EPA-660/2-74-056
June 1974
                        Environmental Protection Technology  Series
    Ground  Water  Contamination
     In  The  Northeast States
                                  Office of Research and Development
                                  U.S. Environmental Protection Agency
                                  Washington. D.C. 20460

-------
            RESEARCH REPORTING SERIES
Research reports of the  Office  of  Research  and
Monitoring,  Environmental Protection Agency, have
been grouped into five series.  These  five  broad
categories  were established to facilitate  further
development  and  application   of   environmental
technology.    Elimination  of traditional grouping
was  consciously  planned  to  foster    technology
transfer   and  a  maximum  interface  in  related
fields.  The five series are:

   1.  Environmental Health Effects Research
   2.  Environmental Protection Technology
   3.  Ecological Research
   4.  Environmental Monitoring
   5.  Socioeconomic Environmental Studies

This report has been assigned to the ENVIRONMENTAL
PROTECTION   TECHNOLOGY   series.    This   series
describes   research   performed  to  develop  and
demonstrate    instrumentation,    equipment    and
methodology  to  repair  or  prevent environmental
degradation  from point and  -non-point   sources  of
pollution.  This work provides the new  or improved
technology  required for the control and treatment
of pollution  sources to meet environmental  quality
standards.
                    EPA REVIEW NOTICE
 This report has "been reviewed by the Office of Research and
 Development, EPA, and approved for publication.  Approval does
 not signify that the contents necessarily reflect the views
 and policies of the Environmental Protection Agency, nor
 does mention of trade names or commercial products constitute
 endorsement or recommendation for use.

-------
                                                 FILE:  Grndwtr:  Poll/Prot
                                              EPA-660/2-74-056
                                              June, 1974
               GROUND WATER CONTAMINATION

                 IN THE NORTHEAST STATES
                            by
David W.  Miller, Frank A.  DeLuca, and Thomas L. Tessier
                 Contract No. 68-01-0777
                 Program Element 1BA024
                     Project Officer

                     Marion R. Scalf
   Robert S. Kerr Environmental Research Laboratory
          U.  S. Environmental Protection Agency
                      Ada,  Oklahoma
                       Prepared for
           OFFICE OF  RESEARCH AND DEVELOPMENT
          U. S. ENVIRONMENTAL PROTECTION AGENCY
                 WASHINGTON, D.C. 20460
            For sale by the Superintendent of Documents, U.S. Government Printing Office
                      Washington, D.C. 20402 - Price $3.30

-------
                          ABSTRACT
An evaluation of principal sources of ground-water contami-
nation has been carried out in  11 northeast  states, includ-
ing all of New England, New York, New Jersey, Pennsylvania,
Maryland, and Delaware.  The findings of this study have
been used to determine priorities for research into ways to
reduce the number of sources of contamination and to point
out deficiencies in present control methods  for protecting
against further degradation of  ground-water  quality.

Ground-water quality in the region is generally good to ex-
cellent, except for naturally occurring saline waters in
some coastal and inland aquifers.  Principal sources of
ground-water quality degradation caused by man's activities
that are common to most parts of the region  are septic tanks
and cesspools, buried tanks and pipelines including sanitary
and storm sewers, the application and storage of highway de-
icing salts, municipal and industrial landfills of solid
waste, unlined surface impoundments, spills, and the uncon-
trolled discharge of pollutants on the land  surface.  In New
York and Pennsylvania, mining and petroleum  exploration and
development have caused many instances of ground-water con-
tamination, but the extent of the problem has not been de-
fined.  Salt-water intrusion in coastal areas has been ade-
quately controlled, but little  is known of the potential
threat to fresh-water aquifers  from the encroachment of sa-
line water that occurs in inland formations  underlying the
western portions of the region.

The findings of the investigation indicate that the hundreds
of cases of ground-water contamination recorded to date and
referenced in this report represent only a very small per-
centage of those that actually  exist.  Furthermore, the
technology to adequately solve  problems of ground-water con-
tamination has not been developed and made available to reg-
ulatory agencies.  Basic research is needed  on how to im-
prove methods to inventory and  correct problems of ground-
water contamination and how to prevent future problems
through better management and control of activities that can
affect ground-water quality.

This report was submitted in fulfillment of  Contract
68-01-0777 by Geraghty & Miller, Inc., under the sponsorship
of the U.  S.  Environmental Protection Agency.  Work was com-
pleted as of June,  1974.
                              ii

-------
                         CONTENTS


                                                       Page

Abstract                                                ii

List of Figures                                         v^

List of Tables                                          ix

Sections

I      Conclusions                                       1

II     Recommendations                                   5

III    Introduction                                      7

            Use of Ground Water                          8
            Future Use                                   8
            References Cited                            16

IV     Description of Project Area                      17

            Physiography                                I7
            Population                                  21
            Climate                                     21
            Geology and Ground Water Resources          24

                 Connecticut                            24
                 Delaware                               30
                 Maine                                  32
                 Maryland                               37
                 Massachusetts                          40
                 New Hampshire                          45
                 New Jersey                             4*3
                 New York                               51
                 Pennsylvania                           58
                 Rhode Island                           62
                 Vermont                                65

            References Cited                            69

V      Natural Ground-Water Quality                     78

            Introduction                                78
            Connecticut                                 79
            Delaware                                    81
            Maine                                       89
                              ill

-------
 CONTENTS  (continued)
 V      Natural Ground-Water Quality (continued)

             Maryland                                    89
             Massachusetts                                92
             New Hampshire                                95
             New Jersey                                   97
             New York                                    99
             Pennsylvania                                107
             Rhode  Island                                110
             Vermont                                     110
             References  Cited                           113

 VI      Sources of  Ground-Water Contamination            124

             Definition  of  the Problem                   124

                 Importance of the  Resource             125
                 Health and Other Hazards               128
                 The Relationship of Ground Water
                   to Surface Water                    139
                 The Problem of Monitoring              140
                 Technical and Economic Difficulties    155
                 Summary                                163

             Septic Tanks and Cesspools                  164
             Buried Pipelines and Storage Tanks          178
             Application and Storage of Highway
               Deicing Salts                            185
             Landfills                                  199
             Surface  Impoundments                        219
             Spills and  Surface Discharges               230
             Mining Activity                            236
             Petroleum Exploration and Development       247
             Salt-Water  Intrusion                        251
             River  Infiltration                          265
             Underground Storage and Artificial
               Recharge  of  Waste Water                   272
            Water  Wells                                 279
            Agricultural Activities                     282
            References  Cited                            285

VII    Research and Other  Needs                         301

            General Needs                               301
            Specific Needs                              308
            References Cited                            315
                             iv

-------
CONTENTS (continued)

                                                      Page
VIII   Acknowledgements                                316
IX     Appendix A - Glossary of Terms                  318
       Appendix B - Water Quality Standards            324

-------
                         FIGURES

No.                                                 Page
 1   Locations of the States                         18
 2,  Ground-Water Regions                            19
 3   Precipitation Map                               23
 4   Average Annual Evaporation                      25
 5   Generalized Geologic Map of Connecticut         26
 6   Locations of Principal Sand and Gravel
       Aquifers of Connecticut                       27
 7   Generalized Geologic Map of Delaware            31
 8   Generalized Geologic Map of Maine               35
 9   Location of Principal Sand and Gravel
       Deposits in Maine                             36
10   Generalized Geologic Map of Maryland            38
11   Generalized Geologic Map of Massachusetts       43
12   Generalized Geologic Map of New Hampshire       47
13   Generalized Geologic Map of New Jersey          49
14   Generalized Geologic Map of New York            52
15   Generalized Geologic Map of Pennsylvania        59
16   Generalized Geologic Map of Rhode Island        64
17   Generalized Geologic Map of Vermont             66
18   Depth to Mineralized Ground Water               80
19   Inferred Regional Circulation of Ground
       Water in Western New York                    106
20   Downward Leaching of Pollutants from a
       Salt Stockpile                               130
                            VI

-------
FIGURES (continued)
No.                                              Paqe
21   Plan View of Plume of Contaminated
       Ground Water Caused by Leakage from
       Lagoons and Basins                        131

22   Downward Movement of Contaminated Water
     from a Leaky Sewer                          133

23   Plan View of Contaminated Ground Water
       Caused by Leachate from a Landfill        134

24   Movement of Light-Density Fluid in the
       Ground-Water System                       135

25   Plan View of Water Table Contours
       Associated with a Landfill                142

26   Generalized Hydraulic Profile Beneath
       a Landfill                                143

27   Movement of Contaminated Ground Water
       Beneath Leaky Lagoons and Basins          145

28   Long-term Chloride Fluctuation in a
       Well Tapping the Cohansey Sand            148

29   Conventional Septic Tank - Soil
       Absorption System

30   Relationship of Housing Density to
       Residual Conductance and Accretion
       of Dissolved Solids

31   Increase in Salt Applied to Massachusetts
       State Highways and Chloride Levels in
       Ground-Water Sources                      190

32   Chloride Concentration in Samples from
       Main Pumping Station in Burlington,
       Massachusetts

33   Principal Coal Areas of Pennsylvania and
       Maryland                                  240

34   Principal Oil and Gas Exploration and
       Development Areas                         248
                            VI1

-------
FIGURES (continued)
No.                                              Page

35   Depth to Mineralized Ground Water in
       Major Aquifers in the Coastal and
       Inland  Regions                           252

36   Inland Limit of Saline Ground Water in
       the Coastal Plain Formations              253

37   Occurrence of Salty Ground Water in
       Southeastern Queens and Southwestern
       Nassau Counties                           257

38   Variations of Chemical Quality of Ground
       Water as Related to Recharge and
       Discharge                                 266

39   Local Ground-Water Circulation, Producing
       a Relatively Thin Fresh-Water Zone        267

40   Effect of Infiltration of River Water       270

41   Map of Theoretical Critical Zones           305
                           viii

-------
                          TABLES


No.                                              Page

 1   Estimated Use of Water                         9

 2   Estimated and Projected Use and
       Requirements of Water                       13

 3   Projected Per Capita Water Withdrawals        15

 4   Population                                    22

 5   Coastal Plain Stratigraphic Units             33

 6   Geologic Units and their Characteristics
       in the Maryland Coastal Plain Province      41

 7   Yields and Depths of Selected Wells in
       Sand and Gravel Deposits in
       Massachusetts                               46

 8   Range in and Median Yields of Selected
       Wells in Carbonate Rocks                    56

 9   Range in and Average Yields of Selected
       Wells in Sand and Gravel Aquifers           57

10   Range in and Median Yields of Selected
       Wells in Sand and Gravel Aquifers in
       Vermont                                     68

11   Chemical Analyses of Ground Water in
       Connecticut                                 82

12   Number of Ground-Water Sources Exceeding
       Connecticut Drinking Water Standards        85

13   Chemical Analyses of Ground Water in
       Delaware                                    87

14   Chemical Analyses of Ground Water in
       Maine                                       90

15   Chemical Analyses of Ground Water in
       Maryland                                    91

16   Chemical Analyses of Ground Water in
       Massachusetts                               93
                            IX

-------
TABLES  (continued)
No.                                              Page

17   Chemical Analyses of Ground Water in
        Southeastern New Hampshire                  96

18   Chemical Analyses of Ground Water in
        New Jersey                                  98

19   Chemical Analyses of Ground Water in
        New York                                   100

20   Chemical Analyses of Ground Water in
        Pennsylvania                               108

21   Chemical Analyses of Ground Water in
        Rhode Island                               111

22   Number of Wells Drilled                      127

23   Incidence of Waterborne Disease Due
        to Source Contamination                    137

24   Incidence of Waterborne Disease:
        Treatment Overwhelmed                      138

25   Principal Sources of Ground-Water
        Contamination                              15°

26   Estimated Population Served by Septic
        Tanks                                      151

27   Normal Range of Mineral Pickup in
        Domestic Sewage                            161

28   Comparison of Pollutional Loads from
        Hypothetical City - Street Runoff
       Versus Raw Sanitary Sewage                 179

29   Quantities of Sodium and Calcium
       Chloride Use                               186

30   Sources of Salt Contamination of the
       Burlington, Massachusetts Well Field       193

31   Summary of Data on 34 Selected
       Contamination Cases Related to Deicing
       Salts                                      I94

-------
TABLE (continued)
No.                                              Page

32   Physical Characteristics of Municipal
       Refuse                                     202

33   Comparison of the Chemical
       Characteristics of Leachate                204

34   Analyses of Leachate from Soil 36 Feet
       Below 1962  Refuse Cell                     207

35   Partial Chemical Analyses of Water from
       Wells Located In and Nearby a Landfill
       Site                                       210

36   Summary of Data on 42 Municipal and 18
       Industrial  Landfill Contamination
       Cases                                      212

37   Origins and Pollutants in 57 Cases of
       Ground-Water Contamination Caused by
       Leakage of  Waste Water from Surface
       Impoundments                               222

38   Three Case Histories of Ground-Water
       Contamination from Leakage Out of
       Surface Impoundments                       226

39   Pollutant Reported in 36 Cases of
       Ground-Water Contamination Caused by
       Spills and Surface Discharges              233

40   Land Disturbed by Strip and Surface
       Mining                                     238

41   Abandoned and Inactive Underground
       Mines                                      239

42   Mine Drainage Classes                        243

43   Summary of Water Quality in the Toms
       Run Drainage Basin                         245

44   Summary of Data on Contamination Cases
       Related to Salt-Water Intrusion in
       Coastal Areas                              258

45   Restrictions  on Ground-Water Use in
       Critical Zones                             306
                             XI

-------
TABLES (continued)
No.                                              Page

46   Principal Sources of Ground-Water
       Contamination and the Priority for
       Additional Research and Control            309

47   U. S. Public Health Service Chemical
       Standards of Drinking Water, 1962          325
                           xii

-------
                        SECTION I

                       CONCLUSIONS
1.  Total use of ground water in the 11-state region in
    1970 was approximately 3.4 billion gallons per day,
    with ground water supplying 20 percent of community/
    93 percent of rural, 14 percent of industrial, and 47
    percent of irrigation requirements.

2.  Ground water can be developed almost anywhere in the
    region.  Sand and gravel, and some sedimentary rocks
    are the principal aquifers.

3.  The natural quality of ground water is generally good
    to excellent, except for the occurrence of saline wa-
    ters in some coastal and inland aquifers.

4.  The most common natural water-quality problems in
    fresh-water aquifers are high iron content, often asso-
    ciated with a high concentration of manganese;  low pH;
    and high hardness.

5.  The most significant source of ground-water contamina-
    tion is the discharge of sewage from septic tanks and
    cesspools, serving an estimated 12 million people in
    the region.  Inadequate experience and lack of sound
    scientific planning on the use of on-site disposal sys-
    tems have led to some regional and many local problems.

6.  Buried storage tanks and pipelines, including sanitary
    and storm sewers, are significant sources of ground-
    water contamination where pollutants have leaked di-
    rectly into shallow aquifers.  The most troublesome
    pollutants from this source are hydrocarbons and indus-
    trial wastes containing toxic substances.

7.  The storage and spreading of several million tons of
    highway deicing salts each year in the northeast have
    led to numerous problems of ground-water quality degra-
    dation.  Some domestic and public supply wells have
    been abandoned, and records of water quality from many
    others have shown a gradual but significant trend of
    increasing concentrations of chloride, sodium, and
    other ions.

8.  The thousands of acres of landfills containing munici-
    pal and industrial solid wastes are an almost universal
    source of ground-water contamination in the region.

-------
  9.   Lagoons,  pits,  and basins,  which are  a  common means  for
      treating,  handling, and storing liquids and  sludges,
      are  leaking  many million gallons per  year  of potential-
      ly hazardous substances to  ground water.

 10.   Spills  and uncontrolled surface discharges of pollut-
      ants have  resulted in  some  severe problems of ground-
      water quality degradation.  Various types  of hydrocar-
      bons and  industrial process and waste liquids are  the
      principal  pollutants.

 11.   The  extent of ground-water  contamination from mining
      activities,  principally involving coal  in  western  Penn-
      sylvania and Maryland,  has  not  been well defined.  How-
      ever, available  data indicate that mine drainage,
      leachate from waste rockpiles,  and leakage from tailing
      ponds may  be significant  sources  of ground-water con-
      tamination in areas containing  numerous abandoned  and
      active workings.

 12.   The  high yield of  salt water from tens  of  thousands of
      marginally producing oil  and gas  wells  in  western  Penn-
      sylvania and western New  York represents the principal
      threat to  fresh-water aquifers  from petroleum explora-
      tion and development.  Little information  has been col-
      lected on  the actual extent and character  of ground-
      water quality problems related  to activities involved
      in petroleum exploration  and development.

 13.   Salt-water intrusion in coastal areas of the region was
      widely recognized about forty years ago as a major
      threat to  fresh-water aquifers.   Consequently, the
      problem has  been well-defined and adequately controlled.

 14.   The movement  of natural saline waters into fresh-water
      aquifers in  the inland areas of the western portion of
      the region,  as influenced by pumping, has  not been
      studied in detail except  in a few locations and repre-
      sents a continuing  problem.

 15.   In spite of  the large number of municipal  and indus-
      trial high capacity wells that are pumping water infil-
      trated from  surface streams which are considered pol-
      luted, few cases of severe ground-water contamination
     have been recorded.  The major problem commonly re-
     ported is a build-up of iron and manganese concentra-
     tions requiring ultimate treatment of the well water.

16.  The practice of disposing of industrial and sewage
     wastes through deep injection wells in saline-water

-------
     aquifers is almost non-existent in the region and repre-
     sents an unimportant source of ground-water contamina-
     tion.

17.   The disposal of storm waters and, in a few cases, indus-
     trial and sewage wastes through recharge basins and
     wells into fresh-water aquifers is common in some parts
     of the region.   Although few instances of ground-water
     contamination have been reported, long-term effects on
     ground-water quality have not been studied in enough de-
     tail to determine the importance of this potential
     source of contamination.

18.   The spraying of liquid wastes onto land as a means of
     disposal and treatment has been carried out on a limited
     basis in each of the 11 states of the study region.
     However, because of a general lack of monitoring and/or
     inadequate evaluation of data collected from monitoring
     wells, little is known at present with regard to the
     feasibility of protecting ground-water quality when mu-
     nicipal and various types of industrial wastes are ap-
     plied to the land surface.

19.   Abandoned and poorly constructed water wells can serve
     as a means for transmission of pollutants from one aqui-
     fer to another, or from land surface to an aquifer.
     This problem is most severe in areas underlain by forma-
     tions containing naturally occurring saline water, in
     highly industrialized areas where spills and uncon-
     trolled surface discharges of pollutants are common, and
     in rural areas where there is a high incidence of shal-
     low, dug wells.

20.   A number of cases of ground-water contamination related
     to agricultural activities have been reported in the re-
     gion.  The principal pollutants are nitrates from fer-
     tilizers and animal wastes, and a variety of substances
     from pesticides.  The potential for ground-water contam-
     ination in suburban areas, from the heavy use of fertil-
     izers and pesticides by individual home owners, may be
     considerably greater than in farmed areas.

21.   Only a very small percentage of the instances of ground-
     water contamination from all sources that probably exist
     in the region has been discovered to date.  Of the more
     than one thousand cases inventoried in this investiga-
     tion, almost all were reported only after a water-supply
     well or spring had been noticeably affected or the pol-
     lutant was being discharged to the surface.

-------
22.  The problem of ground-water contamination has not been
     corrected from either the standpoint of removing the
     source of contamination or significantly improving the
     quality of the affected ground-water supply in most of
     the cases inventoried.

23.  The principal reasons for the lack of success in deal-
     ing with existing ground-water contamination problems
     in the northeast are deficiencies in the technology
     presently available to satisfy economic, social, and
     political restraints;  inadequate budgeting and staff-
     ing together with the diverse interests of regulatory
     agencies;  and the general lack of understanding in the
     region as to how the various activities of man can de-
     grade ground-water quality.

-------
                         SECTION II

                      RECOMMENDATIONS
1.   A basic need in the region is a reevaluation of priori-
     ties governing present budgetary allocations to regula-
     tory agencies, with a greater appreciation of the in-
     creasingly important role that ground water plays in
     meeting essential needs for high quality water.

2.   Chemical analyses of ground-water quality must be ex-
     panded to cover a wider variety of inorganic and or-
     ganic compounds on a more routine basis.

3.   More effective methods must be developed for conducting
     inventories of potential sources of ground-water con-
     tamination on a regional basis.

4.   The monitoring of suspected sources of ground-water con-
     tamination must be expanded, especially those that might
     be introducing pollutants into the ground that could be
     harmful to health, and those that are situated in areas
     where existing wells may be threatened.

5.   Additional research is needed on the development and ap-
     plication of more scientific and dependable ways to de-
     lineate the areal extent and characteristics of pollut-
     ants contained in aquifers and their fate over the long
     term.

6.   Basic research is needed on how to economically remove
     or control the movement of various types of pollutants
     affecting ground-water quality.

7.   The various options presently available to regulatory
     agencies for the future protection of ground-water
     quality must be reevaluated.  Alternatives should be
     made available through research and analysis that are
     suitable on the one hand to meet various geologic and
     hydrologic conditions and on the other hand to overcome
     economic, social, and political restraints.

8.   Additional research is needed on how to reduce the sus-
     ceptibility of aquifers to water-quality degradation
     through the development and application of improved
     methods for analyzing the many factors involved in the
     siting, design, and operation of various activities
     that could become sources of ground-water contamination.

-------
Increased regulation and control is needed to reduce,
as much as possible, new instances of ground-water con-
tamination.  This includes calling for procedures to
contain toxic pollutants on the land surface, requiring
detailed information on which environmental decisions
can be based, and enforcing design and operational pro-
cedures that are productive.

-------
                        SECTION III

                        INTRODUCTION
Three basic factors determine the feasibility of developing
ground water in the northeastern United States:  (1) availa-
bility, (2) water quality, and (3) economics.  This report
discusses the role that water-quality problems play in lim-
iting ground-water use in the region.  It is based on an in-
vestigation supported by the U. S. Environmental Protection
Agency and covers 11 states including Connecticut, Rhode Is-
land, Massachusetts, Vermont, New Hampshire, Maine, New York,
New Jersey, Pennsylvania, Delaware, and Maryland.

Similar reports have been published for four southwestern
states and five south-central states. 1/2)  An investigation
of ground-water contamination is underway in six northwest-
ern states. 3)  The rest of the nation will be covered in
subsequent reports.

Natural ground-water quality together with the geologic set-
ting and occurrence of principal aquifers are described in
the next sections of this report on a state-by-state basis.
This is followed by a discussion of the principal sources of
ground-water contamination in the region.  The final section
recommends research and other needs required to combat the
problems of ground-water pollution and contamination, based
on the findings of the investigation.

Information on natural water quality and aquifer systems was
obtained from a careful review of literature on the region.
Published data were also surveyed in an effort to obtain
data on specific cases of ground-water contamination and
many valuable references were used in the following discus-
sion.  However, few of the known instances of contamination
have been reported in the literature.  In order to gain a
true perspective on the status of ground-water contamination
it was necessary to contact, mostly by personal visit, sev-
eral hundred public officials, consultants, scientists, well
drilling contractors, representatives of industry, and
others involved in water supplies so that their files and
individual experience could be applied to the study.

Throughout the report, the terms "pollution" and "contamina-
tion" are synonymous and mean the degradation of natural wa-
ter quality, as a result of man's activities, to the extent
that its usefulness is impaired.  There is no implication of
any specific limits  (such as those in the U. S. Public

-------
 Health Service drinking water standards),  since the degree
 of permissible pollution depends upon the  intended end use,
 or uses,  of the water.   Increases in concentration of one or
 more constituents as the natural result of movement of
 ground water through an aquifer are referred to as "mineral-
 ization" .

 It is recognized that these definitions are perhaps simplis-
 tic, but  at least they  avoid the logical impasses  to which
 some other  definitions  lead.   Also, they are readily under-
 standable.   "Pollution" has long implied the activity of  man,
 and hence the term "natural pollution"  is  confusing as well
 as unnecessary.  4)

 USE OF GROUND WATER

 In 1970, the total fresh ground-water withdrawal in the na-
 tion was 68 billion gallons per day or  21  percent  of all
 fresh water withdrawn.  5)   For the  project area, 18 percent
 of total water used was from ground-water  sources.   Water
 use in the  11 states of the region  is shown on  Table 1;   wa-
 ter for hydroelectric and thermoelectric power  is  excluded
 in all computations.  Surface and ground-water  withdrawals
 for public  and rural supply,  self-supplied industry,  and  ir-
 rigation are given as of 1970.   Ground  water provided 20  per-
 cent of public,  93 percent of rural,  and 14 percent of indus-
 trial supplies.   Forty-seven  percent  of the water  required
 for irrigation was also ground water.   States in which
 ground water comprises  approximately  25 percent or  more of
 the total water  needs are Connecticut,  Massachusetts,  New
 Jersey, Rhode Island, and Vermont.  Ground water in these
 states is used mostly for public supply or industry,  which
 is true for the  region  as a whole.  Vermont is  the  exception
 because of  its largely  rural  population;   in this case,
 ground water is  used mostly for on-site, domestic supply.
 New Jersey  has the largest total ground-water withdrawal
 (1,027 mgd)  even though it ranks third  in  population
 (7,200,000).   The  state with  the smallest  amount of ground-
 water diversion  is Maine (35  mgd),  even though  it has  the
 seventh largest  population (990,000).

 FUTURE USE

 Future need  for  water should  increase considerably  over ex-
 isting requirements  and consumptive uses.   The  U. S.  Water
 Resources Council  in  1968  published a comprehensive report
 on  the  nation's  water resources.  6)  A  portion  of the  report
deals  with water needs  for  the  future on a regional basis.
Table  2 is a  compilation of the  data  for the  North  Atlantic


                              8

-------
Table 1.  ESTIMATED USE OF WATER IN THE NORTHEAST UNITED STATES
                                   IN 1970.
                          (million gallons per day)  '
Public   Rural
                                        Industrial b)
State
CONNECTICUT
Ground water
Surface water
Total:
Percent of total
that is ground water
DELAWARE
Ground water
Surface water
Total:
Percent of total
that is ground water
MAINE
Ground water
Surface water
Total:
supply

86
270
356

24

30
46
76

40

20
89
109
supply a'

40
1.2
41.2

97

13
0.1
13.1

99

12
2.8
14.8
Fresh

20
55
75

27

22
64
86

26

3
400
403
Saline

1
130
131

1

0
300
300

0

0
24
24
Irrigation

0.5
5.4
5.9

8

2.2
0.5
2.7

81

0.2
8.7
8.9
Total

147.5
461.6
609.1

24

67.2
410.6
477.8

14

35.2
524.5
559.7
Percent of total
that is ground water
   18    81
a) Domestic and livestock supplies.
b) Water for hydroelectric and thermoelectric power excluded.

-------
Table 1  (continued).  ESTIMATED USE OF WATER IN THE NORTHEAST UNITED
                               STATES  IN 1970.   5
                          (million gallons per day) '
                    Public   Rural        Industrial15)
State
MARYLAND
Ground water
Surface water
Total:
Percent of total
that is ground water
MASSACHUSETTS
Ground water
Surface water
Total:
Percent of total
that is ground water
NEW HAMPSHIRE
Ground water
Surface water
Total:
supply
42
380
422
10
170
590
760
22
32
38
70
supply a'
57
0.5
57.5
99
30
0.8
30.8
97
12
1
13
Fresh
43
450
493
9
140
390
530
26
12
180
192
Saline
0
820
820
0
0
160
160
0
0
0
0
Irrigation
2.1
4.3
6.4
33
18
40
58
31
0
2.8
2.8
Total
144.1
1,654.8
1,798.9
8
358
1,180.8
1,538.8
23
56
221.8
277.8
Percent of total
that is ground water
46    92
0
0
20
                                      10

-------
Table 1 (continued).  ESTIMATED USE OF WATER IN THE NORTHEAST UNITED
                              STATES IN 1970.
                          (million gallons per day)  '
                   Public   Rural        Industrial
State
NEW JERSEY
Ground water
Surface water
Total:
Percent of total
that is ground water
NEW YORK
Ground water
Surface water
Total:
Percent of total
that is ground water
PENNSYLVANIA
Ground water
Surface water
Total:
supply
340
560
900
38
460
2,200
2,660
17
250
1,500
1,750
supply a'
81
0.9
81.9
99
140
13
153
92
120
14
134
Fresh
550
450
1,000
55
140
1,300
1,440
10
400
5,000
5,400
Saline
0
0
0
0
1.7
64
65.7
3
0
50
50
Irrigation
56
20
76
74
14
13
27
52
0.8
9.4
10.2
Total
1,027
1,030.9
2,057.9
50
755.7
3,590
4,345.7
17
770.8
6,573.4
7,344.2
Percent of total
that is ground water     14    90           7       0        8          10
                                      11

-------
Table 1  (continued).  ESTIMATED USE OF WATER IN THE NORTHEAST UNITED
                              STATES IN 1970.  5
                          (million gallons per day)  '
State
RHODE ISLAND
Ground water
Surface water
Total:
Percent of total
that is ground water
VERMONT
Ground water
Surface water
Total
Percent of total
that is ground water
GRAND TOTAL
Ground water
Surface water
Total:
Public
supply
18
85
103
18
14
29
43
33
1,462
5,787
7,249
Rural
supply a)
4.7
0.1
4.8
98
16
3.1
19.1
84
525.7
37.5
563.2
Industrial °'
Fresh
15
23
38
39
12
34
46
26
1,357
8,346
9,703
Saline
0.4
0
0.4
100
0
0
0
0
3.1
1,548
1,551.1
Irrigation
0.4
4.1
4.5
9
0
0.1
0.1
0
94.2
108.3
202.5
Total
38.5
112.2
150.7
26
42
66.2
108.2
39
3,442
15,826.8
19,268.8
Percent of total
that is ground water
20    93
14
0.002    47
18
                                     12

-------
Table 2.  ESTIMATED AND PROJECTED USE AND REQUIREMENTS OF WATER
             FOR THE NORTH ATLANTIC REGION, UNITED STATES.
                          (million gallons per day) °^
Total estimated water use
and projected requirements

Municipal water
requirements

Rural domestic water
requirements
                                                 Withdrawals
                             Use in          Projected Requirements
                              1965       1980        2000         2020
37,467     54,920     113,860     236,290
 5,446      7,100      10,000      14,200
   390
  400
  400
400
Total estimated water use
and projected requirements

Municipal water
requirements

Rural domestic water
requirements
                                               Consumptive Use
                             Use in           Projected Requirements
                              1965        1980       2000        2020
 2,023


   905


   186
2,870       4,960
1,210
  200
  200
            8,490
1,750       2,550
200
                                      13

-------
Region, which includes a major portion of the 11-state study
area.  According to this projection, water requirements dur-
ing the period 1980 to 2020 will increase more than four-
fold.  Self-supplied industrial water needs alone for the
year 2020 have been estimated at almost 35 billion gallons
per day in the North Atlantic Region. 7)  The national aver-
age per-capita use also is anticipated to increase.  Table 3
is projected per-capita use within the conterminous United
States.

With the increased competition for water supplies, several
interrelated factors become obvious.  The demand for land
for housing has significantly reduced the already limited
sites suitable for surface-water impoundments.  The present
high cost of land will continue to have a profound influence
on the present trend of municipalities and other large water
users to give increased consideration to the development of
supply wells, which take up comparatively little space,
rather than surface-water supplies.  As urban and industrial
expansion takes place, there will be a greater need to trans-
port water from areas of surplus to areas experiencing short-
ages.  The high cost involved in piping large quantities of
surface water should accelerate exploitation of local ground-
water supplies.  Also, by the year 2020, it is estimated that
the population in the region will almost double to over 100
million. ''  With the rise in population will come a rise in
water demand, satisfied to a significant degree by the devel-
opment of additional ground-water sources.
                             14

-------
Table 3.  PROJECTED PER CAPITA WATER WITHDRAWALS FOR PUBLIC AND
                   INDIVIDUAL WATER-SUPPLY SYSTEMS.
                        (gallons per capita per day)  '
Year       Public water-supply systems       Individual water-supply systems

1965                157                               51

1980                163                               58

2000                168                               71

2020                170                               83
                                   15

-------
                      REFERENCES CITED

                        SECTION III
1.  Fuhriman, D. K. and J. R. Barton, "Ground Water Pollu-
    tion in Arizona, California, Nevada and Utah," Environ-
    mental Protection Agency, Water Pollution Control Re-
    search Series 16060ERU, December 1971.

2.  Scalf, M. R., J. W. Keeley and C. J. LaFevers, "Ground
    Water Pollution in the South Central States," Environ-
    mental Protection Agency, Environmental Protection Tech-
    nology Series EPA-R2-73-268, June 1973.

3.  van der Leeden, Frits, L. A. Cerrillo, and D. W.  Miller,
    "Ground Water Contamination in the Northwest States,"
    Environmental Protection Agency, Office of Research and
    Monitoring, Contract No. 68-03-0298, Report in Prepara-
    tion.

4.  Hem, J. D., "Study and Interpretation of the Chemical
    Characteristics of Natural Water," U. S. Geological Sur-
    vey Water-supply Paper 1473 (2d ed.), 1970.

5.  Murray, C. R. and E. B. Reeves, "Estimated Use of Water
    in the United States in 1970," U. S. Geological Survey
    Circular 676, 1972.

6.  U. S. Water Resources Council, "The Nation's Water Re-
    sources," U. S. Government Printing Office, 1968.

7.  North Atlantic Regional Water Resources Study Coordi-
    nating Committee," North Atlantic Regional Water  Re-
    sources Study," U. S. Corps of Engineers,  1972.
                              16

-------
                         SECTION IV

                DESCRIPTION OF PROJECT AREA
The project covers the 11 states of Connecticut, Delaware,
Maine, Maryland, Massachusetts, New Hampshire, New Jersey,
New York, Pennsylvania, Rhode Island, and Vermont, an area
of over 180,000 square miles.  Six percent of the total con-
terminous United States land surface is represented.  Figure
1 shows the locations of the states in the study area.  Typi-
cal of this region are hilly to mountainous areas, coastal
plains, and some marshy lowlands, with most of the land in
the first category.  Altitude ranges from sea level along
the Atlantic Coast to nearly 6,300 feet in the White Moun-
tains of New Hampshire.  Much of the region has been sub-
jected to urban development but large sections are still
rural with agricultural and forest lands.

PHYSIOGRAPHY

The project area exhibits a wide variety of physical fea-
tures.  These different land forms have a profound effect as
to the use of the land, location of population centers, and
occurrence of natural resources.  In the southeastern por-
tion, the land is characterized by broad areas of relatively
minor relief, while to the west and north the land rises to
hilly and rugged mountainous terrain.

The classification devised by Thomas divides the continental
United States into ten ground-water regions. •*•'  Based on
this system, the study area includes portions of five of
these regions (Figure 2):

1.  Coastal Plain
2.  Unglaciated Appalachians
3.  Glaciated Appalachians
4.  Glaciated Central Region
5.  Unglaciated Central Region

The Coastal Plain is characterized by seaward-dipping uncon-
solidated strata, consisting of clay, marl, silt, sand and
gravel, Cretaceous to Quaternary in age.  The surface relief
is very moderate with topographic highs rarely exceeding a
few hundred feet above sea level.  The sediments range in
thickness from a thin veneer along the Fall Line, which is
the western limit of this province, to as much as 10,000
feet along the eastern coast of Maryland.

The Coastal Plain contains prolific ground-water resources.


                              17

-------
                   NORTH

Figure 1.  Locations of the states in the northeast study area
                           18

-------
                    NORTH
             GLACIATED
          CENTRAL  REGION
             UNGLACIATE
             APPALACHIANS
Figure 2. Ground-water regions in the northeast United States
                                 19

-------
 Because of the presence of thick and permeable sand and
 gravel  zones and the great areal extent of individual aqui-
 fers, high capacity wells and major ground-water supplies
 have been developed throughout the province.

 The Unglaciated Appalachians are characterized by folded
 consolidated rock units forming a ridge and valley topogra-
 phy.  The upland relief is characteristically 1,000 to
 3,000 feet above sea level.   Aquifers include sand and
 gravel  beds in alluvium associated with perennial streams,
 dense crystalline or sedimentary rocks,  and some cavernous
 limestones.

 The alluvial deposits,  although of limited areal extent,  of-
 fer the best potential  for high-yielding wells,  especially
 where infiltration from surface streams  can increase re-
 charge.   The limestones can  be excellent aquifers where so-
 lution  cavities  are  encountered by a particular  well.   The
 dense igneous, metamorphic,  and sedimentary formations are
 the poorest aquifers in the  province but are  important be-
 cause they are  so extensive.   Typical well yields from
 these dense rocks range from only a few  gpm (gallons per
 minute)  to as much as 200  gpm.

 The Glaciated Appalachians are characterized  by  hilly or
 mountainous  terrain, with  thin glacial drift  on  the uplands
 and thick outwash and lacustrine deposits  in  the valleys.
 Local relief can be  between  1,000 and 3,000 feet,  with sev-
 eral mountain crests above 5,000 feet in elevation,  the
 highest being just under 6,300  feet.   Bedrock is predomi-
 nantly  crystalline.  However,  two broad  belts of Triassic
 sandstone and shale  are important aquifers.   One underlies
 a portion of northern New  Jersey and the other occupies the
 central  lowlands of  Connecticut and Massachusetts.

 The glacial  deposits are by  far the most important aquifer
 in the  region.   Although individual sand and  gravel beds
 are limited  in areal extent,  they are sometimes  thick  and
 permeable  enough to  supply municipal  or  industrial water-
 supply  systems that  pump millions  of  gallons  per day.   The
 greatest  ground-water potential occurs where  recharge  is
 supplemented by  river infiltration.

 The crystalline  rocks have been developed  over the entire
 region but have  generally  been  used only for  domestic  or
 small commercial water  supplies because  of  the character-
 istically  low yields of  individual  wells.   The Triassic
 sandstone  and shale, especially in  New Jersey, is  a  princi-
pal source of ground water for  municipal and  industrial
purposes.  Wells yielding  from  100  to 500  gpm are  common.
                             20

-------
The Glaciated Central Region is characterized by glacial
drift overlying crystalline and sedimentary rocks.  The land
is one of gentle slopes and only moderate relief, character-
istically between 100 and 300 feet.  The sedimentary forma-
tions are the most productive of the consolidated rocks.
For the most part, the glacial deposits are thin or of low
permeability and are primarily used for domestic supplies.
Exceptions to this are those areas where thick beds of sand
and gravel occur in existing stream courses or abandoned
pre-glacial bedrock valleys.

The Unglaciated Central Region is found only in western Penn-
sylvania within the study area and is characterized by nearly
horizontal sedimentary rocks of Mississippian, Pennsylvanian,
and Permian age.  Local relief is on the order of 300 to 500
feet.  The principal aquifers consist of alternating strata
of shale, siltstone, sandstone, and limestone.  Well yields
average about 50 to 75 gpm.

POPULATION

As of the 1970 Census, 53.5 million or 26.3 percent of the
nation's 203.2 million people reside in the project area
(Table 4).  The population is heavily concentrated in the
urban areas, particularly in the Boston to Washington, D. C.
megalopolis.  Population for the entire region increased by
11 percent between 1960 and 1970.

CLIMATE

The overall climate of the 11-state region is humid and is
characterized by frequent weather changes.  The dominant
characteristics of the climate are provided by masses of
cold, dry air from the northern interior of the continent
and by masses of warm, humid air from the Gulf of Mexico.
A secondary climatic influence is represented by masses of
cool, damp air from the North Atlantic Ocean.

The climate is moderated by the ocean along the coast and
the Great Lakes in the northwest.  Interior land areas and
particularly the mountainous regions exhibit more marked ex-
tremes in temperature and precipitation.  The average annual
temperature in the region varies from less than 38°F in
northern Maine to more than 58*F in southern Maryland. 3)

Precipitation is distributed fairly evenly throughout the
four seasons in most of the region.  The average annual pre-
cipitation is shown on Figure 3.  Annual snowfall averages
18 inches in Delaware to over 100 inches in parts of north-
ern New York and New England.
                            21

-------
           Table 4.  POPULATION OF ELEVEN NORTHEAST STATES.
                                                                 2)
                     1970      Percent increase       Population distribution
State	Population	1960 to 1970     Percent urban   Percent rural
Connecticut
Delaware
Maine
Maryland
Massachusetts
New Hampshire
New Jersey
New York
Pennsylvania
Rhode Island
Vermont
3,032,217
548, 104
993,663
3,922,399
5,689,170
737,681
7,168,164
18,241,266
11,793,909
949,723
444,732
19.6
22.8
2.5
26.5
10.5
21.5
18.2
8.7
4.2
10.5
14.1
77.3
72.2
50.7
76.6
84.6
56.4
88.9
85.5
71.5
86.9
32.1
22.7
27.8
49.3
23.4
15.4
43.6
11.1
14.5
28.5
13.1
67.9
    Total:       53,521,028         11.0             81.5           18.5
                                    22

-------
                           NORTH
40
  LEGEND





PRECIPITATION IN INCHES
        Figure 3.  Precipitation map of the northeast United States
                                                                     5)
                                O 'j

-------
 The average annual evaporation from open water surfaces
 varies from 20 to 38 inches (Figure 4),  generally increasing
 from north to south.  Most of the evaporation occurs from
 May to October.

 GEOLOGY AND GROUND-WATER RESOURCES

 Following is a discussion of the general geology in relation
 to the ground-water resources on a state-by-state basis.
 Where the water-bearing characteristics  of the aquifers are
 known,  they are  included to allow a more complete picture of
 the system.  Since it is beyond the scope of this study to
 present a detailed breakdown of the geology and aquifer prop-
 erties, the statements are couched in general terms.   Specif-
 ic references are given in the event that additional informa-
 tion is desired.

 Connecticut

 The bedrock in Connecticut consists of three significant
 rock groups:   pre-Triassic crystalline rocks,  Triassic sedi-
 mentary rocks, and Paleozoic carbonate rocks.   They can
 yield water,  in  at least limited quantities,  to individual
 wells almost everywhere.   Unconsolidated deposits,  mainly of
 glacial origin,  can be found mantling the rock throughout
 the state.   However,  these deposits of sand,  gravel,  silt,
 and clay are  only important from a water-supply point of
 view where  a  sufficient thickness  is encountered,  usually in
 the valleys of the principal drainage features and the
 coastal lowlands.   Figures 5 and 6 are generalized geologic
 maps  showing, respectively,  the  major bedrock  units  and the
 locations of  the  major coarse-grained, water-laid  deposits.

 Crystalline Rocks -

 Crystalline rocks are  the  most areally extensive  type found
 in the  state.  They are of pre-Triassic  age  and consist pri-
 marily  of granites,  gneisses,  and  schists.   These  rocks are
 the principal sources  of well-water supplies  in the  upland
 regions and are primarily  tapped by domestic,  light  indus-
 trial,  and  small  public water-supply system wells.

 In spite of their diverse  origin and appearance, all  of the
 crystalline rocks of Connecticut have similar  water-bearing
 properties  in that they generally  have a  limited capacity
 to  store and  transmit  water.   However, they  represent an  im-
 portant source of water supply.  Approximately 15  percent of
 the total population is dependent  upon individual  domestic
wells,  the  vast majority of  which  tap the  crystalline-rock
 aquifer.  An  analysis  of records for more  than 100 such
                             24

-------
                      MOUTH
                                               LEGEND

                                              AVERAGE ANNUAL EVAPORATION
                                              IN  INCHES
Figure 4. Average annual evaporation from open water surfaces

                            25

-------
                                                                          MASS.
;.
                                                                                                 CARBONATE ROCKS

                                                                                                 TRIASSIC SANDSTONE AND SHALE


                                                                                                 CRYSTALLINE  ROCKS
                             10 miles
Figure 5.  Generalized geologic map of Connecticut showing principal  bedrock
                             aquifers in Connecticut

-------
                                                                              MASS.
:
                       NORTH
                                                                                                      SAND AND GRAVEL AQUIFERS


                                                                                                NOTEj DATA FOR NORTHWESTERN SECTION
                                                                                                    NOT  COMPLETE.
                            IO miles
                                                Figure 6.  Locations of principal  sand and gravel aquifers in Connecticut

-------
wells  reveals  that the range in yield is  from less  than  one
to more  than 100 gpm,  with an average of  five gpm.  ?)

Sedimentary Rocks -

The second most extensive  rock unit  in Connecticut  consists
of siltstones,  shales,  and conglomerates  of  Triassic age,
with the infrequent occurrence of diabase intrusives.  Ex-
cept for the intrusives, the rocks were deposited originally
as unconsolidated continental sediments,  and consequently
the grain size  varies  greatly both horizontally  and verti-
cally  from bed  to bed.  This variation in rock type has  an
effect on the availability of ground water in joints and
fractures,  along bedding planes,  and in intergranular pore
spaces.   Beds of sandstone are generally  more permeable  than
beds of  shale because  some water  in  the former is contained
between  individual sand grains where the  cementing  material
has been dissolved or was  never formed.   Water in the shale
is contained almost entirely in fractures, many  of  which are
along  bedding planes.

There  has  also  been some faulting of the  sedimentary rocks.
In a few places,  this has  created large fractures which,
upon being  penetrated by a well,  will yield  a considerable
quantity of water.   Several wells drilled into sedimentary
rock penetrate  interbedded basalt flows as much  as  50 or
more feet  thick.   These basalts are  poor  aquifers,  but deep-
ening  of some of  the wells into underlying sedimentary rocks
has  improved yields  substantially.

The  water-bearing zones in the  sedimentary rocks normally
extend to depths  greater than  several hundred feet, and
evidence obtained from  the drilling  of some  wells shows  a
definite increase in yield as  the bore hole  is deepened  to
as much  as  400  feet.  An analysis of records of  688 wells
tapping  sedimentary  rocks  shows a range in yield from about
one  to as much  as 600 gpm.  8)   The average yield of the  in-
ventoried wells  is  54 gpm.   However,  it should be noted  that
many of  these wells  are used only for domestic purposes, and
the  reported yield may  simply  reflect the installed pump
capacity rather than the ability  of  the sedimentary rocks
to  furnish  water.

In  summary,  the  sandstones  and  shales  of  Triassic age are a
more dependable  source of  water than the  crystalline-rock
aquifers  in Connecticut.   In many places, the  sedimentary
formations  yield  enough water  to  wells to satisfy small
municipal,  commercial, and industrial  demands.
                             28

-------
Carbonate Rocks -

Found only in the western portion of the state, the carbon-
ate rocks consist of limestones that have been metamorphosed
to marble.  Generally, these are less resistant to weather-
ing and erosion than the adjacent crystalline rocks and thus
occupy the lowlands.

The carbonate rocks have virtually no primary porosity, and
the saturated zones contain water in fractures and, to a
lesser degree, in solution channels.  A study of well yields
indicates that the carbonate rocks have a somewhat higher
yield than the crystalline rocks.  The median yield of wells
in crystalline rocks in the western portion of the state is
about seven gpm. whereas the median in the carbonates is
about 12 gpm. 9'

Unconsolidated Deposits -

The most prolific aquifers in Connecticut, from the stand-
point of yields of individual wells and well fields, are the
localized beds of unconsolidated sand and gravel laid down
in bedrock valleys during the glacial epoch.  In addition,
some layers of sand and gravel of relatively recent age have
been deposited by existing streams.  Where beds of sand and
gravel are well-sorted and relatively free of fine silt and
clay, they tend to be very permeable.

Data on test borings and wells show that the thickness of
unconsolidated materials throughout the state varies from a
few feet to more than 200 feet in areas associated with many
of the major river valleys, such as the Connecticut, Quinni-
piac, Quinebaug, and Housatonic.  Although some of the sand
and gravel beds are very limited in areal extent, others
cover as much as several square miles.  Where thick perme-
able beds of sand and gravel are present below the water
table and are areally extensive, yields in excess of 100 gpm
can be developed from an individual well, and some wells can
produce many hundreds of gpm.

In the case where the sand and gravel beds are in direct hy-
draulic connection with a surface-water body, a well yield
is not limited by natural recharge from precipitation but is
dependent upon the ability of water to infiltrate from the
nearby stream or river.  Individual wells finished in highly
permeable unconsolidated deposits adjacent to large rivers
in Connecticut are commonly capable of producing a sustained
yield of more than one mgd  (million gallons per day), and a
number of well fields along the Housatonic, Connecticut,
Hammonassett, and Quinebaug Rivers have a rated capacity in
                             29

-------
 excess of five mgd.  7 through 11)

 The other type of unconsolidated aquifer,  used primarily  in
 rural areas,  is till.  It consists  of poorly sorted  rock
 material:  silt, sand, boulders, and clay.   Although till
 deposits  blanket most of the state, they are generally  thin
 and of low permeability.  Development is usually  by  large-
 diameter, shallow dug wells  capable of producing  a maximum
 of a few  gpm.

 The potential  for development of additional  high-capacity
 well fields in Connecticut is extremely good,  especially  in
 sand and  gravel beds  associated  with the major rivers.  Re-
 gional investigations carried out by the U.  S.  Geological
 Survey indicate numerous areas where untapped  reserves  of
 ground water exceed five to  10 mgd.   For example, in the
 Quinebaug River basin,  covering  an  area of 425 square miles,
 the estimate of ground water in  sand and gravel aquifers
 available for  development is 315 mgd.  ID  In  the Housatonic
 River basin, covering an area of 678 square  miles, the  esti-
 mate  is about  660 mgd.  9)

 Delaware

 There are  two  basic rock types in Delaware;  the crystalline
 rocks found in  the Piedmont  Province,  and the  unconsolidated
 sediments  of the Coastal Plain.  The crystallines in the
 northern  part  of the  state consist  of  gneiss,  marble, gran-
 odiorite,  gabbro and  serpentine, and comprise  about  six per-
 cent  of the total land  area.   The unconsolidated deposits of
 the Coastal Plain consist  of Cretaceous, Tertiary and Qua-
 ternary age sediments,  consisting largely of sand and clay
 beds  of marine  and non-marine  origin.   They  form a wedge-
 shaped mass, dipping  to the  southeast  where  they attain a
 thickness  of over 8,000 feet.  Figure  7 is a generalized
 geologic  map of Delaware.

 Crystalline Rocks -

 Gneiss and gabbro comprise the bulk  of the crystalline  rocks
 found in  the Piedmont  of Delaware.   Small patches of marble,
 serpentine  and  granodiorite  are  present, and narrow  pegma-
 tite  dikes  can  be found throughout much of the  province.
 The rocks  are  mantled  by clays and  sands which  are a result
 of  in-situ weathering.   Alluvial materials are  present in
 the lower  sections of  the  river  valleys.

 Both  the  fresh  rock and the  weathered  zone store consider-
 able  quantities of water.  However,  yields of  individual
wells are  generally low in sections  of the gabbro, which is
                             30

-------
                       Pfc
NORTH
t
                                                        JLEGEND

                                                        CRYSTALLINE  ROCKS
                                                        CARBONATE ROCKS
                                                        UNCONSOLIDATED SAND
                                                        AND GRAVEL DEPOSITS
                                                	FALL LINE
                                  MD.
 Figure 7.  Generolized geologic mop of Delaware
              Bowing principal aquifers 12, 13)
                               31

-------
 extremely tight with few saturated fractures.   The marble
 generally provides higher yields than the other crystalline
 rocks.

 The weathered zone is extremely variable in thickness within
 relatively short distances but is known to be  greater than
 85 feet thick in places.  12^  It is primarily tapped by dug
 wells for domestic supplies.   The material is  clayey in na-
 ture, although thin limited sand zones are occasionally
 present.   Reports indicate that the main water-contributing
 zone occurs at the contact with the unweathered rock.   Well
 yields  average a few gallons  per minute.

 Unconsolidated Deposits  -

 The unconsolidated deposits of the Coastal Plain cover a ma-
 jor portion of the land  area  in the state.  Table 5 lists
 the stratigraphic units,  their generalized lithologic  char-
 acter,  and their estimated average withdrawals during  1970
 in Delaware.   The hydraulic characteristics vary among the
 aquifers  and from place  to place within the same aquifer.

 Quaternary age  aquifers  consist primarily of sandy material.
 They are  the  most highly  developed and areally extensive in
 the state.   Yields  of  individual wells have been reported to
 be as high as 4,000 gpm.  14)

 Several different aquifers of  Tertiary age are recognized  in
 Delaware.  Many contain residual salt  water in their down-
 dip portions.   The  sediments are of marine origin and  vary
 widely in  composition, the basal and down-dip  portions  con-
 taining increasingly finer material.   Well yields of more
 than 600 gpm  have been reported.  ^4'

 Cretaceous  age  deposits overlie  the basement crystalline
 rocks and  consist of a complex series  of both  non-marine and
 marine sediments.   The marine  Cretaceous sediments  are  of
 limited extent,  thickness,  and use  in  Delaware,  containing
 salt water  in much  of the  down-dip  portion.  The  non-marine
 deposits, which attain a thickness  of  more than  6,000  feet,
 constitute the  bulk of the unconsolidated sediments.  Yields
 of  wells tapping  the Cretaceous  deposits  range  from about
 three to 300  gpm.  14>

Maine

Maine is located  entirely  within  the Glaciated Appalachians
ground-water  region.  From a hydrogeologic  standpoint,  the
state has two types  of aquifers,  consolidated  rock, and  un-
consolidated  glacial sand  and  gravel.  The  consolidated  rock


                             32

-------
           Table 5.  COASTAL PLAIN STRATIGRAPHIC UNITS AND ESTJMATED AVERAGE
                      WITHDRAWALS DURING 1970  IN DELAWARE. 12'13/'4)
System
Series
     Stratigraphic units
                        Generalized lithologic character
Estimated
average
withdrawals
during  1970
 (mgd)
Quarternary
Holocene

Pleistocene
                             Columbia Group
                             undivided
                              Fluvial sand and gravel sand

                              Littoral and shallow marine
                              clay,  silt and sand
                                                          33.32
             Pliocene

             Miocene
                 Chesapeake Group
                 undivided
                              Marine sediments; gray quartz
                              sand,  gray silt and clay, shells
                              and fragments of shells and dia-
                              tomaceous material are common
Tertiary
Oligocene
                                        SECTION NOT PRESENT
             Eocene
                 Piney Point Formation

                 Nanjemoy Formation
             Paleocene
                 Vincentown Formation

                 Hornerstown Sand
                              Marine sediments;  dark gray
                              and greenish-gray clay, silt
                              and sand with glauconite
                                                                14.10
                              Mount Laurel Sand
                                          Marine sediments;  dark gray and
                                          greenish-gray clay, silt and
                                          sand with glauconite
Cretaceous
 Upper
 Cretaceous
* 9-
£ o
Marsha 11 town Formation

Englishtown Formation

Merchantville Formation
                                                       Transition zone
             Lower
             Cretaceous
                 Magothy Formation

                 Potomac  Formation
                              Nonmarine sediments; gray and
                              white quartz sand interbedded
                              red, gray purple, brown yellow
                              silt and clay
                                                                                         14.34
                                                 33

-------
 types range from igneous through high-rank to low-rank meta-
 morphic.   These include gneiss, schist, marble,  slate, phyl-
 lite and limestone.   Figures 8 and 9 show the locations of
 the bedrock formations and the principal deposits of glacial
 outwash,  respectively.

 Consolidated Rocks -

 On the Moosehead Plateau, comprising the northwestern 40
 percent of the state,  the intensity of metamorphism of the
 rocks increases southeastward.  Nearly unmetamorphosed lime-
 stone,  sandstone,  and  shale near the northwestern border
 with Canada grade  into slate,  marble, and guartzite,  with
 occasional intrusive granite and diabase north of Moosehead
 Lake.

 South of  Moosehead Lake,  high-rank metamorphic and meta-
 igneous rocks  occur  more  frequently.   Wells  in bedrock on
 the Moosehead  Plateau  generally yield reliable domestic sup-
 plies.  Where  greatly  fractured or only slightly  metamor-
 phosed, the consolidated  rock  aquifer may yield sufficient
 water for small industries.  Yields of as much as 300  gpm
 have been reported for wells penetrating the low-degree
 metamorphosed  limestone.  4)

 The  Aroostook  Valley area occupies the northeastern edge of
 the  state.   The intensity of metamorphism as reflected in
 the  rocks  is less  systematic here,  but generally  metamor-
 phism increases from north to  south.   Wells  in the  igneous
 and  metamorphic rock usually yield less  than 10 gpm.   In the
 limestone  and  marble,  well yields  are relatively  high  when
 solution  channels  are  present.   Of 317 bedrock wells in the
 Lower Aroostook River  basin, reported yields range  from less
 than one  to  560 gpm. 16)   in the Meduxnekeag River-Prestile
 Stream basin,  the  range for  137  wells is  from less  than one
 to  400 gpm.  17)

 The  Central Uplands  region occurs  as  a broad band of rolling
 and  hilly  terrain  across  the center of the state.   Its  geo-
 logic sequence,  in a line  from east to west,  is similar to
 that of the north-south sequence in the Moosehead Plateau.
 The  bedrock well yields are  usually sufficient for  domestic
 and  small  municipal  and industrial  supplies.   Carbonate
 rocks are  not  as extensive  in this  region as  compared  to  the
Moosehead  Plateau.   Of 186 wells reported in  the  lower  Ken-
 nebec River basin, the yields range from  less  than  one  to  67
 gpm and the median is  seven  gpm. 18)

 In the Coastal  Lowlands, where the population  of Maine  is
concentrated,  igneous  and metamorphic  gneiss,  schist, and


                             34

-------
                                            NORTH
                                       0      25     50 miles
                                               LEGEND
                                             SEDIMENTARY  ROCKS

                                             CRYSTALLINE  ROCKS
Figure 8.  Generalized geologic map of Maine showing
                 principal  bedrock aquifers
                      35

-------
                                                      NORTH
                                                        25      50 miles
                                                         LEGEND

                                                        SAND AND GRAVEL
                                                         DEPOSITS
Figure 9.  LocaHon of principal sand and gravel deposits in Maine
                          36

-------
pegmatite are more abundant than slate and shale.  In this
area, reported bedrock well yields range from less than one
to 150 gpm with a median of about five gpm. 19/20,21)

Unconsolidated Deposits -

Four large sand and gravel areas are found in Maine:  in the
southwest and west central region southwest of Moosehead
Lake;  in the east central area in southern Aroostook County
and eastern Penobscot County;  in the St. John River valley
southeast of the Canadian border;  and in the Aroostook
River valley.  Only limited data are available on the yields
and depths of wells in sand and gravel.  Individual wells
tapping these aquifers might be expected to yield from a few
to upwards of 1,000 gpm and depths would rarely exceed more
than 150 feet. 4,18,19,20,2lT *

Maryland

Based on Thomas's classification of ground-water regions,
Maryland includes portions of the Coastal Plain, Unglaciated
Appalachians and a small segment of the Unglaciated Central
Region, which is located in the northwest corner of the
state.  Because this latter region contains a relatively mi-
nute land area, it is included in the general discussion of
the Unglaciated Appalachian Region.  From a ground-water
standpoint, the basic difference between the two major re-
gions is that aquifers in the Coastal Plain are unconsoli-
dated, whereas those in the Unglaciated Appalachians are
consolidated.  Figure 10 shows the locations of the two ma-
jor ground-water regions, separated by the Fall Line.

Consolidated Rocks -

The Unglaciated Appalachians contain rocks of Precambrian,
Paleozoic and Mesozoic (Triassic) age.  The eastern portion
of the region contains crystalline igneous and metamorphic
rocks, including gneiss, slate, phyllite, schist, marble,
granite, and gabbro.  These are weathered and decomposed to
depths greater than 100 feet in some locales;  the average
depth of weathering is about 40 to 50 feet. 23)  Well yields
in this region are usually around five to 10 gpm. 24)  How-
ever, higher yields are obtained locally in fault zones, and
in the lowlands where the overburden and weathered rock
zones are thick.

To the west are found two distinct Paleozoic age sequences
of limestone, dolomite, and shale, separated by Precambrian
crystalline and Triassic sedimentary rocks.  The crystalline
rocks include meta-basalt, meta-rhyolite, granodiorite, and


                             37

-------
                                                                                                                  NORTH

^
; C c
j "•~_ 	 ,:>
^. / "V^
/~--. x1
^ ^ \W^
vfe
v^
-
-"•-r-.-r-Tji
1 i i j i J{^
1 ' JC^^v
i ' i^5^>o
oc
            LEGEND

SEDIMENTARY ROCKS - SANDSTONE, SILTSTONE,
SHALE,THIN BEDS OF  LIMESTONE AND COAL

CARBONATE  ROCKS - LIMESTONE,DOLOMITE
AND  SHALE


CRYSTALLINE ROCKS

TRIASSIC SANDSTONE  AND  SHALE

UNCONSOLIDATED SAND AND GRAVEL DEPOSITS

FALL LINE
                                                                                              0   10    20   30   40"»il«i
                                                                                                      OO OQ  O A\
                     Figure 10.  -Generalized geologic map of Maryland showing principal aquifers   '  '

-------
granite gneiss, which form the highlands.  About 18 percent
of the wells in this area yield less than five gpm.

Triassic rocks overlie the limestone.  The sequence varies
in width from less than a mile to as much as 15 miles, and
consists primarily of shale, siltstone, and sandstone.  Well
yields are variable;  the highest reported yield of 300 gpm
was obtained from a well penetrating a fractured sandstone
stratum.  Nine wells in shale yielded an average of 1.5
gpm. 25)

In the lowlands bordering the crystalline rocks, the thick
sequence of carbonate rocks has been subjected to complex
folding and faulting.  The carbonates are good aquifers,
with high-yielding wells found in fault areas, and at shal-
low depths where there has been development of solution
cavities.  Wells generally range between 100 and 300 feet in
depth, and indications are that increases in yield are se-
verely limited with greater depths.  Some limestone wells
yield as much as 400 gpm, and a limestone spring discharging
3,000 gpm has been reported. 4)

The western part of the state contains sedimentary rocks of
Ordovician to Pennsylvanian age:  sandstone, siltstone, and
shale, with thin beds of limestone and coal.  These rocks
were subjected to folding and faulting, particularly in the
central and eastern portion.  They decrease in permeability
below depths of a few hundred feet.  Well yields are gener-
ally less than 10 gpm, although higher yields are obtained
in the faulted areas.  Water occurs mainly in fractures, but
some of the sandstone strata are porous, which adds signif-
icantly to the water availability and the yields of wells.

Unconsolidated Deposits -

The unconsolidated deposits of the Coastal Plain form a
wedge-shaped mass that starts at the Fall Line and thickens
to the southeast.  These deposits overlie a crystalline rock
complex and consist of sand, gravel, silt, clay, marl, and
shell beds ranging in age from early Cretaceous to Holocene.
They attain a thickness of nearly 10,000 feet along a por-
tion of the Atlantic Coast.  Various formations outcrop in a
sequence from the oldest to the youngest in a southeastward
direction.  The succession of deposits is generally similar
to that found in Delaware.

Coastal Plain deposits are thin along  the Fall Line,  and
yields from wells are generally lower  than those from wells
located further east.  To the east, well yields range  from
a few hundred gallons per minute to as much as  1,200  gpm  on
                              39

-------
 the western shore/ and as much as 1,700 gpm on the eastern
 shore of Chesapeake Bay.  Table 6 summarizes the geologic
 units of the Coastal Plain and describes their water-bearing
 properties.

 Massachusetts

 Massachusetts is located within the Glaciated Appalachians
 region.   Physiographically,  the state consists of four prin-
 cipal divisions, the mountainous, western Glaciated Appala-
 chians (known locally as the Berkshires), a central upland
 Piedmont,  the Triassic Lowland, and the Coastal Plain of
 Cape Cod and associated coastal areas.

 Figure 11  is a generalized geologic map showing the six major
 aquifers in Massachusetts.  Four of these are composed of
 consolidated rocks:   crystalline rocks, Hoosic-Housatonic
 Valley carbonate rocks,  coastal basin sedimentary rocks,  and
 Connecticut Valley sedimentary rocks.  Two unconsolidated
 aquifers also occur:   unstratified till,  and sand and gravel.

 Crystalline Rocks -

 The most areally-extensive bedrock aquifer is the crystal-
 line rock  complex:   a broad  spectrum of igneous and metamor-
 phic types  ranging in age  from Precambrian to Carbonifer-
 ous (?).  They are generally  similar in water-bearing charac-
 teristics ,  with  well  yields  usually sufficient for domestic
 supplies.   Occasional yields of 30 to 40  gpm,  adequate  for
 small-scale industrial and municipal use,  and a few yields
 of  100 to  200  gpm have been  reported.   However,  the median
 yield of wells in the crystalline  aquifer  is  about 10  gpm.
 Well depths range between  100  and  200 feet.  28 through  35)

 Carbonate Rocks  -

 In  western  Massachusetts,  the  valley of the  Hoosic and  the
 Housatonic  Rivers is  underlain principally by carbonate
 rocks, which  continue southward into Connecticut  and possi-
 bly northward  into Vermont.  Occurring between hills of pre-
 dominantly  gneiss and quartzite to the east  and schist  to
 the west, these  units  of limestone and dolomite  represent a
 productive  aquifer in this portion of the  state.   The yields
 of wells are  controlled to a great extent  by  the  size and
 number of solution channels  encountered.   In  Berkshire
 County, well yields ranged from less  than  one  to  1,700 gpm
with a median of  nine  gpm. 29)
                             40

-------
             Table 6. GEOLOGIC UNITS AND THEIR CHARACTERISTICS IN THE MARYLAND COASTAL PLAIN PROVINCE. 23'24'26)
System
Series
Stratlgraphic unit's
Generalized lithologic character
Water-bearing properties
Quaternary
Tertiary
Holocene
Pleistocene
Pliocene
Miocene
Oligocene
Eocene
Paleocene
-
Columbia Group undivided
Brandywine Formation
Chesapeake Group
Yorktown Formation
St. Mary's Formation
Choptank Formation
Calvert Formation
Soil, sand, peat and silt
Sand, silt, gravel and clay
Clay, sand and gravel
Gray, fine to medium sand, gray
or blue clayey silt
Clay, silt, fine sand, shells
Gray and green silt and clay,
some shells and fine sand
Gray and blue silt and clay,
shells, some sand
/// SECTION NOT PRESENT /^/////,
Piney Point Formation
Nanjemoy Formation
Aquiq Formation
Brightseat Formation
Dark gray to green sand, silt
and clay
Black to green glauconitic sand,
silt and clay
Green gtauconitic sand, clay
and shells
Gray to green fine to coarse
sand and clay
Small yields to shallow wells
Important aquifer with localized high
permeability, well yields up to
1,500 gpm
Limited areal extent along the Fall line
Sand section yields fair amounts of wa-
ter, locally high in iron, functions as
a semiconfining layer
Functions chiefly as a confining layer
Low yield to wells, locally hard and
high in iron
Locally yields moderate quantities of
water, occasionally highly mineralized,
primarily a confining layer
////////////////,
Important artesian aquifer, well yields
up to 1 ,200 gpm, downdip section
probably saline
Confining layer, saline in southeast
Locally an important aquifer, moderate
well yields up to 250 gpm
Limited area! extent and thickness

-------
                           Table 6 (Continued).  GEOLOGIC UNITS AND THEIR CHARACTERISTICS IN THE MARYLAND COASTAL
                                                              PLAIN PROVINCE.  23,24,26)
System Series Stratigraphic units Generalized lithologic character Water-bearing properties
Cretaceous
Upper
Cretaceous
Lower
Cretaceous
Monmouth Formation
Matawan Formation
Magothy Formation
Raritan Formation
Q_
u
o
i_
O
0
o
I
£
Patapsco Formation
Arundel Formation
Patuxent Formation
Green glauconitic sand, gray clay,
shells
Black clay and brown sand
White, yellow and gray sand with
gray and brown clay
Gray fine grain sand, gray, brown
and red clay
Clay, shale, white, gray and
green sands
Dark gray and maroon clay
Fine to very coarse sand, gray,
brown and green shale
Confining layer, saline in downdip
section
Chiefly a confining layer, locally
used as an aquifer
Well yields of up to 600 gpm, saline
in downdip section
An aquifer with saline water in
downdip section
A limited aquifer in the sandy zones,
saline in downdip section
Limited in areal extent, chiefly a
confining layer
Not developed, limited information
available, saline water thought to be
present downdip
N)

-------
                                                                           NORTH
                                                                                         50 miles
                          LEGEND

                        CRYSTALLINE  ROCKS

                        SEDIMENTARY ROCKS

                        CARBONATE  ROCKS

                        TRIASSIC  SANDSTONE
                         AND  SHALE
                 .*•:'*
UNCONSOLIDATED  SAND
AND  GRAVEL  DEPOSITS

UNCONSOLIDATED
WATERCOURSE DEPOSITS
                                                                                    ATLANTIC
                                                                                     OCEAN
                         >VMI c.nv*wunoc.  uc.rwoi i o                                o~7\
Figure 11. Generalized geologic map of Massachusetts showing principal aquifers

-------
 Coastal Basin Sedimentary Rocks -

 Within the crystalline terrain in southeast and northeast
 Massachusetts, portions of the upper bedrock consist of sed-
 imentary rock units.  The dominant rocks, dated as Carbonif-
 erous (?),  are elastics, such as sandstone, shale, and con-
 glomerate, metamorphosed to varying degrees.  They were
 originally deposited in sedimentary basins;  the two largest
 are the Narragansett and the Boston.  Some minor outcrops of
 similar age rocks occur throughout Rhode Island and eastern
 Massachusetts.

