the dimensionless parameter Em/Ey'
which Is defined as the turbulent Schmidt number, S^., on the con-
taminant particle size is the major objective of this work.  Its
value will.be found from measured concentration  flux distributions
and equations (VI-25),  (VI-27) or .(VI-28)..
                            20

-------
                       SECTION VII

     EXPERIMENTAL SETUP AND MEASUREMENT PRINCIPLES


The main purpose of the experimental part of this work is the
measurement of the concentration distribution of bubbles in
an axi-symmetric jet.  The basic setup employs a submerged
axi-symmetric water jet as the flow field, a series of constant
size bubbles generated through a capillary tube placed at
the center of the mouth of the jet as the contaminant, and a
hot film sensor as the bubble concentration flux sampler.
The experimental equipment and the measurement procedures are
described in more detail in the following sections.

JET PLOW FIELD

Axi-symmetric Turbulent Water Jet

A schematic diagram of the experimental setup is shown in
Figure 1.  The system consists of a constant head tank, a
jet tank, a reservoir, a pump and a water filter.  The constant
head tank has an adjustable elevation permitting changes of
the jet efflux velocity.  In addition, two interchangeable
nozzle contracting sections, of 1/4 and 1/2 inch diameter,
permit further variation of the efflux velocity of the submerged
jet.  The maximum jet velocity reached with the non-metallic
1/4 HP pump and a Cuno Model SS-8 super flow water filter is
20 feet per second.  This corresponds to a Reynolds number
based on the jet nozzle diameter in the order of 8X10^.
Figure 2 shows the constant head tank, water filter and pump.
A deionizer, also shown in Figure 2, is used to treat the
water introduced into the flow system.

The entire flow system is mounted on a level steel frame
structure.  Figure 3 shows a photograph of the jet tank.  It
is rectangular in shape to permit optical inspection of the
flow field.  The top edge of the side wall serves as an over-
flowing weir so as to maintain a constant water level inside
the jet tank.  The side gutter which is attached to the outside
of the tank wall collects the overflow water and returns it
to the reservoir.  The overall dimensions of the tank are
18"xl8"x25" in height.  The jet tank provides a turbulent jet
flow field with an axial distance of up to 40 jet diameters
when the 1/2 inch nozzle is in use.  A traversing mechanism is
included to be able to position the measuring probe in the
jet.  As designed, it allows variations in position in the
longitudinal, transverse and vertical directions.

Velocity Measuring System

The mean velocity component of the turbulent water jet was
measured with a straight-leg Prandtl-type Pitot-static tube

                           21

-------
                                           ELSZOTHOrJIC  INSTRUMENTS
                ELEVATED



                 TANK
                                              TRAVERSING MECHANISM
                                          NGZNTRATION PROFILE
      NITROGEN



        TANK
                                        \\\\\\\\\\\
FIG.  1  SCHISMATIC DIAGRAM OF EXPERIMENTAL EQUIPMENT
                             22

-------
                                           HEAD
                                           TANK
                                          NITROGEN
                                            TANK
FIG. 2 CONSTANT HEAD TANK. WATER  FILTER,DEIONIZKK

-------
TRAVERSING
MECHANISM
    JET TANK
  SUPPORTING
   FRAME
    FIG    3      PHOTOGRAPH   OF   JET   TANK

-------
 and checked with the hot film anemometer.   The pitot tube used
 has an  outside diameter of 3/32  inch and a dynamic tap opening
 of 1/32 inch.   Two lines of 4 mm inside diameter tygon tubings
 were connected from the pitot tube to a differential manometer.
 The indicating fluid of the manometer was  Meriam No. D-8325  fluid
 with a  specific gravity equal to 1.75.

 The speed of reading depends on  the length and the diameter
 of the  pressure passages inside  the probe, the size and the
 length  of the pressure tubes to  the manometer, and the dis-
 placement volume of the manometer.  The time constant in this
 system  was found to be in the order of a few seconds.

 The mean velocity measurement was also checked by a TSI 12l7-20w,
(Thermo  Systems Inc., 2500 Cleveland Ave.,  N.  Saint Paul,
 Minnesota 55113)  quartz coated hot film and TSI 1050 anemometer
 with TSI 1025  Temperature Compensator in series.   The axial
 fluctuation velocity components  were also  measured with the
 same hot film sensor.

 BUBBLE  GENERATION

 Generation of a more or less uniform series of air bubbles is
 possible when supplying a constant air pressure to a small
 tube submerged in the  water.   The intent was to generate
 bubbles and introduce  them upstream of the jet mouth in order
 to permit the  study of their undisturbed motion in the
 turbulent jet.   The objective was fulfilled with the system
 shown in Figure 1.   A  long glass tube,  drawn to a small diameter
 nozzle  at the  tip was  introduced at the base of the jet tank.
 Use of  a constant pressure nitrogen source (filtered and
 carefully regulated)  resulted in bubbles being generated
 slightly upstream of the jet mouth.

 The sizes of the  syringe tubes used were very small when compared
 with the jet nozzle.   The outside diameter of the capillary
 tubes used was less than.120  microns.   (The ratio of the tube
 cross sectional area to the jet  nozzle  opening  area is
 correspondingly less than 10~4.)    The  fragile nature  of the
 glass nozzles  caused frequent breakage.  The smallest  one used
 had a tip inside  diameter of 13.6 microns, and the largest
 one used had a tip inside diameter of 96 microns.

 An analytical  and experimental study of bubble formation due
 to a submerged capillary tube in quiescent and co-flowing streams
 has been made,  and published (Chuang and Goldschmidt (1970)).
 An abstract is included in the Appendix of Section XVI.

CONCENTRATION  FLUX MEASURING  SYSTEM

 Several techniques  for measuring the concentration of  the
 bubbles were considered (such as a laser sampling device,

                           25

-------
photographic techniques and hot film anemometer sampler).
The use of the laser system is discussed in a separate report.
The hot film anemometer system was selected in this first
phase of the work as the bubble concentration sampler primarily
because of its availability.  The method described herein was
originally developed by Goldschmidt (1965)  and then modified
by Goldschmidt and Householder (1969)  for the diffusion
measurement of oil aerosols in a two dimensional air jet.

The applicability of the hot film anemometer for the bubble
in water measurement was first described by Hsu et al (1963)
and then by Delhaye (1969)  and Chuang   and Goldschmidt (1969).
The principles and the techniques for the application of the
hot film sensor to bubble concentration measurement are
described in the following.

    Principle

The. mean concentration of the bubbles at a certain position of
an axi-symmetric turbulent jet can be obtained by knowing the
mean concentration flux and mean velocity component at that
location.  The mean concentration flux is measured by counting
the number of bubbles impacting on a hot film sensor.  The
heated sensor of a hot film anemometer when  placed in a
turbulent water stream contaminated with gas bubbles will
suffer unsteady cooling due to the carrier stream velocity
fluctuations and the low heat capacity gas bubbles which
impact on the sensor.   The response of the hot film anemometer
to a bubble in a laminar water stream has been extensively
discussed and is given in Chuang and Goldschmidt (1969).,
(see section XVI).

By discrimination,  either through frequency filters or amplitude
discriminators, the decrease of the cooling signal due to
the impaction of the gas bubbles may be isolated and measured.
Since the characteristic frequency of the bubble impaction
signal is above 1 KHz and most of the turbulent energy of the
carrier stream is below 1 KHz, frequency discrimination was
adopted.

The possible errors due to the uncertainty in the impaction
coefficient caused by the curving pathlines around the
cylindrical sensor are noted in Section VIII.

    Frequency Discrimination

In order to use the hot film anemometer as a bubble sampler
in a turbulent flow field, it is necessary to frequency dis-
criminate the decrease of the cooling signal from the impacting
bubble.  The electronics used to accomplish this are shown in
Figure 7.  The band pass filter was set at the analyzing
frequency where the impacting signal has the highest energy
density.  Discrimination is then possible provided that most
of the energy due to the turbulent cooling of the fluid lies
at values of frequency below that selected.  It is desired,

                           26

-------
then, to first determine the energy spectrum of the signal  for
a single bubble impaction.

By harmonic analysis a bubble impaction signal can be transformed
from a time-dependent  function into a frequency-dependent
function, namely the energy density function.  Let e(t) be  a
random time-dependent function such that e(t)=0 for t-j_>t and
t2) = t-  I 2   e(t) e~ia)t dt = ~  I 2 e (t)  (cos wt - isinwt)dt

                                                            (VII-2)
                              = ~  I
                                ^  Jt
the energy density is then defined as
 g(u») | 2 = i-«-/  f  I 2 e(t) coswtdt 2 + f  f 2 e(t) sin wt dtl
     1     4lT  /  L  Jt,             )    I   Jt,               1
                                                            2
                                                            (VII-3)

The bubble impaction signal was obtained  from the TSI  constant
temperature anemometer and displayed on a Tektronix Type  564
Storage Oscilloscope.  A photograph of the cooling signal
was then taken with a polaroid camera.  The resulting  photo-
graph was digitized and a numerical integration of Equation
(VII-3) was performed.

The energy density function of the cooling signal due  to  a
bubble of about 500 microns in diameter approaching the sensor
at 3.5 fps is shown in Figure 4.  The over heat ratio  of  the
sensor was 1.1, the same as that used in  the actual concentra-
tion flux measurements.  Figure 4 shows that the bubble signal
energy is a maximum at 1.'8 KHz.  This frequency is well above
the maximum frequency for the turbulence  energy in an  axi-
symmetric turbulent water jet  (discussed  in the next chapter) .

It was then decided to set up a frequeccy band between 1.5 and
2.2 KHz for the concentration flux measurements in such a
manner. that all frequencies below 1.5 KHz and above 2.2 KHz
were cut off.

All of the electronic components are linear in their response
to a signal with the exception perhaps of the band pass filter.
To ascertain that the band pass filter did not introduce  any
non-linearity, a calibration of the filtered output e  f compared


                           27

-------
oo
                                  1.2     1.6     2.0
                                        frequency,  KHz
                       FIG.  4  ENERGY DISTRIBUTION OF BUBBLE SIGNAL

-------
to the unfiltered input e  was made for this band pass setting.
Figure 5 exhibits the expected linearity.  Similar results at
other band pass settings had been found by Householder (1968)
for the same equipment.

The output of the filtered and the un-filtered cooling signal
on a sensor in a bubble contaminated turbulent water stream
is shown in Figure 6.  The upper trace is the filtered signal
and the lower trace is the unfiltered signal.  It is seen
that the low frequency turbulent signals have been properly
filtered.

    Counting

The components of the system are a hot film anemometer, a
tunable band pass filter, an  AC amplifier, a Schmitt trigger,
and an electronic counter.  Due to the active components of
the filter, the output is oscillatory as shown in Figure 6.
To eliminate erroneous multiple counts from a single bubble
impaction, the decaying oscillatory signal was fed to a Schmitt
trigger, the output of which was just longer in duration than
the oscillatory signal.  The trigger, in turn, when provided
with an adjustable gate, was used for amplitude sampling.
The output from the Schmitt circuit was fed to an electronic
counter which recorded the rate of bubbles hitting the sensor
and causing a decrease of the cooling signal larger than the
trigger level of the Schmitt  circuit.

    Equipment

The block diagram of the system is shown in Figure 7-  The
specific components used in this system are shown in Figure 8.
Their specifications follow:

TSI Constant Temperature Anemometer, Type 1050
     Frequency response:  0-400 KHz
     Output noise level:  corresponding to less than 0.02%
                          turbulent intensity
     Stability:  drift less than 2 microvolts per °F and less
                 than 2,0 microvolts in 24 hours.
TSI Model 1217-20w Quartz Coated Cylindrical Hot Film
     Sensing size:  0.002" diameter, 0.02" long
     Relative frequency response:  40 KHz
     Nominal resistance:  4-8 Ohms
Hewlett Packard Model 450A Amplifier
     Frequency response:  20+ 1/2 db, 5 Hz to 1 meg. Hz
Kron-Hite Band Pass Filter, Model 310C
     Frequency range:  20 Hz to 200 KHz
     Attenuation slope:  24 db per octave
Tektronix Oscilloscope, Type 564 Storage Scope with Type
2B67 Time Base
     Gate width:  adjustable from 10 micro sec. to 50 sec.
     Trigger level:  adjustable from 0.002 to 160 volts


                           29

-------
  0.5
to
.p
r-l
O
CO





H

£0.1

 «-<
 O.
O
                                                                o
                                                               •o-
0.2
                                    0.^              0.6

                             unfiltered  peak voltages  (volts)
0.8
IX)
                   PIG.  5  FILTERED vs UNPILTERED PEAK VOLTAGES

-------
                           0.5 MJ  Ptfi OfV,
               o HOT FILM
                  SENSOR

ANEMOMETER



1.5 TO £.E KHZ
BAND PASS FILTER

SIGNAL 1

                                                           SI6NAL I
BUMLES IN THE STREAM
      FIG.
FILTERED AND  UNFILTERED  SIGNALS
                                31

-------
 HOT  FILM




ANEMOMETER
 20-30 DB




AMPLIFIER
BAND PASS




  FILTER
SCHMITT





TRIGGER
ELECTRONIC





  COUNTER
                     FIG.  7  BLOCK DIAGRAM OF ELECTRONIC  INSTRUMENTATION

-------
             c r kiftJIT T
STROBOSCOPE            TIMER
             TRIGGER
AMPLIFIER
OSCILLATOR
                                          -   COMPENSATOR
        PIC.  8  ELECTRONIC INSRUMENTATIGN

