AIR   POLLUTANT   EMISSION   INVENTORY
         OF  NORTHWEST   INDIANA
             A  PRELIMINARY SURVEY
                    1966
U.S. DEPARTMENT OF HEALTH, EDUCATION, AND WELFARE
             PUBLIC HEALTH SERVICE


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    AIR  POLLUTANT  EMISSION   INVENTORY

           OF  NORTHWEST   INDIANA
                A  PRELIMINARY SURVEY
                       1966
                        by
                     G. Ozolins
                     C. Rehmann
         CONDUCTED FOR NORTHWEST INDIANA
         AIR RESOURCE MANAGEMENT PROGRAM
U. S. DEPARTMENT OF HEALTH, EDUCATION, AND WELFARE
                 Public Health Service
   Bureau of Disease Prevention and Environmental Control
                Durham, North Carolina

                      April 1968

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National Center for Air Pollution Control Publication APTD-68-4

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                                  FOREWORD
    The Northwest Indiana Air Resource Management Program is a. cooperative
effort initiated in March, 1965, by the cities  of Gary and East Chicago, the
State of Indiana,  and the U. S. Public Health Service.  The primary purpose
of this program is to assist and strengthen local agencies in developing and
implementing an area-wide air resource management plan.  This study was
prepared at the request of the Program Executive Committee.  Its purpose
is threefold:  (1)  to provide a preliminary but comprehensive inventory of
the air pollutant emissions from the entire area;  (2)  to help initiate the air
resource management programs in Hammond and Whiting, Indiana; and
(3) to provide guidelines for  future,  more detailed surveys, similar to those
presently conducted by the  cities of Gary and East Chicago.
    This report is the result of a joint effort  by the air pollution  control
agencies and health departments of East Chicago, Gary, Hammond,  Whiting,
and the  National  Center for Air Pollution Control.  As in all emission surveys,
the data presented here are estimates and should not be  interpreted  as actual
values.   They are, however,  of sufficient accuracy and validity to allow their
use in developing and improving an air resource management program.
                                       111

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                                  ABSTRACT
Sources of air pollutant emissions were surveyed to quantify the total pollution
load emitted to the air over the Northwest Indiana communities of East Chicago,
Gary,  Hammond,  and Whiting.   The emissions are reported on an annual basis
and subdivided into the five major pollutants:  particulates,  sulfur oxides, nitro-
gen oxides, hydrocarbons,  and carbon monoxide.  The four  major source cate-
gories that were utilized in reporting emissions from area and point sources are:
fuel combustion in stationary sources, fuel  combustion in mobile sources, com-
bustion of refuse,  and industrial process  losses.  The results of this survey are
reported by city and illustrated on the grid system established by the Northwest
Indiana Air Resource Management Program.

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                                  CONTENTS
INTRODUCTION	     1
STUDY AREA    	     2
SUMMARY OF RESULTS	     6
     Emissions by Category	     3
           Fuel Combustion in Stationary Sources	     8
                Industry	    13
                Steam-Electric Utilities   	    13
                Residential  	    14
                Other	    15
           Fuel Combustion in Transportation Vehicles	    15
           Combustion of Refuse Material	    15
           Industrial Process Emissions   	    18
                Steel Manufacturing	    21
                Oil Refineries	    21
                Chemical Industry	    21
                Cement Manufacturing   	    21
                Foundries	    21
     Emissions by Geographical Area	    22
SUMMARY	    34

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                     AIR POLLUTANT EMISSION  INVENTORY
                                       OF
                              NORTHWEST INDIANA
                            A PRELIMINARY SURVEY
                                      1966
                               INTRODUCTION
    This report presents the results of a rapid emissions inventory of air pollu-
tant sources in Northwest Indiana. The objectives of this study are to determine
the total quantities of the various air pollutants emitted and to estimate, as
accurately as possible, the geographical variation in air pollutant emissions.
To accomplish this, the study area was divided into a grid system and the emission
quantities are reported in terms of tons of pollutant per grid on an annual basis.
    The pollutants considered in this survey  carbon monoxide, hydrocarbons,
nitrogen oxides,  sulfur oxides and particulates  - are those emitted in large
quantities from the variety and multitude of sources  dispersed throughout the
area.  The emissions  of pollutants not considered herein are generally associated
with a specific process or operation and, in general, are not distributed through-
out the community.
    The sources of air pollution, as used in this report, are subdivided into the
following four categories:
    1.  Fuel combustion in stationary sources.
    2.  Fuel combustion m transportation vehicles.
    3,  Combustion of refuse material.
    4.- Industrial process emissions.

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                                 STUDY AREA
      The study area,  shown on Figure 1, includes the Northwest Indiana com-
munities of East Chicago, Gary,  Hammond,  and Whiting.  The total land area
involved in the study is approximately 85 square miles.  The 1960 population
was 355, 824.
      According to census figures the population in the study area has increased
by 24. 6 percent from 1950 to I960, and in the Gary-Hammond-East  Chicago
Standard Metropolitan Statistical Area,  which includes Lake and Porter Counties,
the population has increased by 40. 5 percent.  The population of the area outside
the central cities has increased by 70. 5 percent.  Of the four cities, Gary  has
had the largest increase in population, 33 percent, and Whiting has  the only
decrease in population, 15. 8 percent. Figure 2 shows the distribution of the
population  of the study area by grids.
      The area included in this study has a  variety of industries, but three  large
steel mills and four large petroleum refineries located near or on the shores of
Lake Michigan dominate the industrial complex.  Other industries in the area
tend to be  support activities for the steel and petroleum industries.  Foundries,
steel fabricators, and chemical plants are  the largest group of support industries
while two large power utilities and a large  cement manufacturing plant make up
the large single industries not directly supported by these two major industries.
      The study area also includes some  industry that is divorced from the
petroleum  and steel industries.  The printing and publishing, grain, soap,
textile, and building material industries  are  well represented.  Various types of
small manufacturing plants are also located in the four communities.
      Almost 200 of the 400 industrial plants-in-_the area .employ more than 20
employees.  The total number of employees in the study area is approximately
100, 000; approximately 60 percent of them  are in the primary metals industry,
and 9 percent are employed in both the petroleum and metal  fabrication industries.
      The automobile traffic in the study area is handled by a number of major
arteries.   The Indiana toll road and the  Tri-State Highway, which bound the study
area on the north and south, handle most of the east-west traffic, Indianapolis
Boulevard, Calumet Avenue,  Kennedy Avenue,  Grant, and Broadway handle a
large portion of the north-south traffic.
2

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                380  385  390  395
LAKC CJ>LUHir
1530


1525
          1515
   CAIUMET
     CITY
          1505


          1500


          1495


          1490


          1485


          1480
                                  400 405 410  415
                                                           LAKE MICHIGAN
                                                   420  425  430 435 440  445  450 455  460 465
                                                                                      1505
                 380  385 390  395  400 405  410  415  420


                                                  1470


                                                  1465
                                                        425  430 435  440 445
                                                                                        MILES
                                 Figure  1.   Location map of study  area.