 Little  data are  available on yields from wells in these
 rocks.   For one  area,  yields reported for 92 wells range
 from one to 170  gpm, with a median yield of eight gpm.  36)

 Connecticut Valley Sedimentary Rocks -

 In the  central part of the state,  Triassic age rocks occupy
 a  tectonic basin along the trend of the  Connecticut River.
 These rocks are  primarily sedimentary:   sandstone,  shale,
 and conglomerate,  with minor limestone and intruded diabase.
 The rock types and structures are  similar to those found in
 Triassic basins  in Connecticut,  Pennsylvania,  New Jersey,
 and Maryland.

 Little  specific  ground-water data  are  available  on the  Tri-
 assic age  rocks  of Massachusetts.   For 63 wells  believed to
 be  finished in Triassic rocks, the yields ranged from less
 than one to 760  gpm, with an average of  41 gpm,  and a me-
 dian of 12  gpm.  37)

 Till and Fine-Grained  Stratified Deposits -

 Extensive  deposits  of  unstratified glacial drift,  called
 till, cover the  bedrock over most  of the  state.   Till gener-
 ally has a  low permeability  and  for that  reason  is  normally
 a poor aquifer.  During prolonged  periods of drought, wells
 in  till frequently  go  dry.   However, it is still  a  useful
 aquifer in  many  areas  because of its accessibility.   Well
yields are  typically about one to  two gpm.

Where stratified deposits of  fine-grained material  are  found,
the water-yielding  characteristics  may be similar to  those
of till.  Eolian, marine-swamp, and lacustrine deposits  are
typical fine-grained stratified units.
                              44

-------
Sand and Gravel Deposits -

The most prolific aquifers in Massachusetts are the uncon-
solidated stratified deposits, predominantly sand and gravel.
There are three major types of sand and gravel deposits, all
composed of water-borne material.  They were deposited in
contact with glacial ice during the Pleistocene Period,
as outwash in drainage areas of the melting glaciers, or as
alluvial materials associated with streams not related to
glaciation.

Sand and gravel deposits are common in many areas of the
state, particularly in the southeastern portion and on Cape
Cod.  Slightly different water-yielding characteristics for
ice-contact and outwash deposits are observed, even where
all wells are in the same drainage basin  (Table 7).  Yields
of wells in ice-contact deposits are generally higher than
those in outwash deposits in the same area.  However, yields
of wells from outwash relative to yields of wells from ice-
contact deposits do seem to improve toward the east and
south.  Outwash is thicker and more extensive in the north-
east and southeast portions of the state.

New Hampshire

New Hampshire is located within the Glaciated Appalachians
region.  Figure 12 is a generalized geologic map of the
state showing the principal aquifers.

Consolidated Rocks -

Within New Hampshire, the upper bedrock is composed of a
full suite of rock types.  Approximately two-thirds of the
state is underlain by sedimentary and volcanic rocks of
middle-Paleozoic age which have been metamorphosed to vary-
ing extents;  the remaining one-third is underlain princi-
 §ally by middle and late Paleozoic intrusives. 4)  For hy-
 rogeologic purposes, all of these rock types may be consid-
ered as one unit.  At present, sufficient ground-water
studies have not been completed to distinguish between the
water-yielding properties of various rock types.

Wells were inventoried in 228 towns in New Hampshire by G. W.
Stewart;  approximately 80 percent of the wells penetrated
bedrock. 39)  In the southeastern area, drilled wells pene-
trating bedrock yield small to moderate quantities of water
suitable for domestic and small industrial use. 40)in the
lower Merrimack River valley, yields are  similar  to those  in
the southeast. 41)  In one report, it was noted that of
1,482 wells for which a yield-was reported, the median was
                             45

-------
          Table 7. YIELDS AND DEPTHS OF SELECTED WELLS IN SAND AND GRAVEL DEPOSITS
                               IN MASSACHUSETTS.  30,32,33,35,36,38)
Drainage basin
Housatonic River
Millers River
Assabet River
Ipswich River
Parker River and
Rowley River
Type of deposit
Outwash
Ice -con tact
Outwash
Ice -contact
Outwash
Ice -con tact
Outwash
Ice -contact
Outwash
Ice -contact
Reported
number
of wells
N
N
13
43
6
56
28
128
3
18
Range in
yield
(gpm)
900
273
720
70
300
690
718
76
500
Median
yield
(gpm)
N
N
22
31
11
40
34
40
14
17
Reported
number
of wells
N
N
N
N
40
178
217
363
23
55
Range in
depths
(feet)


3
2
5
8
5
7
N
N
N
N
- 112
- 115
- 90
- 80
- 51
- 115
Median
depth
(feet)
N
N
N
N
40
25
16
21
21
39
Taunton River
All types of sand
and/or gravel
373
2   -   900
40
408
7- 173
45
N - Not reported

-------
                                      NORTH


!,:


-.••'.ill
         MASS.
                                        15    30miles
                                            LEGEND
                                          CRYSTALLINE  ROCKS
                                        ] SEDIMENTARY ROCKS
                                          UNCONSOLIDATED
                                          WATERCOURSE
                                          DEPOSITS
                                       ATLANTIC
                                        OCEAN
Figure  12.  Generalized geologic map of New Hampshire
                   showing principal aquifers
                   47

-------
 6.5 gpm;  most of these wells penetrated bedrock.   '

 Unconsolidated Deposits -

 Sand and gravel comprise the major water-yielding unit,  oc-
 curring mainly as outwash deposited by melt waters from
 Pleistocene glaciation, and as outwash and alluvium deposit-
 ed in narrow stream valleys during late Pleistocene glacial,
 post-glacial,  and recent times.   Minor sand and gravel de-
 posits occur as kames,  eskers, and lenses of sorted material
 within till.

 Long-term yields are limited by the thickness and extent of
 the deposits.   The best yields usually occur in wells  adja-
 cent to perennial streams,  where pumping may induce surface
 water into the aquifer.  Available information suggests  that
 yields of a few hundred gpm are  common.  40,41)   The deposits
 are reported to be as much  as 200 feet thick.  40)

 New Jersey

 Segments  of three ground-water regions are found in New  Jer-
 sey:   the Unglaciated Appalachians,  the  Glaciated Appala-
 chians,  and the Coastal Plain.  1)   The rock types and  water-
 bearing characteristics are  different  among the regions,  and
 from location  to location within the same region.   The major
 aquifers  northwest of the Fall Line  are  mostly consolidated
 rocks,  while those to the southeast  are  unconsolidated de-
 posits.   Figure 13 is a generalized  geologic map of the
 state,  showing the principal water-bearing rocks.

 Consolidated Rocks -

 The northwestern portion  of  the  state  is characterized by
 broad  valleys  and ridges  containing  rocks composed of  lime-
 stone,  shale,  sandstone,  and quartzite of Early Paleozoic
 age.   Glacial  deposits  cover most  of these  rocks and,  in
 some areas  in  the major stream valleys,  are  thick  and  perme-
 able enough to be important  aquifers.  The  sandstone and
 quartzite  strata are poor aquifers, partially  because  of
 their  irregular and variable thickness but primarily due  to
 the  lack  of major fracturing.  Where these rocks are found,
 the average thickness is  50  to 100 feet.   However,  in  many
 areas,  they are  completely absent. 44)    Wells  penetrating
 these  rocks usually obtain water at the  contacts with  over-
 lying  or underlying formations.

The major aquifer  is the  Kittatinny Limestone.   It  is  com-
posed primarily  of  dolomite, but the distinction between
 limestone and  dolomite  is of no importance with  regard to


                             48

-------
	FALL LINE
       LEGEND

       CARBONATE ROCK
       AND SHALE

       CRYSTALLINE ROCKS
       TRIASSIC  SANDSTONE
       AND SHALE

       UNCONSOLIDATED  SAND
       AND GRAVEL DEPOSITS

       UNCONSOLIDATED
       WATERCOURSE  DEPOSITS
                                                                     NORTH
            Figure 13.  Generalized geologic map of New Jersey

                              showing principal aquifers
                                49

-------
 hydrologic characteristics.  Some large solution cavities
 are present, in addition to vugs and fractures.  Well yields
 are highly variable from one location to another, with many
 in excess of 100 gpm.

 In the northwest, the most extensive formation areally is
 the Martinsburg, which consists of a thick sequence of
 shales, slates, and sandstone.  Generally, these rocks are
 poor aquifers,  with well yields averaging a few gpm.  How-
 ever, wells penetrating fault systems can yield several hun-
 dred gpm.

 To the east, the belt of Precambrian rocks consists prima-
 rily of gneiss, schist, and granite.  Typical well yields
 are in the range of five to 10 gpm,  with only those wells
 located near major fracture systems  having substantially
 higher yields.  4)

 Further east, Triassic age sandstone, shale,  argillite, trap-
 rock, and local occurrences of conglomerate are found.  The
 Stockton sandstone is a good aquifer with some primary po-
 rosity, especially in the poorly cemented sections.   However,
 the lower section is typically well  cemented  with only minor
 fractures.

 The Brunswick shale constitutes the  bulk of the rock of Tri-
 assic age.   It  has a low porosity, but locally well-devel-
 oped fractures  are known to occur and may extend to a few
 hundred feet in depth.   Well yields  are generally greater
 than 100 gpm.   The Lockatong argillite is an  accumulation of
 fine-grained lake deposits.   It is dense,  very hard, and
 forms the crests  of ridges because of its resistance to ero-
 sion.   The  formation is  a poor aquifer with very low poros-
 ity and few joints.   Wells tapping this formation have low
 yields.

 Basalt and  diabase rocks,  known as traprock,  are also found
 in the Triassic section.   The basa.lt was formed by a series
 of lava flows,  and the  diabase intruded as a  sill,  a por-
 tion of which makes up  the Palisades bordering the Hudson
 River.   The sill  is extremely tight  with only minor  joints.
 Well yields from  these  units are generally only a few gpm.

 Unconsolidated  Deposits  -

 Unconsolidated  deposits  of Pleistocene age cover a major
 portion  of  the  Triassic  rock area, with the southernmost
 terminal  morraine dividing it almost in half.   The northeast
 portion  contains  mostly  fine-grained lake  deposits and till,
with  some scattered deposits of glacial outwash.   In the
                             50

-------
southwest, glacial outwash is found in the southwest-trend-
ing valleys.  Wells tapping thick and permeable outwash de-
posits frequently have yields in excess of one mgd.

The Coastal Plain region south and east of the Fall Line in-
corporates about three-fifths of the state.  The unconsoli-
dated deposits consist of sand, gravel, clay, silt and marl,
forming a wedge-shaped mass which thickens to the southeast.
They attain a thickness of over 6,000 feet, with an average
dip of about 100 feet per mile. 45) The sequence of deposi-
tion is similar to that of Delaware and Maryland.

Of the total thickness of the Coastal Plain deposits, ap-
proximately half is made up of non-marine sediments of Cre-
taceous age forming the basal part of the section.  Overly-
ing these sediments are marine deposits of late Cretaceous
to early Tertiary age, which attain a thickness of over
1,000 feet.  These in turn are overlain by a sequence of
marine and non-marine deposits of late Tertiary age, which
attain a thickness of about 1,000 feet.  Quaternary age
sediments blanket the older deposits and, in some buried
channels, are 200 or more feet thick. 45)

The most productive and developed aquifers are the Raritan
and Magothy formations of Cretaceous age, with well yields
of 500 gpm or more.  Several other important Cretaceous
aquifers are the Englishtown, Wenonah, Mount Laurel, and Red
Bank Sand formations.  Well yields in these aquifers are
commonly 100 gpm or more, with some yields up to 500 gpm. 4)

The Tertiary sequence contain some formations that are im-
portant aquifers, including the Vincentown, Kirkwood, and
Cohansey formations.  Moderately-high well yields are common.
The Quaternary deposits are important aquifers locally, par-
ticularly along the coast and the Delaware River.

New York

The geology of New York is as varied as that of any  state in
the study area.  Basically, however, the rock types  of New
York may be classified into six hydrogeologic units  based on
similar water-bearing characteristics  (Figure 14).   These
units include crystallines;  shales;  sandstones;  and car-
bonate rocks;  as well as glacial  and pre-Pleistocene
Coastal Plain deposits.

Crystalline Rocks -

The crystalline rocks in New York  are the most complex and
variable of all the rock groups in the  state.  The component


                             51

-------
                                                                                             CANADA
•
                                                      50
                    NORTH
                                                                                                              VERMONT
                     ^
                                                                                                             -'  MASS.
                                                                                                             CONN.
                                                     LEGEND
                                       SANDSTONE

                                       SHALE
                        |j UNCONSOLIDATED  SAND
                         AND  GRAVEL DEPOSITS

                  11.*.*-'" *| UNCONSOLIDATED
CRYSTALLINE ROCKS          WATERCOURSE DEPOSITS
                                       CARBONATE  ROCKS
            Figure 14.  Generalized geologic  map of New York showing principal aquifer

-------
rocks are primarily metamorphosed sedimentary and igneous
units and are the oldest in New York.  Most have been sub-
ject to many periods of deformation and recrystallization.

Crystalline rocks outcrop almost exlusively in two areas of
the state.  The largest portion is found in the northeast,
where a blocky mass of granite, gneiss, and schist forms the
Adirondack Mountains.  The other major outcrop area occurs
in the southeast, where crystalline rocks underlie most of
New York City and its northern suburbs.

Despite the complex geology and structure of the crystalline
rocks, they exhibit very similar water-bearing characteris-
tics, and can be lumped into one hydrogeologic unit.  The
crystalline rock aquifer is acknowledged to be the least
productive bedrock unit in the state. 46)  Yields of from
one to 10 gpm are common.

Shales -

The areas designated as shale in Figure 14 actually include
shale, slate and a low-rank, metamorphosed rock usually de-
scribed as schist.  Shale is the predominant unit in the
areas so mapped, but interbeds of sandstones, limestones,
and evaporites commonly occur.  Except in the easternmost
part of the state, the shale is only moderately folded and
faulted.

Typically, well yields are sufficient only for domestic and
small industrial supplies  (a few to several tens of gpm).
Exceptions may occur where a well drilled into shale has a
source of adequate recharge, such as an adjacent surface-
water body or thick overlying unconsolidated deposits.
Large yields  (up to 3,000 gpm) reported for wells pene-
trating the Salina Group in the Buffalo area are probably
due to induced recharge from major streams in the area. ^)

Sandstones -

Sandstone constitutes the upper bedrock surface over two
broad areas:  in the northeastern region flanking the north-
ern limit of the Adirondacks, and in the central region
forming an upland area skirting the southeast shore of Lake
Ontario.  Isolated sandstone units occur in the extreme
east-central region of the state in the Taconic Mountains
east of Albany, and in the southeastern region in Rockland
County.

The sandstone aquifer, though fairly productive, is not  used
extensively because of a number of factors.  First, this

                             53

-------
 resistant rock forms uplands which are not conducive to res-
 idential and commercial development.  Also, surface-water
 sources and better aquifers are often available in the same
 area.   As with the crystalline and shale aquifers, the fre-
 quency of fractures, faults, and bedding planes, along with
 a good source of recharge, primarily determine yield of
 wells  of sandstone aquifers.  Where the material cementing
 sand grains is calcitic,  solution channels often increase
 permeability.

 Yields of wells tapping sandstone are typically 10 to 15 gpm.
 However,  in Rockland County (southeastern region), 265 wells
 penetrating the Newark Group of Triassic rocks (in which
 sandstone is the predominant water-bearing unit)  range in
 yield  from three to 1,515 gpm;   the average yield is 80 gpm
 and the median 30 gpm. 48)   Selected public-supply wells
 tapping these rocks have  an average yield of 300 gpm for 25
 wells.  48)

 Carbonates -

 The carbonate rocks as a  whole  are the most productive bed-
 rock aquifers in New York.   There are three types of carbon-
 ate rocks:   limestone,  dolomite,  and marble,  all of which
 have similar water-bearing properties.

 Three  major carbonate rock areas  in New York are considered.
 The first area  outcrops on the  flanks of the Adirondacks in
 the northeast.   Usually outcropping in valleys eroded by
 streams flowing off the Adirondack highlands,  the carbonate
 aquifer in  this section is  rarely used for more than domes-
 tic supply  because  of the  availability of good quality sur-
 face-water  sources.   Individual well yields,  depending upon
 the carbonate unit  tapped,  average from nine to 35 gpm.  49,
 50,51)

 A  second  important  carbonate-rock area  occurs  as  two bands
 10  to  20  miles  apart  across  the western and central portions
 of  the  state.   The  southernmost band can be traced eastward
 to  the  Hudson River valley,  where it flanks the northeastern
 Catski11s and trends  southwest  toward the juncture of New
 York, New Jersey, and Pennsylvania.   Along most of its
 length, this band is  a very  important aquifer  because it
 often is  the best-producing  aquifer in  an area of question-
 able surface-water  quality.

The strips  of carbonate rock outcropping east  to  west across
the central and western region  consist  of a northerly band
of predominantly dolomite  (Lockport formation)  and a  south-
erly band of predominantly  limestone (Hamilton-Onondaga


                              54

-------
group).   Table 8 illustrates the characteristic yields of
wells in these units.  Most of the wells in the Buffalo area
which exhibit unusually high yields appear to derive much of
their water by infiltration from the Niagara River and Tona-
wanda Creek Basins.

A third area of the state, in which carbonate rock is the
principal bedrock aquifer, is in the southeast sector.  Here,
the carbonates associated with the Appalachian mountain-
building have been metamorphosed to varying degrees.  Aver-
age yields reported for selected wells in Dutchess, Putnam
and Westchester Counties are 22, 10 and 40 gpm, respectively.
52,53,54)

Unconsolidated Deposits -

Two types of unconsolidated glacial deposits are present,
the most extensive being till.  The till deposits vary from
a few to several hundred feet thick.  Till is not considered
to be a productive aquifer other than for domestic supplies.

Sorted deposits, although more limited in areal extent than
unsorted deposits, are usually the most productive water-
bearing units in the state.  However, isolated areas exist
in which dune deposits or lacustrine deposits are found.
These are generally too thin and/or too fine grained to
yield significant quantities of water.  They have the gener-
al water-bearing characteristics of till deposits.

The most significant water-lain, unconsolidated sediments
consist chiefly of sand and gravel which have been deposited
under one of the following conditions:  a) pre-Pleistocene
(pre-glacial) period of erosion of the bedrock uplands;  b)
during the Pleistocene period when the glacial front was
melting and the meltwater was transporting large quantities
of sediment, or;  c) by large post-Pleistocene streams car-
rying significant quantities of sediment.

Several areas are found in the state in which productive
sand and gravel aquifers afford large-scale diversions.  In
the Lake Champlain-Upper Hudson River Basin, along the lower
Hudson River Valley  (a band along the eastern border  30
miles wide), and throughout the central and western portions
of the state, sand and gravel are found in the major  drain-
age systems, especially those trending north-south.   Table 9
provides data on wells tapping non-Coastal Plain sand and
gravel deposits.

Individual sand and gravel aquifers in central and western
New York have been reported to have available yields  as

                             55

-------
         Table 8.  RANGE IN AND MEDIAN YIELDS OF SELECTED WELLS IN
                 CARBONATE ROCKS IN THE CENTRAL REGION. 41,55,56,57)
Area
Syracuse vicinity

Rochester vicinity

Buffalo vicinity

Rock Unit
Dolomite
Limestone
Dolomite
Limestone
Dolomite
Limestone a'
Number
of wells
reported
13
19
21
81
16
60

1
3
5
0.
5
5
Range
(gpm)
30
- 700
- 500
5 - 300
- 2,300
- 3,000
Median
(gpm)
4
25
180
22 b)
200
323 b)
a)  Combined data from yields of wells finished in two formations.

b)  Average
                                    56

-------
Table 9. RANGE IN AND AVERAGE YIELDS OF SELECTED WELLS
AND GRAVEL AQUIFERS. 47,48,49,52,53,55,58
Region
Northeast
Southeast



West-Central

Central
Area
Lake Champlain-Upper Hudson
Columbia
Dutchess
Putnam
Rock land
Rochester area
Buffalo-Niagara
Sullivan
I^SAND
Number Range
of we Ms (gpm)
- °) o -
51 0-
37 3 -
55 1 -
-a) 8 -
23 10 -
20 30 -
40 2 -
400
350
625
450
1,700
1,016
800
700
Average
(gpm)
28
27
25
33
183
287
209
175
-38
b)
b)

b)



a) Information not provided




b) Median
                                     57

-------
 great as 31 mgd in the Jamestown area and 12 to 20 mgd in
 the Syracuse area. 60,56)  Kantrowitz estimated that all of
 the sand and gravel aquifers in the central New York area
 centered about Syracuse had an available yield of 240 mgd
 although the estimated 1970 withdrawal from all ground-water
 sources in the area was only 27 mgd. 56)

 The area of the most extensive sand and gravel deposits is
 the Coastal Plain of Long Island and lower Staten Island.
 Here the bedrock is overlain by deposits  of Cretaceous age,
 which in turn are capped by Pleistocene sediments.

 The aquifer system of the Coastal Plain in New York is com-
 prised of four major water-bearing zones  more or less sepa-
 rated by confining beds.  Yields of from  several hundred to
 a thousand gpm can be developed from individual wells.  Well
 depths are most commonly 300 to 1,000 feet.   The available
 ground water in storage in Long Island's  sand and gravel
 aquifers is estimated at 5 to 10 trillion (million-million)
 gallons. 61)

 Pennsylvania

 In Pennsylvania,  six basic hydrogeologic  units exist (see
 Figure 15).  Each of these is represented by a predominant
 or characteristic rock type.   The units are  Precambrian and
 early Paleozoic crystalline rocks,  Cambro-Ordovician car-
 bonate rocks,  middle Paleozoic clastic  rocks,  late  Paleo-
 zoic sedimentary  rocks with coals,  Triassic  sedimentary
 rocks, and unconsolidated sand and  gravel deposits.

 Crystalline Rocks  -

 The crystalline rocks  are the oldest rocks in  Pennsylvania.
 Although extremely variable geologically,  they have  been
 grouped into  a single  hydrogeologic unit  based on similar
 water-bearing characteristics.   Found exclusively in the
 southeastern  portion of the state,  the  crystalline  rocks
 encompass a full  suite of igneous and metamorphic rock types,
 including gneiss,  greenstone,  serpentine,  anorthosite,
 schist and  quartzite.   The crystalline  rocks have been ex-
 tensively deformed by  tectonic  activities  associated with
 formation of  the present  Appalachian Mountains.  The yield
 of  a particular local  rock unit is  directly related  to the
 degree of deformation.

 Ground water  in the  crystalline rocks is  found within frac-
 tures  and weathered  zones  under water-table and  semi-
 artesian  conditions. 63'   Lohman reported  that of selected
wells  in  crystalline rock  in  southeastern  Pennsylvania,  50

                              58

-------
                                                                                                                                  NORTH
Ul
£
                              TRIASSIC SANDSTONE AND SHALE

                              MIDDLE  PALEOZOIC SANDSTONE,
                              SHALE  AND  LIMESTONE

                              LATE PALEOZOIC  SANDSTONE,
                              SHALE,LIMESTONE AND  COAL
CAMBRIAN-ORDOVICIAN CARBONATE
ROCKS

PRECAMBRIAN-EARLY PALEOZOIC
CRYSTALLINE  ROCKS
UNCONSOLIDATED SAND AND
GRAVEL DEPOSITS

UNCONSOLIDATED
WATERCOURSE DEPOSITS
                                                 Figure  15.  Generalized geologic map of Pennsylvania  showing principal aquifers
                                                                                                                                            62)

-------
 percent yield from five to 20 gpm,  and 25 percent yield from
 20  to 100  gpm.  64>

 Carbonate  Rocks -

 The rocks  mapped in this hydrogeologic unit are  not  all car-
 bonates but  include some shales  and sandstones.   The carbon-
 ates are the principal  water-yielding  units,  and occur  as
 both limestone  and  dolomite which have been deformed to vary-
 ing degrees.  They  appear as  the upper bedrock unit  primarily
 in  three northeast-southwest  trending  bands,  two in  the
 southeastern region enclosing a  wedge  of  Triassic rocks and
 one in the central  region surrounded by Silurian elastics.

 Wells tapping the southeasternmost  carbonate  band in the
 Chester Valley  have variable  yields, often as high as 2,000
 gpm where  solution  channels are  tapped. 65)   The Schuylkill
 River Basin  is  traversed by both the Great Valley and Chester
 Valley.  The valleys mark the outcrop  of  the  two southeastern
 carbonate  bands;  median yields  of  wells  tapping various car-
 bonate units in the Schuylkill River Basin range from nine to
 220 gpm. 66)  Farther west in the Great Valley near  Harris-
 burg,  it is  reported that 1,000  gpm wells have been  devel-
 oped in the  carbonate rocks.  67)

 Middle Paleozoic  Clastic Rocks -

 In  the central  and  northeastern  sections  of Pennsylvania,
 the upper  bedrock surface is  composed  of  shales,  sandstones,
 and limestones  deformed  during the  mountain-building period
 which  produced  the  Appalachians.  In some areas,  these  rocks
 are flat lying  to gently dipping, but  elsewhere  they are ex-
 tremely  deformed.   The sandstones are  usually ridge  forming,
 while  the  shales  and limestones underlie  valley  floors.
 Most of  the  rocks were deposited during Silurian   and Devon-
 ian time except for some  elastics which had been  deposited
 during later  Ordovician  time.

 Yields of wells finished  in the clastic rocks are  generally
moderate, but yields locally depend  on geology and structure.
The  higher yields from wells in elastics  as compared  to
 crystalline  rocks may be  attributable  to  intergranular po-
rosity of the sandstones  and a tendency for fractures to
continue to  greater depths.  Median  yields  from wells fin-
ished  in various clastic  units in the  upper Schuylkill River
Basin are reported  to range from 54  to 175  gpm. 66)
                             60

-------
Late Paleozoic Sedimentary Rocks and Coal -

Occurring in the western part of Pennsylvania, flat lying to
gently dipping beds of sandstone, shale, limestone, and coal
form a broad plateau with incised stream valleys.  Sandstone
is the best water-yielding formation;  the limestone is com-
monly very thin.

Well yields of up to 300 gpm have been reported in certain
sandstone formations. 68)  Many wens have reported yields
of greater than 50 gpm and a mean yield of 50 to 75 gpm is
indicated. 64,4)  Little information is available on depths
of wells in the western area.  Generally, wells are shallow
because highly mineralized ground water occurs at depth.

Triassic Sedimentary Rocks -

Separating the two areas of crystalline and carbonate rocks
in the southeastern region is a strip of rocks, mainly sand-
stones and shales with minor conglomerate, limestone, coal
and intrusive diabase, varying from five to 25 miles in
width.  Of Triassic age, these rocks trend northeast to
southwest and beyond the borders of Pennsylvania into Mary-
land and New Jersey.  Physiographically, this section is the
Triassic Lowland.  The three major Triassic rock units are
Stockton sandstone, Lockatong argillite and Brunswick shale.
Range of yields for wells finished in the Stockton sandstone
has been reported to be from 100 to 300 gpm in Chester
County, although the upper one-third of the unit is not
particularly productive. 65)  in the Landsdale area, 120
wells in the Brunswick shale have a reported range in yield
of from 10 to 350 gpm, with a median yield of 70 gpm. °9)
Except in fault zones as in Chester County north of Phila-
delphia, yields of wells finished in the Lockatong average
10 gpm.  Where faults are penetrated, yields of  100 gpm may
be attained. 65)

Unconsolidated Deposits -

The two most prolific aquifers in Pennsylvania are the un-
consolidated watercourse and Coastal Plain deposits.  Water-
course deposits are commonly found in all the major stream
valleys.  They may consist of sand and  gravel eroded by
streams flowing off the uplands.  Where a major  stream had
its headwaters in the glaciated region  (most of  the north-
eastern and northwestern areas of Pennsylvania as  seen in
Figure 2, glacial drift and meltwater-borne sediment pro-
vided additional material.  Some watercourse deposits which
formed before Pleistocene glaciation were buried by glacial
                             61

-------
 drift;   others which formed during the glacial period were
 buried by finer sediments (silt and clay)  during the late
 glacial and post-glacial periods when streams could not com-
 petently carry a coarse sediment load.  These buried valley
 deposits are often as valuable as aquifers as are sand and
 gravel still in contact with a stream.

 In the southwestern region,  selected wells are reported to
 yield 200 to 600 gpm. 08)   in Clinton County (south-central
 region)  several wells yield  about 150 gpm. /O)   in the north-
 west,  the maximum reported yield from a sand and gravel well
 was 183 gpm.  71)

 Watercourse deposits have  been most extensively developed in
 the southwestern region in Allegheny and Beaver Counties.
 Of 147  wells  in the Pittsburgh area, 101 wells  have reported
 yields  of greater than 100 gpm,  with 17 greater than 500
 gpm.  72)   Forty-six selected wells in the  Ohio  River Valley
 in Beaver County have a mean yield of 544  gpm and a mean
 specific capacity of 48.3  gpm/foot of drawdown.

 The Coastal Plain deposits are found in only a  small area in
 southeasternmost Pennsylvania,  near Philadelphia.   These de-
 posits  consist  of gently southeast dipping non-marine Creta-
 ceous units overlain by Pleistocene marine terrace deposits.
 The two  deepest sand and gravel  units are  the Farrington and
 Sayreville  sand members of the Raritan formation which are
 artesian aquifers.   The shallowest (Old Bridge  sand)  member
 of the Raritan  formation and the Pleistocene terrace de-
 posits are  water-table  aquifers.  73)

 In Philadelphia,  the Farrington  sand is the  principal aqui-
 fer, and well yields commonly are 700 to 1,100  gpm;   north-
 east of  Philadelphia in southeastern Bucks County,  the Say-
 reville  sand is  the  most prolific aquifer  in the area al-
 though it is not  often  used  (yields  commonly 300 to 700  gpm).
 Water-table wells  in southeastern Bucks County  in  sand and
 gravel commonly yield about  400  gpm.  '•*'   A  summary of se-
 lected wells in  southeastern Bucks  County  indicates that 41
wells had an average yield of 320  gpm and  a  maximum of
 1,050 gpm.  74)

Rhode Island

Except for  Block  Island, which lies  to  the south and  is  in
the Coastal Plain, all  of  Rhode  Island  lies within  the Gla-
ciated Appalachians  region.   Crystalline rocks are  promi-
nent in the eastern  and western  parts of the  state,  sepa-
rated by a  sequence  of  sedimentary rocks trending north  to
south.  Mantling these  consolidated  rocks  nearly completely


                             62

-------
are unconsolidated deposits, primarily unstratified, unsort-
ed glacial till but with important areas of sorted sand and
gravel.  Figure 16 is a generalized geologic map showing
locations of the principal aquifers.

Crystalline Rocks -

The crystalline rocks of Rhode Island are found in the west-
ern half and in the southeast corner of the state.  The
rocks are quite variable in type and age.  Metamorphic rocks
include schist, gneiss, quartzite, marble, and greenstone,
and igneous rocks include granite, diorite, gabbro and vol-
canics. 75)  The ages of these rocks vary from Precambrian(?)
to post-Pennsylvanian.  From a water-yielding standpoint,
little distinction has been made between crystalline types.

Crystalline rocks are generally tapped for domestic supplies,
and yields are usually small.  For 369 wells reported, the
range in yield is from less than one to 96 gpm with an aver-
age of 12 gpm.  Sixty percent of these wells yielded less
than 11 gpm. 76)

Sedimentary Rocks -

The upper bedrock in about one-third of Rhode Island is com-
posed of sedimentary rocks of Pennsylvanian(?) age.  These
rocks occur in three structural basins, the Narragansett,
the North Scituate, and the Woonsocket.  The rocks are pre-
dominantly non-marine elastics, ranging in composition from
conglomerate to shale.  Coal beds occasionally occur in the
sequence.  These rocks have been slightly to extensively de-
formed and metamorphosed.

The sedimentary rocks have a higher water-yielding capabil-
ity than the crystallines.  Reported yields for 418 wells
range from less than one to 500 gpm with an average of 31
gpm.  Fifty-two percent of the wells yield less than 11
gpm. 76)

Till -

Till mantles the bedrock nearly completely in all areas not
covered by sand and gravel.  In the upland areas, till is
the exclusive bedrock cover.  Wells finished in till gener-
ally yield less than two gpm. 76)

Sand and Gravel -

The aquifer in Rhode Island which can produce the highest
yields to individual wells is composed of sand and  gravel.


                             63

-------
        MASS
                                           NORTH
                                                  8 miles
                                          LEGEND
                                       ] CRYSTALLINE ROCKS
                                 (j&ffffi SEDIMENTARY  ROCKS
                                        UNCONSOLIDATED SAND
                                         AND GRAVEL DEPOSITS
Figure  16.  Generalized geologic map of Rhode Island

               showing principal aquifers   '
              64

-------
These deposits are sorted and stratified, primarily composed
of outwash but with associated alluvium and ice-contact
units.  They lie along nearly all the major streams, and
especially in the central and southwestern portions, also
occur in some interstream areas. 4)

Properly constructed and developed sand and gravel wells may
be capable of high yields.  For wells ending in outwash, one
report noted a range in yield from three to 2,700 gpm. 76)
For 21 public and industrial supply wells in outwash in the
Providence area where the aquifer is extensive, a range of
from 75 to 1,600 gpm is reported with a median yield of 425
gpm. 77)

On Block Island, yields of 11 wells believed to penetrate
the Upper Cretaceous sediments range from five to 15 gpm,
with a median of 12 gpm;  yields from wells penetrating gla-
cial deposits range from four to 65 gpm, with a median of
10 gpm. 78)

Vermont

In Vermont, three major consolidated rock aquifers are found;
the Cambro-Ordovician carbonates of the Vermont Lowland;
the Precambrian and early Paleozoic sedimentary elastics and
metasediments of the Green and Taconic Mountains;  and the
Paleozoic crystalline rocks of the Vermont Piedmont.  Uncon-
solidated aquifers consisting of sand and gravel are found
in major stream valleys.  Figure 17 is a generalized geo-
logic map showing the principal aquifers.

Consolidated Rocks -

The Vermont Lowland located in the western portion of the
state is a sequence of carbonates, quartzites, shales and
slates in which carbonates dominate. 80)  The carbonates are
generally the principal water producer.  Data on the yields
and depths of wells are scanty.  Reported yields of ten
wells range from one to 100 gpm. 81,82,83)

Lying east of the Vermont Lowland is a highland area com-
posed of a sequence of deformed clastic rocks metamorphosed
to varying degrees.  The highlands are called the Green
Mountains, consisting of Precambrian and early Paleozoic
argillaceous slate, schist, gneiss, phyllite, quartzite, and
marble.  In the southwest part of the state, a mass of  simi-
lar rocks lie distinct from the Green Mountains, separated
from them by the Vermont Valley.  This mass forms the Ta-
conic Mountains.
                             65

-------

                                   NORTH
                                     IS
30 miles
                                      LEGEND
                                    CARBONATE ROCKS
                             V////A  SEDIMENTARY CLASTIC  AND
                             *ff''fA  META SEDIMENTARY ROCKS
                                   I  IGNEOUS AND
                                     METAMORPHIC  ROCKS
                                     UNCONSOLIDATED
                                     WATERCOURSE
                                     DEPOSITS
Figure  17.  Generalized geologic map of Vermont
                                      27 79^
             showing principal aquifers   '
               66

-------
Data on wells penetrating the Green and Taconic Mountain se-
quences are limited.  In the Hoosic and Walloomsac River Ba-
sins of extreme southwest Vermont, four wells had a range of
from four to 25 gpm with a median of seven gpm.  In the West-
Deerfield River Basin due east of the Hoosic River Basin,
five wells penetrating bedrock range in yield from four to
100 gpm, but the median is only four gpm. 84)

The rocks of the Piedmont of eastern Vermont are similar to
those of the Green Mountains with two notable exceptions —
the Piedmont has prominent carbonates and acidic intrusives.
Physiographically, the Piedmont has a gently rolling, dis-
sected surface and is separated from the Green Mountains by
a series of north-south trending valleys.  Because of great-
er frequency of occurrences of carbonates in the Vermont
Piedmont as compared to the Green Mountains, yields tend to
be higher.  Yields of 30 bedrock wells in five eastern Ver-
mont river basins range from one to 100 gpm with median
yields of from three to 16 gpm. 84 through 88)

Unconsolidated Deposits -

The sand and gravel aquifer in Vermont occurs in major
stream valleys.  Variations in yields of wells very often
depend upon the quantity of water desired.  Data from se-
lected wells in 11 major river basins were compiled by A. L.
Hodges and D. Butterfield and are presented in Table 10.
                             67

-------
Table 10.  RANGE IN AND MEDIAN YIELDS OF SELECTED WELLS IN SAND AND
               GRAVEL AQUIFERS IN VERMONT. 81 "trough 91)
River basin
Batten Kill, Waloomsac and Hoosic
Otter Creek
Winooski
LaMoille
Missisquoi
West Deerfield
Ottanquechee-Saxton
White
Wei Is-Ompomanoosuc
Nulhegan-Passumpsic
Lake Memphremagog
Number
of wells
8
18
13
6
5
12
25
18
10
4
3
Range
(gpm)
12-
6-
5 -
20 -
20 -
6 -
7 -
5 -
3-
60-
50 -
250
450
600
560
600
465
1,140
250
1,100
800
550
Median
(gpm)
175
95
100
155
60
35
40
43
68
350
350
                               68

-------
                     REFERENCES CITED

                        SECTION IV
 1.  Thomas, H. E.,  "Ground Water Regions of the United
    States - Their  Storage Facilities/" U. S. 83rd Congress,
    House Interior  and  Insular Affairs Committee, The Phys-
    ical and Economic Foundation of Natural Resources,
    Vol. 3, 1952.

 2.  Bureau of  the Census, "General Population Characteris-
    tics, United States Summary," U. S. Department of Com-
    merce, January  1972.

 3.  National Oceanic and Atmospheric Administration,  "Cli-
    mates of the States," Port Washington, New York,  Water
    Information Center, Inc., Vol. 1 - Eastern States,  1974.

 4.  McGuinness, C.  L.,  "The  Role of Ground Water  in the
    National Water  Situation," U. S. Geological  Survey  Wa-
    ter-supply Paper 1800, 1963.

 5.  Geraghty,  J. J., et al,  "Water Atlas of the United
    States," Port Washington, New York, Water Information
    Center, Inc., 1973.

 6.  Connecticut Interagency  Water Resources Planning  Board,
    "Statewide Long-Range Plan for the Management of  the
    Water Resources of  Connecticut," Office of State  Plan-
    ning, Connecticut Department of Finances and Control,
    1971.

 7.  Geraghty & Miller,  Inc., "Availability of Water Re-
    sources in the  Midstate  Region of Connecticut," 1965.

 8.  Cushman, R. V., "Ground-Water Resources of North  Cen-
    tral Connecticut,"  U. S. Geological  Survey Water-Supply
    Paper  1752, 1964.

 9.  Cervione,  M. A.,  D. L. Mazzaferro, and R. L.  Melvin,
     "Water  Resources  Inventory of Connecticut, Part 6,  Up-
    per Housatonic  River  Basin," Connecticut Department of
    Environmental Protection, Water Resources Bulletin  No.
    21, 1972.

10.  U.  S.  Geological  Survey, North Atlantic Regional  Water
    Resources  Study,  "Appendix D:  Geology  and Ground Wa-
    ter," North Atlantic  Regional Water  Resources Study
    Coordinating  Committee,  1972.


                             69

-------
 11.   Randall, A.  D.,  et  al,  "Water  Resources  Inventory of
      Connecticut,  Part 1, Quinebaug River Basin," Connecti-
      cut Water  Resources Commission, Water Resources Bulle-
      tin No.  8,  1966.

 12.   Marine,  I. W., and  W. C. Rasmussen, "Preliminary Report
      on the Geology and  Ground-Water Resources of Delaware,"
      Delaware Geological Survey Bulletin No.  4, 1955.

 13.   Kraft, J.  C., and M. D. Maisano,  "A Geologic Cross Sec-
      tion of Delaware,"  University  of  Delaware Water Re-
      sources Center,  1968.

 14.   Gushing, E. M.,  I.  H. Kantrowitz, and K. R. Taylor,
      "Water Resources of the Delmarva  Peninsula," U. S. Geo-
      logical Survey Professional Paper 822, 1973.

 15.   Prescott, G. C., Jr., "Reconnaissance of Ground-Water
      Conditions in Maine," U. S. Geological Survey Water-
      Supply Paper 1669-T, 1963.

 16.   Prescott, G. C., Jr., "Lower Aroostook River Basin Area,"
      Maine Public Utilities Commission Basic-Data Report No.
      5, Ground-Water Series, 1970.

 17.   Prescott, G. C., Jr., "Meduxnekeag River-Prestile
      Stream Basins Area," Maine Public Utilities Commission
      Basic-Data Report No. 7, Ground-Water Series, 1971.

 18.   Prescott, G. C., Jr., "Lower Kennebec River Basin Area,"
     Maine Public Utilities Commission Basic-Data Report No.
      4, Ground-Water Series, 1968.

 19.   Prescott, G. C., Jr., "Lower Penobscot Basin Area,"
     Maine Public Utilities Commission Basic-Data Report No.
      2, Ground-Water Series, 1964.

 20.   Prescott, G. C., Jr., "Lower Androscoggin River Basin
     Area," Maine Public Utilities Commission Basic-Data Re-
     port No. 3, Ground-Water Series,  1967.

 21.  Prescott, G. C., Jr., and J.  A. Drake,  "Southwestern
     Area," Maine Public Utilities Commission Basic-Data Re-
     port No. 1, Ground-Water Series,  1962.

22.-  Cleaves, E. T., Jonathan Edwards,  Jr.,  and J. D.  Glaser,
     "Geologic Map of Maryland," Maryland Geological Survey,
     1968.
                             70

-------
23.   Cleaves,  E.  T.,  "Piedmont and Coastal Plain Geology
     Along the Susquehanna Aqueduct,  Baltimore to Aberdeen,
     Maryland," Maryland Geological Survey, Report of In-
     vestigation 8,  1968.

24.   Otton, E. G., "Geologic and Hydrologic Factors Bearing
     on Subsurface Storage of Liquid Wastes in Maryland,"
     Maryland Geological Survey, Report of Investigation 14,
     1970.

25.   Myer, Gerald, "The Water Resources of Carroll and Fred-
     erick Counties,  Maryland," Maryland Department of Geol-
     ogy,  Mines and Water Resources,  Bulletin 22, 1958.

26.   Glaser, J. D.,  "Coastal Plain Geology of Southern Mary-
     land," Maryland Geological Survey, Guidebook No. 1,
     1968.

27.   U. S. Geological Survey, "The National Atlas of the
     United States of America," U. S. Department of the In-
     terior, 1970.

28.   Petersen, R. G., "Ground Water Favorability Map of the
     Westfield River Basin, Massachusetts," Massachusetts
     Water Resources Commission, 1964.

29.   Massachusetts Water Resources Commission, "Special Re-
     port of the Water Resources Commission Relative to the
     Water Supply of Berkshire County," Legislative Report
     House No. 5170, January 1967.

30.   Pollock, S. J., D. F. Farrell, and W. W. Caswell, "Wa-
     ter Resources of the Assabet River Basin, Central
     Massachusetts," U. S. Geological Survey Hydrologic In-
     vestigations Atlas HA-312, 1969.

31.   Baker, J. A., and R. G. Petersen, "Lowell Area," Massa-
     chusetts Department of Public Works Basic-Data Report
     No. 3, Ground-Water Series, 1962.

32.   Sammel, E. A., J. A. Baker, and R. A. Brackley, "Water
     Resources of the Ipswich River Basin, Massachusetts,"
     U. S. Geological Survey Water-Supply Paper 1826, 1966.

33.   Wiesnet, D. R., and W. B. Fleck, "Millers River Basin,"
     Massachusetts Metropolitan District Commission Basic-
     Data Report No. 11, Ground-Water Series, 1967.
                             71

-------
34.  Petersen, R. G.,  "Generalized Surficial Geology Ground
     Water Favorability Map of the Ware-Quaboag-Quinebaug-
     French River Basins, Massachusetts," Massachusetts Water
     Resources Commission, Hydrologic Investigations Chart
     HI-2, 1962.

35.  Sammel, E. A., "Water Resources of the Parker and Rowley
     River Basins, Massachusetts," U. S. Geological Survey
     Hydrologic Investigations Atlas HA-247, 1967.

36.  Williams, J. R. , and R. E. Willey, "Taunton River Ba-
     sin," Massachusetts Water Resources Commission Basic-
     Data Report No. 12, Ground-Water Series, 1970.

37.  Kammerer, J. C., and H. L. Baldwin, "Water Problems in
     the Springfield-Holyoke Area, Massachusetts," U. S. Geo-
     logical Survey Water-Supply Paper 1670, 1962.

38.  Norvitch, R. F., and M. E. S. Lamb, "Housatonic River
     Basin," Massachusetts Water Resources Commission Basic-
     Data Report No. 9, Ground-Water Series, 1966.

39.  Stewart,  G.  W., and Carole Ouelette,  "Progress Report:
     Rock Well Survey in New Hampshire," New Hampshire De-
     partment of Resources and Economic Development, Divi-
     sion of Economic Development, 1964.

40.  Bradley,  Edward,  and R. G. Petersen,  "Southeastern Area,"
     New Hampshire Water Resources Board Basic-Data Report
     No. 1,  Ground-Water Series,  1962.

41.  Weigle,  J. M., and Richard Kranes,  "Lower Merrimack
     River Valley," New Hampshire Water Resources Board
     Basic-Data Report No. 2,  Ground-Water Series, 1966.

42.  Goldthwait,  J. W., Lawrence Goldthwait, and R. P. Gold-
     thwait,  "The Geology of New Hampshire,  Part 1 - Surfi-
     cial Geology," New Hampshire State Planning and Devel-
     opment Commission, 1951.

43.  Lewis,  J. V., and H. B. Kummel,  "Geologic Map of New
     Jersey,"  New Jersey Department of  Conservation and
     Economic  Development, Atlas Sheet  No.  40, 1950.

44.  Banino,  G. M., F. J. Markewicz,  and J.  W. Miller, Jr., .
     "Geologic, Hydrologic,  and Well  Drilling Characteris-
     tics of the  Rocks of Northern and  Central New Jersey,"
     New Jersey Bureau of Geology and Topography, 1970.
                             72

-------
45.   Richards,  H.  G.,  F.  H.  Olmstead,  and J.  L.  Ruhle,  "Gen-
     eralized Structure Contour Maps  of the New  Jersey
     Coastal Plain," New Jersey Geological Survey,  Geologic
     Report Series No. 4, 1966.

46.   Heath, R.  C., "Ground Water in New York," State  of New
     York Conservation Department,  Water Resources  Commis-
     sion Bulletin GW-51, 1964.

47.   Reck, C. W.,  and  E.  T.  Simmons,  "Water Resources of the
     Buffalo-Niagara Falls Region," U. S. Geological  Survey
     Circular 173, 1952.

48.   Perlmutter,  N. M., "Geology and  Ground-Water Resources
     of Rockland County,  New York," State of  New York Depart-
     ment of Conservation, Water Power and Control Commis-
     sion Bulletin GW-42, 1959.

49.   Giese, G. L., and W. A. Hobba, Jr., "Water  Resources of
     the Champlain-Upper Hudson Basins in New York State,"
     New York State Office of Planning Coordination,  1970.

50.   Arnow, Theodore,  "The Ground-Water Resources of Fulton
     County, New York," State of New  York Department of Con-
     servation, Water  Power and Control Commission Bulletin
     GW-24, 1951.

51.   Heath, R. C., F.  K. Mack, and J. A. Tannenbaum, "Ground
     Water Studies in  Saratoga County, New York," State of
     New York Department of Conservation, Water Resources
     Commission Bulletin GW-49, 1963.

52.   Simmons, E. T.,  I. G. Grossman,  and R.  C. Heath,
     "Ground-Water Resources ofJ utchess County, New York,"
     State of New York Department of  Conservation, Water
     Resources Commission Bulletin GW-43, 1961.

53.   Grossman, I. G.,  "Ground-Water Resources of Putnam
     County, New York," State of New York Department of Con-
     servation, Water Power and Control Commission Bulletin
     GW-37, 1957.

54.   Carman, S. P., "Preliminary Report:  Water Supply Prob-
     lems, Westchester County," Westchester County Water
     Agency, 1955.

55.   Grossman, I. G.,  and L. B. Yarger,  "Water Resources of
     the Rochester Area, New York," U. S. Geological Survey
     Circular  246, 1953.
                             73

-------
 56.  Kantrowitz,  I.  H.,  "Ground-Water Resources in the East-
     ern Oswego River Basin, New York," State of New York
     Conservation Department, Water Resources Commission Ba-
     sin Planning Report ORB-2, 1970.

 57.  Mack, F. K., and R. E. Digman, "The Ground-Water Re-
     sources of Ontario County, New York," State of New York
     Department of Conservation, Water Resources Commission
     Bulletin GW-48, 1962.

 58.  Arnow, Theodore, "The Ground-Water Resources of Colum-
     bia County,  New York," State of New York Department of
     Conservation, Water Power and Control Commission Bulle-
     tin GW-25, 1951.

 59.  Soren, Julian,  "The Ground-Water Resources of Sullivan
     County, New  York," State of New York Department of Con-
     servation, Water Resources Commission Bulletin GW-46,
     1961.

 60.  Grain, L. J., "Ground-Water Resources of the Jamestown
     Area, New York," State of New York Department of Con-
     servation, Water Resources Commission Bulletin 58, 1966.

 61.  Cohen, Philip, 0. L. Franke, and B. L. Foxworthy, "At-
     las of Long  Island's Water Resources," State of New
     York Water Resources Commission Bulletin 62, 1968.

 62.  Willard,  Bradford,  "Pennsylvania Geology Summarized,"
     Pennsylvania Topographic and Geologic Survey Educa-
     tional Series No. 4, 1970.

 63.  Emrich, G. H., "Ground-Water Geology," Pennsylvania De-
     partment of Health, Division of Sanitary Engineering,
     Publication No.  11, 1966.

 64.  Lohman, S. W., "Ground-Water Resources of Pennsylvania,"
     Pennsylvania Topographic and Geologic Survey Bulletin
     W-7, 1941.

 65.  Chester County Planning Commission, "Chester County
     Natural Environment and Planning:   Landforms,  Geology,
     Soils, Woodlands, and Climate," Chester County Planning
     Commission, 1963.

66.  Briesecker, J. E.,  J.  B. Lescinsky, and C.  R.  Wood,
     "Water Resources of the Schuylkill River Basin,"  Penn-
     sylvania Department of Forests and Waters,  Water  Re-
     sources Bulletin No. 3, 1968.
                            74

-------
67.  Parizek,  R.  R.,  W.  F.  White,  Jr.,  and Donald Langmuir,
     "Hydrogeology and Geochemistry of  Folded and Faulted
     Rocks of  the Central Appalachian Type and Related Land
     Use Problems,"  Pennsylvania State  University Earth and
     Mineral Sciences Experiment Station Circular 82,  1971.

68.  Piper, A. M., "Ground Water in Southwestern Pennsyl-
     vania," Pennsylvania Department of Internal Affairs,
     Topographic and Geologic Survey Bulletin W-l, 1933.

69.  Rima, D.  R., "Ground-Water Resources of the Lansdale
     Area, Pennsylvania," Pennsylvania  Department of Inter-
     nal Affairs, Topographic and Geologic Survey Progress
     Report 146,  1955.

70.  Lohman, S. W.,  "Ground Water in South-Central Pennsyl-
     vania," Pennsylvania Department of Internal Affairs,
     Topographic and Geologic Survey Bulletin W-5, 1938.

71.  Mangan, J. W.,  D. W. Van Tuyl, and W. F. White, Jr.,
     "Water Resources of the Lake Erie  Shore Region in Penn-
     sylvania," U. S. Geological Survey Circular  174, 1952.

72.  Adamson,  J. H., J. B. Graham, and N. H. Klein, "Ground-
     Water Resources of the Valley Fill Deposits  of Alle-
     gheny County, Pennsylvania," Pennsylvania Department of
     Internal Affairs, Topographic and Geologic Survey
     Bulletin W-8, 1949.

73.  Greenman, D. W., et al, "Ground-Water Resources of the
     Coastal Plain Area of Southeastern Pennsylvania,"
     Pennsylvania Department of Internal Affairs, Topographic
     and Geologic Survey Bulletin W-13, 1961.

74.  Graham, J. B., J. W. Mangan, and W. F. White, Jr.,  "Wa-
     ter Resources of Southeastern Bucks County,  Pennsyl-
     vania," U. S. Geological Survey Circular 104, 1951.

75.  Quinn, A. W., "Bedrock Geology of Rhode  Island," U. S.
     Geological Survey Bulletin 1295,  1971.

76.  Allen, W. B., "The Ground-Water Resources  of Rhode Is-
     land, A Reconnaissance," Rhode  Island Development
     Council,  Geological Bulletin No.  6,  1953.

77.  Bierschenk,  W. A.,  "Ground-Water  Resources  of the  Prov-
     idence Quadrangle, Rhode Island," Rhode  Island Water
     Resources Coordinating Board, Geological Bulletin  No.
     10,  1959.
                            75

-------
 78.   Hansen,  A.  J.,  and G.  R.  Schiner,  "Ground-Water  Re-
      sources  of  Block Island,  Rhode Island,"  Rhode  Island
      Water Resources Coordinating Board,  Geological Bulle-
      tin No.  14, 1964.

 79.   Jacobs,  E.  C.,  "The Physical Features  of Vermont,"
      Vermont  State Development Commission,  1950.

 80.   Stewart,  D. P., "Geology  for Environmental Planning in
      the Rutland-Brandon Region,  Vermont,"  Vermont  Water Re-
      sources  Department,  Environmental  Geology No.  2, 1972.

 81.   Hodges,  A.  L.,  Jr.,  and David Butterfield, "Ground-Wa-
      ter Favorability Map of the  Lamoille River Basin, Ver-
      mont," Vermont  Department of Water Resources,  1967.

 82.   Hodges,  A.  L.,  Jr.,  and David Butterfield, "Ground-Wa-
      ter Favorability Map of the  Missisquoi River Basin,
      Vermont  Department  of Water  Resources, 1967.

 83.   Hodges, A.  L.,  Jr.,  "Ground-Water  Favorability Map of
      the Otter Creek Basin, Vermont," Vermont Department of
      Water Resources, 1967.

 84.   Hodges, A.  L.,  Jr.,  and David Butterfield, "Ground-Wa-
      ter Favorability Map of the  West-Deerfield River Basin,
      Vermont," Vermont Department of Water Resources, 1968.

 85.   Hodges, A.  L.,  Jr.,  and David  Butterfield, "Ground-Wa-
      ter  Favorability Map of the  Ottauquechee-Saxtons River
      Basin, Vermont," Vermont Department  of Water Resources,
      1968.

 86.   Hodges, A.  L.,  Jr., and David  Butterfield, "Ground-Wa-
      ter  Favorability Map of the  White  River  Basin, Vermont,"
     Vermont Department of Water  Resources, 1968.

 87.  Hodges, A.  L.,  Jr., and David  Butterfield, "Ground-Wa-
      ter  Favorability Map of the Wells-Ompompanoosuc River
     Basin, Vermont," Vermont Department of Water Resources,
     1968.

 88.  Hodges, A.  L.,   Jr., and David Butterfield, "Ground-Wa-
     ter Favorability Map of the Nulhegan-Passumpsic River
     Basin, Vermont," Vermont Department of Water  Resources
     1967.

89.  Hodges, A. L.,  Jr., and David Butterfield, "Ground-Wa-
     ter Favorability Map of the Winooski River Basin, Ver-
     mont," Vermont Department of Water Resources,  1967.

                            76

-------
90.   Hodges,  A.  L.,  Jr.,  and David Butterfield,  "Ground-Wa-
     ter Favorability Map of the Lake Memphremagog Basin,
     Vermont," Vermont Department of Water Resources,  1967.

91.   Hodges,  A.  L.,  Jr.,  "Ground-Water Favorability Map of
     the Batten  Kill, Walloomsac River and Hoosic River Ba-
     sins," Vermont  Department of Water Resources, 1966.
                            77

-------
                          SECTION V

                 NATURAL GROUND-WATER QUALITY
 INTRODUCTION

 The natural quality of ground water is not considered by
 users in the region to be a problem unless the recommended
 limits for chemical concentrations of selected constituents
 as set by the states for potable public water supplies are
 exceeded.   For the most part,  the allowable chemical limits
 for the 11 northeast states are similar to those  of the U.S.
 Public Health Service.  D   Ground water which contains con-
 stituents  exceeding state health department or U.  S.  Public
 Health Service recommended limits of chemical concentrations
 occur to some extent throughout the study  area.   Although it
 is recognized that certain industrial processes require ex-
 tremely polished water,  these  are the exceptions,  and ground
 water found in the northeast is suitable in quality for most
 purposes with little or  no treatment.

 Other than the natural occurrence of saline waters in aqui-
 fers and pollutants resulting  from man's activities,  the
 chemicals  found in ground water result from the interaction
 of water with rock materials.   Natural ground-water quality
 is intimately related to the solubility of the minerals in
 the rocks  through  which  the water moves.   The chemical char-
 acter of ground water can be associated with a particular
 rock type.   Where  the rocks are similar in mineralogy over
 broad areas,  the chemical  character of the water  is gener-
 ally consistent.   Where  localized occurrences of  soluble,
 atypical mineral suites  are present,  the chemical  quality of
 local ground water reflects these minerals.

 Since ground water is not  static,  but  constantly  in motion,
 there often is  a change  in quality as  water moves  within the
 aquifer, and from  one rock type to another.   The  capability
 of an aquifer to circulate water has  a distinct influence  on
 the  mineral content.  In the highly permeable but  areally-
 limited  glacial aquifers,  circulation  is rapid and water
 quality  is  generally good.   In  some Coastal  Plain  deposits,
 water  can migrate  many miles from the  intake area  to  the dis-
 charge area,  and generally increases  in mineral content  due
 to  the very long travel  time associated with such  a migra-
 tion.  Changes  in  relative composition may also occur,  such
 as the softening that takes  place  during movement  through
 greensands.

Consolidated  rock  aquifers  are  extremely variable  in  their

                             78

-------
circulation capability.  Generally, these aquifers have only
limited circulation below depths of 500 feet.  Below this
depth/ water can be highly mineralized, with high chloride
and total dissolved solids the primary objectionable constit-
uents.  Figure 18 is a map of the 11-state study area show-
ing the depth to mineralized ground water in the major aqui-
fers.  Fortunately, saline-water aquifers are normally over-
lain by fresh-water aquifers.  Although the remaining por-
tion of the region is shown to be less than 1,000 mg/1,
(milligrams per litre), there may be some localized areas
where mineralized water occurs at depth.  However, because
there is no need to drill deep wells for fresh-water sup-
plies at these locations, little or no information is avail-
able on the quality of water below the fresh-water zones.

By far the most widespread problem in the northeast region
is the naturally high iron content of ground water  (often
associated with a high concentration of manganese), low pH,
and sometimes high hardness.  This problem is not confined
to any region or aquifer type, but occurs in the three major
water-yielding units:  the unconsolidated deposits of the
Coastal Plain, the unconsolidated glacial deposits, and the
consolidated rocks.

Individual domestic wells, even when they yield water high
in iron content, rarely are equipped with treatment facili-
ties.  However, many municipal and industrial supplies must
be treated for iron and manganese, or the pH must be ad-
justed and the hardness reduced.  Some supplies must be
treated for more than one of the above parameters.

Following is a state-by-state discussion of natural water
quality.  Tables have been prepared for each state, and they
present information on natural water quality in the prin-
cipal aquifers.  In some cases it was not possible  from the
reported data to determine whether the occurrence of high
concentrations of certain mineral constituents in specific
wells is actually natural or has been caused by man's activ-
ities.  Therefore, median values have been computed and are
probably the most representative of natural water quality
conditions.

CONNECTICUT

The natural quality of the ground water in Connecticut is ex-
tremely variable among aquifers and within relatively short
distances in the same  aquifer.  The concentrations  of many
constituents have wide ranges which may impose some con-
straints on the industrial utilization of water,  especially
where extremely high-quality process water is required.
                              79

-------
                                NORTH
                                                  DEPTH BELOW LAND SURFACE TO SHALLOWEST
                                                  ZONE OF GROUND WATER CONTAINING MORE THAN
                                                  1,000 MG/LOF DISSOLVED SOLIDS.
                                               |     I   LESS THAN 500 FEET

                                                        500- 1,000 FEET

                                                        GREATER THAN 1,000 FEET

                                                        LESS THAN 1,000 MG/L (NO WELLS
                                                        KNOWN TO PRODUCE MINERALIZED
                                                        WATER IN QUANTITIES GREATER THAN
                                                        0.01 MOD)
Figure 18.  Depth to mineralized ground water in major aquifers in the  northeast
                                      United States 2)
                                        80

-------
Table 11 is the compilation of chemical analyses from the
various aquifers, taken from several published sources in-
cluding regional and river basin reports.  A wide range of
concentrations exists throughout the regions of the state
for almost all of the constituents.  Many of the upper val-
ues far exceed recommended limits of drinking water stand-
ards.  However, where more than three analyses are tabulated,
only rarely does the median value exceed these limits.  The
median manganese value of six analyses in the south-central
sand and gravel deposits is above the recommended limit.
Based on analyses of 96 water samples from wells tapping the
crystalline rocks in the southeastern coastal region of Con-
necticut, 27 percent contained iron concentrations equal to
or exceeding the State Health Department limits.  Of 89 well
samples, 31 percent contained objectionable manganese con-
centrations.  Approximately 50 to 75 percent of the wells
tapping the bedrock  (schist) in eastern Connecticut yield
water that would require treatment for iron and manganese. 4)

Naturally-occurring salt water in aquifers along the coast
and estuaries has not been studied in great detail.  However,
it is known to be present in some areas of the coastal re-
gion and also in areas several miles inland along estuaries,
particularly in less permeable unconsolidated deposits where
flushing by fresh water has been incomplete.

The occurrence of high concentrations of sulfate has been
noted in some ground-water supplies, generally limited to
the sedimentary rocks of the central portion of the state.
However, only two public-supply systems using ground water
have average concentrations exceeding the state standard.

The average concentrations of chemical constituents over a
five year period  (1966 through 1970) from all the individual
sources for public supply indicate that the water is of good
quality.  Table 12 lists the maximum concentrations of  se-
lected constituents for drinking water allowed by the state
and the number of public supply wells and springs where the
average concentration over a five-year period was equal to
or exceeded the limits.  As can be seen, the major natural
water-quality problem is iron concentration.  It should be
noted that many of the excessive concentrations, particularly
iron, manganese, color, and turbidity, were found in the
same water sources.  The natural chloride content found in
water throughout the state is low, rarely exceeding 20 mg/1,
except in some locales along coastal areas  and  estuaries.