-------
Hewlett Packard Electronic Counter, Model H22-5211B
     Maximum counting rate:  300 KHz
     Number of digits:  4
     Time base accuracy:  +0.1%

Other Instrumentation

Other supplementary instruments were used while measuring the
fluctuation components of the velocity field,  the energy
spectrum, and the frequency of bubble generation.   They are
itemized in the following:"

     Bruel & Kjaer Frequency Analyzer, Type 2107
     Dana DC Amplifier Model 2000
     Hewlett Packard 200 CD Wide Range Oscillator
     Hewlett Packard Vacumm Tube Voltmeter, Type 400 AB
     Honeywell Accudata 105 Gage Control Unit
     Honeywell Accudata 120 DC Amplifier
     Honeywell Visicorder Oscillograph Model 2106
     TSI Model 1025 Temperature Compensator
     TSI Model 1125 Calibrator
     General Radio Electronic Stroboscope, Type 1531-A
     General Radio Strobolume, Type 1532-B
     Dimco-Gray Model 172 Timer
     American Optic Model 371734 Long Focusing Distance Microscope
     Nikorex 35 mm Camera.
                          34

-------
                      SECTION VIII


                   EXPERIMENTAL RESULTS
Mean velocity profiles in subsonic axi-symmetric jets have
been widely investigated, for instance Kuethe (1935),
Corrsin (1943) , Squire and Trouncer  (1944) , Hinze and Van
Der Hegge Zijnen  (1948) , Albertson et al  (1948) , Keagy and
Weller  (1949) , Corrsin and Uberoi  (1949), Trentacoste and
Sforza  (1967) in air jets and Binnie (1942), Forstall and
Gaylord (1955), and Liu  (1967) in water jets.  In general,
there is a satisfactory agreement among the experimental
results obtained by the various investigators.  For axial
coordinate x greater than the length of the potential core
x  (as defined in Appendix II), the following are observed:
(I) radial distributions showing good similarity in con-
secutive sections,  (2) a linear spread of the jet, and (3)
a hyperbolic decrease of the jet center-line velocity with
distance from some apparent source.  These three character-
istics have been already noted in Section VI.

The jet flow field used in this experiment is somewhat dif-
ferent from the ordinary jet in that there is a bubble
generating capillary tube in the center of the jet nozzle.
Hence the well known characteristic of the jet mean flow
field obtained by the previous workers probably is not
applicable to this specific jet flow.  An actual flow field
measurement becomes a necessity.
MEAN VELOCITY PROFILE MEASUREMENT AND ITS CHARACTERISTICS
                    Measured Results

The axial velocity profiles were measured with a pitot
static tube and checked with a hot film anemometer.  The
efflux velocity of the jet was 10.83 feet per second.
The corresponding Reynolds number was 45,000, based on
orifice diameter.  The velocity profiles were measured
at x/D =10, 15, 20, 25 and 30.  Figure 9 shows a plot of
U/U  versus n, where r\ is the dimensionless variable defined
in Sppendix II as r/(x+a).  The assumed similarity is con-
firmed.  The predicted curves shown in Figure 9 will be
further discussed in a later part of this section.
                            35

-------
o.9
0.8
O.V
0.6
0-5
0.4
0.2
O.I
o




X




A




D



O
                15




                20




                25



                30
                0-04
                      0.06



                       I
0.12
0.16
      FIG.  9  NORMALIZED VELOCITY PROFILE  (WITH SYRINGE  TUBE)

-------
The corresponding half width, b , and center line velocity
decay, (V /UQ)-I, are shown in figures 10 and 11.  The
half width, as defined in Equation (VI-4) follows the re-
lationship
              ^u = 0.0952  (£ + 0.8)                   (VIII-1)
               D


for the pitot tube measurement and
              bu = 0.0978  (£ + 0.5)                   (VIII-2)
              ~            D
for the hot film measurement.

The possible error due to the pitot tube as a mean velocity
measuring device is found to be negligible.  The detailed
analysis of the error due to the hot film anemometer as a
mean velocity measuring device has not been investigated
here.  Intuitively, a hot film sensor will sense the total
velocity component,  / 2    2, instead of only the axial
velocity component.  At the half width location the ratio
of the radial to the axial mean velocity component reaches
its maximum of about 3 percent and this will cause a posi-
tive error in the axial mean velocity reading.  Further-
more, the radial and the tangential fluctuation components
will also give a positive error in the axial mean velocity
reading (Heskestad (1965)).  For these reasons the coeffi-
cient of the jet widening rate given in Equation (VIII-2)
appears to be larger than the coefficient given in Equation
VIII-1).  It is felt that Equation (VIII-1) should be the
more accurate of the two.

From the principle of momentum conservation, the axial
velocity component along the jet axis should decrease
hyperbolically.  This was noted in Equation (VI-5).
Figure 11 shows the linear relationship of (Um/UQ)-l
versus x/D.  The best fit linear relationship reads:
                           37

-------
U)
CD
                2.
            b
             u
            D
                                                                         /.
                                                                           A
                         -^-0.09?8(x/D-»-0.5)—Hot Film
                                                  -^-0.0952(x/D-»-0.8)—Pltot Tube
                                                    o      Pitot Tube Measurement
                                                —-o-—  Hot Film Measurement
                                     10
                                                 X/D
20
30
                    PIG.  10  VELOCITY HALF WIDTH  (WITH SYRINGE TUBE)

-------
               6.
U)
vO
Um  3-
               2.
                                                 o  Pitot Tube Measurement
                                                 o  Hot Film Measurement
                                  10                 20                 30                40
                                                   x/D

                       FIG.  11   VELOCITY DISTRIBUTION ALONG JET AXIS (WITH SYRINGE TUBE)

-------
            Ul"1 = 0.1626 (  + 0.8)                   (VIII-3)
b  = 0.0806 (  + 0.6)
      = 0.1562 (- + 0.6)
for both the pitot tube and the hot film measurements.

Equations (VIII-1) through (VIII-3) are the empirical
results describing the axi-symmetric jet in which the
dispersion experiments will be performed.  It is in-
teresting to compare these results with those for the
jet flow without the syringe tube.  The results are
shown in Figures 12 through 14.  The corresponding
relationships are

         =p- = [ 1 + 63. 8n2] ~2                         (VIII-4)
          m

                                                       (VIII-5)
                                                       (VIII-6)
Equation (VIII-4) is the relationship obtained by Hinze
and Van Der Hegge Zijnen (1949) which agrees very well
with the present measurements.  The curve given by Equa-
tion (VIII-4) is also shown in Figure 12.

The results show that the presence of the syringe tube
has little effect on the virtual origins, but it does
cause a faster spreading of the half width and a faster
decreasing of the axial velocity in the jet.

In table 1 the characteristics of the submerged jet
used in this experiment are compared with those of other
investigators .

Comparison with proposed Models for Mean Velocity Profiles:

Three phenomenological models were proposed in Section VI
for describing the jet mean velocity field.  These resulted
in Equations, (VI-11),  (VI-14) and (VI-17) .  The measured
mean velocity profiles will be used to calculate the
diffusion coefficient.  Consequently they should be compared
to the analytical predictions.

The axial velocity profile from the first proposed model
with e  constant everywhere is given in Equation • (VI-11) .
The constant coefficient U  (x+a)/8e , obtained by mini-
mizing the mean square error of the measured data fitted
to this model is found to be 46.02.  The corresponding
                           40

-------
Table  1    Comparison of Various Axi-synmetrlc Turbulent Jet Measurements
Half Width Virtual Origin
Author Soreading Eased on the
Coefficient ^b Half Width
(see Sq.EI-'O Spreading
Keathe
(1935)
Squire 4 Irouncer
(19W)
Hinze 4 Van Der
Hegge Zijnen
(19<*S)
Albertson et al
(19^8)
Kea^ry & Weller
(19^9)
Corrsin & Uberoi
(1950)
Porstall & Gaylord
(1955)
Trentacoste &
Sforza. (1966)
With
Syringe
Present Tube
Study Without
Syringe
lube
0.068 l».^D
0.0906 3.6
0.0826 0.6D
0.0956
0.0638 0
0.085 0
0.0920 o
0.093 -1.2D
0.0952 0.8D
0.0973 0.5D
0.0806 0.6D
Center Line
Vel. Decaying
Rate ^u
(See Eq. UI-5)
-
0.1506
0.1563
0.1612
0.1722
0.1^8
0.161
0.1^3
0.1626
0.1626
0.1562
Virtual i
Based on
Center L:
Vel. Dec!
-
3.4
0.6D
-
0
0
0
-1.2D
0.8D
0.8D
0.6D
Core       Reynolds
Length      ,  .
            Number
                                                                                 Remark
                                                                                 Air Jet
                                                                                 Alr
                                                                     6.7(10")    Air Jet
                                                           6.20     2-10(10*)    Alr Jet
                                                                                 Air Jet
                                                           6.0D      5-5(10")    Alr Jet
                                                                       'H10'*)   water Jet
                                                           7-OD          -       Air Jet
                                                                            )   Water Jet
                                                                                (Pitot Tube)
                                                                            )   (Hot Film)
                                                                                (Pitot Tube)

-------
                                                       0.16
FIG. 12  NORMALIZED VELOCITY PROFILE (WITHOUT SYRINGE TUBE)

-------
1.
                          0.8)
            (Equation (V-l))
-^-0.0806(x/D+0.6)
                                    o     Without Syringe Tube



                                    	 With Syringe Tube
                     10
    20
                                r/D
        FIG. 13   VELOCITY HALF WIDTH  (WITHOUT SYRINGE  TUBE )

-------
2.
1.
    Without Syringe Tube




    With Syringe Tube
                    10
20
  PIG. 1>  VELOCITY DISTRIBUTION ALONG  JET AXIS (WITHOUT SYRINGE TUBE)

-------
constant eddy viscosity, e , is then equal to 0.0027U
(x+a) and the resulting velocity profile reads:
         !L- = (1 + 46.02n2)"2                         (VIII-7)
          m

The similar regression procedure applied to the secon
proposed model yields a numerical coefficient  (C /2)~
equal' to 11.8 and a velocity profile given by   w

U_ = 1-2/2 (11.8n)3/2 + 11 (11. 8n)- 1363/2  (11.8n)9/2
   -                    81          6123673
                                                      (VIII-8)

Similarily, the third proposed model gives:


          U  _   -73.04n2                             (VIII-9)
The analytical curves given in Equations  (VIII-7) through
(VIII-9) are plotted together with the measured data in
Figure 9 .  It is seen that the velocity profile given by
Equation (VIII-7) fits the experiment data best of all.

As discussed in Chapter VI, the corresponding eddy viscos-
ities e  for the second and third models are not constant
in the rlow field.  They depend on TI as described in
Equation (VI-16) and (VI-18) , respectively.  Figure 15
depicts the dependence of e  on n in this particular jet
flow measurement as inferrea for the three different models.


FLUCTUATION VELOCITY MEASUREMENT

Since the velocity components in a turbulent jet flow field
are random functions of space and time, it would be necessary
to measure moments and cross moments of all orders to under-
stand the whole statistics of the flow field.  In this study
only the rms value of the axial fluctuation component was
measured.

The sensor was calibrated in the potential core of the water
jet.  The calibration curve is shown in Figure 16.  From
Figure 16 the corresponding sensitivity S  , the slope of the
calibration curve which is directly measured from the cali-
bration curve, can be obtained.  It is shown in Figure 17.
                                          — o"            o
The fluctuation level is then defined as /e /S  where /e
is the rms value of the fluctuation voltage output.  The
axial turbulent levels were measured at x/D = 10, 15, 20,
and 25.  The data are shown in Figure 18.  It is seen that
the turbulent levels at each section are approximately similar

                           45

-------
      .004
      .003  •
                         First Model
                         (constant eddy viscosity)
                         Second Model  (Eq.  M-16)
                         Third Model  (Eq.  m-18)
                 .02
FIG. 15  DISTRIBUTION  OF EDDY VISCOSITY BASED ON DIFFERENT MODELS

-------
   E
(volts)
                                                 o   pre-callbration

                                                 «   post-calibration
                                                                            8
                                          U (fps)
                          FIG. 16  SENSOR CALIBRATION CURVE

-------
           0.9
           0.8
           0.?
           0.6
sensitivity
    
-------
NO
               0.3
           u
            m
               0.2
               0.1







1
"



















1 I '6
A o °
.. A
o ° V o *
A **


o ' * '
O O
O ° 0
A A « A
A A A Q A
0 A
0 0
a
A 0 °
0oO * 0

„ o *
o ••»
0 ° A x^
A /
/ .. <
a / X ""x.
• O/ •** *"*
o / ^
/ /'
• * /•/
t£>
If
tf — — x/D
a //^ _^. X/D
/A ^ x/D
/ a x/D
a/ ° A x/D
.• a/^A- o ' :-:/D
er'/^\ . i
-2.0 -1.0

O A
b °a 0 «
a 0
m
-^-^
O N,^0 A
> \0
_.•••***•• V.
X 'x. \
-X_..,V \\A° 0
\ \ M
\\A > 0
*mP\
\ \
• \ ^J
•.\
S\ o •
V °
* 10 Corrslh ° x\
= 20 Corrsln A \
= 10 A
= 15 o A\o
= l°5 ° V ^
^ A ^\
f . •! . £»\ \
0 1.0 2.0
r/b..
                     FIG.  18  TRANSVERSE  DISTRIBUTION  OF  TURBULENCE  INTENSITIES

-------
in shape and have the maxima at r/b  about equal to
± 0.5 to ± 0.8.  The measured turbulent levels reveal
that there is a trend of increasing turbulence level
along the axial direction.