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                380 385  390  395
                   1
Ltff C4iUMfT
   CALUMET
    CITY
                                 400 405 410 415
                                                          LAKE MICHIGAN
                                                  420  425 430  435 440 445  450 455 460  465
POPULATION DENSITY,
    persons/mi^
[     ;[   1,000 -" 5,000
        5,000 -  10,000
       10,000 -  15,000
385 390 395 400  405  410 415  420

                            1470

                            1465
                                                                           450  455  460 465
                                                                          1475
                        HOBART
                     1470

                     1465
I
N
425 430 435 440 445
                                                                 MILES
              Figure 2.  Population densities in Northwestern Indiana communities.

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     In the development of the Northwest Indiana Air Resource Management
Program,  the Executive Committee adopted a grid system encompassing the
entire  study area covered  in this report.  The grid system consists of 10, 000-
foot squares designated on the United States Coast and  Geodetic Survey maps
of the Northwest Indiana Area.  The grid system used throughout this report
is the same grid system as that adopted by the Northwest Indiana Air Resource
Management Program except that this grid system is subdivided into 5, 000-
foot squares.

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                             SUMMARY OF RESULTS

      The following is a brief summary of pollutant emissions and sources in the

 study area:

      1.  Particulate matter is  emitted primarily from industrial processes,  coal

 combustion, and refuse disposal.  Particulate emissions from industrial processes

 contribute 76 percent,  from coal combustion contributes 20 percent,  and from

 refuse disposal contributes 1 percent of the total emissions.

      2.  The burning of fossil fuels  contributes approximately 86 percent of the

 total amount of sulfur oxides emitted in the study area.  The combustion  of coal

 accounts for 66 percent,  and the combustion of fuel oils contributes 19 percent

 to the total amount of sulfur oxides emitted. Industrial process emissions account

 for 14 percent of the total amount of sulfur oxide emissions, but lack  of data on

 certain industrial processes  does not give a complete picture  of this source.

      3.  Oxides of nitrogen are emitted primarily from two sources, combustion

 of fuels and transportation.   The  combustion of coal accounts  for 38 percent of

 the total emissions and the combustion of fuel oils accounts for 40 percent of the

 total.  The combustion of natural gas accounts for 13 percent, and the combustion

 of gasoline in automobiles accounts for 8 percent of the total amount of nitrogen

 oxides emitted.

     4.  The emission of hydrocarbons is accounted for in three major sources

 industrial processes, transportation,  and refuse disposal.   Industrial processes

 account for 58 percent of the total emissions, the motor vehicle accounts for  24

 percent, and the disposal of refuse contributes 15 percent to the total emission of

 hydrocarbons.

     5.  Industrial process  emissions account for 24 percent  of the total amount

 of carbon monoxide emitted,  and motor vehicles account for 72 percent of the

 total.

     The emissions  of pollutants discharged in the study area are listed in Table

 1.   The accuracy of the results  depends on the  accuracy and applicability of the   (

available emission factors and the information available concerning the specific

processes  in which large quantities of pollutants are emitted.  The emission

factors, for the most part, represent the average emission rates for  a particular
 6

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Table 1.  SUMMARY OF AIR POLLUTANT EMISSIONS IN NORTHWEST INDIANA

                                  (tons/year)
Partic-
Source category ulates
Transportation
Combustion of fuels
Stationary sources
Industry
Steam-electric utilities
Residential
Other
Subtotal
Refuse disposal
City dumps
On-site burning
Subtotal
Industrial process
emissions
Totals
780


39,260
13,390
1, 520
1,170
60,340

280
2,680
2,960

208,800
272,880
Sulfur
oxides
630


138,960
149,500
10,180
2,320
300,960

10
50
60

49,000a
350,650a
Nitrogen
oxides
7,910


58,930
25,330
2,920
430
87,610

--
30
30

840
96,390
Hydro-
carbons
27,700


1,080
230
610
230
2, 150

1,680
15,960
17 , 640

66,800
114,290
Carbon
monoxide
204,000


2,000
570
2,840
1, 120
6,530

500
4,785
5,285

66,800
282,615
  Does not include sulfur oxide emissions from 3 refineries.


industry or fuel group.  Because of the differences in emissions  rates among the

plants or fuel users within a given category, the application of the emission
                              \
factors, as applied to an individual plant,  could result in a considerable dis-

crepancy between the actual and calculated emissions.


      The incompleteness of data relating to pollutant emissions from some

processes and fuel uses has resulted in the omission of some  air pollutants and

air pollution sources in the area.   These omissions have primarily been confined

to area sources or to sources contributing a relatively small amount of pollu-

tants.  The emissions inventory should therefore be fairly representative of

total area emissions of the  principal pollutants.

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EMISSIONS BY CATEGORY

      For purposes of compiling basic data and calculating emission quantities,

the air pollution  sources are grouped into four categories:

      1.  Fuel combustion in stationary sources.

      2.  Fuel combustion in transportation vehicles.

      3.  Combustion of refuse material.

      4.  Industrial process emissions.

      Each of these categories is,  in turn,  subdivided in a number of subgroups

some according to type or size  to allow estimates of the geographical variation

in pollutant emissions.  In the following discussion the various information

sources  are documented, assumptions made are cited, and the resulting emission

quantities are summarized.

Fuel  Combustion in Stationary Sources

      The combustion  of fuels is one of the principal sources  of air pollutant

emissions in urban areas.  The combustion of fuels releases various products

that deteriorate the quality of the urban air.