DELAWARE

The natural ground water of Delaware is  generally of  suitable
                              81

-------
                   Table 11. CHEMICAL ANALYSES OF GROUND WATER IN CONNECTICUT.  (Concentrations in milligrams per liter.
                                                                                                                              3 through 13)
CD
to


Location
Northeast


Southeast


North Central



South Central



Northwest


Southwest



Rock
Type
X
S/G
T
X
S/G
T
X
Tr
S/G
T
X
Tr
S/G
T
X
C
S/G
X
S/G
T

N
104
34
14
98
51
7
20
35
79
2
3
5
6
2
76
27
29
58
18
3
Iron (Fe)

Range
0.00 -4.8
0.00 -2.8
0.00-0.49
0.00-8.2
0.01 -2.3
0.02 -8.1
0.02 -3.6
0.00 - 1.5
0.01 -0.32
0.84 -2.0
0.02 -0.20
0.01 -0.19
0.02 -0.16
0.03-0.19
0.00- 1.0
0.00 -3.4
0.00-2.1
0.01 -8.6
0.01 -0.84
0.04-0.48


M
0.07
0.06
0.09
0.10
0.10
0.14
0.28
0.15
0.10
-
_
0.10
0.06
-
0.09
0.06
0.06
0.14
0.06
-

N
105
33
12
91
49
7
19
15
68
2
3
5
6
2
76
27
29
58
18
3
Manganese (Mn)

Range
0.00-0.94
0.00-5.7
0.00-0.10
0.00 - 0.94
0.00-0.78
0.00-0.27
0.00 - 0.25
0.00-0.12
0.00 -9.9
0.02 - 0.08
0.03-0.20
0.02-0.18
0.02-0.29
0.07-0.22
0.00 - 0.65
0.00-0.23
0.00-0.59
0.00 - 0.66
0.00 - 0.24
0.01 -0.17


M
0.00
0.01
0.00
0.02
0.02
0.01
0.03
0.01
0.03
—
-
0.04
0.11
-
0.02
0.01
0.04
0.03
0.03
-

N
68
34
12
44
38
2
20
28
64
2
4
5
9
3
76
27
29
58
18
3
SulFate

(S04)

Range
2.4
0.2
6.9
1.6
1.2
30
6.4
3
2.3
7.2
7.1
9.1
15
12
3.2
8
7.2
8.9
12
52
39
- 37
26
- 1,040
- 109
41
- 39
- 1,500
- 292
21
22
35
- 83
16
- 178
74
- 178
72
39
- 274


M
13
12
13
17
17
-
14
27
26
-
_
29
27
-
19
23
23
20
19
-
                    X  - Crystalline rocks
                    T  - Till
                  S/G  - Sand and gravel
                    Tr — Sedimentary rocks
                    C  - Carbonate rocks
N - Number of samples
M - Median

-------
                                       Table 11 (continued).  CHEMICAL ANALYSES OF GROUND WATER IN CONNECTICUT.
                                                           (Concentrations in milligrams per liter.)  3 ^rou9h 13)
                                                                        Chloride (CI)
Nitrate
CO
co

Location
Northeast


Southeast


North Central



South Central



Northwest


Southwest


Rock
Type
X
S/G
T
X
S/G
T
X
Tr
S/G
T
X
Tr
S/G
T
X
c
S/G
X
S/G
T

N
27
15
2
51
58
5
22
54
82
2
4
5
9
3
76
27
29
58
18
3

Range
2.0 -
2.8-
3.2-
0 -
4.0-
5.3 -
0.4-
0.6- 1,
0 -
1.5-
1.5 -
3.0-
3.2-
1.5-
0.8-
0.9-
0.3 -
2.6-
2.0-
350 - 1,


70
84
14
362
607
16
10
029
48
3.5
3.0
22
70
3.6
78
72
92
140
37
700

M
6.5
7.1
-
13
17
9.0
2.7
5.3
4.6
-
_
9.0
9.5
—
5.4
8.0
8.0
9.6
12
~

N
100
30
12
22
18
4
22
45
79
2
_
-
1
-
76
27
29
58
21
3


0
0
0
0
0
0
0
0
0
0


60

0
0
0
0
0
0

Range
-60
-44
.3 -26
.1-32
.3-43
-52
-24
-20
-86
.5
_
-

-
- 39
- 16
-25
-40
-34
- 1.4

M
0.9
2.9
8.3
3.7
3.2
-
0 .45
0.71
5.7
-
-
-
-
—
0.6
4.6
1.0
0.3
2.2
"•

-------
                    Table  11 (continued). CHEMICAL ANALYSES OF GROUND WATER IN CONNECTICUT. (Concentrations in milligrams per liter.)
                                                                      3 through 13)
00


Location
Northeast


Southeast


North Central



South Central



Northwest


Southwest


Total
Rock
Type
X
S/G
T
X
S/G
T
X
Tr
S/G
T
X
Tr
S/G
T
X
C
S/G
X
S/G
T

N
97
34
13
97
51
8
21
42
73
2
3
5
6
2
76
27
29
58
18
3
Dissolved Solids

Range
24 - 409
31 - 330
79 - 434
24- 1,830
36 - 1,270
40 - 678
42 - 184
43 -2,510
30 - 821
44 - 58
39 - 145
89 - 212
86 - 233
56 - 67
34 - 404
84 - 496
60 - 513
52 - 354
71 - 225
718 -3,300
Total

M
100
80
108
118
96
82
111
161
132
-
_
157
131
-
136
275
237
124
112
—

N
100
35
12
97
51
8
22
52
78
2
4
5
9
3
76
27
29
58
18
3
Hardness (as CaCO^)


7
9
38
3
2
22
21
14
6
22
20
28
40
30
15
76
36
30
21
99

Range
- 279
- 108
- 211
- 1,120
- 296
- 100
- 132
-2,500
- 486
- 26
- Ill
- 143
- 266
40
- 264
- 378
- 365
- 266
- 188
- 777

M
54
37
50
57
42
36
61
110
64
-
_
83
103
-
85
230
190
73
53
-

N
104
35
14
97
51
8
22
42
80
2
4
5
8
3
76
27
29
58
18
3
PH

Range
5.1 -8.6
4.8 -9.3
5.8 -7.7
4.4 -8.1
5.8 -7.7
5.0 -7.3
6.3 -8.2
5.7-8.9
5.0 -8.3
6.1 -6.5
6.3 -7.4
6.5 -8.7
6.4 -7.8
6.4 -6.9
6.4 -7.9
7.1 -8.1
6.7-8,1
5.7-8.2
6.4 -7.7
6.9 -7.1


M
7.0
6.5
6.6
7.2
6.9
7.0
7.1
7.4
6.8
-
_
7.7
6.8
-
7.4
7.7
7.7
7.5
6.9
—

-------
Table 12. NUMBER OF GROUND-WATER SOURCES USED FOR PUBLIC SUPPLY
         EQUAL TO OR EXCEEDING STATE OF CONNECTICUT DRINKING
             WATER STANDARDS FOR SELECTED CONSTITUENTS.
                            Maximum
                            concentrations
Number of public wafer-
supply sources yielding
ground water equal to or
Constituent
Chloride (Cl)
Total Hardness (as CaCO3)
Iron (Fe)
Manganese (Mn)
Sodium (Na)
Sulfate (SO4)
Fluoride (F)
Turbidity
Color (true)
allowed
250 a)
150 a)
0.3 a>
0.05 a)
20 a)
250 a)
1.2
5 units
15 units
exceeding standard
3
86
115
85
71
2
6
43
10
a) These limits should not be exceeded if better quality water can be made
   available.
                                  85

-------
 quality for most purposes, with only minor treatment re-
 quired in isolated instances.   Table 13 is a compilation of
 chemical analyses of selected constituents in natural ground
 waters.  Usually the water from the shallow zones is of bet-
 ter quality than that obtained from the deep zones.   Little
 is known about the quality of water at depths of 1,000 feet
 or greater, but it is inferred that these waters would be
 high in dissolved solids.

 There is little information available on the water quality
 in the Unglaciated Appalachians.   Waters from the carbonate
 rocks have a higher hardness than from the other crystalline
 rock types.  Normally,  the calcium and magnesium content is
 higher in water from the basic crystalline rocks, such as
 gabbro, than from the acidic rocks.   Occasionally, high iron
 content is encountered  locally in concentrations that may
 require treatment.

 The natural water quality  of the  Coastal Plain deposits is
 good and,  with  the  exception of spotty high iron content,
 little or no treatment  is  required for most purposes.   Brack-
 ish or salty water  can  be  found in portions of nearly all of
 the aquifers.   The  locations of the  salt-water interface
 have been fairly  well documented  and mapped.

 The ground water  from Quaternary  age aquifers  is character-
 istically slightly  acidic, with a pH of around 6.  The iron
 content is  often  troublesome,  requiring some  form of treat-
 ment.   The  water  is usually  soft,  and contains low concentra-
 tions  of  total  dissolved solids.  15)

 The Tertiary sediments  of Miocene age yield water with a pH
 above  7 and low dissolved  iron  content.  The bicarbonate and
 silicate  concentrations are  higher than  other  aquifers  in
 the region.   The  underlying  deposits  of  Eocene and Paleocene
 age have  water  with a wide range  of  pH values,  and occasion-
 ally high iron  content.  Moderately  high dissolved solids
 and hardness  are  found.

The  Upper  Cretaceous marine  sediments  are not  extensively
tapped  in  the state.  Pew  chemical analyses of the water are
available,  but  indications are  that  the  quality  is very  good.
Chemical  analyses of water from the Magothy formation  show
both basic  and  acidic pH values.  The  basic waters  are  typi-
cally found  at  depth and downdip.  Total iron  and  sulfate
concentrations  are relatively high.   Water  from  the Lower
Cretaceous basal  unit is similar  to  the Magothy  formation.
                            86

-------
                    Table 13.  CHEMICAL ANALYSES OF GROUND WATER IN DELAWARE.  (Concentrations in  milligrams per liter.)  15 trough 23)
CO
-o


Locotion - Age
Piedmont Province
Precambrian
Coastal Plain
Cretaceous


Tertiary

Quaternary

Rock
Type

X

Nm
Mt
Ma
Pe
Mio
PI

N

9

68
4
9
2
16
117


Iron


-------
00
CO
               Table 13 (continued). CHEMICAL ANALYSES OF GROUND WATER IN DELAWARE.  (Concentrations in milligrams per liter.)

                                                      Total Dissolved Solids          Total Hardness (as CaCC^)                 pH
                                                                                                                                    15 through 23)
Location - Age
Piedmont Province
Precambrian
Coastal Plain
Cretaceous
Tertiary
Quaternary
Rock
Type
X
Nm
Mt
Ma
Pe
Mio
PI
N
3
23
4
1
10
20
Range
35 -
33-
50-
152
100 - 1,
177 -
34-1,
M
353
350 86
64
000
248 208
280 84
N
11
75
8
9
31
149

32
5
18
6
15
6.
1.
Range
- 158
- 245
- 44
- 162
- 200
6 -1,500
7-2,320
M
60
34
23
87
101
32
N
17
87
8
9
30
107
Range
5.0 -7.4
5.4-7.6
5.9 - 7.2
5.5-7.9
5.6 -8.6
4.9-8.3
3.4 -7.5
M
6.3
6.6
6.7
6.2
6.6
6.2
Chloride (Cl)
Nitrate (NO3)
Location - Age
Piedmont Province
Precambrian
Coastal Plain
Cretaceous
Tertiary
Quaternary
Rock
Type
X
Nm
Mt
Ma
Pe
Mio
PI
N
14
83
9
9
31
100
Range
5.5-
1.5-
1.5-
3.5-
1 -
1.5-4,
4 -6,

550
218
16
82
200
000
300
M
9.3
6.5
3.0
28
11
13
N
4
33
6
8
20
96

7
0
0
0
0
0
0
Range
.6 - 20
- 24
.6
.2 - 68
.1-30
- 29
- 120
M
_
0.6
0.3
37
0.1
9,25

-------
MAINE

Except for the common problems caused by high iron and man-
ganese, and high hardness of water from carbonate rocks,
Maine has natural ground water of excellent quality.  How-
ever, it does have local water-quality problems that are un-
usual.  Table 14 is a compilation of chemical analyses of
selected constituents in natural ground waters.

In two areas of the state, one in the Central Uplands and
one in the Coastal Lowlands, the ground water shows levels
of radioactivity considerably higher than usual.  The source
of this activity is believed to be radioactive minerals
present in the pegmatites found in these areas.

In the Coastal Lowlands, it is not uncommon for a well to
produce water with high total dissolved solids and chloride
concentrations.  Sea water entered aquifers in the coastal
area when they were submerged between periods of Pleistocene
glaciation.  Many of these aquifers have not been completely
flushed by circulating fresh ground water since that time.

MARYLAND

Natural ground water in Maryland is generally of good qual-
ity, with exceptions in localized areas.  Table 15 is a com-
pilation of chemical analyses of selected constituents in
natural ground waters.

Although saline waters can be found in the deeper Coastal
Plain formations, the overlying aquifers contain an abun-
dance of fresh water which is available for development for
most purposes with little or no treatment required.  Gener-
ally, mineralized water can be found below depths of 500
feet in the consolidated rock aquifers.

In the consolidated rock aquifers west of the Fall Line, the
water quality is greatly dependent on the chemical nature of
the aquifer material.  For example, the water from the crys-
talline rocks is usually softer and has a lower pH than wa-
ter obtained from the carbonate rocks.  Although a wide
range of dissolved solids is found in water from wells tap-
ping the crystallines, the highest concentrations are in
waters from the carbonates.  High iron concentrations of wa-
ter from both types of rocks are fairly localized problems.
Not much data are available on the natural water quality of
the aquifers in the sedimentary rocks  in the western portion
of the state.  In many places saline water can be found be-
low a depth of 500 feet, although some deeper wells report-
edly yield potable water supplies.
                              89

-------
 Table 14.  CHEMICAL ANALYSES OF GROUND WATER IN MAINE.  (Concentrations
                       in milligrams per liter.) 24 trough 30)

                                                               Total Hardness

Rock
Type
C
U

N
19
17
Iron (Fe)

Range
0 -1.3
0 - 1.5


M
0.02
0.05

N
19
26
Chloride (Cl)

Range
2.2 -36
0.2 -22


M
11
6.1

N
16
13
(as CaCOs


Range
20 - 281
5-225
)


M
197
61
Total Dissolved Solids
Rock
Type
C
U

N Range M
14 41 -355 153
20 2 - 230 58

N
17
19
PH

Range
6.6 -8.1
5.7-8.4


M
7.3
6.9
C  - Consolidated rock
U  -  Unconsolidated deposits
N  -  Number of samples
M  - Median
                                   90

-------
      Table 15.  CHEMICAL ANALYSES OF GROUND WATER IN MARYLAND. (Concentrations in milligrams per liter.)
                                               31 through 36)
vo
Rock
Location Type N
Central Maryland X 53
Central Maryland C$ 7
Coastal Plain U 105
Iron (Fe)
Range
0 - 4.6
0 - 1.2
0 - 15
Chloride (Cl)
M N Range M
0.16 52 0.1 - 26 4.8
0.09 7 2.1 - 64 5.8
0.20 123 0.2-1,830 7.1
Total Hardness (as CaCO3)
N Range M
54 7-246 40
7 93 - 198 130
110 2.0-615 60
Total Dissolved Solids pH
Rock
Location TyP® N
Central Maryland X 46
Central Maryland Cs 7
Coastal Plain U 113
X - Precambrian crystalline rocks
Cs - Carbonate rocks and shale
U - Unconsolidated deposits
N - Number of samples
M - Median
Range
13-321
128 -274
12 -698


M N Range M
73 54 5.4-8.3 6.7
182 7 6 -8.1 7.7
84 207 3.8-8.7 6.5






-------
 It is difficult to generalize on the water quality of the
 extensive Coastal Plain aquifers.   Water quality is known to
 change as ground water migrates from the recharge to the
 discharge areas, and inter-aquifer transfers of water may
 have a considerable effect on concentrations of chemical
 constituents.   The occurrence of saline water is generally
 at shallower depth in an easterly  direction.  Although some
 local conditions modify the situation,  the inland third of
 this province  contains the deepest fresh-water aquifers,
 possibly to depths of 2,000 feet.   The  central section con-
 tains fresh water to depths of about 1,500 feet, and the
 eastern area aquifers are probably saline below depths of
 500 feet.

 The Quaternary age aquifers,  because of relatively rapid
 ground-water circulation,  contain  water which is low in dis-
 solved mineral constituents.   Those areas containing cal-
 careous shell  material yield  hard  water.   High iron content
 is commonly a  troublesome factor.

 Of the Tertiary age  aquifers,  water derived from the Miocene
 units is high  in total dissolved solids and has a pH of 7 or
 above.   The hardness  is high,  especially in water from for-
 mations containing a  large amount  of shell material.   The
 Eocene and  Paleocene  aquifers  yield water with a wide range
 of pH values.   High  iron concentrations are often associated
 with glauconitic material  in  these aquifers.

 The Cretaceous aquifers yield  water having a relatively high
 iron content and a wide range  of pH values.   The sulfate
 content is  often high,  and is  thought to  be derived from
 sulfide minerals.

 MASSACHUSETTS

 The quality of natural ground  water in  Massachusetts  is gen-
 erally good.   However,  mineralization problems do occur,
 frequently  associated with a particular rock type.   Table 16
 is  a compilation of chemical analyses of  selected constitu-
 ents in natural  ground waters.

 Ground  water is  generally  soft.  However,  in the carbonate
 belt in western  Massachusetts, a large  percentage of  wells
 in  all  of the  aquifers  yield water with at least moderate
 hardness.   For 43  wells  in all aquifers in the Housatonic
 River Basin, all but  four  produced at least  moderately  hard
water.  37)

Wells in the Triassic  sedimentary  rocks of the Connecticut
River Valley yield water high  in total  dissolved solids.


                             92

-------
 Table  16.  CHEMICAL ANALYSES OF GROUND WATER IN MASSACHUSETTS. (Concentrations in milligrams per liter.) 37 through 50)
                                         Iron (Fe)
                  Chloride (Cl)
Sulfate ($04)

Location
Northeast


Southeast


West




Rock
Type
X
S/G
T
X
. S/G
T
X
Tr
C
S/G
T

N
20
88
9
8
19
4
34
3
17
102
8

Range
0.05 - 4.4
0 - 2.4
0.03- 1.4
0 - 2.0
0 - 0.69
0.03- 1.1
0 - 6.0
0.12- 1.0
0 - 0.27
0 - 10.0
0.01 - 0.20

M
0.24
0.08
0.14
0.10
0.10
-
0.06
-
0.04
0.10
0.05

N
19
91
9
8
19
4
37
3
17
97
9


1.6
2.0
0.3
4.0
5.0
5.9
1.0
4.6
0.8
1.0
0.5

Range
54
-2,400
56
16
36
13
37
25
- 138
- 325
28

M
5.3
10
6.0
10
10
-
6.0
-
6.0
4.4
4.8

N
17
47
7
8
19
4
15
3
17
31
6

Range
0.4 - 51
0.2 - 89
4.2 - 47
1.2-40
5.6 - 60
14 - 18
0-48
24 - 208
3.8 - 28
3.4 - 29
8.8 - 27

M
16
19
12
13
8.2
-
16
-
19
12
14
X    - Crystalline rocks
Tr   - Triassic sedimentary rocks
C    - Carbonate rocks
S/G - Sand and gravel
T    -Till
N  - Number of samples
M  - Median

-------
Table 16 (continued). CHEMICAL ANALYSES OF GROUND WATER IN MASSACHUSETTS.  (Concentrations in milligrams per liter.)
                                                   37 through 50)


Location
Northeast


Southeast


West




Total
Rock
Type
X
S/G
T
X
S/G
T
X
Tr
C
S/G
T

N
18
87
7
8
18
4
30
3
17
83
8
Hardness {as

Range
17- 150
8-424
15- 140
13- 130
9-70
18- 33
14-213
18 - 109
1 -356
10 - 259
30 - 204
CaCOs)

M
55
38
43
38
15
-
88
-
215
56
77

N
17
54
9
8
19
4
24
3
17
28
6
Total Dissolved Solids


13
32
25
0.
33
68
40
90
120
48
48

Range
- 267
-4,510
- 444
16 - 197
- 268
- 89
- 263
- 468
- 509
- 278
- 245

M
99
180
94
92
62
—
127
-
236
144
120

N
19
90
9
8
19
4
38
3
17
120
9
ftL

Range
6.5 -8.1
5.3 -8.1
5.7-7.8
5.9 -7.9
5.3 -6.8
6.0 -6.6
6.2 -9.0
6.3 -7.8
7.1 -8.2
5.6 -8.2
6.1 -8.4


M
7.3
6.5
6.4
6.8
6.0
-
7.5
-
7.7
6.5
7.1

-------
Like ground water in the carbonate belt of western Massachu-
setts, the ground water in this area is alkaline.  High pH
is usually equated with high hardness and alkalinity, but
this is not the case in the Connecticut River Valley.  What
does occur is dissolution of sulfide and sulfate minerals in
the Triassic rocks, producing ground water high in sulfates
and total dissolved solids. 38,51)

In the northeastern portion of the state, where crystalline
rocks form the bedrock, calcic minerals raise the pH and
hardness.  Of 18 wells in the lower Ipswich River Basin,
nine produced water which could be classified as at least
moderately hard.  The wells with water of highest hardness
were those in bedrock.

The most prevalent natural ground-water problem in Massa-
chusetts is excessive concentrations of iron and manganese
in ground water.  This is especially common where the ground
water has an acidic pH, which includes most areas of the
state. 38)  in the Housatonic River Basin, where the ground
water is commonly alkaline, 11 wells out of 43 reportedly
produced water with a pH less than 7, and four out of 43 ex-
ceeded the U. S. Public Health Service recommended limits
for iron or manganese. 37)  in the Deerfield River Basin,
northeast of the Housatonic River Basin, in 33 analyses of
the 90 for which pH was reported, the pH was less than  7;
out of analyses for 87 wells for which iron or manganese^
concentrations were reported, 34 exceeded the U. S. Public
Health Service limits. 40)

NEW HAMPSHIRE

The quality of natural ground water in New Hampshire is ex-
cellent.  Table 17 is a compilation of chemical  analyses of
selected constituents in natural ground waters.  Hardness is
generally less than 60 mg/1.  A hardness level of 100 mg/1
is rarely exceeded. 51)

High concentrations of iron and manganese can be troublesome,
particularly in sand and gravel wells, as in most of the
northeast states.  From the scanty data  available, high iron
and manganese concentrations appear to be a spotty problem,
but concentrations rarely  exceed  1.0 mg/1 and 0.20 mg/1, re-
spectively.

An unusual natural water-quality problem in New  Hampshire is
the occurrence of high fluorides, especially in  wells  in the
Ossipee Mountains north of Lake Winnipesaukee and in the La-
conia area south of the lake.  At Conway, well waters  are re-
ported to commonly contain 2.5 mg/1 of fluoride.  In Lincoln
                             95

-------
 Table 17. CHEMICAL ANALYSES OF GROUND WATER IN SOUTHEASTERN NEW
              HAMPSHIRE.  (Concentrations in milligrams per liter.) 52,53)
             Iron (Fe)
Chloride (Cl)
Sulfate (SO4)
Rock
Type
X
S/G
T

N
7
30
6
Total
Rock
Type
X
S/G
T

N
6
35
3


Range
0.01 -
0
0
Hardness

0.66
0.80
0.07
(as Ca

Range
32-
9- 1
7-
95
39
64

M
0.12
0.035
0.005

N
7
52
7
COs) Total

M
46
43
-

N
6
24
2

Range
0.8 - 240
0.1 - 133
5.9- 28
Dissolved

Range
72 - 525
36 - 191
33 - 134

M
4.1
9.5
14

N
6
24
2
Solids

M
93.5
78.5
-

N
7
52
4

Range
2.6 - 24
1 .4 - 54
4 -15
PH

Range
5.9 -8.2
5.7-8.3
6.4-7.6

M
— •— —
9.3
12.5



M
— ~— — —
7.9
6.8
_
X    -  Crystalline rock
S/G -  Sand and gravel
T    -  Till
N    -  Number of samples
M    -  Median
                                    96

-------
and Waterville Valley, some wells 200 to 300 feet deep have
similarly high values.  East of Concord, near Bow, a large
number of wells have been sampled, and there is an obvious
fluoride problem.  Near Wolfboro, at the southeastern end of
Lake Winnipesaukee, a well serving a restaurant was reported
to have a fluoride content over 10 mg/1. 54)

NEW JERSEY

In general, the quality of natural ground water in the vari-
ous regions of New Jersey is good.  Table 18 is a compila-
tion of chemical analyses of selected constituents in nat-
ural ground waters.

The major aquifer in the westernmost part of the state is
the Kittatinny limestone.  Water from this  formation is hard,
in excess of 150 mg/1 and up to 500 mg/1, with a pH of over 7.
The younger Richenback and Epler formations locally have a
moderate to high hydrogen sulfide content.  The Martinsburg
formation produces water with a low pH, in  the range of 5 to
6.  The hardness, although highly variable, is moderate —
usually less than 100 mg/1.  However, in some locales hard-
ness concentrations can be very high, with  levels up to 500
mg/1.  Another problem associated with water from this unit
is the high hydrogen sulfide content.

The Precambrian crystalline rocks to the east contain ground
water with a wide range of iron concentrations, dependent on
the mineral content of the rock.  Usually the pH of the wa-
ter is low with only minor concentrations of hardness.  High
iron content is associated with water from  the darker colored
rocks and can be as much as 12 mg/1.

The Triassic rock aquifers are widely utilized by municipal
and industrial supply wells.  Water from the Stockton forma-
tion has a pH from 6 to 7, with a hardness  between 100 and
200 mg/1.  The iron and sulfate contents are variable, with
high concentrations found in the deeper sections.  Wells
penetrating the Lockatong and Brunswick formations yield wa-
ter with a pH greater than 7 and locally high sulfate con-
centrations.  Hardness is highly variable,  with many wells
yielding water that exceeds the state drinking water recom-
mended limits.

Ground water from the Pleistocene deposits  is highly vari-
able, particularly with regard to concentrations  of iron.
Most waters can be expected to have values  of  less than one
mg/1 of iron.  The hardness is low to moderate with a
slightly acid pH.
                              97

-------
                 Table 18. CHEMICAL ANALYSES OF GROUND WATER IN NEW JERSEY. (Concentrations in milligrams per liter.) 55 thro(J9h 72)
CO


Location
Precambrian region
Carbonate region
Triassic region

Coastal Plain



Rock
Type
X
C
Tr
Qt
K
T
Qc

N
7
3
31
13
118
141
28
Iron (Fe)

Range
0.02 - 12
0.10- 0.40
0 - 3.6
0.03 - 3.0
0 - 114
0 - 25
0.01 - 22


M
0.10
-
0.13
0.07
2.5
0.55
0.25

N
18
2
35
25
122
170
34
Total Dissolved Solids

Location
Precambrian region
Carbonate region
Triassic region

Coastal Plain


Rock
Type
X
C
Tr
Qt
K
T
Qc

N
18
-
26
7
92
114
18

Range
51 - 246
-
45-4,780
134- 230
27- 543
15-3,030
14- 482

M
118
-
448
156
123
103
51

N
18
3
35
25
102
174
30
Chloride (Cl)

Range
1 - 40
6 - 8
1 -1,900
2.1 - 27
1.1 -2,057
1.9-1,510
3.1 - 160
£H_

Range
5.2 -8.1
6.9 -8.2
6.0-8.9
6.1 -8.2
3.9 -8.9
4.0-9.2
4.4-8.1
Total

M
6
-
11
7.5
12.5
9.1
9.7

N
18
3
33
25
63
161
27


M
6.8
-
7.4
7.6
6.9
7.1
5.8
Hardness (as CaCO3)

Range
13 - 157
52 - 176
18 - 2,870
32 - 375
4- 580
0- 492
4- 182











M
61
-
187
116
76
34
31










                X  - Precambrian crystalline rocks
                C  - Paleozoic carbonate rocks
                Tr  - Triassic sedimentary rocks
                Qt - Quaternary deposits over Triassic rocks
K   - Cretaceous unconsolidafed rocks
T   - Tertiary unconsol! dated rocks
Qc - Quaternary unconsolidated rocks
N - Number of samples
M - Median

-------
The natural ground-water quality in the Coastal Plain is
generally very good.  However, not all the deep aquifers can
be used for potable water supplies.  Some formations contain
saline water below a depth of 1,000 feet in the downdip sec-
tions.

Water from the Cretaceous age Raritan and Magothy formations
occasionally has a high iron content.  Dissolved solids are
low and appear to increase downdip.  The pH is only slightly
acid.  The other important aquifers of Cretaceous age, in-
cluding the Englishtown, Wenonah, and Mount Laurel, contain
water with low dissolved solids.  Spotty occurrences of high
iron content are found, particularly within the Englishtown
formation.

The Tertiary age aquifers vary in water quality among the
different formations and also within the same formation.
The Vincentown is characterized by water which is moderately
hard to hard, and the dissolved solids and iron content are
occasionally very high.  The Kirkwood yields soft water,
with relatively minor problems associated with excessive
iron concentrations.  The Cohansey contains very soft water
with localized high iron concentrations.

Thick Quaternary deposits of sand and gravel yield good
quality water, although some supplies require treatment for
iron.

NEW YORK

Natural ground water in both the consolidated and unconsoli-
dated rock aquifers of New York is generally of excellent
quality, but hard.  Specific problems do occur, however,
which are usually related to the presence of some distinct
geologic rock units and are most apparent in the shale and
limestone aquifers.  Table 19 is a compilation of chemical
analyses of selected constituents in natural ground waters.

The principal natural problem is the occurrence of high iron
and manganese concentrations in water from the major  aqui-
fers.  The presence of excessive iron and manganese results
from the leaching of these ions from rocks and sediments by
acidic circulating ground water.  Certain consolidated rocks
are commonly high in iron sulfide minerals and trapped hy-
drogen sulfide gas.  When dissolved in water, the sulfides
produce an acidic solution.  The presence of sulfide  miner-
als is common in carbonate rocks of western New York  and
shales across the state;  therefore iron and manganese prob-
lems are also common in these aquifers.
                              99

-------
                  Table 19. CHEMICAL ANALYSES OF GROUND WATER IN NEW YORK.  (Concentrations in milligrams per liter.) 73 thr°u9h 87)
o
o
Location
West
Buffalo-Niagara Region






Oswego River Basin







N - Number of samples
M - Median
a) - Queenston shale and
b) - Albion Group
Rock
Type

Lh°)
Lc
Mh
Uc
Uh
Sb>
T
S
Lh
Lc
Mh
Uc
S/G
T
Uh
N

1
24
1
2
4
-
3
4
2
3
10
6
47
4
8


Clinton Group

Iron (Fe)
Range

1.0
0.05 -8.4
0.07
0.08 -5.6
0.10 -0.53
-
0.03 - 0.98
0.10 -0.78
0.03 -0.43
0.19 - 1.3
0 -3.5
0.02 -0.90
0 -2.4
0.03 - 1.2
0.06 - 0.58


shale

Chloride (Cl)
M

_
0.71
-
-
-
-
"
-
-
_
0.43
0.04
0.22
_
0.12
N

14
67
21
13
85
2
8
4
2
3
14
6
50
4
8
X - Crystalline
Sh - Shale
S - Sandstone
T - Till
Range

54
2.2
4.5
0.1
1
820
1.5
9.8
18
2.2
3.6
3
0.2
1.9
2.1
rocks




- 6,300
- 1,530
- 2,520
860
- 1,000
- 4,450
461
269
- 10,000
59
-21,200
15
-42,500
4.4
- 6,690




C - Carbonate rocks
M

900
49
34
38
28
-
68
_
_
_
64
7
18
_
9.3
Sulfare
(S04)
N Range

14 18 -
64 62 -
21 134 -
13 16 -
85 0 -
2 344 -
8 17 -
3 9.1 -
2 0.2-
3 24 -
11 439 -
2 45 -
17 0.7-
2 24 -
6 3 -
Lh - Lower shale
Lc - Lower carbonate
Mh - Middle shale
Uc - Upper carbonate
Uh - Upper shale

3,620
1,600
1,950
560
789
794
644
46
0.9
72
3,510
182
3,360
69
1,310





M

547
209
1,120
69
21

55
^
_
_
1,320
_
129

8.4





                                                                                               S/G - Sand and gravel

-------
Table 19 (continued).  CHEMICAL ANALYSES OF GROUND WATER IN NEW YORK. (Concentrations in milligrams per liter.)  73 throu9h 87)


Location
Northeast
St. Lawrence County



Lake Champlain -
Upper Hudson Region




Southeast
Albany Region





Lower Hudson Region





Long Island
Total
Rock
Type

S
C
T
S/G
X
Sh
S
T
S/G
C

X
Sh
S
T
S/G
C
X
Sh
S
T
S/G
C
S/G

N

5
42
4
4
_
2
21
-
-'
14

4
51
5
9
58
10
11
6
22
18
47
30
84
Hardness (as

Ranae

221 - 345
41 - 9,420
308 - 467
52 - 405
89 - 134
220 - 283
48- 342
32 - 129
39 - 526
84- 318

50 - 200
1 -5,340
30- 280
30 - 508
32 - 390
42- 360
15 - 173
36 - 291
24 - 210
18 - 269
22- 480
106 - 590
2 - 381
CaCOa)

M

278
283
-
-
_
-
242
-
-
175

_
100
108
172
159
240
104
115
97
38
95
185
21

N

5
36
7
3
_
2
21
-
-
13

4
35
5
4
31
10
10
6
11
9
14
15
89
Total



277
240
288
295
89
268
81
60
66
113

60
105
39
95
29
84
60
192
48
36
115
178
16
Dissolved

Range

- 458
-20,900
558
- 432
- 200
355
550
134
625
378

- 261
-21,700
282
359
505
534
- 276
- 425
296
419
600
513
763
Solids

M

345
692
348
—
•
-
286
-
-
226

_
313
148
-
222
315
183
225
168
55
181
287
76

N

5
35
4
4
-
2
21
-
-
15

4
51
5
7
54
10
11
6
20
17
41
31
91
pH_

Range

7.2-8.3
6.8 -8.3
7.1 -7.8
6.7-7.5
6.8 -8.0
7.2 -7.9
6.3 -8.2
7.5 -8.1
6.7-8.4
7.2 -8.1

6.5 -7.5
6.0 -9.3
6.8 -7.8
6.3 -8.1
6.3 -8.4
6.4-7.5
6.1 -9.6
6.6-8.3
5.8 -8.4
6.0-8.3
6.1 -8.4
7.0 -8.1
4.5-7.7


M

7.6
7.5
-
—
-
-
7.6
-
-
8.0

_
7.5
7.6
7.0
7.6
7.4
7.4
7.8
7.6
6.8
7.2
7.4
6.3

-------
               Table 19 (continued).  CHEMICAL ANALYSES OF GROUND WATER IN NEW YORK.  (Concentrations in milligrams per liter.)  73 through 87)
                                                          Iron (Fe)
Chloride (Cl)
Sulfate ($04)

Location
Northeast
St. Lawrence County



Lake Champlain -
Upper Hudson Region




Southeast
Albany Region





Lower Hudson Region



-

Long Island
Rock
Type

S
C
T
S/G
X
Sh
S
T
S/G
C

X
Sh
S
T
S/G
C
X
Sh
S
T
S/G
C
S/G

N

5
18
2
2
-
2
21
-
-
12

4
48
5
6
60
10
11
6
19
16
42
27
89

Range

0.09 - 0.90
0 -15
0 - 0.08
0.14- 0.16
0.01 - 2.0
0.25- 0.29
0 - 9.1
0.09 - 0.26
0.01 - 2.6
0.02 - 10

0.03 - 0.38
0 .03 - 43
0.1 - 0.25
0.03- 0.5
0 - 2.5
0.03- 1.3
0.1 - 2.4
0.03- 0.97
0 - 0.74
0.03- 3.0
0 - 4.6
0.03- 1.0
0 -17

M

0.39
0.20
-
-
-
-
0.58
-
-
0.15

_
0.2
0.2
0.15
0.1
0.16
0.19
0.39
0.2
0.1
0.10
0.11
0.13

N

5
55
10
5
-
2
21
-
-
15

4
66
5
29
85
10
10
6
22
18
46
33
83



6
1
1.2
0.8
1.8
2.6
1
0
0.1
1

0.8
0.4
0.2
0.4
0.2
0.2
0.6
2.4
1.1
1
1.6
0.7
2.5

Range

38
- 12,800
49
32
29
16
115
2
104
9

2.2
- 10,800
15
198
76
31
18
26
35
55
480
60
235

M

14
46
16
15
-
—
10
-
-
2.4

_
15
3.0
15
8.2
7.1
8.4
5.8
6.4
2.1
4.6
4.0
7.6

N

5
41
4
2
-
2
21
-
-
14

4
36
5
4
36
10
10
6
13
14
33
22
91

Range

45 -
0 -2,
48 -
36 -
0.2-
18 -
10 -
1.8-
0.4-
3.8-

2.6-
0 -
9.4-
6.8-
1 -
17 -
9.3-
10 -
3 -
6 -
6.6-
4 -
0.2 -

M

79 70
020 92
156
64
22
48
101 38
10
227
61 18

32
302 30
20 14
46
109 26
55 30
62 24
87 45
64 24
56 12
190 22
182 29
160 11
o
NJ

-------
               Table 19 (continued).  CHEMICAL ANALYSES OF GROUND WATER IN NEW YORK.  (Concentrations in milligrams per liter.) 73 throu9h
o
U)
Location
West
Buffalo-Niagara Region






Oswego River Basin







Rock
Type

Lh°)
Lc
Mh
Uc
Uh
Sb>
T
S
Lh
Lc
Mh
Uc
Uh
S/G
T
Total
N

14
63
21
13
85
2 1,
8
4
2
3
14
6
6
51
4
Hardness (as
Range

219-4,840
120 -2,660
319-2,780
200- 1,040
52 - 1,180
260 -2,790
137 - 1,310
66 - 185
96-2,710
118- 300
490 -5,050
319 - 680
10- 1,280
52 - 4,420
136 - 600
CaCOs)
M

1,154
482
1,570
338
232
_
367
_
_
_
1,400
425
137
320
™
Total Dissolved Solids
N

8
58
1
2
4
1
3
3
2
1
4
2
6
10
1


533
299
1,500
1,720
193
2,790
154
141
219
344
1,560
372
80
100
199
Range

-11,200 2
- 5,000

- 2,000
841

878
- 642
- 16,200

- 4,320
531
- 13,200
- 2,100

M

,820
689
-
-
-
-
-
_
_
-
_
_
193
372
™
N

14
64
21
13
85
2
8
4
2
3
13
6
8
48
4
PH
Range

5.7-7.8
6.6-8.1
7.0 - 8.0
6.3-7.7
6.8-8.3
6.5-7.1
6.1 -8.5
7.2-7.9
7.3-7.6
7.6-7.8
7.0-7.6
7.3-7.9
6.5-7.9
6.8-8.4
7.5-7.9
M

7.2
7.2
7.4
7.3
7.4

7.7
-
_
-
7.4
7.5
7.0
7.5
"

-------
 Two  problems  which occur regionally are  high total  dissolved
 solids  and  hardness.   Total dissolved solids are  generally
 higher  in the shale aquifer across  the state than in  any
 other consolidated rock aquifer.   It also follows that  total
 dissolved solids  values for water from unconsolidated de-
 posits  overlying  shale are  generally higher  than  unconsoli-
 dated deposits  overlying other rocks.  Hardness is  higher in
 wells in carbonate rocks, and  in  unconsolidated deposits
 overlying carbonate rocks.

 In the  eastern  half of New  York,  high  concentrations  of iron
 and  manganese are  the  major problems associated with  water
 from the shale, limestone,  and unconsolidated rock  aquifers.
 However, other  natural problems occur  in specific areas.  At
 the  extreme northern border in the  St. Lawrence River Basin,
 a large percentage of  wells in two  areas yield water  with
 high concentrations of total dissolved solids.  In  the  ex-
 treme northeast corner of the  state,  some wells penetrating
 the  carbonate and  the  sandstone aquifers have reported  total
 dissolved solids concentrations of  greater than 500 mg/1. 86)

 One  hundred miles  west of this area,  limestone is penetrated
 by many wells which produce highly mineralized ground water.
 Of 39 samples analyzed,  17  contained more than 500 mg/1 of
 total dissolved solids,  and two analyses were reported  with
 nearly  20,000 mg/1.  Chloride  and sodium are  the  predominant
 ions;   three  wells  were  reported  to  have greater  than 10,000
 mg/1 of chloride,  and  two of these were  reported  to have a
 sodium  content over 3,500 mg/1. 87)

 The  inland occurrence  of mineralized and saline water is not
 unusual in the northeast.   Periodic  flooding  by the sea has
 occurred throughout geologic time in the Paleozoic Era  and
 most recently during the Pleistocene Period.   Where the Pa-
 leozoic rocks were  not flushed with  fresh water before  their
 burial, salt  water  may have  been entrapped.   Similarly,  sea
 water that may have percolated into  an aquifer during Pleis-
 tocene  flooding may not yet  be flushed out.

 In Saratoga and Washington  Counties, southeast of the Adiron-
 dack crystalline area, highly  mineralized water is brought
 to the  surface in wells and  springs.  This water  is used at
 the  famous Saratoga Spa and  other spas in the  region. 88,89)

The aquifers  of the western  portion  of New York exhibit the
typical iron/manganese and hardness  problems  associated with
their rock types.   In  addition, some unusual  geologic condi-
tions have caused other ground-water problems.  Generally,
the three oldest rock  units have severe  water-quality prob-
lems.  The lower shale and middle shale  aquifers  are  typi-
                             104

-------
cally salty at depth and may receive sulfate-charged circu-
lating water from the adjacent Lockport dolomite.  In the
west-central area (Wayne County) near Rochester, reported
analyses of the water from wells in the lower shale aquifer
show concentrations that approached 9,000 mg/1 of total dis-
solved solids and 3,500 mg/1 of chloride;  reported analyses
for wells in the middle shale aquifer show concentrations
near 5,500 mg/1 in total dissolved solids, and a water sam-
ple from one well (for which total dissolved solids analysis
was not run) shows a concentration of 21,000 mg/1 of chlo-
ride.  The middle shale aquifer is known to contain some
evaporite beds.  Sulfate concentrations of water from wells
in the middle shale aquifer were reported to be near 2,500
mg/1. 90)  In the next most southerly county (Ontario) the
quality of the middle shale aquifer does not seem to be as
poor.  The maximum total dissolved solids concentration re-
ported is 2,360 mg/1 and the maximum reported sulfate con-
centration is 1,490 mg/1;  unconsolidated aquifers above the
middle shale yield water with a maximum total dissolved
solids of 2,500 mg/1. 91)

At the western edge of the carbonate bands in New York  (near
Niagara Falls), analyses of water from all five of the prin-
cipal aquifers indicate relatively poor quality.  Figure 19
shows how ground-water quality could become affected by nat-
ural inter-aquifer movement of mineralized water.  Total dis-
solved solids content here is commonly greater than 800 mg/1,
and in the upper part of the middle shale aquifer, the range
is reported as 800 to 5,000 mg/1. 92)  The lower shale aqui-
fer in this area discharges connate water averaging 2,600
mg/1 of total dissolved solids and 646 mg/1 of chloride. 93)

Farther south, in the area of the upper-shale aquifer, water
quality is generally adequate in wells in both the upper
shale and overlying sand and gravel aquifers.  However, a
few wells in shale yield highly mineralized water with total
dissolved solids greater than 1,000 mg/1 and chlorides
greater than 500 mg/1. 94)  it was originally believed that
the only source of the minerals in this water was natural
and caused by the presence of evaporite deposits below the
lower shale aquifer.  However, it is now becoming apparent
that improperly constructed or improperly plugged abandoned
oil and gas wells are acting as conduits to bring saline wa-
ter from depth into the surface aquifers.  The volume of con-
taminated water in the shallow aquifers is unknown compared
to the total volume of mineralized ground water.  However,
the rising chlorides observed in water from the  sand  and
gravel aquifer provide a clue that the volume may be  signif-
icant.
                              105

-------
                                             Discharge area of secondary
                                              flow  system. Shallow ground
                                              water with  chloride concen-
                                            t  trot Ions  of 100—SOOppm.
                                                                                  CATTAKAUGUS
                                                                                     CREEK
                Discharge area of primary
                flow system. Shallow ground
                water with  chloride coneen-
                trotlens of  800-2(50Oppm  ,
TONAWANDA
        Figure  19.  Inferred regional circulation of ground water to explain variations in
                         chemical constituents in ground water at shallow depth  in
                                           western New York

-------
Unconsolidated deposits of glacial origin and unconsolidated
deposits associated with the Coastal Plain area of Long Is-
land yield water which is generally of good quality.  Iso-
lated problems that occur are normally related to high con-
centrations of iron and manganese and low pH.

PENNSYLVANIA

Natural ground-water quality is variable in the major aqui-
fers of Pennsylvania, and a high degree of mineralization
has been encountered in some areas.  Selected analyses of
water from wells in various aquifers around the state are
tabulated in Table 20.

A water-quality problem in Pennsylvania, as in nearly all of
the states in the study area, is the occurrence of high iron
and manganese concentrations in water from wells in uncon-
solidated deposits.  Although Table 20 does not record chem-
ical analyses for manganese, it can be seen that median
values of iron concentrations is high in wells in the uncon-
solidated material of the Coastal Plain  (southeast) and Un-
glaciated Appalachians  (south central).  Not so obvious, but
still significant, are the high range values for water from
wells in the northwest, north central, and southwest areas.
The high iron and manganese concentrations in ground water
in these deposits appear to result from leaching of sedi-
ments by natural acidic percolating water.

It can also be seen that iron concentration is rather high
in ground water in late Paleozoic sedimentary rocks.  To
some extent, this phenomenon is related to processes of min-
eralization, where seasonal fluctuations of the water table
expose to oxidation the iron-bearing minerals that commonly
occur in these rocks.  This problem is aggravated where
coal mining has caused an artificial but temporary lowering
of the water table.

Median and range values for calcium, magnesium and bicarbon-
ate are often high in the aquifers of Pennsylvania.  Two
reasons for their prominence in consolidated rock aquifers
are the frequency of interbedded limestones in the Paleozoic
clastic sequences and, in the north, the volume of carbonate
rock debris in the glacial overburden from which recharge is
derived.

A major problem associated with the western region of Penn-
sylvania is the general occurrence of highly-mineralized
ground water in the shallow subsurface  (less than  500 feet
deep). 2)  in the Pittsburgh area especially, it has been
stated that the ground water in bedrock more than  100 feet
                             107

-------
                  Table 20.  CHEMICAL ANALYSES OF GROUND WATER IN PENNSYLVANIA.  (Concentrations in milligrams per liter.) 95 tnrou9h 104>
                                                         Iron (Fe)
                Sulfate (SO4)
   Total Dissolved Solids
O
00

Location
Northeast


Southeast



North Central


South Central



Northwest


Southwest

Rock
Type
SD
PD
U
X
C
Tr
U
SD
PD
U
C
SD
PD
U
SD
PD
U
PD
U

N
22
6
7
87
52
-
70
15
12
12
5
15
11
2
5
72
42
80
9

Range
0.01 - 6.6
0.04 - 3.4
0.01 - 0.12
0.02 - 25
0 - 1.1
-
0.02 -429
0.1 - 0.5
0.1 - 22
0.01 - 14
0.01 - 0.03
0.01 - 16
0.11 - 28
0.31 - 5.8
0.02 - 0.84
0 - 42
0 - 4.03
0.05 - 51
0.07 - 108

M
0.07
0.09
0.02
5.2
0.07
0.14
1.75
0.2
1.5
0.10
0.02
0.18
0.4
-
0.39
1.2
0.14
0.52
0.16

N
61
11
25
38
52
-
86
16
13
12
9
44
32
2
7
50
41
80
9


1
1
1
15
14

1.
2
3
2
3
2
2
14
2
1.
5.
2.
5

Range
- 1,266
66
97
- 412
72
-
1 - 1,340
- 470
- 345
60
27
- 1,764
- 630
40
48
5- 227
1 - 331
3 - 1,618
- 120

M
10
6
9.4
138
43
38
21
10
6
10
10
20
16
-
13
18
31
23
77

N
65
14
27
39
52
-
78
16
13
12
9
43
30
2
7
77
53
78
8

Range
10 -2,102
11 - 393
10- 134
58-1,810
218 - 805
-
124 -4,270
18 -3,155
21 - 584
53 - 972
59 - 312
14 -2,565
19 - 1,042
113- 227
136- 1,488
23 - 3,826
119- 881
62 -8,595
83 - 485

M
124
56
50
357
343
302
239
254
54
137
206
218
163
-
177
311
230
321
316
                   X   - Crystalline rocks
                   C   - Cambrian and Ordovician carbonates
                   SD - Silurian and Devonian sedimentary rocks
PD - Post Devonian sedimentary rocks
Tr - Triassic sedimentary rocks
U  - Unconsolidated deposits
N - Number of samples
M - Median

-------
                                      Table 20 (continued).  CHEMICAL ANALYSES OF GROUND WATER IN PENNSYLVANIA.

                                                          (Concentrations in milligrams per liter.)  95 ^rough 104)
                                                             Total Hardness (as
Chloride (Cl)
o
vo

Location
Northeast


Southeast



North Central


South Central



Northwest


Southwest

Rock
Type
SD
PD
U
X
C
Tr
U
SD
PD
U
C
SD
PD
U
SD
PD
U
PD
U

N
62
14
23
42
52
-
69
16
13
12
9
44
32
2
7
77
54
78
9


6
4
3
52
185

40
15
10
29
51
10
14
74
34
1
43
13
29

Range
- 1,447
- 148
- 198
- 780
- 564
-
- 945
- 544
- 388
- 347
- 273
- 1,994
- 852

- 137
- 622
- 582
- 1,843
- 350

M
94
32
28
232
288
218
120
98
52
104
192
172
101
-
99
110
148
160
136

N
64
12
27
62
52
-
106
16
13
12
9
44
31
2
7
77
54
80
9


1
1
1
13
3

11
1
0
1.
0.
0.
1
24
2.
1
1.
0.
4

Range
- 254
- 168
68
- 400
8 - 82
-
- 302
- 1,820
- 142
6- 465
6- 28
2 - 1,250
70
72
4- 716
- 1,868
2 - 190
5 -60,000
- 145

M
3
2
2
62
8.7
9.7
28
27
4
11
2.0
6
3
-
10
34
14
14
18

-------
 below the valley bottoms is usually too highly mineralized
 for most uses.  103)   The problem is indicated by the high
 median values of total dissolved solids in the northwest and
 southwest areas.  Additionally,  saline water is reported
 locally across  the northern and  western parts of the state,
 as  indicated in Table 20 by the  high range values for chlo-
 ride concentrations.   The high values may be primarily asso-
 ciated with natural  oil seeps which bring saline water to
 the surface, in addition to improperly plugged or abandoned
 oil and gas wells. 104)

 RHODE ISLAND

 The natural chemical  quality of  ground water in Rhode Island
 is  generally excellent.   Table 21 is a compilation of chem-
 ical analyses of selected constituents in natural ground wa-
 ters.   Total dissolved  solids concentration rarely exceeds
 recommended u.  S.  Public Health  Service limits.   For 85 sam-
 ples of ground  water  from various aquifers,  no analysis ex-
 ceeded 500  mg/1 in total dissolved solids.  51)   Water is
 generally soft  to  moderately hard, few analyses exceeding
 120 mg/1  of hardness.

 As  in  most  of New  England,  the prevailing natural problem
 appears to  be the  occurrence of  excessive concentrations of
 iron and  manganese.   In  the Providence area,  waters  from
 most of the wells  in  the sedimentary rock aquifer contain
 objectionable amounts of iron, as do about  one-half  of the
 wells  in  outwash.  106)   in  the Woonsocket basin,  many wells
 in  the  Greenville  area have iron concentrations  of 6 to 7
 mg/1;   some wells  in  overlying unconsolidated deposits also
 produce water with high  iron.  107)   On Block  Island,  iron
 concentrations  as  high as 22 mg/1 have been  reported for
 ground-water  samples  from the unconsolidated  deposits.  108)

 One natural water-quality problem in Rhode  Island is  related
 to  its  long coastline.   In  the southern part  of  the  state
 and on  Block  Island,  salt spray  and  relatively high  quanti-
 ties of dissolved  salt in precipitation cause high concen-
 trations  of chloride  and sodium  in water  from the various
 aquifers.   However, these levels  rarely approach  the  upper
 limit  of  250  mg/1  for chloride recommended by the U.  S.  Pub-
 lic  Health  Service.   On  Block Island,  for example, chloride
 concentrations  in  perched water  bodies  range  from 14  to  248
mg/1, with  a  median of 34 mg/1.  108)

VERMONT

Very little published data  are available on natural  ground-
water quality in Vermont.   According to one report, both
                             110

-------
  Table 21. CHEMICAL ANALYSES OF GROUND WATER IN RHODE ISLAND.  (Concentrations in milligrams per liter.) ]05 through 109)
Location
Providence Co.


Kent Co. and Washing-
ton Co. and Block Island
Newport Co. and Bris-
ton Co.
Location
Providence Co.

Kent Co. and Washing-
ton Co. and Block Island
Newport Co. and Bris-
ton Co.
Rock
Type
X
S
S/G
X
S/G
X
S/G
Rock
Type
X
S
S/G
X
S/G
X
S/G
N
19
14
35
7
19
4
9
Iron (Fe)
Rang'e
0 - 0.
0 - 24
0 - 5.
0.03 - 25
0 - 0.
0 - 5
0.03 - 0.
Total Dissolvec
N
19
11
20
3
18
1
7
Range
22 - 299
53 -319
20 - 168
91 - 227
33 - 147
161
61 - 164
M
4 0.05
0.34
2 0.05
0.5
71 0.03
5 0.08
N
18
13
22
6
18
2
7
Sulfate (SO4)
Range
4.3 - 92
5.1 - 66
5.4 - 109
9.7 - 65
4-32
7.4 - 19
13 - 34
Solids Total Hardness (as
M
117
157
70
52
99
N
18
12
21
4
18
2
7
Range
8 - 182
22 - 228
17 - 179
34 - 198
11-82
89 - 1 10
21 - 62
M
20
29
22
27
8.1
21
CaC03)
M
58
103
53
27
32
N
17
17
36
8
19
4
9
N
17
8
25
4
14
1
3
Chloride (Cl)
Range
1.9 - 17
5 -37
3 -61
0.5 -35
3.8 -38
12 -55
9 -55
PH
Range
6.1 -8.5
6.3 -7.8
5.6 -8.6
6.3 -7.3
5.9-7.4
7.4
6.5 -7.1
M
9
15
14
15
8
17
M
7.2
7.2
6.5
6.7
-
   X  - Crystalline rocks
   S  - Sedimentary rocks
S/G  - Sand and gravel
N - Number of samples
M - Median

-------
ground-water and surface-water quality in Vermont are gener-
ally good.  Of 10 cities using ground and/or surface water,
only two supplies exceeded 100 mg/1 of either dissolved
solids or hardness.
However, the state does have areas with specific problems.
In northwestern Vermont, especially from Middlebury to Col-
chester in the Champlain Lowland, it has been noted that
many wells yield water high in sulfides and hydrogen sul-
fide. HO)  South of Lake Dunmore in the Vermont Lowland,
local rock-well drillers report a problem with "okra",
limonite-pellet concretions which move through and clog
fractures. HI)  There are also frequent reports of high
concentrations of iron and manganese in water from indi-
vidual wells throughout the state.
                        112

-------
                     REFERENCES CITED

                        SECTION V
 1.   U.  S.  Public Health  Service,  "Drinking Water Standards,"
     U.  S.  Public Health  Service Publication  956, 1962.

 2.   Feth,  J.  H., et  al,  "Preliminary Map of  the Conterminous
     United States  Showing Depth to  and Quality of Shallowest
     Ground Water Containing More  Than 1,000  Parts Per Mil-
     lion Dissolved Solids," U. S. Geological Survey Hydro-
     logic  Investigations Atlas HA-199, 1965.

 3.   Connecticut Water  Resources Commission,  Report to the
     General Assembly,  1957.

 4.   Thomas, C.  E., Jr.,  M. A. Cervione, Jr., and I. G.  Gross-
     man,  "Water Resources Inventory of Connecticut, Part 3,
     Lower  Thames and Southeastern Coastal River Basins,"
     Connecticut Water  Resources Bulletin No. 15, 1968.

 5.   Thomas, C.  E., Jr.,  A. D. Randall, and M. P. Thomas, "Hy-
     drogeologic Data in  the Quinebaug River  Basin, Connecti-
     cut,"  Connecticut  Water Resources Bulletin No. 9,  1966.

 6.   Cervione, M. A., Jr., I. G. Grossman, and C. E. Thomas,
     Jr.,  "Hydrogeologic  Data for  the Lower Thames and  South-
     eastern Coastal  River Basins, Connecticut," Connecticut
     Water  Resources  Bulletin No.  16, 1968.

 7.   Cushman,  R. V.,  J. A. Baker,  and R. L. Meikle, "Records
     and Logs  of Selected Wells and  Test Borings and Chemical
     Analyses  of Water  in North-Central Connecticut," Connec-
     ticut  Water Resources Bulletin  No. 4, 1964.

 8.   Ryder, R. B.,  and  L. A. Weiss,  "Hydrogeologic Data for
     the Upper Connecticut River Basin, Connecticut," Con-
     necticut  Water Resources Bulletin No. 25, 1971.

 9.   Randall,  A. D.,  "Records of Logs and  Selected Wells and
     Test  Borings,  Records of Springs, and Chemical Analyses
     of Water  in the  Farmington-Granby Area,  Connecticut,"
     Connecticut Water  Resources Bulletin  No. 3,  1964.

10.   Panozeck, F.  H., "Chemical  and  Physical  Quality  of Water
     Resources in  Connecticut,  1955-1958," Connecticut  Water
     Resources Bulletin No.  1,  1961.
                             113

-------
 11.   LaSala, A. M.,  Jr.,  "Ground-Water Resources of the Ham-
      den-Wallingford Area,  Connecticut," Connecticut Water
      Resources Bulletin No.  14,  1968.

 12.   Cervione, M. A., Jr.,  D. L. Mazzaferro, and R. L. Mel-
      vin,  "Water Resources  Inventory of Connecticut, Part 6,
      Upper Housatonic River  Basin," Connecticut Water Re-
      sources Bulletin No. 21, 1972.

 13.   Ryder, R. B., et al, "Water Resources Inventory of Con-
      necticut, Part  4, Southwestern Coastal River Basins,"
      Connecticut Water Resources Bulletin No. 17, 1970.

 14.   Connecticut State Department of Health, "Analyses of
      Connecticut Public Water Supplies, Five Year Averages
      1966-1970," Seventh Edition, 1971.

 15.   Woodruff, K. D., "General Ground-Water Quality in Fresh
      Water Aquifers of Delaware," Delaware Geological Survey
      Report of Investigation No. 15, 1970.

 16.   Rasmussen, W. C.,  et al, "The Water Resources of North-
      ern Delaware," Delaware Geological Survey Bulletin No.
      6, Vol.  1, 1957.

 17.  Groot, J. J., and W. C. Rasmussen, "Geology and Ground-
     Water Resources of the Newark Area,  Delaware," Delaware
     Geological Survey Bulletin No. 2,  1954.

 18.  Woodruff, K.  D., et al, "Geology and Ground Water, Uni-
     versity of Delaware, Newark, Delaware," Delaware Geo-
      logical Survey Report of Investigation No.  18, 1972.

 19.  Marine,  I. W.,  and W. C. Rasmussen,  "Preliminary Report
     on the Geology and Ground-Water Resources of Delaware,"
     Delaware Geological Survey Bulletin  No. 4,  1955.

 20.  Rasmussen, W.  C.,  J. J. Groot, and N.  H. Beamer,  "Wells
     for the Observation of Chloride and  Water Levels in
     Aquifers that Cross the Chesapeake and Delaware Canal,"
     Delaware Geological Survey Report  of Investigation No.
     3, 1958.

 21.  Gushing, D.  R., I.  H. Kantrowitz,  and K. R. Taylor,
      "Water Resources of the Delmarva Peninsula," U. S. Geo-
     logical Survey Professional Paper  822, 1973.

22.  Rima, D. R.,  0. J.  Coskery, and P. W.  Anderson, "Ground-
     Water Resources of Southern New Castle County, Delaware,"
     Delaware Geological Survey Bulletin  No. 11, 1964.

                              114

-------
23.  Rasmussen,  W.  C.,  et al,  "Water Resources  of  Sussex
     County, Delaware/1 Delaware Geological Survey Bulletin
     No. 8,  1960.

24.  Prescott,  G.  C.,  Jr.,  "Lower Kennebec River Basin  Area,"
     Maine Public  Utilities Commission Basic-Data  Report
     No. 4,  Ground-Water Series, 1968.

25.  Prescott,  G.  C.,  Jr.,  and J. A. Drake, "Southwestern
     Area,"  Maine  Public Utilities Commission Basic-Data  Re-
     port No. 1, Ground-Water  Series, 1962.

26.  Prescott,  G.  C.,  Jr.,  "Lower Penobscot River  Basin Area,"
     Maine Public  Utilities Commission Basic-Data  Report  No.
     2, Ground-Water Series, 1964.

27.  Prescott,  G.  C.,  Jr.,  "Lower Androscoggin River Basin
     Area,"  Maine  Public Utilities Commission Basic-Data  Re-
     port No. 3, Ground-Water  Series, 1967.

28.  Prescott,  G.  C.,  Jr.,  "Lower Aroostook River  Basin Area,"
     Maine Public  Utilities Commission Basic-Data  Report  No.
     5, Ground-Water Series, 1970.

29.  Prescott,  G.  C.,  Jr.,  "Lower St. John River Valley Area,"
     Maine Public  Utilities Commission Basic-Data  Report  No.
     6, Ground-Water Series, 1971.

30.  Prescott,  G.  C.,  Jr.,  "Meduxnekeag River-Prestile Stream
     Basins Area," Maine Public Utilties Commission Basic-
     Data Report No. 7, Ground-Water Series, 1971.

31   Rasmussen,  W. C., et al,  "The Water Resources of Caro-
     line, Dorchester and Talbot Counties," Maryland Board
     of Natural Resources,  Department of Geology,  Mines and
     Water Resources Bulletin 18, 1957.

32.  Rasmussen,  W. C., et al,  "The Water Resources of Somer-
     set, Wicomico and Worcester Counties," Maryland Board of
     Natural Resources, Department of Geology, Mines and
     Water Resources Bulletin 16, 1955.

33.  Rasmussen,  W. C., and G.  E. Andreasen, "A Hydrologic
     Budget of the Beaverdam Creek Basin, Maryland," U. S.
     Geological Survey Open-file Report, 1957.

34.  Overbeck,  R.  M., T. H. Slaughter, and A. E. Hulme, "The
     Water Resources of Cecil, Kent and Queen Annes Counties,"
     Maryland Board of Natural Resources, Department of Geol-
     ogy, Mines and Water Resources Bulletin 21, 1958.
                             115

-------
35.  Otton, E. G., "Ground-Water Resources of the Southern
     Maryland Coastal Plain," Maryland Board of Natural Re-
     sources, Department of Geology, Mines and Water Re-
     sources Bulletin 15, 1955.

36.  Dingman, R. J., H. F. Ferguson, and R. 0. Martin,  "The
     Water Resources of Baltimore and Harford Counties,"
     Maryland Board of Natural Resources, Department of Geol-
     ogy, Mines and Water Resources Bulletin 17, 1956.

37.  Norvitch, R. F., and M. E. S. Lamb, "Housatonic River
     Basin," Massachusetts Water Resources Commission Basic-
     Data Report No. 9, Ground-Water Series, 1966.

38.  Motts, W. S., and Marvin Saines, "The Occurrence and
     Characteristics of Ground-Water Contamination  in Massa-
     chusetts," Water Resources Research Center Publication
     No. 7, 1969.

39.  Sammel, E. A., and J. A. Baker, "Lower Ipswich River
     Drainage Basin," Massachusetts Department of Public
     Works Basic-Data Report No. 2, Ground-Water Series, 1962

40.  Hansen, B. P., F. B. Gay, and L. G. Toler, "Hydrologic
     Data of the Deefield River Basin, Massachusetts,"
     Massachusetts Water Resources Commission Hydrologic
     Data Report No. 13, 1973.

41.  Wiesnet, D. R., and W. B. Fleck, "Millers River Basin,"
     Massachusetts Metropolitan District Commission Basic-
     •Data Report No. 11, Ground-Water Series, 1967.

42.  Petersen, R. G., and Anthony Maevsky, "Western Massa-
     chusetts Area," Massachusetts Department of Public
     Works Basic-Data Report No. 6, Ground-Water Series, 1962

43.  Sterling, C. I., Jr., "Special Report on Ground-Water
     Resources in the Mattapoisett River Valley," Massa-
     chusetts Water Resources Commission Bulletin No. W.R. l
     1960.

44.  Perlmutter, N. M., "Ground-Water Geology and Hydrology
     of the Maynard Area, Massachusetts," U. S. Geological
     Survey Water-Supply Paper 1539-E, 1962.

45.  Brackley, R. A., W. B. Fleck, and R. E. Willey, "Hydro-
     logic Data of the Neponset and Weymouth River  Basins,
     Massachusetts," Massachusetts Water Resources  Commis-
     sion Hydrologic-Data Report No. 14, 1973.
                         116

-------
46.   Baker,  J.  A.,  and R.  G.  Petersen,  "Lowell Area," Massa-
     chusetts Department of Public  Works  Basic-Data  Report
     No.  3,  Ground-Water Series,  1962.

47.   Pollock, S.  J.,  and W. B.  Fleck,  "Assabet River Basin,"
     Massachusetts  Water Resources  Commission Basic-Data  Re-
     port No. 8,  Ground-Water Series,  1964.

48.   Baker,  J.  A.,  and E.  A.  Sammel,  "Wilmington-Reading
     Area,"  Massachusetts  Department  of Public Works Basic-
     Data Report  No.  1, Ground-Water  Series,  1961.

49.   Maevsky, Anthony, and J. A.  Drake, "Southeastern Massa-
     chusetts," Massachusetts Water Resources Commission
     Basic-Data Report No. 7, Ground-Water Series,  1963.

50.   Petersen,  R. G., "Brockton-Pembroke  Area,"  Massachusetts
     Water Resources  Commission Basic-Data Report No.  5,
     Ground-Water Series,  1962.

51.   McGuinness,  C. L., "The  Role of  Ground Water in the  Na-
     tional Situation," U. S. Geological  Survey  Water-Supply
     Paper 1800,  1963.

52.   Bradley, Edward, and  R.  G. Petersen, "Southeastern Area,"
     New Hampshire Water Resources Board  Basic-Data Report
     No.  1,  Ground-Water Series,  1962.

53.   Weigle, J. M., and Richard Kranes, "Lower Merrimack
     River Valley," New Hampshire Water Resources Board
     Basic-Data Report No. 2, Ground-Water Series,  1966.

54.   Dragon, A.,  Personal  Communication,  New Hampshire State
     Health Department, 1973.

55.   Rosenau, J.  C.,  et al, "Geology  and Ground-Water  Re-
     sources of Salem County, New Jersey," New Jersey  Depart-
     ment of Conservation  and Economic Development  Special
     Report No. 33, 1969.

56.   Anderson, H. R., and  C.  A. Appel, "Geology and Ground-
     Water Resources  of Ocean County, New Jersey,"  New Jer-
     sey Department of Conservation and Economic Development
     Special Report 29, 1969.

57.   Vecchioli, John, and M.  M. Palmer, "Ground-Water Re-
     sources of Mercer County, New Jersey," New Jersey De-
     partment of Conservation and Economic Development
     Special Report 19, 1962.
                             117

-------
 58.   Hardt,  W.  F.,  and G.  S.  Hilton,  "Water Resources and
      Geology of Gloucester County, New Jersey," New Jersey
      Department of  Conservation  and Economic Development
      Special Report 30,  1969.

 59.   Gill, H. E., "Ground-Water  Resources of Cape May County,
      New  Jersey,  Salt  Water Invasion  of Principal Aquifers,"
      New  Jersey Department of Conservation and Economic De-
      velopment  Special Report 18, 1962.

 60.   Rush, F. E., "Records of Wells and Ground-Water Quality
      in Burlington  County,  New Jersey," New Jersey Depart-
      ment of Conservation  and Economic Development, Water
      Resources  Circular No. 7, 1962.

 61.   Clark,  G.  A.,  et  al,  "Summary of Ground-Water Resources
      of Atlantic County, New Jersey," New Jersey Department
      of Conservation and Economic Development, Water Re-
      sources Circular No.  18, 1968.

 62.   Hardt,  W.  F.,  "Public  Water Supplies in Gloucester
      County, New Jersey,"  New Jersey Department of Conserva-
      tion and Economic Development, Water Resources Circular
      No.  9,  1963.

 63.   Herpers, Henry, and H. C. Barksdale, "Preliminary Re-
      port on the Geology and Ground-Water Supply of the New-
      ark, New Jersey Area," New Jersey Department of Conser-
      vation and Economic Development Special Report 10, 1951.

 64.   Gill, H. E., and John Vecchioli, "Availability of
      Ground Water in Morris County, New Jersey," New Jersey
      Department of Conservation and Economic Development
      Special Report 25, 1965.

 65.   Kasabach, H. F.,  "Geology and Ground-Water Resources of
      Hunterdon County,  New Jersey," New Jersey Department of
      Conservation and Economic Development Special Report
     No. 24,  1966.

66.  Gill, H. E., et al, "Evaluation of Geologic and Hydro-
      logic Data from the Test-Drilling Program at Island
     Beach State Park,  New Jersey," New Jersey Department of
     Conservation and Economic Development,  Water Resources
     Circular No. 12, 1963.

67.  Jablonsky,  L. A.,  "Records  of Wells  and Ground-Water
     Quality in Monmouth County,  New Jersey,"  New Jersey De-
     partment of Conservation  and Economic Development,
     Water Resources Circular  2,  1959.


                             118

-------
68.   Donsky,  Ellis,  "Records of Wells  and Ground-Water Qual-
     ity in Camden County,  New Jersey,"  New Jersey Depart-
     ment of Conservation and Economic Development, Water
     Resources Circular No. 10, 1963.

69.   Barksdale, H. C.,  et al, "The Ground-Water Supplies  of
     Middlesex County,  New Jersey," New  Jersey State Water
     Policy Commission  Special Report  8, 1943.

70.   Langmuir, Donald,  "Iron in Ground Waters of the Magothy
     and Raritan Formations in Camden  and Burlington Coun-
     ties, New Jersey," New Jersey Department of Conserva-
     tion and Economic  Development, Water Resources Circular
     No. 19,  1969.

71.   Anderson, H. R., "Geology and Ground-Water Resources of
     the Rahway Area, New Jersey," New Jersey Department  of
     Conservation and Economic Development Special Report
     No. 27,  1968.