The results of air jet turbulence level distribution
measured by Corrsin (1943) for x/D = 10 and 20 are also
shown in Figure 18.  It is seen that the turbulence level
obtained from the present measurement is higher than
Corrsin's results.


ENERGY SPECTRUM AND TURBULENT SCALES

Experimentally the energy spectrum is obtained by taking
                                               2
the ratio of the mean square voltage response ef at a
particular frequency band centered at a_frequency f to the
total mean square fluctuation voltage  2 of the sensor out-
put divided by the effective band widtn of the filter  (Curtis
(I960)).  Energy spectra were obtained from measurements per-
formed at stations with x/D=10, 20, and 30 along the jet axis.
The resulting curves^are plotted in a normalized form as F(K)
versus K such that / F(K)dK = 1 where K is the wave number and
is defined as K = 2-irr/U, where f is the frequency and U is the
mean velocity at the measurement location.  Figure 19 shows
such plots.  The procedure for making energy spectrum measure-
ments was the following:

     a.  Determined the characteristics of the wave
         analyzer used  (General Radio Type 1900-A
         Wave Analyzer) by feeding in a known fre-
         quency sine wave signal and measuring the
         output of the wave analyzer at various
         center frequencies,*/  2.  The attenuation
                               f     f  ~~2   ~~2
         factor, which is defined as    efdf/e , was
         then calculated and found to-'Be equal to 5.17.
     b.  The turbulent signal was then fed into the wave
         analyzer and the output at various center fre-
         quencies  2 was measured.  With it  2 was cal-

         culated.  The normalized energy specixum F  (f)
         is then defined as  2/,_ ,_ 2 where  2 is the
                            e.e  (5.17e        e
         total fluctuation energy and was simultaneously
         measured through a Br'uel and Kjaer Wave Analyzer.

     c.  The measured data were then plotted as F(f) versus
         f.  The total area under the F(f) curve should be
         equal to unity.  If not, another correction factor
         is obtained and the values of F(f) corrected through
         this factor.
                           50

-------
      0.05
F'K)
(ft)
      0.01-
20
                                                                           160
ISO
               FIG. 19  ENERGY SPECTRUM ALONG CENTER LINE OF THE JET

-------
     d.  The curves were then changed to F(K) versus K,
         where K is as previously defined and F(K) =
        _— F(f).  The resulting curves of F(K) versus
         K are shown in Figure 19.

The longitudinal macro scale of the turbulence, defined
as

         A  = £ lira F(K)                                (VIII-10)
          x   2 K+0

can be calculated from Figure 19.  Figure 20 shows the
plot-of A /D versus x/D.  The longitudinal macro scale
increases linearly along the jet axial direction, fol-
lowing the approximate relationship

         A                                              (VIII-11)
         £*- = 0.0492 (*- + 2.5)


Comparing Fig. 20 with Fig. 13 shows that the longi-
tudinal macro scale along the jet axis is approximately
half the value of the half width b , and follows the ex-
pected linear growth.             u
CONCENTRATION FLUX MEASUREMENT

In this experiment the efflux velocity of the turbulent
water jet was 10.83 feet per second.  The generated bub-
bles were measured directly through a microscope for four
different sets of runs.  When the stroboscopic illumin-
ation frequency is synchronized with the bubble generation
frequency, the generated series of bubbles will appear
stationary.  Their size can then be measured by a micro-
scope placed outside the jet tank.  The corresponding
average bubble sizes were 343, 527, 780 and 970 microns
with a standard deviation of less than 15 percent.

As described in Section VII the mean concentration flux
is obtained by counting the number of bubble impactions on
a cylindrical hot film sensor.  If A  is the upstream
cross sectional area containing bubbles ultimately touch-
ing the cylindrical hot film, * the actual number of
bubbles per unit volume of the flow field at the measuring
location, and V,  the mean bubble velocity at this locationi,
the concentration flux measured will be N=VV].jAs.  Theore- /
tically AS is related to the impaction coefficient (defined
as the ratio of the area containing particles touching the
collector to the frontal area of the collector) and is not
a constant value with velocity.  Householder (1968) made
an extensive study of the impaction coefficient by assuming
that the particle trajectory in the vicinity of a cylind-
rical collector is governed by the particle inertial and
                           52

-------
       2.0
Ax
 D
       1.6  -
       1.2  -
       0.9  -
       0.4  -
                     •  = 0.0492r*2.5)
                               10
20
30
   FIG.  20  LONGITUDINAL MACRO SCALE ALONG THE TURBULENT JET AXIS

-------
viscous forces only.  He further assumed that the stream
flow field is not affected by the presence of the parti-
cles.  He obtained a solution for two extreme cases.  The
first case is when the Reynolds number is extremely low
such that the stream is solely viscous flow; and the
second case is when the Reynolds number is very high and
the stream is assumed non-viscous.  He went further by
empirically extrapolating two solutions into the middle
Reynolds number range by fitting a model simultaneously
satisfying the two extreme cases.  It is attempted here,
by applying such results, to predict the possible cor-
rection on the intercepting area A  at the different
locations of the flow field.  In tnis work the range of
the carrier stream velocity in the axi-symmetric water
jet within which the bubble concentration flux measurements
are performed is from 1.4 to 7 feet per second, and the
corresponding range of the collector Reynolds number is
from 24 to 120 based on sensor diameter.  Based on the
reported results the maximum difference in the impaction
coefficient would then be less than 2 percent.  This error
is within the accuracy of the concentration flux measuring
system and any correction in the impaction coefficient
was neglected.

If the impaction coefficient is then assumed constant
in the whole flow field and if furthermore the partial
hit effect is similar throughout, then for e/ep fixed
the intercepting area, A ,within which every bubble hitting
the sensor will give a signal perceptible by the meas-
uring system will be constant.  e and e  are as defined
in the Appendix; for all sets of measurlments e/e  was
fixed to be 0.15.                                p

The absolute concentration flux was measured by two dif-
ferent means.  First the flux over a whole cross section
was measured at the jet nozzle by counting the number of
bubbles generated per unit time.  This was achieved by
snychronizing the bubble generation frequency with a
stroboscope.  Second the actual concentration flux meas-
urements were integrated over a whole cross sectional
area assuming an impaction coefficient and neglecting
partial hit effects.  The actual wire sampling area was
6.5xlO~4cm2_ " A count of 200/min. on the counter would
then correspond to a concentration flux of 4.8xl05 counts
per ft2 per second.
                            54

-------
                          TABLE 2

       Total Bubble Concentration of the Experiments
Diffusion
Experiments
                     N (Erflux bubble rate,l/sec.)
by Stroboscope
Measurement
by Hot Film
Measurement
Efflux Volume
Concentration
  (percent)
343y
527y
780y
970y
case
case
case
case
9
6
4
3
.64x10
.26x10
.24x10
.41x10
3
3
3
3
11
5
4
2
.13x10
.93x10
.02x10
.97x10
3
3
3
3
0
0
0
0
.048
.116
.252
.390
The concentration flux was measured at x/D=10, 15, 20 and
25.  All the data were obtained in a form of N versus r.
The data so obtained were normalized in terms of N .

        Check for Bubble Coalescence and/or Breakage

If there is neither bubble breakage nor bubble coalescence,
the conservation of mass requires that at each successive
section the following relation must be satisfied:
         N r dr = M                                     (VIII-12)

Equation (VIII-12) was calculated by graphical integration
f,or four sets of measurements.  Figure 21 is the plot of
M normalized by the mean of the four section measurements.
It shows that M at four different sections deviated by
less than 6 percent from the mean.  As a 6 percent devia-
tion is probably due to the inaccuracy of the measurements,
H can be considered to be essentially constant.  This sug-
gests the absence of coalescence and/or breakage of the
bubbles.                  \

       Transverse Profiles of the Concentration Flux

In order to check the similarity of the concentration
flux profiles, the measured data were normalized and
plotted as N/N (r/b ), where N  is the maximum value of
the concentration f^ux profile and b  is the half width
of the concentration flux profile defined as the radial
distance from the center line to the point where the
concentration flux is one-half the maximum value.  The
resulting plots for four bubble sizes are shown in Fig-
ures 22 through 25.  All of these figures indicate that
the similarity characteristics of the concentration flux
are preserved.

-------
Uv
l.JZ
1.08
1.04
A»
\ Nrdr
Jo
mean 1.00
0.96
0.92
0
° ^es970 microns
x 780
m M
A 527
o 0 3*3
D
D
* 0
ad*
0
A
X
D
i i i i i.
10 20 30
                                                    X/D
                            FIG.  21  VARIATION OF THE INTEGRATED CONCENTRATION FLUX



                                          ALONG THE AXIAL DIRECTION

-------
JL
Nm
  0.9
           —— ^»
          — A A.
                                 A'x/D = 20
              D D
               °y                D x/D =25
  0.8
              D
                Po
  °"7i
                   o
                     i
                   o
  0.6
      _ Az>-,	,	,	,	r
         a
         Ax                   x X/D =
             MA
                    D
                      A
                     *
0.5
                            x
                             D
                               AQ>
                                     X
                                  X,
  0.3
  0.2
                                       &k
                                         o
                                         A
                                              X «>
  0.1"
          (db= 3^3/0                           o •
            0.2     0*^     0.6     0.8     1*0
                               n
              FIG.  22  CONCENTRATION FLUX PROFILE



                            57

-------
    .o<4.£
  0.9
  0.8
  0.7
  0.6
 N
N,
 m
   0.5
   0.3
   0.2
   0.1

               A
s
 o
A
                x
                A
                a
 oA
   f
                     x
                     O
                           ;.A
                           a
               A o
                  AX
15
20
25
                                            D
                                           'O   K
                                 n
             0.2     O.J*    0.6     0.8     1.0     1.2
                             r/2b
               FIG.  23  CONCENTRATION FLUX PROFILE
                             58

-------
   0.8
   0.7
   0.6
 N
N,
 m
   0.5
   0.3
   0.2
   0.1
1.0 9fc*~5	1	r
      Aft

    0
   0.9
                  a


                 k*
                 V
                              1 - 1
                                  ox/D= 10



                                  *      15


                                  A      20



                                  o      25
                            "to
                                        X

                                        A
                                              o
                                              0
                      I        I  	I	I
             0.2     0.^     0.6    0.8     1.0    1.2
                             r/2b
                                 n
              FIG.  2^  CONCENTRATION FLUX PROFILE
                              59

-------
   1.0
   0.9
   0.8
  0.7
       &*
A
8
    O
    c»P
o  x/D= 10
x      15
A      20
D      25
  0.6
 N
N
 m
  0.5
        0
      *X  A
         A
          X
  0.3
  0.2
  0.1
                              X  O
                                  **
                                         oA
            0.2     0.4     0.6    0.8     1.0     1.2
              FIG.   25  CONCENTRATION FLUX PROFILE
                            60

-------
                   Half Width Dependence

The values of b  versus x/D for four different  bubble  sizes
are plotted in § dimensionless form as  b /D  versus x/D
in Figure 26.  Figure 26 indicates that £he  concentration
flux half width spreads linearly along  the axial direction
from a virtual origin at 0.8D from the  jet nozzle plane.
Coincidentally, this coincides with the virtual origin
of the momentum flux.  The plots of Figure 26 give:

     for dfe = 343y   b /D = 0.0650(x/D  + 0.8)           (VIII-13)

         db = 527y   b /D = 0.0683(x/D  + 0.8)           (VIII-14)

         db = 780y   bn/D = 0.0708 (x/D  + 0.8)           (VIII-15)

         db = 970y   bn/D = 0.0735(x/D  + 0.8)           (VIII-16)

From the above four expressions it is seen that the  rate
of spread of the concentration flux half width  consistently
increases when the bubble size increases. Qualitatively
this implies that larger size bubbles diffuse faster.
To evaluate the diffusion coefficients  a careful quan-
titative analysis accounting for all the measured data
will be done in the next Section.

            Center Line Concentration Flux Decay

From the similarity requirement and the principle of mass
conservation, the following relations must be true
             (°°
     N b2 ~    Nrdr = Constant                        (VIII-17)
     JNmDn    J Q

Furthermore, from the form of equations  (VIII-13) to
(VIII-16)

     N  b2 ~ N  x2 = Constant                          (VIII-18)
      m  n    m

and hence


     N  ~1/2~ x                                        (VIII-19)
      m

The center line decay of the concentration flux is thus
plotted as  (N /Nm)l/2 versus x/D in Figure  27,  where Nf
is defined as
          2TT

            irD^
-n:
                          61

-------
 D
 or
           half  width  spreading  of the  velocity
           concentration flux
           half  width  spreading
             o

             X
                 db=970
FIG. 26  HALF WIDTH SPREADING OF THE CONCENTRATION  FLUX
                           62

-------
 100
                             x/D
FIG. 2?  CENTERLINE CONCENTRATION FLUX DECAY

-------
The slopes of the corresponding plots in Figure 27 depend
upon the size of the bubbles.  The following results are
noted
for  db = 343y    (No/Nm)    = 29. 2 (^ + 0.8)             (VIII-21)


     db = 527y    (N0/Nm)1/2 = 30.5 <§ + 0.8)             (VIII-22)
        = 780y   (No/Nm)    = 31'5(5> + °'8)

     db = 970y   (N0/Nm)1/2 = 32.5 (| + 0.8)             (VIII-24)


EFFECT OF BUBBLE CONTAMINATION ON THE CARRIER STREAM

When a turbulent flow field is contaminated with foreign
particles the characteristic of the flow field itself will
probably be changed.