      The major fuels used in the  study area are coal, fuel oil, natural gas, and

process  gas.   The primary consumers of the three major fuels are: industry,

steam-electric utilities,  and residential dwellings.*



      Table 2 summarizes the  annual fuel consumption for the study area, and

Table 3 subdivides the annual fuel  consumption into use category and political

subdivisions.  The fuel consumption data for the  study area were obtained

through the use of a variety of techniques and from numerous information

sources.  Where possible, data have been cross-checked by using different

techniques and other sources of information.  The annual consumption of

natural gas was furnished by the local utility, and Bureau of Census data for

1962 were used for annual consumption of coal and fuel oil.
 *To more accurately define the sources of pollution and provide better estimates
 of emissions, a fourth category,  Other Consumers, was used.  Included in this
 category are commercial sources that primarily use fuel for space heating.

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       Table 2.  ANNUAL FUEL CONSUMPTION IN NORTHWEST INDIANA
Fuel
Coal, tons /yr



Fuel oil, gal/yr



Gas, million ft /yr



Consumer category
a
Industry
Steam-electric utilities
Residential
Other
Total
Industry
Steam-electric utilities
Residential
Other
Total
Industry
Steam -electric utilities
Residential
Other
Total
Annual
consumption
1,306, 000
2,290,000
111,000
45,000
3,752,000
271,656,000
	
54,600,000
b
na
326,256, 000
79,445
12,461
9,534
4,487
105, 927
Percent
of total
34.8
61.0
3.0
1.2
100.0
83.3
--
16.7
b
na
100.0
75.0
11.8
9.0
4.2
100.0
 aAn additional 12, 488, 000 tons is used in the production of coke.

  na - Information not available or not reported.
      Table 4 specifically locates the major fuel consumer categories in the study

area and gives total consumption of each of the specific fuels used in both process
                             |
heating and area or space heating.  The steam - electric  utilities, the major

users of coal,  consume 61 percent of the area total annually.  Industry consumes

83 percent of the fuel oil and 75 percent of the natural gas.  Industry,  consuming

35 percent annually, is also the second largest user of coal.


      The Mid-West Coal Producers Institute provided the quantities of coal of

Midwestern origin that was shipped into this area. Table 5  shows the  distribu-

tion , usage, and chemical composition of this coal.  This information was not

made available until after the calculations  were completed.  The sulfur and ash

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                 Table  3.  ANNUAL FUEL CONSUMPTION BY POLITICAL SUBDIVISIONS
                                     OF  NORTHWEST INDIANA, 1966

Fuel
Coal, tons/yr

Fuel oil,
gal/yr

Gas, million
ft3/yr


Jurisdiction
Hammond
East Chicago
Gary
Whiting
Totals
Hammond
East Chicago
Gary
Whiting
Totals
Hammond
East Chicago
Gary
Whiting
Totals
User category

Industry
115,870
726,060
308,850
125,000
1,275,780
3,798,700
308,247,400
96, 886,300
9,430,000
418,862,400
4,334
48, 178
22,407
4,526
79,445
Steam -electric
plants
1,161,000
1, 129,000
2,290,000
--
--
11,561
900
12,461

Residential
33,520
25, 900
47,630
3,950
111,000
15,558,000
8, 030,000
30,070,000
942,000
54,600,000
3,273
1, 103
4,963
195
9,534

Other
15,000
7,000
22,000
1,000
45,000

na
1,311
775
2,288
113
4,487

Totals

3,752, 000

326,256,000

105,929
na - Information not available or not reported.

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Table 4.  MAJOR FUEL CONSUMERS IN STUDY AREA
            BY INDUSTRIAL CATEGORY

City
East Chicago

Gary

Hammond

Whiting



Category
Chemical and allied products
Stone, clay, glass products
Primar y_metals industries
Petroleum and coal products
Totals
Chemical and allied products
Stone, clay, glass products
Primary metals industries
Transportation equipment
Power utilities
Totals
Chemical and allied products
Stone, clay, glass products
Primary metals industries
Power utilities
Food and kindred products
Printing and publishing
Paper and allied products
Totals
Petroleum and coal products
Chemical and allied products
Totals
Area totals
Annual fuel consumption
Coal,
tons
92, 500
5, 561
628,000
726, 061
280,000
34,856
1, 129,000
1,443,856
5,876
1, 161,000
110,000
1,276,876
125, 000
125, 000
3,571,793
Fuel oil, gallons

Residual
211,800
63, 900
242,270, 000
64, 364, 000
306, 909, 700
520, 000
2, 000, 000
91,389,700
392, 000
94,301, 700
389, 200
1, 725, 000
854, 000
400, 000
3, 368,200
9,500, 000
430, 000
9, 930, 000
414, 509, 600

Distillate
31,700
1, 306,000
1,337,700
4, 585, 000
4,585,000
388,000
42, 500
430, 500
— —
--
6, 353,200
Gas, 106ft3

Natural
1, 307
412
36,617
38,336
3
921
22,557
900
24, 381
1, 585
264
912
11, 561
170
310
14,802
4
2, 500
2, 504
80, 023

Process
43, 000
26,460
69,460
382,931
382,931
--

16, 000
2, 000
18, 000
470, 391

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            Table 5.  MIDWEST COAL ASSOCIATION SUMMARY OF


        MIDWESTERN COAL SHIPPED TO NORTHWEST INDIANA AREA


To Whiting from:
Western Kentucky
Southern Illinois
Western Kentucky
Total and Averages
To Hammond from:
Southern Illinois
Indiana
Fulton County
DuQuoin
Indiana
Western Kentucky
Belleville and
South Illinois
Total and Averages
To Gary from:
Central Illinois
Southern Illinois
Indiana
Western Kentucky
Danville
Belleville
Southern Illinois
Indiana
Western Kentucky
Belleville
DuQuoin
Total and Averages
To East Chicago from:
Fulton County
Central Illinois
Belleville
Southern Illinois
Indiana
Western Kentucky
Southern Illinois
Total and Averages
a
Use