72.   Barksdale, H. C.,  R. W. Sundstrom,  and M. S. Brunstein,
     "Supplementary Report on the Ground-Water Supplies of
     the Atlantic City  Region," New Jersey State Water Pol-
     icy Commission Special Report 6,  1936.

73.   U. S. Geological Survey, "Water Resources Data for New
     York:  Part 2.  Water Quality Records 1966,"  U. S.  De-
     partment of the Interior, 1966.

74.   Kantrowitz, I. H., "Ground-Water Resources in the East-
     ern Oswego River Basin, New York,"  New York State Con-
     servation Department, Water Resources Commission Basin
     Planning Report ORB-2, 1970.

75.   LaSala, A. M., Jr., "Ground-Water Resources of the Erie-
     Niagara Basin, New York," New York State Conservation
     Department, Water  Resources Commission Basin Planning
     Report ENB-3, 1968.

76.   Johnston, R. H., "Ground Water in the Niagara Falls
     Area, New York," New York State Conservation Department,
     Water Resources Commission Bulletin GW-53, 1964.

77.   Mattingly, A. L.,  "Chemical and Physical Quality of Wa-
     ter Resources in the  St. Lawrence River Basin, New York
     State," New York State Department of Commerce, Bulletin
     No. 4, 1961.
                             119

-------
 78.  Arnow, Theodore,  "The Ground-Water Resources of Albany
     County, New York," New York  State Department of Con-
     servation, Water  Power and Control Commission Bulletin
     GW-20, 1949.

 79.  Cushman, R. V., "The Ground-Water Resources of Rensse-
     laer County, New  York," New  York State Department of
     Conservation, Water Power and Control Commission Bulle-
     tin GW-21, 1950.

 80.  Winslow, J. D., et al, "Ground-Water Resources of East-
     ern Schenectady County, New  York," New York State Con-
     servation Department, Water  Resources Commission
     Bulletin 57, 1965.

 81.  Perlmutter, N. M., "Sources  of Ground Water in South-
     eastern New York," U. S. Geological Survey Circular
     417, 1960.

 82.  Simmons, E. T., I. G. Grossman, and R. C. Heath,
     "Ground-Water Resources of Dutchess County, New York,"
     New York State Department of Conservation, Water Re-
     sources Commission Bulletin GW-43, 1961.

 83.  Perlmutter, N. M.  , "Geology and Ground-Water Resources
     of Rockland County, New York," New York State Depart-
     ment of Conservation, Water Power and Control Commis-
     sion Bulletin GW-42,  1959.

 84.  Frimpter,  M.  H., "Ground-Water Basic Data, Orange and
     Ulster Counties, New York," New York State Conserva-
     tion Department, Water Resources Commission Bulletin
     GW-65,  1970.

 85.  Grossman,  I.  G., "The Ground-Water Resources of Putnam
     County, New York," New York State Department of Con-
     servation,  Water Power and Control Commission Bulletin
     GW-37,  1957.

 86.  Giese,  G.  L.,  and  W.  A.  Hobba, Jr.,  "Water Resources of
     the Champlain-Upper Hudson Basins in New York State,"
     New York State Office of Planning Coordination,  1970.

87.  Trainer,  F. W.,  and E.  H.  Salvas, "Ground-Water Re-
     sources of the Massena-Waddington Area,  St. Lawrence
     County, New York,  with Emphasis on the Effect of Lake
     St. Lawrence  on Ground Water," State of New York De-
     partment of Conservation,  Water Resources Commission
     Bulletin GW-47,  1962.
                             120

-------
88.    Cushman,  R.  V.,  "Ground-Water  Resources  of  Washington
      County, New  York,"  State  of New York  Department  of Con-
      servation, Water Power  and  Control  Commission  Bulletin
      GW-33,  1953.

89.    Heath,  R.  C.,  F. K.  Mack, and  J. A. Tannenbaum,  "Ground-
      Water Studies  in Saratoga County, New York," State of
      New York  Department of  Conservation,  Water  Resources
      Commission Bulletin GW-49,  1963.

90.    Griswold,  R. E., "The Ground-Water  Resources of  Wayne
      County, New  York,"  State  of New York  Department  of Con-
      servation, Water Power  and  Control  Commission  Bulletin
      GW-29,  1951.

91.    Mack, F.  K., and R.  E.  Digman, "The Ground-Water Re-
      sources of Ontario  County,  New York," State of New York
      Department of  Conservation, Water Resources Commission
      Bulletin  GW-48,  1962.

92.    LaSala, A. M., Jr.,  "Ground-Water Resources of the
      Erie-Niagara Basin, New York," State  of New York Con-
      servation Department, Water Resources Commission, Basin
      Planning  Report ENB-3,  1968.

93.    Johnston,  R. H., "Ground-Water in the Niagara  Falls
      Area, New York," State  of New York  Conservation Depart-
      ment, Water  Resources Commission Bulletin GW-53, 1964.

94.    Grain,  L.  J.,  "Ground-Water Resources of the Jamestown
      Area, New York,  with Emphasis on the  Hydrology of the
      Major Streams,"  State of New  York Conservation Depart-
      ment, Water  Resources Commission Bulletin 58,  1966.

95.    Biesecker, J.  E., J. B. Lescinsky,  and C. R. Wood,
      "Water Resources of the Schuylkill  River Basin," Penn-
      sylvania  Department of Forests and Waters Bulletin
      No. 3, 1968.

96.    Meisler,  Harold, "Hydrogeology of the Carbonate Rocks
      of the Lebanon Valley,  Pennsylvania," Pennsylvania
      Geological Survey Bulletin W18, 1963.

97.    Greenman, D. W., et al,  "Ground-Water Resources of the
      Coastal Plain Area of Southeastern Pennsylvania," Penn-
      sylvania Geological Survey Bulletin W13, 1961.

98.    Lohman, S. W.,  "Ground Water in South-Central Pennsyl-
      vania," Pennsylvania Geological Survey Bulletin W5,
      1938.

                             121

-------
  99.  Piper, A. M.,  "Ground Water  in  Southwestern Pennsyl-
      vania," Pennsylvania Geological  Survey Bulletin Wl,
      1933.

 100.  Lohman, S. W.,  "Ground Water in  Northeastern Pennsyl-
      vania," Pennsylvania Geological  Survey Bulletin W4,
      1937.

 101.  Lohman, S. W.,  "Ground Water in  North-Central Pennsyl-
      vania," Pennsylvania Geological  Survey Bulletin W6,
      1939.

 102.  Leggette, R. M., "Ground Water in Northwestern Penn-
      sylvania," Pennsylvania Geological Survey Bulletin W3,
      1936.

 103.  Adamson, J. H., J. B. Graham, and N. H. Klein, "Ground-
      Water Resources of the Valley Fill Deposits of Alle-
      gheny County, Pennsylvania," Commonwealth of Pennsyl-
      vania Department of Internal Affairs, Topographic and
      Geologic Survey Bulletin W8, 1949.

 104.  Mangan, J. W., D. W. Van Tuyl, and W. F. White, Jr.,
      "Water Resources of the Lake Erie Shore Region in
      Pennsylvania," U. S. Geological  Survey Circular 174,
      1952.

 105.  Bierschenk, W. H., "The Ground-Water Resources of the
      Kingston Quadrangle, Rhode Island," Rhode Island De-
      velopment Council Geological Bulletin No. 9, 1956.

 106.  Bierschenk, W. H., "Ground-Water Resources of the
      Providence Quadrangle,  Rhode Island," Rhode Island
      Water Resources Coordinating Board, Geological Bulle-
      tin No. 10, 1959.

 107.  Allen, W.  B., "The Ground-Water Resources of Rhode Is-
      land," Rhode Island Development Council, Geological
      Bulletin No.  6, 1953.

 108.  Hansen, A. J., and G. R.  Schiver, "Ground-Water Re-
      sources of Block Island,  Rhode Island," Rhode Island
      Water Resources Coordinating Board, Geological Bulle-
      tin No. 14, 1964.

109.  Allen/ W.  B., and J. A.  Blackhall, "The Ground-Water
      Resources of Bristol, Warren and Barrington, Bristol
      County, Rhode Island,"  Rhode Island Port and Indus-
      trial Development Commission, Scientific Contribution
      No. 3, 1950.

                            122

-------
110.   Doll,  C.  G.,  Personal Communication,  Vermont State
      Geologist,  1973.

111.   Hodges,  A.  L.,  Personal Communication,  U.  S. Geolog-
      ical Survey,  1973.
                             123

-------
                          SECTION VI

            SOURCES OF GROUND-WATER CONTAMINATION
 DEFINITION OF THE PROBLEM

 As discussed in the previous section,  natural ground-water
 quality in the region is  associated with geologic  and hydro-
 logic processes.   Although problems of natural poor-quality
 water are unavoidable and can limit the development  of
 ground water in specific  areas,  only an extremely  small  num-
 ber of these instances of mineralization present a potential
 health hazard.   Furthermore, overall ground-water  quality  in
 the northeast can be described as  good to excellent.   Rela-
 tively few public-supply  systems find  it necessary to treat
 well water to correct biological and chemical problems re-
 lated to natural  conditions.

 On the other hand,  contamination or degradation of water
 quality due to man's actions can be avoided.   Problems of
 this type often represent severe hazards,  both to  the ground-
 water resource  itself and to public health.   This  section
 describes the principal sources  of contamination in  the
 northeast and discusses their importance in the region.  How-
 ever,  before dealing with such specific details as case  his-
 tories,  frequency of occurrence, and regional trends,  it is
 important to define  the problem  of ground-water contamina-
 tion and to point out the cause  for concern.

 For many years, public  agencies  on all  levels of government
 have been concerned  about the contamination of surface wa-
 ters.   The  loss of rivers and lakes  as  sources of  water  sup-
 ply and recreation can  have  a tremendous impact on a  par-
 ticular region, leading to construction of a  long  pipeline
 to import acceptable  water,  for  example,  or the closing  of a
 popular swimming  area to  local residents.  Degradation of
 the quality of water  in a stream or  lake can  be rather ob-
 vious with  discoloration,  odor,  and  floating  debris.

 Problems  of ground-water  contamination,  on the other  hand,
 have  never  received much  attention because they are usually
 local in  nature,  and  the  effects are hidden from view.   Only
when  a  regional water source  is  threatened, due to such
problems  as  salt-water  encroachment  and widespread pollution
 from  septic  tanks, are  broad controls recommended  and  imple-
mented.   However, protection  of  ground-water  resources from
 all types of  pollutants is an essential part  of any program
 involving the solution  of environmental  problems.  In  many
ways, the correction  of ground-water quality  degradation is
                             124

-------
considerably more complex than in the case of surface waters.

A discussion of the impact of ground-water contamination in
the northeast takes on many aspects including:

1.  The important role of ground water as a water-supply
    source.

2.  The hidden and often misunderstood nature of ground-
    water pollution and the resulting health and other
    hazards.

3.  The dependence of surface-water quality on ground-water
    quality.

4.  The problems involved in monitoring ground-water quality.

5.  The technical difficulties and high costs associated
    with the investigation, control, and correction of
    ground-water pollution.

Importance of the Resource

In the 11 northeastern states covered in this report, ground
water plays a major role in meeting the water-supply require-
ments of communities, individual homes and commercial estab-
lishments, self-supplied industrial facilities, and irri-
gated farm lands.  Total ground-water use in the region in
1970 has been estimated at more than 3.4 billion gallons per
day, which is 18 percent of all the water diverted for all
purposes exclusive of that used for generation of thermo-
electric and hydroelectric power. D

Twenty percent of the water served by community systems is
derived from wells.  Of even greater significance is the
fact that the vast majority of individual utilities is de-
pendent upon ground water because this source of supply is
generally less costly to develop and treat than surface wa-
ter.  Thus, the smaller water purveyors use wells and
springs, where feasible, rather than surface reservoirs,
lakes, and rivers.  For example, two thirds of the 378 pub-
lic water-supply systems in New Jersey use ground water to
meet at least a portion of the demands of the residents they
serve. 2)  it should be noted also that some of the larger
municipalities in that state, such as Atlantic City and
Camden, are included in the two-thirds.  A similar statistic
holds true for Maryland, where 43 out of the  65 community
water systems serving a population of 1,000 or more are com-
pletely dependent upon ground-water  sources.  3)  in jjew York,
at least two and one-half million urban residents are drink-

                             125

-------
 ing well water supplied by 650 municipal utilities.  4)   Con-
 necticut estimates 600,000 persons are served by public wa-
 ter supplies using ground water. 5)

 Ground water plays an even more significant role with regard
 to rural population or those not served by community systems,
 The rapid growth of suburbs after the Second World War in
 areas around major cities in the region has outpaced the
 ability of local utilities to build  the necessary facilities
 to serve these outlying developments.  Consequently, more
 and more homes and small commercial  establishments have con-
 structed their own on-site water supplies.   Invariably, they
 depend on a drilled well.  The widespread use of ground wa-
 ter is possible because rock formations normally are capable
 of yielding at least the few gallons per minute  required to
 supply a single home or store.

 There are probably several million domestic wells presently
 in use within the  11 states.   Table  22 shows the estimated
 number of wells by state constructed in 1964 in  the  region.
 The 78,312 total for that one year represents mostly domes-
 tic wells.

 Statistics on self-supplied industries in the study  area are
 scanty,  but the 1970 U.  S.  Geological Survey compilation
 (see Table 1)  shows a total ground-water use of  1.4  billion
 gallons  per day. D   Many large  manufacturing plants are
 either located beyond the service  areas of  public utilities
 or require such large quantities of  high-quality water  that
 economics  and the  need for  reliability dictate develop-
 ment of  an independent ground-water  source.   In  many cases,
 ground water  is  the only readily available  supply of water.
 For example,  in  the highly  industrialized area along the
 lower  Delaware  River,  a  large number of factories both  in
 New Jersey and  Pennsylvania have tapped the  prolific aqui-
 fers in  the  region  in order to meet  their water-supply  needs
 and have  used the  river  and its  tributaries  only for dis-
 posal  of  their  treated wastes.

 The  potential  for  additional  development  of  ground-water re-
 sources  for  all  purposes  in the  region is quite  large.   For
 example,  the  ultimate daily yield  of New  Jersey's aquifers
 has  been estimated  at five  billion gallons.  7)   jn New  York
 State, glacial outwash deposits  along the Mohawk River
 should be  capable  of  yielding approximately  200  mgd;  the
potential  of  Long  Island's  aquifers  has been  placed  at  1,200
mgd;  and  ground-water resources within the  Susquehanna
River Basin have been estimated  at several hundred mgd.  8)

Ground water  is  available for development by wells every-


                              126

-------
 Table 22.  NUMBER OF WELLS DRILLED IN THE NORTHEAST IN  1964.







State                                  Estimated number of wells drilled




Connecticut                                      6,500




Delaware                                         3,400




Maine                                            17700




Maryland                                         6,902




Massachusetts                                     9,000




New Hampshire                                    4,400




New Jersey                                       3,440




New York                                        25,000




Pennsylvania                                      16,220




Rhode Island                                        250




Vermont                                           1,460






                    Total:                        78,312
                             127

-------
 where  within the region,  and individual  wells  are  presently
 pumped at  rates  ranging up to many thousands of  gallons per
 minute.  Reliance on  ground water  will increase  in the re-
 gion in the  future, not only because  of  its widespread avail-
 ability and  the  growing need for water but because surface
 waters are becoming increasingly more difficult  and expen-
 sive to develop.   Some  principal causes  for this include the
 rising costs  of  treating  surface waters  and the  stricter
 regulations  being imposed by public health agencies for
 their  treatment.   Another involves the problems  inherent to
 obtaining  large  tracts  of land for surface reservoirs.  In
 addition,  there  is the  competition for surface-water rights
 and the  more  active environmental  concern over the effects
 of surface-water  diversions.   Finally, the extreme drought
 conditions experienced  in the region  in  the early  1900's re-
 vealed to  many water managers the  vulnerability  of surface
 water  during  adverse climatic conditions.  On  the  other hand,
 ground water  was  shown  to be  a more reliable water source.
 Because  of this,  a large  number of high-capacity wells have
 been installed as  a back-up  system for municipal and indus-
 trial  surface-water supplies.

 In summary, the importance of ground  water in  the  northeast
 is obvious.   The  availability of this high-quality water
 source is  essential to  the physical and  economic well-being
 of the region, and the  loss of aquifers  or even  individual
 wells  due  to  contamination, which  can be avoided by proper
 controls,  is  unacceptable.

 Health and Other Hazards

 In order to fully  understand  health and  other hazards asso-
 ciated with ground-water  contamination,  it is necessary to
 review the principles governing the movement within  the
 ground-water  system of  a water body containing pollutants.
 Most problems of contamination begin  when an objectionable
 fluid  arrives at the water table.   The fluid may have leaked
 out of an  unlined  industrial-waste  lagoon, for example, or
 could  have been spilled on the  land surface from a  ruptured
 oil storage tank.  Another source  of  contamination  is the
 leaching by precipitation of  salt  in  stockpiles, solid waste
 in landfills, and  fertilizers  and pesticides spread on the
 land surface.  In  other words,  the  rain water is contam-
 inated by contact with the soluble  solid material either
 stored or  spread on the land  surface, and then slowly seeps
downward into the  underlying  aquifer  under the influence of
gravity.  Finally, the pollutant may  have been discharged
directly into the  subsurface  from septic tanks,  leaky buried
pipes or recharge wells.


                            128

-------
Once the fluid containing the pollutant reaches the water
table, it becomes responsive to the local pattern of ground-
water movement, and from that time on, its velocity and
direction of travel will be governed primarily by the laws
of fluid movement in saturated materials.  Ground water is
almost always in motion through geologic formations, follow-
ing paths from areas of intake to areas of discharge.  The
rate at which a liquid travels depends on the permeability
of the deposits and on the hydraulic gradient in the ground-
water system.  In unconsolidated fine-grained sands, ground-
water movement can be very slow, normally less than one foot
per day.  On the other hand, the rate of travel can be con-
siderably greater if the contaminated fluid is moving
through fracture zones or solution cavities of rock forma-
tions.  Where pumping from wells has affected water levels
in the aquifer in the area containing poor-quality ground
water, the rate and direction of travel are also affected,
and the pollutant will move more quickly, and toward the
center of pumpage.

Other factors important to the occurrence and movement of
contaminated ground water are the various processes that can
affect the concentration of the pollutant, such as adsorp-
tion by the materials through which it passes, its density
with respect to that of natural ground water, and the manner
in which it spreads out or disperses as it travels.  Adsorp-
tion or physiochemical forces can remove pollutants from
solution and concentrate them on soil, clay, or fine-grained
sand materials.  Ion exchange and precipitation can also
alter the character of the contaminant.  Differences in den-
sity may cause a contaminant to travel in a direction some-
what different from that of the natural ground water.  For
example, gasoline will tend to float on the water table,
even where there is a strong downward component of flow in
the aquifer system.  Dense brines introduced into a fresh-
water aquifer may tend to sink under the influence of grav-
ity, even though the natural direction of ground-water flow
may be horizontal.

Of great importance is the fact that a pollutant contained
in and moving through an aquifer tends to form an enclave or
plume of contaminated water, extending along its flow path
from the source where it was introduced to the point where
it is either attenuated within the aquifer or is discharged
to a well or a surface-water body such as a river, a lake,
or the sea.  Although dispersal in the direction of flow
tends to reduce the concentration of a pollutant, the fluid
normally does not fan out, and dispersal across the direc-
tion of flow is considerably less than the distance traveled.
Figures 20 and 21 illustrate this effect in an unconsoli-

                            129

-------

-
                                 SALTWATER RECHARGE
                                                                ^T." AQUICLUDE  ^ZT
                     Figure 20.  Flow pattern showing downward leaching of pollutants from a salt stock-
                                            pile and movement toward a pumped well "'

-------
                                                    LEAKY BASINS
                                                           DIRECTION OF GROUND-WATER  FLOW
•
                                 CONTAMINATED
                                 GROUND-WATER
                                                                                         LEAKY
                                                                                          LAGOONS
                     Figure 21.  Plan view of plume of contaminated ground water caused by leakage from
                                lagoons and basins into a water-table aquifer discharging into a river

-------
 dated sand and gravel aquifer.   Movement of  a  contaminated
 fluid in the  fractured zone of  a rock aquifer  is  shown  in
 Figures  22 and 23.   In this latter case,  dispersion  is  very
 slight and the fracture pattern controls the shape and  areal
 extent of the plume.   Finally,  Figure 24 illustrates the
 phenomena associated with  a light-density fluid such as gas-
 oline and the associated plume.

 Thus,  one of  the principal factors involved  in ground-water
 contamination is the character  of the environment in which
 it  occurs.  Although movement underground is normally slow,
 the pollutant is hidden from view,  and given enough  time it
 can travel  undetected thousands  of feet  and  even  miles  be-
 fore  reaching a well or a  stream which is used, perhaps, as
 a source of drinking water.  Two cases of contamination on
 Long  Island,  New York,  illustrate these  points.   In  one in-
 stance,  industrial waste water  containing high concentra-
 tions  of chromium and cadmium has percolated to the  water
 table  principally through  recharge  basins into which the
 pollutant had been discharged.  11)  During a period  of  about
 25  years, starting in the  early  1940'sf  this seepage had
 formed a plume of contaminated ground water  approximately
 4,200  feet  long, 1,000  feet wide,  and as  much  as  70  feet
 thick.   Presence of  contamination went undetected for many
 years  even  though water  from some private wells in the  area
 used  for drinking purposes had been affected.  The maximum
 observed concentration of  hexavalent  chromium  in  the ground
 water  was 40  mg/1 and of cadmium was  10 mg/1.  In contrast,
 the mandatory limits  of  concentrations in mg/1 as set by the
 U.  S.  Public  Health  Service drinking  water standards  are no
 greater  than  0.05 for hexavalent  chromium and  no  greater
 than  0.01 for  cadmium.   In the second case,  leachate  from a
 municipal refuse dump has penetrated  as much as 80 feet into
 the underlying sand and  gravel aquifer, and  the plume of
 contaminated  ground water has extended, unobserved until re-
 cently,  a distance of almost two  miles.  12)  in another case,
 in Warren County, New Jersey, silver  chloride  from a  photo-
 processing  laboratory traveled over a  mile from a seepage
 pit to domestic wells tapping a  limestone  aquifer. 13)

 Contaminated  ground-water bodies  containing  concentrations
 of highly toxic materials are not uncommon throughout the
northeast.  One case  in  Pennsylvania  is noteworthy where
ground-water  pollution,  to the extent  of  10,000 mg/1  of
arsenic,  was  discovered when an  industrial site was  sold,
and a routine  inspection by the new owner uncovered  the fact
that chemical wastes  containing  arsenical  compounds previ-
ously discharged on the property  had  seeped  down  into the
underlying aquifer.  14)  All in  all,  literally hundreds of
cases of contamination of ground water by chemical constitu-
                             132

-------
                                                                             LAND  SURFACE
1*1
                                                                      : LEAKY   SEWER  PIPE
                                               CONTAMINATED WATER
                       Figure 22.  Downward movement of contaminated water from a leaky sewer into the
                                          bedding planes and fractures of a rock aquifer             "v

-------
                                                                      DIRECTION  OF
                                                                      GROUND-WATER FLOW
       EXPLANATION
I .     j   Contaminated groundwater
                                                 ^         ^**~
           Figure 23.  Plan view of contaminated ground water in bedding planes and fractures
                              in a rock aquifer, caused by leachate from a landfill

-------
                                                   ,LAND  SURFACE
UJ
U
             WATER TABLE
                                                     OIL  IN PHASE  FORM (BODY OF OIL)
                         DIRECTION  OF
                         GROUND-WATER FLOW
                                                             OIL IN DISSOLVED FORM
                          Hgure 24.  Movement of light-density fluid in the ground-water system.  Contamina-

                                                    tion caused by a spill of hydrocarbons ^

-------
ents  at  levels  greater  than  those  set by  drinking-water
standards were  uncovered  in  the  northeast investigation.
Undoubtedly,  these  known  cases are only a very  small per-
centage  of  those  that have actually occurred  in the area and
remain undetected.

Another  broad example of  the hazards of ground-water contam-
ination  is  the  large number  of instances  in the northeast of
the presence  of hydrocarbons in  the subsurface  environment.
Many  of  these cases involve  the  loss of private wells and
public water-supply sources.  In others,  petroleum products
have  migrated into basements or  underground conduits causing
explosions  and  fires, or  asphixiating people  working in tun-
nels  and sewers.

In upstate  New  York, two  workers were killed  recently when
they  were asphixiated while  excavating a  tunnel for a sewer
line  at  an  industrial plant. 15)   The cause of  the accident
was traced  to an  unreported  leak of toluene from a ruptured
buried pipeline at the  site.  The  hydrocarbon had remained
floating on the water table  in the vicinity of  the leak.  In
Mechanicsburg, Pennsylvania, leakage of gasoline into a lime-
stone aquifer resulted  in the formation of an underground
pool  about  one-third square  mile in area.  16)   Fumes from
this  pool seeped  into basements  of homes  and  resulted in
several  explosions.

Although the  role that  ground-water contamination plays in
waterborne-disease outbreaks in  this particular region is
obscure, national surveys have shown that pollution of this
source of water supply  is an important factor.   One major
problem  is  that almost  all privately supplied homes, most
small community systems,  and even  some larger public utili-
ties  are supplied with  untreated ground water.   Therefore,
the user is susceptible to bacteria and virus which have en-
tered the well  supply because of poor well construction,
improper location with  respect to  septic  tanks,  or flooding
of the land surface with  polluted  surface water such as
sewage overflow.

Tables 23 and 24  show the results  of an inventory of water-
borne disease outbreaks in the United States  related to
ground-water  sources for  the period 1946-70.  The more than
47,000 cases  are  significant, especially  in view of the fact
that most cases of illness related to contaminated ground
water are probably not  reported  because they  are either iso-
lated cases,  or no death  has occurred, or the source of the
disease was not suspected or investigated.  For example,
studies have  revealed that only  35  to 50 percent of the out-
breaks of disease in New  York State had been  reported to the

                             136

-------
      Table 23.  INCIDENCE OF WATERBORNE DISEASE IN THE UNITED STATES, 1946-70, DUE TO SOURCE CON-
                                TAMINATION:  GROUND WATER (UNTREATED) 17)
                                               Private
                           Public
                                      All Systems
CO
Cause
Improper construction or location of
well or spring
Surface contamination nearby
Overflow or seepage of sewage
Seepage from abandoned well
Source of contamination not
determined
Flooding
Contamination through creviced
limestone or fissured rock
Chemical or pesticide contamination
Data insufficient to classify
Outbreaks


21
49
1

8
4

10
4
46
Cases


640
2,779
50

235
66

555
17
2,001
Outbreaks


1
4
-

1
3

1
-
3
Cases


2,500
531
-

400
4,400

70
-
16,350
Outbreaks


22
53
1

9
7

11
4
49
Cases


3,140
3,310
50

635
4,466

625
17
18,351
                Total:
143
6,343
13
24,251
156     30,594

-------
      Table 24.  INCIDENCE OF WATERBORNE DISEASE IN THE UNITED STATES, 1946-70, GROUND WATER

               (CHLORINATED ONLY): TREATMENT OVERWHELMED DUE TO SOURCE CONTAMINATION. }7>
Private Public
Cause
Overflow or seepage of sewage
Flooding
Outbreaks Cases Outbreaks
3
1
Cases
16,273
600
All Systems
Outbreaks
3
1
Cases
16,273
600
      Contamination of raw-water trans-

        mission line or suction pipe
31
                          31
u>
00
                      Total:
31
16,873
16,904

-------
National Office of Vital Statistics during the period of
1938-60. 18)

The Relationship of Ground Water to Surface Water

One particular aspect of ground-water contamination often
overlooked is the close relationship between ground-water
and surface-water quality in the humid east.  Most programs
directed toward clean streams neglect to take into account
the fact that ground-water discharge represents a major por-
tion of flow in rivers in the northeast, and that during
dry times of the year stream flow is often 100 percent
ground-water discharge.  Since the base flow  (low flow) of
most streams is ground water, and stream quality criteria is
based on low flow quantities and quality, it is essential to
maintain the quality of ground water to protect surface
water.

Great effort is being directed toward improving the quality
of surface water by seeking out sources of pollution dis-
charging directly into streams and by requiring treatment or
some other means for upgrading waste-water quality.  Few in-
vestigations include an evaluation of the quality of ground
water entering a particular stream, or an inventory of poten-
tial sources of ground-water contamination that are already
or might ultimately discharge into a surface-water body.

To illustrate the relationship between surface water and
ground water, it is helpful to review two detailed water-
budget investigations that have been carried out in the re-
gion.  The first, undertaken by W. C. Rasmussen and G. E.
Andreasen of the U. S. Geological Survey, involved the 19.5
square-mile drainage basin of Beaverdam Creek, Maryland. 19)
The chief purpose of the study was to measure and examine
the various factors of the water cycle in a small, homogen-
eous drainage basin in an area of humid climate.  Over a
two-year period, it was found that ground-water drainage was
almost 26 percent of the total precipitation and 72 percent
of the total runoff carried by Beaverdam Creek.  In a simi-
lar study, in the 287 square-mile Brandywine Creek Basin of
Pennsylvania, F. H. Olmsted and A. G. Hely concluded that
as an average for periods of several years, about two-thirds
of the total runoff was base flow  (chiefly ground-water dis-
charge to the streams). 20)

A consequence of this close relationship has been recently
investigated in the Ipswich and Shawsheen River Basins in
Massachusetts. 21)  Many housing developments in the metro-
politan area of Boston are beyond the reach of municipal
                             139

-------
 sewer systems  and waste water,  disposed of through  septic
 tanks and cesspool systems,  percolates  to ground-water  res-
 ervoirs  and eventually reaches  the  streams.   The  investiga-
 tors  were able to use residual  conductivity data  from vari-
 ous sites within the  two basins and develop a relationship
 between  housing density per  square  mile and concentration of
 dissolved solids in base flow of streams.   They concluded
 that  in  the range of  housing densities  observed  (0  to 900
 per square miles),  dissolved solids in  stream base  flow can
 be expected to increase 10 to 15 mg/1 per 100 houses  per
 square mile.   Also, the data indicated  that most  dissolved
 solids from septic tank systems reach the streams.

 Numerous case  histories have been uncovered in this investi-
 gation where contamination of ground water from a point
 source has significantly affected surface-water quality, at
 least in the general  vicinity of the area into which  the
 plume of contaminated ground water  is discharging.  These
 include  problems  related to  leakage from lagoons, pits   and
 basins receiving  industrial  wastes,  mine drainage,  spills,
 and percolation  from  landfills.

 The Problem of Monitoring

 Another  major cause for concern with ground-water contamina-
 tion  is  the problem of  monitoring chemical and biological
 quality.   The principal factors  involved in  the difficulty
 of monitoring this resource,  and of  providing a means for
 adequate warning  against use  of waters  that  may be harmful
 include  the following:

 1.  The  complex nature  of aquifer systems  and movement  of
    ground water.

 2.  The  large number  of individual wells  and springs present-
    ly being used.

 3.  The  great variety of potential  sources of contamination
    such as septic tanks,  landfills, waste  lagoons, etc.,
    and  their relative  abundance  in  the  northeast.

 4.  The  lack of information on  the quantity  and type of  chem-
    ical compounds being discharged  to  the air, soil, and
    water  each day.

The movement of contaminants  through aquifer  systems, as de-
scribed earlier,  is dependent upon  local and  regional ground-
water  flow patterns,  which, unlike  surface streams, are not
discernible with  a visual  or  casual  inspection.   If a load
of chemical waste is  dumped into  the Susquehanna River,   for
                             140

-------
example, it is expected to move downstream, and it is not
very difficult to determine in which direction the river is
flowing.  Furthermore, if the river is polluted with high
counts of coliform bacteria, a sample dipped from almost any
portion of the stream will give some indication of pollution.
Not so with ground water:  it is under laminar flow condi-
tions and "downstream" may be in any direction, not neces-
sarily related to surface topography at any particular loca-
tion.  Also, fluids of different densities and bacteria do
not always move with the main body of ground water.  They
can float on the water table or sink toward the bottom of
the aquifer.

Thus, determination of the direction of flow and areal ex-
tent of a contaminated ground-water body can be complex, and
often can only be determined by a rather detailed and costly
program of test drilling, and water-level and water-quality
analyses.  Even determining the shape of the water table may
not be adequate for defining the problem, because this only
indicates the horizontal direction of flow and gives no in-
dication of how deeply a drop of contaminated fluid may de-
scend along its path to a point of discharge.

For example, under some conditions, a drop of water may
travel at fairly shallow depths from the place where it
reaches the water table to the place where it leaves the
ground-water system.  Elsewhere, it may descend rather
steeply to invade aquifers many hundreds of feet below the
water table, and may move through those aquifers in a direc-
tion quite different from that followed by water in the
shallow beds.  Therefore, a proper evaluation of ground-
water flow involves a knowledge of what is taking place in
the vertical dimension as well as in the horizontal.

Figures 25 and 26 illustrate this principle.  Both diagrams
are hypothetical but are based on detailed studies of the
hydrology of several solid waste landfills in the northeast.
Figure 25 is a water-table map revealing that the highest
point of the water table underlies the landfill area.  Ac-
cording to one basic law of ground-water flow, the direction
of movement of any drop of ground water in an unconfined
aquifer is at right angles to the water-table contours.
Thus, a drop starting at point "A", for example, will ulti-
mately discharge into the adjoining marsh.  Figure 26, which
is a cross section through the hypothetical landfill along
line X-X1, shows, by means of arrows, the vertical pattern
of flow.  A drop of contaminated fluid reaching the water
table at "B" would penetrate quite deeply  into the under-
lying sediments before being discharged into the river.
Actually, in the northeast region, abnormally high levels  of

                             141

-------
NJ
                                                                                            MARSH

                                                                               EXPLANATION

                                                                           I	Height of water table in feet
                                                                                  above river  level

                                                                          -^—X  Line of section in Figure
                                                                            Path of a drop of water starting
                                                                            at point "A"
                          Figure 25.  Plan view of water table contours associated with a landfill

-------
•
               *-DISCHARGE AREA—»
                                                                                                          DISCHARGE AREA
                                                                                                                             RIVER
           \
                                                                                                        EXPLANATION

                                                                                                     :-  i Contaminated ground water

                                                                                                    -5-  Trace of equipotential surface
                                                                                                           on plane of section
                                                                                                    *	 Path of a drop of water starting
                                                                                                         at point "B"
                                    Figure 26.  Generalized  hydraulic  profile  beneath a landfill

-------
 iron,  chloride,  and hardness have been  found in observation
 wells  screened more than  100 feet below the water table be-
 neath  a  landfill,  indicating penetration to this depth of
 ground water that  had become contaminated by contact with
 the refuse.

 Stratification of  sediments, such as a  clay lens contained
 within a sand and  gravel  aquifer, can locally modify the
 movement of ground water  and distort the overall pattern of
 flow.  This is illustrated by a situation in southern New
 Jersey involving contamination of ground water from leaky
 waste  lagoons, pits, and  basins containing industrial wastes.
 As a protective device, the owner of the industrial site had
 drilled  several monitoring wells but had not realized that
 they were all screened below a clay zone which was prevent-
 ing the  contaminant from  penetrating deeply into the aquifer.
 For several years, water  from the monitoring wells was peri-
 odically analyzed  but showed no change  compared to base line
 conditions.  Thus, it was concluded that the lagoons were
 not leaking and ground-water contamination was not taking
 place.   It was only after new monitoring wells were designed
 and installed under state guidance that the problem was dis-
 covered.  Further  detailed study revealed that about 200
 million  gallons of contaminated ground water, with zinc and
 chromium concentrations of up to 50 and 150 mg/1 respective-
 ly, underlie the immediate area of the property. 22)

 The situation is illustrated in Figure 27.  Wells A and B
 represent the early monitoring wells that were improperly
 screened below the sand and clay zone.  Well C represents
 the wells drilled under state guidance, which indicated
 there was a problem, and Wells D-l, D-2, and D-3 represent
 wells drilled during the detailed investigation which helped
 define the areal extent of the contaminated ground-water body.

 Thus,  locating pollutants in the ground-water system is a
 complicated matter.  Even after contamination is indicated,
 defining the problem calls for use of all the various tech-
 niques available to the investigator.

The second problem with regard to monitoring is the diffi-
 culty in keeping track of quality of water from the large
number of public supply, industrial, and domestic wells in
 the region.  The widespread use of ground water was discus-
sed in an earlier  section.  However, it is interesting to
note some of the results of personal interviews with repre-
sentatives from the various state agencies charged with
health and water pollution matters.

 In none of the 11 states of the project area are accurate


                             144

-------
              EXPLANATION
          A-Location of monitoring well


          I Well screen
•
                                                                               PRECIPITATION
                                                                      LEAKY BASIN     ' D'2
DIRECTION  OF \ \ \ '. I \ \ \ \ '. :V I
GROUND-WATER FLOW
                                    CONTAMINATED
                                    :6ROU*D- WATER
                   Figure 27.  Movemenl1 of contaminated ground water beneath leaky lagoons and basins

-------
 figures available on the number of wells drilled each year,
 how many are in use, or what proportion are abandoned.   Even
 in those states where permits are required for new well con-
 struction,  such as New Jersey and Maryland, the estimate is
 that applications for permits are received for only about
 half of the wells drilled.   New Jersey presently has about
 100,000 well permits on file and, for  the period July 1969
 to July 1973,  Maryland issued permits  for more than 31,351
 wells.   During this four-year period,  the number of applica-
 tions per year almost doubled in Maryland.   In addition to
 the tremendous number of individual ground-water sources,
 only for a  relatively small  percentage of new wells is  the
 water analyzed.   Exceptions  to this, of course,  are public
 water-supply wells which invariably must be approved by some
 type of health authority before they are put into service.
 However,  domestic wells and  those used by industry for  drink-
 ing-water purposes do not normally fall within the authority
 of public health agencies.

 Many state  and local agencies offer the free service of run-
 ning analyses  for selected chemical constituents and bac-
 teria in water from private  sources when the sample is
 brought in  on  a  voluntary basis.   In fact,  many  of the  state
 laboratories report that their personnel and facilities are
 sorely  taxed trying to keep  up with this activity.   Never-
 theless,  again only a relatively  small percentage  of the
 wells drilled  are  sampled initially, and,  just as  critical,
 even fewer  are sampled on a  periodic basis.   In  a  detailed
 investigation  of the quality of water  from  domestic wells in
 York County, Maine,  it was found  that  461 of the 511 sup-
 plies sampled  (90  percent) had never been inspected by  a
 health  agency.  23)

 In some  states and local  areas, there  has been a growing
 trend toward requiring analysis of  new private well-water
 supplies  and certification by a health agency  before the
well can  be put  into service in the home or  factory.  This
 trend undoubtedly  will continue but  there still  will be a
need to  sample wells that have been  in service for  many
years,  to conduct  periodic analyses of water  from  new wells,
and  to  locate  the  large number of unreported wells  installed
each year in the region.

Even the present effort given  to public  water-supply wells
may  not be enough  to guard against  the  threat  of possible
use  of contaminated  water.   Again,  the number  of individual
sources is startling.  For example, the  Connecticut  Health
Department must  inspect and  monitor 639 wells  and  springs
used for public-supply purposes. 24)
                             146

-------
The need for continuously monitoring such supplies on a peri-
odic basis also relates to the manner in which a contaminant
can migrate through the ground-water system.  As explained
earlier, a body of highly contaminated fluid can move as a
distinct plume and can advance as a front through a particu-
lar aquifer.  Thus, water from a pumping well can be of safe
quality for many years and then become adversely affected
over a relatively short period of time when an advancing
front of poor-quality water reaches the well.  The advancing
front characteristic of salt-water encroachment in heavily
pumped coastal areas has been well documented, and the dras-
tic change in water quality that can occur by movement of
such a front into a well field is illustrated in Figure 28.
In this case, periodic chloride analyses of water from a
well being used in the Cape May City area of New Jersey
showed very little change from late 1945 to late 1950.  Then
within a matter of weeks, after lateral encroachment of a
salt-water front reached the well, chloride concentration
began to rise significantly and continued on an upward trend
for the duration of the record shown.  Horizontal movement
of such fronts in coastal plain aquifers has been measured
at rates of a few feet to more than 100 feet per year.

In Endicott, New York, high counts of coliform bacteria sud-
denly showed up in a million-gallon-per-day municipal well
after 19 years of trouble-free operation. ^6)  Excavation of
the bed of the Susquehanna River, which was locally contam-
inated by sewage, appears to be responsible for the problem.
Higher infiltration rates caused by the excavation allowed
bacteria to enter the sand and gravel aquifer tapped by the
well, and the bacteria traveled 180 feet to contaminate
this ground-water source.  Routine weekly water samples re-
vealed the problem, and the well was immediately taken out
of service.

Unfortunately, such frequent sampling of public water sup-
plies is not universal.  A recent survey by the Comptroller
General of the United States of federal and state programs
needed to insure purity of drinking water included three of
the states in the northeast study region:  Maryland, Massa-
chusetts, and Vermont. 27)  A review of the most recent
chemical analyses on file for two of these  states revealed
that for Maryland, 27 percent and for Vermont,  49 percent
were more than one year old.  In addition,  only in Maryland
were public health officials satisfied that the frequency  of
surveys of water supplies is adequate enough  to detect po-
tential sanitary problems.

Some idea of the wide variety of potential  sources of  ground-
water pollution can be gained from  the compilation given  in

                             147

-------
           240
Figure 28.  Long-term chloride fluctuation in a well tapping the Cohansey Sand in
                       the Cape May City area, New Jersey
                                   148

-------
Table 25, which is based on an analysis of actual reported
cases of ground-water contamination inventoried during the
northeast investigation.  Representative examples of the
various categories listed were obtained from public agencies
involved in health and environmental matters, from well-
drilling contractors, from private organizations such as con-
sulting firms and business associations, and from literature
sources.  It can be seen that many activities of man can
lead to degradation of ground-water quality.  Monitoring of
the potential source, either by means of accurate measure-
ment of losses of fluid and soluble material to the ground-
water system or through the installation of enough wells for
periodic water-quality sampling, is an almost insurmountable
task.  Even inventorying the location of potential sources
of contamination is a major problem for regulatory agencies.

Although no list could contain all causes of subsurface pol-
lution, Table 25 does include the key sources, and an at-
tempt has been made to rank them according to their impor-
tance and to assess the degree of environmental hazard.  It
is interesting to note that some items listed, such as
septic tanks and cesspools, are a major problem throughout
the entire region whereas others vary in importance from
area to area.  For example, many public officials in the
northern and central New England States feel that salts from
highway deicing are the most significant factor in ground-
water quality degradation.  In New York and Connecticut, the
major factor tends to be high densities of septic tanks in
new housing developments.  Landfills and industrial-waste la-
goons, pits and basins appear to be receiving the most at-
tention in New Jersey, Maryland, and Delaware.  Finally, in
Pennsylvania, major emphasis is being placed on permitting
programs for solid waste, coal refuse disposal, surface im-
poundments, and spray irrigation.

The third column in Table 25 is an estimate for the region
as a whole of the rate of new occurrences for each of the
sources listed.  Each estimate is based on an evaluation of
such factors as awareness of the particular type of problem;
the predicted degree of activity creating incidences of
contamination;  anticipated staffing of federal, state and
local environmental programs;  laws, rules, and regulations
in effect or proposed;  and the level of technology avail-
able to prevent future problems.

The abundance of septic tanks and cesspools is a good illus-
tration of the difficulty in monitoring the source.  Table
26 lists the populations not served by central sewer systems
on a state-by-state basis.  These statistics would indicate
that there are millions of individual septic tanks and cess-


                             149

-------
 Table 25.  PRINCIPAL SOURCES OF GROUND-WATER CONTAMINATION AND THEIR
                           RELATIVE IMPACT IN THE NORTHEAST
 Sources
     Relative
     importance
     to region q'
Typical size
of a rea
affected °>
Estimated future
trend in rate of
new occurrences
                                                                                            c)
 Septic tanks and cesspools

 Buried pipelines and storage tanks

 Application and storage of highway
   deicing salts

 Landfills

 Surface impoundments

 Spills and surface discharge

 Mining activity

 Petroleum exploration and develop-
   ment

 Salt-water intrusion

 River infiltration

 Underground storage  and artificial
   recharge of waste water

Water wells

Agricultural activities
       I
                           III

                           III

                           III

                           II
                           IV
                           IV
                          III

                          II
a)   I   - High
    II  - Moderate
    III  - Low
I    - Regional
II   - Point source but can be regional
     in nature due to high density of
     individual occurrences
III  - Can affect adjacent properties
IV  - Effects usually contained within
     the boundaries of one property
                c)  I   - Increase
                   II  - No significant
                        change
                   III - Decrease
                                             150

-------
Table 26.  ESTIMATED POPULATION SERVED BY SEPTIC TANKS IN 1968, BY STATE.






State                  Estimated population served       Percent of total population




Connecticut                     1,344,845                       46




Delaware                         131,390                       26




Maine                            413,885                       43




Maryland                       2,049,395                       57




Massachusetts                   1,661,990                       31




New Jersey                     1,131,290                       17




New Hampshire                    392,200                       57




New York                      2,918,640                       17




Pennsylvania                    1,435,929                       13




Rhode Island                      331,975                       38




Vermont                          211,700                       51









            Total:             12,023,239                       22.5
                                  151

-------
 pools,  each discharging domestic  wastes  into the  subsurface
 environment.   In  addition,  there  are  hundreds of  areas where
 their density is  great  enough  to  have caused significant
 rises in  nitrate  concentration in ground water, created prob-
 lems of detergent in well supplies, or threatened health  due
 to migration  of bacteria and viruses  into  poorly  constructed
 and improperly located  wells.   Also,  migration of nitrate
 from aquifers into surface  water  is most important because
 nitrogen  constraints for many  streams are  more severe than
 drinking  water standards.

 Examples  that are typical of unsanitary  conditions experi-
 enced by  many domestic  well owners, mostly in the rural por-
 tions of  the  region, are as follows:

     *In  a  six-year survey  (1955-1960),  personnel of the
 Rensselaer  County,  New  York, Health Department carried out
 sanitary  surveys  of 2,100 private dwellings  served by on-
 site water-well supplies. 29)   On the average, 38 percent of
 the water samples collected showed the presence of contam-
 ination,  and  42 percent of  the wells  were  ruled improperly
 constructed,  protected,  or  located.   At  least 25  percent  of
 the home  owners that were informed of an unsanitary condi-
 tion in their water-supply  system made corrections based  on
 the Health  Department recommendations.   In 1970,  County per-
 sonnel surveyed 94  wells in one semi-rural area and found
 that 49 percent were producing water  of  unsanitary quality
 and 30 percent more of  questionable quality.  30)

     *The Connecticut State Department of  Health  surveyed
 individual  wells  in one  rural  town which has  neither a pub-
 lic water supply  nor a  central  sewer  system.   Based prim-
 arily on  coliform count  and supported by data  on  concentra-
 tions of  nitrogen compounds, it was concluded  that 30 per-
 cent of the 50 wells sampled were  producing water that was
 probably  unsafe for drinking.  31)

     *In  the  York County, Maine,  investigation mentioned
previously, 17 percent of the  462 water  wells  sampled were
considered by  the  investigators to be  contaminated.  Well
construction  appeared to be the key factor because water
 from 30 percent of  the dug wells was  found to be  contami-
nated as compared to four percent  for  driven and  seven per-
cent for drilled wells.  23)

     *More than half of  40 wells  sampled in a rural area  of
Pennsylvania underlain by carbonate rock were found to yield
water containing  "excessive bacteria". 16)

Community landfills and open dumps are also more  numerous in

                             152

-------
the northeast than generally realized.  Literally thousands
of sites exist where domestic refuse,  industrial solid and
liquid waste, and septic tank cleanings have been deposited
for many years.  Investigations have shown that landfills
are an almost universal source of ground-water contamination,
yet less than one percent are monitored by periodic sampling
of wells specifically drilled to watch over possible changes
in ground-water quality.  This is true even though surveys
indicate that 15 to more than 20 percent of the operators of
community landfills have reported surface drainage and
leaching problems, and that the lowest part of the fill is
in the water table, an excellent indication that subsurface
contamination is occurring. 32)  Effects on ground-water
quality include increased concentrations of such constitu-
ents as chloride, iron, manganese, hardness, and total dis-
solved solids.  Where solid-waste sites have also received
industrial liquids and sludges, the presence of heavy metals
in the leachate has been observed.  Connecticut estimates
that in 1972, 33 million gallons of industrial liquid and
sludge wastes were probably deposited in municipal landfills
in that state, of which 7.5 million gallons were oils and
hydrocarbons and more than 3.5 million were solvents. 33)
Until recently, only in Pennsylvania was the installation of
monitoring wells mandatory at landfills. 34)  Now, however,
most of the other states in the region are beginning to call
for monitoring at new and old landfills, especially those
suspected of causing ground-water contamination.

Two other important examples of sources from Table 25 that
are most difficult to monitor are salts from highway deicing
and leaks from buried pipes and storage tanks.  During the
winter season of 1966-67, almost two million tons of sodium
chloride and 70,000 tons of calcium chloride were spread on
highways in the 11 northeast states. 35)  Monitoring the
thousands of miles of roadways to locate areas where melt
water has carried these highly soluble substances to the wa-
ter table and has significantly affected ground-water qual-
ity is physically and economically impossible.  A similar
situation exists with regard to the length and number of
buried pipelines and storage tanks that may be leaking toxic
or hazardous liquids into the ground.  There are no strict
regulations governing the monitoring of storage tanks as to
maintenance or replacement.  Pennsylvania alone estimates
that 2,600 new or replacement  subsurface storage tanks are
buried in the ground each year. 36)  Most are probably used
until they fail, which means the liquid they contained was
lost to the subsurface.

Another problem in monitoring  is the great variety of inor-
ganic metals, salts, acids or bases,  synthetic organics,

                             153

-------
 flammables  and other  compounds  produced  each year  in  the
 northeast.   Much  of this  material  is  toxic  and  finds  its way
 into  industrial waste streams.   It has been pointed out that
 of  496  organic chemicals  considered likely  to be found in
 water,  only 66 have been  positively identified. 37)   Hazard-
 ous substances such as  arsenic,  cadmium,  chromium, chlorin-
 ated  hydrocarbons, cyanides, lead,  mercury, copper, and zinc
 are widely  used in many industrial activities including
 metallurgy;  paint, rubber, and  paper manufacturing;  and
 the production of batteries, Pharmaceuticals, and  textiles.

 Unfortunately,  many toxic substances  are  not included in
 normal  analyses conducted on water-supply sources.  In fact,
 in the  11 northeast states, analyses  for  some of the  hazard-
 ous elements such as  barium, selenium, and  silver, included
 in the  U. S. Public Health Service  Drinking Water  Standards,
 1962, are not  usually required  for  a ground-water  source to
 be approved, nor are  they often  included  in routine analyses
 unless  contamination  is suspected.  38)  in  the Comptroller
 General survey mentioned previously, Massachusetts did not
 make  analyses  of water  from public  supplies for any of the
 nine  chemicals  included in the Public Health Service  manda-
 tory  standards, except  for those supplies serving  interstate
 carriers. 2?)  Vermont  did not run  analyses for 7  of  the 20
 chemicals included in the mandatory and recommended stand-
 ards.   Interviews with public health personnel in  the region
 did indicate that more  effort is being made to determine the
 possible presence of  toxic substances, and  that there is an
 overall trend  toward  more complete  analyses of drinking wa-
 ter.  However,  again  this is difficult to accomplish  due to
 limitations of budget,  staff, and  laboratory facilities.

 It is interesting to  note that the vast majority of the
 hundreds of ground-water contamination case histories inven-
 toried  in this  investigation came to the attention of
 authorities because of complaints of taste or odor, notice-
 able effects on surface waters or vegetation, or through the
 investigation  of an accident such as a ruptured storage tank
 or a spill of hazardous material.  Few were uncovered in the
 course  of routine analysis of the water itself.  Where
hazardous substances were involved, for example, in those
cases involving high  concentrations of arsenic, hexavalent
chromium, cyanide, or lead, it was a change in the non-toxic
constituents which are normally determined, such as iron,
chloride, and hardness, that led to more complete analysis
of the water from the affected source.  Only after the more
detailed testing was the presence of the toxic substance de-
termined.

Several case histories in Connecticut illustrate these

                             154

-------
points.  A family supplied by a domestic well suffered mys-
terious loss of hair. 31)   Analysis of routine constituents
in the well water revealed no indicator that could be traced
as a cause of the phenomenon.  It was only after a test for
thallium, rarely included in water analyses, was conducted
that the source of the problem was determined.  Heavy use of
thallium-bearing agricultural sprays in the area had con-
taminated the aquifer tapped by the domestic well.

In another case, presence of a chlorinated hydrocarbon was
only detected in a high school well because of the foul
taste and odor associated with this substance. 31)  rphe
source was the dumping of waste solvents on a neighboring
industrial property.  Finally, during a routine pumping test
to determine the yield of an industrial well that had been
in service for a number of years, it was noticed that the
water being pumped to waste during the test had a distinct
yellow color. 39)  This had not been observed before because
chemical analyses of ground water had not been run for many
years and the water from this well was mixed with water from
other sources in the industrial plant.  Analysis showed that
the color was caused by the presence of chromates in concen-
trations of as much as 26 mg/1.  The source of the contami-
nated water was leakage out of the bed of a lagoon, about
1,000 feet away, receiving wastes from a metal-plating com-
pany .

Technical and Economic Difficulties

One particular aspect of ground-water contamination that
makes it quite different from river pollution, and in many
ways a more difficult problem to solve, is the long time
factor required for decay, adsorption, or dispersion of the
contaminant in the ground-water system even if the source of
contamination is removed.  Correcting a situation causing
ground-water contamination, such as lining a  leaky basin in-
to which a liquid industrial waste has been discharged, will
prevent an increase in the volume of the highly mineralized
fluid arriving at the water table but will not result in an
end to the problem itself.  Because the polluted ground-
water body normally moves and disperses slowly, and is
little affected by dilution from the recharge of or mixing
with unaffected water, contaminants in ground water tend to
be reduced in concentration over a period usually measured
in years and even decades.  In fact, long after a source of
pollution has been removed, the contaminated  ground-water
body actually can expand in areal extent and  can travel sig-
nificant distances before it disperses.
                             155

-------
 Few studies  have  been carried out that  would define  in  de-
 tail the  degree to which  contaminants will  become  attenu-
 ated with time and distance  traveled after  the  source of
 pollution has been removed.   One  recent investigation by
 George  F.  Finder  of Princeton University applies a mathe-
 matical model capable of  predicting  the transient  behavior
 of  a plume of contaminated ground water over a  wide  range of
 field conditions.  4°)  Use was made  of  the  chromium  contam-
 ination case on Long Island  referred to in  a previous sec-
 tion. 11)  in this situation, the point of  discharge for the
 4,300 foot long plume of  contaminated ground water is a
 creek,  which drains the water-table  aquifer in  the area.
 Pinder  has computed that  ground-water contamination  of  the
 creek would  continue for  seven years after  disposal  of  the
 pollutant  to the  land surface is  ended.   Ground-water veloc-
 ity was computed  to average  1.4 ft/day.

 Within  the northeast region,  there are  several  widely used
 methods for  combating contamination  of  ground water  after it
 occurs.  The first step,  once the problem has been discover-
 ed,  is  an  attempt to prevent the  activity from  continuing to
 degrade water quality, in other words,  eliminating the
 source  as  quickly as possible.  For  example,  a  specific
 activity  such as  the discharge of industrial wastes  into a
 limestone  sinkhole can be ended immediately if  action is
 brought to bear by a public  agency equipped with evidence
 that a  well  supply has been  rendered unfit  or is threatened
 because of the industry's disposal method.  A storage tank
 can be  pumped dry and taken  out of service  if it is  traced
 as  the  source of  a gasoline  leak  that has affected ground-
 water quality in  the area.

 However, it  is not always possible to immediately  end some
 types of activities  that  contribute  to ground-water  contam-
 ination .   For example, because no adequate  substitute has
 been  found for highway deicing salts, the process  is con-
 tinued  even  in areas where wells  have been  shown to  be  ad-
 versely affected.   In some communities,  the quantity of
 salts normally used  has been  reduced, but this  is  not an
 ultimate solution  to the  problem.  In the case  of  municipal
 landfills, it is  a  difficult  and  time consuming project to
 find  a  substitute  site for the dumping of refuse even though
 an existing  site  is  found to  be a  source of ground-water
 contamination.   Additional water-quality degradation of an
 aquifer from septic  tank wastes can  be halted by the in-
 stallation of collecting  sewers, but again  planning  and im-
plementation of such a system can  be slowed drastically by
 economic and political considerations.

Of course, if a well supply has been affected by a pollutant,


                              156

-------
especially if the substance is toxic, the other initial step
taken in combating the problem is the abandonment of the
well or wells and replacement with a new source, if avail-
able.  In fact, based on the inventory of case histories in
the region, the abatement procedure often ends with the aban-
donment of the water-supply source or the physical treatment
of the water pumped in order to reduce the concentration of
the pollutant to an acceptable level.  This course of action
is more or less typical due to the technical difficulties
inherent in correcting the souurce of some types of ground-
water contamination and the physical and economic problems
involved in controlling or removing the pollutant.

Nevertheless, there are two basic approaches that have been
used in the region to control the spread of or to clean up
contaminated ground water.  The first is containment and the
second is actual removal of the pollutant.

Containment involves the use of methods to protect against
the spread of degradation of water quality within the aqui-
fer already affected, to other aquifers that might be af-
fected, or to surface water bodies into which the contami-
nated ground water might discharge.  It is an approach often
used to protect existing ground-water and surface-water
users but does not help well owners whose supplies are al-
ready damaged, nor does it fully restore water quality in
the aquifer to its natural state within what might be con-
sidered a reasonable length of time.

An excellent example of containment is the widespread effort
being given to salt-water encroachment problems in the re-
gion.  This form of ground-water contamination was one of
the earliest recognized in the northeast, and such states as
New York and New Jersey began to control, many years ago,
diversion of ground water in critical areas in order to im-
pede the movement of saline water inland in heavily pumped
aquifers.  The strict control of pumping patterns through
the enforcement of state permit systems for use of ground-
water has been very successful in slowing down and, in most
cases, ending the threat of additional well supplies being
lost because of salt-water encroachment.  However, areas al-
ready affected before such controls were initiated have not
fully recovered because of the slow movement of the salt-
water front.

This slow rate of recovery is illustrated by the salt-water
encroachment problem experienced in Kings County, New York,
during the period 1903 to 1947. 41)  Salt water from estu-
aries and embayments bordering the County had moved several
miles inland and had contaminated numerous public supply and


                             157

-------
 industrial wells.   The  problem had been  created by  a  severe
 decline  in ground-water levels caused by excessive  pumping
 from both the water-table  and  deeper confined aquifers, the
 wasting  to sewers  of  all water from public  supply and many
 industrial wells/  and a substantial decrease in natural re-
 charge from precipitation  owing to extensive paving of aqui-
 fer intake areas with streets  and buildings.  A severe cut
 back in  ground-water  pumpage took place  in  1947 because of
 condemnation of a  private  water company,  which had  supplied
 as much  as 27 million gallons  per day of ground water to
 residents in central  Kings County.  This  factor combined
 with such conservation  measures as the passage of legisla-
 tion that required the  artificial recharge  of water used for
 air-conditioning and  cooling,  eventually reversed hydraulic
 gradients in most  of  the County.  Further encroachment has
 been halted, but it is  estimated that 30  to 40 years  may be
 required to flush  out the  remaining salt  water that intruded
 the aquifers.

 Containment of leakage  from industrial waste lagoons, pits,
 and basins at a site  in New Jersey is an  example of a case
 in which it was found that removal of the pollutants  from
 the aquifer would  not be feasible because of the slow move-
 ment of ground water  in the affected aquifer, even  under
 pumping conditions. 42)   in this situation, ground  water con-
 taining extremely  high concentrations of  heavy metals, in-
 cluding chromium,  zinc,  and copper, is confined to  a  30-foot
 thick zone in the water-table  aquifer.  The estimated sev-
 eral hundred million  gallons of contaminated fluid  was
 threatening to leak into deeper heavily pumped aquifers in
 the area and also was slowly moving toward  a tributary to
 the Delaware River.   Discharge of the pollutants into the
 surface stream would  have had  an adverse  effect on  its water
quality.   A series of shallow wells pumping at a rate great-
er than natural recharge to, and discharge  from, the water-
table aquifer were installed between the  source of  contami-
nation and the stream to prevent the pollutants from  reach-
ing the surface-water body.  Also, pumping  the wells has
lowered the water  level in the  shallow deposits so  that down-
ward movement of ground water  to deeper aquifers is impeded.
Some of the contaminated water is being removed and is being
treated before discharge to waste, but the well system is
primarily acting as a containment system.  The aquifer will
remain contaminated in the vicinity of the  industrial site
for many years, even  though the lagoons,  pits, and basins
that were the original source  of the problem have been lined
with concrete and  no  longer leak.

Another form of containment and its associated problems is
demonstrated by the case of a  landfill pollution problem in


                             158

-------
southern Connecticut located adjacent to Long Island
Sound. 43)   Highly mineralized ground water formed by the
leaching of soluble substances from municipal and industrial
refuse contained in the landfill is moving toward and dis-
charging into the Sound in the vicinity of a beach heavily
used for swimming.  The flow of subsurface water is being
influenced by an abnormally high water table that has been
formed within the landfill.

In order to prevent deterioration of Long Island Sound water,
further discharge of the contaminated ground water should be
prevented.   Installing a system of pumping wells to remove
the leachate or to intercept it before it reaches the Sound
is not feasible because of the fine-grained nature of the
sediments underlying the site.  The only reasonable approach
to the solution of the problem appears to be sealing off the
surface of the landfill to prevent further infiltration of
rain water.  In this way, the production of new leachate
would be reduced;  the abnormally high water table would
drop;  and the rate of discharge of contaminated ground wa-
ter to the Sound would become insignificant.  However, the
body of water already contaminated and contained within the
aquifer will remain beneath the site for many decades with
such constituents as iron and manganese considerably above
the concentrations recommended for potable waters.  Computa-
tions based on detailed drilling and water-level data show
ground water to be moving at a maximum rate of only 0.25
foot per day, and that contaminated water underlies an area
in excess of 75 acres.  Of course, sealing the surface of
the landfill will require gas venting.  Also, periodic main-
tenance of the seal itself will be needed to prevent deteri-
oration and to counteract subsidence and erosion.

Actual removal of the pollutants from the ground-water res-
ervoir has been attempted at a number of locations in the
northeast but is not practiced on a broad scale again be-
cause of technical and economic considerations.  Use of
wells drilled specifically for the purpose of pumping out
the contaminated fluid is the most common approach to re-
moval.  The water is then subjected to treatment on-site,
discharged to a sewer or nearby surface-water body, or col-
lected for reprocessing and reuse.  Existing supply wells,
to which the polluted water has migrated, have also been
pumped in an attempt to reduce the volume or concentration
of the pollutant.  A third approach has been the construc-
tion  of surface drains and ditches in order to skim the pol-
lutant off the water table.

Generally, removal has been applied only  in those  cases
where ground-water contamination represents a severe health

                              159

-------
 or economic hazard.  The presence of hydrocarbons in the
 ground-water system is an example of a severe hazard espe-
 cially in urbanized or industrialized areas where there is a
 good potential for loss of life and damage to property un-
 less as much as possible of the oil or gasoline is removed.
 Another example is the discovery of a highly toxic substance
 in ground water, such as arsenic or mercury, which is an ob-
 vious hazard to health if the contaminated fluid were to be
 left in the ground to perhaps migrate to a supply well or
 surface stream.   Attempts also have been made to remove con-
 taminated ground water if there is a distinct economic ad-
 vantage,  such as recovery of an affected community or indus-
 trial well that is vital to the water-supply system or pro-
 tection of an important aquifer.

 One of the most  difficult types of removal operation is that
 dealing with hydrocarbons.   Here,  the problem involves a two
 fluid system due to the light density and low solubility of
 the hydrocarbon.   The pollutant floats and migrates on top
 of the water table.   Drawing down  water levels and inducing
 the fluid to migrate toward a pumping well will trap only a
 portion of the hydrocarbon.   Ultimately,  as the lens thins,
 less and  less of the substance is  removed.   Thus,  in addi-
 tion to pumping  wells,  use  has been made  of ditches and
 trenches  to skim oil off the water table,  biological proc-
 esses to  break down gasoline in the ground,  and water-flood-
 ing techniques to drive solvents and other hydrocarbons to
 central collection points,  all with limited success.   In
 fact,  when raw gasoline was  detected in shallow deposits be-
 neath a business  section in  Queens County,  New York,  and al-
 ternative  methods  of removal had failed,  an entire city
 block was  excavated  from curb to curb  in  order to  physically
 expose  the  contaminated sand beds  so that  the  gasoline  could
 be  removed.  44)   Special non-ferrous tools  were  employed in
 the  digging  to eliminate the danger of sparks.

 Even when  a  pollutant can be successfully  removed  from  an
 aquifer, the  time  period involved  and  the  quantity of water
 pumped  is  usually  considerable.  For example,  two  public
 supply  wells  about  100  feet  deep tapping a  limestone  aquifer
 in  southeastern Pennsylvania were  contaminated by  wastes
 from a  tool-plating  factory,  that  had  been  discharging  into
 a sinkhole three-quarters of a mile  away.  45)  Concentra-
 tions  of hexavalent  chromium in  the  water  from the wells was
 0.35 mg/1 when the problem was discovered.   It took a period
of 2-1/2 years, pumping  at a  rate  of more than one-half mil-
 lion gallons per day, to  reduce  the  concentration  of the
contaminant to a  level  of 0.02 mg/1.   Use of the sinkhole by
the  factory had been halted  immediately.  The water pumped
from the wells during the removal  operation is treated be-

                              160

-------
fore being discharged to a stream.

In another case/ along the Delaware River in New Jersey, an
industry is pumping at an average rate of 4,025 gallons per
minute in an attempt to remove from a shallow aquifer, pollu-
tants that were moving toward existing wells. 14)  The with-
drawn contaminated water is used for process and cooling be-
fore being treated and discharged to the Delaware River.  A
detailed monitoring system is being employed to determine
how successfully the system is working and the degree to
which the pumped water will require treatment.

Any discussion of the problems associated with the control
and correction of existing ground-water contamination prob-
lems would not be complete without consideration of the high
costs involved.  The best method to illustrate the important
impact of this factor is to explore a number of case his-
tories that have come to light during the northeast investi-
gation.

As indicated in Table 25, landfills of municipal and indus-
trial wastes rank high in the number of significant occur-
rences of ground-water contamination in the region.  In one
case in southeastern New York State, litigation was brought
against a county by the U. S. Attorney because the operation
of a regional solid waste landfill did not meet the require-
ments of the 1899 Refuse Act, which prohibits discharge of
wastes without a permit into navigable interstate streams. 46)
In a court action, the County was directed to define the ex-
tent of ground-water contamination problems associated with
the landfill and to determine the environmental impact on
the river and wetlands bordering on the landfill.  The hy-
drologic, geologic, and biologic studies extended over a
period of two years.  Legal fees plus the scientific inves-
tigations amounted to more than $250,000.  This figure does
not include engineering design and other costs involved in
completing the landfill to the satisfaction of the court or
in finding, purchasing, and designing a new site for refuse
disposal.