Soo et al (1960) carried out measurements on the diffusion
of helium gas in air and in suspensions which contained
0.0005 to 0.003 volume fraction of glass beads of diameter
less than 0.01 inches in a horizontal pipe.  They found
that the presence of the solid particles did not affect the
diffusion in the fluid phase.

Kada and Hanratty (1960) investigated the effect of parti-
cles on the diffusion characteristics of turbulence.  They
concluded that foreign particles with volume concentration
less than 2.5 percent do not appear to have a large effect
on the diffusion rate unless there is an appreciable average
slip velocity between the solid particles and the fluid.

Brandon  (1968) investigated the effect of glass beads on the
longitudinal turbulent intensity and the friction coefficient
of a pipe flow.  He concluded that (1) there is no detectable
effect of the solids on the longitudinal turbulent intensity
for particle sizes ranging from 20 to 60 microns and solid
sphere volume fraction of about 0.003, (2) the friction
factor increases with particles size from 20 up to 170 microns
and remains constant for sizes up to 560 microns for volume
fraction less than 0.01.

Hetsroni and Sokolov (1969) measured the longitudinal turbulent
intensity in an aerosol contaminated two dimensional jet with
aerosol consisting of oil droplets 13 microns in size.  They
reported that the intensity of turbulence is lowered by the
particles and that the suppression of turbulence is pro-
portional to the concentration of the droplets .

In this section the effect of the bubbles on the characteristics
of the flow field is considered both in the mean flow property,
fluctuation components, momentum flux deviation and the
energy spectrum.  For the case treated the bubble concentration
                           64

-------
is about 0.4 percent volume at the nozzle efflux of the jet.
It compares to the highest concentration used in the diffusion
measurements  (see Table 2).  The bubble size used in this
experiment is about 950 microns which is comparable to the
largest bubble size (970 microns) used for the diffusion
measurements.

           Effect on the Mean Flow Properties

The mean velocity profiles in the now bubble contaminated
flow field were re-measured with the hot film anemometer.
The bubble when impacting on the sensor will change the
cooling of the sensor and hence introduce errors both in the
DC and RMS voltages.  For the bubble concentrations treated
they may be neglected.

The measured velocity profiles are shown in Figure 28.  They
are noted to preserve the similarity characteristics and to
practically coincide with the bubble-free profiles.  The half
width spreading coefficient k,  in this measurement is of 0.0961.
This value is comparable to the kb of 0.0978 obtained for the
single phase jet.  The distance from the virtual origin ob-
tained by the intersection of the half width spreading line and
the jet axis to the jet nozzle plane, a, is now 0.9D and this
value is comparable to the value of 0.5D obtained for the
single phase jet  (Figure 29).  The center line velocity de-
caying rate, k , in this measurement is 0.162 which agrees well
with the single phase jet measurement.  However, the distance
from the virtual origin to the jet nozzle plane obtained by
the decay of the center line velocity is now 2.3D.  This is
bigger than the single phase result of 0.8D (Figure 30).  This
is probably due to the fact that the presence of the bubbles
in the potential core disturbs and shortens the length of the
potential core thus shifting the virtual origin toward the
upstream end.

          Effect on the Turbulence Intensities

When a turbulent flow field is contaminated with foreign par-
ticles distinguishable in their size and density from the
carrier stream, the relative motion of the particles with
respect to the fluid (slip velocity)  may cause extra dissi-
pation of the turbulent kinetic energy of the turbulent
fluid and hence a decrease in the turbulent intensity
(Hetsroni and Sokolov (1969) ).  Plots of the measured tur-
bulence levels at x/D=10, 15, 20 and 25 for the bubble con-
taminated flow field are shown in Figure 31.  For compari-
son, the fluctuation levels for the single phase jet measure-
ment (_as per Figure 18)  are re-plotted in Figure 31.  The
following intensities are noted at the axis of the jet.
                          65

-------
       1.
     0.9
     0.8
     0.7
     0.6
     0.3
     0.2
                       •
              ^>
              o
                • v
                 TBO
Without   With
Bubbles  Bubbles
   o        •
x/D-10

     15

     20


     25
                                                .V
                                                   v°.
                                                  j	I
                    o.ou
                      a 08
                       n
                   0.12
0.16
FIG. 28  NORMALIZED  VELOCITY PROGILE (WITH 6, WITHOUT CONTAMINATION
                                 66

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      2.
      1.
                                                0.0961 (x/D + 0.9)
                                                  With Contamination
                                          —O-— Without Contamination
                          10
20
30
                                      x/D
PIG. 29  VELOCITY HALF WIDTH  (WITH & WITHOUT BUBBLE CONTAMINATION)

-------
00
       0.3
       0.2
       0.1
                            °ODoD°
                                                   fc*
                                                   a A
                            a a  a
                            A
                            o
                                                   a* •   a  AB   B
                                                  9       On
                                                          O   A30 A

                                                 B  ° S '   a •*/ >
                                                _  aa      «   A   o  ^
                         a   A
                    <  a
                     a   A
                                    x/D = 1 0 \
                                    x/D = 1 5              °
                                             wlthbasbl"
                                                       «    A
                                                          o
                       8
                                                                      A
                                                                      «
                                                            8
                   A •
                                                    « 10
                                                z/D=15
                                                z/D= 20
                                             without
                                             bubbles
         -2.0
                                     .1.0
0
                                        r/b
1.0

                                                                       2.0
                                           u
FIG. 30  VELOCITY DISTRIBUTION ALONG JET AXIS  (WITH & WITHOUT BUBBLE  CONTAMINATION)

-------
              6.
ON
           u
            m
              2.
              1.
                                                                   With Contamination



                                                                —  Without Contamination
                                                  x/D
                                                    20
30
        FIG.   31  TRANSVERSE FLUCTUATION LEVEL  (WITH AND WITHOUT BUBBLES CONTAMINATION)

-------
     x/D     With Bubbles    Without Bubbles     Percent Decrease
     10         0.220            0.225                  2
     15         0.275            0.285                  3
     20         0.318            0.336                  5
     25         0.305            0.35                  12

It is seen that the fluctuation levels are attenuated due to
the bubble contamination.  This is especially so at large
axial distances.

The result seems reasonable since the relative motion of the
contaminants would dissipate more kinetic energy and hence damp
out the turbulent fluctuations.  At a relatively large x/D
the range of mixing, and hence the amount of energy dissipated,
will be greater, and consequently the deviation between the
two sets of turbulent fluctuation measurements (with and
without the bubbles) becomes greater.  This result, as dis-
cussed previously, has been observed by Hetsroni and Sokolov
(1969).

CONCENTRATION PROFILES

It must be noted that the measured quantities were the
concentration flux, N, and the mean velocity, U.   From these
the corresponding half widths, bu and bn were determined.
The actual concentration profiles,^, are obtained from the
measured N and U as discussed in the following section.
When looking at figures such as Figure 26 it must be noted
that although the concentration flux half width always grows
slower than the velocity half width, the concentration half
width need not.
                           70

-------
                        SECTION  IX

                 TURBULENT DIFFUS.IVITIES

The bubble concentration, ^,  can be  obtained  from  the measured
concentration  flux, N,  as
       V _
            N
In the above AS is the  effective  area  sampled by the  sensor,  as
defined in Chapter VIII,  and Vb is the  velocity of the bubbles.
The bubble velocity  is given  as Vj-^U+v^, where U  is the mean
velocity of the carrier  stream and v^  is the mean relative
velocity between the bubble and the  carrier stream.  Baker  and
Chao  (1965) suggest  that the  mean relative velocity between
the bubble and the mean  flow  of the  turbulent carrier  stream can
be taken as the rise velocity of the bubble in a  quiescent
liquid.  Based on this assumption, vb  is then a function only
of bubble size.  Haberman and Morton (1953) measured rising
bubble velocities leading to  the following:

Table 3 Rising Bubble Velocity


      d,  (Microns)                          v,  (fps)


           343                              0.105
           527                              0.186

           780                              0.301
           970                              0.397
The normalized concentration  is then calculated by
      V     VT  U
            N   m
         -
      Y    N~  U + v.     ,                                  (IX-2)
      xm    m        a     '
where N/N  is obtained from Section VIII, U and Um are described
by one ofmthe three  different models as given in Section VIII
and Vfc is obtained from Haberman and Morton's measurement.  The
normalized concentration profile can thus be calculated based
on Equation  (IX-2) and the corresponding dif fusivities computed
with Equations (VI-25) ,  (VI-27) , or  (VI-28) .

First Model:  (Constant Eddy Viscosity and Constant Eddy Diffusivity)

Assuming the velocity profile to be given by Equation  (VHI-6) the
normalized concentration profiles can then be calculated from
Equation (IX-2).   The profiles  for 343, 527, 780 and 970 micron

                          71

-------
                           Table 4   Turbulent Schmidt Number
to
First Model
Bubble Size
(Microns)


343
527
780
970
(Constant

ey
Um(x+a)
0.0025
0.0029
0.0030
0.0031
E and £ Model)
in y
St

1.06
0.92
0.90
0.88
(Tomotika's Solution)

st

1.19
1.00
0.98
0.94
(Gaussian Solution)

st
t
1.17
1.07
1.00
0.93
     Note:  In the second and third models, e  and e  are dependent on n as shown in
            Figure VII-17                    Y

-------
bubbles are respectively shown in Figures  32 to 35.   It is
seen that the normalized concentration data  preserve the
similarity characteristics.   (This point will be  further
discussed in the next section) .

Combining Equations  (VIII-6)  and Equation  (VI-25) , one  obtains
                 46.02ri2)~2 en/eY
The computed concentration profiles  are given in  terms of r\ .
The corresponding turbulent Schmidt  number  for the bubble
diffusion,  (S^e^ey) , can be obtained by comparing Equation
(IX-3) with the data  of Figures 32 to 35.   The resulting
coefficients of the eddy particle dif fusivities and the
corresponding turbulent Schmidt -numbers for the four bubble
sizes tested are tabulated in" Table  4.  These were obtained by
minimizing the mean square difference between the data and
Equation  (IX-3) with  different exponents.   The theoretical
curves given by Equation  (IX-3) with the regressed coefficients
are also plotted in Figures 32 to 35.  It is seen that the
general shape of the  curves agrees very well with the values
computed based on the actual measurements.

Second Model:  (Taylor's Vorticity Transport Theory)

Assuming that the velocity profile of the flow field is given
by Equation  (VIII- 8) , the normalized concentration profiles
calculated with Equation  (IX-2) for  the 343, 527, 780 and "970
micron bubbles will differ from those of figures  32 to 35.
The corresponding values are shown in  Figures 36 to 39.

Combining Equations (VIII-8) and Equation  (VI-27) the assumed
concentration profile takes the form

                         1                      7

                                         .(ii.8n) -
v    f   ff11'811 idi.sn) -ia, (ii,8Ti)2+
— =/ExP  ii.san- - '-± -
Vm   V   Uo      _ 3 ^ +  3a2  (11.8n)3
                                      3/2 -      (ii.BTi)3
                                                            (IX-4)
Equation  (IX-4) can be numerically integrated for various values
of TI provided the exponent £ni/eY ^s assumed to be known.
In this manner, repeating the calculation, of the concentration
profile by considering different  values for Em/Ey/ the value
for which the calculated ! concentration profile appears to best
fit the measured data can be found.  This is then taken to be
the representative turbulent Schmidt number.
                           73

-------
  1.0
  0.9
  0.8
  O.?
  0.6
L
Pm
  0.5
  0.4
  0.3
  0.2
  0.1
X  X/D=15

A  x/D=20'

o  x/D = 25
            0.02      0.04    0.06      0.08     0.1 0     0.1 2    0.1 1|
                  FIG.   32  CONCENTRATION PROFILE

-------
 i.o
     ,*0 A
 0.8
 0.6
Tin
0.2
o  x/D=10
¥        15
A        20
o        25
          0.02    o.o^    0.06     a 08    0.10    0.12    ai*f
                  FIG. 33  CONCENTRATION PROFILE
                                 75

-------
i.o Vti
        --ft
0.8
0.6






JL

ft*




0,4
0.2
            \
           o
           X


           A
x/D» 10


     15


     20
                    25
         (db«780/i)
         0.02    0^4    0.06    0.08   0^0    0.12
                   PIG. 34  CONCENTRATION  PROFILE
                                  76

-------
 1.0
0.8
0.6
           O
           K

           A
0.2
X/D« 10
     15
     20
     25
         (db=9?o/O
        0.02    O.QJ*    0.06     aos    0.10   0.12
                 FIG.  35  CONCENTRATION PROFILE
                                77

-------
The corresponding theoretical curves calculated with the best
fit coefficients of em/£y are shown in  Figures 36 to 39.
In order to see how sensitive the plots given in Figures 36
to 39 are to a change in St the curves of Equation  (IX-4)with
St=0.8, 1.0 and 1.4 are also included in Figure 36.  The
numerical values of EH/EY leading to a best fit are shown in
Table 4.