RT
IN
IN


RT
RT
IN
IN
IN
IN

UT


RT
RT
RT
RT
IN
IN
IN
IN
IN
UT
UT


IN
IN
IN
IN
IN
IN
MT

Coal shipped,
tons

101
36, 900
165,814
252,815

108
1,453
6,234
371
2, 098
1,469

1, 673, 944
. 1,685,677

54
306
576
584
13,619
52,864
32, 117
79,236
121,821
996,987
249,424
1,547, 588

101,570
6, 146
633
44, 175
5,834
18, 078
351, 632
528, 068

Moisture, %

10. 10
7.90
8.34
8. 19

7.22
13.00
14.78
10.00
13.77
8.34

13.66
13.66

12.00
7.22
13.00
10. 10
13.35
10.68
7.90
13.77
8.34
10.60
9.80
10.43

14.74
13.40
10.68
7.90
13.77
8.34
9.20
10.23

Ash, %

6.00
7.84
6.36
6.87

7. 90
7.50
7.03
8.60
6.47
6.36

10.26
10.24

8. 10
7. 90
7. 50
6. 00
7. 51
9.71
7.84
6.47
6.36
9.93
15. 10
10.23

7. 18
8. 60
9.71
7.84
6.47
6. 36
5. 90
6.37

Sulfur, %

2.95
1.88
2.91
2.56

1.86
2.72
2.77
2. 72
2.29
2.91

3.38
3.38

3.44
1.86
2.72
2.95
2.67
3.27
1.88
2.29
2.91
2. 87
2. 60
2.79

2.52
3.40
3.27
1.88
2.29
2.91
1.03
1.50
aRT   coal used for retail purposes; IN - coal used for industrial purposes;

 UT - coal used for electric utility purposes;  MT  coal used for metallurgical
 purposes.

12

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contents of the coal were assumed when they were not made available by the parti-

cular consumers of coal, and the sulfur contents of the residual and distillate

fuel oil were also assumed and used under the same circumstances.  A sulfur

content of 2. 7 percent and an ash content of 10 percent for coal,  and a sulfur

content of 0. 4 percent for distillate (number 1 and 2 oil) and a sulfur  content of

1. 5 percent for residual (numbers 4 and  5  oil) fuel oil were assumed  for the fuels

that did not have their composition reported.  A weighted average of all the re-

ported fuels with their respective compositions was  calculated to estimate the

assumed composition of the other fuels. Pollutants should  be  recalculated to be

comparable with the analysis as stated in Table 5.


      Air pollutant emissions from fuel combustion in stationary sources are

summarized in Table 6 by user category.  The combustion of coal accounts for

over 70 percent by weight of all the pollutants emitted from this source category.

Coal combustion accounts for 99 percent of the carbon monoxide, 93 percent of

the particulates, 77 percent of  the sulfur oxides, 42 percent of the nitrogen oxides,

and 77 percent of the hydrocarbons emitted from fuel combustion.  Fuel oil

accounts for 23 percent of the sulfur oxides and 44 percent of the nitrogen oxides

emitted.  Gas accounts for only 14 percent of the nitrogen oxides emitted from

fuel combustion.


Industry - Industry consumes 1, 306, 000  tons of coal,  271, 656, 000 gallons of fuel

oil (mostly residual),  and 79,445 million cubic feet of gas for process heat,

power generation,  and space heating and 12, 488, 000 tons  of coal for coking

annually. The emissions from the combustion of fuel amount to 39, 260 tons

of particulates, 138, 965 tons of  sulfur oxides, 58, 930 tons  of nitrogen oxides,

2, 000 tons of carbon monoxide,  and  1, 080  tons of hydrocarbons annually.  The

following percentages of the total amount of pollutants emitted from fuel combus-
                              I
tion in the study area are attributed to industrial fuel combustion:

                      particulate            65 percent

                      sulfur oxides          46 percent

                      nitrogen  oxides        67 percent

                      hydrocarbons          50 percent

                      carbon monoxides      30 percent


Steam-Electric Utilities   Utilities are the major user of  coal; they consume

2, 290, 000 tons annually.   They also consume 12, 460 million cubic  feet of gas
                                                                               13

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      Table 6.  AIR POLLUTANT EMISSIONS FROM COMBUSTION OF  FUELS



             IN STATIONARY SOURCES IN NORTHWEST INDIANA



                                   (tons/year)

Fuel
Coal




Fuel oil




Gas






User category
Industrial
Steam-electric
Residential
Others
Totals
Industrial
Steam- electric
Residential
Others
Totals
Industrial
Steam-electric
Residential
Others
Totals
Total emissions
Carbon
monoxide
2, 000
570
2,780
1, 120
6,470
5
--
55
--
60
n
n
2
n
2
6, 532
Hydro-
carbons
650
230
560
225
1,665
430
--
55
--
485
n
n
n
--
n
2, 150
Nitrogen
oxides
13,060
22,900
400
180
36,540
36,490
—
1,970
—
38,460
9,380
2,430
550
245
12,605
87,605
Sulfur
oxides
74, 150
149, 500
6, 750
2, 320
232, 720
64,800
--
3,430
--
68,230
15
2
2
n
19
300, 970

Particulates
35,625
18, 300
1, 100
1, 125
56, 150
2,920
--
330
--
3,250
715
90
90
40
935
60,335
n   Negligible.





annually as a secondary fuel.   The use of electrostatic precipitators in both of



the power plants reduces the emission of particulates to  18,390 tons annually.



Steam generating plants are one of the major sources of  sulfur oxides, however,



with annual emissions  of 149,500 tons.  The amounts of nitrogen oxides,  carbon



monoxides, and hydrocarbons emitted annually from, fuel combustion for power



generation are, respectively,  25,330 tons, 570 tons,  and 230 tons.





Residential - The combustion of fuels  in residential dwellings accounts for



111, 000 tons  of coal,  54, 600, 000 gallons of fuel oil (mostly distillate), and



9, 500 million cubic feet of gas. Annual emissions from  the combustion of this



14

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fuel are:  1, 545 tons of particulates,  10, 180 tons of sulfur oxides, 2, 610 tons of



nitrogen oxides,  620 tons of hydrocarbons,  and 2,840 tons of carbon monoxide.




Others   The  commercial establishments use 45, 000 tons of coal and 4, 500



million cubic  feet of gas primarily for space heating.  The quantity of fuel oil



consumed by commercial establishments is not available from the sources con-



tacted.   This  quantity of fuel should be defined to complete the fuel balance for



the study area.   The amount of pollution from this  source is not as great in



quantity as from residential fuel combustion; but the concentration of the



commercial sources is confined to specific areas within the four cities  and their



contribution is, therefore,  significant.  Pollutants  from commercial sources



amount to 1, 170  tons of particulates,  2, 320 tons of sulfur oxides,  425 tons of



nitrogen oxides,  225 tons of hydrocarbons,  and 1, 120 tons of carbon monoxide



emitted annually.