In another landfill case, in Delaware, solution of a ground-
water contamination problem may cost upward of $2,000,000.
Leachate generated by the landfill is moving through the af-
fected aquifer toward two large well fields, one owned by a
chemical company and the other by a private water company,
which has already reduced its pumpage significantly in order
to slow down the movement of the contaminant.  A line of
high capacity wells is being installed for the capture of
the leachate, which will require treatment after removal
from the ground.  The surface of the landfill may be re-
                             161

-------
 graded in  an attempt to prevent infiltration of  rainwater
 into the refuse.   The mass  of  solid waste  measures  1.0  mile
 by 0.1 mile  by 30  feet thick.   The  site  had  been abandoned
 for four years before contamination was  detected in a pri-
 vate well  650 feet from the landfill.  48)

 In a third case, located in western Connecticut,  a  landfill
 had been operated  by a town for many years in what  was  con-
 sidered a  remote area.   As  population  increased  in  this
 suburb, new  housing developments encroached  on the  landfill
 site.   The town has no central  water-supply  system,  and
 homes  are  supplied by domestic  wells.  Ultimately,  about 50
 such wells for a new housing development were drilled adja-
 cent to the  landfill into an existing  zone of contaminated
 ground water contained in the crystalline  bedrock aquifer on
 which  te landfill  is situated.   The aquifer  had  been contam-
 inated over  the years  by leachate moving through  the refuse
 and into the water-bearing  bedrock  fractures tapped by  the
 new wells.

 Immediate  containment  or removal of the  pollutants  so that
 the home owners can continue using  their wells does  not ap-
 pear to be technically  feasible.  Instead, the town  must de-
 velop  a community  supply off-site and  pipe potable water to
 the affected homes.  The capital cost  alone  for this utility
 is  estimated to be  about $500,000 with an  annual  carrying
 cost of $55,000. 49)

 Highway deicing salts  are another widespread source  of  con-
 tamination in  the northeast  and the  yearly rate of  increase
 in  the number  of well  supplies  affected  is rising.   In
 several New  England States, the problem  has  become  routine
 enough to  actually  budget each  year  an amount of  money  to be
 spent  in replacing  wells  adversely  affected  by highway  salts.
 For example,  New Hampshire allotted  $100,000  in 1973 to the
 Department of  Public Works and  Highways  to provide relief to
 land owners who had their water supplies damaged  by  state
 operations of  all types.  Most  of this money  has  been used
 to  drill replacement wells for  road-salt damaged  water  sup-
 plies.  The  1974 budget  is estimated at  $200,000. 50)   Maine
 has  a  system similar to  New Hampshire's  and  spent more  than
 $46,000 during  the  fiscal year  July  1, 1971  to June  30, 1972
 settling claims almost exclusively arising out of wells that
 had  been contaminated by highway  salts.  51)

Finally, some  costs  involved in solving ground-water contam-
 ination problems are related to treating the  affected water
 in  order to  reduce  the concentration of the  substance to ac-
ceptable levels.  Water  supplies  in  some portions of Nassau
County, New York, exceed the U.  S. Public Health  limit  for

                             162

-------
nitrate content (as N) of 10 mg/1.  This regional ground-
water contamination problem has been related primarily to
septic tank and cesspool effluent, fertilizers, and animal
wastes.  In one situation, the Garden City Park Water Dis-
trict was required to reduce its water-supply capacity by 60
percent because of the forced shutdown of nitrate contami-
nated wells.  Blending of water from different wells and ex-
tending existing wells into deeper aquifers were ruled out
as possible solutions to the problem, and the District was
forced to explore the possibility of treatment.

After considerable experimentation and research, an ion-
exchange process, originally developed to demineralize in-
dustrial process water, was recommended.  A treatment system
was devised and the plant constructed at a total cost of
about $400,000.  An average of 1,200 gallons per minute of
water containing more than 20 mg/1 nitrate  (as N) is handled
in the treatment system. 52)

Summary

The various factors discussed above should indicate the
cause for concern regarding ground-water contamination and
the need for more research, control, and education to help
prevent new occurrences and to aid in correcting existing
problems.  This investigation revealed the fortunate cir-
cumstance that there are a few dedicated technicians on dif-
ferent levels of government in each of the states working
toward educating the public on the importance of protecting
ground-water quality, in addition to developing guidelines
and manuals to prevent practices that might adversely affect
this underground water source.  However, activities involved
in the protection and monitoring of ground-water quality,
with a few notable exceptions that will be discussed later
in this report, are too splintered among various agencies to
be effective.  In addition, the agencies are hindered by
lack of sufficient budget to staff properly and to carry out
the functions necessary for ground-water management programs
to be successful.

In the following portions of this section, key sources of
contamination will be explored in greater detail.  By this
means, it is hoped that the principal problem areas, which
require the greatest  effort, can be illustrated.  A review
of case histories on  ground-water quality degradation pro-
vides the best means  for understanding the nature of the
problem in the northeast.  In this regard, selected instances
of contamination are  tabulated.  Where possible, locations
and references are provided for each of the cases included.
However, where future litigation may be involved, for exam-

                             163

-------
 pie,  and the data shown does not appear in the literature,
 the  location and reference may not be listed in order  to
 respect  the  confidential nature of the information.

 SEPTIC TANKS AND CESSPOOLS

 Certainly one of the  most significant sources of ground-
 water contamination in  the northeast  is discharge from
 septic tanks.   A large  number of cesspools are still in use,
 and  privies  or direct discharges to surface waters can still
 be found in  some rural  areas.   However,  the septic-tank,
 tile-field system has been almost universally adopted
 throughout the region to provide a means for disposing of
 wastes from  homes, stores,  laundries,  small office buildings,
 hospitals, and industries in areas where community sewer
 systems  are  not available.   The major growth in septic-tank
 use  has  taken  place since the  second  World War due to  the
 explosive  development of suburban areas  on the fringes of
 the  major  cities.

 In the 11  states  of the  study  region,  approximately 12 mil-
 lion  people  or 23 percent of the total population is served
 by individual  home waste water treatment systems.  28)  As-
 suming an  average domestic water-use  of  40 to 80  gallons per
 day per  capita,  as much  as one-half to one billion gallons
 of raw sewage  is discharged  from residences directly into
 the  subsurface  each day  in the study  region.   To  this  figure
 must  be  added  the millions of  gallons  per  day discharged to
 the ground from commercial and industrial  septic  tanks.

 The complete septic-tank and tile-field  system consists of
 three basic  components.   The  first is  the  septic  tank  itself,
 which is a water tight,  non-corrosive,  and covered recepta-
 cle designed to remove solids  by settlement and to trap and
 store scum and  sludge.   The  second is  the  distribution box,
 which is needed to insure equal  distribution  of effluent to
 the several  lateral lines of the tile  field.   The  third com-
 ponent is the  soil absorption  system  or  tile-field.  This
 consists of  a  series  of  pipes,  usually made of perforated
 orangeburg fiber or plastic  material,  the  purpose  of which
 is to distribute as evenly as  possible the sewage  effluent
 over  an  area of  soil  large enough  to  absorb it.   The distri-
 bution lines are normally.laid in  trenches, backfilled with
 filter material consisting of  washed  gravel,  crushed stone,
 or slag.   Figure  29 shows the  layout  of  a  typical  septic-
 tank, soil-absorption system.

Another  device  commonly  used in  conjunction with or instead
 of the septic  tank system for  discharging  effluent into the
 soil  is  the  cesspool.  It is a large buried chamber, which
                             164

-------
            PRODUCTION
                                                         DISPOSAL

                                               EVAPOTRANSPIRATION

Figure 29.  Disposal of household wastes through a conventional septic tank-soil
                                  absorption system
                                     165

-------
is walled up with  a  porous material  such  as precast perfo-
rated concrete rings or  concrete blocks.  The size of the
chamber varies according to hydraulic  loading and other de-
sign considerations.

It is a generally  accepted fact that as much as  300 mg/1 of
total dissolved  solids are added to  water by domestic use,
and, thus,  the effluent  from  septic  tanks can increase the
concentration of minerals in  ground  water.  Table 27 shows
the range of mineral pickup in domestic sewage.  Under nor-
mal conditions of  soil pH, efficient removal of  phosphates
can take place,  but  chlorides, nitrates,  sulfates, and bi-
carbonates  can enter and move freely within a ground-water
body.  Bacteria  and  viruses are normally  removed by the soil
system, but, under conditions favorable for their survival,
can reach the water  table and can travel  significant dis-
tances through an aquifer.  Some other pollutants that have
been found  associated with septic tanks include  synthetic
detergents, excessive chlorides from water softener regen-
eration, and a number of toxic and non-toxic constituents in
special cases where  industrial wastes have been  discharged
to a septic tank.

The percolation  test  is  used as the  principal deciding fac-
tor on whether or not septic tanks would  be acceptable for
particular  sites.  This  test measures the rate of decline of
the level of clear water in a series of wetted holes.  The
faster the water dissapates in the hole,  the greater the as-
sumed performance of the proposed septic  system.  However,
there are a number of limitations on this method.  Clear wa-
ter and sewage effluent  can react quite differently in soil.
More important to ground-water contamination, coarse-grained
deposits that will perform the best  in percolation tests can
be the least effective in removing bacteria and  nutrients.
Finally, reliance on percolation tests will not  indicate
long-term effects on ground-water quality from various den-
sities of septic tank installations.

Case Histories

Inadequate experience and lack of sound scientific planning
on the use of septic  tank disposal systems have  led to a
number of regional ground-water quality problems in the
northeast.  In addition  to regional  problems, there are in-
dividual cases of water  from domestic wells being contami-
nated by on-site waste disposal systems.  This latter number
probably ranks in the thousands.  Discussions on ground-
water contamination held during this investigation with
county and municipal health authorities throughout the re-
gion invariably  included a number of references  to private

                             166

-------
Table 27.  NORMAL RANGE OF MINERAL PICKUP IN DOMESTIC SEWAGE.  54)



Mineral                                              Mineral range (mg/l)


Dissolved solids                                          100   - 300


Boron (B)                                                0.1 -   0.4


Sodium (Na)                                             40-70


Potassium (K)                                             7-15


Magnesium (Mg)                                          3-6


Calcium (Ca)                                             6-16


Total Nitrogen (NOg)                                    20-40
                                                             1C

Phosphate (PO4)                                         20   -  40


Sulfate (SO4)                                             15   -  30


Chloride (Cl)                                            20   -  50


Alkalinity (as CaCO%)                                    100   - 150
                                 167

-------
 wells condemned because of pollutants from septic-tank ef-
 fluent or because of the failure of septic-tank systems.

 A few of the numerous studies carried out in the region have
 been selected for discussion below.  They have been chosen
 on the basis that they might be indicative of the varied
 conditions under which ground-water contamination from this
 source can take place and that they would be most illustra-
 tive of the effects of septic tanks on ground-water quality.
 Unfortunately,  it is difficult to prepare a table based on
 the results of  these investigations because the methodolo-
 gies used and parameters measured differ so greatly.

 Eastern and Western Connecticut -

 A number of studies carried out in the region point up the
 need for a broad technical approach for determining the
 feasibility of  using on-site disposal systems rather than
 relying on an engineering analysis of whether or not the
 soil underlying a particular piece of property will absorb
 septic tank effluent at an acceptable rate.   For example,
 Dr.  Thomas L. Holzer of the University of Connecticut points
 out that the relatively small amount of natural ground-water
 recharge available in much of the crystalline rock regions
 of eastern and  western Connecticut is the most important
 limiting factor to septic-tank use.  55)   in  nonurban por-
 tions  of these  areas,  on-site disposal systems and individ-
 ual  domestic wells are located on the same lot.   Only seven
 inches or less  of the average annual precipitation of 45
 inches infiltrates into the ground where crystalline rock  is
 overlain by relatively thin glacial till.   In one year,  a
 home may easily use and discharge to the septic  tank the
 equivalent of 3.5 inches of water spread over an acre.   "As
 development in  the nonurban areas increases,  recycling  of
 liquid waste will become an inevitable fact  of life".   In
 other  words, unless low density zoning is  enforced,  there
 simply may not  be enough natural  recharge  to counteract the
 build-up of nutrients  in the aquifers  tapped by  domestic
 water  wells.

 Holzer stresses that the small  capability  of fractured  crys-
 talline  bedrock to renovate waste water  and  the  thinness of
 the  overlying soil zone indicate  the precariousness  of  de-
 velopment  in nonurban  areas  unless  the hydrogeology  of  the
 aquifer  systems  is  clearly  understood.

 Boston Suburban Area, Massachusetts  -

Another  study in  the Glaciated Appalachian Region  of partic-


                              168

-------
lar interest and mentioned previously was carried out by the
U. S. Geological Survey in the Ipswich and Shawsheen River
Basins of Massachusetts, north of Boston. 21)   The investiga-
tors concluded that "development of housing beyond the reach
of the municipal sewer systems of metropolitan areas has
lowered the quality of the environment in many of the (hous-
ing) developments and has created health hazards in others".
Using chloride and specific conductance as tracers and cor-
recting for highway deicing salts which are the only mate-
rials other than septic tank discharge contributing signifi-
cantly to water-quality degradation, the investigators were
able to develop a correlation between the relationship of
housing density to residual conductance and accretion of dis-
solved solids in the baseflow of streams  (see Figure 30).

Seventeen small drainage basins, all but one less than one
square mile in area, were selected for study.  All basins
are served by public water supplies, but none have municipal
sewer systems, and individual houses are served by on-site
disposal systems.  Housing density ranges from zero to 900
units per square mile.  The concentration of chloride is
about 50 mg/1 higher in the septic tank effluent than in the
tap water entering the home.  Septic tank flow per house is
estimated to be 200 gallons per day.  The results of the in-
vestigation indicated that the reduction of mineral concen-
trations during travel of the septic tank effluent through
the soil and bedrock aquifer is slight, and most dissolved
solids from septic tank systems reach the streams.

Long Island, New York -

A comprehensive study involving intensive field research of
the effects on ground-water quality of synthetic detergents
and other constituents in effluent discharged by typical in-
dividual sewage disposal systems has been carried out in
Long Island, New York, located in the Coastal Plain Region
of the study area. 56)  six home sites were selected for ob-
servation in Nassau and Suffolk Counties, monitoring wells
were installed, and the home owners agreed to fully partici-
pate in the project and cooperate in the use of several
types of detergents.  Based on the results of the project,
which was carried out over a period of about five years, the
investigators concluded that individual subsurface disposal
systems provide insufficient treatment of wastes.  This con-
dition allows objectionable concentrations of biological and
chemical sewage constituents to reach the water table.  Sep-
tic tanks in combination with leaching dry wells and septic
tanks in combination with leaching tile-fields, do not pro-
vide significant improvement in the effluent quality com-
pared to single cesspools.  The investigators also found

                             169

-------
                                                             -; 140
          12345678
             HOUSING  DENSITY, IN  HUNDREDS  OF HOUSES
                         PER SQUARE  MILE
10
Figure 30.  Relationship of housing density to residual conductance and
               accretion of dissolved solids in base flow of streams,
              Ipswich and Shawsheen river basins, Massachusetts   '
                            170

-------
that viable bacteria can pass through the unsaturated soils,
can reach the water table, and can travel downgradient as
part of the waste stream in the aquifer.

In an investigation of nitrate in ground water and streams
in southern Nassau County, the U. S.  Geological Survey con-
cluded that the two chief sources of  nitrate contamination
of major aquifers in a 180-square mile area were infiltrated
sewage (mostly from several hundred thousand active or aban-
doned cesspools and septic tanks) and leachate from chemical
fertilizers. 5?)  Nitrate content of  water in the shallow
glacial aquifer, expressed as nitrate ion, averaged 30 mg/1
and in seven places equaled or exceeded 100 mg/1.  Nitrate
enriched water has also penetrated hundreds of feet into the
underlying artesian unconsolidated aquifer.  The nitrate
content of water from 16 public supply wells screened in
this deeper aquifer zone ranged from 45 to 94 mg/1.

Part of the Nassau County study area  was sewered between
1952 and 1964.  Nitrate content of ground-water fed streams
averaged 11 and 25 mg/1 in the sewered and unsewered areas
respectively in 1970.  The investigators concluded that im-
provement in the quality of chemically deteriorated ground
water after construction of sanitary sewers is a slow proc-
ess that may require several decades  for effective natural
dilution and discharge of most of the residual nitrate in
the ground water.  Also, a nitrate front in the deeper arte-
sian aquifer, defined as the zone of contact between nitrate-
enriched water and natural water, is  moving vertically into
unaffected portions of the aquifer at a rate of 5 to 25 feet
per year, and horizontally at a rate of 130 feet per year.
Tongues of nitrate-enriched ground water may be moving
faster than the average estimated rate in local areas due to
heavy pumping from wells.

Another investigation carried out in the same area of Nassau
County during the period 1966 to 1970 by the U. S. Geologi-
cal Survey involved a determination of the distribution of
MBAS  (methylene blue active substances - a detergent con-
stituent) in ground water. 5^)  MBAS was found to be widely
distributed in water from the shallow glacial aquifer, but
relatively few analyses of well water showed concentrations
greater than the U. S. Public Health recommended limit of
0.5 mg/1.  Presence of MBAS in the deeper artesian aquifer
is not a significant problem.  Also,  a slight downward trend
in MBAS content during the five-year study period was indi-
cated and may be due to natural dilution after a regional
drought of the early 1960's and the introduction of a more
biodegradable detergent in 1966.  In the sewered area, the
presence of residual MBAS in the glacial aquifer, after  10

                             171

-------
to 20 years of public sewer operation, may be related to a
combination of factors including continued infiltration of
effluent from residual active or abandoned cesspools and
septic tanks, leakage from sanitary sewers, and the slow
rate of recovery in the quality of chemically deteriorated
ground water after sewering.

State of Delaware -

In a 1972 report, John C. Miller of the Delaware Geological
Survey states, "inspection of water analyses on file at the
Delaware Geological Survey revealed that 25 percent of the
shallow  (less than 50 feet deep) wells in the state yield
water with nitrate levels above 20 mg/1". 59)  This indica-
tion of the potential for widespread ground-water contami-
nation has led to an evaluation of some of the principal
sources of nitrate enrichment of ground water in the state,
including septic tank discharges.

Two suburbanized areas in the coastal plain were chosen for
analysis of potential problems of ground-water quality deg-
radation due to septic tanks. 60)   The first area was se-
lected on the basis that it is characterized by an extremely
high water table and poorly-drained soils.  In addition,
there had been numerous reports of overflowing septic-tank
systems during rainy periods.  For comparison purposes, the
second area selected is underlain by deep, well-drained
soils on uplands.  In both areas, homes are situated on one-
quarter to one-half acre lots, each of which has its own
septic tank and shallow well-water system.

The results of the study showed that in the first area of
poorly drained soils, nitrate (as N03) levels averaged 6.9
to 11 mg/1 during the period of sampling.  A number of wells
were contaminated by coliform bacteria.  In the second area
of well drained soils, nitrate content ranged from 22 to
136 mg/1, and concentrations in water from many wells was
above the recommended U. S. Public Health limit of 45 mg/1.
No wells were found to be contaminated with coliform bac-
teria.

The State investigators concluded that "the standard percola-
tion test is not a suitable means for determination of the
acceptability of a site for septic-tank effluent".  Percola-
tion tests in the first area were conducted during dry peri-
ods, and the favorable results led to installation of septic
tanks.  After installation, the systems overflowed during
wet periods, and bacteriological contamination of domestic
wells took place because of the introduction of sewage ef-
fluent from the land surface around well casings.  On the

                             172

-------
other hand,_ the ^ movement of the effluent through the fine
soils has minimized the build-up of nitrate concentrations
in the ground water.  In the second area, the physical opera-
tion of the septic tanks has been successful because of the
permeable soil sediments, which also apparently filtered out
pathogenic organisms.  However, nitrate contamination of
ground water in the area is severe because of the favorable
environment for oxidation of nitrogen compounds and rapid
movement of septic tank and tile-field effluent to the water
table.

Montgomery County, Maryland -

The Montgomery County Health Department has been issuing
permits for septic tanks since 1945 and for wells since 1960.
By 1968, this mostly suburban area had an estimated 15,000
to 16,000 wells and 16,500 to 17,500 septic systems.  In or-
der to determine the status of the safety of these systems,
the Health Department conducted a number of housing surveys
in selected portions of the county.  Some of the results are
of interest.  61)

Based on these studies, it was estimated that more than
1,000 of the approximately 17,000 septic tanks were malfunc-
tioning or had failed.  About 800 wells, more than five per-
cent of the total for the county, were rated as totally un-
fit for drinking water because they are yielding ground
water contaminated from sewage effluent.  In 1964, the
county had passed an ordinance requiring grouting all new or
reconstructed wells in order to seal the annular space be-
tween the outer well casing and soil.  Basically, the code
called for casing and grouting the wells to a depth of 40
feet or into solid rock.  It was concluded that this measure
had not been effective in protecting the safety of well sup-
plies.  Contamination of the aquifer from septic tank ef-
fluent eventually led to contamination of the water yielded
from a well tapping the aquifer, whether or not the well was
grouted.  The study revealed that the most probable cause of
contaminated well supplies was extensive use of underground
disposal systems in areas underlain by fractured porous
rocks that allowed free passage of sewage effluent to con-
siderable depths in the aquifer.  Also, the information ob-
tained indicated that the average life of a septic system
using current design standards may be as short as eight to
ten years.

Northern New England Recreational Areas -

The development of recreational areas in the mountainous re-
                             173

-------
 gions  of the  northern tier of New England  States,  namely
 Vermont, New  Hampshire,  and Maine,  has  been  of  concern  to
 health authorities  because of the unsuitability of some of
 these  areas for  installation of  either  high-capacity  single
 septic tank systems serving central facilities  such as  mo-
 tels,  lodges,  and condominiums or the proliferation of  indi-
 vidual systems serving a growing number of vacation homes.
 Topography is  rugged,  soils are  thin, and  the bedrock aqui-
 fer  is highly  susceptible to the intrusion and  transmission
 of pollutants.

 These  conditions are  prevalent at one ski  area,  where
 studies were conducted on the effect of large quantities of
 sewage effluent being discharged to a septic tank  and leach-
 ing  field in shallow  fill deposits  overlying crystalline
 bedrock.  62)   Laboratory tests were conducted on water  sam-
 ples taken from test  pits and streams draining  the area in
 which  the leaching  field was located.   They  indicated that
 certain constituents  considered  to  have an adverse effect on
 public health were  not being reduced to safe levels within
 distances up to 275 feet away.   Phosphate  and COD  values up
 to 90  feet away were not appreciably different  from those
 near the  field.  It appeared that the sewage effluent was
 moving laterally through the soil and was  entering surface
 streams  and perhaps fractures  in the bedrock.   In  order to
 alleviate the problem, pretreatment was subsequently  pro-
 vided  for the sewage effluent  before discharge  to  the septic
 tank system.

 Miscellaneous Effects  of Septic  Tank Discharges  -

 As mentioned previously,  discharge  into septic  tanks  of
 toxic  chemicals or  salts  used  for regenerating water  soften-
 ers can  lead to specialized  problems of ground-water  contam-
 ination  other than  those  associated with typical household
 wastes.   The use of water softeners  in  Connecticut, for ex-
 ample,  and the discharge  of  salts used  for regeneration of
 home units has been linked  to  high  chloride concentrations
 in North  Stamford,  although  it was  concluded that  the appli-
 cation  of deicing salts  on  roadways  was  the most significant
 problem.  63)   it was estimated that, based on regeneration
 practice  in the area,  as  much  as  2,000  pounds of salt are
 discharged to a septic tank  each  year from a home with  a
water  softener.

Two noteworthy cases of  ground-water contamination in Rhode
 Island may be indicative  of  specialized problems in the re-
gion related to septic tanks and  cesspools. 64)   The  first
involved  contamination of domestic well water with metal
                             174

-------
plating wastes, which were being discharged to a septic sys-
tem from a private residence.  The owner had been running
the plating operation in his home, and by the time the con-
tamination problem was discovered, the concentration of
nickel in the well water was 11.8 mg/1 and copper 2.28 mg/1.
In the second case, acid, commonly used by cesspool and sep-
tic tank owners to improve the operation of the system, mi-
grated to the domestic well on the same property and notice-
ably affected the taste of the well water.

Future Trends

In spite of their potential for ground-water contamination,
millions of septic tanks will continue to be used in the re-
gion, and their overall numbers may increase over at least
the next decade.  The reasons for this situation include:

1.  The lack of other acceptable alternatives for domestic
    waste disposal in unsewered areas where septic tanks are
    correctly installed and adequately maintained and where
    geologic and hydrologic conditions are favorable.

2.  Existing limitations on local, state, and federal bud-
    gets which prevent installation of public sewers to meet
    waste disposal needs of expanding suburban communities.

3.  New environmental criteria calling for the upgrading of
    community sewage treatment plants.  This slows down the
    expansion of these central systems into unsewered areas.

4.  The continued resistence by residents in many parts of
    the study region to approve the large expenditures neces-
    sary for conversion from complete dependence upon on-
    site disposal systems to sewered communities.

5.  The long time period required for a public system to be-
    come fully operational, even in areas where the density
    of housing and problems of ground-water contamination
    have justified to all concerned the need for conversion
    to collecting sewers and treatment plants.

Therefore, the need for improved methods of design and con-
trol of septic tank installations is obvious.  A number of
variations of traditional on-site disposal systems have been
proposed or are being used in various parts of the United
States.  One example is the aerobic tank in which air is in-
troduced and bubbled through the sewage to maintain aerobic
rather than septic conditions for more efficient treatment
of the waste.  Some of these units also have mechanical  fil-
ters.  Another approach is the use of incinerator toilets  or

                             175

-------
 privies  that  have  been  proposed  for  areas particularly  sen-
 sitive to  contamination from septic  tanks,  such as  lakefront
 lots.  The principal  drawback to these  systems for  single
 homes is the  need  for periodic mechanical maintenance and
 the  comparatively  high  initial cost.  Artificial mounds of
 soil or  sand  and gravel have been employed  in areas where
 natural  conditions are  not  suitable  for an  underground  sep-
 tic  tank and  tile  field.  However, the  entire system, in-
 cluding  the mound  itself and leaching field, must be design-
 ed very  carefully.

 Probably the  best  approach  to limiting  future problems  is
 better governmental control and  planning.   Zoning and land-
 use  planning  in areas where septic tanks will be required
 should be  based on a  thorough understanding of regional
 variations in topography, soils,  aquifer characteristics,
 and  recharge  and discharge  relationships involving  ground
 water and  surface  water.  An initial study  in a particular
 region leading to  recommendations on planning procedures
 and  guidelines for on-site  waste  disposal facilities will be
 expensive  and create political controversey but would be the
 most environmentally  sound  approach and could prevent errors
 that might be even more  costly and controversial over the
 long term.  Research  is  needed to develop the tools that can
 be used  for decision making related to  septic-tank  feasi-
 bility and density.   In  this  way, ground-water quality  can
 be better  protected.

 Some methods  have  been developed  and applied to septic-tank
 usage that illustrate the type of approach  recommended  above.
 The  Water  Resources Center  of the University of Delaware,
 supported  by  funds from  the  U. S. Department of Interior,
 Office of  Water Resources Research, has used a computerized
 technique  to  categorize  land areas in the Christina River
 Basin into site classes  on  the basis of a common relation-
 ship to  the water  regimen.  65)  A site's vulnerability to
 development is indicated by  the  cost of the measures neces-
 sary to  protect water resources while still permitting de-
 velopment.  One of the parameters used  in the study was con-
 trol of  pollution  from  septic tanks.  Sites were classified,
 for  example,  according to those  areas where septic  tanks
 should be  banned on less than one acre, where septic tanks
would be allowed only if public water supply was available,
 and where  only single home  aerobic sewage-treatment systems
would be permitted.

Another  approach employed in  Connecticut by a Geology-Soil
Task Force, consisting of representatives from state and
 federal  agencies,  involves a  master-mapping technique in
which as much natural resource information  as possible is
                             176

-------
applied to a land-use problem, such as where to allow a par-
ticular density of septic tanks. 66)   Soil characteristics,
water-table elevations, rock types, slopes, etc., are mapped
separately for the particular region in question.  Guide-
lines, such as required depth to the water table, are formu-
lated.  These determine whether a particular piece of prop-
erty or group of properties would be acceptable for the pro-
posed density of septic tanks.  The resource data for the
region is collated on a single map, and those areas that
meet all of the parameters set by the management guidelines
can then be considered for additional on-site investigation.

Of course, codes, regulations and permit requirements are
already in force in much of the region on a state and local
basis.  Strengthening the enforcement of proper sanitation
practices undoubtedly would help to reduce the number of
ground-water contamination problems.  The need for this type
of action plus educational programs for installers, devel-
opers, public officials, and planners was pointed out in a
survey of septic-tank system installation practices in Con-
necticut. 67)  This study by the Agricultural Engineering
Department at the University of Connecticut showed that a
wide variety of specifications were being followed by in-
stallers in the same general area including publications
from the Federal Housing Administration, State Health Depart-
ment, and U. S. Public Health Service;  recommendations by
local health officers;  and instructions from consulting en-
gineers.

The ban of certain types of pollutants that are discharged
into septic tanks has also been tried in the region as a
means for ground-water quality protection.  The prime exam-
ple is the Suffolk County, New York, ordinance passed in
November of 1970 which prohibits the sale  (but not the use)
of laundry and manual dishwashing detergents containing
alkyl benzine sulfonate  (ABS), linear alkylate sulfonate
(LAS), alcohol sulfate, and any other surface active agent
which can be detected by the methylene blue  (MBAS) test pro-
cedure.  In effect, the ban removed virtually every brand-
name detergent, all of them biodegradable, from stores in
the County.  Justification for the ban was linked directly
to the need to protect the quality of ground water from fur-
ther degradation by septic-tank effluent.  This action came
about only a few years after the detergent industry had
spent in excess of $150 million to make its products bio-
degradable. 68)

Controversy over septic tanks, and their effects on ground-
water quality will continue in the region  for the foresee-
able  future.  Hopefully, out of this controversy will come  a


                              177

-------
 more scientific and technical approach to the design  and  use
 of on-site waste disposal systems resulting in less of  an
 impact of septic systems on ground-water quality.

 BURIED PIPELINES AND STORAGE TANKS

 Pollutants from leaky and ruptured buried pipes,  sewer  lines,
 and storage tanks can directly enter  and contaminate  aqui-
 fers.   Within  the study region,  the principal pollutants
 from these sources are sewage, storm  water,  and petroleum
 products.   Chemicals used in industrial  processes have  also
 been reported  in a number of ground-water contamination'
 cases.

 Exfiltration and infiltration occurring  in sanitary and
 storm sewers is a recognized engineering phenomenon.  Where
 the system originally was poorly designed and improperly  in-
 stalled or where the pipelines are old and in disrepair,
 leakage of substantial quantities  of  poor-quality water into
 the soil system can take place,  eventually leading to con-
 tamination of  an aquifer.   Storm sewers  are  especially  sub-
 ject to exfiltration because joints are  normally not  com-
 pletely sealed against leakage.  A comparison of the  levels
 of selected constituents in street runoff and raw sanitary
 sewage  is  given in Table 28.   As indicated by the table,  the
 pollutional loads  from both sources can  be substantial.
 Thousands  of miles of sanitary and storm sewers exist in  the
 study region.

 Petroleum  and  petroleum products are  contained in hundreds
 of miles of transmission pipelines throughout the region  and
 in thousands of home  fuel  and gasoline station tanks.   In-
 terstate and some  intrastate  transportation  pipelines are
 regulated,  but they are  still subject  to accidental rupture
 and external corrosion.

 Details  on the number of cases of  ground-water contamination
 due  to  leakage from buried tanks and pipes that occur in  the
 region  each year  are  not available.  However,  Maryland  alone
 had  over 60  cases  recorded by county health  departments and
 the Maryland Department  of Water Resources in 1969-1970.  70)
 The  Pennsylvania Department of Environmental  Resources  esti-
mates that 2,600 new  or  replacement subsurface  storage  tanks
 are buried in  the  ground in that state each year. 71)    if
 those replaced have  failed,  then the product  originally con-
 tained had been  lost  to  the  ground.

 If a leak  of gasoline, oil, or a chemical  fluid occurs  in
the soil zone  above  the  water table, the  liquid pollutant
will either  remain  in the  vicinity  of the  leak, move  within

                              178

-------
Table 28.  COMPARISON OF POLLUTIONAL LOADS FROM HYPOTHETICAL
          CITY-STREET RUNOFF VERSUS RAW SANITARY SEWAGE.  69)
Settable +
Suspended Solids "'
BODb)
CODb)
Total Col i form
Contaminant
loads in sur-
face runoff
from streets
(Ib/hr) a)
560,000
5,600
13,000
40 x 1012
Raw sanitary
(mg/l)
300
250
270
250 x 106
sewage
(Ib/hr) c)
1,300
1,100
1,200
4.6 x 1014
Bacteria
Organisms/hour      Organisms/liter     Organisms/hour
Kjeldahl Nitrogen b)
Phosphates
Zinc
Copper
Lead
Nickel
Mercury
Chromium
880
440
260
80
230
20
29
44
50
12
0.20
0.04
0.03
0.01
0.07
0.04
210
50
0.84
0.17
0.13
0.042
0.27
0.17
a) During first hour of a storm.

b) Weighted averages by land use, all others from numerical mean.

c) Loading discharged to receiving waters (average hourly rate).
                                 179

-------
 the backfill in the trench or excavation, or migrate down-
 ward through the natural soil under the influence of gravity.
 The actual route and rate of travel taken by the pollutant
 depends on several factors including the volume of fluid re-
 leased, the comparative permeabilities of the soil materials
 in the vicinity of the excavation,  and the density, viscos-
 ity, and miscibility of the liquid.  If enough of the fluid
 enters the soil system so that it is not completely exhaust-
 ed by adsorption on soil particles, the pollutant eventually
 may reach the water table and if miscible with water, extend
 into the saturated zone.  Subsequent rainfall can drive  the
 pollutants that are coating the soil particles down to the
 saturated zone and add to the contamination of the water-
 table aquifer.

 The above is a very simplified description of the mechanisms
 involved in contamination from buried tanks and pipelines.
 Considerable technical literature has been written on the
 most common type of pollutant,  petroleum products.   Espe-
 cially valuable for general reference are those that de-
 scribe research carried out in Europe.  10* 72 through 75)

 Case Histories

 So few case histories  involving leakage of contaminants  from
 buried tanks  and pipelines  have appeared in United States
 literature  that it  is  worthwhile to describe in some detail
 selected occurrences that have  been recorded in the north-
 east.   These  are outlined below.

 Kings  County,  New York -

 Leakage from sewers may be  a  principal  source of the nitrate
 and total nitrogen  in  the ground water  of Kings County,  Long
 Island,  New York, according to  a recent study by the U.  S.
 Geological  Survey.  76)   At  the  present  time,  the County  is
 served by a dense network of  sanitary and storm sewers;
 about  1,700 miles of common sewer lines as of 1962.   The
 area  is highly urbanized, and other potential sources of
 nitrate contamination  such  as agricultural activities and
 domestic water-disposal systems  are lacking.   Sewerage began
 in  the  northwestern part of the  County  in about 1850,  and
 1,300 miles of the  sewer lines  are  more than  40 years old.
Total  leakage  is  estimated  to be  very high and actually  may
represent a  significant source  of artificial  recharge to the
ground-water  system in the  county.   Total  nitrogen  content
in water from  key monitoring wells  in the  unconsolidated
water-table aquifer ranges  from  about five  mg/1 to  30 mg/1.
                             180

-------
Mechanicsburg, Pennsylvania -

The Ground-Water Section, Division of Water Quality, of the
Pennsylvania Department of Environmental Resources has con-
ducted two interesting investigations of pipeline leaks in
the Mechanicsburg area of Hampden Township, Cumberland
County.  The first involves a sewage-line break and the
second, leakage of gasoline from petroleum transmission
pipelines.  The area is located in a gently rolling lime-
stone valley with approximately 10 feet of relief.  The wa-
ter table is very near the land surface and is extremely re-
sponsive to rainfall conditions.  Ground water is contained
in joints, fractures, and solution cavities of the limestone
aquifer.

Sewer line break - 77)

In September 1968, the operator of a sewage treatment plant
in the area noted a drop in the normal flow entering the
facility.  Investigation revealed that about 350,000 gallons
of raw sewage had apparently been lost to the limestone
aquifer through a rupture in a 15-inch diameter trunk line.
The break in the sewer was attributed to an abnormally high
rainfall, which had led to an increase in hydraulic pressure
on the line.

Water samples were collected from private and commerical
wells in the area and four pounds of Fluorescein dye was in-
jected into the ground at the location of the break to serve
as a tracer.  Two days after the dye was injected,  it was
detected in a well three-quarters of a mile northwest of the
break.  Three to five days after the break had occurred, dye
was detected in an additional 12 wells approximately one and
one-half miles northwest.  In many of the wells in which dye
was detected, coliform bacteria counts were high on the
first day of sampling but decreased with time, indicating
that the main body of the raw sewage had passed through the
area.  In the portion of the aquifer affected by the pollu-
tant, individual wells yielded water containing coliform
organisms with a median value as high as 163 per 100 ml.
Repairs to the sewer  line were  carried out and about 50
pounds of chlorine were  flushed into the break site.

Gasoline pipeline break  - 16,78)

In February 1969, a  local businessman drilling an  illegal
drainage well for a  parking  lot discovered gasoline in the
ground water underlying  his  property.  The site  is  located
near three petroleum product storage tank  farms  and two
product transmission lines.  After being informed  of  the


                              181

-------
 condition,  one of the pipeline companies pumped 55,000 gal-
 lons of gasoline out of the well in about one month.

 In June 1969,  the State Highway Department encountered gaso-
 line in borings for bridge foundations.   Further investiga-
 tion,  including the drilling of observation and gasoline re-
 moval  wells and the use of a truck-mounted gas chromatograph
 which  analyzed soil vapor samples taken  from the upper two
 feet of the soil mantle,  revealed that a layer of gasoline
 was floating on the water table in an area of about one-
 third  square mile.   The thickness of the gasoline layer was
 found  to be as much as seven feet.  Initial removal rate of
 gasoline was as high as 1,800 gallons per day from a  single
 well.   Between February 1969 and July 1971, 216,000 gallons
 of gasoline were pumped from about 40 wells in the area,  in
 the two and one-half year period, the maximum measurable
 thickness of gasoline in  wells shrank to less than one foot
 and the maximum rate of removal from any single well  declin-
 ed to  100 gallons per day.

 One of the  major problems encountered in the clean-up opera-
 tion has been  the fluctuation in the level of the water
 table.   High water-table  conditions  caused by heavy rainfall
 periods  have forced gasoline and gasoline vapors into base-
 ments  of buildings.   Also,  abnormal  rises in the water table
 can temporarily float the gasoline above the intakes  of re-
 moval  wells.

 Montgomery  County,  Pennsylvania - 42)

 In  this  case,  a transmission pipeline leak caused an  esti-
 mated  80,000 gallons  of gasoline to  enter the ground  water
 and contaminate wells  in  the area.   In July 1971,  gasoline
 was  observed in a 60-foot deep  well  and  in August of  the
 same year in a  247-foot well, both tapping a limestone aqui-
 fer.   Pumping  the affected wells to  waste over a period of
 one year  proved to  be  no  longer useful in removing the gaso-
 line after  approximately  45,000  gallons  had been recovered.
 The pipeline company  then proposed use of natural biological
 agents to break down  the  remaining 35,000 gallons  of  gaso-
 line,  and this  experiment has been approved by the regula-
 tory agency  involved.

The system  consists of 24 wells  into which 10  tons  of  nitro-
gen and  10  tons  of  phosphate will  be  injected  as  nutrients
over a period of  five months.  Air will  also  be  injected in-
to the wells at  a rate of 2.5 to 3.5  cubic feet  per minute,
in order  to maintain  aerobic conditions  in the  aquifer.
The project will  be carefully monitored  to determine the


                              182

-------
success of this method for removing fractions of hydrocar-
bons that cannot be recovered through the use of wells,
trenches, and other skimming procedures.  The project is un-
derway, but results are not yet available.

Tabulation of Case Histories -

Cases of ground-water contamination from leaky and ruptured
buried pipelines and tanks were found in all of the 11
states included in this investigation.  Unfortunately, very
few have been studied in detail but a review of about 50 of
the better documented cases reveals again that petroleum and
petroleum products are the most common complaint.  Sources
of petroleum contamination from buried tanks included gaso-
line stations, commercial facilities and homes heated with
fuel oil, fuel storage areas, and industrial plants.  Most
of the problems recorded were local in nature, for example,
affecting five or six domestic wells in the vicinity of a
gasoline station.  However, others were more regional in na-
ture, as in an area of Connecticut where the shallow aquifer
along a five-mile stretch of a tributary to the Housatonic
River reportedly is contaminated with hydrocarbons and chem-
icals, presumably from leaky gasoline station, home fuel oil,
and industrial tanks. 79)

The effect on ground-water supplies caused by a leak from a
home heating oil tank is illustrated by a case in New York
State.  The pollutant penetrated 20 feet of overburden and
moved 700 feet through a dolomite aquifer, contaminating wa-
ter from a 100-foot deep domestic well.  A new well was
drilled 150 feet away from the affected well, and within one
month after start of pumping, the second well was abandoned
because of oil in the water.  It took three years for the
body of oil to dissipate enough so that the second well
could be used for domestic supply. 30)

A number of cases have been reported where wells have been
affected by leaky sewers and industrial pipeline systems
transporting chemical fluids.  In Camden, New Jersey, at
least one public-supply well, yielding  a million gallons per
day and tapping shallow coastal plain deposits, has been
shut down because of high levels of chromium in the water.  80)
The source of the problem is apparently due to leakage from
municipal sewers in the general area that carry a heavy load
of industrial wastes.  In upstate New York, a pipeline carry-
ing natural brine from the source to the  location of the in-
dustrial plant where it is used for processing leaked peri-
odically for many years.  81)  The industry has had  to  re-
place many dug wells along the pipeline route with  deeper
wells.


                              183

-------
 Methods used for the control and solution of problems caused
 by leakage from tanks and pipelines have been only partially
 successful, especially with regard to hydrocarbons.  Repairs
 to the source of contamination, of course, are immediately
 undertaken, but in a number of cases, it was not possible to
 detect the source.  Flushing the area with water has been
 reported as a method for attempting to dilute the pollutant
 in the shallow aquifer zone;  ruptured tanks have been dug
 out,  and to prevent future problems, clay barriers have been
 installed in the excavation before a replacement tank was
 buried;  and trenches and wells for skimming have been dug
 to remove hydrocarbons from the water table.  Nevertheless,
 well  owners in some areas of the region report that taste
 and odor problems from petroleum contamination of aquifers
 have  existed for 20 to 25 years, in spite of all abatement
 efforts.

 Future Trends

 As in the case of spills,  a certain proportion of ruptures,
 breaks,  and leaks in buried tanks  and pipelines is unavoid-
 able,  and contamination of ground  waters  near such facili-
 ties  will be  a continuing problem.   Leakage from sanitary
 and storm sewers  will continue  because so many of these
 systems  are old.   It is doubtful that a major portion of the
 old leaky sewers  will be replaced  in the  foreseeable future.
 Thus,  even though the materials used and  today's design and
 installation  practices for new  sewers have improved greatly,
 this  source of ground-water contamination will remain an im-
 portant  factor to be considered in  decisions regarding the
 siting and construction of water wells.

 Much more  promising  from the  standpoint of ground-water pro-
 tection is  the  greater scrutiny by  public agencies  of major
 petroleum  pipeline projects because of new environmental
 laws.   Before  the  pipeline is constructed,  codes and regula-
 tions  call  for  consideration  of factors involving design and
 management  of  the  system related to possible effects of
 leaks  on  the  underlying aquifers.   For example,  an  oil  pipe-
 line recently  authorized in .Long Island,  New York,  that
 crosses important  aquifers in the region,  was  equipped  with
 special valving and  all  connections were  carefully  inspected
when installed  in  order  to minimize  leakage  from breaks  or
 failures that might  occur.  Public-supply and  domestic  wells
were mapped along  the  route to  determine  the  sensitivity  of
water  supplies  to  possible contamination.  The  flow  of  fuel
oil through the line  is  carefully monitored  so  that  losses
in product  can be quickly  discovered,  and an emergency  pro-
gram has been developed  for containment and  clean-up in  the
event of a  leak.  82)


                              184

-------
Concern for the environment undoubtedly will lead to better
protection of pipelines and tanks from corrosion, and the
use of materials such as clay and tar to line excavations
for tanks and even pipelines where leakage might affect
nearby water wells.  Most of these efforts are presently di-
rected toward minimizing the possibility of fire or explo-
sion or the escape of toxic substances.  However, the need
for protecting ground-water resources is becoming better
recognized in the region because of the growing number of
cases of contamination of water wells from hydrocarbons re-
ported to state agencies each year.

Research is most needed in developing new methods for remov-
ing hydrocarbons from the ground-water reservoir.  Abatement
by pumping or ditching is widely used and only partially ef-
fective.  However, other means for cleaning up petroleum
contaminated soils and aquifers have been suggested that
should be further investigated.  They include water-flooding
techniques to better control and collect the body of fluid
for more efficient removal;  biodegradation of hydrocarbons
by aerobic and/or anaerobic bacteria;  and the use of chem-
icals to precipitate or immobilize the pollutant.

APPLICATION AND STORAGE OF HIGHWAY DEICING SALTS

In those states that have colder climates and lie within the
snow belt of the northeast region, road maintenance during
the winter months is a major problem, especially in the
densely populated, industrial-urban areas.  The need for un-
impeded vehicular travel on highways has led to increased
use of sodium and calcium chloride by state and local agen-
cies in coping with winter storms.  Salt has become popular
as a means of snow and ice removal because of its ease of
handling as compared to such abrasives as sand and cinders,
its efficiency in providing a "bare" pavement, and its rela-
tively low cost.  In fact, sodium chloride, or rock salt, is
the least expensive of all deicing chemicals  (costing about
one-third as much as calcium chloride) and, therefore, is
purchased in the greatest volume by state, county, and mu-
nicipal agencies in the region.  83)

Table 29 gives the estimated quantities of sodium chloride
and calcium chloride used by state highway departments and
the application rate for eight of the  11 states in region
for the winter season of 1965-66.  Total use of deicing
salts in all eleven states for the winter period of 1966-67
is estimated at close to two million tons. 35)

The large amount of salt used and the  quantities of these
soluble inorganic compounds applied per lane mile year after

                             185

-------
Table 29. QUANTITIES OF SODIUM AND CALCIUM CHLORIDE USE AND THE
         APPLICATION RATE PER SINGLE-LANE MILE FOR THE WINTER SEA-
                           SON OF 1965-66. 84)
State
Connecticut
Delaware
Maryland
Massachusetts
New Hampshire
New Jersey
New York
Vermont
Calcium
Chloride
(tons)
8,000
820
465
5,855
540
3,195
3,900
500
Sodium
Chloride
(tons)
74,600
2,770
44,893
120,304
82, 737
17,495
245,300
83,122
Quantity Applied
(tons/single-lane mile)
8.98
4.48
6.82
20.70
11.95
3.33
7.50
18.22
Note;  All figures represent use by State Highway Departments only.
                               186

-------
year (more than 20 tons per lane mile per year for Massa-
chusetts, for example, with an eight-fold increase in total
salt applied between 1954 and 1971)  should have an impact on
both surface-water and ground-water quality. 85)   Runoff
from road surfaces eventually finds its way into streams and
rivers within the drainage basin occupied by the highway or
percolates into the soils adjacent to the highway.  The so-
dium, calcium, and chloride ions in the soil can be carried
down to the water table by the runoff water itself or during
periods of recharge from rainfall.  Contaminated water can
then move through the saturated zone until it is discharged
into a surface water body, has leaked into an adjacent aqui-
fer, or is pumped from a well.  Although sodium and chloride
ions can both move through the unsaturated and saturated
zones, the former is more attracted chemically to various
types of soils.  This characteristic accounts for the rela-
tively higher ratio of chloride to sodium encountered in
contaminated ground water than normally found in  surface
water receiving direct runoff of salt-laden waters.

Another source of ground-water contamination related to
salts used for highway deicing is storage of this material
in piles at central distribution points.  There are well
over a thousand such storage sites throughout the study re-
gion, based on conversations with highway officials, and in
the fall, each holds from several hundred to several thou-
sand tons of salt.  The low solubility of rock salt permits
outside storage over relatively long periods of time without
hard caking or noticeable loss in volume.  Thus,  many such
salt piles are left uncovered on open land.  This condition
is especially common where the salt has been mixed with sand,
resulting in a large volume of stored material that would
require an expensive structure if the pile were to be
sheltered.

Rain falling on the stockpile dissolves a portion of the
salts and can carry them into the ground-water system.  Typ-
ically, salt-spreading trucks are washed at such  storage
areas, and infiltration into the ground of  the resulting
brine solution can aggravate the contamination problem.  In
some cases, drainage  from salt piles and wash areas  is  col-
lected and fed into dry wells.  Thus, the pollutant  is  in-
troduced directly into the geologic  formation underlying the
site.

The principal hazard  of road salts contaminating  water  sup-
plies is the potential for exceeding established  public
health standards  for  chloride concentrations.  The  U.  S.
Public Health Service  Drinking Water Standards of 1962  sets
a maximum limit of 250 mg/1 for  chloride, where more suit-


                              187

-------
 able supplies are or can be made available.       This stand-
 ard also is adherred to by the various state health agencies
 in the region.   If other water sources are not available,
 concentrations' of up to 500 mg/1 are generally tolerated.

 In addition,  medical authorities have recommended against
 the use of waters containing more than 20  mg/1 of sodium for
 patients with heart disease, hypertension, renal  disease,
 and cirrhosis,  as well  as for many pregnant  women.  86)
 These potential health  problems have led at  least two states
 in the region,  Connecticut and New Jersey, to adopt a limit
 for sodium of 20 and 50 mg/1 respectively, as a standard not
 to be exceeded  if better quality water is  available.  87,88)

 Other hazards include the possible corrosion of well  casings,
 screens,  and  pumps.   Also,  substances have been added to de-
 icing salts to  prevent  caking and to inhibit corrosion.  For
 example,  sodium ferrocyanide has been added  to deicing salts
 to prevent caking.  84)   Not enough is known  about the solu-
 bility or toxicity of the additives  nor their fate  in the
 soil  and  ground-water system to comment further.  Detailed
 chemical  analyses to determine whether such  additives are
 present in ground water contaminated by deicing salts should
 be incorporated into future research studies.

 Some  controversy has existed over the importance  of highway
 deicing salts as  a cause  of increasing chlorides  in ground
 waters  of the northeast states.   The controversy  exists  be-
 cause  there are  many other  sources that can  contribute to
 rising  levels of  concentration of this ion in the subsurface
 environment.  These  other sources  include  septic  tanks and
 cesspools, water  softener regeneration,  leaky sanitary sew-
 ers,  landfills,  air  pollution,  and ocean spray.  Even
 drought conditions can  lead to temporary increases  in min-
 eralization of  ground water because  of the reduced  amount of
 fresh-water recharge during such  periods.  The  pollutant can
 be  concentrated  in the  soil zone  during an extended dry
 period  and  then  later carried  to  the water table in high
 concentrations during the initial  periods  of  normal or above
 normal  rainfall.

 However,  enough research has been  conducted on  this problem
 to  at least establish a relationship between  highway  deicing
 salt and  ground-water contamination.   For  example,  F. E.
 Hutchinson of the University of Maine  has  studied environ-
mental effects caused by an average  annual application rate
 of  25 tons of sodium chloride  to  each  mile of paved highway
 in Maine.  89)  During the period  1967-69, water from  approx-
 imately 100 wells was sampled  at  random locations along ma-
 jor highways.  Although natural chloride concentrations  from

                             188

-------
the various aquifers in Maine are normally less than 20 mg/1
(see Table 14), the three-year average April chloride con-
tent of water from the sampled wells was 171 mg/1.  About
one-fifth of the wells yielded water exceeding the 250 mg/1
chloride standard.  Average distance from the roadway for
all wells was 40 feet, with an average of 24 feet for those
wells containing water with concentrations of chloride in
excess of 250 mg/1 average.  The highest concentration of
sodium encountered was 846 mg/1 and for chloride was 3,150
mg/1.  The level of contamination for almost all wells each
year was less in August than in April, which is the month of
greatest snow melt and runoff from the roadways.

Hutchinson also participated in research on sodium and chlo-
ride ion levels in the soils bordering major highways. 90'
The findings of this investigation at 27 sites revealed that
levels of these ions were greatest both nearest to the road-
ways and where salting had been practiced for the longest
period of time.  At one site, along the edge of a road em-
bankment, sodium sampled before the highway was opened in-
creased nearly five fold to 235 mg/1 after only one season
of salting.

Considerable research has been carried out and is still un-
derway in Massachusetts regarding the environmental effects
of road salt application and storage.  In one recent study
by Arthur D. Little, Inc., for that State's legislature, a
correlation has been noted between the upward trend in use
of road salts and the rising chloride levels in ground-water
supplies during the same period. 86)  Figure 31 shows this
correlation.

Of course, increased activity involving other potential
sources of contamination is probably contributing to rising
levels of chloride concentrations, but the report concludes
that deicing salts are the major cause.  This theory is sup-
ported by a case of ground-water contamination in Burling-
ton, Massachusetts, where the U. S. Geological Survey
studied the potential causes of a problem of rising chloride
levels in that Town's well supply. 91)  jn 1949, a suction-
well system of 70 shallow wells tapping glacial sands and
gravels was installed about 3,500 feet from a major highway,
which was opened the same year.  In 1961, when the Burling-
ton Town Highway Department began storing salt, uncovered
and approximately 400 feet from the well field, the chloride
content of water from the wells averaged about 15 mg/1.  AS
noted on Figure 32, the chloride concentration began to rise
at a relatively rapid rate by 1963.  In spite of such reme-
dial measures as sheltering the salt pile from rain water in
1968 and banning the use of deicing chemicals on Town


                             189

-------
900
800
700
600
500
400
300
200
100
         INDEX: 1955 = 100
— TOTAL CHLORIDES APPLIED TO HIGHWAYS BY MASS. DEPT. OF PUBLIC WORKS
.— AVERAGE CHLORIDES IN  GROUND-WATER 5-20 MILES  FROM COAST
	 AVERAGE CHLORIDES IN  GROUND-WATER 20-36 MILES FROM  COAST
	 AVERAGE CHLORIDES IN GROUND-WATER 57-IOO MILES FROM COAST
                            I     I
                                                    I    I     I    I     I     I
        1955
                   I960
                                                       1965
                                                                              1970
  Figure 31.  Index of increases in salt applied to Massachusetts state highways and
                     chloride levels  in ground-water sources, 1955-1971 °°)
                                     190

-------
   400
LJ
S  300
K
S2  200
J  '00
g
a
a

5    o
         Q O
         -I a:
         u
                                   ZOOO
         1955
I960
1965
1970
                    Figure 32.  Chloride concentration in samples from main pumping station in

                                                Burlington,  Massachusetts °°>

-------
 streets in 1970,  the concentration of chloride reached a
 peak level of 283 mg/1 in 1970 and was still at a level of
 over 100 mg/1 in  late 1971.

 The U.  S. Geological Survey  developed a "salt-budget"  for
 the Burlington well field area and, taking into account such
 factors as time of travel of contaminated ground water,  rain-
 fall effects,  and the various activities  in the river  basin,
 tabulated the  estimated importance of the various sources of
 contamination.  Table 30 shows that,  according to the  esti-
 mate,  85 percent  of the contamination, as of 1971,  was re-
 lated to highway  salts and only 15 percent to other sources.

 Case Histories

 Additional supporting evidence of  the relationship  between
 highway deicing salts and ground-water contamination has
 been developed  in this investigation  based on data  from the
 files of public health agencies and other environmental  or-
 ganizations working in the region.  Information from select-
 ed  case histories of those inventoried is given below.

 As  mentioned previously,  a number  of  areas in the northeast
 have experienced  a rise  in chloride concentrations  in  water
 from municipal, industrial,  and domestic  wells.   In some,  as
 in  Massachusetts  discussed above,  enough  regional analysis
 has been made to  indicate  that the  problem is related  prin-
 cipally to highway deicing salts.   In others,  this  source  is
 suspected, but  not enough  data has  been collected to pin-
 point specific  salt  storage  areas  or  road salting practices
 as  the  prime reason  for  ground-water  contamination.  For ex-
 ample,  in many  of the  glacial  sand  and gravel aquifers of
 northern New Jersey,  long-term records of the quality  of
 water from a number  of municipal wells have  shown a gradual
 but significant trend  of  increasing chloride  concentra-
 tions.  92,93)   Some  of these  systems  operated for decades
 with no  indication of  contamination but,  starting in the
 early 1960's, chlorides began  to rise  in  the  well waters,
 and if  the present  rate of increase continues  for another
 decade,  many wells will be yielding water  that  exceeds 250
 mg/1 of  chloride  and  that  also  contains high  levels  of so-
 dium.   Similar  conditions  were  frequently  cited within the
 course of this  investigation by community  sanitarians,
 county and state  health authorities,  and well drilling con-
 tractors, throughout the northern tier of  states.

 In  addition, data on a number of specific  and documented
 cases of  ground-water contamination caused by storage or ap-
plication of deicing salts were obtained  and  information on
 34  of these is tabulated in Table 31.  Those  shown were


                             192

-------
Table 30.  SOURCES OF SALT CONTAMINATION OF THE BURLINGTON,
                   MASSACHUSETTS WELL FIELD, 1971.  86)
1.  Highway Salt:

      (a)  Used by the Town of Burlington (including storage
          and application to roads)

      (b)  Applied by Massachusetts Department of Public
          Works

      (c)  Applied by Town of Lexington (42 percent of
          which  lies in same drainage basin as the well
          field)
40 percent


30 percent



 15 percent
                                              Sub Total:       85 percent
2.  Septic Tanks and Industrial Contamination:
    percent
                                              Total:
100 percent
                                  193

-------
 Table 31.  SUMMARY OF DATA ON 34 SELECTED CONTAMINATION CASES
                          RELATED TO DEICING SALTS.
 Type of problem

 Maximum observed chloride concentration

     100 to 250 mg/l
    250 to 500 mg/l
    More than  500 mg/l

 Principal aquifer affected

    Unconsolidated deposits
    Sedimentary rocks
    Crystalline rock

 Observed distance traveled by pollutant

    Less than 100 feet
    100 to 1,000 feet
    More than  1,000 feet
    Unknown or not reported

Maximum observed depth penetrated by pollutant

    Less than 30 feet
    30 to 100 feet
    More than  100 feet
    Unknown or not reported

Action taken regarding source of contamination

    Road salting banned or modified
    Drainage modified
    Salt storage pile removed
    Salt storage pile enclosed
    No known action

Action taken regarding ground-water resource

    Water supply well(s) abandoned
    No known action
Road
salting
   3
   5
   3
   6
   0
   5
   4
   3
   1
   3
   3
   3
   3
   2
   2
   2
Salt storage
   piles
     4
     7
    12
    11
     4
     8
     3
     9
     6
     5
     2
    10
     7
     4
  6
  5
     2
    10
     5
     6
    10
    13
                                  194

-------
selected on the basis of the reliability and the amount of
the data provided.

As indicated by the table, in a large percentage of the
cases that actually came to the attention of regulatory
agencies and, thus, are recorded, chloride concentrations
are greater than 500 mg/1.  For some of those cases listed,
especially where salt storage piles were involved, chlorides
exceeded 2,000 mg/1 and sodium exceeded 100 mg/1.

Of interest is the fact that in most instances for which
long-term records are available, chloride concentrations in
the water from affected wells show seasonal fluctuations
with the highest levels in early spring and the lowest
levels in late fall.  Bodies of contaminated water, which
may have been introduced into the ground the same year or
many years before, arrive at a pumping well as separate salt-
water fronts.  This condition temporarily raises the chlo-
ride concentration, which then declines somewhat until a new
front arrives about a year later.  This surging phenomenon
in chloride content relates to the periods of maximum and
minimum runoff and infiltration of salt-laden waters.  Fig-
ure 32 illustrates the typical peak and trough character re-
ferred to and also the normal, overall rising trend in chlo-
ride concentration from year to year.

Studies by the U. S. Geological Survey at one Massachusetts
site have indicated that salt water has moved through uncon-
solidated glacial deposits at a rate of about 200 feet per
year from a salt storage pile to a municipal well 1,000 feet
away. 9D  Therefore, it takes more than five years for con-
taminated water infiltrated into the ground at the source to
reach the well.  At another site, it is estimated that the
minimum period is six to twelve months, from the time of ap-
plication of deicing chemicals to the highway to the appear-
ance of contaminated water in the affected well.  It should
be noted that considerably more time is required than often
appreciated for ground-water quality damaged by salt water
to be restored to an acceptable condition after a remedial
action, such as removal of a salt storage pile, has been
taken.  Pumping to waste, in order to reduce the volume of
contaminated water in the aquifer, is a frequently used
method for recovering use of a production well.  However,
the operator is rarely equipped with enough hydrologic in-
formation to be able to estimate how long and at what rate
the well must be pumped before chloride concentrations will
show a. significant decline.

Another problem that becomes obvious in the review of case
histories is the difficulty in replacing wells abandoned be-


                            .195

-------
 cause of extreme contamination.  After the pollutant has ar-
 rived at a domestic supply well or has moved into a munici-
 pal well field, an attempt generally is made to drill the
 existing wells deeper,  especially when the aquifer consists
 of crystalline or sedimentary rocks.  Another procedure is
 to move farther away from the suspected source of contami-
 nation and construct new wells on the same property.  Be-
 cause chlorides are not considered toxic,  casing off the af-
 fected aquifer zone or  moving away from the source but tap-
 ping the same formation are accepted as reasonable risks.
 However, even though initial chloride concentrations at
 greater depths or at new locations are low, the salty ground-
 water body is still present and may be within the influence
 of pumping of new wells.   Ultimately, they too may have to
 be abandoned.

 This situation is illustrated by a case in Freeport, Maine,
 where a 185-foot deep domestic well was contaminated by de-
 icing salts from an uncovered storage pile and, to some de-
 gree,  by salt applied to  an interstate highway adjacent to
 the storage area.  94)   when this well, which was 700 feet
 from the salt pile,  was abandoned because  chloride content
 reached 600 mg/1,  a second well was drilled into the crystal-
 line rock aquifer,  300  feet farther from both the salt pile
 and the highway.   Initial chloride concentration of water
 from the new well  was 50  mg/1,  but within  four months,  it
 had risen to 2,000 mg/1.   The limited size of the property
 available (which  is a typical problem in finding new well
 locations in such  situations)  prevented moving the new well
 any more than the  300 feet.

 In  another  situation  in southeast Connecticut,  a site was
 chosen,  based on an extensive test-drilling program,  for de-
 velopment of a future municipal well field.  31)   During the
 initial testing in 1968,  chlorides in water from test-pro-
 duction wells  installed on the  property ranged from 12  to  36
 mg/1.   Two  years later, a gasoline leak from an underground
 storage tank in a  nearby  automobile  service station was re-
 ported,  and as  a matter of routine,  the city resampled  the
 test-production wells,  which  were screened in glacial sand
 and  gravel  deposits.  No  hydrocarbons were found but chlo-
 rides had risen to almost 400 mg/1.

 Investigation  into the  problem  revealed that a  salt storage
 area was  located about  1,000  feet from the wells.   All  run-
 off  from a  salt pile and  from truck  washing operations  had
been drained into  a  series  of dry wells  over a  10-year  peri-
od from 1955, when the  facility was  constructed,  until  1965
when the  salt  pile was  covered  and the drainage  system  was
converted to a  concrete pipeline  carrying  the waste water
                             196

-------
away from the property.  A water sample taken from a rock
well used at the storage area also showed contamination,
with a chloride content of 1,100 mg/1.  Additional testing
and pumping at the proposed well field indicated that almost
the entire property was underlain by salty ground water.
Not enough area was available to find new sites on the same
piece of property or on adjacent properties to move far
enough away from the existing problem. The proposed well
field, capable of producing several million gallons of water
per day, was abandoned.

In all of the cases used in the preparation of Table 31, wa-
ter supply-wells had been affected.  It should be noted that
in many of these instances, the pollutant had traveled
several thousand feet from the source to the affected well
and had penetrated to depths of more than 100 feet, actually
to almost 400 feet in a few wells.  Most of the deeper wells
tap crystalline rocks, which are particularly susceptible to
relatively rapid movement of the pollutant through fracture
zones and bedding planes with little chance for dispersion
and dilution.

With regard to the action taken once the problem is discov-
ered, little can be done if one or two domestic wells have
been affected adjacent to a major highway because of the ap-
plication of deicing salts to the roadway.  However, if a
problem of regional magnitude has come to the attention of
authorities, a reduction in the amount of salt applied has
been implemented and actual bans on deicing salts on a city-
wide basis have been put into effect, at least temporarily,
for a number of municipalities in the northeast.

Very often, if road salting or salt storage areas are pin-
pointed as a source of contamination, drainage in the area
is modified as a partial solution to the problem.  This pro-
cedure normally takes the form of collecting and piping the
salty water away from the suspected ground-water intake
area, often directly into a nearby surface-water body.  In
many cases, where contamination from a salt pile has af-
fected a school well or municipal water supply, the stored
salt is removed because it is much simpler and less costly
than abandoning the well system.  If this action occurs be-
fore gross contamination of a large portion of the aquifer
has taken place, the wells may slowly recover.  Salt storage
piles also have been enclosed by a shed and the area paved
to prevent infiltration of the salt-contaminated water.  Al-
though many of the states and municipalities in the region
have begun a program to shelter salt storage piles, this
process will take a long time to effectively accomplish be-
cause of the high cost and the large number of existing sites,


                             197

-------
 Treatment of the affected water is not practiced in the re-
 gion because of the extreme expense in desalting water sup-
 plies.   Some municipalities are mixing contaminated water
 with water from unaffected wells in order to dilute the sa-
 linity.   Many domestic well owners report continuing the use
 of their affected supply.   Because of the difficulty in
 drilling a replacement well on  a relatively small piece of
 property,  they "carry their drinking water."

 Future Trends

 A review of the literature reveals no adequate  substitute
 for highway deicing salts.   Therefore,  it is reasonable to
 assume that their use will continue but probably not at the
 accelerated rate experienced in the past.  In fact,  some
 states,  especially those  in New England,  have already begun
 programs for reducing the  amount of salt applied each year
 to roadways.   In Maine, equipment modification  and driver
 education  has reportedly  reduced the amount of  salt used by
 20 percent without decreasing the effectiveness  of deicing
 efforts.  95)   New Hampshire has embarked on a similar pro-
 gram and hopes to lower its current use of salt  on state
 highways from an average  of 150,000 tons  per year to 100,000
 tons. 50)   This  action has  been prompted, to a  great degree,
 by the 250  complaints  of  road salt contamination of wells
 received each year.   However, the few hundred thousand dol-
 lars  that  New Hampshire projects  spending on the replacement
 of affected wells each year still does  not make  it econom-
 ically feasible  to consider changing over from  salting to
 the  very expensive alternative  of increased snow-plowing.

 The  growing awareness  that  salt spreading could  have an ad-
 verse effect  on  ground-water  quality has  led to  efforts by
 agencies on various  levels  to modify drainage plans  for pro-
 posed highways  in an  attempt  to protect the resource.   As
 previously  mentioned,  storage areas  are also being cleaned
 up and more  attention  is being  paid  to  covering  exposed
 piles and keeping salty water out  of the  ground.