In comparing the general shape of the theoretical curves with
the measurements, it is seen that the theoretical curves show
a greater curvature at small values of TI .  The general shape
of the curves does not agree with the measured concentration
profiles very well.  The same deviation (between measured
values and model) was observed in the velocity profiles as
shown in Figure 9.

Third Model:  (Reichardt's Inductive Theory)

The data can also be analyzed considering the third model
proposed.  Assuming that the velocity profile is given by
Equation (VIII-9), the corresponding concentration profiles
calculated from Equation (IX-2)  for the 343, 527, 780 and
970 micron bubbles are shown in Figures 40 to 43.  From
Equations (VIII-9) and VT-28)  the assumed concentration profile
takes the form



      —  = Exp/*- 73.04 — n2 V                             (IX-5)
      * m      L        £Y   J
The corresponding turbulent Schmidt number em/ev Ieac^in9 to a
best fit, as shown by the plots of Figures 40 to 43 are tabulated
in Table 4.  The calculated curves show a smaller curvature near
the center line region and  under predict near the edge of the
jet.  The general shape of the analytical curve does not agree
very well with the measured data.  The same deviation has been
observed in the velocity profile when calculated using this
model as shown in Figure 9.

The comparison of the analytical and semi-empirical curves
given by the above models indicates that the first model seems
to fit the measured concentration profile best.  Hence it is
concluded that the particle diffusivity and the corresponding
turbulent Schmidt number obtained from the first model should
be the most reliable of the three.  No thorough statistical
measures were sought to compare the predictions made by the
three models.  An attempt at using a simple regression analysis
did not lead to a better interpretation of the results.
This was primarily due to the spread of the data.
                          78

-------
 0.9
 0.8
 o.?


 0.6
[V
T~
 m
 0.51
 0.3
 0.2
0.1
                     o   rm i
                                  «*   1  o  o
                                         -
                        HS*P(K^
                                ^J<
            o  x/D =10
            x  x/D =15
            A  x/D =20
            D  x/D = 25
            (db=
                     J.
                                      JL
_L
           0.02
                   0.04     0.06     0.08     0.10      0.12     0.14
                 FIG.  36  CONCENTRATION  PROFILE
                               79

-------
                    Eq. ( IX-^ ) wi th 
-------
BqL'  (IX-4) with
                                       = 0.98
o.02     o.o4    o.o6     a oe    a 10    0.12
    FIG. 58  CONCENTRATION  PROFILE
              (With Bubble Rising Vel.  Corr.)
                   81

-------
1.0
0.8
0.6
£_

Tm
0.2
                             Eq.(VE-4) with £*/<* = 0.94
o  X/D=10


x       15

A       20


0       25



b= 970/4.)
   0     0.02    0.04     a 06    0.08     0.10    0.12     0.14
               fIG. 39  CONCENTRATION PROFILE
                        (With Bubble Rising Vel. Corr.)
                            82

-------
0.1  •
                                  ku=73.04


                                  |2=1.17
         0.02
           FIG. 40  CONCENTRATION PROFILE
                     (With Bubble Rising Vel. Corr.)
                          83

-------
0.2
         0,02    0.04     0.06     0.08     OJ'O     0.12
             FIG. 41  CONCENTRATION  PROFILE
                       (With  Bubble Rising Vel. Corr.)
                            84

-------
Q  O
                   Eq.  (IX-5) with
     o x/D= 10
       = 780/4)
           0.0^     0.06    0.08    0.10    0.12
0.14
    FIG. 42  CONCENTRATION PROFILE
              (With Bubble Rising Vel. Corr.)
                      85

-------
1.0
0.8
0.6
0.2
                          Eq.(lX-5)  With £m/6r=0.93
o  x/D=10

*        15
A        20

D        25
              = 970/t)
         0.02     0.01*    o.06    0.08     0.10     0.12

                               1

           FIG.  ^3  CONCENTRATION PROFILE
                    (With Bubble Rising Vel. Corr.)
                            86

-------
                         SECTION X

            TURBULENT DIFFUSION CHARACTERISTICS

 Dependence of Turbulent Schmidt Number on the Particle
 Parameter ^

 The results reported in the previous sections dealt with the
 dispersion of bubbles in a liquid jet.  As noted by Householder
 and Goldschmidt  (1969) it is possible to compare the diffusion
 of particles in entirely different flow fields by using a cor-
 relation based on ty .

 This is because the turbulent transport is related primarily
 to the immediate structure of the turbulent flow and the
 particle size, shape and density.  In selecting a parameter
 to make this comparison they selected the ratio of the Stokesian
 response time of the particle in a carrier stream to a charac-
 teristic time scale of the flow.  Ahmadi (1970) extended this
 idea using the turbulent time macroscale as the specific charac-
 teristic time.  He defined the corresponding particle parameter
 as
                                                          (X-l)

 where A  is the longitudinal turbulent macroscale of the
 flow field.  What is to be investigated is whether or not S
 is a function of fy .  Knowledge of such a function would permit
 comparison of experimental results of the previous section to
 those of other investigators and an extension to other flow
 fields as well.

 When the particle in concern is a bubble of gas in water the
 particle parameter given in Equation  (X-l) simplifies to
                        \  x
 which can then be re-written as

Vs?
 y u /U , U /U  and A /D are given in Figures 31, 11 and 20,
 respectively™  An average value of $T can be computed for each
 bubble size throughout the region in which measurements were
 taken.  The relationship used is ip_ = 7.25x10  ,_bx  , an average
                            87

-------
for 10T for the four bubble sizes
is shown in Figure 44.  The dynamic numerical prediction of
Ahmadi (1970) and the data for the pipe and open channel ex-
periments collected by Householder and Goldshmidt (1969) are
also included.  In addition, results of two other jet diffusion
experiments by Singamsetti (1966) and Brush (1962) , one plane
jet diffusion experiment by Householder (1968) and one "iso-
tropic" turbulent diffusion experiment by Kennedy (1965) are
included in Figure 44.  The results of Householder include
one questionable data point currently under a separate study .

From Figure 44, it is seen that the data obtained from the
circular jet measurements (i.e. Singamsetti, Brush and present
study) seem to fall below the other measurements and Ahmadi 's
prediction.

Such deviation suggests that the relationship between S  and
fy  may have different trends, one for the reported pipe,
channel and plane jet measurements (which follow the theore-
tical curve predicted by Ahmadi) and another for the circular
jet measurements.

The difference between these may be either due to an essential
difference in their geometries or to some inherent difference
in the specific experiments reported.  The predictions of Ahmadi,
as well as the selection of ^T assumed that the particle Rey-
nolds number  (which according to Ahmadi is defined as
R   = 0 / 2 ,  , .  is in the order of one or smaller.  This condi-
  D        db/v)
tion was satisfied for Householder ' s experiment and most of the
data gathered by him.  Unfortunately it was not for the current
measurements nor for the other reported for circular jets (all
of which has values of R   in the order of 10 -10 ) .
                         P
It is desirable to attempt to find another particle parameter.
Hopefully a university relationship could be found between S.
and this new particle parameter

Dependence of Turbulent Schmidt Number on the Particle Parame-
ter ^

Recalling the definition of Tj>_, one can decompose it as

                 *y J £•   «O             —
         .    36 u  a b ,  p , ,,   36 u^                 ,v ..
                                         Ts              (X'4)
                X         X.           X
Where T  is the Stokesian response time of the particle.  It
is quite obvious then that the particle parameter ty  is meaning
ful in describing the particle diffusion only for the/ cases
where the particle Reynolds number lies within the
                            88

-------
00
VO
        ,-1
    collected by Householder & cjoldsehmidt
 *   Ipipe and channel)
 V  Kennedy  tisoxropic  turbulence?
 D  Brusn         >
 A  JJingmasetti   I .(axi.-symmetriG jet)
 •  present  stu'Sy J
 o  "Householder  (plane  jet)
                                           •
	dynamic simulation (Ahmadi'-)
                                       V   .

                                                                          •    •
10'
                                             10
                                               -1
                                        10
10J
              FIG. Mf  DEPENDENCE OF S"1 ON PARTICLE PARAMETER

-------
Stokes range.  For the present and the other two circu-
lar jet measurements where the particle Reynolds numbers
are in the order of 10  to 10  another particle parameter has
to be defined.  Let this be
              X

where T is the actual particle response time.  An expression
is then sought for T.

Neglecting the potential force, nonlinear effect and Basset
term, the B.B.O. Equation takes the form
      at  
-------
Assuming that the initial condition is | vp - vf|t_0 =2^u ,
Equation (X-9) can be integrated to yield
 Vp - vf
             db8/5(2
Defining particle response time   as the value of t where
|vp-Vf l/2/tt2" equals to e"1 = 0.368 the expression for  becomes


               d I-*  {2 !P + D
 T  = 0.0335 x -£-— - Ki - for 2
-------
With T defined, the values of ty' in Equation  (X-5) can be
calculated for various measurements.  These are shown in
Table 5.

Figure 45 shows the relationship now between S    and ty .
Better agreement is now noted.  However the deviation be-
tween the circular jet measurements and the two dimensional
flow field measurements (together with the theoretical two-
dimensional prediction) is still noted.

In comparing the results of the present bubble diffusion
measurements with the other diffusion measurements in circu-
lar jets with solid particles as contaminants  (i.e. sediment
in Singamsetti1s and glass beads in Brush's), it is seen that
the agreement is very good except for a point in Brush's data.
This interesting result could be explained in the following
conjecture.  For a relatively small bubble moving in a turbu-
lent liquid stream the bubble shape will remain approximately
spherical due to the surface tension effect.  If this is the
case, the bubble can be considered as a rigid particle.  The
density effect of the particle has been accounted for by the
particle parameter i|j' .  Consequently the, measured results
unified through i^' give a comparable S ~  - i^J, relationship
as shown in Figure 45.  Such results lead to_rhe conclusion
that with i|>' so defined the dependence of S.   on the particle
parameter i|c is universal for measurements in similar flow
fields regardless on whether the particle is heavier or lighter
than thecarrier stream.  In other words the relationship be-
tween S.    and ijj' is the same for similar flow fields for
bubbles in water, solid particles in water or even aerosols
in air streams.

One point yet unclarified, as noted previously, is that a two-
dimensional and a three-dimensional flow field, appear to
give different trends of S    - ij;'.  This dilemma could be
clarified by extending the experimental study to larger ^'
domain, such as measuring the diffusion of larger aerosols
in both circular and plane air jets to see whether there
exists a large deviation in between these two.

The relationship for S.   versus ^' as just described is ori-
ginated form a rather intuitive background.  The theoretical
basis for the universality of such relationship is rather
weak, and although confirmed by experiments, it deserves
further study.
                        92

-------
TABLE
Calculation of Si  versus
Particle Reynolds
Authors db(/f) Number, Rep fs
2 7? dfc/V , (10r3Sec. )
Present
fork


Singa.msetti




Brush


343
527
780
970
68
115
230
320
460
190
320
550
338
519
768
954
136
227
454
631
907
374
631
1034
3.
8.
18.
28.
3.
9.
33.
73.
152.
17.
49.
147.
52
32
07
10
43
54
20
70
20
55
90
80
"^
T T/T
5.
12.
27.
42.
4.
13.
•53.
101.
213.
23.
67.
196.
28
46
30
30
68
38
40
50
00
50
00
00
0.154
0.161
0.109
0.088
0.223
0.182
0,138
0.132
0.092
0.148
0.132
0.080
(0.203)
(0.172)
(0.147)
(0.134)
(0.293)
(0.238)
(0.180)
(0.158)
(0.138)
(0.195)
(0.158
(0.160)
0.81
2.00
2.97
3. 70
1.04
2.43
7-37
13.40
19.60
3.48
8.85
15.60
(1.07)
(2.14)
(4.01)
(5.6?)
(1.37)
(3-18)
(9.61)
(16.00)
(29.40)
(4.58)
(10.60)
(31.30)
*?
0.94
1.09
1.11
1.14
1.23
1.20
1.24
1.37
1./44
1.00
2.00
6.70

-------
,-t
7
6

$

*


3

2
1
0
1C

collected by
pip* a-oii £-h3
1
1 1 1 1 1 I
Ho;:i3«hol:l-er & .Goldschmidt
•'Tia-e!!. ( T/^m = l//ip)
V Kennedy .(isotropic turbulence)
a Brush
£ Singassetti
present study
|
( {axi-s^mmetric jet) .. .
J -
o householder (plane jet) " ,
, 	 Dynamic simul
•
*•

-
V
/ —
,,ior U-a-; '. ._ / .
' ' /°
... /
bX-
• • -^/ ' °

v A a^a""'21
^ . «. — B- TJ
•
1 1 1 1 1 1
>~^ 1 0~
10~2 10'1 10° 101 102 105
                                          Vr'
                             "1
    FIG. 45  DEPENDENCE OF S"   ON  PARTICLE PARAMETER

-------
                       SECTION XI

                 SIGNIFICANCE OF RESULTS


The experiments convincingly show that the turbulent trans-
port coefficient of suspended particles is not necessarily
equal to that of momentum.  As a matter of fact an increasing
eddy diffusivity coefficient with particle size is noted.
This is observed for small particles in the Stokes regime,
smaller than the turbulent macroscale of the carrier stream.