Fuel Combustion in Transportation Vehicles



      The transportation sources  of air pollution include any vehicles that are



powered by the combustion of fuels.   The lack of traffic surveys and the lack of



data on gasoline  and dies el fuel consumption limited  this category to automobile



emissions in the total study area.




      The total emissions from automobiles were estimated  by using gasoline



sales in the area and converting this figure to gallons of gasoline. Although only



an estimate, the results correlated well with similar surveys conducted in other



areas.




      Automotive exhaust is estimated to contribute 204, 000 tons of carbon mo-



noxide, 27,700 tons of hydrocarbons, 7, 910 tons of nitrogen oxides, 630 tons of



sulfur oxides, and 780 tons  of particulates.  This amounts to 72 percent of the



total emission of carbon monoxide and 24 percent of the total emission  of hydro-



carbons from all sources in the study area.




      Since traffic flow maps were not available for the entire area,  no attempt



was made to distribute the  emissions from transportation throughout the study



area.





Combustion of Refuse Material



      Most of the refuse generated in the study area  is disposed of in three ways:



city-controlled landfills, industrial dumps,  and on-site burning.  On-site means
                                                                               15

-------
 that the refuse is disposed of on the premises on which it is produced.  Certain
 industries,  large apartments, and some commercial establishments are equipped
 with incineration facilities; but this factor was not considered because of the
 lack of specific data.
       Municipal landfills are subject to intermittent burning,  which along with
 on-site burning,  constitutes a substantial source of pollution. Estimating  air
 pollutants emitted annually from open burning and incineration of refuse was
 difficult because accurate data on the quantities of refuse burned was unknown.
       To estimate air pollutants from solid wastes,  information  from local sani-
 tation and health agencies was gathered to determine the  amount of wastes
 generated.  This total amount was subdivided among the  different modes of
 disposal.
       Certain assumptions and estimates had to be made  in order to determine
 the quantity of  refuse generated and disposed in the area. National averages of
 1. 0 pound per capita per day for noncombustible and 3. 5  pounds  per capita per
 day for combustible 'were used to determine the quantity  of refuse generated in
 the four communities.  As shown in Table 7, the total quantity was estimated
 to  be  290, 500 tons of refuse per year.  The refuse is composed of 227, 000 tons
 of  combustible  refuse and 63, 500 tons of noncombustible  refuse.
       The location of this refuse in the communities was accomplished by using
 information received from the local sanitation agencies.  From  this information
 the amount of refuse disposed of by on-site burning was estimated by taking the
 difference between the amount of refuse generated in the  area and the amount
 of  refuse taken to the city dumps.  On-site disposal was  assumed to be exclusive-
 ly  by  burning.
       The amount of refuse burned openly in the city landfills  is unknown.  Calcu-
 lation of the pollutants emitted from the city landfills was based  on burning of an
 estimated 10 percent of the combustible material  received.   This estimate is  an
 arbitrary assumption and should be interpreted as such.
       Table  8 shows  the amounts of pollutants  emitted from the burning of  refuse
 from  the different modes of disposal.  Disposal by on-site burning accounts for
 approximately 40 percent of the total refuse generated in the  study area.   This
 method of disposal accounts for over 80 percent of the pollutants emitted in each
16

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            Table 7,  REFUSE DISPOSAL IN NORTHWEST INDIANA
"
Location
Hammond

E. Chicago

Gary

Whiting


Population
111, 648

57,669

178, 320

8, 137

Total Refuse
Types and quantities of
refuse generated
Type
Combustible
Noncombustible
Combustible
Noncombustible
Combustible
Noncombustible
Combustible
Noncombustible

Quantity,
tons/yr
71, 000
20,000
37, 000
10, 000
114,000
32,000
5, 000
1, 500
290, 500

Mode of disposal
City dump
Landfill
28, 000
20,000
27, 000
10,000
43, 000
32,000
3,000
1, 500
164,500
Burned
3, 000
--
3, 000
--
5, 000
--
1, 000
--
12,000
On-
c
site
40,000
--
7,000
--
66,000
--
1, 000
--
114,000
 Quantities of refuse generated were based on observed national averages of 3. 5
 pounds per capita per day for combustibles and 1.0 pound per capita per day for
 noncombustible.
 Quantities of refuse taken to city dumps are based on estimates from local
^sanitation agencies.
"On-site quantity was taken as the difference between refuse generated and de-
 posited at city dumps.

         Table 8.  AIR POLLUTANT EMISSIONS FROM REFUSE BURNING


Location
Hammond

E. Chicago

Gary

Whiting

Totals


Source
City dump
On-site
City dump
On-site
City dump
On-site
City dump
On-site

Pollutants, tons/yr

Particulates
70
9,40
70
20
120
1,550
20
20
2,810
Sulfur
oxides
2
16
2
3
3
26
n
n
52
Nitrogen
oxides
n
10
n
1
1
16
n
n
28
Hydro-
carbons
420
5,600
420
980
700
9,240
140
140
17,640
Carbon
monoxide
125
1,630
125
295
210
2,770
40
40
5,285
 n   Negligible.

-------
category from refuse burning.  The amounts of each pollutant from on-site burn-
ing were distributed by population densities throughout the study area.  Since
these totals were obtained by differences,  any error in the assumed per capita
generation or in the quantities handled at the collective disposal sites will be
reflected in these figures.
      Although 60 percent of the total refuse is estimated to be disposed at the
city landfills,  only approximately 10 percent of the total pollutants are ascribed
to this method of disposal.   The amounts burned at these locations is only an
estimate, and  the air pollution estimates are,  therefore, thought to be conservative.
      Additional information on amounts  of refuse burned at the landfills at
specific industrial dumps, and at commercial  and domestic incinerators is
needed to refine the emission quantities  from refuse disposal.  Emissions from
refuse disposal are small in comparison with most of the other types of sources,
but the proximity of these sources (on-site disposal) to the individual citizen can
cause irritation and  concern.
Industrial Process Emissions
      The quantities  of the various pollutants discharged to the atmosphere from
industrial and commercial establishments are generally attributable to two types
of operations,  the combustion of fuels and industrial processes.  Unfortunately,
emission factors are available for only a small number of processes and industries.
      Data relating to the industrial processes and the materials  handled in these
processes were collected through questionnaires distributed  by local air pollu-
tion agencies and by personal contact with a number of industrial groups.
Several smaller sources did not have the necessary information, and these
exceptions are noted where  applicable.
      In the Northwest Indiana area the two predominant types of industry are
petroleum refining and steel manufacturing.  Allied industries in the area are
chemical plants,  foundries, and metal fabricators.   As stated previously, the
petroleum and steel industries employ approximately 60 percent of the 100, 000
workers in the study area.  A summary of the emissions from the industrial
processes in the study area is shown in  Table 9.  Because of insufficient data,
not all existing industrial processes are listed in this table.   The data  on this
table are subject to change when more specific process information is available..
18