 In early 1974, Massachusetts  enacted a  very strong law de-
 signed to  curb oversalting  of roads  and resultant  water pol-
 lution.  96)   n-  requires users  of  more  than one  ton  per year
of sodium  chloride, calcium chloride  or other road deicing
chemicals to  report how much  they  use and store.   The  state
will compile  data  on amounts  of salt  used and, where  surface
waters or ground waters are threatened, can  ban  or restrict
the use  of  salts.  The passage  of  the law was prompted  by
information  from  the state's health  authorities  that  the  wa-
ter supplies  in  88 communities  exceed 20  mg/1 sodium.
                             198

-------
Although other states will probably consider similar legis-
lation, not enough is known regarding the overall trend in
rising chloride and sodium being experienced in many parts
of the region.  Because road salting will continue, more re-
search is needed regarding the role that deicing salts play
in comparison with other potential forms of ground-water
contamination.  In addition, based on more knowledge of the
environmental effects of highway salts, guidelines are need-
ed for the siting, construction, and protection of wells on
properties located near highways, the design of drainage
systems where highways cross aquifer intake areas, and
methods for studying, monitoring, and eliminating contamina-
tion problems when they occur.  Finally, research is needed
to determine the fate of deicing salt additives after they
have entered the hydrologic cycle.  For example, are these
substances stable, do they react with soils, or do they re-
main permanently in solution in ground water and surface
water?

LANDFILLS

The principal method currently used in the northeast for
disposal of solid wastes generated by communities and indus-
tries is open dumping in landfills.  Sites receiving refuse
are operated by private profit-making organizations, which
have contracted to communities and industries for the pur-
pose of disposing of their solid wastes, or by public agen-
cies such as municipal or county governments.  In addition,
numerous landfills serve one particular industrial site.
Still others are used as uncontrolled community dumps by
local residents.

No comprehensive inventory exists regarding the number and
size of landfills in the states making up the study area,
but an idea of the potential for ground-water contamination
can be gained by a review of the data that are available.
The information contained below was derived from a number of
sources including published reports, files of public agen-
cies, and interviews with personnel in private and govern-
mental organizations.  One regional analysis that should be
noted and is most important with regard to municipal land-
fills is the 1968 national survey of community solid-waste
practices. 32)

Until recently, an evaluation of geologic and hydrologic
conditions was rarely included among the various considera-
tions that determined site selection for landfills in the
northeast.  Thus, one environmental hazard created by past
refuse disposal practices is the possible effect on ground-
water quality.  Existing landfills or dumps invariably were

                             199

-------
 placed  on  land  that had  little  or  no  value  for  other uses.
 The  site chosen was located,  for example, in  a  marshland, an
 abandoned  sand  and gravel  pit,  an  old strip mine,  or a  lime-
 stone sinkhole, each  of  which is a favorable  environment for
 the  development of ground-water contamination problems.  The
 above statement holds true for  the manufacturer who has a
 20-acre plant site where refuse is being dumped in a low-
 lying wet  area  in a remote corner  of  the property, just as
 it does for  the large regional  municipal landfill  that may
 be occupying a  particular  location only because it was the
 least objectionable site from a political and economic stand-
 point.

 The  situation in the  City  of  New York is a  prime example of
 the  large  amount of property  required for refuse disposal
 and  the type of land  used  for this purpose.   At present, it
 has  approximately 3,500  acres of landfills  receiving refuse
 at a rate  of 26,000 tons per  day.  97)  Almost all  of these
 properties are  filled marshlands,  with the  base of the ref-
 use  at  or below the water  table.   In  New Jersey, 331 land-
 fills owned  by  municipalities,  county agencies, or private
 contractors  are consuming  land  at  a rate of about  750 acres
 per  year.  98)   Some 10,600  acres not  yet used for  landfill
 operations are  committed to such use  in the future, but it
 is estimated that all of this land will be  exhausted by
 early 1982.  One hundred and  eighteen New Jersey municipali-
 ties haul 36,000 tons of solid  waste  per week to landfills
 in the  Hackensack Meadowlands,  located within the  northeast-
 ern metropolitan area of the  state.   Connecticut estimates
 that 200 acres per year  are being  consumed  for  landfills. 33)
 Of the  144 municipal  sites  surveyed recently  in Connecticut,
 only 13 were satisfactorily meeting all requirements of the
 State's Department of Environmental Protection  from the
 standpoint of ground-water protection. 99)

 The State of Pennsylvania has developed some  interesting
 statistics that bear  on  the number  of sites that may be con-
 tributing to ground-water contamination. 100)   It  ^s esti-
mated that within that state  there  are 2,617  "promiscuous"
 dumps existing along  roadsides, and in open fields and lots.
 Of 648 major landfill sites investigated in a 1966-68 inven-
 tory, 258 were contributing to water  pollution.  The latter
 figure  includes 30 located in strip mines.  It  should be
noted that most of these sites were in existence long before
Pennsylvania had a Solid Waste Management Act.

Landfills in the region  are receiving a wide  variety of mate-
 rials including paper products, food  wastes,  septic-tank
 sludge,  demolition debris, tires,  automobiles,  leaves, plas-
tics, textiles,  glass, aluminum cans,  liquid  chemicals, oils

                              200

-------
and hydrocarbons,  street sweepings,  dead animals,  and water
and waste-water treatment sludge.  In municipal refuse,
paper and paper products make up the major category by
weight.  Table 32  indicates the physical characteristics of
typical municipal  refuse.

An average of about 5.3 pounds of solid wastes per day per
capita is collected in the United States.  A more realistic
figure on waste generation should be based on collected plus
uncollected refuse.  The total would then approach eight to
ten pounds per day per capita, but still would not include
some solid wastes  from industry and agriculture that are
disposed of on-site. 102)  if the eight pound-estimate is
used, then at least 214,000 tons of solid waste is generated
in the 11-state region each day.

The processes that can lead to contamination of ground water
from the disposal of wastes in landfills are relatively sim-
ple.  The various organic compounds in refuse  (with the ex-
ception of most plastics) are decomposed or stabilized by
aerobic and anaerobic organisms to simple substances that
will decompose no further.  These products of decomposition
include gases and soluble organic and inorganic compounds.
If sufficient water is available from precipitation, or from
surface drainage in contact with the refuse, these compounds
can be dissolved and carried with the water that infiltrates
the landfill and ultimately recharges the ground-water res-
ervoir or discharges into adjacent surface-water bodies.

Solid inorganic refuse,  such as tin cans and metal pipes,
can also be slowly dissolved by percolating waters, result-
ing in a solution with an increased concentration of metal-
lic ions.  Finally, disposal of liquid industrial wastes,
septic-tank pumpings, and waste-water treatment sludges can
contribute to an overall increase in dissolved solids  con-
centration of water passing through the  landfill.  The term
"leachate" has been applied to highly contaminated water
contained in or directly associated with a refuse disposal
site.

Not so simple is the composition of leachate and the changes
in concentration that can occur  as the various pollutants
move through the subsurface environment.  Significant  indi-
cators of pollution in leachate  from landfills containing
municipal refuse include BOD  (Biological Oxygen Demand), COD
 (Chemical Oxygen Demand), iron,  chloride, and  nitrate.  The
interaction of C02  (Carbon Dioxide) with soil  and rock mate-
rials  as it travels through permeable soils may contribute
to the hardness of  ground water  in the area and result in
the release of iron and  manganese held on soil particles.


                              201

-------
Table 32. PHYSICAL CHARACTERISTICS OF MUNICIPAL REFUSE:  TYPICAL 100-lb
                     SAMPLE, MUNICIPAL REFUSE.  101)
Item
Paper
Garbage
Leaves and grass
Wood
Synthetics
Cloth
Glass
Metals
Ashes, stone, dust, etc.
Wet Weight (Ib)
48.0
16.0
9.0
2.0
2.0
1.0
6.0
8.0
8.0
Dry Weight (Ib)
35.0
8.0
5.0
1.5
2.0
0.5
6.0
8.0
6.0
                               202

-------
In addition, biological pollution can be associated with wa-
ters discharging from a municipal landfill.  Heavy metals
and other toxic compounds can be found in ground water con-
taining leachates from municipal landfills where toxic
wastes have been accepted, and from private landfills serv-
ing particular industries where special types of wastes are
dumped.

The concentration of chemical and biological pollutants
travelling through soil decreases with distance from the
landfill.  The effectiveness, however, of such processes as
adsorption, ion exchange, dispersion, or dilution varies
considerably with the type of pollutant involved, the char-
acteristics of the soil underlying the landfill, and geo-
logic and hydrologic conditions at the site.  Thus, no broad
generalizations can be made.

The volume of leachate developed by any particular landfill
is a function of its absorptive capacity and areal extent,
and the amount of recharge water available for infiltration.
Most landfills assume a relatively flat surface with no veg-
etation, which is more conducive to infiltration than to
runoff and evapotranspiration.  They are normally  covered
with a relatively coarse-grained material, again increasing
infiltration efficiency.  Therefore, it is reasonable to as-
sume that at least one-half of the annual precipitation can
become recharge to the ground-water reservoir, after it has
come in contact with the solid waste contained in  the land-
fill.  Average annual rainfall in the northeast region is  42
inches per year.  Thus, a 100-acre site would be capable of
producing 57 million gallons of leachate per year  after
field capacity of the refuse has been reached.  The more
than 10,000 acres set aside in New Jersey  for landfilling,
mentioned above, theoretically would be capable of producing
5.7 billion gallons of leachate in one year.

Research on the question of how long after abandonment a
landfill can be expected to generate leachate has  been min-
imal.  However, one investigation under a  grant from the
U. S. Public Health Service to the Pennsylvania Department
of Health sheds some light on this question.  A study was
made of a landfill in southeastern Pennsylvania, part of
which had been closed in 1950 but was still producing leach-
ate.  This was sampled along with leachate from a  new sec-
tion of the same landfill site still in operation  in  1970.
The comparison of the chemical characteristics of  the two
leachate samples is shown in Table 33.  It should  be  noted
that there  is a difference of a hundred-fold or more  in  BOD
and COD between the leachate from the old  abandoned  section
and the new section of the landfill.  Differences  in  specific

                             203

-------
Table 33.  COMPARISON OF THE CHEMICAL CHARACTERISTICS OF LEACHATE
          FROM AN OPERATING SECTION AND A TWENTY-YEAR OLD ABAN-
          DONED SECTION OF A LANDFILL IN SOUTHEASTERN PENNSYL-
            VANIA. ^3)  (All constituents in mg/l, where applicable.)
                                     Operating            Abandoned
                                      landfill               landfill

Specific Conductance (y mhos)            3,000               2,500

BOD                                  1,800                  18

COD                                  3,850                 246

Ammonia (NH3 as N)                      160                 100

Hardness (as CaCO^)                       900                 290

Iron (Total Fe)                             40.4                 2.2

Sulfate (SO4)                             225                 100
Note:  Samples collected in 1970
                                204

-------
conductance, ammonia nitrogen, and sulfate are not as sig-
nificant.  Although concentrations of iron and hardness are
considerably lower in the leachate from the older portion of
the landfill, this site must still be considered a source of
contamination, even 20 years after being abandoned.

Case Histories

The results of research on two landfills are described below
in some detail.  The first case is a continuing investiga-
tion of a regional municipal landfill at State College,
Pennsylvania, by the Pennsylvania State University.  It was
chosen because it is a study of the character and movement
of landfill leachate through unsaturated soil. 104,105)  The
second case history involves a municipal landfill in south-
ern Connecticut.  It is included because of its typical wet-
land location in an area where the water table is actually
in contact with the refuse. 43,106)  Finally, significant
data from other selected case histories are tabulated, based
on a survey of available information in the 11-state study
area.

Case History Number One -

The State College, Pennsylvania, landfill occupies a gently
sloping dolomite valley with the water table more than 200
feet below land surface.  The approximately 100 tons of
municipal refuse brought to the 108-acre site each day is
placed, unprocessed, in trenches excavated into sandy clay
to sandy-loam soils and then covered.  In some portions of
the landfill, the buried refuse lies directly on bedrock of
Cambrian Age consisting of an interbedded series of dolo-
mites, sandy dolomites, and quartzites.  In other portions,
the refuse is underlain by layers of residual soils which
can be as much as 70 feet thick.

Suction lysimeters were placed beneath two cells  (trenches
containing refuse), one filled with waste material in  1962
and the other in 1967.  During July, 1970 and at other peri-
ods, soil moisture and water samples were extracted at dif-
ferent depths from beneath the two refuse cells and analyzed
for various physical and chemical characteristics.

The data collected indicate that the leachate front result-
ing from water percolating through the 1962 refuse cell, and
to some degree through other cells nearby, had moved down-
ward about 50 feet in eight years or at an average rate of
six feet per year.  Beneath the 1967 installation, the leach-
ate front had moved at an average rate of 11 feet  per  year
and had penetrated to a depth 30 feet below the bottom of

                              205

-------
 the cell after only two years and nine months.

 It has been concluded that leachate beneath the two cells
 has been reduced in mineral concentrations  during its down-
 ward movement through the subsoil.   The mechanisms observed,
 together with supporting evidence,  include  the  following:  104)

 1.   Dilution and dispersion (decrease in chloride with depth)

 2.   Oxidation (Eh and pH measurements - decrease in BOD and
     iron with depth)

 3.   Chemical precipitation (decrease in soil extractable
     phosphate after leachate  percolation)

 4.   Cation  exchange (increase in  percent base saturation of
     clays affected by leachate, and depletion of ammonia un-
     der reducing conditions - bacterial growth  may also re-
     tard or remove ammonia)

 5.   Anion exchange (decrease  in sulfate with depth)

 However,  even though  renovation does occur,  it  is not suffi-
 cient to prevent  highly  contaminated water  from moving to
 significant depths beneath the cells.   For  example,  Table  34
 shows the analysis of water collected in July 1970,  from
 soil  36  feet  below the 1962 cell.

 In  addition,  water from  a  well drilled into  the bedrock at
 the  landfill  site  showed an indication of contamination from
 leachate  entering  fractures and sinkholes, or infiltrating
 through  the  soils  along  the valley  bottom.   Chloride concen-
 tration  in  water  from this well,  for example, was 50 mg/1
 during  1970-71 as  compared to  a normal for unaffected ground
 water in  the  area  of  about two mg/1.   Alkalinity as  HC03 was
 as much  as  520 mg/1 during the same  period as compared to  a
 normal of about 130 mg/1.

 This  research  is especially significant  when  related to cur-
 rent  regulations regarding design of new landfills in the
 study region.  Many states call for  a  separation of  three  to
 five  feet between  the base of  the refuse and  the top of the
water table as one of the  protective measures against poten-
 tial  contamination of ground water.  As  indicated above, at
 least under some conditions, pollutants  can move through un-
 saturated soils to depths  greater than called for by exist-
 ing and proposed codes.  Consequently, Pennsylvania  has been
 requiring the  lining of new landfills with materials  of low
permeability  in combination with  leachate collection systems.
Delaware has proposed the  lining  of  new  landfills constructed

                             206

-------
Table 34.  ANALYSIS OF LEACHATE FROM SOIL 36 FEET BELOW 1962 REFUSE
          CELL, STATE COLLEGE PENNSYLVANIA REGIONAL LANDFILL.  104)
                   (All constituents in mg/l, where applicable.)
Specific Conductance  (pmhos)                          6,600

Chloride (Cl)                                            600

BOD                                                 9,000

Ammonia (NH3 as N)                                      40

Iron (Total  Fe)                                           100
Note; Sample collected in July 1970.
                                 207

-------
 in  its  Coastal  Plain  region.  Also,  instances exist in other
 states,  such  as New Jersey  and New York,  in which new munic-
 ipal  solid-waste  sites  are  being  lined with clay, bentonite,
 or  plastic membranes  in order to  prevent  the migration of
 leachate into the subsurface.  Treatment  of leachate col-
 lected  from such  sites  is planned, but little experience
 exists  with regard to the various methods that might be suc-
 cessful in the  handling of  this complex fluid.

 Case  History  Number Two -

 The results of  the 1973 investigation described below were
 obtained from a detailed study of a  90-acre landfill site in
 southern Connecticut.   The  refuse, consisting of municipal
 solid wastes  plus a small percentage of solid and liquid
 wastes  from local industries, has been deposited in a wet-
 land  for more than 30 years.  Portions of the refuse had
 reached  a thickness of  30 feet above the original marsh
 level.

 The purpose of  the investigation  was to determine whether
 the presence  of the landfill had  degraded natural conditions
 at  the  site to  the point where it no longer was suitable for
 consideration as  a future recreational area.  To accomplish
 this  task, a  detailed program of  test drilling, and chemical
 and physical  sampling of surface  water and ground water was
 carried  out.  Geophysical methods were employed along with
 other survey  techniques  to establish geologic and hydrologic
 conditions.   Finally, multispectral imagery was used to help
 define areas  where  remaining vegetative communities had been
 affected  by the presence of the landfill.

 The site  is adjacent to  Long Island Sound, a salt-water body
 separating the  Connecticut coast  from Long Island, New York.
 The area  occupied  by the landfill is directly underlain by
 40  to 60  feet of  generally unsorted glacial sands and silts
 which, in turn, rest on  crystalline bedrock.  The landfill
 itself has a  relatively  flat surface and is covered with
 relatively coarse-grained fill or partially shredded garbage
 from a recently constructed volume-reduction plant.  A sepa-
 rate portion  of the site contains fly ash, landfilled by a
nearby power plant.

The results of  the  investigation  of conditions at the site
revealed  the  following:

 1.  The water table has been raised more than eight feet into
    the refuse due  to infiltration of precipitation falling
    on the landfill.
                             208

-------
2.   The abnormally high water table has adversely affected
    the remaining vegetation around the landfill and has
    created standing surface water bodies of leachate,  where
    the water table intersects the land surface.

3.   An average of approximately 80,000 gallons per day of
    new leachate is being formed and is moving through the
    unconsolidated sediments beneath the landfill at a rate
    of approximately 0.25-foot per day.  This water is con-
    tinuously discharging to Long Island Sound, standing
    surface water bodies, and streams draining the area.

4.   The total volume, at any given moment, of ground water
    in storage that has been contaminated because of dis-
    posal of solid waste at the site is about several hun-
    dred million gallons.  This body of contaminated ground
    water underlies an area approximately 3,500 feet long
    and 3,000 feet wide.  It has been found in test holes to
    a depth of 60 feet below the base of the landfill.

5.   High counts of coliform bacteria have been determined in
    the standing surface-water bodies affected by leachate
    and also in seeps and springs issuing from the landfill.

6.   Very high concentrations of such constituents as alka-
    linity, total hardness, specific conductance, COD, am-
    monia, chloride, iron and manganese were found in water
    directly beneath the landfill itself.  However, some
    renovation of contaminated ground water is taking place
    as it moves through the subsoils.  Test wells drilled
    200 feet or more from the landfill yield water signifi-
    cantly less contaminated than that found directly be-
    neath the refuse.

Table 35 shows chemical analyses of selected constituents of
water from wells drilled into the water-table aquifer under-
lying that portion of the landfill containing refuse and
that portion containing fly ash.  These  analyses are com-
pared with those of water from a well drilled 200 feet  from
the toe of the landfill and an off-site  well, where the
glacial aquifer is essentially unaffected by leachate from
the landfill.

The table shows the typical contamination of ground water
that has been affected by refuse, as indicated by the high
concentrations of each of the constituents  in water from the
refuse-area well.  In addition, the pH is on the acid side.
When these concentrations are compared to those  in water
from the well 200 feet from the landfill, a marked differ-
ence is apparent, but ground water is still contaminated,

                             209

-------
Table 35.  PARTIAL CHEMICAL ANALYSES OF WATER FROM WELLS LOCATED
          IN AND NEARBY A LANDFILL SITE IN SOUTHEASTERN CONNEC-
            TICUT.  ^'  (All constituents in mg/l, where applicable.)
Well location
Date sampled
PH
Alkalinity (CaCOs)
Total Hardness
(CaC03)
Calcium Hardness
(CaC03)
Specific Conductance
(y mhos/cm)
Chemical Oxygen
Demand (COD)
Ammonia (N)
Chloride (CI)
Iron (Fe)
Manganese (Mn)
Off-site
5-10-73
5.9
8.0

64

28
142
34
0.018
7.0
0.25
0.08
200 feet
from toe
of landfill
7-12-73
8.9
540

300

40
1,840
NA
NA
280
2.4
0.14
Refuse
area
7-6-73
5.8
1,700

2,240

1,300
5,990
12,400
103
650
63
12
Fly-ash
area
5-10-73
3.8
3,885 a)

540

80
4,610
227
6.0
40
252
6.25
NA - Not analyzed

a)  Total acidity
                              210

-------
with levels of such constituents as iron, manganese, and
chloride above limits recommended for drinking waters.  The
quality of ground water beneath the fly ash is most interest-
ing.  The highly acid leachate created by infiltration of
rain water through the fly ash apparently has dissolved pre-
cipitated iron, which occurs naturally in the underlying
glacial sediments.

It has been recommended that the existing landfill be aban-
doned because of the inadequacy of the site for solid-waste
disposal.  An attempt will be made to contour the final
shape of the landfill and cover it with a material of low
permeability in order to increase runoff and decrease infil-
tration of precipitation into the refuse.  If successful,
this procedure would cause the abnormally high water table
to decline, reducing the generation of additional leachate.
The landfill also generates considerable gas, including
methane and carbon dioxide, which will require venting as
part of the final design.

The case history discussed above is typical of the  situation
at numerous landfills throughout the northeast.  Large land-
fills placed in unsuitable sites can generate considerable
quantities of leachate that enter the ground-water  system.
Also, if placed directly above the water table, a portion of
the refuse can become permanently saturated and create prob-
lems of an esthetic nature in addition to those associated
with contamination of ground-water resources.  Finally,
leachate flowing directly out of such landfills, and  the dis-
charge of contaminated ground water, can degrade the  chemi-
cal and biological quality of nearby surface waters.

Although determination of whether toxic  substances  in ground
waters associated with the sites discussed above was  not a
part of the studies, analyses of water from wells near some
other landfills in the region have shown the presence of
such pollutants.  Information on this problem is included in
the tabulated case histories given below.

Tabulation of Case Histories -

This inventory of ground-water  contamination problems in the
northeast uncovered about 100 cases  in which landfills were
pinpointed as the source.  Table 36  summarizes the  key data
developed from 60 of these cases,  selected on the basis of  a
high level of reliability of the information available.  In
addition to those obtained from interviews and public agency
files, a number were taken from published  sources and unpub-
lished reports.  107,108,109)
                             211

-------
Table 36. SUMMARY OF DATA ON 42 MUNICIPAL AND 18 INDUSTRIAL LANDFILL
                               CONTAMINATION CASES.

                                                                 Type of Landfill
                                                           Municipal        Industrial

Assessment of principal damage
     Contamination of aquifer only                               9                8
     Water supply well(s) affected                               16                9
     Contamination of surface water                             17                1

Principal aquifer affected
     Unconsolidated deposits                                    33               11
     Sedimentary rocks                                           7                3
     Crystalline rocks                                           2                4

Type of pollutant observed
     General contamination                                     37                4
     Toxic substances                                            5               14

Observed distance traveled by pollutant
     Less than 100 feet                                           6                0
     100 to 1,000 feet                                           8                4
     More than 1,000 feet                                      11                2
     Unknown or unreported                                     17               12

Maximum observed depth penetrated by pollutant
     Less than 30 feet                                          11                3
     30 to 100 feet                                             11                3
     More than 100 feet                                          5                2
     Unknown or unreported                                     15               10

Action taken regarding source of contamination
     Landfill abandoned                                          5                6
     Landfill removed                                           1                2
     Containment or  treatment of leachate                        10                2
     No known action                                          26                8

Action taken regarding ground-water resource
    Water supply well(s) abandoned                             4                5
     Ground-water monitoring program established                 12                2
     No known action                                          26               11

Litigation
     Litigation involved                                         8                5
     No known action taken                                     34               13
                                          212

-------
The landfills have been separated according to type.  The 42
municipal landfills are operated primarily as sites to re-
ceive domestic garbage and other wastes generated in a com-
munity, such as leaves, road sweepings, construction debris,
and commercial rubbish.  Many of these also accept septic-
tank pumpings, sewage-plant sludges, and some industrial
sludges and liquids.  The 18 industrial landfills listed are
privately owned and accept primarily industrial solid wastes
from manufacturing processes and some sludges and liquids
from water and waste-water treatment systems.  The vast ma-
jority of these serve one industrial site and are located on
the plant property.  A few are operated by contractors who
accept waste from several industries in a particular area.

Although more municipal than industrial landfills are repre-
sented in the table, the latter are much more abundant in
the northeast.  However, the location and even the existence
of industrial landfills rarely are recorded with any public
agency.  Thus, they are not inspected on a routine basis,
and problems do not become evident unless ground-water con-
tamination is obviously taking place.  In the case of the
municipal landfills, although their locations are generally
known to regulatory agencies, few are monitored and, again,
contamination of ground water normally takes place unob-
served .

The most important aspect of Table 36 is that there are
thousands of other landfills in the northeast located in the
same types of geologic environments and designed in the same
manner as those appearing on the table.  There is no tech-
nical or scientific reason why the vast majority of these
are not additional sources of ground-water contamination.

The lack of ground-water monitoring is indicated by the high
number of cases in Table 36 where contamination of  surface
water is reported as the principal damage.  Many problems
are first observed when the discharge of contaminated ground
water affects nearby surface waters, which are more often
subjected to periodic measurement of water quality  than are
ground waters.  The cause of pollution in a stream  or lake
near a landfill can be traced with  little difficulty.  In
addition, it is considerably less costly, if contamination
is suspected, to sample ground-water discharge from the land-
fill in the form of seeps and springs than it is to drill
and test water from observation wells.  Thus, because the
damage done to the aquifer is not known, the problem is re-
ported initially as one of surface-water pollution.

As indicated, there are a number of instances in which water-
supply wells have been affected by municipal and  industrial

                             213

-------
 landfills.   In some cases, the wells must be abandoned,
 especially where public supplies are involved and chemical
 concentrations exceed recommended health limits,  or a toxic
 substance is present in the water.  An example of this is
 the loss of 10 percent of the well-supply capacity of the
 City of Newark, Delaware, because of contamination from a
 community landfill. 110)

 A number of examples exists where only the aquifer has been
 affected so far, but the  plume of contaminated ground water
 is moving toward and threatening a well supply.   Such a
 case was recently discovered in southern New Jersey where
 leachate, containing up to 18 mg/1 of lead,  has traveled at
 least 500 feet through coastal plain deposits toward city
 supply wells located 4,000 to 6,000 feet away from an indus-
 trial landfill.   A ground-water monitoring program has been
 established and the landfill has been closed down.

 In some cases,  wells have been affected by a contaminant but
 their use is continued because either the various constitu-
 ents have not reached critical levels or a treatment system
 has been installed.   For  example,  several domestic wells in
 Ledyard,  Connecticut,  tapping a crystalline  rock  aquifer,
 were contaminated by styrene,  an aromatic hydrocarbon.   The
 maximum lateral  observed  distance  of travel  through joints
 and fractures was 110  feet,  to a well 180 feet deep.   Acti-
 vated-charcoal filters were  installed for treatment on some
 of the  affected  wells.  The  source of the contaminant, par-
 tially-filled drums  of styrene that had been buried at
 various locations in the  area,  was removed by excavation of
 both the  drums and the affected soil.   After removal  of  the
 source,  it  took  about  two years before styrene was  no longer
 detected  in the  water  from any of  the wells.  HI)

 Table  36  also shows  that  in  most of the cases recorded,  the
 principal aquifer affected consists of unconsolidated e-
 posits.   Because the wastes  are disposed of  at land surface,
 it  is these shallow  deposits,  which mantle the bedrock
 throughout  the region,  that  are affected first.   Furthermore,
 many landfill sites  are chosen where there are relatively
 thick beds  of sand available,  which can be used on-site  for
 cover material or can  be  trenched  easily for  burial of the
 refuse.

 In a few  instances,  such  as  that described above  in Connec-
 ticut,  the  contaminant  infiltrates  through the overburden
 into the  bedrock before discharge  to a  surface-water  body.
 In others,  the solid waste is  deposited in direct contact
with a bedrock aquifer, for  example,  at such  sites  as  strip
mines,  sinkholes,  and  abandoned deep mines.   Garbage  dumped

                             214

-------
over a period of many years into a deep abandoned and flood-
ed mine in northern New Jersey has contaminated at least two
wells in the area. 112)  The methane content in water from
both wells, one of which is 250 feet away from the mine
shaft, has been rising over the years, as have chloride and
iron concentrations, which have reached levels of 160 mg/1
and 16 mg/1, respectively.

Toxic substances were reported associated with contamination
from industrial landfills in almost all cases, because mate-
rials containing heavy metals and synthetic organics, for
example, are a part of so many manufacturing processes.  Al-
so, hazardous industrial wastes are kept on-site at many
plants because they are unacceptable at municipal landfills.
Toxic substances would probably be observed at more munici-
pal landfills if more detailed analyses were made of the
leachate.  Typically, the lack of staff and budget prevents
a public agency from conducting complete analyses on enough
samples to definitely establish toxicity.  In contrast, the
type of product disposed of in the industrial landfill is an
excellent indication of the nature of the pollutant, and an
analysis of selected constituents can be run initially if
contamination is suspected.

Determination of distance and depth penetrated by a pollu-
tant requires a rather elaborate test-drilling program, and
therefore this information is not available for many of the
landfills included in the table.  The data shown were based
on those cases where water-supply wells had been affected,
and distances and construction details for the affected
wells had been reported by the investigating  agency or or-
ganization.  In a few  instances, monitoring wells had been
installed or a detailed investigation, including test drill-
ing, had been carried  out.  One such  case involves a large
regional landfill in southeastern New York State. 113) Here,
test wells  drilled into a  60-foot thick municipal landfill
situated in a wetland  have shown contaminated ground water
to a depth  of 70  feet  below the base  of the landfill.  The
aquifer underlying the site consists  of lacustrine and
coarse-grained glacial sediments.  The leachate bailed  from
wells  located in  the landfill  itself  and drilled into the
water  table, which had risen a maximum of 14  feet above the
old marsh  level,  contained high concentrations of such  con-
stituents  as chlorides, total  dissolved solids, total hard-
ness  (as CaCOs),  and iron  (2,900 mg/1;  9,416 mg/1;   480 mg/1;
and  48 mg/1, respectively).  Natural  ground water from  the
same aquifer in this area  is of high  quality.

One  interesting aspect of  that  investigation  is  the  fact
that  anomalous temperatures could be  used to  trace the  plume


                             215

-------
 of  contaminated  ground water  as  much as  700  feet  from the
 toe of the  landfill.   For example/  the termperature  of
 ground water  at  the  top of the water table within the land-
 fill itself was  120°F.   Seven hundred feet away and  70 feet
 below the landfill  ground-water  temperatures were still
 three degrees above  the normal 51°F for  ground  water in the
 region.

 The lack of any  cases  of industrial landfills where  the max-
 imum distance traveled by the pollutant  is less than 100
 feet may be related  to the fact  that most of the  industrial
 sites are located on private  lands, and  the  contamination
 does not become  a matter of public  concern until  the pollu-
 tant has moved beyond  property limits.   Also, only a small
 percentage  of industrial wells are  sampled by regulatory
 agencies, and if contamination is dicovered  by  the industry
 in  its own  wells, there is an obvious reluctance  in  report-
 ing the problem  to local and  state  health authorities.   To
 date,  little  regulatory action has  been  concentrated in this
 area.

 Because of  the large volumes  of  waste material  involved, re-
 moving the  source of contamination  when  dealing with land-
 fills  is obviously almost  impossible.  Thus, most of the
 cases  included in Table 36  are listed under  the category "no
 action taken".   In a few,  involving small quantities of tox-
 ic  wastes,  the material causing  the problem  was excavated.
 In  others,  the landfill has been closed, but this alterna-
 tive  also is  difficult  to  accomplish because a  new landfill
 site must be  found and  approved, or new  facilities must be
 designed and  constructed for  handling the waste in a manner
 different from landfilling, such as  recovery, treatment, or
 incineration.  Even in  cases  where  well  supplies  have been
 affected, abandonment of the  wells  is a  last resort  because
 of  the high costs involved  in developing and piping  a new
 source of water  supply.

 Finally, a  few landfill  contamination cases  are known to
 have resulted in litigation.  This  procedure normally takes
 the  form of a local or  regional  regulatory agency using ex-
 isting laws in order to  force the polluter to take action in
 cleaning up the problem.   In  one instance, the  Federal
 government has brought  action against a county  landfill  and
based the suit on the 1899 Refuse Act.

Future Trends

Because water pollution associated with landfills  is  becom-
ing such an obvious problem,  state  and other regulatory  agen-
cies in the region are  in the process of preparing new
                             216

-------
regulations or modifying old ones to better control this
activity.  To a large degree, these are directed toward the
design and siting of new municipal landfills.  Industrial
landfills will continue to be difficult to control, if lo-
cated on a particular plant property, unless more successful
methods for inventorying solid-waste sites are developed,
perhaps using advanced aerial photographic techniques.

New regulations normally call for geologic and hydrologic in-
vestigations of proposed sites and require such information
as water-table elevation;  direction of ground-water flow;
distances to existing well supplies in the area;  depth,
thickness, and character of the overburden;  and details of
the bedrock aquifer.  Although there is much variation in
the details included in regulations and guidelines, a 60-
inch separation between the highest anticipated level of the
water table and the base of the landfill is a typical re-
quirement.  A buffer zone of 50 to 100 feet between the ref-
use area and the property boundary is called for by most
agencies.  Distances to the nearest operating wells normally
are not specified but are to be determined on a case by case
basis.  Finally, the majority of new regulations call for
1) the sloping of the surface of the landfill to maximize
runoff and minimize infiltration, 2) prohibition or curtail-
ment of the dumping of hazardous or toxic solid and liquid
materials, and 3) installation of monitoring wells.

Undoubtedly, these new regulations and the greater interest
on the part of public agencies will help to reduce some
serious ground-water contamination problems that otherwise
would have occurred.  However, the guidelines are based on
insufficient research into such factors as the true charac-
ter of leachate from various types of landfills, the  ability
of different soils to reduce the concentrations of different
types of leachates, and the effects of landfill cover mate-
rial, slopes, and thickness on infiltration of precipitation,
Therefore, it is not known how effective the new codes will
be in actually preventing ground-water contamination.   In
fact, some of the guidelines mentioned above may have little
effect, based on known cases of ground-water contamination
where pollutants have moved through unsaturated materials
and have traveled horizontally for thousands of feet.

Some new landfills in the region are being constructed with
clay or  synthetic liners.  These are used in combination
with a system of drains to collect leachate before it can
seep into an underlying aquifer.  One of the first of this
type has been installed in Pennsylvania, in which  an  acid-
resistant bituminous mat was placed on the base of a  160-
foot deep, 10-acre limestone quarry. 114)  others  are being
                              217

-------
 proposed or are  under construction in  sections  of New York,
 New Jersey,  Pennsylvania,  and Delaware.   The  major problem
 involved with this  approach is the lack  of experience and
 difficulties involved in the collection  and treatment of
 leachate.   Undoubtedly,  the use of liners will  be required
 more and more in the  study area,  especially where critical
 aquifers would otherwise be threatened or where nearby ex-
 isting  landfills have already been proven as  sources  of
 ground-water contamination.

 Another approach being considered toward diminishing  the
 many types  of problems involved in landfilling  is to  reduce
 the volume  of solid waste  to be handled.   Alternatives al-
 ready in practice or  proposed include  incineration, pyrol-
 ysis, composting, or  recycling.   All of  these either  create
 other environmental hazards,  such as air pollution in the
 case of incineration,  or are  not  economically attractive
 enough  to have received  the  acceptance required to make a
 significant  impact.   Thus,  solid-waste generation will prob-
 ably continue to increase  at  its  present accelerating rate,
 unless  environmental  restraints on siting,  including  re-
 quirements  for artificial  liners,  make the various alterna-
 tives listed  above  economically more attractive.   Finally,
 concern over  air pollution  and surface-water  quality  may
 actually lead to a  greater use of the  land for  disposal of
 wastes  that  formally were  discharged into these other two
 environments.

 With the trend toward  greater  use  of monitoring wells by
 public  agencies  as  a means to  regulate ground-water quality,
 it  is reasonable  to predict that  there will be  an accelera-
 tion of  new problems discovered at  existing landfills.  Un-
 fortunately,  adequate  alternatives  for eliminating the land-
 fill as  a continuing source of  contamination  have not been
 developed, and, because  of this,  there do  not appear  to be
 any  clear-cut  guidelines or policies that  can be  followed.
 The  same holds true for  how to  contain or  remove  the  pollu-
 tant after it  has entered the ground.

 Contouring or  grading  and then  covering  the landfill  with  a
 relatively impermeable material on which  soil can be  placed
 and vegetation established is being attempted at  a number  of
 sites in the  region as a means of  limiting the  formation of
new  leachate.  However,  not enough history on this method
has been developed  to  comment on potential for  success.
Pumping from properly  spaced and  constructed wells is  another
alternative for containing or removing the pollutant,  but
this has been proposed only as a  last  resort.    Pumping is  a
 slow and costly process, which is not  always successful and
can create other serious environmental problems.   Research


                              218

-------
on these vital aspects of ground-water quality protection is
badly needed.

SURFACE IMPOUNDMENTS

Contamination of ground water caused by leakage of pollu-
tants from any type of surface impoundment, either natural
or man made, is dicussed in this section.  Such an impound-
ment may be a rock quarry into which an industry is dumping
untreated waste that is unacceptable for treatment by the
local municipal sewage treatment plant.  It can be a sink-
hole in a limestone area where liquid and sludge from the
cleaning of septic tanks are deposited by a local contractor,
or it can be a kettle hole in the glaciated region used as a
holding pond for metal plating wastes.

Some impoundments for wastes are constructed by diking off a
wetland, for example, or by excavating a lagoon or basin in
unconsolidated deposits.  These sites are typically used for
storing industrial and sewage sludges in order to settle out
the solid material from the wastes or to allow evaporation
or oxidation to take place.  They may temporarily hold
brines for later treatment and disposal or for concentration
and recovery of heavy metals.  Some lagoons and basins are
lined with clay, concrete, asphalt, or plastic membranes.

Both lined and unlined pits are other widely used types of
surface impoundments constructed to hold storm-water runoff
from highways and from paved areas at industrial sites.
They are normally designed to deliberately discharge liquids
to the soil or to feed a buried sewer collection system.
Some pits are used as sumps to house pumping installations
for sewage, industrial wastes, or fluids from a particular
manufacturing process.  Concrete and metal sheeting are the
most frequently used materials for lining.

The size of surface impoundments varies  considerably.  They
can be a series of cooling ponds receiving thousands of gal-
lons per minute of hot waste water and covering hundreds of
acres.  On the other hand, a small unlined pit can be only
a few feet in diameter and used to dispose of highly toxic
wash water from a photographic laboratory.  Most lagoons,
pits, and basins are relatively shallow, holding less than
10 feet in depth of material on the average at any given
moment.  Exceptions are deep quarries or mine shafts re-
ceiving liquid wastes and sludges.

Statistics on the number and location of surface impound-
ments that may be a potential threat to  ground-water quality
have never been compiled for the northeast.  Pennsylvania


                              219

-------
has made  the  only known  inventory  on  a  regional basis.  By
means of  low-level  aerial  survey flights  conducted  over
selected  portions of  the state, it was  estimated  that more
than 1,500  industrial waste  impoundments  exist in the Com-
monwealth of  Pennsylvania. 36)  Because lagoons,  pits and
basins  are  such  a common means for treating, handling, and
storing liquids  and sludges,  it is conceivable that seven to
ten thousand  of  these impoundments are  present in the study
region.   Their potential for  leaking  many millions  of gal-
lons per  year of potentially  hazardous  materials  into the
ground-water  system is significant enough to be of  consider-
able concern  to  water regulatory agencies.

This concern  is  justified on  the basis  of a number  of fac-
tors inherent to the  design and operation of surface im-
poundments.   First, few  were  designed with any consideration
given to  protecting ground-water quality, and many  operate
on the  principle that at least some fluid will be lost to
the ground.   Typical  is  the so-called evaporation pond which
contains  industrial waste and only operates successfully in
this humid  region if  enough leakage is  taking place through
the bottom  and sides  of  the impoundment to create additional
storage space for continued waste  discharges.  Many unlined
surface impoundments  are located in geologic settings that
are highly  susceptible for leakage to take place.   Data on
case histories collected in this investigation have shown
that abandoned sand and  gravel pits,  sinkholes, swamps over-
lying permeable  unconsolidated deposits,  mine excavations in
highly  fractured rock, and other areas  where pollutants have
easy access to important aquifers  are quite typical sites
for surface impoundments.  No general guidelines  have been
enforced  until recently  regarding  siting  or designing new
surface impoundments  from the standpoint  of ground-water pro-
tection.  Consequently,  lagoons, pits,  and basins are lo-
cated and constructed to meet other criteria, such  as con-
venience  and  lowest possible  cost.

Even in the case of some lined impoundments, the  potential
for leakage can  be  significant.  Various  types of clay are
probably  the most universally employed  lining materials.
However,  they are not impermeable, and  enough volume of a
highly concentrated pollutant can  leak  from a large  lagoon
to damage ground-water supplies under certain conditions.
For example,  a lagoon 20 acres in  size  and 10 feet  deep,
lined with a  two-foot thick clay blanket with a typical
permeability  of  0.001 gallons per  day per square  foot can
leak about 1.5 million gallons of  fluid per year  into the
ground-water  system.  If the  fluid is an  industrial waste
and little change in  water quality from contact with the
natural soil occurs before the pollutant  arrives  at the

                              220

-------
water table, then a potentially serious contamination prob-
lem can occur.  If 1,000 feet is the distance from the la-
goon to the nearest well tapping the water-table aquifer,
and ground water is moving toward the well at a rate of 0.5
foot per day, it would take more than five years before the
plume of contaminated water would be detected.  Meanwhile,
7.5 million gallons of the waste water would have leaked
into the aquifer.

It is quite probable that much leakage of fluids takes place
through the sides of excavated lagoons and basins rather
than the bottom which can become clogged with settled solids
and sludges.  In some well documented cases of ground-water
contamination, it was the erosion of the natural soils or
the rupture of artificial linings on the sides of the im-
poundment that allowed leakage to occur at a rate great
enough to significantly degrade ground-water quality.

Another major concern is the general lack of metering of
waste discharges into holding ponds, lagoons, and basins.
If losses of fluids to the ground-water system are taking
place, this condition generally continues unobserved for ex-
tended periods.  In addition, the use of monitoring wells to
determine whether leakage is occurring and is affecting
ground-water quality in the vicinity of existing surface im-
poundments is rare.

Also, a large variety of wastes is treated in lagoons and
oxidation and stabilization ponds.  Most of the substances
are complex, and many of the constituents that could find
their way into ground waters are not normally included in
routine analysis of water supplies.  E. B. Besselievre in
his book "The Treatment of Industrial Wastes" lists about 80
types of industrial, municipal, and agricultural activities
in which lagoons and ponds are used as part of the waste-
water treatment process. H5)  where industrial and domestic
sludges have been placed in surface impoundments, the solu-
bility of heavy metals in rain water has not been researched
in detail, nor has the fate of potentially toxic substances
that might enter the soil system.

Case Histories

The results of the inventory of ground-water contamination
problems involving surface impoundments, carried out as  part
of this 11-state investigation, emphasize the variety of the
pollutants and the diversity of the origins of waste water
that can be encountered.  Table 37 is based on 57 cases  of
contamination taken from the files of public agencies and
private organizations.  Each involves a separate location

                             221

-------
 Table 37. ORIGINS AND POLLUTANTS IN 57 CASES OF GROUND-WATER
          CONTAMINATION IN THE NORTHEAST CAUSED BY LEAKAGE OF
                WASTE WATER FROM SURFACE IMPOUNDMENTS.
 Type of industry or activity

 Chemical
Number
of__cqs_es_

   13
Metal processing and plating
Electronics
Laboratories (manufacturing and processing)
Paper

Plastics
   3

   3
 Principal pollu-
 tant(s) reported

 Ammonia
 Barium
 Chloride
 Chromium
 Iron
 Manganese
 Mercury
 Organic chemicals
 Phenol
 Solvents
 Sulfate
 Zinc

 Cadmium
 Chromium
 Copper
 Fluoride
 Nitrate
 Phenol

 Aluminum
 Chloride
 Fluoride
 Iron
Solvent

 Arsenic
 Phenols
 Radioactive
   materials
Sulfate

Sulfate

Ammonia
 Detergent
Fluoride
                                 222

-------
Table 37 (continued). ORIGINS AND POLLUTANTS IN 57 CASES OF GROUND-
                    WATER CONTAMINATION IN THE NORTHEAST CAUSED
                    BY LEAKAGE OF WASTE WATER FROM SURFACE IM-
                                  POUNDMENTS.
Type of industry or activity

Sewage treatment


Aircraft manufacturing


Food processing


Mining sand and gravel

Oil well drilling


Oil refining

Battery and cable


Electrical utility


Highway construction

Mineral processing

Paint

Recycling

Steel


Textiles
Number
of cases
 2

 2


 2

 1
Principal pollu-
tant(s) reported

Detergents
Nitrate

Chromium
Sulfate

Chloride
Nitrate

Chloride

Chloride
Oil

Oil

Acid
Lead

Iron
Manganese

Turbidity

Lithium

Chromium

Copper

Acid
Ammonia

Chloride
                                 223

-------
 where leakage of pollutants out of some form of surface im-
 poundment has entered the ground-water reservoir.   In most
 cases,  water-supply wells have been affected,  and  this is
 the only reason that the specific incident has been reported
 or investigated.   In a few, simply observing operation of
 the lagoon or basin has led officials  of an environmental  or
 health  agency to investigate whether ground-water  contamina-
 tion has taken place.   In others,  the  polluter has noted the
 loss of a highly toxic substance to the ground and has
 brought this  to the attention of authorities.   Wells em-
 placed  before contamination was suspected and  drilled specif-
 ically  to monitor possible changes in  ground-water quality
 were not listed as the reason for  discovery of any of the
 cases.

 The types of  surface impoundments  represented  in the 57
 cases vary considerably,  but lagoons and basins are listed
 most frequently.   An interesting example other than a la-
 goon or basin is  a small  limestone quarry located  immedi-
 ately behind  a  battery manufacturing plant in  Pennsylvania.
 The impoundment was  spotted during an  aerial survey by a
 geologist of  the  State's  Department of Environmental Re-
 sources.   It  was  noted that the quarry contained water but
 should  have been  dry under natural conditions  based on the
 geology and topography of the  area.  Further investigation
 revealed that the  quarry  had been  used for about six years
 as  a discharge  area  for plant  effluent with a  pH level of
 2.9  and a lead  content of 4.12  mg/1.   The waste disposal
 practices were  altered, but the extent of the  damage of the
 aquifer remains unknown.  36)

 Other examples  include  a  case  in Maryland where a  three-foot
 wide, 48-foot long,  and 10-foot deep concrete  canal,  used
 for  storage of  radioactive  material  at a private laboratory,
 leaked  an estimated  20,000  gallons  of  slightly radioactive
 water into a  thin  soil  layer overlying Triassic shale  and
 sandstone.  The leak was  reported  to state authorities  by
 the  company,  and  to  date,  six monitoring wells  have  been in-
 stalled in and  around  the facility  to  determine where  the
 pollutant  has traveled.   A small amount  of cobalt-60  activ-
 ity  has  been  picked  up  in some  observation wells,  and  the
 investigation is  continuing.  Meanwhile,  use of the  canal
has  been  curtailed.  116)

An abandoned  sand  and  gravel pit was used by a  paint manu-
 facturer  in Maryland to place  liquid and sludge wastes  re-
moved from a  stream  during  a clean-up  operation.  Monitoring
wells installed later  on  the edges of  the  pit  and  driven to
a depth of 15 feet produced  water with  a chromium  (hexa-
valent)   content of as much as 7.2 mg/1.  117)

                              224

-------
Many of the pollutants reported in Table 37 are related to
hazardous wastes, as indicated by the large number of heavy
metals listed.  The concentrations of these toxic substances
can be very high at sites where the untreated industrial ef-
fluent is leaking from a surface impoundment and reaching
the saturated zone almost unchanged in chemical composition.
Concentrations of some of the heavy metals in water from a
lagoon containing untreated industrial sludges and liquid
wastes were:  copper 5,250 mg/1;  chromium (trivalent) 1,380
mg/1;  and lithium 280 mg/1.  The site was investigated by a
public agency after a stream near an abandoned plant prop-
erty showed indications of contamination.  The source of
pollution in the stream was traced to the lagoon which was
leaking the waste effluent to the ground-water system.  The
contaminated ground water, in turn, was discharging into the
stream.  The problem is presently in litgiation. 118)

The concentration of total chromium in water from a domestic
well, 700 feet away from leaky lagoons containing metal
plating waste, was measured at 150 mg/1 in a recent incident
discovered in New Jersey. 42)  The most grossly contamin-
ated ground water encountered in this investigation is a
case in which the pollutant was 10,000 mg/1 arsenic. 14)
Liquids and sludges containing arsenate compounds had been
deposited by a chemical company in unlined surface impound-
ments for many years, and the plume of contaminated ground
water had reached a stream adjacent to the plant site where
arsenic concentrations as high as 40 mg/1 were observed.
The lagoons were abandoned after the problem was recognized
and the wastes stored in plastic-lined drums.  Also, an at-
tempt has been made to pump out the contaminated ground wa-
ter.  After 2-1/2 years of careful pumping and monitoring,
concentrations of arsenic in both ground water and surface
water have been greatly reduced, but the condition is still
dangerous.

Few of the 57 cases in Table 37 have been investigated in
great enough detail to develop statistics on size of area
contaminated and the nature of the pollutant in the ground.
There are reported instances of large plumes of contaminated
ground water extending for several miles from waste lagoons,
but the little information gathered has never been published
nor verified by detailed subsurface exploration and testing.
Even where some investigation has been carried out, a pri-
vate company is normally involved as the polluter, and the
information is not made readily available to the public,
especially if litigation is involved.

However, to provide some insight into typical ground-water
contamination cases, Table 38 has been prepared based on

                              225

-------
 Table  38.  THREE CASE HISTORIES OF GROUND-WATER CONTAMINATION FROM
                      LEAKAGE OUT OF SURFACE IMPOUNDMENTS.
 Description of Surface
   Impoundment
 Type of Waste

 Principal  Pollutant(s)
 Observed and Maximum
 Concentrations Reported
 in affected wells (mg/l)
   Chromium (Hexavalent)
   Cadtmum
   Cyanide
   Zinc
   COD
   Copper
   Chromium (Total)
   Nickel
 Dimensions of Plume of Con-
 taminated Ground Water
   Maximum Length (feet)
   Maximum Width (feet)
   Maximum Depth (feet be-
      low the water table)

 Estimated Maximum Volume
 of Contaminated Ground
 Water in millions of gallons
 and year
 Two disposal basins,
 65x65x15 feet and
 one disposal basin,
 130x54x15 feet
 One storage lagoon
 approximately
 50x50x10 feet
Aircraft manufacturing    Metal plating
      40
      10
      2.3

      0.4
      1.4
   4,300
   1,000
       70
   1,000
    200
     60
Year Reported

Remedial Action(s) and
Status of Problem
   200 (1962)
      1949
Periodic research and
monitoring;  affected
wells abandoned;  some
treatment and reduction
of waste effluent;  con-
centrations of chromium
and cadimum have de-
clined but problem still
present in  1974
    50 (1969)

    1969

Lagoon  and affected
wells abandoned;  no
further action; prob-
lem still present in
1974
Series of lagoons and
basins covering an
area of about 15 acres
and average about
six feet in depth

Chemical
                                                       50
                                                    5,000
                                                       135
                                                       150
                                                       10
    2,200
    1,200
        30
      20 (1972)

      1971

Lagoons and basins
sealed with cement
and/or plastic liners;
continuing program of
monitoring;  system of
pumping wells installed
to contain pollutants in
area of plant site and
in shallow aquifer zones;
problem still present in
1974
                                                 226

-------
three detailed studies in the region.   The first is the well
documented and frequently published case of the dispersal of
plating wastes in ground water in southeastern Nassau County,
Long Island, New York.  The most complete discussion of this
problem appears in U. S. Geological Survey Water Supply Pa-
per 1879-G. H9)  The other two investigations were carried
out by Geraghty & Miller, Inc., one in southern New Jersey
and the other in central Connecticut.  22,39)

All three situations are related to industrial waste water
having leaked out of surface impoundments.  This has result-
ed in a plume of contamined ground water migrating slowly
toward an area of discharge.  In two of the cases, major dis-
charge is to streams draining the affected water-table aqui-
fer.  In the third, the pattern of ground-water movement was
controlled by pumping from a series of water-supply wells,
which were abandoned after contamination was discovered.
What effect cessation of pumpage has had on the characteris-
tics of the body of contaminated ground water is unknown.

In two of the three cases, the plume of contaminated ground
water had moved beyond the property limits of the polluter
before the problem became known and was defined.  In only
one of the cases is hydraulic control over the vertical and
horizontal movement of the contaminated water being attempt-
ed by means of special pumping wells.

Future Trends

The severe cases of ground-water contamination related to
surface impoundments, that have become known in the region,
have led a number of states and at least one interstate
agency to develop regulations and programs directed at con-
trolling this problem.  Some of these controls are broadly
written to cover a wide variety of activities that might af-
fect ground-water quality but are particularly effective in
dealing with this source of contamination.  For example, the
Delaware River Basin Commission includes in their ground-
water quality control resolution of December 12, 1972, all
activities involving "the processing, handling, transporta-
tion, disposal, storage, excavation or removal of any solid,
liquid, or gaseous material on or beneath the ground surface
of the Basin."  In addition, the resolution states  "no sub-
stance or properties which are harmful or toxic concentra-
tions or that produce color, taste, or odor of the water
shall be permitted or induced by the activities of man to
become ground water." 120)

Maryland has established its general control over leakage
from surface impoundments on the basis of a discharge permit


                             227

-------
 requirement.   That  state's  regulation of May 1,  1973,  states
 "Any  discharge or disposal  of waters  or  waste waters  into
 the ground  waters of the  state will require  the  approval  of
 the Water Resources Administration."  121)

 Pennsylvania's regulations  are more specific and refer di-
 rectly  to impoundments. 122)   A 1971  Special Water  Pollution
 Regulation  includes the following: "no person or municipal-
 ity shall operate,  maintain or use or permit the operation,
 maintenance or use  of an  impoundment  for the production,
 processing, storage,  treatment or disposal of polluting sub-
 stances unless such impoundment is structurally  sound,  im-
 permeable,  protected from unauthorized acts  of third parties
 and is  maintained so that a free board of at least  two feet
 remains at  all times."  The regulation goes  further to de-
 fine  an impoundment as "any depression,  excavation, or facil-
 ity situated  in or  upon the ground, whether  natural or arti-
 ficial  and  whether  lined  or unlined."

 Of particular  importance  is the term  "impermeable"  in  the
 Pennsylvania  regulation which automatically  calls for  the
 use of  artificial liners  in any surface  impoundment contain-
 ing anything but  natural  waters.  Artificial liners are also
 being required by the Delaware River  Basin Commission,  New
 Jersey,  Maryland, Delaware  and in a few  counties in New York
 for new lagoons,  pits or  basins which  will hold  untreated
 industrial wastes.  Also, lining old  impoundments that have
 been  found  to  have  been leaking wastes to the underground is
 a common practice throughout  the region.

 Because  of  the awareness  of this source  of contamination,
 the rate of development of  new problems  should decline,
 especially  in  the southern  tier of states  (Pennsylvania,  New
 Jersey,  Delaware, and Maryland), where regulations  are  being
 enforced.   However, what  is  needed is  a  broader  understand-
 ing and  acceptance  by municipal and industrial waste treat-
 ment  facility  operators that  surface  impoundments must  be
 sited,  designed,  and operated with greater attention paid to
 hydrologic  and geologic conditions.

 The development of  guidelines,  an approach being used  by
 state agencies  to protect ground water from  contamination by
 landfills, might be considered for surface impoundments.
 However, before such guidelines  could  be established,  addi-
 tional research is  required,  as  with  landfills,  on  the  char-
 acteristics and effectiveness  of the different materials
 available for  artificial  lining.  Acceptable  methods for
metering loss  of  liquids  from lagoons, pits  and  basins  must
 be developed and tested.  More  information must  be made
 available on what happens to  different types  of  soil beneath
                             228

-------
and around impoundments containing various wastes with re-
spect to changes in permeability, adsorptive power, and po-
tential for ion exchange.  Finally, more must be learned
about many of the wastes placed in surface impoundments,
especially the municipal and industrial waste sludges, which
if not already wet when impounded soon become wet from pre-
cipitation.  What compounds can be leached from these
sludges must be determined along with the ultimate fate of
these compounds when they reach the saturated zone.  In too
many cases, not even the chemical make-up of the original
material impounded is known in any detail.

What may be more important from an overall ground-water
quality standpoint than the control of new surface impound-
ments are the thousands of existing and already leaking
sites throughout the region.  A major difficulty will be
locating those that may be damaging ground-water quality.
Many surface impoundments are on private lands and are
therefore difficult to inventory, except by air.  Industries
and municipalities have not had to register the existence of
surface impoundments with regulatory agencies in the past,
and thus, no central statistical file exists in the various
states on where they are and how they are used.  Also, ba-
sins with a very small area of say only 2,500 square feet
can be as potentially dangerous as extensive lagoon systems,
depending on such factors as the type of pollutant being
lost, the rate at which leakage is taking place, the sus-
ceptibility of the aquifer to extensive contamination, and
the proximity of wells supplying drinking water.  These
small basins would be difficult to locate even from the air.

A second difficulty is how to contain the pollutant and
clean up the aquifer that has been contaminated.  Regulatory
agencies hestiate to place heavy economic burdens on the
owner of the leaky surface impoundment.  Because of the prob-
lems inherent with attempting to remove a pollutant from an
aquifer under the limitations of the present state of the
art, clean-up operations when large volumes of contaminated
ground water are involved are for the most part ineffective.
In the long run, most of the pollutant is left in the ground.
Cases of ground-water contamination first reported decades
ago which  still exist today are not uncommon.  In some in-
stances, ground-water contamination was dicovered after an
industry had gone out of business or abandoned the site.
Clean up in such cases can be difficult to enforce, and liti-
gation over this and other conditions of ownership and re-
sponsibility can be time consuming.

Most efforts toward containment or clean up are hindered by
what to do with the pollutant after it has been removed from

                             229

-------
 the  aquifer  and  brought  to  the  surface.   This  is  the  situa-
 tion in  one  of the  cases shown  in  Table  38.  The  pollutant
 is too toxic to  discharge into  a nearby  stream.   The  volume
 is too large to  leave  in the  ground  but  too  small to  justify
 the  construction of a  special treatment  plant  on  the  site.
 If a nearby  municipal  or privately owned waste-treatment
 plant could  be found to  accept  the effluent  removed from  the
 aquifer,  then perhaps  it could  be  taken  away by tank  truck
 at a reasonable  cost.  However, in this  particular instance,
 the  polluter no  longer exists as a corporate entity,  and  it
 is questionable  as  to  who would pay  for  any  corrective meas-
 ures.  Except for abandonment of the waste lagoon and af-
 fected wells, the problem remains  unsolved.

 SPILLS AND SURFACE  DISCHARGES

 This section discusses ground-water  contamination caused  by
 hazardous and non-hazardous liquids  that are discharged onto
 the  land  surface  in an uncontrolled  manner and then seep  in-
 to the underlying soils.  If  the volume  of the fluid  is
 great enough, the pollutant can migrate  down to the satu-
 rated sediments  in  the vicinity of the discharge,  and ground-
 water quality will  be  degraded.  Activities  leading to
 spills and surface  discharges can  be separated into three
 main categories:  poor housekeeping  at large industrial com-
 plexes and airports;   intermittent disposal  of wastes at
 gasoline stations,  in  remote wooded  areas, and at small com-
 mercial establishments;   and  failures of above-ground tanks
 and  pipelines, or accidents involving railroad cars and tank
 trucks.

 Spills and surface  discharges at industrial  sites  are widely
 variable and differ  in character from plant  to plant.  How-
 ever, they are generally  caused by boil-overs  and blow-offs,
 by overpumping during  transfer  of  liquids to or from  storage
 and  carriers, by  leaks from faulty pipes  and valves in pro-
 duct  distribution systems, and  by  poor control over waste
 discharges and storm-water runoff.   At airports,  the  washing
 down  of planes with  solvents  and small spills  of  fuel can
 build up as  an extensive  body of hydrocarbons  floating on
 the water table.

Examples of  degradation of ground-water  quality over  broad
 areas due to poor housekeeping  are well  known  in  sections of
 the study region where there  is a  considerable density of in-
dustrial plants.   Oil has saturated  the  soils  beneath sev-
eral refineries and petroleum storage areas  in New Jersey. 112)
During periods of high water  table,  oil  actually  appears  as
pools on the land surface.  Furthermore,  storm sewers in
these areas continuously  discharge oil-laden ground water

                              230

-------
that has leaked into them.  It is felt that even though
there may be some leakage from underground pipes contrib-
uting to the problem/ the principal cause has been a long-
term build-up of ground-water contamination from periodic
spills and from leakage of oil onto the ground from surface
tanks and pipes.  In south Philadelphia, Pennsylvania, gross
contamination of the unconsolidated water-table aquifer has
been attributed principally to intermittent and long-term
accidental spillage of liquid chemicals and uncontrolled
runoff from chemical stockpiles in this highly industrial-
ized area. 123)  The ground water contains some inorganic
constituents in greater concentration than is characteristic
of raw sewage.

Contamination of ground water has also occurred in the re-
gion from the intermittent dumping of pollutants on the land
surface, especially at gasoline stations and other types of
small commercial establishments.  A recent study of the ul-
timate fate of automotive waste oil generated in Massa-
chusetts revealed that 650 thousand gallons of the oil is
dumped each year on the ground on or near service station
premises. 124)  Another two million gallons is disposed of
in a similar manner by car dealers and garage owners, by
operators of equipment at construction sites, by fleet op-
erators on their premises, and by persons changing their own
oil.  Although industry disposes of most of its uncollected
oil in town landfills, it is estimated that at least some
lubricating, hydraulic, and straight cutting oils are dumped
locally on the ground.  Each year these hydrocarbons are
added to the shallow aquifers of Massachusetts with little
chance of biodegradation or any other process that would
naturally remove them from the ground-water system.

In a recent study of the disposal and management of waste
oil in 18 counties of the New York metropolitan region, it
was determined that eight million gallons per year of auto
lube and crankcase oil, which is apparently changed by indi-
viduals or others not working through filling stations, are
either given to the neighborhood garbage collector or are
simply dumped on the ground.  Industry dumps another six to
21 million gallons per year in this same region. 125)  sim-
ilar practices must be present throughout the region and
contribute to ground-water contamination.

Dumping of small quantities of liquid wastes in and around
other types of commercial facilities has been observed by
regulatory agency personnel interviewed in this investiga-
tion.  Open discharge pipes draining sinks in commercial
laboratories are one example.  Disposal on open or wooded
lands of small quantities of liquids, when it is not eco-
                             231

-------
 nomic  to  store  them in  drums  or to haul to municipal waste
 treatment plants  or landfills,  is  probably quite  common  at
 commercial establishments  that  are not served by  community
 sewers.   Although such  facilities  have cesspools  or septic
 tanks,  the liquids may  be  judged too potent to be allowed to
 enter  and upset the septic system.

 Accidents involving above-ground pipes and tanks,  railroad
 cars,  and trucks  can lead  to  the release of large quantities
 of  a pollutant  at a particular  site.   For example, rupture
 of  a surface  pipe at an Air Force  test facility in New Hamp-
 shire  in  1957 spilled 30,000  gallons  of jet fuel  on the
 ground. 50)   The  crystalline  rock  aquifer underlying the
 site was  contaminated so badly  that in 1972,  wells origin-
 ally supplying  the base with  high  quality water were still
 unusable,  15  years after the  spill took place.

 Case Histories

 Table  39,  based on data selected from case histories inven-
 toried  in  this  investigation, lists the type  of pollutant
 documented as having affected ground-water quality.  The
 table  is  divided  into cases involving accidental  spills
 where  there was a one-time  discharge  of fluid onto the
 ground  and those  where  long-term poor housekeeping has been
 traced  as  the source  of contamination.   In the  former, the
 volume  of  the spill  is  given  where the information is avail-
 able.  As  can be  seen,  the majority of cases  involve hydro-
 carbons of some form, and it  is  reasonable to believe that
 these are  the most common pollutant in the region  related to
 spills  and surface discharges.

 In  every one  of the  36  cases  included in  the  table, oper-
 ating wells or  a  surface-water body were  noticeably affected.
 For this reason,  the  cases were  recorded  in the health de-
 partment or other environmental  agency files  that were re-
 viewed to  develop the information  for this  study.  Undoubt-
 edly, hundreds  and perhaps thousands  of other instances of
 ground-water  contamination of this type exist throughout the
 study region  but  have not come to  the attention of those
 concerned  with  ground-water quality.   It  is important to
 note that, in about  one-half  of  the 35  cases,  either munici-
 pal public water-supply or high-capacity  industrial wells
were affected and had to be abandoned.   In those where do-
mestic wells  were  involved, usually more  than one had to be
 abandoned  in  each instance.

 Several case  histories  from New  York  and  New  Jersey are typ-
 ical of the damage that can occur  and illustrate the problem
of contamination  from spills  and surface  discharges.  In the

                              232

-------
Table 39.  POLLUTANT REPORTED IN 36 CASES OF GROUND-WATER CON-
          TAMINATION CAUSED BY SPILLS AND SURFACE DISCHARGES.
Gasoline
Diesel fuel
Fuel oil
Caustic soda
Fuel oil  and gasoline
Formaldehyde
Jet fuel
Ketone and alcohol
Trichloroethylene
Chlorinated phenols
Number of cases

       4
       2
       2
       1
       1
       1
       1
       1
       1
       1
Volume of spill
  (gallons)

up to 2,500
up to 4,000
up to   200
Unknown
 6,000
 4,000
30,000
   300
50,000
Unknown
Surface discharges

Nitrates
Phenols
Crank case oil
Fuel oil
Heavy metals
Ammonia and mercury
Chlorinated benzine
Chloroform tetrachloroethane
Diesel fuel
Gasoline
Manganese
Chromium
Sulfate
Water softener effluent
Number of cases

       3
       3
       2
       2
       2
       1
                                 233

-------
 first New York instance,  50/000 gallons of trichloroethylene
 were spilled on the ground in a railroad accident.  126)   At
 least seven private wells in the area were contaminated  with
 up to 40  mg/1 of the pollutant, which moved quite readily
 through fractures and solution cavities of a limestone under-
 lying the site.   Flushing the area with fresh water was  un-
 dertaken  in an effort to  dilute the trichloroethylene, but
 this appears to have aggravated the problem by spreading the
 pollutant over a larger area.

 In another case,  several  petroleum storage tanks  were tilted
 during the flood conditions that struck portions  of upstate
 New York  in the  spring of 1972. 127)   Tne Spinage  resulted
 in an area of approximately one-half mile by one  mile being
 contaminated by  hydrocarbons.  No action has been taken  yet
 to remove the petroleum products from the ground, but some
 remedial  methods  may be attempted under the federal disaster
 relief program.

 In a third case  in New York,  small quantities of  liquid
 wastes from a fertilizer  production operation were  dis-
 charged onto the  ground over a period of many years. 127)
 Nitrates  as high  as 100 mg/1 have been found in water from
 nearby private wells,  and methemoglobinemia cases have been
 reported.   The manufacturer has begun to treat the  wastes
 and as domestic wells  become contaminated,  to replace them
 with water from  a central community system.

 In New Jersey, well fields operated by a municipality in the
 east-central  part of the  state are yielding water containing
 high levels of iron, manganese,  lead,  zinc,  and aluminum.
 The problem was investigated by the Bureau of Water Pollu-
 tion Control,  and it was  concluded that spillage  and gen-
 erally poor housekeeping  at industrial sites upstream of the
 well fields were  two of the principal  cause  of the  prob-
 lem.  128)   Pollutants  seeped  into the  ground and  were later
 discharged to or  allowed  to enter directly the streams that
 ultimately recharge the well  fields.   Other  sources of con-
 tamination included discharges of wastes to  an unlined pit,
 a  ruptured or unconnected industrial  sewer  line,  and accumu-
 lations of sludges  from water treatment lagoons.