The results of Figure 44 exhibit then when a particle can
be considered to have a turbulent transport same as that
for the momentum of the carrier stream.  As an example, a
grain of sand, 50 microns in diameter, when suspended in
water flowing from a plane 2 inch nozzle at about 5 ft./sec.
would have a ^T parameter of about 0.05.  For such a case
the transport coefficients (of the sand and carrier stream
momentum)  would be equivalent.  However, if the channel
width were to be in the order of 1/16 of an inch (then
T|J  - 1.5 and) the transport coefficient of the sand would
now be in the order of three times more than that of the
momentum of the fluid!  Estimates of the corresponding
dispersion of the effluent sand should then correctly ac-
count for this somewhat startling result.

-------
                     SECTION XII


                  ACKNOWLEDGEMENT S
The reported work was the result of the Ph.D. research
of Dr. Strong C. Chuang. Professor Victor W. Goldschmidt
acted as supervisor of his work.

The support of the project by the Water Quality Office
Environmental Protection Agency, and the help provided
by Mr. George Ditsworth, Project Representative is
acknowledged.

The assistance of the staff of the School of Mechanical
Engineering and its Ray W. Herrick Laboratories during
the final stages of the work reported is also gratefully
acknowledged.
                         97

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                        SECTION XIII
                         REFERENCES


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Brooks, N. H. Discussion of "Acceleration Motion of a Spherical
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-------
Brush, L. M., Ho, H. W., and Singamsetti, S. R. "A Study of Sediment
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Cermak, J. E. "Lagrangian Similarity Hypothesis Applied to Turbulent
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Chuang, S. C. and Goldschmidt, V. W. "The Response of a Hot Wire
Anemometer to a Bubble of Air in Water", Symposium on Turbulence
Measurement'in Liquids, 9, 1969, Univ. of Mo., Rolla, Mo.

Chuang, S. C. and Goldschmidt, V. W. "Bubble Formation Due to a
Submerged Capillary Tube in Quiescent and Co-flowing Streams",
ASME Nucleonics Symposium, May, 1970.   (ASME, Paper No. 70-FE-21)

Collis, D. C. and Williams, N. J. "Two-dimensional Convection from
Heated Wires at Low Reynolds Number," J. of Fluid Mech., Vol. 6,
1959, pp. 357-384.

Corrsin, S. "Investigation of Flow in an Axially Symmetric Heated
Jet of Air," NACA W-94 ACR No. 3123, 1943.

Corrsin, S. and Uberoi, M. S. "Further Experiments on the Flow and
Heat Transfer in a Heated Turbulent Air Jet," NACA Tech. Note No.
1865, 1949.

Corrsin, S. and Lumley, J. "On the Equation of Motion for a Particle
in Turbulent Flow," Appl. Sci. Research, Vol. 6A 1956, pp. 114.

Corrsin, S. "Theory of Turbulent Dispersion", Proc. for Turb. Diff.,
Marseille, France, 1962, pp. 27-52.

Curtis, A. J. "Shock and Vibration Handbook", Edited by Harris and
Crede, McGraw-Hill, 1960, Ch. 22.

Datta, R. L., Mapier, D. H. and Newitt, D. M. "The Properties and
Behavior of Gas Bubbles formed at a Circular Orifice," Trans. Inst.
Chem. Engr., Vol. 28, 1950, pp. 14-26.

Davidson, L. "A Study of the Formation of Gas Bubbles from
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1951.

Davidson, L. and Schuler, B. 0. G. "Rapid Formation of Gas Bubbles
in a Viscous Liquid," Trans. Inst. Chem. Engr. Vol. 38, 1960, pp.
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Delhaye, J. W. "Hot-film Anemometry in Two Phase Flow," Two Phase
Flow Instrumentation, Presented at llth Nat'l American Society of
Mechanical Engineering, American Institute of Chemical Engr. Heat
Transfer Conf. 8 1969, Minneapolis, Minn. pp. 58-69.

                           1.00

-------
Eckert, E. R. G. and Drake, R. M. Jr. Heat and Mass Transfer, McGraw
Hill, Inc., N. Y., 1959.

gversole, W. G.; Wagner, G. H. and Stackhouse, E., "Rapid Formation
of Gas Bubbles in Liquids," Ind. Engr. Chem.,  Vol. 33, 1941, pp.
1459-1462.

Flora, J. J. J. and Goldschmidt, V. W. "Virtual Origin of a Free
Plane Turbulent Jet" AIAA Journal Vol. 7, No.  12, 12, 1969, pp.
2344-2346.

Folsom, R. G. "Review of the Pitot Tube", Trans. ASME, Oct., 1956,
pp. 1450.

Forstall, W. and Gaylord, E. W. "Momentum and Mass Transfer in a
Submerged Water Jet," J. of Applied Mech., ASME Trans., Vol. 22,
No. 2, 1955.

Frenkiel, F. N. "Turbulent Diffusion of Mean Concentration Dis-
tribution in a Flow Field of Homogeneous Turbulence," Advance in
Applied Mech., Academic Press, Inc., 1953, pp. 61-107.

Frielander, S. K.  "Behavior of Suspended Particles in a Turbulent
Fluid" AIChE J. Vol. 3, No. 3, 9, 1957, pp. 381-385.

Goldschmidt, V. W. "Measurement of Aerosol Concentrations with a
Hot Wire Anemometer," J. of Colloid Science, Vol. 20, No. 6, 1965,
pp. 617-634.

Goldschmidt, V. W. and Eskinazi, S., "Two-Phase Turbulent Flow in
a Plane Jet," Journal of Applied Mechanics, Vol. 33, Series E, No.
4, Dec., 1966, pp. 735-747.

Goldschmidt, V. W. and Householder, M. K. "Measurement of Aerosols
by Hot Wire Anemometry," AFOSR Final Report, AFOSR No. 68-1492, July
1968, pp. 134-152.

Goldschmidt, V. W. and Householder, M. K., "The Hot Wire Anemometer.
as an Aerosol Droplet Size Sampler," Atmospheric Environment, Vol.
3, Nov., 1969, pp. 643-652.

Haberman, W. L. and Morton, R. K. "An Experimental Study of Bubbles
Moving in Liquids," ASCE Trans. Paper No. 2799, 1953, pp. 227-252.

Heskestad, G. "Hot Wire Measurements in a Plane Turbulent Jet," J.
of Applied Mech. Dec., 1965, pp. 721-739.

Hetsroni, G. and Sokolov, M. "Distribution of Mass, Velocity and
Intensity of Turbulence in a Two Phase Turbulent Jet," Dept. of
Nuclear Sci. and Mech. Engr.,  Technion, Israel Institute of Tech-
nology, Haifa, Israel, 1969.

Hinze, J. 0. Turbulence McGraw Hill Co.,  Inc.  1959.
                        101

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Hinze, J. O., and Van Der Hegge Zijnen B. G. "Transfer of Heat and
Matter in the Turbulent Mixing Zone of an Axially Symmetrical Jet,"
Applied Sci. Research A. Mech. Heat, Vol. 1, 1949, pp. 435.

Ho, H. W. "Fall Velocity of a Sphere in a Field of Oscillating Fluid."
Ph.D Thesis, Univ. of Iowa, Iowa City, Iowa, 1964.

Householder, M. K. "Turbulent Diffusion of Small Particles in a Two-
dimensional Free Jet," Ph.D Thesis, School of Civil Engr., Purdue
Univ., W. Lafayette, Ind., 1968.

Householder, M. K. and Goldschmidt, V. W. "Turbulent Diffusion and
Turbulent Schmidt Number of Small Particles-Part I," Journal of the
Engineering Mechanics Division, EM6, December 1969, pp. 1345-1367.

Hsu, Y. Y., Simon, F. F. and Graham, R. W. "Application of Hot-wire
Anemometer for Two Phase Flow Measurements Such as Void Fraction
and Slip Velocity," ASME Winter Meeting, Philadelphia, Pa.,  Nov., 1963,

Ismail, H. M.  "Turbulent Transfer Mechanism and Suspended Sediment
in Closed Channels," Trans. ASCEE Vol. 117, 1952, pp. 409-446.

Jones, B. G.,  Chao, B. T. and Shirazi, M. A. "An Experimental Study
of the Motion of Small Particles in a Turbulent Fluid Using Digital
Techniques for Statistical Data Processing," Nuclear Engr. Dept.,
Univ. of 111., Urbana, 111., 1966.

Kada, H. and Hanratty, T. J. "Effects of Solids on Turbulence in a
Fluid," AIChE J. Vol. 6, No. 4, 12, 1960, pp. 624-630.

Kalinske, A. A. and Pien, C. L. "Eddy Diffusion," Ind. Engr. Chem.,
Vol. 36, 1944, pp. 220.

Kampe de Feriet, J., Proc. 5th Intern. Congr., Appl. Mech.,  Cambridge,
Mass., 1938, pp. 352.

Keagy, W. R. and Weller A. E., Proc., Heat Transfer and Fluid
Mechanics Inst., Berkeley, Calif., 1949, pp.89.

Kennedy, D. A. "Some Measurements of the Dispersion of Spheres in a
Turbulent Flow," Ph.D. Thesis, Dept. of Mechanics, The John Hopkins
Univ., Baltimore, Maryland, 1965.

Kraichnan, R.  H. "Dispersion of Particle Pair in Homogeneous
Turbulence" The Physics of Fluids, Vol. 9, No. 10, 1966, pp. 1937-
1943.

Kuethe, A. M.  "Investigations of the Turbulent Mixing Regions Formed
by Jets," J. Appl. Mech., Vol. 2, No. 3, 1935, pp. A-87-95.

Kumar, A. "Bubble Formation in Fluids of Low Viscosity Under Constant
Flow Conditions," Chem. Tech., Vol. 19, 1967, pp. 78-82.

Laursen, E. M. "The Total Sediment Load of Stream," Proc., ASCE, Feb.,
1958, pp. 1-36.


                         102

-------
Leibson, I., Holcomb, E.G., Cacoso,  A.G.  and Jacmic,  J.J.  "Rate
of Flow and Mechanics of Bubble Formation From Single Submerged
Orifices," AICHE J., Vol. 2, 1956,  pp.  296-306.

Levich, V.G. and Kuchanov, S.I. "Motion of Particles  Suspended in
Turbulent Flow," Soviet Physics Doklady,  Vol. 12,  No. 6,  12,  1967,
pp. 546-548.

Lin, C.C. "On a Theory of Dispersion by Continuous Movement-T,"
Proc. Nat. Academy of Sci. , Vol. 46, 1960a, pp.  566-570.

Lin, C.C. "On a Theory of Dispersion by Continuous Movement-II,"
Stationary Anisotropic Process," Proc., Nat. Academy  of Sci., Vol.
46, 1960b, pp. 1147-1150.

Liu, C.L. "Characteristics of Hot Wire and Hot Film Sensors for
Turbulence Measurements in Liquids", Ph.D. Thesis, School of
Civil Engr., Purdue University, W.  Lafayette, Indiana, 1967.

Longwell, J.P. and Weiss, M. "Mixing and Distribution of  Liquid  in
High Velocity Air Streams," Ind. Engr.  Chem., Vol. 45, 1953,  pp.
667-677.

Maclntyre, F. "Vibrating Capillary for Production  of  Uniform
Small Bubbles," Review of Sci. Inst., Vol. 38, No. 7, 1967,
pp. 969.

Majumdar, H. and Carstens, M.R. "Diffusion of Particles by
Turbulence: Effect of Particle Size," Final Report G. R.  No.  5,
Vol. WP00912-02ESE, C.E., Git., Atlanta, Ga., 1967.

Milne-Thomson, L.M. Theoretical Hydrodynamics, 3rd Edition,
London: MacMillan & Co., Ltd., 1955.

Pattle, R.E. "The Aeration of Liquids, Pt. II.  Factors in the
Production of Small Bubbles," Trans. Inst. Chem. Engr., Vol.
28, 1950, pp. 32-37.

Ramakrishnan, S., Kumar, R. and Kuloor, N.R. "Studies in Bubble
Formation-I, Bubble Formation Under Constant Flow Conditions,"
Chem. Engr. Sci., Vol. 24, 1969, pp. 731-747.

Rennie, J. and Evans F. "The Formation of Froths and  Foams above
Sieve Plates/' Brit. Chem. Engr., Vol. 7, 1962, pp. 498-502.

Roberts, P.H. "On the Application of a Statistical Approach of
the Theory of Turbulent Diffusion," J. of Math, and Mech., Vol.
6, 1957, pp. 781-799.
        ^
Roberts, P.H. "Analytical Theory of Turbulent Diffusion",  N.Y.U.,
June, 1960, Research Report No. HSN-2.
                          103

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Rouse, H. "Experiments on the Mechanics of Sediments Suspension,
"Proc., Fifth Intern. Cong, of Appl. Mech., Cambridge, Mass., 1938,
pp. 550-554.

Sayre, W. W. and Chang, F. M. "A Laboratory Investigation of Open-
Channel Dispersion Process for Dissolved, Suspended, and Floating
Dispersants," Geological Survey Professional Paper 433-E. 1968.

Schlichting, H. Boundary Layer Theory, McGraw Hill Book Co., 1960.