-------
        Table 9.  SUMMARY OF INDUSTRIAL PROCESS EMISSIONS

                      IN NORTHWEST INDIANA,  1966

                                  (tons/yr)
Pollutant and sources
Particulates
Refineries
Cement plants
Chemical plants
Foundries
Steel
Grey iron
Other
Other sources
Steel mills
Blast furnace
Open hearth
Basic oxygen furnace
Sintering plant
Coke plant
Total
Sulfur oxides
Refineries
Sulfuric acid manu-
facturing
Other sources
Total
Hydrocarbons
Refineries
Storage
Slowdown system
Waste water
separator
Leakage
Catalytic cracking
Vacuum distillation
Other sources
Total
Carbon monoxide
Refineries
Total
S.Chicago

900
na

-_
na
na
--

3, 380
40,600
36, 400
6, 050
87, 300

na
18, 000a
18,000

--
20,075 i
8,400 '
9,860
2,560
2, 190
1,095
6,220
50,400

60,200
60, 200
Gary

26,600
182

1,420
—
na

3,800
26, 900
450
53, 100
7, 500
120,000

--
--
--

--
—
--
--

--
--
Hammond

~ ™*

__
10
20
20

--
50

na
18,000
18,000

--
--
--
--

--
--
Whiting

1,500

-_
—
--

--
1,500

13,000
--
13,000

16,400
--
--
16,400

6,600
6,600
Study area

2,400
26,600
182

1,420
10
20
17

7, 180
67, 500
450
88,500
13,550
208,800

13,000
36,000
49,000

16,400
20,075
8,400
9,860
2,560
2, 190
1,095
6,220
66,800

66,800
66,800
aEstimated figure.
na - Information not available or reported.
19

-------
 Steel Manufacturing   Three major steel plants within the boundaries of the study
 area operate a full line of equipment including:  blast furnaces, oxygen-lanced
 and nonoxygen-lanced  open hearths,  sintering plants,  coke plants, basic
 oxygen furnaces, and individual power plants.  As shown in Table  10, the steel
 manufacturing industry emits 186, 780 tons of particulates per year,  which
 amounts  to 89.4 percent of the total particulates from industrial processes and
 68. 5 percent of the total particulates  emitted in the study area.
 Oil Refineries  The study area has four complete oil refineries and a number
 of storage  and distribution centers.  The most  important air pollution consider-
 ations with respect to refinery emissions are crude oil processing capacity, the
 processing techniques employed,  types of fuels used and their composition,
 maintenance and housekeeping,  and the air pollution control measures used.
 Hydrocarbons, oxides of sulfur and nitrogen, carbon monoxide, and  odors are
 the primary pollutants emitted from these operations.
      Table 11 shows the different sources and  amounts of pollutants emitted
 from the petroleum refineries.  Of the hydrocarbons emitted in the study area,
 62 percent are from the industrial processes of the refineries.
 Chemical Industry - A number of large chemical plants are located in the study
 area,  but lack of emission factors and production data for most of the plants
 make it impossible to estimate emissions from the chemical industry's  opera-
 tions.  Sulfuric acid is produced at two of the chemical plants.  Information for
 one plant permitted an emission estimate of 18,000 tons of  sulfur dioxide per
 year.
 Cement Manufacturing - A large cement manufacturing plant in the area has an
 annual capacity of 8. 3 million barrels.  By the nature of this  process,  particu-
 late material is the pollutant of prime concern.   The amount of particulate matter
 emitted from the cement kilns was estimated by applying emission factors and
 control efficiency information from the local air pollution agency.  An estimated
 26, 600 tons of particulate is discharged annually from this  plant.
 Foundries  - The lack of process information on area foundries makes it virtually
 impossible to estimate their total emission contribution.  Data were available
 for two foundries; one, a steel foundry, emitted approximately 1,420 tons of
 particulates annually,  and the second, a grey iron foundry with a capacity of
20

-------
     Table 10.  AIR POLLUTANT EMISSIONS FROM STEEL INDUSTRY
                     IN NORTHWEST INDIANA (tons/yr)


Operation
Blast furnaces
Open hearths
Basic oxygen furnaces
Sintering plants
Coking plants
Combustion of fuel
Total

Number
of units
23
101
3
5
3
--

Pollutants
Particu-
lates
7, 180
67, 500
450
88, 500
13,550
9,600
186,780
Sulfur
oxides
--
--
--
--
--
77,850
77,850
Nitrogen
oxides
--
--
--
--
--
54, 000
54, 000
Hydro-
carbons
--
--
--
--
-•-
820
820
Carbon
monoxide
--
--
--
--
--
920
920
           Table 11.  POLLUTANT EMISSIONS FROM PETROLEUM

               REFINERIES IN NORTHWEST INDIANA (tons/yr)

Pollutant source
Storage
a
General Processes
Catalytic cracking
b
Auxiliary equipment
Fuel combustion
Total
Partic-
ulates
--
--
2,240

--
1,050
3,290
Sulfur
oxides
--
13, 000
--

--
51,990
64,990
Nitrogen
oxides
--
--
840

--
14,860
15, 700
Hydro-
carbons
20, 070
23,720
2,200

20,840
--
66,830
Carbon
monoxides
--
--
66,825

--
--
66,825
General processes include vacuum distillation, loading, cooling towers,  etc.
Auxiliary equipment includes blowdown systems, waste water separators,  leak-
age, etc.
                                                                             21

-------
 12,500 tons of material per year, emits only  10 tons per year because of control



 equipment.  More data should be collected because of the significant nature  of



 this process in the quantities of pollutants  emitted.