Abandonment of the  affected water source is  the most common
means  for  coping  with  problems arising from  this  type of
contamination.  Successful  means  for  removing hydrocarbons,
the most  common pollutants,  once  they  have  reached  the water
table  and  extended  over a broad  area  have  not been  developed.
Pumping from  the  affected wells  or specially constructed
wells  and  skimming  from trenches  or pits dug to the water
table  has  had  only  limited  success.   In a  number  of cases,
                             234

-------
where a spill has been reported immediately, excavation of
the soil before the hydrocarbon has had a chance to migrate
to the water table has been successful in preventing a seri-
ous ground-water contamination problem.

Paving industrial sites and correcting poor-housekeeping
practices have been undertaken in some instances where inter-
mittent spills and surface discharges have been shown to
have contaminated water from wells in and around such areas.
Also/ carbon filters have been used with some success to
treat water from wells contaminated by hydrocarbons.

Future Trends

The accidental spill is an unavoidable hazard that is part
of the risk inherent to the storing and transportation of
fluids.  Thus, the number of new occurrences of this poten-
tial source of ground-water contamination will continue at
about the same or at an even greater rate in the future.  It
is in the handling of spills after they have taken place
that better protection of ground-water resources can be
achieved.  In the past, for example, liquids spilled on high-
ways have been removed at the expense of pollution to adja-
cent properties and aquifers in order to have a minimal ef-
fect on traffic flow.

Time appears to be the most important factor associated with
minimizing the contamination of ground-water supplies from
accidental spills.  If clean-up operations are carried out
quickly, especially when hydrocarbons are involved, then
there is a chance to either remove much of the pollutant
from the surface before it enters the ground or to excavate
affected soil in the immediate area before the pollutant
reaches the water table.  On the other hand, if action is
taken only after a broad area of an aquifer is affected, con-
tainment or removal of the contaminated ground-water body is
almost impossible.

Recognizing the importance of quick action, Pennsylvania has
adopted a regulation that requires individuals responsible
for a spill to immediately notify the Department of Environ-
mental Resources Regional Office when an incident occurs.
If ground water is threatened, the Regional Geologist at-
tached to the State's Ground Water Section attempts to re-
spond within a maximum of two hours. 36}   in this manner,
a technical appraisal of the situation is available within a
short period of time, and clean-up operations and assessment
of damage can begin in a more orderly manner.  Also in Penn-
sylvania, certain industries are required to develop a Pol-
lution Incident Prevention Program, which establishes a
                             235

-------
 specific  procedure  for informing the state  of spills  or
 other  major  pollution problems.   New Jersey has  a  similar
 program including a "hot line"  for reporting spills.

 Certainly, the  Pennsylvania and  New Jersey  approaches to
 this problem should be considered by other  regulatory agen-
 cies throughout the region.  Also,  there  should  be more
 recognition  and better understanding by the carrier and
 other  industries of the need for reporting  spills  to  the
 proper authorities.   Finally, guidelines  should  be developed
 for state and local highway personnel, railroad  operators,
 and industrial  plant managers defining such procedures as
 who should be informed of accidental spills and  how to han-
 dle the incident initially.

 Industry  has long appreciated the ills associated  with poor
 housekeeping and a  number of trade  organizations such as the
 Manufacturing Chemists  Association  and the  American Petro-
 leum Institute  have  published manuals and educational book-
 lets on the  prevention  and  control  of surface  discharges. 73,
 1^9,130)  Nevertheless, more controls are needed on prac-
 tices  that can  lead  to  contamination of ground-water  re-
 sources beneath and  in  the vicinity of industrial, commer-
 cial,  and construction  sites.  Elimination  of  open discharge
 of wastes to the  ground surface,  paving and control of run-
 off in areas susceptible  to  infiltration of pollutants, and
 maintenance  of  above-ground  distribution systems are  espe-
 cially important  and may  require  more attention  from  regula-
 tory agencies.   The  long-term effects on ground-water qual-
 ity of traditional practices of dumping waste  petroleum
 products  at  the point of  use should be evaluated and  again
 controls  established  if the  problem is of great  enough magni-
 tude to justify regulation.

 The need  for research into how to remove pollutants from an
 aquifer after it  has been contaminated has  been  pointed out
 in other  sections of  this report.   The specific  problems in-
 volved with  hydrocarbons  are discussed in the  section on
 "Buried Pipelines and Storage Tanks".

MINING ACTIVITY

A major activity  in the 11-state  study area that has  resulted
in a wide variety of ground-water contamination  problems is
mining.  Coal,  stone, sand,  and gravel are  the principal
products,  but iron,  copper,  zinc, and lead  have  been  impor-
tant minerals to the region  in the  past.  Extraction  of salt
by solution  and underground  excavation, carried  out princi-
pally  in western New York State,  is  not included in this sec-
tion.   The mining activity itself does not  normally lead to
                             236

-------
ground-water contamination.  Problems that have occurred
have been mostly related to the handling and transportation
of brine solutions, and they are characteristic of ground-
water contamination  occurrences from leaky pipelines,
spills, and surface impoundments.

Mines in the northeast are of two basic types, surface mines
and underground mines.  Economics dictate the nature and ex-
tent of the mining.  Where the ore deposit is close to the
land surface or where rock is incompetent, surface mining is
the most economical means of extraction.  Where the mineral
is deep or is unworkable from the surface because of local
geologic conditions, shafts and drifts follow the trend of
the deposit underground.  Many mines in the area have been
opened and closed periodically over the years depending on
market conditions for the particular product.

The number and size of mines in the northeast is not known
in detail.  Underground mines are hidden  from view and many
were never recorded or adequately mapped.  Some idea of the
amount of area involved in mining operations is indicated in
Table 40, which lists the number of acres in each state dis-
turbed by strip and surface mining as of  January 1965.  Ac-
cording to the table, Pennsylvania is by  far the leading
state because of extensive coal deposits.  It also is the
state with the most underground mines, again because of coal
production.  Table 41 lists the number of abandoned and in-
active underground mines in the northeast.  Figure 33 shows
the principal coal mining areas of Pennsylvania and Maryland.

Because of the nature of mining, in which land as a resource
must be consumed, the dollar value of production per amount
of land used is high relative to that of  all other indus-
tries except agriculture and silviculture.  Last year in the
United States, an average of 1,000 acres  of land per week
was consumed by active surface coal mine  operations alone.
134)  Reclamation may never fully restore this acreage.
Even where mines are operated underground, there may be sig-
nificant land consumption through the placement of waste
piles and surface impoundments, and land  subsidence and col-
lapse.

Mining is one of the few activities causing ground-water con-
tamination in the region for which the geologic and hydro- •
logic setting has been extensively studied.  Historically,
the presence of ground water in mines has been a severe prob-
lem hindering operations, and a principal concern of the
mining industry is keeping the work area  free of water.  For
example, in the 1870's the Ueberroth zinc mine near Friedens-
ville, Pennsylvania, was being pumped at  a rate of 12,000

                             237

-------
Table 40.  LAND DISTURBED BY STRIP AND SURFACE MINING IN THE NORTHEAST AS OF JANUARY 1,  1965, BY COMMODITY
                                             AND STATE (acres).  131>
State
Connecticut
Delaware
Maine
Maryland
Massachusetts
New Hampshire
ro
00 New Jersey
New York
Pennsylvania
Rhode Island
Vermont
Clay
200
400
1,200
700
1,400
1,700
10,400
-
-
Coal
(Bituminous,
Lignite and
Anthracite)
-
-
-
2,200
-
—
-
302,400
-
-
Stone
100
200
4,400
2,200
1,200
100
2,000
12,500
24,400
20
2,300
Sand and
Gravel
16,100
5,200
28,200
18,800
36,400
8,000
27,600
42,200
23,800
3,600
4,000
Iron Ore
-
100
100
20
1,100
1,000
700
8,800
-
-
All Other
100
10
1,712
800
900
200
1,800
605
402
-
400
Total
16,300
5,710
34,812
25,220
40,300
8,300
33,800
57,705
370,202
3,620
6,700

-------
Table 41. ABANDONED AND INACTIVE UNDERGROUND MINES IN THE NORTH-
                           EAST AS OF 1966.  133)
                         Coa[             Metal             Non metal

Connecticut                 -                 o                  o

Delaware                   -

Maine                                        7

Maryland                  564                7

Massachusetts                -                 7                  i

New Hampshire              _                24                  o

New Jersey                 -                26

New York                   -                61                  j7

Pennsylvania              7,824               160                  55

Rhode Island                 -                 2                  4

Vermont                    -                ]7                  3
                                 239

-------
•
«k
 -
               |—MAJOR  COAL  DEPOSITS
                Figure 33.  Principal coal areas of Pennsylvania and Maryland

-------
gpm from a depth of 250 feet. -^5)   Underground mines are
almost invariably below the water table, and surface mines
are often excavated into the water table.  Dewatering has
led directly or indirectly to the two major ground-water
problems resulting from mining activity — a regional lower-
ing of the water table, and excessive mineralization of
water associated with mines.  In an attempt to keep the
working areas of the mine dry and to remove as much of the
mineral deposits as possible, operators may lower the water
table by allowing water to drain from the mine by gravity,
by pumping water directly from the mine, or by the use of
wells in the vicinity of the mine.

The effects of lowering the water table on the ground-water
system may be threefold.  In the first place, the volume of
ground water in storage is reduced, thereby limiting ground-
water availability.  Second, the water level may fall below
the intakes of productive wells in the area forcing their
abandonment.  Third, lowering the water table can expose
minerals to the process of oxidation.  Percolating waters
can dissolve these minerals in significant concentrations.

It is the increased mineralization of ground water that is
the problem of greatest concern with regard to contamination
of both surface waters and ground waters.  Many economic de-
posits in bedrock are associated with sulfide minerals, the
most prominent in the northeast being that of coal with
pyrite  (FeS2).  Pyrite may be found in the adjacent sedi-
mentary rocks such as shale, sandstone, and limestone, as
well as within and between the coal seams.  Other examples
are the copper ores of New Jersey, which are sulfides. 136)
Chalcopyrite is a principal copper mineral in Vermont, oc-
curring in an iron sulfide ground mass. 137)

If there is no change in the hydrogeologic environment, py-
rite and most other sulfides are stable under the conditions
that exist below the water table.  If the water table is
lowered, oxidation of the sulfides takes place in the dewa-
tered zone.  Oxidation of sulfides by itself does not con-
tribute to ground-water contamination because oxidation oc-
curs above the water table.  However, when water is brought
into contact with the mineral system, for example, if a mine
is abandoned and dewatering  activities  stop, the result is
quite different.  Oxidation  of pyrite followed by contact
with water produces ferrous  sulfate  (FeSOa) and sulfuric
acid  (H2SO4) in solution.  Downward percolating rainwater,
or a rise in the water table will introduce this solution
into the ground-water  system, causing a  drop in pH,  and  a
rise in sulfate and iron content.
                              241

-------
 The highly mineralized water associated with mine workings
 is normally referred to as  "acid mine drainage."   Although
 there is no typical analysis for mine drainage  and it  can
 vary in quality from place  to place,  water discharging from
 coal mines has  been divided into four general classes  as
 shown in Table  42.

 Other sources of ground-water contamination associated with
 mining activities include leachate  from waste rock piles and
 leakage from tailing ponds.   These  processes of contamina-
 tion are similar to those described in the sections of this
 report entitled "Landfills"  and  "Surface Impoundments".

 Case Histories

 The principal areas where ground-water contamination from
 mining activities is of importance  are the regions of  Penn-
 sylvania and Maryland underlain  by  coal deposits.   The major
 emphasis of regulatory agencies,  to date,  has been directed
 toward control  and  correction of the  complex problems  of
 acid mine drainage  to surface waters.   It  is estimated that
 Pennsylvania alone  has over  2,300 miles of streams that are
 adversely affected  by coal mine  drainage.  139)  Many of
 these streams contain water with  a  pH of less than 4.0, iron
 concentrations  greater than  several hundred mg/1,  and  sul-
 fates greater than  1,000 mg/1.   The problem of  poor-quality
 water is  of  such  long standing and  is  so areally  extensive
 that  contamination  of both surface  waters  and ground waters
 is  looked upon  as an almost normal  occurrence in  the heavily
 mined regions.  The  widespread effects  of  mining  have  made
 it  difficult to drill  wells yielding  a  satisfactory quantity
 of  water  with acceptable quality.   Dewatering and excavation
 of  underground mines  have created physical problems, in
 addition  to water-quality problems, that make the  construc-
 tion  of wells in  some  areas almost  impossible.  Thus,  ground
water  as  a source of  supply has probably declined  in impor-
 tance.

Compilations of individual cases involving degradation of
well-water quality are not available, but  the problem  has
been  investigated on  a regional basis.   The  results  of such
a study in the Toms Run Basin  located in Clarion County,
northwest Pennsylvania, is probably typical  of  the  effects
that mining  can have  on ground-water quality. 140)   The area
has been mined for coal, and drilled for oil  and  gas for
nearly 100 years.  Coal mining has  occurred  exclusively in
the western half of the basin, in the extreme north  and
along the southwest edge.  Oil and  gas wells have been
                             242

-------
     Table 42. MINE DRAINAGE CLASSES.  139>
Class
Class II
Class III
Class IV

PH
Acidity, mg/l, CaCC>3
to Ferrous Iron, mg/l, Fe
U)
Ferric Iron, mg/l, Fe
Aluminum, mg/l, Al
Sulfates, mg/l, SO^
Acid
discharges
2.0- 4.5
1,000 -15,000
500 - 10,000
0
0 - 2,000
1,000 - 2,000
Partially
oxidized
and/or
neutralized
3.4-
0 -
0 -
0 -
0 -
500 -
6.6
100
500
1,000
20
10,000
Oxidized and
neutralized
and/or
alkaline
6.5 - 8.5
0
0
0
0
500 - 10,000
Neutralized
and not
oxidized
6.5 - 8.5
0
50 - 1,000
0
0
500 - 10,000

-------
 drilled throughout the entire basin into Devonian  sandstones
 between 2,200  and 2,500 feet deep.   The Mississippian  and
 Pennsylvanian  rocks of the area comprise a three-aquifer
 system separated by shale and siItstone confining  beds.   At
 the top of the geologic section lies the only mineable coals
 within a sequence of sandstone and  shale.

 The investigation showed that coal  mine drainage has a dele-
 terious effect on ground water.   Highly fractured  bedrock
 together with  abandoned gas,  oil, and water wells  have al-
 lowed poor quality water to migrate from areas of  mining  in-
 to the principal fresh-water aquifers of the region.   Be-
 cause of deterioration of cement seals and casings, the aban-
 doned wells act as conduits for  interchange of water between
 the aquifers in the basin,  thereby  aggravating the problem.
 Small diameter,  uncased holes drilled to define coal deposits
 also allow aquifer interchange.  Detailed  mapping  of water-
 quality relationships  in two of  the principal fresh-water
 aquifers revealed a very low pH  and abonormally high concen-
 trations of iron and sulfate  in  the vicinity of the coal
 mines.   Table  43 shows the  effects  of mining on ground-water
 quality for two of the major  aquifers in the basin.

 As mentioned above,  slag piles and  settling ponds  are  also
 sources of  contamination from mining activities.   In north-
 eastern Pennsylvania,  water with a  zinc content of up  to
 200 mg/1 has been leached from a slag pile at a smelter and
 has entered a  shallow  sandstone  aquifer.   The contaminated
 ground  water is  discharging into and severely affecting
 aquatic life in  a nearby creek.  14D   in Port Washington,
 New York, ponds  used in  a sand and  gravel  operation for
 settling silt  and clay particles have contaminated several
 important coastal  plain  aquifers in the area.  142)  The
 source  of supply for the ponds is salt water from  a harbor
 adjacent to the  mining operation.   Long-term use of the salt
 water in the sand  and  gravel  pits,  which cover an  area of
 about two square miles,  has raised  the chloride content of
 some nearby shallow  and  deep  wells  from a  normal level of
 less than 20 mg/1  to over 1,000  mg/1.

Future  Trends

As with  so  many  other  problems of ground-water  contamination,
mine drainage  would  essentially  be  ignored were it not for
its  surface  manifestation.  Active  mines appear to be  less
significant  as sources of contamination than  are abandoned
mines for a  number of  reasons.   First,  in  an  active mine,
the water table  is held  at  or just  below the  working floor
of the mine  in a parastable state,  reducing  drainage that
has come in  contact  with oxidized minerals.   Secondly, pol-

                              244

-------
Table 43. SUMMARY OF WATER QUALITY IN THE TOMS RUN DRAINAGE BASIN. 141>
Lower Aquifer

  Non-mining areas

  Areas near mining


Upper Aquifer

  Non-mining areas

  Areas near mining
   pH_



6.3 -6.8

2.9-5.4
6.5-6.7

3.0 -5.5
                                            Total Iron
                                             (mg/l)
 3-16

25 - 160
10-  15

20 -  70
                 Sulfate
                 (mg/l)
 4-13

30 - 620
10 -  15

39-  80
                                   245

-------
 luted-surface water discharges can be traced to the source
 mine, so operators are more careful about the water that
 they discharge.   Finally,  recently developed regulations  in
 some states  require engineering practices be applied to
 active mines that will reduce the volume  of polluted water
 generated or discharged, both during operations and after
 abandonment.  Unfortunately,  the major volume of mine drain-
 age  comes from abandoned mines.   Of the 1,500 significant
 mine discharges  in the Susquehanna River  Basin of New York,
 Pennsylvania, and Maryland producing acidity, 75 percent
 comes from abandoned mines.  143)

 No single method to control  acid mine drainage has  been ef-
 fective in all cases.   Partially successful measures have
 been applied by  mining companies and enforcement agencies,
 and  they fall into the following categories:

 1.   Minimizing the water-mineral-oxygen content

 2.   Regulating flow of surface waste water

 3.   Protecting minerals from  weathering and erosion follow-
     ing completion of  mine operations

 4.   Neutralization of  acid

 One  pollution abatement method for  abandoned  underground
 mines has  been sealing with either  air- or water-tight seals.
 In theory, the air seal prevents  oxygen from  entering the
 mine.   In  practice,  the procedure has had minimal success.
 Such seals are created by constructing walls  across mine
 openings  or  by collapsing portions  of the mine.

 Water-tight  seals  have become  more  popular for sealing aban-
 doned mines.   Theoretically,  the water-tight  seal should
 eliminate  surface  discharge,  restore the  pre-mining ground-
 water level,  and  exclude oxygen  from the  mine,  provided that
 the  bedrock  has not  been extensively fractured by the  mining
 operations.   Cost  of water-tight  sealing  at Moraine  State
 Park,  Pennsylvania,  was $1,266,213  for 65  mine seals,  an
 average of $19,480 per seal.  144)   Sealing boreholes  or
 fracture  zones can range from  $100  to $1,200  per hole  and
 sealing shafts from  $7,000 to  $25,000  per  shaft. 145)

Neutralization of  acid mine drainage  and  precipitation of
 iron  has been  an alternative proposal  for  controlling  con-
 tamination.  This method, however,  carries  a  high cost of
 treatment.   Capital  cost of a  mine  drainage treatment  plant
 in southwestern Pennsylvania was  $200,000  a few years  ago.
Capital recovery costs  run as  high  as  $29,000  per year, and

                             246

-------
the annual outlay for lime can range from $12,000 to $64,000,
depending on how much acid must be treated.   To treat mildly
acid water, one company incurred costs of $0.13/1,000 gal-
lons;  for highly acid water $0.72/1,000 gallons. 146)

Preventing pollution from abandoned surface  mines has been
attempted by backfilling.  However, this type of reclamation
is also very costly.  For example, backfilling recently cost
$672,208 for 462 acres in the area of Moraine State Park,
Pennsylvania. 144)

Many of the northeast states have provisions in their water
laws that can cover ground-water degradation due to mining
activity.  The difficulty of enforcement in the case of
abandoned mines has been a major hindrance to alleviating
the problem.  Pennsylvania has water statutes specifically
referring to operation of mines and disposal of mine wastes,
including acid mine drainage. 34)  The Clean Streams Law
(1965) requires that active mine discharge to surface water
not exceed seven mg/1 of iron, have a pH of six to nine, and
have no acidity. 139)  Mining permits in Pennsylvania in-
clude a section on mine closing which must be approved by
the Sanitary Water Board. 146)  These statutes have no ef-
fect upon pre-1965 abandoned mines.

The tremendous costs involved in correcting existing contam-
ination of surface waters and ground waters from mining
activities will prevent public agencies  from making major
headway toward solving this problem in the foreseeable fu-
ture.  Considerable research has already been carried out
and is underway on the subject of mine drainage, which may
lead to the development of more effective control over con-
tamination from both abandoned and operating mines.  However,
at present, this source of contamination appears to be one
that will continue as a significant problem in portions of
the study region.

PETROLEUM EXPLORATION AND DEVELOPMENT

Exploration for and development of oil and gas resources is
no longer a significant industry in the  study region.  Most
of the petroleum exploration has occurred in New York and
Pennsylvania;  minor exploration has taken place in New
Jersey and Maryland.  Virtually no exploration has been car-
ried out east of New York, where geologic conditions have
been considered unfavorable for the formation of petroleum.
Figure 34  shows the general area where oil and gas explora-
tion and development has  taken place.

'Petroleum  exploration and development may cause  ground-water

                              247

-------
          NORTH
Figure 34.  Principal oil and gas exploration and development areas
                          248

-------
contamination at sites of both active and abandoned wells.
At many oil fields in New York and Pennsylvania, initial de-
velopment took place around the turn of the century, at
which time most of the production occurred, followed by a
period of declining activity.  Today, individual wells in
the region produce a minimum of oil and gas, and large quan-
tities of salt water must be separated from the fluid pumped
from a well in order to obtain the petroleum product.
Nevertheless, the number of active oil and gas wells in the
region is still significant.  In 1973, according to the In-
terstate Oil Compact Commission, there were 32,596 operating
oil and gas wells in Pennsylvania, 5,400 in New York, and 15
in Maryland.  During 1972, 1,632 wells were abandoned in
Pennsylvania, 573 in New York, and one in Maryland. 147)

The high yield of salt water from producing wells represents
the principal threat to ground-water quality in fresh-water
aquifers in the petroleum recovery region.  Natural brines
from deep strata tapped by the oil and gas wells is brought
to the surface with the petroleum product.  The oil and wa-
ter mixture is then subjected to separation processes.  The
waste water produced from the separation process is a brine
solution, which is usually disposed of in unlined settling
pits or discharged to the ground.  Pipelines and separation
tanks may be in disrepair at these installations and can
discharge to the surface.  The saline waters from these
various sources can infiltrate into shallow fresh-water aqui-
fers and cause contamination.

Abandoned oil and gas wells  also present problems to ground-
water quality.  For example, abandoned oil wells can dis-
charge brine continuously, contaminating shallow fresh-water
aquifers.  Abandoned gas wells can discharge brine  where the
gas reserve has been depleted and salt water has migrated to
the wells.  Even where the exploration and production  com-
pany has conscientiously capped and/or plugged  the  abandoned
well, the casing may eventually leak  or corrode, introducing
brine or brine and waste oil and gas  into near-surface  aqui-
fers.

Most of the oil and gas exploration  in the  study region has
taken place on the Appalachian Plateau.  This broad area of
gently dipping rock strata has been  dissected by major
streams.  The stream valleys have been partially  filled with
alluvium and are discharge areas  for  ground water  circu-
lating out  of the uplands.   Non-degradable  pollutants  such
as brine introduced into  leaky oil and gas wells  in the up-
lands can eventually  find their way  to natural  discharge
areas in the valleys.  As a  result,  regional  problems can
result from ground-water  contamination due  to petroleum ex-

                              249

-------
 ploration and development.

 Case Histories

 An estimation of the  number of cases  in which water wells  in
 the northeast have  been contaminated  as a  result  of petro-
 leum exploration and  development  is not possible.  Individ-
 ual cases and regional  effects have been noted, but the over-
 all problem has  not been studied  in detail.

 One typical area where  contamination  from  this source has
 been observed is Chemung County,  in the western part of New
 York adjacent to the  Pennsylvania border.  Here concentra-
 tions of  chloride and total dissolved solids in water from
 many domestic wells have shown a  rising trend over many
 years.  The upper bedrock of Chemung  County is composed of a
 sequence  of sandstone and shale,  overlain  by glacial drift.
 Within the  major stream valleys,  the  sand  and gravel de-
 posits are  productive aquifers.   Elsewhere, the bedrock
 aquifer is  utilized.  Salt  beds and zones  of highly mineral-
 ized water  are known  to underlie  the  area  at depth.  Al-
 though never a highly productive  petroleum area,  a number  of
 gas wells were drilled  and  later  abandoned.  It is believed
 that many of these  old  wells are  conduits  for the upward
 migration of the mineralized water. 148)   Whereas natural
 chloride  content of the  shallow fresh-water aquifers in the
 County is less than 10 mg/!7 concentrations of this constit-
 uent in water  from  domestic wells believed to be  contamin-
 ated by brine  from  the  deeper  gas strata range from 100 to
 500  mg/1.  Analyses of water from many domestic,  industrial
 and  municipal  wells in  the  Susquehanna River Basin in New
 York indicate  similar conditions. 149)

 In  the  Jamestown area of New York, salt beds are known to
 occur at  depths  of  1,500  to 2,000 feet below land surface.
 Oil  and gas wells have been drilled through these beds, and
 it  is  suspected  that many of those abandoned are now allow-
 ing  mineralized  water to migrate  into the  shallow fresh-
water  aquifers.   Water  from some  of the shallow wells is re-
ported  to also contain  traces  of  oil and natural gas. 150)

 In Venango County,  Pennsylvania,  discharge of oil field
brines  to unlined surface impoundments and directly onto the
 land  surface has  contaminated  a number of privately-owned
springs and wells used  for  water  supply.  The problem is un-
der  study by the  state and  some seepage basins have been
moved.
                             250

-------
Future Trends

In a 1969 report on ground-water contamination from natural
gas and oil production in New York, prepared by Leslie J.
Grain of the U. S. Geological Survey, the author recommends
that the first step toward attacking this problem should be
"to delineate more exactly the area involved and to deter-
mine the magnitude of the pollution in these areas." 151)
This statement clearly defines the present status of know-
ledge on contamination from petroleum exploration and devel-
opment in the study region.  For the most part, present con-
tamination problems pass unnoticed because they generally
occur in sparsely populated areas.  However, as urban and
suburban development proceeds, reports of contamination from
petroleum exploration and development probably will increase.
The continuing corrosion of casings and failure of seals in
abandoned oil and gas wells also will aggravate the problem.

These factors, however, may be partially offset by a growing
effort on the part of public agencies to have abandoned
wells properly plugged.  Pennsylvania has statutes that
specifically refer to "the control and prevention of pollu-
tion of surface and underground waters resulting from drill-
ing, operation, abandonment or plugging of oil or gas
wells." 34)  New York has had regulations on the drilling
and plugging of wells since 1963.  152)  However, little con-
trol can be exerted on operators who abandoned wells before
such regulations were enacted.

SALT-WATER INTRUSION

Intrusion of salty water into fresh-water aquifers is one
form of ground-water contamination that is widely recognized
as a potential problem in the northeast.  There are two
principal regions in which salty water is found under natu-
ral conditions and, thus, fresh-water aquifers are prone to
the intrusion of  salt water caused by pumping  from domestic,
municipal, and industrial wells.   The two regions are shown
on Figure 35 and  are referred to in  this discussion as the
Coastal Region and the Inland Region.  The former borders
the Atlantic Ocean, and the latter is in the western por-
tions of New York and Pennsylvania.

Coastal Region

Salt water occurs naturally in water-table and artesian
aquifers along the Atlantic coast.   Boundaries between nat-
ural fresh water  and salty water in  the principal aquifers
of the Coastal Plain are shown on  Figure  36.   The fresh-salt
water boundaries  of the relatively shallow  aquifers  of

                             251

-------
                                                         A.
                        NORTH
L
   DEPTH BELOW LAND SURFACE TO SHALLOWEST
   ZONE OF GROUND WATER CONTAINING MORE THAN
   1,000 MG/L OF DISSOLVED SOLIDS.

^    |  LESS THAN 500 FEET

        500- 1,000 FEET

        GREATER THAN 1,000 FEET

        LESS THAN 1,000 MG/L ( NO WELLS
        KNOWN  TO PRODUCE MINERALIZED
        WATER  IN QUANTITIES GREATER THAN
        0.01 MGD )
Figure  35.  Depth to mineralized ground water in major aquifers in the
                           coastal and  inland regions
                                     252

-------
                                                          75°
                                                                                          73°
                                                                                                          72o
NJ
--'
UJ
                       NORTH
                                                                                          PLEISTOCENE

                                                                                          TERTIARY

                                                                                          CRETACEOUS
                                   Figure 36.  Inland  limit of saline ground water in the coastal plain formations of
                                                               the northeast United States  155)

-------
 Pleistocene  age  correspond  closely with  the  present-day
 shoreline.   However,  in  some  of  the  deeper aquifers  of Ter-
 tiary  and Cretaceous  age, natural salty  water occurs many
 miles  from the sea.   Also,  at some localities near the shore,
 deep wells may penetrate alternating zones of fresh  and
 salty  water.

 The Coastal  Plain  deposits  consist of a  wedge-shaped mass of
 unconsolidated rock materials that thickens  in a direction
 roughly perpendicular to the  coast of the Atlantic Ocean.
 The unconsolidated sediments  range in thickness from a thin
 veneer along the Fall Line, which is  the western limit of
 the physiographic  province, to as much as 10,000 feet or
 more along the east coast of  Maryland.   Aquifers consisting
 of sands and gravels  are areally extensive,  underlying hun-
 dreds  of square miles, and  the major  aquifer units that have
 been identified are separated by aquicludes  of silt  and clay.
 According to Upson, the  seeming anomalies in the pattern of
 occurrence of salty water in  the Coastal Plain deposits are
 thought to stem from  differences in the  circulation  pattern
 of fresh ground water in the  different aquifers, controlled
 at least in  part by the  relationship  between intake  areas
 and discharge areas for  each  aquifer. 154)

 In the glaciated New  England  states bordering the Atlantic
 Ocean, salty water is found in the shallow unconsolidated
 deposits and  in the bedrock aquifers  along the shoreline
 and underlying tidal  estuaries of the major  rivers.  No
 large  saline water bodies have been noted that extend many
 miles  inland as in the case of some of the coastal plain
 aquifers.

 Large-scale movement  of  salt water through an aquifer can
 occur, displacing fresh  ground water, either permanently or
 temporarily,  for a period of  time in  some cases measured in
 years.  The  salt water encroaches into the fresh-water aqui-
 fer as a front, which moves laterally.   However, in  the
 vicinity of pumping wells tapping a fresh-water zone situ-
 ated above a salty-water zone, vertical  migration of salt
water also can occur.  Lateral migration is  characteristic
 of salt-water intrusion  in the Coastal Plain.  In the New
England states, salt-water intrusion  is  characterized prin-
 cipally by small-scale and temporary  intrusions of salt-
water tongues induced by local pumping from wells construct-
 ed close to  an existing  salt-water body.

 Salt-water intrusion occurs as the result of some change in
the head relationship between  the fresh-water aquifer and
 interconnected bodies of salt water.   The body of salt water
 in contact with the aquifer may be in a  seaward direction or
                             254

-------
in a deeper section of the aquifer or may be in a tidal por-
tion of a surface stream, bay, or estuary.  Pumping from
wells lowers the water level in the aquifer and induces the
salt-water body to move either laterally or vertically to-
ward the wells.  If pumpage is great enough, the decrease in
amount of fresh ground water in storage is being compensated
for by an increase in the amount of salty ground water in
storage.  If the pumpage from wells induces recharge from a
saline surface-water body, the salty water can enter the
fresh-water aquifer and begin to move toward the wells.

One of the mechanisms that can aggravate a problem of salt-
water intrusion is leaky or corroded well casings.  They can
act as an avenue for saline water to migrate from an aquifer
containing salt water to an underlying or overlying aquifer
containing fresh water.  Another is the dredging of a rela-
tively impermeable soils from the bottom of a bay or tidal
river.  This can result in infiltration of saline surface
water to underlying aquifer which is being pumped heavily
for water-supply purposes.

The intrusion of salty water into a fresh-water aquifer is
characterized by a rise in chloride concentration and total
dissolved solids content.  For the purpose of this discus-
sion, fresh ground water is defined as water having a chlo-
ride content of less than 40 mg/1 and generally less than
100 mg/1 total dissolved solids.  Salty water is defined as
water having a chloride content of 40 to  about 16,500 mg/1
and a total dissolved solids content of about 100 to 31,000
mg/1.  Determination of whether salt-water intrusion has
occurred in the principal aquifers of the Coastal Region is
relatively simple because normal baseline conditions in the
fresh-water zones are generally represented by chloride
concentrations of less than 20 mg/1.

Case Histories -

Intrusion of salty water is almost always a very  slow proc-
ess.  In most  heavily pumped  areas in the Coastal Region,
no contamination has been reported.   In some  localities
where encroachment has taken  place, records show  that many
decades have elapsed before the salt  content  of the ground
water rose to  a point where it becomes objectionable.
Records also show that the  encroachment tends to be re-
stricted to relatively small  areas immediately adjacent  to
the wells that are being pumped.  Few cases of broad region-
al encroachment are known in  the  study area,  and  even  in
those cases, the rate of movement of  the  advancing  salt wa-
ter is  usually only a few feet per year.
                              255

-------
 For example,  one  of the most intensively studied salt-water
 intrusion cases is that involving Coastal Plain deposits  in
 southern Nassau and southeastern Queens  Counties,  Long Is-
 land,  New York. 155,156,157)   One wedge  of salty water is
 found  in the  shallow glacial deposits  and two  more are in
 the upper and lower portions of the  underlying artesian
 aquifer.  Another artesian aquifer,  in which no intrusion
 has been observed under the land area, lies directly  on the
 bedrock.  Figure  37 shows  the relationship of  the  salty and
 fresh  ground-water bodies.

 For the  most  part, the  position of the shallow wedge  of
 salty  ground  water has  not changed during historic time.
 However, the  salty ground-water bodies in the  underlying
 artesian aquifer  are actively advancing  inland in  response
 to  pumpage of about 100 mgd from this  aquifer.  Much of the
 water  pumped  is discharged directly  to sea from sewage treat-
 ment plants,  and  the consumption of  water and  the  lowering
 of  water levels has led to salt-water  intrusion.   Neverthe-
 less,  it is estimated that the  two salty-water wedges in  the
 artesian aquifer  have moved inland an  average  of about 1,000
 feet or  less  since the  early  1900's.   Locally,  in  the vicin-
 ity of some well  fields, the  deep salty-water  wedge has
 moved  more than a  mile  inland during the past  several dec-
 ades at  a rate of  about 300 feet per year.

 Table  44 is a summary of data on known ground-water contami-
 nation cases  in the northeast.   It is  based on the results
 of  a 1969  survey by the American Society of Civil  Engineers
 Task Committee on  Saltwater Intrusion  and a review of pub-
 lished and unpublished  information on  file with regional
 offices  of the U.  S.  Geological  Survey and state geological
 surveys  throughout the  study  area. 159)

 In  spite of the fact  that  the northeast  coastline  is  more
 than 1,000  miles in length, relatively few serious problems
 of  ground-water contamination have occurred.   One  of  the
 principal  factors  for this, as already mentioned,  is  the
 relatively slow lateral movement of  salt-water  fronts  that
 may  be advancing into fresh-water portions  of  the  Coastal
 Plain  aquifers.  Another important factor,  unlike  many other
 sources  of  ground-water contamination, is  the  general  wide-
 spread knowledge of the positions  of salty-water bodies in
 the  region.  Considerable research and monitoring  of  salt-
water/fresh-water  relationships  have been  carried  out  since
 the  early  1930's,   and because of the information available,
 drilling of supply wells in areas  prone  to  salt-water  intru-
 sion has been limited.  Finally,  every state within the
Coastal  Plain province  (New York,  New  Jersey, Delaware  and
Maryland)  is  regulating pumpage from  the  Coastal  Plain
                             256

-------
                          NORTH —
i
                  -i   SEA
                  £  LEVEL
                  -
                  tn

                      3OO
o

LJ   600
CD

•
-
-
                  -   900


                  o
                  •

                   •
                  u

                  u   1200
                                                                            Shallow salty ground water
                                                                                                  BAY
                                                                                            -SOUTH

                                                                                             ATLANTIC
                                                                                             OCEAN
                                      SAND AND GRAVEL ARTESIAN AQUIFER
                                       DEEP SAND AND  GRAVEL  ARTESIAN AQUIFER

                                                                      1/2
                                                              I mile
                           Figure 37,,  Occurrence of salty ground water in southeastern Queens and southwestern

                                              Nassau Counties,  Long Island, New York, in 1961

-------
to
en
CO
     Table 44.  SUMMARY OF DATA ON CONTAMINATION CASES  RELATED TO SALT-WATER INTRUSION IN COASTAL
                                                         AREAS.
     Location

     CONNECTICUT

       Long Island Sound coastal area
       including the Cities of New
       Haven and Bridgeport
DELAWARE

 Coastline and Delaware River
     MAINE

       Town of Bowdoinham,
       Sagadahoc County
                                   Nature of problem
                                   Lateral intrusion of salty water from harbors
                                   and tidal river estuaries has contaminated
                                   water from several dozen industrial and mu-
                                   nicipal wells tapping glacial sand and
                                   gravel,  Triassic sandstone and shale,  and
                                   crystalline rock aquifers in areas of heavy
                                   pumping.
                                         Lateral and vertical intrusion of salty water
                                         from the  Delaware River and Delaware Bay
                                         and from the Ocean has contaminated wa-
                                         ter from three municipal well fields because
                                         of intensive pumping from shallow aquifers
                                         and the dredging of impermeable soils.
                                   Salty water from tidal reach of Kennebec
                                   River has contaminated a well 300 feet
                                   deep, tapping the bedrock aquifer.
Remedial action
Pumpage relocated inland or re-
duced; some wells abandoned;
and at least one scavenger well
installed to hold back salty
water.
Pumpage relocated inland; wells
abandoned;  wells deepened;
tidal gate constructed to hold
back salty surface water in one
tributary to the Delaware River.
Well abandoned

-------
     Table 44 (continued).  SUMMARY OF DATA ON CONTAMINATION CASES RELATED TO SALT-WATER INTRUSION
                                                   IN COASTAL AREAS.
to
en
vo
      Location

      MARYLAND

       Harbor District, City of
       Baltimore
       Joppatowne, Harford County;
       and Westover, Sommerset
       County
       Cambridge, Dorchester County;
       Annapolis, Anne-Arundal County;
       and Solomons-Patuxent River
       area, St. Mary's County
     MASSACHUSETTS

      Provincetown; Scituate; and
      Sommerset
 Nature of problem
Salty water from Patapsco River estuary has
intruded the water table and shallow arte-
sian aquifers.

Salty water from Chesapeake Bay has been
induced into fresh water aquifers tapped
by two municipal well fields because of
heavy pumpage and leaks in casings of
abandoned wells.

Lateral and vertical intrusion of salty water
from tidal river estuaries has contaminated
shallow water table and artesian aquifers
affecting water quality from numerous do-
mestic and industrial wells.  Problem has
been aggravated by leaks in casings of
abandoned wells.
Minor lateral intrusion from ocean and
salt-water marshes has affected water from
wells tapping shallow aquifers.
 Remedial action
Many industrial wells aban-
doned.
Several wells abandoned,
others being monitored.
Abandoned wells are being
plugged; pumpage has been
reduced; and water quality
is being monitored.
New wells drilled farther in-
land;  pumpage from old wells
reduced.

-------
     Table 44 (continued).  SUMMARY OF DATA ON CONTAMINATION CASES RELATED TO SALT-WATER INTRUSION
                                                 IN COASTAL AREAS.
N)
O\
O
     Location
     NEW HAMPSHIRE
       Portsmouth
NEW JERSEY

 Sayreville, Middlesex County;
 Gibbstown-Paulsborough area,
 Gloucester County;  Newark,
 Essex County;  Rahway area,
 Union-Middlesex Counties;
 Salem, Salem County

 Atlantic City, Atlantic County;
 and several areas in Cape
 May County
                                   Nature of problem
                                  Minor lateral intrusion from tidal water in
                                  Piscataqua River.
Salty water from tidal estuaries and bays
has intruded water table and artesian
aquifers due to intensive pumping and
harbor and canal dredging
                                        Salty and brackish water from saline-water
                                        aquifers has intruded shallow and deep
                                        fresh-water aquifers due  to heavy pumping
                                        and corroded well casings.  Problem mostly
                                        local in nature
       Sommers Point, Atlantic County     Wedge of salty water has moved about
                                        3,000 feet landward into the Cohansey
                                        aquifer.
                                             Remedial action
                                             Unknown
                                                                                     Pumpage relocated inland;
                                                                                     and many wells abandoned.
                                             Pumpage has been reduced in
                                             a few wells;  wells with leaky
                                             casings have been sealed; and
                                             new, double-cased wells have
                                             been drilled  into the artesian
                                             aquifer. Some tidal  gates
                                             have been installed.

                                             Pumpage has been reduced;
                                             monitoring;  new wells are
                                             planned inland.

-------
     Table 44 (continued).  SUMMARY OF DATA ON CONTAMINATION CASES  RELATED TO SALT-WATER INTRUSION
                                                   IN COASTAL AREAS.
to
a\
     Location

     NEW JERSEY (continued)

      Artificial Island,  Salem County



     NEW YORK

      Kings Count/, Long Island
      Queens, Nassau, and Suffolk
      Counties, Long Island
    PENNSYLVANIA

      Philadelphia
 Nature of problem
Salt-water intrusion at nuclear generating
plant.
Salt-water intrusion resulting in severe
contamination of glacial aquifer due to
lowering of water table below sea level
over a broad area.
Lateral and vertical intrusion of salty
water from ocean into the water table and
artesian aquifers, but only immediately
adjacent to shorelines.  Problem caused
by pumping, leaky well casings, and
dredging.
Lateral intrusion of salty water from the
tidal Delaware River has contaminated
industrial wells in the shallow aquifer
due to pumping. Leaky well casings and
dredging the Delaware River has aggra-
vated the problem.
 Remedial action
 Pumpage has been concentrated
 at southern end of island where
 aquiclude is thickest.
 Pumpage reduced; all public
 and many industrial water-supply
 wells abandoned; artificial re-
 charge of cooling water re-
 quired.

 Pumpage near shorelines re-
 duced;  ground-water diversions
 under strict control;  artificial
 recharge of cooling water re-
 quired.
Some industrial wells aban-
doned.

-------
to
0\
to
    Table 44 (conHnued). SUMMARY OF DATA ON CONTAMINATION CASES RELATED TO SALT-WATER INTRUSION
                                               IN COASTAL AREAS.

    Location                          Nature of problem                           Remedial action

    RHODE ISLAND

      City of Providence;  Town of       Salty water from tidal river estuaries and        Pumpage has been reduced,
      Barrington                        bays has contaminated water from some mu-     the ground-water supply may
                                      nicipal wells tapping the glacial outwash       be replaced with surface
                                      aquifer due to heavy pumping.                 water.

-------
aquifers.  These regulations, which involve complete control
over rates and patterns of pumpage from proposed significant
ground-water^diversions, were prompted to a great degree by
the recognition of the need for management of water re-
sources in areas subject to salt-water intrusion.

Although serious problems of ground-water contamination are
not numerous,  the presence of salty water in coastal aqui-
fers throughout the region has a limiting effect on the
availability of ground water.  Well diversions must be kept
within certain limits in order to maintain salt-water fronts
in as much of a status-quo position as possible, which is
the present philosophy of regulatory agencies in the region.
In fact, in order to aid in reducing the threat of contami-
nation from this source, artificial recharge of cooling wa-
ters and storm waters has been encouraged in Long Island,
New York and in some parts of New Jersey.  There are more
than 1,000 recharge or diffusion wells returning used ground
water to the aquifers underlying Long Island. 160)  in 1965,
an average of about 77 mgd was injected, mostly cooling wa-
ter used for air conditioning.  In addition, there are more
than 2,000 recharge basins in Nassau and Suffolk Counties
ranging from about 10 to 20 feet in depth and from about one
to 30 acres in size.  The basins are unlined excavations
which receive storm-water runoff from streets and highways.

A method used in the region to limit encroachment of saline
surface water inland in rivers and streams, in areas where
salty surface-water intrusion into underlying aquifers might
occur, is the installation of tidal gates.  These structures
hold back saline water from flowing upstream during high-
tide periods.   A number of tidal gates have been placed
across small coastal streams in Cape May County, New Jersey,
for example. 161)  Relief wells have also been installed in
a few locations.  The purpose of these wells is to pump salt
water, thereby lowering the head in the saline ground-water
body and retarding or preventing movement of saline water
toward wells pumping from a fresh-water zone.

Future Trends -

Because of the close regulatory control over diversion of
ground water near coastal regions in some of the states and
the general knowledge of where saline ground-water bodies
might be encountered in most of the states, it is unlikely
that the number of problems of contamination from this
source will rise significantly in the near future.  However,
one possibility that might lead in the future to the estab-
lishment of new positions farther inland for salt-water
fronts in some areas is a change in water-management atti-

                             263

-------
 tudes.   These  changes might  occur  in  response  to  greater  de-
 mands  for water-supply  development because  of  continuing
 population  growth  in coastal areas.

 The  landward extent of  a wedge  of  salty water  is  controlled
 by the  rate at which ground  water  is  discharging  from the
 aquifer into the ocean.  Some of the  counties  within the
 Coastal Plain  area may  become water-short in the  near future
 and  the decision will have to be made on how to meet in-
 creased water  needs.  One alternative, of course, is the  im-
 portation of surface water into those areas presently depend-
 ent  upon ground water.  Another alternative would involve
 abandoning  the present  management  concept of maintaining
 salt-water  fronts  in a  status-quo  position, withdrawing more
 fresh ground water for  consumptive use, and permitting salt
 water to move  inland to a new position of stabilization.
 The  replacement of wells contaminated and lost in the proc-
 ess  may be  considerably less  costly than importing surface
 water or some  other alternative that  might be  proposed for
 solving water-supply needs.   A  technical-economic evaluation
 of the  feasibility of removing  more ground water  from stor-
 age  would be of considerable  aid to water planners in the
 Coastal Region.

 Inland  Region

 Little  information has been collected and analyzed, or pub-
 lished,  on  salt-water intrusion in the Inland  Region of New
 York and Pennsylvania.  Natural saline water occurs at depth
 in consolidated rock formations.   However, these  areas are
 usually overlain by aquifers  containing fresh  water.  Saline
 water also  has been encountered in unconsolidated glacial
 deposits in some locations that are discharge  areas for min-
 eralized ground water originating  in  the rock  formations.
 As in the Coastal  Region, saline water tends to move toward
 wells when  the fresh-water head is reduced by  pumping.  Ver-
 tical rather than  lateral encroachment is more characteris-
 tic of  the  Inland  Region.  The  presence of natural saline
 water may be related to one or  more of the following causes:
 retention in the rock formation of the salty water in which
 the formation was  deposited  (connate  water);   solution of
 salt from the  formation itself  or  from adjacent formations;
 and entrance of salt water into the formation  after it was
 deposited and  subsequently exposed to another  source of salt
water.  162)

 Because of  the widespread and complex occurrence of saline
water in the region, it can be  difficult to determine whether
 salt-water  intrusion has occurred  or  whether poor quality
water yielded by a particular well is the result of natural


                              264

-------
conditions.  In addition, unlike the Coastal Region where
fresh waters are only slightly mineralized, ground water can
be considered "fresh" by well owners in the Inland Region
and have high concentrations of hardness, sulfates, chlo-
rides, and dissolved solids.

Figure 38 illustrates how variations of chemical quality can
occur in ground water as a result of natural recharge and
discharge relationships.  In the uplands, recharge from pre-
cipitation reaches the water table and becomes ground water.
Some of the ground water travels through deeper rock zones;
comes in contact with carbonate, sulfate, and chloride min-
erals, which are taken into solution;  and ultimately dis-
charges to the unconsolidated deposits in the valley.  If
wells are being pumped in the valley, the salinity of water
in the sand and gravel aquifer may be increased because of
vertical intrusion of a higher percentage of saline water
from deeper, more highly mineralized zones.  Figure 39 shows
how local ground-water circulation can produce a relatively
thin fresh-water zone above salt water.  Heavy pumpage in
this situation from wells tapping the shallow deposits can
produce vertical salt-water intrusion.   It should be noted
that Figures 38 and 39 are only two examples of many types
of different conditions that could be encountered in various
parts of the Inland Region.

The natural occurrence of saline water and the potential for
salt-water intrusion are limiting factors on the development
of ground water.  Some regional investigations of ground-
water resources have been carried out by federal and state
agencies, and as more are completed, the nature and occur-
rence of saline water will become better defined.  Because
of this/ problems of salt-water intrusion should be more
easily avoided through proper well location and construction.
Governmental controls over diversions of ground water in the
Inland Region, as a protective measure against salt-water
intrusion, do not exist and would be difficult to  enforce un-
til the problem is better defined by additional area-wide
studies.

RIVER INFILTRATION

Throughout the northeast, rivers and lakes are a major
source of recharge to high  capacity public supply and indus-
trial water wells.  Where a surface-water body is hydrauli-
cally connected with an aquifer, pumping from wells and the
resulting drawdown of water levels in the  aquifer  can in-
duce  surface water to infiltrate through the stream bed and
into  the ground-water reservoir.  This infiltrated water can
then  migrate to the pumping wells.  Studies of the relation-


                             265

-------
NJ
9
-
               RECHARGE  AREA

                          .WATER TABLE
                         DISCHARGE    AREA
RECHARGE  AREA
                                  ZONE OF WATER LOW
                                   IN DISSOLVED SOLIDS
                                                 GROUND-WATER
                                                   FLOW LINES
                                                SAND AND GRAVEL
                                                   DEPOSITS
ZONE OF WATER
 MODERATELY HIGHX
 IN DISSOLVED SOLIDS
                                                      ZONE OF WATER
                                                    HIGH  IN  CHLORIDE
                                                     x/  x  x  x \x  x
                    Figure 38.  Variations of chemical quality of ground water as related to recharge
                                                and discharge relationships

-------
~
                                        STREAM
                                                           WATER TABLE
SWAMP
                                                  JN£ONSOLl5ATED/  DEPOSITS
                                     FRESH-WATER FLOW PATH


                                 ^   SALT-WATER FLOW PATH
            20


            40


            60




            100
                                                                                                     or o
                                                                                                     Q. CO
                      Figure 39. Local ground-water circulation, producing a relatively thin fresh-

                                               water zone above the salt water

-------
 ship between  surface water  and  ground water have  shown  that
 wells  drilled within a  few  hundred  to as much  as  a  thousand
 feet away  from rivers and lakes can yield  a high  percentage
 of water derived  from infiltration.  For example, pumping
 tests  conducted along the Delaware  River in the vicinity of
 Camden, New Jersey, indicate that,  at a pumping rate of six
 mgd from one  major field, about 60  percent of  the well water
 is derived from river infiltration  and only 40 percent  from
 ground-water  storage. 165)  Discussions with water-well
 drillers, municipal water works operators, and representa-
 tives  of state agencies indicate that infiltrated surface
 water  pumped  from wells in  the  study region amounts to many
 hundreds of millions of gallons per day.   Individual well
 capacities range  from one-quarter of a million to as much
 as six mgd.

 If the infiltrated water passes through a  large enough vol-
 ume of soil and aquifer materials before arriving at the
 pumping well, natural filtration,' adsorption,  and ion ex-
 change can take place.  Turbidity,  organic materials, patho-
 genic  bacteria, and some chemical constituents can be effec-
 tively removed or reduced.  Thus, high-quality ground-water
 supplies can  be developed adjacent  to many poor-quality
 streams.  This feature of infiltrated ground water plus the
 large  amount  of potential recharge  available from major
 streams have  made the development of wells adjacent to sur-
 face-water bodies very attractive to water-works operators.

 Unfortunately, few investigations have been made to deter-
 mine whether  trace amounts  of such pollutants as heavy
 metals, organic compounds and viruses can migrate through
 aquifer materials to pumped wells.  In a few cases, bacteria
 have been known to survive  infiltration from the surface-
 water  source  to the well.  Also, acid or reducing surface
 waters that come  in contact with some aquifer materials can
 dissolve iron and manganese that naturally occur in a pre-
 cipitated form in the sediments.  This action has resulted
 in a build-up of  iron and manganese in the well water and
 has required  the  construction of treatment plants for reduc-
 tion of these constituents.   In some instances, iron and
manganese concentrations have been great enough to result
 in abandonment of the well  supply.

Case Histories

 Several documented case histories in the study area illus-
trate  some of the problems  of ground-water contamination
that can occur from surface-water infiltration.  For exam-
ple,  infiltrated water from a polluted tributary of the
Hudson River  dissolved iron and manganese in the natural

                             268

-------
sand and gravel sediments tapped by a high capacity caisson
well in southeastern New York. 166)  Analyses of water from
the stream had never shown high levels of manganese, but the
surface water was contaminated with wastes from two paper
mills, a textile plant, and several sewage treatment plants.
The aquifer consists of manganese-rich debris from glacially
eroded crystalline rock.

Manganese concentration in water from the caisson well,
which was capable of producing several mgd, rose from less
than one mg/1 when the well was first drilled to more than
14 mg/1 after several months of pumping.  Tests at the site
definitely established that a major portion of the water
pumped from the caisson well was derived from infiltration
from the stream.  Water temperature in the well varied ac-
cording to the water temperature of the tributary and the
manganese content of water from an observation well located
halfway between the stream and the caisson well rose and
fell in direct relation to the amount of induced river water.
Even though the caisson well is 100 feet from the stream,
high counts of coliform bacteria were detected in the ground
water, and it was concluded that the source of this contam-
inant was also related to infiltration of the surface water.
No means were found for diverting  the polluted surface water
away from the well without reducing its yield to an unac-
ceptable level.  Treatment for the high concentration of
manganese was considered to be uneconomic, and the well was
abandoned.

In a case in Connecticut, a six-mgd well field was developed
adjacent to the Connecticut River.  Again, the reducing en-
vironment created by the infiltrated river water moving
through iron-rich unconsolidated sediments resulted in a
water-quality problem. 167)  Pumping tests at the site re-
vealed that production wells capable of producing two mgd
each and located 150 feet from the bank of the river were
recharged with up to 90 percent induced infiltrated surface
water and with only 10 percent ground-water storage.  Figure
40 shows the relationship between  pumping from one of the
test wells and changes in iron and hardness concentrations.
The initial total hardness  (as CaC03) of the well water
ranged from about 120 to 160 mg/1.  The initial concentra-
tion of iron was less than 0.1 mg/1.  Concentrations of hard-
ness and iron in the Connecticut River adjacent to the site
averaged 44 and 1.0 mg/1 respectively.  The diagram shows
that during periods of pumping, the iron content rose in the
well water and stabilized at a level similar to that found
in the river.  Meanwhile, the concentration of hardness in
the well water declined to a level of 80 mg/1.  An  iron-
treatment plant was constructed at the site so that the

                              269

-------
•j
3
                 1.0


                  9


              a:   .8
              bl
              i-
              _i
              a.   .7
              ui
              a
              en
               a
               o
                  6
                  .5
E   4
-J
o
-  .3
                  2
H   800

                                                                                                           r
                                                                                                       60 £
                                                                                                           -
                                                                                                           -
                                                                                                       40 H
                                                                                                          m
                                                                                                           I

                                                                                                       20
                     APR. MAY JUN.   JUL.  AUG.   SEP OCT   NOV.  DEC
                                         1964
                                                        JAN  FEB.   MAR.  APR.  MAY.  JUN.  JUL  AUG
                                                                            1965
                         Figure 40.  Effect of infiltration of Connecticut river water on quality of water
                                                       from test production well

-------
ground water could be used for public supply.

A public-supply well in Onondaga County, New York, has oc-
casionally yielded water with high concentrations (0.15 mg/1)
of lead. SI)  Tjie source of the pollutant is concluded to be
a river several hundred feet away, which provides a major
portion of the recharge to the well.  The amount of the pol-
lutant reaching the well during any given period depends on
the character of industrial discharges to the stream and its
flow stage.

Future Trends

Cases similar to those described above involving iron and
manganese are very common throughout the northeast.  However,
in spite of the cost for treatment brought about by this
type of problem, the development of ground water as compared
to surface water is still economically favorable.  The drill-
ing of wells recharged by rivers and lakes will continue,
and infiltrated ground water will remain as a vital source
of supply for municipalities and industries.

Unfortunately, few detailed chemical analyses are available
for water from wells which depend on a high percentage of re-
charge from polluted streams.  More information is needed on
the fate of such trace substances as heavy metals and or-
ganic compounds in waters that are infiltrated from rivers
and lakes.  Herbicides and pesticides, for example, can con-
centrate in bottom sediments of surface-water bodies, and
data are lacking on whether these substances can be leached
by surface waters induced into underlying aquifers.  In
addition, many of these ground-water supply  systems have
been in operation for many years.  Conceivably, the ion ex-
change and adsorptive capacities of the aquifer sediments
for removal of potential pollutants may be nearly exhausted.
Information is lacking on the ability of various types of
sediments to treat infiltrated surface water and the time
factors involved.

Health agencies in the region generally rely on maintaining
an arbitrary distance between the well supply and the sur-
face-water source as a safeguard against ground-water con-
tamination.  Also, codes covering well construction call for
sealing the well against possible leakage of surface water
along the annular space outside the casing and require the
site to be protected against flooding from the nearby  stream.
Pumping tests of up to five days are another requirement,
the purpose of which theoretically  is to provide  enough  data
for determination of the effects of infiltrated  surface  wa-
ter on  ground-water quality.

                             271

-------
Because  of  the highly  complex  geologic  and hydrologic condi-
tions  that  occur  in  the  study  area, especially in the gla-
ciated portion, these  safeguards may not be adequate.  The
ability  for surface  water to infiltrate to high-capacity
wells  varies greatly from place to place.  For example, a
uniform  distance  of  200  feet for wells  located near two
polluted streams  of  similar quality may be safe in one in-
stance but  not in the  other, depending on the percentage of
surface  water infiltrated, the time of travel for a drop of
infiltrated surface  water to migrate from the bottom of the
stream bed  to the well screen, and the ability of the sedi-
ments  in the aquifer to  modify the quality of the surface
water.   Weeks, and in  some cases months, of pumping may be
required for a detectable volume of infiltrated surface wa-
ter to reach a particular well.  Only then can a proper
judgement be made on long-term water-quality relationships
between  surface water  and ground water.

Regulation  of well development adjacent to streams should be
based  on a  more specific and technical analysis of hydraulic
and water-quality conditions at each particular site under
consideration.  In some  cases, ground-water supplies that
may be perfectly  safe  for public consumption are not being
developed because they do not  meet arbitrary requirements
set by regulatory agencies.  At other sites, the parameters
are being met but may not be protective enough.

One problem that  appears to be quite common to infiltrated
ground-water supplies containing high concentrations of iron
is the growth of  iron bacteria in water from wells after
some period of use.  Little is known about the cause of this
phenomenon,  for example whether the bacteria originates in
the aquifer as a  result  of the addition of trace amounts of
organic  matter due to infiltration of surface water or
whether  it  may be related to conditions in the particular
water-supply distribution systems.  Also, long-lasting
methods  for cleaning up  this form of contamination have not
been developed.

UNDERGROUND STORAGE AND ARTIFICIAL RECHARGE OF WASTE WATER

Waste water is purposely disposed of or recharged to the un-
derground in the  northeast region in a number of different
ways.   Discharge  of  sewage effluent to septic tanks and cess-
pools is  the most common method and is discussed separately
in another  portion of the report.  Other means of disposal
include  deep wells drilled into saline aquifers, shallow
wells discharging into fresh-water aquifers, pits and basins
for rapid infiltration,  and spray irrigation.  Each of these
is discussed separately  in the following paragraphs.


                             272

-------
Deep Disposal Wells

Disposal of industrial wastes in saline aquifers through
wells more than 1,000 feet deep has been practiced in only
two of the states of the study region, New York and Penn-
sylvania.  Four injection wells have been constructed in New
York and nine in Pennsylvania. 168,169)  To date, only one
of the wells has ever been placed into operation in New York.
In Pennsylvania, all but perhaps one or two of the original
nine injection wells have been shut down. 169)

Most of the wells have not been put into operation or have
been abandoned because of difficulties in the physical oper-
ation of the system.  One 1,600 foot-deep injection well did
fail in Erie, Pennsylvania, in 1968. 170)  Apparently, after
four years of operation during which approximately 55,000
barrels per day of spent sulfite liquor containing fiber,
titanium dioxide, clay, and lignin-like compounds were pump-
ed into the well under pressure, the injection tubing cor-
roded, and the pressure was released to the outer well
casing.  It is not known whether shallow fresh-water aqui-
fers were contaminated, but a considerable volume of the
pollutant was discharged into Lake Erie.

Few if any new industrial-waste injection wells will be con-
structed in the region in the foreseeable future.  Inter-
views with representatives of environmental agencies in the
11 states covered by  this report revealed a very negative
attitude toward deep  well disposal.  The principal reason
given is that geologic conditions  are  not considered to be
favorable for the safe disposal and storage of  chemical
wastes underground.   In most  states,  a proposal  for deep dis-
posal of industrial wastes would not  even be  considered.   In
others,  rigid constraints imposed  by  regulatory  agencies
would most likely rule out consideration of such an alterna-
tive for waste disposal.

Shallow  Disposal Wells

Shallow  wells,  less  than  1,000  feet deep, completed in  fresh-
water aquifers  are used  in the  northeast to dispose of  a
variety  of liquid wastes  including storm water,  sewage,  cool-
ing water, and  industrial effluent.   They can be constructed
for the  specific purpose  of  injecting the fluid under con-
trolled  conditions,  sometimes under pressure, or they simply
can be abandoned water wells  converted to receiving waste
water.   Public  agencies  in some portions of the study region
have encouraged experimentation with  or use of  shallow  wells
for disposal or recharge  of  storm-water runoff from streets
and buildings,  unadulterated cooling  water  from air  condi-


                              273

-------
 tioners,  and tertiary-treated sewage effluent.   Although
 shallow wells recharging fresh-water aquifers with  untreated
 sewage  effluent  or industrial waste water exist, they  are
 considered  to be illegal throughout the  region.

 The  type  and degree of contamination of  fresh ground-water
 aquifers  that can occur as  a  result of waste-water  recharge
 through wells depends, of course,  on the source  of  the pol-
 lutant.   For example,  storm waters can contain high levels
 of BOD, COD, nitrates, phosphates, chlorides, and heavy
 metals. 69)   The injection  of heated waste waters from air
 cooling systems  can raise ground-water temperatures.

 Case Histories -

 Storm-water  runoff from paved areas at industrial sites, air-
 ports,  and  roadways is sometimes collected in dry wells,
 which consist of perforated or porous concrete rings set in
 a hole  usually dug five to  10 feet below land surface  or to
 the  top of  the water table.   If the water contains  fertil-
 izers,  pesticides,  and insecticides used on  lawns in a
 housing development, or a high level of  chlorides from ap-
 plication of deicing salts, contamination of the shallow
 aquifer can  occur in the vicinity  of the disposal well.  The
 injection of drainage  water,  and possible injection of in-
 dustrial  wastes  through disposal wells has produced some
 ground-water contamination  in the  Buffalo, New York,
 area. 163)   use  of  dry wells  or "sumps"  is common in sub-
 urban Long Island,  New York.   The  wells  are placed  in  park-
 ing  lots  at  apartment,  office, industrial and shopping cen-
 ter  complexes, or in cloverleafs of housing developments, to
 collect and  dispose  of runoff.  Tens  of  thousands of dry
 wells are probably  used throughout the region for a similar
 purpose.  However,  their construction is not normally  super-
 vised by  public  agencies  and  their locations in  any partic-
 ular area are  unknown.

 Controlled experiments  involving injection of municipal
 sewage wastes  have  been carried out in at least  two loca-
 tions in  the  study  region.  A major research project in the
 treatment and  injection of  renovated  water has been underway
 for a number of years  at  Bay  Park  in  Nassau County, New York
 under the direction  of  the  U.  S. Geological Survey. 171,172)
Tertiary-treated  sewage  has been injected periodically  at a
 test rate of as high as  350 gpm into  a fresh-water  zone of
the Magothy aquifer  at  a  depth of  418 to 460 feet below land
surface.  Data are being  collected  to determine  the feasi-
bility of this method  for replenishment  of the aquifer.

The second experiment  involved disposal  of filtered sewage


                              274

-------
from the Town of Riverhead,  Suffolk County,  New York,  into
shallow wells screened in the glacial outwash.  173)   Consid-
erable plugging of the well  screens was encountered, and the
system has not been adapted  to permanent use.

Instances of uncontrolled disposal of domestic wastes to
wells that have led to recorded cases of ground-water con-
tamination include one in Berks County, Pennsylvania,  in
which it was discovered that sewage from a number of houses
was being discharged into wells about 100 feet deep. 174)
It is feared that both the unconsolidated and consolidated
aquifers in the area have been contaminated.  In several
villages in Connecticut, water softener effluent discharged
into dry wells at apartment buildings has raised chloride
and sodium concentrations in water from nearby domestic
wells tapping shallow glacial deposits. 175)

Since 1933, New York State has required the return to the
ground of water pumped for industrial air-conditioning pur-
poses "in an uncontaminated condition through diffusion
wells or other approved structures." 176)  The regulation
covers all new industrial wells with capacities in excess of
100,000 gpd.  The term "diffusion wells" actually refers to
a recharge or injection well, and they have been used almost
exclusively for disposing of waste water from air condition-
ing or cooling systems.  Estimates are that 1,000 such wells,
screened in the glacial and Magothy aquifers of Long Island,
are in operation today and inject about 80 mgd of heated
water into the subsurface. 160)  Reports of problems related
to thermal pollution of ground water in Long Island are not
numerous, but as far back as 1937, an investigation in Kings
County noted a rise of 14°F in the sediments surrounding a
diffusion well in the shallow glacial aquifer. 158)  The
well injected about one mgd of cooling waste water  from  an
ice manufacturing plant.  Natural temperature of shallow
ground water on Long Island is 52° to 56°F.  The temperature
of the recharge water was about  83°F.  A few wells  in other
parts of Kings County have yielded water with temperatures
about 80°F. 177)

In New Jersey, protection of ground-water diversion rights
in critical areas of the state has encouraged recharge of
waste cooling water from air conditioning systems at commer-
cial and industrial sites rather than disposal of the waste
water to sewers.  Normally, the  only form of pollution is  a
rise in temperature because the  ground water is circulated
through a closed  system and chemicals for corrosion control
are not added to  the cooling water.  Whether enough recharge
wells of this type have been drilled in urbanized areas  of
New Jersey to locally modify the normal ground-water temper-

                             275

-------
 ature  of  about  52°F  has  not been investigated.

 Use  of wells  completed in  fresh-water  aquifers  for  disposal
 of industrial wastes is  probably rare  in  the  region.   How-
 ever,  one case  that  came to light in Pennsylvania a few
 years  ago is  worthy  of note.   Plating  wastes  that were being
 injected  illegally through shallow wells  contaminated  a  lime-
 stone  aquifer.  178)   The principal pollutant  is hexavalent
 chromium.   Water  from public-supply wells several thousand
 feet away were  affected  before the source of  contamination
 was  discovered  and eliminated.