Shirazi, M.  A., Chao, B. T. and Jones, B.C. "On the Motion of
Small Particles in a Turbulent Fluid Field," Nuclear Eng. Dept.
Univ. of 111., Urbana, 111., 1967.

Siemes, W. "Gas Bubbles in Liquids-I, the Formation of Gas Bubbles
at Upward Pointing Circular Orifices," Chem. Ing. Techn., Vol. 26,
1954, pp. 479-496.

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Hy-2, 1966,  pp. 153-168.

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                                    "-V
Tomotika, S.,  Proc. Roy. Soc. London, 165A, 1938, pp. 65.
                                                        /  i
Trentacoste, N. and Sforza, P. "Further Experimental Results for
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                         104

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Valentin, F. H. H. "Absorption in Gas-Liquid Dispersions" Spon's
Chemical Engr. Senis, London, 1967.

Vanoni, V. A. "Transportation of Suspended Sediment by Water"
Trans. ASCE., Vol. Ill, 1946, pp. 67-133.
                         105

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                        SECTION XIV

                        PUBLICATIONS

The following is a list of publications which resulted due
(in part or fully) to the sponsorship of Grant 16070DEP
by The Water Quality Office, EPA.  Abstracts are presented
in Appendix V.

     1.  S. C. Chuang and V. W. Goldschmidt "The Response
         of a Hot Wire Anemometer to a Bubble of Air in
         Water" Symposium on Turbulence Measurements in
         Liquids, University of Missouri, Rolla, Missouri,
         September 1969.

     2.  S. C. Chuang and V. W. Goldschmidt "Bubble
         Formation Due to a Submerged Capillary Tube in
         Quiescent and Co-Flowing Streams" ASME, J. Basic
         Engineering, Vol. 92, D, No. 4, December 1970,
         pp 705-711.

     3.  G. Ahmadi and V. W. Goldschmidt "Dynamic
         Simulation of The Turbulent Diffusion of
         Small Particles" Hydrotransport I, First
         International Conference on The Hydraulic
         Transport of Solids in Pipes, University of
         Warwick, Sponsored by The BHRA Cranfield,
         Bedford, England, September 1-4, 1970.

     4.  G. Ahmadi and V. W. Goldschmidt "Analytical
         Prediction of The TurbulentDiffusion of Small
         Particles," Fluid Dynamics Symposium, McMaster
         University, Hamilton, Ontario, August 25-27,
         1970.

The following articles are currently under the review and
pre-publication process:

     5.  V- W. Goldschmidt and S. C. Chuang "Energy Spectrum
         and Turbulent Scales in an Axi-Symmetric Water Jet"
         Submitted to the ASME.

     6.  V. W. Goldschmidt, M. K. Householder- G. Ahmadi and
         S. C. Chuang "Turbulent Diffusion of Small Particles
         Suspended in Turbulent Jets" Submitted for consi-
         deration at a forthcoming Symposium on Two Phase
         Flows.
                        107

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                       SECTION XV

                   GLOSSARY OF SYMBOLS

           numerical constants

           intercepting area of the sensor

           virtual origin of the jet, defined by equation VI-4
           and VI -5

           coefficients given in Eg.  (VI-15)

b          characteristic jet width;  temperature coefficient
           of the electric resistivity of the sensor

bu         half width of the velocity profile

bR         half width of the concentration  flux profile

b          half width of the concentration  profile

C          drag coefficient

GW         specific heat of the sensor

c          correction factor in pitot tube  measurement

c          numerical constant related to the vorticity transport
           mixing length

Cp         numerical constant related to the scalar quantity
           transport mixing length

D          jet nozzle diameter

d,          bubble diameter
d.         inside diameter of the syringe tube

d          outside diameter of the syringe tube
 o

do         Vdi

 w         sensor diameter

E          mean DC voltage output (measured)

e          peak voltage drop in the sensor due to an impacting
 p         bubble
                       109

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E          mean DC voltage output (true value)

e          fluctuation voltage output due to the turbulent
           velocity fluctuation

e^         DC voltage output at a particular frequency f

e          voltage drop due to an impacting bubble
 s
F          Proude number = d.f  /gd.

f          bubble generating frequency; frequency of turbulence

h          distance from the center of the sphere to the wall

h^h-      heat transfer coefficients per unit length of the
           wire exposed to the air and the water phase respectively

K          axial conductivity of a sensor; wave number

Ku         constant in Eq. (VI-17)

k,,k2      heat conduction coeff. of the air and of the water at
           the film temperatures T-, and T,.  respectively

k,          rate of half width spreading in a jet, Eq. VI-4

k          decaying rate of the jet center line velocity,
 U         Eq. VI-5

k,          rate of concentration half width spreading, Eq. VI-22

k          center line concentration decaying rate, Eq. VT-23

L          length scale in r-direction

L          length scale in x-direction
 X

Lfi         length scale in 6-direction

H          mixing length related to the momentum transport;
           effective length of the sensor

S,          mixing length related to the vorticity transport

M          PWTT d£/6

N          bubble concentration flux

N          bubble concentration flux at the jet mouth
 o
N ,,N £    Nusselt number for sensor exposed to air and water
           phase respectively
                        110

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n          number of bubbles impacting in a time period T
-»•
n          mass flux vector of gas
->•
^w         mass flux vector of water

P          mean pressure

pm         measured static pressure by pitot tube

PT         true static pressure

P1         instantaneous pressure

p          fluctuation pressure

PQ         static pressure in the outside field of a jet

Pr2        Prandtl number of the water

Q          gas flow rate through a syringe tube

R          correlation coeff. of two fluctuating velocity
           components; total electric resistance of a sensor;
           Reynolds number

R , R , ,R - orifice Reynolds number of the jet, Reynolds number
           of the air and water phases based on the sensor
           diameter


Re                                   |v  - vf | d,  2 u  d,
  p        particle Reynolds numbers — 2 — - -- • -  or
             /—                          v           V
              V
r          radial coordinate

r,          gas bubble radius
 b         3
                       \
r          electric resistance at wire temperature T
 o                                                  o
S          area of the stagnation pressure tap of a pitot tube

S          turbulent Schmidt number related to the bubble
           diffusion; sensor sensitivity based on the traverse
           time, t, of an impacting bubble

S          sensor sensitivity to the impacting bubbles based on
 E         the voltage drop, e

S          sensor sensitivity to the velocity of the water
 u         stream
                         111

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s         distance from sphere center to the syringe tube orifice

T         time period measurement

T         ambient temperature of a sensor in water
Tf 1 'Tf 2   film temperature of the sensor in the air and water
          phases respectively

t         time coordinate; traverse time of a bubble; outside
          diameter of a pitot tube

U         mean axial velocity

U  .  ,U   mean axial velocity at the jet axis
 axis' m                    JT        j

U'        instantaneous axial velocity

U         jet efflux velocity

u         axial fluctuating velocity

uf        fluctuating velocity scale

u         radial fluctuating velocity scale

u         axial fluctuating velocity scale
 Ji

           /J

ufl        tangential fluctuating velocity

V         mean radial velocity; co-flowing velocity for bubble
          generation; general stream velocity

V         general stream velocity measured by pitot tube

V         mean velocity of the flow field with velocity gradient
          measured by the pitot tube

V        instantaneous radial velocity

V,         bubble velocity

V         average impressed velocity due to the wake of the
          detached bubble

V*        V/(d±f)

v         radial fluctuating velocity

v         velocity vector of bubbles and water mixture

v         velocity vector of bubbles
                        112

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vw         velocity vector of water

W          Weber number

W         instantaneous tangential velocity

w          tangential fluctuating velocity

x          axial coordinate

XG         potential core distance of the jet

xt         axial distance between dynamic and static taps
           of a pitot tube

P/PwfPa    fluid density, water density, gas density
pg
           Reynolds stress


 (.)        maximum quantity of  (.)


 n          r/(x+a)

            (c2/^)-1/3"


 C           (x+a)/D

 ^          mean concentration

 ^          concentration at efflux of the jet


 ^          instantaneous concentration

y          fluctuating component of the concentration

6          tangential coordinate

v          kinematic viscosity

 e  ,e  ,e    eddy diffusivity of momentum, bubble and marked
 » Y  YO  fiuid particle respectively

 V          mass diffusivity  (molecular effect)
                         113

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e         instantaneous DC voltage output of the total  signal
£         instantaneous DC voltage output of the turbulent
          signal
X         numerical constant related to mixing length
0)         27Tf
          particle parameter, defined in Equation  (X-l) and
          (X-5), respectively
A         longitudinal macroscale
 X
E(f)      energy spectrum in terms of frequency
F (K)      energy spectrum in terms of wave number
F(n)      J^dnf(n),
f(t)      half length of the wire exposed to the air bubble
f(n)      u/um
g(n)      v/um
g(w)      Fourier coefficient of E(f)
                ,2
h(n)
I(t)      instantaneous current across the sensor
K(i>      T/
-------
                       SECTION XVI

                       APPENDICES
APPENDIX I

Derivation of Equation VI-1

The averaged steady Navier Stokes equation in cylindrical
coordinates for an axi- symmetric turbulent jet, assuming
0* = U + u, V1 = V + v, W = w, P1 = P + p, 3_       92_

                                            rT9 = °'  2
                                                           = °' reads'
x-component  u   + v   - -
                                            v
r-component  uf| + vfj - - ±
                                                 v?)
where U1 , V , W are instantaneous velocities in the axial,
radial and tangential directions respectively and U, V, and W
are respectively the mean velocities and u, v, w are the
fluctuation  components .

The length scales LX, Lj. and LQ for the x, r and 0 directions
respectively may be defined.  Then L  Lft      (since the range
of mixing in axial direction is much larger than in the radial
direction) .  Letting ux/ ur and UQ be the corresponding velocity
scales and assuming that ur and UQ have the same order of
magnitude, the equation of mass conservation then gives the
following relationship
        Lx   Lr   Le
Furthermore, a fluctuation velocity scale uf such that
        u
             v
                  w
                           115

-------
     —  —    -     2
and  uv ^uw MTW ^R uf


can be defined.  R is the correlation  coefficient between two
fluctuation components and ranges between  0  and 1.   The order
of magnitude of the various terms in Equations  A-I-1 and A-I-2
is then given by
     ft "J"^ I  \f v ** ,ri   •
       l3x     "3r ~ " p" Ix    3x     r  ^r
        22             2             2
       u      u      Ap     u.p          R u..

order  =^     =^     -~    =r^-          -^-±
       it      I,      AI.     I.            Jj
        V      V       V     V            T*
        J»      «%       «•     *»            i
or
4
ux
Ruf Lx
-J'r
     »^+vg-,i-||. 1^(^-1=2^           (A-I-4,
              2,        .           2
      ux r   ux r       pr       uf

      Lx     Lx         pLr       Lr      Lx    Lr
                       .2      22       2      2_2
                       *r 
-------
         3U  .  „ 3U     1 3p   18  ,  —.
            +V=-"      (rUV)
       1  8p  .  9   ~T   v2 - w2
       p"  3r    Ir" V  + 	r	 = °

Equation A-I-6  can be integrated with respect to r to give

                        ~~2
                     dr 	
where PQ  is  the  pressure at the same section but outside the
turbulent region.   Equation A-I-7 states that the pressure in
a jet flow field is only a function of r and is independent
of x.  With  such equation (A-I-5)  simplifies to


      u|£+V|^=-i  |- (r a  )                           (III-l)
        9x     9r   pr  dr     xr


where
APPENDIX  II

Derivation of  Equations  (VI-3)  to (VI-5)
                              2
Dividing  Equation  (VI-1)  by U  one obtains


U   9    ,U .   V    9     U .    1 8   ,  r gxr
TT   "5v"   vn  '    TT   ay  VTT '    1- 3 T-  v     9  '
U   dX    U      U   dr   U     r dj.     -TT''                  /A TT  ^ '\
 o        o      o         o             pU                   (A-ll-1;


where U0  is  the jet efflux velocity.   The conservation of
momentum  requires  that

       00
          r dr  (L_) 2 = constant                              (A-II-2)
       o         o

Now denoting


      U   _                   ^J_ _ 1 'Jf  9 •_
      fT"  = ^^              ¥r ~ D   3n
       m
                         117

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V  _    ,  ,              3j_ _  *•_  3rj.  3£ ,  3»   9C
Ug  in;              3x ~  3t]  3?  3x   3?   3x            (A-II-



um                      _  i  n   d  a*  .  i
                                         D
CTxr
 xr = h  (n)
where n = §  *(£) and
then Equations A-II-1 and A-II-2 become
                               af
       d n n f  = Constant                                  (A-II-5


Now consider more closely the term occuring in Equation A-II-5.
It appears to consist of the product  of  two terms,  one of
which is a function of 5 alone.  Hence similarity can be achieved
only if these functions of C are constant,  i.e.  TJJ=A^(() where
is a numerical constant.  Substituting this relation into
Equation A-II-4 then
     <"f If + f2> + *3 Cg if - £ In

The terms in the above expression also  appear to consist of
two parts, one a function of C the  other  a function of n alone.
Hence similarity requires that


       -j|- = B 4)  , where B is an arbitrary constant.