 EMISSIONS BY GEOGRAPHICAL AREA



      The Northwest Indiana communities  of East Chicago, Gary,  Hammond, and



 Whiting are geographically interrelated to  the extent that each community



 borders two or more of the other communities.  This factor adds to the com-



 plexity of the  air resource management program because air pollution does  not



 respect municipal boundaries.





      Figures 3 through 13 indicate the geographical locations  of point and area



 source emissions.   Point sources are those specific industries with total



 emissions above a particular figure, and area sources are  domestic,  com-



 mercial,  manufacturing, and refuse burning sources that are below a specified



 amount of emissions and are  reported in tons per year per grid.  Not all sources



 that could be listed  in the point source category are included on these maps



 because of the lack  of specific data, mostly on process  capacities,  that would



 make it possible to  calculate  their emissions.





      The location of the point sources in the study area  are  illustrated on



 Figures 3, 4,  and 5.  Figure 3 shows the location of point sources that annually



 emit 250 tons or more of particulates.  This map locates 20 such sources with



 a range of emissions from 250 tons per year to 92, 000 tons per year.   Because



 of the location of these point sources, all but three of them could  influence the



 air pollution problem  in all of the four communities located in the study area.





      Sulfur oxide emissions from point sources are located  in Figure 4.   This



 map shows  17  point sources with a  range of 250 to 75, 000 tons per year.




      Figure 5 shows the point sources that emit more than 250 tons of nitrogen



 oxides per year.  The map locates  13 such sources; these emissions are in  the



 range of 250 to 23, 000 tons per year.




      The Northwest Indiana study area includes over 400 manufacturing plants,



 over 102,000  domestic dwelling units,  and numerous commercial establishments.



 Figures 6 through 12 illustrate the  estimated geographical location  of the pollu-



 tant emissions from these sources.  The area manufacturing sources include



22

-------
t-Aff CALUHCT
      380  385  390 395


1530    TT  "^^"      40°  405 41° 415
       Illfe   Ny-^   .
1525
                                                  1525
                                                          LAKE MICHIGAN
          1515
                                                   420  425  430  435 440  445  450 455  460 465
                                               JL
                       HAMMOND


                      TRI-STATE
CALUMET    L
  CITY  1505  -


       1500


       1495


       1490.--


       1485


       1480


PARTICIPATES, 380 385 390  395  40Q 405 4,Q  415

   tons/yr

   250 -   1,000


 1,000 -   5,000


 5,000 -  10,000


    OVER 25,000
                                                                                              -1505
1470


1465
                                                                            450  455  460  465
                                                                           1475
                                                                               HOBART
                                                                           1470


                                                                           1465
                                                                                   1
                                                                                   N
                                                       425  430  435  440 445
                                                                                       MILES
                        Figure 3.  Particulate emissions  from point sources.

-------
tv
           itft tumuli
              CALUMET
                CITY
                                                                     LAKE MICHIGAN
                                                             420 425 430  435  440  445  450 455  460  465
                                                                                                         1505
                                  HAMMOND

                                 TRI-STATE
                           380  385  390  395  400 405 410  415  420
               SOX,  tons/yr
                 250 -  1,000
               1,000 - 10,000
              10,000 - 20,000
              20,000 - 50,000
                  OVER 50,000
425 430 435 440 445
                                MILES
                                  Figure  4.   Sulfur  oxide  emissions  from point sources.

-------
                  380 385  390  395
                     »•  :
  Hire CALUHCT
           1530

            1525
    CALUMET
      CITY
 1515

 15KI

1505

1500

1495

1490-

1485

1480
                        400 405 410  415
                                                             LAKE MICHIGAN
                                                     470  425 430  435  440  445  450  455  460 465
                                                 JL
                                                 i     i
NOX EMISSIONS, tons/yr
 •     250-1,000
 •   1,000  -   5,000
 0   5,000  -  10,000
    10,000  -  20,000
        OVER  20,000
                         HAMMOND

                        TRI-STATi
                                                      ,
                  380  385  390  395 400  405  410 415 420
                                             425  430  435  440 445
                                                                              MILES
                      Figure 5.  Nitrogen  oxide emissions from point sources.

-------
rv
CT-
                           380  385 390 395
           LttXl CALUUET
                    1530
                I     1525
              f
              CALUMET
               CITY
400 405 410  415
                         LAKE MICHIGAN
                                                            420  425  430  435 440 445  450  455  460 465
             PARTICIPATES,
               tons/yr
                           380  385 390  395  400  405  410 415 420
                   50 - ' Ik
                !   75-99

                  100 - 199

                 200 - OVER
                                                                 425  430  435  440 445
                                                                                                MILES
                                   Figure 6.  Participate emissions from area sources.

-------
                          380  385  390 395
                                           400  405  410  415
                                                                    LAKE MICHIGAN
                                                            420  425  430  435 440 445  450  455  460 465
             CALUMET
               CITY
                                                                                                        1505
          SO   EMISSIONS,  38°  385  39°  395 4°° 405  41°  41S  42°
                                                           1470
                                                 , ..        1465
tons/yr
3   50  -   99
   100  -  299
   300  -  600   .
    OVER  600
                                                                425 430 435  440  445
                                                                                                MILES
                            Figure 7.  Sulfur oxide emissions from  area  sources.
IN,

-------
00
                           380  385 390  395
           LtKC CiLVUtl
                                            400  405 410 415
                                                                    LAKE MICHIGAN
                                                            420  425  430  435 440  445 450 455  460 465
              CALUMET    L
               CITY 1505
                           380  385 390 395 400  405  410  415  420
             NOX,  tons/yr
                  50 -  7k




                  OVER  200
425 430 435  440 445
                                MILES
                                  Figure 8.   Nitrogen  oxide  emissions  from  area  sources.

-------
                380 385  390  395
                                 400 405 410  415
                                                          LAKE MICHIGAN
                                                  420 425 430  435 440  445  450 455  460 465
          1495



          1490-



          1485



          1480
  PARTICULATES,
    tons/yr

n~-~i  50  -  ik
75 -  99


100  -  200


OVER  200
                 H A MM ON D




                TRI-STATE
                380  385  390  395 400 405 410  415  420
                                                      425 430 435 440 445
                                                                                      MUES
         Figure 9.   Particulate emissions from commercial  and area manufacturing sources.