 Future Trends -

 Recharge  of waste water  through shallow wells will  probably
 not  be an important  source of  contamination in  the  northeast
 in the future except in  the case  of dry wells used  for dis-
 posal  of  storm-water runoff.and recharge  wells  used to in-
 ject waste cooling waters.   Such  waters generally are  not
 considered as sources of contamination to ground water.  How-
 ever,  more controls  are  needed to guard against use of dry
 wells  and recharge wells for disposal  of  waters that may
 contain chemical pollutants  originating from  industrial
 processes.  Furthermore, runoff from highways,  roadways,
 parking lots  and lawn areas  can contain fertilizer,  salt,
 pesticide,  and  other organic and  inorganic residues.   Re-
 search is  needed to  determine  the effects  of  these  sub-
 stances on ground-water  quality in urban  areas.

 Additional  research  on well-construction  techniques and  wa-
 ter  renovation  is needed to  solve current  problems  of  plug-
 ging of screens and  clogging of aquifer materials before
 disposal  of treated  sewage  effluent in shallow  wells can be
 widely practiced.  The New  England River  Basins Commission
 in their  1973-1974 Long  Island  Sound Regional Study has  con-
 cluded 'that technological  capability for  recycling  treated
 waste  water into underground supplies  will not  be available
 before  1985.  179)  Industrial-waste water  is  regarded  by
 regulatory  agencies  as too hazardous for  injection  into
 fresh-water aquifers because of the hazardous materials  that
may  be  contained in  the  effluent,  and  injection will con-
 tinue  to be prohibited.

 Recharge Basins

Recharge basins are  used in the region to  dispose of storm-
water  runoff, industrial and commercial wastes, and treated
 sewage.  They are unlined rectangular  excavations up to  20
 feet deep, and  they  range in size  from a  few thousand  square
 feet to more than 10 acres.  Where rapid  infiltration  is de-

                             276

-------
sired, or the water table is shallow, basins are sometimes
constructed partially or completely above ground within a
set of dikes in order to raise the head of the recharge
water.

Probably the greatest density of recharge basins in the
study area is on Long Island, New York, where more than
2,000 are used for disposal of storm-water runoff and about
200 for discharge of industrial and commercial wastes.  It
is estimated that in 1966 about 100 mgd was recharged to
shallow aquifers through the storm-runoff detention basins
and about 30 mgd through the 200 industrial and commercial
basins. 180)  Principally as a conservation measure to in-
sure  continued replenishment of the aquifers underlying Long
Island, most new housing and industrial developments in
Nassau and Suffolk Counties have been required over the past
two decades to include the construction of one or more ba-
sins, depending on the size of the drainage area involved.
In addition, much of the runoff from highways and streets on
Long  Island is collected in recharge basins.  Industrial and
commercial waste water disposed of in recharge basins on
Long  Island generally is derived from cooling systems and
thus  heat is the only pollutant.

The use of recharge basins for rapid infiltration of treated
municipal sewage effluent is not widely practiced in the re-
gion.  However, interest in this method of disposal is grow-
ing because of stricter regulation of waste discharge to
surface streams.  For example, in New Jersey, rapid infil-
tration of municipal waste that has  received at  least sec-
ondary treatment has been approved by regulatory agencies
over  the past few years in a number  of cases where disposal
to surface waters available to the treatment plant has been
ruled out because of enforcement of  a stream water-quality
classification system.  In these cases, use of  septic tanks
was also ruled out because individual  lot sizes were  too
small or the projected  flow rate was too  high.

In New York, rapid infiltration of municipal sewage wastes
dates back  to 1936 at the Lake George Village treatment
plant.  Altogether, about a dozen  other municipal systems  in
the state are recharging through  leaching pits  or sand
filters.  Average  flow  rates are  relatively small, with  none
exceeding one mgd. 181)  Massachusetts has  another relative-
ly old rapid  infiltration system  at  Fort  Devens, where
treated  sewage effluent has been  recharged  underground  for
about 30 years.  182)

Because  of  the general  lack  of monitoring of  ground-water
quality  at  such  sites,  it is not  known what effect recharg-


                              277

-------
 ing of treated sewage has  over the long term.   Certainly
 concentrations of nitrates are raised,  along with those  of
 chlorides  and perhaps other minerals, in the immediate
 vicinity of the recharge basins,  but how extensive this  con-
 tamination is under different conditions of  soil,  geology,
 and hydrology is unknown.   Nevertheless, as  an  alternative
 for domestic waste disposal,  rapid infiltration probably
 compares favorably with  the use of septic tanks at many  lo-
 cations because the sewage can be treated to some  degree be-
 fore it is discharged underground.

 Spray Irrigation

 Spray irrigation has  been  defined as "the controlled  spray-
 ing of liquid onto land  at a  rate measured in inches  of
 liquid per week with  the flow path being infiltration and
 percolation within the boundaries of the disposal  site." 183)
 Within the northeast  region,  spray irrigation has  been ap-
 plied to both forested sites  and  agricultural lands.  The
 method has been used  to  dispose of municipal or domestic
 wastes from small  communities,  housing  developments,  and
 recreational areas.   It  has also  been used for  the land
 treatment  of some  industrial  wastes, principally from food
 processing.   As  in the case of rapid infiltration  of  sewage
 effluent discussed above,  the percentage disposed  of  through
 spray irrigation  is small  as  compared to the overall  dis-
 charge of  waste  effluent in the region.   However,  interest
 and activity in  the application of  spray irrigation is grow-
 ing,  again because  of  stricter controls  over discharge of
 sewage and industrial  wastes  to surface  streams.

 Although information is  limited on  the  location  and opera-
 tion  of existing  spray irrigation systems, discussions with
 representatives of public  agencies  in the  region indicate
 that  the practice  is carried  out  in a limited way  or  experi-
 mentally in every  one  of the  11 states.   Information  for
 those  sites  for which  data has  been collected indicates  that
 the average  rate of disposal  of wastes  is  generally less
 than  one mgd.  However,  there  are exceptions.  For example,
 the Hunt-Wesson Foods  Corporation  in Bridgeton,  New Jersey,
 reportedly  spray  irrigates three mgd, and  the H. J. Heinz
Company in  Salem, New  Jersey,  periodically spray irrigates
 1.3 mgd.   Both involve application  of wastes from  food
processing.  183)

The spray-irrigation system that has received the  most re-
search  is  the one  in operation  at State  College, Pennsyl-
vania.  184)  At this site, personnel from  the Pennsylvania
State University have  been studying such factors as infiltra-
tion capacity of the soil, effects  of climate, and the abil-


                              278

-------
ity of the land to treat domestic sewage effluent.   Studies
are continuing and include the collection of information on
long-term effects of spray irrigation of waste water on
ground-water quality.

Because of the general lack of monitoring and/or the evalua-
tion of data collected from monitoring wells, little is
known at present with regard to the relationship between
high rates of sewage application to the land and the ability
of the soils to render the effluent harmless.  However, data
on two cases of ground-water contamination related to spray
irrigation were collected in this survey.  One involved a
well supply that became contaminated with a phenolic mate-
rial from spray irrigation of organic wastes from a chicken
processing plant in Maryland. 185)  The other involved con-
tamination of a limestone aquifer in Pennsylvania caused by
spraying and lagooning of phenolic materials and solvents
from chemical industries.  In this latter case, a contamin-
ated zone 4,000 feet long and 300 feet wide was formed in
the shallow aquifer.  Spray irrigation has been halted and
the waste lagoons have been lined. 141)

Because of the large land area normally required for this
method of disposal of municipal wastes, use of spray irriga-
tion will probably continue to be limited to small communi-
ties and individual  industries.  More information is needed,
based on monitoring  of existing sites, in order to deter-
mine whether spray irrigation represents a significant
source of ground-water contamination.  Two states in the
study region, Pennsylvania and Vermont, have prepared manu-
als on site selection and system design for  spray irriga-
tion. 186,187)  AS interest in this process  increases,  other
states in the region will probably develop similar  standards.
Considerable additional research is needed on  the effects  of
the various types of wastes proposed  for  land  application  so
that future problems related  to  degradation  of ground-water
quality can be avoided.

WATER WELLS

Water wells themselves  are not normally  sources of  ground-
water contamination  except where a casing has  been  corroded
or ruptured, where well screens  or the  open  borehole inter-
connects two separate aquifers,  or where  the surface casing
has not been adequately sealed in soil or rock.  In these
instances, water wells can serve as a means  for transmission
of pollutants from one aquifer to another or from the  land
surface to an aquifer.

One of the most common problems related to this source  of


                             279

-------
 contamination  is  the  vertical movement  of  saline water into
 a  fresh-water  aquifer.   In  a number  of  the cases of salt-
 water  intrusion listed  in Table  44,  the contamination of the
 fresh-water  aquifer was aggravated by the  presence in the
 area of numerous  abandoned  and corroded well casings, which
 allowed saline water  to enter the fresh-water aquifer either
 from an overlying or  underlying  saline-water aquifer or from
 an adjacent  salty surface-water  body.   Probably the most
 classic case of this  type of contamination has taken place
 in Baltimore, Maryland.  188)  Contamination of ground water
 by industrial waste was  first recognized in the late 1800's
 when it was  reported  that soils  in the  heavily industrial-
 ized districts of that  coastal municipality were saturated
 with acid from metal  processing  operations and sulfuric acid
 plants.  A sample of  ground water collected from a 30-foot
 deep well in the  area in 1944 contained 664 mg/1 of chromium,
 Also,  the concentration  of copper sulfate  in ground water
 was sufficiently  high to warrant investigation of the eco-
 nomic  feasibility of  recovering  and  processing this compound,

 This ground-water body  contaminated  with industrial waste,
 together with saline  water that  had  encroached into the
 shallow aquifers  underlying the  industrial area, have led to
 corrosion of abandoned wells and intrusion of saline water
 into the deeper,  fresh-water, artesian  aquifer.  The casings
 have developed holes  or  collapsed and act as conduits allow-
 ing the poor-quality  water to migrate into the deeper arte-
 sian aquifer.  At locations where leaky well casings are not
 in abundance, salt-water intrusion has  not occurred because
 the artesian aquifer  is  protected by an overlying clay forma-
 tion.

 Other  causes of casing  failure have  been related to stray
 electrical currents in the ground in the industrial area,
 which  may cause holes to develop in  well casings.  Also, in-
 adequate sealing  of rotary-drilled water wells has allowed
 saline water to migrate  downward along  the annular space be-
 tween  the outer casing and the bore  hole.

 It is  estimated that  about 1,500 wells  had been drilled in
 the industrial area up to 1950,  of which more than 1,000 are
no longer accessible.  Many are  covered by buildings, paved
 areas,  and artificial fill.  Only about 12 percent of the
more than 1,000 abandoned wells  have been plugged.  A major
portion of the remaining wells are probably the principal
contributing factor to saline-water  intrusion that has af-
 fected most  of the industrial well fields in the area.

Discussions with  drilling contractors in the region have re-
vealed a number of other practices related to abandoned
                             280

-------
water wells that could lead to ground-water contamination.
The most common observation was the destruction of water
wells during demolition of buildings or houses in order to
make way for new highways, to clear the way for road widen-
ing, or to prepare a site for construction of apartments,
offices, and shopping centers.  In most cases, the old wells
serving the demolished houses are simply bulldozed over.
The surface casings and seals are broken, and because of
this, the old wells become a direct route for pollutants,
such as highway deicing salts or sewage from leaky pipelines,
to enter the underlying aquifer.

Operating wells can also act as conduits for pollutants to
migrate into an aquifer.  Normally this occurs because the
annular space between the casing and the borehole is im-
properly sealed.  Surveys of sanitary conditions of domestic
wells in the region, some of which are summarized on page
152 of this report, indicate that a high percentage of pri-
vately-owned water wells in any particular area do not meet
minimum health standards.  Inspections by health authorities
reveal that in numerous cases the well is not properly pro-
tected against contamination from overland runoff contain-
ing septic fluids, barnyard wastes, or storm waters and/or
the water yielded by a particular well shows a relatively
high concentration of bacteria.  It was the general con-
sensus of opinion of those health authorities interviewed
that a high percentage of wells serving individual residences
are sources of contamination in the immediate vicinity  of
the well but that public-supply wells serving communities
are rarely operating under unsanitary conditions.

A number of states and local health agencies  have adopted
regulations and codes governing well construction and the
plugging of abandoned wells.  Also, water-well drillers  must
be  licensed in eight out  of the  11  states.  New  York is  in-
cluded  as one of  the eight  states but  licensing  only ap-
plies to Long Island.

The regulations covering construction  of  public  water-supply
wells normally call for  protection  against flooding of  the
site, minimum distance  from a  potential  source of pollution
such as a  sewer line, and minimum  length  of casing  and  sur-
face grouting.  However,  the  specific  standards  set by  indi-
vidual  states vary  considerably.   For  example, in Connecti-
cut a protective  radius  of  200  feet is  required  between a
public  supply well  and  potential sources  of contamination.
In  the  neighboring  state of Massachusetts the radius  is 400
feet.   In  New Jersey, installation of  a  cement grout  extend-
ing from  land  surface to a  depth of 50  feet is rigidly en-
forced, whereas in  many of  the other  states,  codes  covering
                               281

-------
 this  aspect  of well  construction  are  not  specifically  spell-
 ed  out.

 Only  in  Delaware, Maryland, New Jersey, Pennsylvania,  and
 Long  Island, New York  is  the  plugging of  abandoned wells
 mandatory. 34)  some of these states,  for example in New
 Jersey,  have issued  explicit  requirements that must be fol-
 lowed, such  as material to be used.   Enforcement of plugging
 of  large diameter wells has been  relatively  successful be-
 cause these  are the  same  states where diversion rights for
 ground-water pumpage must be  sought by application to  the
 state.   Thus, the existence and location  of  high capacity
 wells is generally recorded.   Periodic reporting by ground-
 water users  indicates  when wells  with diversion rights go
 out of service or are  replaced.   Thus, the state agency can
 follow up with a request  for  plugging the abandoned well.
 In  the remaining states in the region, locations of oper-
 ating public-supply  and industrial wells  are generally not
 recorded and enforcement  of the plugging  of  abandoned  wells
 would be extremely difficult.  The same holds true for do-
 mestic and small commercial wells throughout the region.

 Certainly more control is needed  over  the construction of
 domestic wells and the fate of abandoned  wells.  Also,  li-
 censing  of well drillers  in those states  where such regula-
 tion does not exist  would aid in  correcting  some of the
 faulty construction  practices now in  use  in  such areas.
 Most important of all, the arbitrary  reasoning behind  some
 of  the rules involving such protective codes as distances to
 potential sources of contamination should be reevaluated.
 The origin of some of these codes dates back many decades,
 before the occurrence and movement of  ground water under
 various  hydrologic and geologic conditions was adequately
 understood.

 AGRICULTURAL ACTIVITIES

 A number  of  activities associated with crop  growing, horti-
 culture,  dairy farming, and cattle raising can lead to  con-
 tamination of ground-water supplies.   Pollutants derived
 from fertilizers, pesticides,  herbicides,  animal wastes, and
 irrigation return flows can infiltrate with  rain water  or
 snow melt and eventually can  be carried down to the underly-
 ing aquifer.  Considerable treatment of waste products  from
 agricultural activities takes  place in the soil zone,  and
 contamination of ground water from this source probably
 ranks very low in importance  compared with other sources
 discussed in this report.  The only exception to this  is the
 application of fertilizers, which have affected ground-water
quality in heavily cultivated areas such  as  the lower Con-


                              282

-------
necticut River valley, where tobacco is a very important
crop, and Long Island, New York, where potato farming is a
major industry.  In both of these regions, urbanization has
changed land-use patterns and agricultural activity has de-
clined radically since the early 1950's.  However, nitrates
related to heavy use of fertili2ers during decades of culti-
vation are still contained in fresh-water aquifers and con-
siderable time will be required before this pollutant has
been flushed out.  Undoubtedly, in other farm areas in the
region, such as southern New Jersey, parts of Delaware and
Maryland, and northern New England, contamination of aqui-
fers over broad areas is occurring.  However, population
density is still low enough so that the problem remains rel-
atively obscure.

One problem related to fertilizers and also herbicides that
should not be overlooked is the potential for significant
ground-water contamination from the large quantities of
these two substances which are applied to lawns in suburban
areas.  It is conceivable that some of the high nitrate con-
centrations observed in ground waters underlying  suburban
areas may be caused by the heavy application of lawn fertil-
izers rather than agricultural activity which took place be-
fore the area became urbanized.  Additional research on this
subject is needed.  In addition, more data is needed on
whether the organic and inorganic compounds found in the
various types of herbicides have penetrated the soil zone
and entered the ground-water system in  suburban areas.

A few cases of contamination of ground water  from the  appli-
cation of pesticides have been noted  in  the region.  Because
of the lack of well-water analyses that  include tests  for
pesticide compounds,  it is difficult  to  tell  whether the
cases given below are unique or whether  they  represent a
widespread problem.

     *Water from a domestic well in Connecticut was  affected
by thallium which had been used  in a  rose spray.  Apparently,
thallium-rich waste water from  the rose  growing operation
had  seeped into the sandstone aquifer tapped  by the  domes-
tic well. 189)

     *Chlorinated hydrocarbons  from pesticide spray  used  on
cranberry bogs in Massachusetts have  affected the water
quality from at least one sand and gravel aquifer used for
public supply.  In another case in Massachusetts, the  pres-
ence of chlorinated hydrocarbons from the operation of a
greenhouse has been confirmed in a sample of water from a
shallow sand and gravel aquifer. 190)
                             283

-------
      *A  spring  in New  Hampshire has  been  found  to  contain
traces of arsenic, presumably  from the  residue  of  pesticide
sprays used  for orchards.  191)

      *Arsenate  compounds used  for insect  control in  the
blueberry barrens of Maine have been found  in surface
streams  and  may have entered shallow ground-water  aqui-
fers. 192)

      *Water  from a domestic well in  Pennsylvania was contam-
inated by chlordane applied to trenches around  the house
served by the well.  The chlordane was  used for termite con-
trol. 142)

With  regard  to  barnyard or animal waste problems,  discussions
with  health  authorities indicate that many  domestic wells in
farm  areas are  contaminated because  of  the  improper handling
of manure combined with poor well construction.  Normally
the only well affected by  a particular  source of animal
wastes is the well serving the same  farm.

Irrigation is not widely practiced in the region and esti-
mates of the proportion of irrigated land to total crop land
are less than two percent.  Based on this fact, it is doubt-
ful that salinity problems related to irrigation return
flows are significant in the study region.  193)

Agricultural activities in the traditional  sense will prob-
ably decline in the future as  the region becomes even more
urbanized.  However, the use of fertilizers, herbicides, and
pesticides by individual home  owners  in suburban areas will
continue, and the potential for contamination of ground
water from these activities has not  received enough atten-
tion in  the past.  There is a  definite need for controlled
studies  of long-term affects from the application  of commer-
cial products sold for suburban agricultural use on lawns,
gardens, trees, and shrubs.  If it is found that ground-
water quality is being affected, then consideration should
be given to controls over  the  use of such products, and pro-
grams directed toward education of the public should be de-
veloped  so that more efficient handling and application can
be achieved.
                             284

-------
                       REFERENCES CITED

                          SECTION VI
 1.  Murray, C. R.,  and E. B. Reeves, "Estimated Use of Water
     in the United States in 1970," U.  S.  Geological Survey
     Circular 676, 1972.

 2.  New Jersey Commission on Efficiency and Economy in State
     Government, "Water Resources Management in New Jersey,"
     1967.

 3.  Thomas, J. D.,  and S. G. Heidel, "Chemical and Physical
     Character of Municipal Water Supplies in Maryland,"
     Maryland Geological Survey Report of Investigation No. 9,
     1969.

 4.  Heath, R. C., "Ground Water in New York," State of New
     York Conservation Department, Water Resources Commission
     Bulletin GW-51, 1964.

 5.  Connecticut Interagency Water Resources Planning Board,
    "Statewide Long-Range Plan for the Management of the Water
     Resources of Connecticut, Phase I Report," Connecticut
     Office of State Planning, Department of Finance and Con-
     trol, HUD Project No. P-128, 1971.

 6.  Todd, D. K., "The Water Encyclopedia," Port Washington,
     N. Y., Water Information Center, Inc., 1971.

 7.  Tippetts-Abbett-McCarthy-Stratton Engineers,  "Survey  of
     New  Jersey Water Resources Development," New Jersey Leg-
     islative Commission  on Water Supply, 1955.

 8.  New  York State Water Resources Commission,  "Developing
     and  Managing  the Water Resources of New York State/'
     New  York State Conservation Department, Division of Water
     Resources, 1967.

 9.  Deutsch, Morris, "Ground-Water Contamination and Legal
     Controls in Michigan," U. S. Geological Survey Water-
     Supply Paper 1691, 1963.

10.  Water and Petroleum Study Group, "Evaluation and Treatment
     of Oil Spill Accidents on Land with a View to the Protec-
     tion of Water Resources," Bonn, West Germany, Federal Min-
     istry of the Interior, Second Edition,  December 1970.


                               285

-------
 11.  Lieber, Maxim, N. M.  Perlmutter,  and H. L. Frauenthal,
     "Cadmium  and  Hexavalent  Chromium  in Nassau County Ground
     Water," Journal American Water Works Association, Vol. 56,
     No.  6, June 1964.

 12.  Suffolk County, New York, Personal Communication, 1973.

 13.  Kasabach, H.  F.,  "Geology and Ground-Water Resources of
     Hunterdon County, New Jersey," New Jersey Bureau of Geol-
     ogy  and Topography Special Report No. 24, 1966.

 14.  Wright, J. F., "Administrative and Legal Considerations:
     An Interstate Viewpoint," University of California Water
     Resources Engineering Educational Series, 1973.

 15.  Albany County Health Department, New York, Personal Com-
     munication, 1973.

 16.  Parizek, R. R., W. B. White, and Donald Langmuir, "Hydro-
     geology and Geochemistry of Folded and Faulted Rocks of
     the  Central Appalachian Type and Related Land Use Prob-
     lems," Pennsylvania State University Mineral Conservation
     Series Circular 82, 1971.

 17.  Gaun, G. R., and L. J. McCabe, "Review of the Causes of
     Waterborne Disease Outbreaks," Journal American Water Works
     Association, Vol. 65, No. 1, January 1973.

 18.  Drewry, W. A., and Rolf Eliassen, "Virus Movement in Ground
     Water," Journal Water Pollution Control Federation, Vol. 40,
     No.  8, Pt. 2,  August 1968.

 19.  Rasmussen, W.  C., and G.  E.  Andreasen, "A Hydrologic Budget
     of the Beaverdam Creek Basin, Maryland," U.  S. Geological
     Survey Open-file Report,  March 1967.

 20.  Olmsted, F. H.,  and A. G. Hely, "Relation Between Ground
     Water and Surface Water in Brandywine Creek Basin, Penn-
     sylvania," U.  S.  Geological  Survey Professional Paper
     417-A, 1962.

21.  Morrill, G. B.,  Ill,  and  L.  G. Toler, "Effect of Septic-
     Tank Wastes on Quality of Water,  Ipswich and Shawsheen
     River Basins,  Massachusetts," U.  S.  Geological Survey
     Journal of Research,  Vol. 1, No.  1,  January-February 1973.

22.  Geraghty & Miller, Inc.,  Consultant's Report, 1972.
                               286

-------
75.  Hepple, Peter, ed., "The Joint Problems of the Oil and
     Water Industries - Proceedings of a Symposium, Brighton,
     England, January 1967," The Institute of Petroleum, Lon-
     don, 1967.

76.  Kimmel, G. E. , "Nitrogen Content of Ground Water in Kings
     County, Long Island, New York," U. S. -Geological Survey
     Professional Paper 800-D, Geological Survey Research, 1972.

77.  Ground Water Section, "Site Memorandum," Pennsylvania
     Department of Environmental Resources, Division of Water
     Quality, January 1969.

78.  Ground Water Section, "Site Memorandum," Pennsylvania
     Department of Environmental Resources, Division of Water
     Quality, May  1970.

79.  Water Compliance Section, Connecticut Department  of  Envi-
      ronmental  Protection, Personal  Communication,  1973.

80.  Department of Health, New Jersey Department of Environmental
     Protection, Personal Communication,  1973.

81.  Onondaga County Health Department, New York,  Personal  Com-
     munication, 1973.

82.  Geraghty & Miller,  Inc., Consultant's  Investigation, 1973.

83.  Legislative Research Council,  "The Use  and Effects of  High-
     way De-icing  Salts," Massachusetts Senate Document 2,  Jan-
     uary 1965.

84.  Hanes, R. E., L. W. Zelazny, and R.  E. Blaser,  "Effects
     of Deicing Salts on Water Quality and Biota," National
     Academy of Sciences, Highway Research Board, National  Co-
     operative Highway Research Program Report 91, 1970.

85.  Highway Research Board, "Environmental Degradation by De-
     icing Chemicals and Effective Countermeasures," National
     Academy of Sciences, Highway Research Record Number 25,
     1973.

86.  National Resources and Agriculture Committee,  "Interim
     Report of the Special Commission on Salt Contamination of
     Water Supplies and Related Matters,"  Massachusetts Senate
     Document 1485, January 1973.

87.  Connecticut State Department of Health, "Analyses of Con-
     necticut Public Water Supplies," Seventh Edition, 1971.


                              287

-------
23.  York County Health Department, Maine, in cooperation with
     U. S. Environmental Protection Agency, Investigation in
     progress, 1973.

24.  Woodhull, R. S.,  "Evaluation of Public Drinking Water
     Supplies in Connecticut," Connecticut Section American
     Water Works Association, unpublished paper presented at
     South Egremont, Mass.,  June 22, 1973.

25.  Gill, H. E., "Ground-Water Resources of Cape May County,
     New  jersey: Salt-Water Invasion of Principal Aquifers,"
     New  Jersey Division of Water Policy and Supply Special
     Report 18, 1962.

26.  Randall, A. D., "Movement of Bacteria from a River to a
     Municipal Well - A Case History," Journal American Water
     Works Association, Vol. 62, No. 11, November 1970.

27.  The Comptroller General of the United States, "Improved
     Federal and State Programs Needed to Insure the Purity
     and Safety of Drinking Water in the United States," U. S.
     General Accounting Office Report to the Congress, Novem-
     ber 1973.

28.  Wenk, V. D., "Water Pollution:  Domestic Wastes," The
     MITRE Corporation, Office of Science and Technology,
     Executive Office of the President, PB 202778-06, Volume
     6, 1971.

29.  Rensselaer County Health Department, "Water Resources in <•
     Rensselaer County," New York State Department of Health,
     1961.

30.  Rensselaer County Health Department, New York, Personal
     Communication,  1973.

31.  Connecticut Health Department, Personal Communication,
     1973.

32.  Muhich,  A.  J.,  A.  J.  Klee, and P.W. Britton, "Preliminary
     Data Analysis:   1968  National Survey of Community Solid
     Waste Practices,"  U.  S. Public Health Service Publication
     No. 1867, 1968.

33.  The General Electric  Company, "A Proposed Plan of Solid
     Waste Management for  Connecticut," Connecticut Department
     of Environmental Protection, June 1973.

34.  van der  Leeden, Frits, "Groundwater Pollution Features of
     Federal  and State  Statutes and Regulations," U.  S. Environ-
     mental Protection  Agency,  Environmental Monitoring Series
     600/4-73-OOla,  July 1973.
                             288

-------
35.   Field,  Richard,  et al,  "Water  Pollution  and  Associated
     Effects from Street Salting,"  U.  S.  Environmental  Protec-
     tion Agency, Environmental  Protection  Technology Series
     R2-73-257,  May 1973.

36.   Westlund,  C. W., Pennsylvania  Department of  Environmental
     Resources,  Personal Communication,  1973.

37.   Anonymous,  "Drink Purified  Sewage?   No,  Say  Experts,"
     Ground Water Age, August 1973.

38.   Public Health Service,  "Drinking Water Standards,  1962,"
     U. S. Department of Health, Education  and Welfare, 1962.

39.   Geraghty & Miller, Inc., Consultant's  Report, 1969.

40.   Pinder, G.  F. , "A Galerkin-Finite Element Simulation of
     Groundwater Contamination on Long Island, New York,"
     Water Resources Research, Vol. 9, No.  6, December  1973.

41.   Perlmutter, N. M., and Julian Soren, "Effects of Major
     Water-Table Changes in Kings and Queens Counties,  New
     York City," U. S. Geological Survey Professional Paper
     450-E, Geological Survey Research,  1963.

42.   Delaware River Basin Commission, Personal Communication,
     1973.

43.   Geraghty & Miller, Inc., Consultant's Report, 1973.

44.   Geraghty, J. J.,  "Movement of Contaminants Through Geo-
     logic Formations," Water Well Journal, Vol.  16,  1962.

45.   Private Water Company Representative,  Personal Communica-
     tion, 1973.

46.   County Personnel, Personal Communication, 1973.

47.   Delaware Division of Environmental Control, Personal
     Communication,  1973.

48.  Miller, J.  C.,  "Ground-Water Contamination in Delaware:
     Hydrogeologic Controls, Case Histories, Prevention and
     Abatement,"  Chesapeake  Section American Water Works As-
     sociation,  unpublished  paper, September  1973.

49.  Town Personnel, Personal Communication,  1973.
                               289

-------
 50.  New Hampshire Department of Public Works and Highways,
     Special Services Division, Personal Communication, 1973.

 51.  Rights and Ways Division,  "Annual Well Claims Report,"
     Maine State Department of  Transportation, July 1972.

 52.  Gregg, J. C., "Ion Exchange System to Treat High-Nitrate
     Well Water," Public Works, September 1972.

 53.  Bouma, J., et al, "Soil Absorption of Septic Tank Effluent,"
     University of Wisconsin, Soil Survey Division, Information
     Circular Number 20, 1972.

 54.  Feth, J. H., "Nitrogen Compounds in Natural Water - A
     Review," Water Resources Research, Vol. 2, No. 1, 1966.

 55.  Holzer, T. L., "Limits to Growth and Septic Tanks," pre-
     sented at Conference on Rural Environmental Engineering,
     Warren, Vermont, September 26, 1973.

 56.  Nassau-Suffolk Research Task Group, "The Long Island
     Ground-Water Pollution Study," State of New York Depart-
     ment of Health, 1969.

 57.  Perlmutter, N. M.,  and Ellis Koch, "Preliminary Hydrogeo-
     logic Appraisal of Nitrate in Ground Water and Streams,
     Southern Nassau County, Long Island, New York," U. S.
     Geological Survey Professional Paper 800-B, Geological
     Survey Research, 1972.

 58.  Perlmutter, N. M.,  and Ellis Koch, "Preliminary Findings
     on the Detergent and Phosphate Contents of Water of
     Southern Nassau County, New York," U. S. Geological
     Survey Professional Paper 750-D, Geological Survey Re-
     search, 1971.

 59.  Miller, J. C., "Nitrate Contamination of the Water-Table
     Aquifer in Delaware," Delaware Geological Survey Report of
     Investigation  No.  20, 1972.

60.  Miller, J. C., "Nitrate Contamination of the Water-Table
     Aquifer by Septic-Tank Systems in the Coastal Plain of
     Delaware," presented at the Conference of Rural Environ-
     mental Engineering,  Warren, Vermont, September 26, 1973.

61.  Division of Environmental Health Service, "A Report on
     Wells and Septic Systems in Montgomery County," Montgom-
     ery County Health Department,  Maryland,  1968.

62.  Confidential Communication, 1973.

                             290

-------
63.  Health Commission,  Stamford,  Connecticut,  Personal  Commu-
     nication, 1973.

64.  Division of Water Supply and  Pollution Control,  Rhode Is-
     land Department of  Health,  Personal Communication,  1973.

65.  Tourbier, Joachim,  "Water Resources as a Basis for  Compre-
     hensive Planning and Development in the Christina River
     Basin," University of Delaware Water Resources Center, 1973.

66.  Hill, D. E., and H. F. Thomas, "Use of Natural Resources
     Data in Land and Water Planning," The Connecticut Geology-
     Soil Task Force, Connecticut Agricultural Experimental
     Station, Bulletin 733, 1972.

67.  Kolega, J.J., W. C. Wheeler,  and G. W. Hawkins, Jr., "Cur-
     rent Septic Tank System Installation Practices in Connec-
     ticut," Journal of the Water Pollution Control Fpr^ra-t-i nn r
     Vol. 38, No. 10, October 1966.

68.  The Soap and Detergent Association, "The Suffolk County
     Detergent Ban - A Clarifying Comment," Water in the News,
     December 1970.

69.  Sartor, J. D., and G. B. Boyd, "Water Pollution Aspects of
     Street Surface Contaminants," U. S. Environmental Protection
     Agency, Office of Research and Monitoring/ 1972.

70.  Matis, J. R., "Petroleum Contamination of Ground Water in
     Maryland," Ground Water, Vol. 9, No. 6, November-December
     1971.

71.  Westlund, C. W., "Groundwater Pollution in Pennsylvania,"
     University of California Water Resources Engineering Edu-
     cational Series, 1973.

72.  Todd, D. K., "Groundwater Pollution in Europe - A Confer-
     ence Summary," U. S. Environmental Protection Agency, Of-
     fice of Research and Monitoring, 1973.

73.  Engineering and Technical Research Committee, "The Migration
     of Petroleum Products in Soil and Ground Water - Principles
     and Countermeasures," American Petroleum Institute, 1972.

74.  Economic Commission  for Europe,  "Proceedings of the Seminar
     on the Protection of Ground and  Surface Waters Against Pol-
     lution by Crude Oil  and Oil Products, Geneva, December 1969,"
     United Nations, Volumes 1 and 2, 1970.
                               291

-------
  88.  New Jersey  State Department of Health, Personal Communi-
      cation, 1973.

  89.  Hutchinson,  F. E.,  "Environmental Pollution from Highway
      Deicing Compounds," Journal of Soil and Water Conservation,
      Vol.  25, No. 4, July-August 1970.                ~      '—

  90.  Hutchinson,  F. E.,  and B. E. Olson, "The Relationship of
      Road  Salt Applications to Sodium and Chloride Ion Levels
      in the Soil  Bordering Major Highways," National Academy
      of Sciences, Highway Research Board, Highway Research
      Record Number 193,  1967.

  91..  Pollack, S.  J., and L. G. Toler, "Effects of Highway De-
      icing Salts  on Ground Water and Water Supplies in Massa-
      chusetts," Massachusetts Department of Public Works and
      U. S. Geological Survey Open-file Report, 1972.

  92.  Geraghty & Miller, Inc., Investigations, 1964-73.

  93.  New Jersey Department of Health, Files, 1973.

  94.  Freeport, Maine Water Department, Personal Communication,
      1973.

  95.  Bried, Raymond, "The Great Salt Controversy," Yankee,
      March 1973.

  96.  Gillies, N. P., ed., "Ground Water Newsletter," Vol. 3,
      No. 4, Port Washington, N. Y., Water Information Center,
      Inc., February 1974.

  97.  City of New York Environmental Protection Administration,
      Personal Communication, 1973.

  98.  State of New Jersey County and Municipal Government Study
      Commission,  "Solid Waste: A Coordinated Approach," Sev-
      enth Report, 1972.

 99.  Connecticut Department of Environmental Protection, Per-
      sonal Communication, April 1973.

100.  Bureau of Housing and Environmental Control, "A Plan for
      Solid Waste Management in Pennsylvania," Pennsylvania
      Department of Health,  Solid Waste Publication No. 3, 1970.

101.  Hagerty, D. J.,    L.  Pavoni,  and J. E.  Heer, Jr., "Solid
      Waste Management,"  New York,  Van Nostrand Reinhold Engi-
      neering Series, 1973.


                              292

-------
102.   Salvato,  J.  A.,  W.  G.  Wilkie,  and  B.  E.  Mead,  "Sanitary
      Landfill  - Leaching Prevention and Control," Journal
      Water Pollution  Control Federation, Vol.  43, No.  10,
      October 1971.

103.   Emrich, G. H.,  "Guidelines for Sanitary  Landfills -
      Ground Water and Percolation," paper  presented at En-
      vironmental Conference on Research and Development on
      Landfill Disposal of Solid Waste,  Deerfield, Massachusetts,
      October 24 - 28, 1970.

104.   Apgar, M. A.,  and Donald Langmuir, "Ground Water Pollution
      Potential of a Landfill Above the  Water  Table," Ground
      Water, Vol. 9,  No.  6,  November-December, 1971.

105.   Emrich, G. H.,  and R.  A. Landon, "Generation of Leachate
      from Landfills and Its Subsurface  Movement," paper pre-
      sented at the Annual Northeastern  Regional Anti-Pollution
      Conference, University of Rhode Island,  July 1969.

106.   Connecticut Department of Environmental Protection,  Files,
      1973.

107.   Otton, E. G., "Solid Waste Disposal in the Geohydrologic
      Environment of Maryland," Maryland Geological  Survey
      Report of Investigations No.  18, 1972.

108.   Thomas, C. E., Jr., M. A. Cervione, Jr., and  I.  G. Gross-
      man,  "Water Resources  Inventory of Connecticut,  Part  3,
      Lower Thames and Southeastern Coastal River Basins,"
      Connecticut Water  Resources Commission, Connecticut Water
      Resources Bulletin No.  15, 1968.

109.  Emrich, G. H., and R.  A. Landon,  "Investigation  of the
      Effects of Sanitary Landfills  in Coal Strip Mines on
      Ground Water Quality,"  Pennsylvania Department of En-
      vironmental Resources,  Bureau of Water  Quality Manage-
      ment  Publication No.  30,  1971.

110.  Delaware  Geological Survey, Personal  Communication, 1973.

111.  Grossman,  I. G., "Waterborne  Styrene  in a  Crystalline
      Bedrock Aquifer  in the Gales  Ferry Area, Ledyard,
      Southeastern Connecticut," U.  S.  Geological Survey
      Professional Paper 700-B,  Geological  Survey Research, 1970

112.  New Jersey  Department of Environmental  Protection,  Bureau
      of  Geology, Personal  Communication,  1973.
                              293

-------
113.  Geraghty & Miller, Inc., Consultant's Report, January
      1973.

114.  A. W. Martin Associates, Inc., "New Concept in Solid
      Waste Disposal in Quarry Conversion," Constructioneer,
      January 1972.

115.  Besselievre, E. B., "The Treatment of Industrial Wastes,"
      New York, McGraw-Hill Book Company, 1969.

116.  Maryland Department of Health and Mental Hygiene, Press
      Release, September 4, 1973.

117.  Schiffman, Arnold, Ground Water Technical Services,
      Maryland Department of Natural Resources, Personal Com-
      munication, 1973.

118.  Confidential Communication, 1973.

119.  Perlmutter, N. M., and Maxim Lieber, "Dispersal of Plating
      Wastes and Sewage Contaminants in Ground Water and Surface
      Water, South Farmingdale-Massapequa Area, Nassau County,
      New York," U. S. Geological Survey Water-Supply Paper
      1879-G, 1970.

120.  Delaware River Basin Commission, "A Resolution to Amend
      the Water Quality Standards in Relation to Protection of
      Ground Water," December 12, 1972.

121.  Maryland Water Resources Administration, "Groundwater
      Quality Standards," Regulation 08.05.04.04, May 1, 1973.

122.  Commonwealth of Pennsylvania, "Rules and Regulations,
      Section 101.4-Impoundments," Clean Streams Law of 1937,
      Chapter 101 - Special Water Pollution Regulations, Sep-
      tember 2,  1971.

123.  Greenman,  D. W., et al, "Ground-Water Resources of the
      Coastal Plain Area of Southeastern Pennsylvania," Penn-
      sylvania Topographic and Geologic Survey Bulletin W-13,
      1961.

124.  Arthur D.  Little, Inc., "Study of Waste Oil Disposal
      Practices in Massachusetts," report to Massachusetts
      Division of Water Pollution Control, 1969.

125.  Council on the Environment of New York City, "Waste Oil
      Study Shows 23 Million Gallons Lost Yearly in Metropol-
      itan Area," Press Release, March 1974.


                             294

-------
126.   New York State Department of Health,  Personal  Communica-
      tion, 1973.

127.   Chemung County Health Department,  New York,  Personal Com-
      munication,  1973.

128.   Bureau of Water Pollution Control, "Investigation Report,"
      New Jersey Department of Environmental Protection, Divi-
      sion of Water Resources, May 1973.

129.   Water Resources Committee, "Guidelines for Chemical Plants
      in the Prevention, Control, and Reporting of Spills,"
      Manufacturing Chemists' Association,  Inc., 1972.

130.   Battelle Northeast, "Oil Spill Treating Agents - A Com-
      pendium," American Petroleum Institute Committee for Air
      and Water Conservation, 1970.

131.   U. S. Department of Interior, "Surface Mining and Our
      Environment: A Special Report to the Nation," Washington,
      D. C., U. S. Government Printing Office, 1967.

132.   Chiu, S. Y., et al, "Methods for  Identifying and Evaluating
      the Nature and Extent of Nonpoint Sources of Pollutants,
      Environmental Protection Agency, Office of Air and Water
      Programs, Nonpoint Source Control Branch, 1973.

133.   U. S. Geological Survey, "The National Atlas of the United
      States of America," U. S. Department of Interior, 1970.

134.   Franklin, B. A., "Strip Mining for Coal in 1973," New
      York Times, February 28, 1974.

135.   Metsger, R. W., A. H. Willman, and C. G. Van Ness,  "Field
      Guide to the Friedensville Mine'," Allentown, Pennsylvania,
      The New Jersey Zinc Company, 1973.

136.   Woodward, H. P., "Copper Mines and Mining in New Jersey,"
      New Jersey Department of Conservation and Development,
      Geologic Series Bulletin 57, 1944.

137.  Murthy, V. R.., "Bedrock Geology  of  the East Barre  Area,
      Vermont," Vermont  Geological Survey  Bulletin No.  10,
      1957.

138.  Hill, R. D.,  "Mine Drainage Treatment, State of the Art
      and Research Needs," U.  S. Department of  Interior,  Fed-
      eral Water Pollution Control Administration, 1968.
                               295

-------
139.  Emrich, G. H., and G. L. Merritt, "Effects of Mine Drain-
      age on Ground Water," Ground Water,  Vol. 7, No.  3, May-
      June 1969.

140.  Merritt, G. L.,  and G. H. Emrich, "The Need for  Hydrogeo-
      logic Evaluations in a Mine Drainage Abatement Program:   A
      Case Study - Toms Run, Clarion County, Pennsylvania,"
      Third Symposium on Coal Mine Drainage Research,  Mellon
      Institute, May 19 - 20, 1970.

141.  Bureau of Water Quality Management,  Pennsylvania Depart-
      ment of Environmental Resources, Personal Communication,
      1973.

142.  Swarzenski, W. V., "Hydrogeology of  Northwestern Nassau
      and Northeastern Queens Counties, Long Island, New York,"
      U. S. Geological Survey Water-Supply Paper 1657, 1963.

143.  Crews, J. E., "Establishing Priorities in Mine Drainage
      Reductions: A Cost-Effectiveness Approach," Water Re-
      sources Bulletin, American Water Resources Association,
      1973.

144.  Foreman, J. W.,  and D. C. McLean, "Evaluation of Pollution
      Abatement Procedures, Moraine State  Park," U. S. Environ-
      mental Protection Agency, Office of  Research and Monitoring,
      1973.

145.  Anonymous, "Digging Into Mine Waste," Environmental
      Science & Technology, Vol. 8, No. 2, February 1974.

146.  Thompson, D. R., and G. H. Emrich, "Hydrogeologic Consid-
      erations for Sealing Coal Mines," Pennsylvania Department
      of Health, Bureau of Sanitary Engineering Publication No.
      23, 1969.

147.  Interstate Oil Compact Commission, Oklahoma City, Oklahoma,
      Personal Communication, 1974.

148.  Wetterhall, W. S., "The Ground-Water Resources of Chemung
      County, New York," State of New York Department  of Conser-
      vation, Water Power and Control Commission Bulletin GW-40,
      1959.

149.  Randall, A. D.,  "Records of Wells and Test Borings in the
      Susquehanna River Basin, New York,"  New York State Depart-
      ment of Environmental Conservation Bulletin No.  69, 1972.
                              296

-------
 161.   Geraghty  & Miller,  Inc.,  Investigation of Ground Water
       Conditions for  the  Cape May County Board of Chosen Free-
       holders,  New  Jersey, May  1971.

 162.   Krieger,  R. A., J.  L. Hatchett, and J. L. Poole, "Pre-
       liminary  Survey of  the Saline-Water Resources of the
       United  States," U.  S. Geological Survey Water-Supply
       Paper 1374, 1957.

 163.   LaSala, A. M., Jr.  "Ground-Water Resources of the Erie-
       Niagara Basin, New  York," State of New York Conservation
       Department, Water Resources Commission Basin Planning
       Report ENB-3, 1968.

 164.   Kantrowitz, I. H.,  "Ground-Water Resources in the Eastern
       Oswego River  Basin, New York," State of New York Conser-
       vation Department,  Water  Resources Commission Basin Plan-
       ning Report ORB-2,  1970.

 165.   Sheppard  T. Powell  Engineers, and Leggette & Brashears,
       "Report on the Effect of  Ship Channel Enlargement Above
       Philadelphia," prepared for The Committee for Study of
       the Delaware  River, May 1954.

 166.   Municipal Files and Confidential Communication, 1973.

 167.   Geraghty  & Miller,  Inc.,  "Availability of Water Resources
       in the Midstate Region of Connecticut," Connecticut Water
       Resources Commission, 1965.

 168.   ORSANCO Advisory Committee on Underground Injection of
       Wastewaters,  "Underground Injection of Wastewaters in the
       Ohio Valley Region," Ohio River Valley Water Sanitation
       Commission, 1973.

 169.   Warner, Donald, Department of Mining and Engineering,
       University of Missouri, Personal Communication, 1974.

 170.   Greenfield, S. 1-1.,  "EPA - The Environmental Watchman,"
      American Association of Petroleum Geologists, Memoir
       18, 1972.

 171.  Vecchioli, John, "Experimental Injection of Tertiary-
      Treated Sewage in a Deep Well at Bay Park, Long Island,
      New York - A Summary of Early Results," New England Water
      Works Association Bulletin, Vol.  LXXXVI, No.  2, June 1972.

172.  Koch, Ellis, A. A. Giaimo, and D.  J.  Sulam,  "Design and
      Operation of the Artificial Recharge Plant at Bay Park,
      New York," U.  S. Geological Survey Professional Paper
      751-B,  1973.
                              298

-------
173.  Baffa, J.  J.,  and N.  J.  Bartilucci,  "Wastewater  Reclama-
      tion by Ground Water  Recharge  on  Long  Island," Journal
      American Water Works  Association,  Vol.  39, No. 3,  March
      1967.

174.  Pennsylvania Department of Environmental  Resources,
      Bureau of Water Quality Management Files,  1973.

175.  U. S. Geological Survey, Hartford, Connecticut,  Regional
      Office Files,  1973.

176.  Johnson, A. H., "Ground Water  Recharge on Long Island,"
      Journal American Water Works Association, Vol. 49, No.
      11, November 1948.

177.  Geraghty, J. J., "Ground-Water Problems in the New York
      City Area," Annals of the New  York Academy of Sciences,
      Vol. 80, Article 4,  September  21, 1959.

178.  Private Water Company, Confidential Files, 1973.

179.  Long Island Sound Regional Study Group, "Toward a Plan
      for Long Island Sound," New England River Basins Commis-
      sion, Special Release, 1974.

180.  Parker, G. G. , Philip Cohen, and B. L. Foxworthy, "Arti-
      ficial Recharge and Its Role in Scientific Water Manage-
      ment with Emphasis on Long Island, New York," American
      Water Resources Association, Proceedings of the National
      Symposium on Ground-Water Hydrology, 1967.

181.  Boggedain, F. O., "New York State's View of Land Disposal,"
      U.  S. Environmental Protection Agency, Proceedings of
      Conference on Land Disposal of Municipal Effluents and
      Sludges, EPA-902/9-73-001, 1973.

182.  Sullivan, R. H., M. M. Conn, and  S. S. Baxter,  "Survey
      of  Facilities Using Land Application of Wastewater," U. S.
      Environmental Protection Agency,  Office of Water Programs
      Operations, EPA-430/9-73-006,  1973.

183.  Reed, Sherwood, et al, "Wastewater Management by Disposal
      on  the Land," U. S. Army Corps of Engineers, Cold Regions
      Research and Engineering Laboratory, Special Report 171,
      1972.

184.  Kardos, L. T., "A New Prospect: Preventing Eutrophication
      of  Our Lakes and Streams," Environment, Vol. 12, No. 2,
      March 1970.


                              299

-------
 The  use  and purpose of monitoring wells  should  be  better  un-
 derstood in the  region.   The  general  philosophy that moni-
 toring wells are protective devices should  be discouraged.
 Monitoring should be applied  when there  is  a need  to deter-
 mine the status  of ground-water quality  at  a particular lo-
 cation and to gain a perspective on long-term water quality
 at selected sites.   At new sites, where  a specific activity
 may  lead to contamination of  ground water,  monitoring wells
 should be used only to determine whether procedures designed
 to protect ground-water quality have  been successful.  The
 monitoring wells themselves should not be considered as a
 method of preserving ground-water quality.

 Existing Problems

 The  present approach toward existing  problems in most states
 of the study region is to attempt corrective action only  af-
 ter  a specific incident of ground-water  contamination has
 been discovered.  This  "brush-fire" approach is not suitable
 in a region where use of  ground water is increasing in im-
 portance.   Furthermore, only  a  very small percentage of the
 existing problems have been discovered to date.  Taking into
 account  the tens  of thousands of ground-water sources pres-
 ently in use,  there is the potential  threat to  the health of
 individuals in addition to the  threat of adverse effects  on
 industrial  and agricultural activities.

 Probably the most revealing aspect of this entire  investiga-
 tion  is  that significant  numbers  of cases of ground-water
 contamination  do  exist and have  been  documented for each  of
 the  sources  discussed in  SECTION VI.  The importance of this
 rather elementary finding is  that many of the activities
 causing  known  ground-water contamination cases are common
 throughout  the region.  Therefore, locating and evaluating
 additional  cases  should be of major concern to public agen-
 cies  charged with the responsibility  of protecting water
 quality.   For example, for every  landfill where pollutants
 have  been discovered leaching into the underlying  aquifer,
 there are hundreds  more located  in similar geologic settings
 and designed in the  same  manner,  but  for which no  ground-
water quality data  are available.  For every surface impound-
ment where  it has been shown  that pollutants are being added
to the ground-water  system, there are hundreds more being
operated, unmonitored, under  similar  conditions.

It is recommended that a major effort be directed, within
the financial resources available to  local, state  and feder-
al agencies, toward defining the  areal extent and  severity
of existing ground-water  contamination problems.   Research
is needed to find the most suitable methods for such inven-


                              302

-------
tories.  One possible method is the use of aerial photo-
graphic techniques, including remote sensing and multi-
spectral photography, to locate potential sources of contam-
ination such as salt piles and industrial waste lagoons.
Another is the compilation of data already available on the
locations of potential sources of contamination, such as
areas containing high densities of septic tanks and routes
of buried pipelines subject to leakage of toxic compounds.
Much of this information has already been collected for
other purposes.  A third method is evaluation of chemical
analyses of ground water already on file with public agen-
cies.  The success of this alternative would depend to a
great degree on the availability of more complete analyses
of water samples now collected from supply wells by public
agencies in the region.

Essential to such inventories are methods that can be used
to delineate the actual size and shape of contaminated
ground-water bodies and the characteristics of the pollu-
tants contained in an aquifer.  The drilling of test holes
is a standard technique used for gathering data on the  areal
extent of contaminated water zones and for collecting water
samples.  Wells will always be essential to such investiga-
tions, but drilling methods, details of design, and the
materials selected must be applicable  to the particular type
of problem involved.  A more scientific approach to present
practices of drilling and constructing wells used  for  data
collection and monitoring in cases of  ground-water contam-
ination  is needed.   Further research into the  application of
geophysical techniques is also warranted.  For example,
electrical resistivity has shown great promise for defining
the presence of highly saline water bodies under  certain
geologic and hydrologic conditions, as has the use of  differ-
ences  in ground-water temperature  for  mapping  the  affected
portion  of an  aquifer.

After  inventories  of ground-water  contamination problems are
underway, the  results can begin  to be  used to  warn against
use of certain aquifers or portions of aquifers for  specific
purposes.  Within  the legal  framework  under which  each state
must operate,  development or withdrawal  of  ground  water
could  be limited in affected  aquifer  zones.  It would  be the
task of  the proper public agency to determine  "critical
zones"  around  each known  significant  case of ground-water
contamination.   In each  "critical  zone",  ground-water  diver-
sion would  be  restricted  from the  standpoint of either the
quantity that  can  be pumped  or the purpose  for which it can
be  used. Wells  and other monitoring  techniques would aid in
determing when and how  to modify the  areal  extent of a
                              303

-------
Table 45.    RESTRICTIONS ON GROUND-WATER USE IN THE CRITICAL ZONES SHOWN
                                           ON FIGURE41.
Zone   Description
       Area in which water-table
       aquifer already contains
       pollutant or ground-water
       quality is threatened be-
       cause of proximity to con-
       taminated area.
Restrictions on use of
water-table aquifer

1.  No ground-water pumpage
    permitted except where poor
    quality water can be used
    safely for special purposes
    or the pollutant can be suc-
    cessfully removed by treat-
    ment.

2.  Ground-water quality
    monitored.
 Restrictions on use of
 shallowest artesian aquifer

 1.  Pumpage regulated so
    that head is maintained
    above water table;
    otherwise pumpoge not
    permitted.

 2.  Well construction strictly
    regulated  to guard
    against inter-aquifer ex-
   change of contaminated
    water.

 3.  Well-water quality
    periodically monitored.
       Area in which natural
       process such as adsorption,
       dispersion,  and ion ex-
       change will have reduced
       the concentration of the
       pollutant significantly but
       not to a level acceptable
       For potable  water supplies.
                                   3.
   Ground-water pumpage
   limited to prevent signifi-
   cant increase in rate of
   travel  of contaminated
   water.

   Ground-water use for pot-
   able water supplies not per-
   mitted unless pollutant can
   be successfully removed by
   treatment.

   Ground-water quality
   strictly monitored.
1.  Pumpage regulated so
    that head is maintained
    above the water table in
    Zone A but con be lower
    than water table within
    this zone.

2.  Well construction regu-
    lated.
       Area in which natural
       processes will have reduced
       the concentration of the
       pollutant to a level accept-
       able for potable water sup-
       plies.
                                   2.
   Ground-water pumpage
   limited to prevent signif-
   icant increase in rate of
   travel of contaminated
   water.

   Ground-water quality
   monitored.
Proposed ground-water users
warned that pumpoge may
be restricted in the future
if ground-water contamina-
tion spreads to Zone B.
                                             306

-------
dealing with such categories as extensive municipal land-
fills or application of highway deicing salts.   Specific
needs for research, regulation and monitoring of these and
other sources are discussed later in this section.

Meanwhile, basic research is needed on how to cope with
those cases in which pollutants in the ground-water system
must be removed.  This condition could present itself if no
other alternative is reasonably available for replacement of
threatened well supplies, or if pollutants being discharged
from a ground-water source are contaminating a stream essen-
tial for water supply and recreational use.  The present pol-
icy of most states in the region is to require that a pollu-
tant be removed from an aquifer and that water quality be re-
stored to its baseline conditions.  However, such a policy
breaks down because present methods available for removal
and even containment of a pollutant are technically too dif-
ficult to apply and too costly to implement effectively.

Prevention of Additional Problems

Equally as pressing as the need to develop methods and  strat-
egies for dealing with existing problems of ground-water con-
tamination is the need to establish ways to prevent future
problems.  Each of the 11 states in the study region  already
appears to have legislation which, although general in  na-
ture, would allow regulations  and policies to be  formulated
and enforced for the prevention of ground-water quality deg-
radation.  Also, as pointed out in the previous section of
this report, many  codes in various states have been adopted
to cover  specific  activities  that can  lead to ground-water
contamination,  such as those  dealing with  landfill siting,
well construction, and sealing of surface  impoundments.   In
addition, such  broad approaches as New York State's classi-
fication  of ground waters have been attempted as  a means for
preventing  "pollution of ground waters",  l)

Nevertheless, there has not been  an overall evaluation  of
the various options available to  regulatory agencies  for
protecting  ground-water quality.   Such alternatives for con-
trol as  the setting of ground-water standards,  enforcement
of land-use restrictions in critical  areas,  imposition  of
restraints  on each individual type  of  activity  that can lead
to ground-water contamination, and  regulation of  patterns  of
ground-water use  should be  explored.   Obviously,  the  choice
of any  control  method must  be influenced by  geologic  and
hydrologic  conditions  in the  area of  interest and must take
into consideration the  type of activity  involved. Further-
more,  any regulation,  code, or policy  must be tested  against
the  following  considerations:
                              307

-------
 3.  Greater enforcement  of proper  construction and installa-
    tion practices.

 4.  Enforcement of bans  on discharge of hazardous wastes to
    septic-tank systems  at industrial  sites.

 Buried Pipelines and Storage Tanks

 1.  Codes and regulations calling  for  consideration of fac-
    tors involving design and management of proposed major
    pipelines carrying organic and inorganic pollutants as
    related to possible  effects of leaks on underlying aqui-
    fers.

 2.  Consideration/ in special cases of high risk to potable
    water supplies, of the use of  liners in excavations con-
    taining buried pipelines and storage tanks.

 3.  More efficient monitoring of potential fluid losses, and
    regulations calling  for the reporting of tank and pipe-
    line failures.

 4.  Additional research  into methods for removing hydrocar-
    bons from unconsolidated and rock aquifers.

 5.  Additional research  into the overall effects of leaky
    sanitary and storm sewers on ground-water quality.

Application and Storage  of Highway Deicing Salts

 1.  Greater effort to reduce wastage of salt by means of
    equipment modification and education of those involved
    in salt spreading.

2.  Additional research  to better determine the role that
    highway deicing salts play in the degradation of water
    quality in the various aquifers of the region.

3.  Consideration of aquifer susceptibility to contamination
    in the design of highway drainage systems.

4.  Guidelines governing the siting, construction, and over-
    all protection of water wells located in close proximity
    to existing and proposed major highways.

5.  Research into the significance of naturally occurring
    and artificially added trace elements in highway deicing
    salts.

6.  Protection of ground water from salt-storage areas.


                             310

-------
Landfills

1.  Inventories of industrial and municipal landfills.

2.  Increased monitoring of ground-water quality in the vi-
    cinity of landfills.

3.  Additional research on:  the character of leachate from
    landfills;  the ability of underlying natural soils to
    reduce the concentrations of different types of leach-
    ate;  the effects of various types of cover material,
    slopes/ and other landfill operational procedures on
    rainfall infiltration rates.

4.  Additional research into the use and composition of clay
    and synthetic liners, methods of leachate collection,
    and processes for the treatment of leachate.

5.  Development of procedures for completing landfills to
    minimize the continued production of leachate after
    waste disposal operations have ended.

6.  Enforcement of regulations prohibiting disposal of toxic
    wastes in  landfills.

7.  Review of  existing  guidelines governing the  siting and
    design of  new landfills.

Surface  Impoundments

1.  Development of guidelines and procedures for the  siting
    and  design of proposed surface impoundments.

2.  Research  into the need for and design  of artificial
    liners for surface  impoundments containing various types
    of  organic and inorganic pollutants.

3.  Inventories of existing  surface impoundments,  chemicals
    and wastes being stored, and design  and operation of
    these  systems,

4.  Increased monitoring of  ground-water quality in  the  vi-
    cinity of surface  impoundments and monitoring  of losses
    of  liquids to the  ground-water system  from surface im-
    poundments .

5.  Evaluation of the  use of surface  impoundments  as a means
    of  treatment  of municipal  and industrial wastes  in the
    northeast versus their potential  for causing ground-
    water quality degradation.
                              311

-------
    used or proposed,

7.  Evaluation of guidelines presently being used to control
    site selection and the type of waste tolerated where mu-
    nicipal and industrial effluent is applied to the land.

Water Wells

1.  More uniform and effective controls over well construc-
    tion practices and the siting of wells.

2.  More effective control over the fate of abandoned wells.

Agricultural Activities

1.  Research into the effects on ground-water quality of the
    application of fertilizers, herbicides, and insecticides
    in urban areas.

2.  Greater control over agricultural practices that lead to
    contamination of shallow aquifers tapped by domestic
    wells in rural areas.
                              314

-------
                REFERENCES CITED

                   SECTION VII
Division of Water Resources, "Classifications and Stan-
dards Governing the Quality and Purity of Waters of
New York State," New York State Department of Environ-
mental Conservation, Parts 700-703, Title 6, Official
Compilation of Codes, Rules and Regulations, April 1968,
                          315

-------
                        SECTION IX

              APPENDIX A - GLOSSARY OF TERMS
Alluvium - Clay, silt, sand, gravel, or other rock materials
transported by flowing water and deposited in comparatively
recent geologic time as sorted or semi-sorted sediments in
riverbeds, estuaries, flood plains, lakes, shores and in fans
at the base of mountain slopes.

Aquiclude  (Confining Bed) - A body of less permeable material
than the adjacent aquifer(s).

Aquifer - A geologic formation, group of formations, or part
of a formation that is water yielding.

Artesian - The occurrence of ground water under sufficient
pressure to rise above the upper surface of the aquifer.

Artesian Aquifer - An aquifer overlain by a confining bed and
containing water under artesian conditions.

Artificial Recharge - The addition of water to the ground-
water reservoir by activities of man, such as irrigation, or
spreading basins.

Base Flow - The fair-weather flow of streams, composed largely
of ground-water effluent.

Biochemical Oxygen Demand (BOD) - The quantity of oxygen util-
ized primarily in the biochemical oxidation of organic matter
in a specified time and at a specified temperature.  The time
and temperature are usually five days and 20°C.

Brackish Water - Water containing dissolved minerals in excess
of acceptable potable water standards, but less than that of
sea water.

Chemical Oxygen Demand (COD) - The measure of the readily
oxidizable material in water which provides an approximation
of the minimum amount of organic and reducing material present,

Chemical Water Quality - The nature of water as determined by
the concentration of chemical constituents.

Clastic - Consisting of fragments of rocks or organic struc-
tures that have been moved individually from their places of
origin.

                              318

-------
Concentration - The weight of solute dissolved in a unit volume
of solution.

Connate Water - Water that was deposited simultaneously with
the sediments, and has not since then existed as surface water
or as atmospheric moisture.

Consumptive Use - The quantity of water discharged to the atmos-
phere or incorporated in the products of vegetative growth or
industrial processes.

Contamination - The degradation of natural water quality as a
result of man's activities, to the extent that its usefulness
is impaired.

Crystalline - Rock composed of crystals or fragments of crystals.

Degradable - Capable of being decomposed, deteriorated, or de-
cayed into simpler forms with characteristics different from
the original.  Also referred to as biodegradable.

Degradation of Water Quality - The act or process of reducing
the level of water quality so as to impair its original use-
fulness.

Demineralization - The process of reducing the concentration of
chemical constituents.

Domestic Well - A well which supplies water  for the occupants
of a single residence.

Drawdown - The lowering of the water table or peizometric  surface
caused by pumping or artesian flow.

Evapotranspiration - The combined processes  of evaporation  from
land, water, and other surfaces, and transpiration by plants.

Fall Line - A line joining the waterfalls on a number of suc-
cessive rivers that marks  the point where each river descends
from the upland  (Piedmont) to the lowland  (Coastal Plain).

Flood Plain - The flat ground along a stream course which  is
covered by water at  flood  stage.

Fluvial Sediment - Those deposits produced by stream or  river
action  (see Alluvium).

Glacial Drift - Boulders,  till, gravel,  sand  or clay transported
by a glacier or its meltwater.


                               319

-------
 Porosity  -  The relative volume of  the pore spaces between
 mineral grains in a rock as compared to the total rock volume.

 Primary Treatment  (Sewage) - The removal of larger solids by
 screening,  and of more finely divided solids by sedimentation.

 Production  Well  - A well from which ground water is obtained.

 Public Supply Well - A well from which ground water is ob-
 tained serving more than one individual or household.

 Recharge  Basin - A basin designed  for the purpose of adding
 water to  the ground-water reservoir.

 Salt-Water  Intrusion  (or Encroachment) - Movement of salty
 ground water so  that it replaces fresh ground water.

 Saturation, Zone of - The zone in which interconnected inter-
 stices are  saturated with water under pressure equal to or
 greater than atmosphere.

 Secondary Treatment - The oxidation of organic matter in sew-
 age through bacterial action.

 Sedimentary Rock - Rocks formed by the accumulation of sediment.

 Soft Water  - Water containing 60 mg/1 or less of hardness.

 Specific Capacity - The rate of discharge of water from a well
 divided by  the drawdown of the water level in it.  Properly
 stated, it  relates to the time of pumping.

 Storage (Aquifer) - The volume of water held in the interstices
 of the rock.

 Surface Water - That portion of water that appears on the land
 surface.

 Tertiary Treatment - Advanced waste treatment which removes
 additional  impurities which remain in the effluent after secon-
dary treatment.

 Transmissivity - The rate at which water is transmitted through
 a unit width of the aquifer under a unit hydraulic gradient.

 Unconsolidated Rocks - Uncemented or loosely coherent rocks.

Water Cycle - The complete cycle through which water passes;
water vapor in the atmosphere, liquid and solid as precipitation
 as part of surface and ground water and eventually back to
 atmospheric vapor.
                             322

-------
Water Quality - Pertaining to the chemical, physical and biolog-
ical constituents found in water and its suitability for a par-
ticular purpose.

Water Table - That surface in an unconfined water body at which
the pressure is atmospheric.  It is defined by the levels at
which water stands in wells that penetrate the water body just
far enough to hold standing water.

Water-Table Aquifer - An aquifer containing water under water-
table conditions.
                               323

-------
SELECTED WATER
RESOURCES ABSTRACTS
INPUT TRANSACTION FORM
                  W
       GROUND WATER CONTAMINATION IN THE
       NORTHEAST STATES
 David W. Miller, Frank A. Deluca, and Thomas L. Tessier
        Geraghty & Miller,  Incorporated
        Port Washington, New York 11050
                       68-01-0777
                                                                          (:d 6V:
                   • do n
      Environmental Protection Agency Report No. EPA-660/2-74-056, June 1974
    An evaluation of principal sources of ground-water contamination has been carried out in II
 northeast states, including all of New England, New York, New Jersey,  Pennsylvania, Maryland,
 and Delaware.  The findings of this study have been used to determine priorities for research into
 ways to correct existing sources of contamination and to point out deficiencies in present control
 methods for protection against further degradation of ground-water quality.  Principal sources of
 ground-water quality degradation caused by man's activities that are common  to most parts of the
 region are septic tanks and cesspools, buried tanks and pipelines including sanitary and storm
 sewers,  the application and storage of highway deicing salts, municipal and industrial  landfills
 of solid  waste, unlined surface impoundments,  spills, and the uncontrolled discharge of pollutants
 on the land surface.  In New York and Pennsylvania,  mining and petroleum exploration and de-
 velopment have caused many instances of ground-water contamination, but the extent of the
 problem has not been defined.  Salt-water intrusion in coastal areas has been  adequately controlled,
 but little is known of the  potential threat to fresh-water aquifers from  the encroachment of saline
 water that naturally occurs  in inland formations underlying the western portions of the region.
    *Ground water,  *water pollution, *landfills, *septic tanks, *waste storage
      Northeast United States, Connecticut, Delaware, Maine, Maryland, Massachusetts,
      New Hampshire, New Jersey, New York, Pennsylvania, Rhode Island, and Vermont.
                                   • ov.,*;,,
                                                        Send To:
                                                        WATER RESOURCES SCIENTIFIC INFORMATION CENTER
                                                        US DEPARTMENT OF THE INTERIOR
                                                        WASHINGTON.D C. 2024O
          Marion R. Scalf
R.S. Kerr Environmental Research Laboratory

-------