A solution of this differential  equation  reads

      $ = -EL
      y   x+a
                            118

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hence
          A,  A,D
      111 = -P±=-±—
      *   C   x+a
In such a manner,  Equation A-II-6 becomes



      f2 + nff  -  gf '  +  i  *- (nh)  = 0                      (A-II-7)



Writing the  equation of  continuity in terms of f (n) and g(ri) ,
the function g(n)  in Equation A-II-7 can then be eliminated
and Equation A-II-7 simplified to



      - IF- rT  (F')2  +   2 F'  =    (rih)
where
              rT\
      F(n) =     n  f(n)   dn
              •"0

Equation A-II-8  after  integration yields

              FF«     f  rn
      h(n)= -^- = - =•     n  f (n)  dn                         (A-n-9)
              n       n  Jo

where the constant of  integration must be zero, since h(n) is
finite at n=0.   Writing  in  the original notation, Equation
A-II-9 becomes
      0        1  TT    f^       TT
       «»^»      T  f T    I '       II
       Xi      J.  U    I   J__  _ / W \                             /TTX O \
      —5- = -  —  rf~     dn  n (y—)                             (vi-3)
      oil          m  •* o        m
      K m


Furthermore, the similarity of the flow field requires that


<|> = En = _E_ , consequentely  n =  —r— or r = n (x+a) .   Now letting
    r'   x+a '      n      J      x+a

b  be the value of  r  where  the velocity is half the  maximum at
elltch section and kj, the  corresponding value of n /  then
      bu = k   (x+a)
                            119

-------
or


      !r = *b  <§ +  cr>

Equation  (VI-4)  states  that the velocity half width increases
linearly along the  axial  direction
          U           A,    A,  D
Moreover, g2L = i|;(5) = £=•  = 5^5- /  and letting l/^ = ku, then
      U
      _°_ = v   (5. + ..£)                                        (VI-5)
      U     u  ^D    D;
       m


Equation (VI-5) states  that  the inverse of the center line
velocity decay is also  linearly proportional to the axial
direction.

Equations  (VI-4) and  (VI-5)  .are the immediate consequences of
the similarity of the jet  flow field.

APPENDIX III

Derivation of Equation  (VI-11)

Introducing F(ri) as given  in Appendix  II into Equation  (VI-7)


                    F  dF
          ffi         TI  dn	
      Um  (x+a)      d   1  dF.
       m
or

                          2  d  ,1  dF,
      -P    -            _
       r dn   u   (x+a.)   '
               m

This equation can be  integrated readily to give


        £m      , dF    _..,,  _    12
      Um(x+a)   (T1dn" ~ 2F)  ~  ' 2 F '


The constant of integration  must be  zero, because at n-0r F(n)
must be zero.  The second  integration yields


                             120

-------
F(n)	:	_JL	
       1 +  [ um(x+a)/2em]cn2


The constant of integration C  follows  from  the  condition that
f(0) = 1.  This yields C=l/4.  Consequently
      u  _	
                                                            (VI-11)
       *»*             ill


APPENDIX IV

Derivation of Equations  (VI-19)  to  (VI-23)

Consider the body of water with  bubbles  as  a  "gas-water"  mixed
solution.  Let

      f-  =  volume of one gas bubble

      ^' =  number of gas bubbles per unit  volume  of solution

      p' =  mass of gas  per unit volume  of  solution  (=pg^v,  where
       g    p  is the gas density)

      p' =  mass of water per unit  volume of  solution (=p (l-Vlv),
            where p  is  the water density)
                   Vr

      p' =  density of the solution (= p' + p')

      v  =  velocity vector of gas  species

      v  =  velocity vector of water species     _,.       _,.
      ^                                       p1  v  + p1 v
      v  =  velocity vector of solution   (  =  —2—2—j	)
                                                   P
      n  =  mass flux vector of  gas (=p' v  )
      -»•                                     •*•
      n  =  mass flux vector of  water  (=p*  v  )
       w                                 w  w

      D  =  mass diffusivity  (molecular  effect)

then Pick's first law gives the  following relation (Bird,
Stewart and Lightfoot (I960)).
      ng -  ?  
-------
superimposed on the bulk convective  flow.  The  conservation
of mass for the gas species reads
          + V • n  =0                                      (A-IV-2)
      u w         g


Substituting Equation A-IV-1 into A-IV-2,  and noting  that
n"  + n"  = p1 v, then


      3p'        _       /     P1 \
      __£ + V-p' v = V /p'DV(^)•>•                          (A-IV-3)


After changing notation, the above becomes
                                                            (A-IV-4)

Since the bubble concentration is very low  (in the order  of
10   in volume) v'v << 1 and P <<:P-  Hence Pvlv +P^1~V ' v) ~P
or p'~p .  and Equation A-IV-4 can be approximated by
                                                            (A-IV-5)

In the present case, the bubble size is relatively small
such that the rising bubble velocity due to the buoyancy
effect is less than the carrier stream velocity, consequentely
Vg and v"^ will be of the same order of magnitude and then
p^v «p'v ,  The following relation is then approximately  true
 g y   w w
             v  + pw vw - pw vw -
               K            K      "

From the above expression, Equation A-IV-5 further simplifies
to

       -)      f        + ^      r        ^
          + V- (p v1 v)v .1 = VMDV(p v'v))-                  (A-IV-6)
              [^  g      wj     (    g    j
  at

In the above pg and v are constant scalars, so they can be
cancelled out.  Finally Equation A-IV-6 becomes

                            122

-------
                                                            (A-IV-7)
It  is noted  that  in  obtaining  the  above  expression the
solenoidality  of  the flow  field  has  been assumed.

In  steady  state axi- symmetric  turbulent  jet flow,  letting
and neglecting the molecular effect,  the final form of the
governing  equation for  the bubble  diffusion becomes
      u    +  v     =  -        (r
Similar  to Appendix  II  the  similarity  requirement gives

       V
       V0     2  x+a



           A2  xTa-k^>

                                   V
                        and  k (r\)  =  — .


Assuming that  the origin of the  apparent  source for concentration
diffusion is the same  as that  for  the momentum diffusion,  the
combination  of Equations  (VT-19),(VI-20)  and (A-II-3)  will give
the following  relationship


       _f *   (nk) +   dk = 1 d   f     S      dk>            (A-IV-8)
         dri        y on  n dri  ^ ' U  (x+a)   dnj


After  eliminating g(n)  by using  the  equation of continuity then

              (Fk) - ^  a^  [n um
where F(n) is as defined in Appendix  II.   Integrating the above
equation and noticing that the constant of integration is zero

                      eY       dk
      F(n) k(n) = - u   (x+a) n ^
                     m

The second integration will give the  expression  for  the


                              123

-------
concentration profile  as


             rn  (x+a) U.
   = exp
 /   fn  (x+a) u   /  ,n   „     -j
/.    	HI      ^(U  ) dT1]

I   J0   eYn     l  Jo   Um   >
Let by denote the value of  r where  the concentration is one
half of the maximum, k^ denote  the  corresponding value of
n then
           k   f- + 2-1
           Kh  1D + D'                                       (VI-22)



The equation  (VI-22) states  that  the  concentration half width
increases linearly along the axial direction.


Furthermore   V
              — = A0 -^—, and  for l/A0=kv then
              r     /. X-ra              £.   I
               O
      ^     Y  D   D                                        (VI-23)
       m

Equation  (VI-23) states that the  inverse  of the center line
decay of the concentration is  also  linearly proportional to
axial distance.
                             124

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                         APPENDIX V

                  ABSTRACTS OF PUBLICATIONS


1. "The Response of a Hot-wire Anemometer to a Bubble
    of Air in Water"

         The sensitivity of peak voltage and duration of the
    change in sensor voltages due to the impaction of differ-
    ent size bubbles are computed and measured.  Excellent
    agreement between these is found for bubbles somewhat larger
    than the sensor diameter and smaller than its effective
    length in water streams in a range of 1.5 to 9 feet per
    second.  The method suggests a reliable method for sizing
    bubbles in a water stream.  The effects due to nondirect
    hits are not treated.

2. "Bubble Formation due to a Submerged Capillary Tube in a
    Quiescent and Co-Flowing Streams"

         The case of bubble formation in both quiescent and
    moving streams due to the injection of a constant gas flow
    through a small tube is considered.  Relationships predicting
    the expected size and quantity of bubbles generated are
    proposed.  These are compared with measurements taken with
    stream velocities up to 9 ft/sec, while generating gas bubbles
    from 40 to 700 microns in diameter.

         For the case of generation in a quiescent stream the
    forces due to the virtual mass, surface tension, viscous
    drag, buoyancy, and the wake formed by the preceding bubble
    are accounted for.  There still remains some question (only
    partly answered by a comparison with measurements)  as to
    the proper added mass coefficient and the geometry of the
    bubble previous to detachment, as well as an adequate
    estimate of the interaction with a preceding bubble's wake.

         The proposed model for generation in a moving stream
    is in good agreement with actual measurements for co-flowing
    velocities between 1 and 9 fps and capillary tubes in the
    order of 10~3cm in dia.

3. "Dynamic Simulation of the Turbulent Diffusion of Small
    Particles"

         The equation of motion of a small spherical nonrotating
    particle was solved numerically in a two-dimensional homo-
    geneous and isotropic turbulent field.  Ensembles of solutions
    were obtained for particles of different sizes and densities...
    It was shown that the turbulent transport coefficient in-
    creases with particle size and decreases with particle
                             125

-------
    density...  The results are in agreement with available
    measurements.

4. "Analytical  Prediction of the Turbulent Diffusion of Small
    Particles"

         A comparison of various measurements has consistently
    suggested an unexplained increase in the turbulent transport
    of small suspended particles with size.  A comparison with
    the momentum turbulent transport coefficient suggests an
    increase of the inverse of the turbulent Schmidt number (or
    the ratio of mass to momentum transport coefficients)  from
    values close to I/ for zero-size particles, to values as
    large as 5, for larger particles.

         Based  on the particle equations of motion, and postula-
    ting certain relationships between the statistics of the
    particle velocity fluctuations and the turbulent carrier
    phase, a prediction of the particle transport coefficient
    is made. The analysis predicts the same increasing trend
    of turbulent transport coefficient with particle size.  By
    limiting the study to a particular range of particle Reynolds
    number good agreement is noted with the experimental data.

5. "Energy Spectrum and Turbulent Scales in an Axi-Symmetric
    Water Jet" :

         The time micro and macroscales are computed from
    measured energy spectra in the fully developed region of a
    circular jet.   The corresponding longitudinal scales are
    approximated using Taylor's frozen turbulence  hypothesis.
    The microscale is found essentially constant whereas the
    macroscale, although increasing linearly along the axis,
    does not show similarity in the total field.

6. "Turbulent Diffusion of Small Particles Suspended in Turbulent
    Jet"

         The dispersion of liquid droplets in plane two dimen-
    sional air  jets has been measured and compared with similar
    results in  the literature.  From careful measurements of
    the concentration flux profiles the corresponding turbulent
    transport coefficient is determined.  The results show that
    within most ranges of interest turbulent transport increases
    with particle size.

    The results are not only compared with each other, but also
    with an analysis based on the assumption of nonrotating
    spherical rigid particles acted upon by viscous drag given
    by Stokes Law.  The approximate analysis predicts the same
    trend as noted in the experiments.
U.S. GOVERNMENT PRINTING OFFICE: 1974- 544-319:391
                             126

-------
 SELECTED WATER
 RESOURCES ABSTRACTS

 INPUT TRANSACTION FORM
                                        Rep"TtNo.
3.  Accession No.
                                                          w
 4.  Tit If

 TURBULENT  DIFFUSION IN LIQUID JETS:  FINAL REPORT
 Strong  C.  Chauno and Victor W. Goldschmidt
 9.  Organ* MtK>n
112. Spo

 IS. Sun
          Engineering Experiment Station
          School  of Mechanical Engineering
          Purdue  University
          Lafayette, IN 47907
nsoring Organization
                                                          5.  ReportD&e

                                                          6.

                                                          8.  Performing Orgae-'fation
                                                             Re port No.
                                                          10.  Project No.
                                                             16070  DEP
                                                                 II,  Contract/Grant No.

                                                                     16070 DEP
                                                                 13.  Type c ' Report and
                                                                    Period Covered
  5. Supplementary Note.*:

  Environmental  Protection Agency Report Number, EPA-660/3-74-004b,  March 1974.
 '5. A bstract

 Laboratory studies were conducted on the dispersion of gas droplets  of different
 sizes  1n turbulent water jets.  The main purpose was to determine  the turbulent
 transport  coefficient of contaminants suspended 1n turbulent flows.

 The experimental  results were compared to measurements of diffusion  of liquid
 droplets 1n air jets as well as to a numerical analysis based on the equations of
 the particles  themselves.

 The results confirm that small particles in turbulent flows have an  increasing
 turbulent  transport coefficient with size.  The collated experimental results
 exhibit when Reynolds analogy (in the transport of mass and momentum) can
 be validly employed.
 17a. Descriptors

 Bubble,  Diffusion, Dispersion, Equations, Instrumentation, Turbulence, *Turbulent
 Flow.
 176. Identifiers
  Bubble  Sampling, Bubble Sizing, Concentration of Contaminants,  Hot Film Anemometer,
  Jet  Flow,  Liquid Jets, *Turbulent Diffusion, *Turbulent Transport.
fjTc.
18.
mbs
COWRR Field &
Group
Availability

G. R.
OR B
/*,
20.
Dltsworth

S -nhy C'iss.
(Report)
Sfcuri ty Class.
(P.jge)
21.
22.

No. of
Pages
Price


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