-------
U)
o
                           380  385 390  395

                    1330


                    1S25
                     1515
   CALUMET
     CITY  1505


          1500


          1495


          1490-


          1485


          1480




   SOX,  tons/yr


I     I  50 -   99


      100 -  199

      200 -  299


       OVER  300
400 405 410  415
                                                                     LAKE MICHIGAN
                                                             470  425 430  435  440  445  450 455  460 465
                                 HAWMOND



                                 TRI-STATE
                           380  385  390 395 400  405  410 415 420
                                                                 425  430 435  440 445
                                                     MILES
                       Figure  10.   Sulfur oxide emissions from commercial and area manufacturing.

-------
                 380 385 390  395
           1530
           1515
    CALUMET
     CITY
           1505


          1500


           1495


          1490


           1485
                                  400 405 410 415
                                                           LAKE MICHIGAN
                                                   420  425 430  435 440 445  450 455 460  465
  PARTI CULATES,
    tons/yr

 "7~|  50  -   Ik

 HI.  75  -   99
380 385 390  395  400  405 410  415  420


                                 1470


                                 1465
                                                                            450  455  460 465
                                                                           1475
   HOBART
1470


1465
I
N
                                                       425  430  435  440 445
                                                                                      MILES
mim 100 -  200

       OVER  200
           Figure 11.  Particulate emissions  from  domestic  heating  and  on-site  burning.

-------
N
                          380 385 390  395
           1,4*1 C4LVHI'
                                          400  405  410  415
                                                                  LAKE MICHIGAN
                                                           420  425  430 435 440 445 450 455  460  465
             CAIUMJT
               cirr
                                                                                     •as*
                                                                                   450 455  460 465
                          380  385  390 395 400 405 410 415 420




                                                          1470



                                                          1465
£0X, tons/yr
                                                               425 430 435 440 445
                                                                                 MILES
                     Figure 12.   Sulfur oxide emissions from domestic heating  and on-site burning.

-------
                380  385  390  395
                                 400 405 410 415
                                                          LAKE MICHIGAN
                                                  420 425 430  435 440 445  450 455  460 465
                       HAMMOND

                       tUl-StATf
NITROGEN OXIDES,
    tons/yr
       50 -  7k
       75 -  S3
       100 -  130
       OVER  130
                 380 385 390  395  400  405  410 415  420
425 430 435  440 445
           Figure  13.   Nitrogen oxide emissions from domestic heating and on-site burning.

-------
those plants that were not considered as point sources, and the pollutants ascrib-
ed to these sources were distributed by finding a percentage of the employees in
the particular grids and assigning that particular percentage of the total pollutant
load from area manufacturing to that grid or by actual location of the particular
plant.   The emissions from commercial sources were calculated, and  this
amount was distributed to the downtown sections  of each of the four  communities.
There is  probably notable error in this distribution; but since detailed  data on
commercial sources were not available,  this method of distribution was used to
incorporate this source of pollutant emissions.
      The domestic source of pollutant emission was distributed in the  following
manner.  The census tracts in this Standard Statistical Metropolitan Area were
available with information on the number of dwellings using specific fuels (see
Table  12).  These numbers were distributed into the grid system, and  a percent-
age of the total amount of dwellings  for each fuel was taken.  This percentage
was then  applied to the total emissions from this source and added to the partic-
ular grid in question.  Another source of pollution, on-site burning  of refuse,
was also  distributed  in a like manner.
         Table  12.  SUMMARY OF DOMESTIC HEATING BY NUMBER OF
                DWELLING UNITS IN NORTHWEST INDIANA, 1960

All occupied units
Heating fuel
Utility gas
Fuel oil, kerosene,
etc.
Coal or coke
Electricity
Bottled, tank, or
LP gas
Other fuel
None
East
Chicago
16,837

4, 855

7,839
3,772
59

100
173
39
Gary
50,283

12,692

29,283
6,935
296

780
251
46
Hammond
32,997

12,271

15,272
4,881
59

470
20
24
Whiting
2,569

1, 035

929
575
--

30
--
--
Study
area
102,686

30,853

53,323
16, 163
414

1,380
444
109
Percent
of total
100. 0

30. 1

52. 0
15.7
0.4

1. 3
0.4
0. 1
34

-------
      Figures 6, 7,  and 8 show the geographical variation of particulates, sulfur
oxides, and nitrogen oxides, respectively, for area sources.  Included in these
area sources are area manufacturing and commercial,  domestic and on-site
burning.
      A breakdown  of the geographical area source emissions is given in Figures
9 through 13.   The commercial and area manufacturing sources in Figures 9 and
10 show emissions of particulates and sulfur oxides,  respectively.  Figures 11,
12, and 13 locate the emissions from domestic fuel combustion and on-site burn-
ing throughout  the study region.  These figures show the amounts  of particulates,
sulfur oxides,  and  nitrogen oxides  and their distribution throughout the study
region. It should be noted that I960 census  figures were used in the calculation
of the domestic emissions and that the amounts of fuels used for domestic heating
were  up-dated  to 1965 when the figures were available.
                                   SUMMARY
      The results of the  emission inventory show the need for further study in
certain areas.  The fuel consumption by industries has been defined well in some
areas and poorly in others.  The consumption of coal and of natural gas have
been  defined to a fairly  accurate degree  from figures provided by area -wide
associations.   The lack of such an organization to provide fuel oil data has left
an emission category that still must be evaluated.  Also, as stated in the report,
recalculation of some of the coal figures could be performed when more informa-
tion on the chemical composition of the coal is received.  This would help to
increase the accuracy of the inventory.
      An inventory should be made to determine the locations of commercial
establishments and the  exact quantity of fuel burned at each.  This information
would complete the fuel combustion inventory.
      Comprehensive traffic flow maps of the four-city area are needed to com-
pute the emissions from transportation on a vehicle-mile basis.  Since emissions
from transportation are approximately 25 percent of the total emission in this
area, geographical distribution of these emissions is important and should be
studied further.
      A detailed  study is also  needed to determine industrial process emissions.
The lack of process information that can be used to estimate the  emissions re-
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 suiting from these sources impaired establishing an accurate inventory.



 Foundries,  chemical plants,  sulfuric acid manufacturing, and refineries  are



 a few of  the processes requiring collection of more detailed information.





       The last area of concern is  refuse disposal.  The quantities of refuse



 burned at the city dumps should be more accurately defined because of the size



 of this source of pollution. An inventory of the industrial and commercial



 incinerators should be made to define the on-site burning more precisely.
36

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