United States Environmental Protection Agency Eastern Environmental Radiation Facility P.O. Box 3009 Montgomery, AL 36109 EPA 520/5-83-028 September 1983 Radiation SEPA Environmental Radiation Data Report 34 (April-June 1983) ------- ENVIRONMENTAL RADIATION DATA REPORT 34 April - June 1983 UNITED STATES ENVIRONMENTAL PROTECTION AGENCY Office of Radiation Programs ------- Preface Environmental Radiation D_ata (ERD) is compiled and distributed quarterlyby the Office of Radiation Programs' Eastern Environmental Radiation Facility (EERF), Montgomery, Alabama. Data from the Environmental Radiation Ambient Monitoring System (ERAMS), and similar networks operated by contributing States, Canada, Mexico, and the Pan American Health Organization are reported in (ERD) when available. ERAMS was established in 1973 by the U. S. Environmental Protection Agency's Office of Radiation Programs (ORP). The ERAMS is comprised of nationwide sampling stations that provide air, surface, and drinking water and milk samples from which environmental radiation levels are derived. The major emphasis for ERAMS is toward identifying trends in the accumulation of long-lived radionuclides in the environment. 1. Sampling locations are selected to provide optimal population coverage while functioning to monitor fallout from nuclear devices and other forms of radioactive contamination of the environment. 2. The radiation analyses performed on these samples include gross alpha and gross beta levels, gamma analyses for fission products and specific analyses for uranium, plutonium, strontium, iodine, radium, krypton and tritium. This monitoring effort also serves to provide ancillary information on releases into the environment from stationary sources such as nuclear power reactors, fuel fabrication and reprocessing plants and natural background levels. ------- ENVIRONMENTAL RADIATION DATA CONTENTS Page DATA - Reporting Rationale and Procedures - Table of Reporting Increments and Minimum Detectable Levels DATA - ERAMS SECTION I. Air Program 1 1. Airborne Particulates 1 and Precipitation 2. Plutonium and Uranium in 10 Airborne Particulates and Precipitation 3. Krypton-85 12 SECTION II. Water Program 13 1. Surface Water 13 2. Drinking Water 16 3. Radon in Drinking Water 19 SECTION III. External Gamma Ambient Monitoring Program 37 ------- SECTION IV. Milk Program 40 1. Pasteurized Milk 40 2. Tritium in Milk 40 3. Carbon-14 in Milk 48 DATA - STATE AGENCIES 49 1. Indiana Pasteurized Milk Program 49 2. Iowa Water Analysis and Milk Analysis 50 1 1 ------- DATA - Reporting Rationale and Procedures The intent of EPA's Office of Radiation Programs in establishing the Environmental Radiation Ambient Monitoring System was to provide continuous, accurate and usable environmental radiation data for the public. Therefore, new data reporting procedures were developed to allow better interpretation of the data. The most significant change in this reporting procedure is that all specific radionuclide analyses will be reported as the counting results indicate, whether the number is negative, zero, or positive. Reporting Rat_ipnale_ Frequently, concentrations of a radionuclide in environmental media are close to zero. When the actual concentration of a nuclide is zero, the net counting results should statistically show a distribution of negative and positive numbers about zero. This occurs when the background count is subtracted from a sample which has only background activity. Prior to July 1975, ERAMS data were not reported numerically when the results were less than a specified reporting level or minimum detectable level. The present reporting procedure allows all the data to be reported and evaluated statistically without an arbitrary cutoff of small or negative numbers. This approach will facilitate estimates of bias in the nuclide analyses and will allow better evaluation of distributions and trends in environmental data. When reviewing the data in this report, caution should be exercised in the interpretation of individual negative values. Obviously, a negative activity value does not have physical significance. Such numbers, however, are significant when taken together with other observations which indicate that the true value of a distribution is near zero. When an average of several measurements produces a result less than zero, this indicates a negative bias in the measurement procedure. (1) Reported Values Specific Analyses - All specific radionuclide analyses will be reported as the counting results indicate, whether the number is negative, zero, or positive. Numerical values given are as of sample collection date. Gross Analyses - The actual value of gross radioactivity measurements will be reported, unless the value is below the minimum detectable level (MDL) at the 2 sigma confidence level, then < minimum detectable level will be reported. i i i ------- MDL is defined as the 3 sigma error of the background. A tabulation of MDL's is given in the following table. (2) Reported Ejrrpr Terms Each reported value for specific analyses will be accompanied by a counting error term at the 2 sigma (95%) confidence interval. Potassium concentrations are determined by specific activity analyses. Error terms are therefore reported as counting errors. At the very low levels characteristic of most ERAMS measurements, counting error is the greatest contributor to overall error. (3) Significant P_igures_ All reported values will be rounded to no more than three significant figures. The last significant figure will be increased by one if the figure following is five or greater, otherwise it is left unchanged. (4) Reporting levels The reporting units, smallest increments for reporting, and minimum detectable levels for each isotope are shown in table 1. Smallest increments are sometimes considerably smaller than minimum detectable amounts to avoid truncation errors in averaging. (5) Averages Averages will be calculated along with appropriate error terms in an annual summary and analysis of ERAMS data. In calculating these averages, all values of individual data including negative numbers will be utilized. Averages will not be included in ERD quarterly reports. 1 V ------- TABLE 1 ERAMS Reporting Increments and Minimum Detectable Levels for Radlonuclide Analyses Radlonuclide Gross alpha Gross beta Tritium Carbon-14 Krypton-85 Plutoniura-238, 239 Uranium-234, 235,238 Radium-226 Strontium-90 Media Water Air Water Precipitation Water Milk Milk Ambient Air Air Milk Water Air Milk Water Water Milk Water Reporting Units pCl/1 pCl/m3 pCi/1 nCi/m2 nCi/1 nCi/1 pCi/1 pCi/m3 aCi/m3 pCi/1 pCi/1 aCi/m3 pCi/1 pCi/1 pCi/1 pCi/1 pCi/1 Reporting Increments 1 pCi/1 .01 pCi/m3 1 pCi/1 .01 nCi/m2 .1 nCi/1 .1 nCi/1 1 pCi/1 .1 pCi/m3 .1 aCi/m3 .001 PCi/l .001 pCi/1 .1 aCi/m3 .001 pCi/1 .001 pCi/1 .1 pCi/1 .1 pCi/1 .1 pCi/1 Minimum Detectable Levels 2 pCi/1 .01 pCi/m3 1 pCi/1 .01 nCi/m2(a) .2 nCi/1 .2 nCi/1 15 pCi/1 2 pCi/m3 .015 pCi(b> per sample .015 pCi per sample .015 PC1 per sample .015 PCi(b) per sample .015 pCi per sample .015 pCi per sample .1 pCi/1 1 pCi/1 1 pCi/1 ------- Radlonuclide Strontium-89 Iodine-131 Iodine-129 Iodine-127 Cesium-137 Barium-140 Potassium Potassium~40 Media Milk Milk Water Water (specific Milk Milk Milk Water Milk Water Milk Water Water Reporting Units pCi/1 pCi/1 pCi/1 pCi/1 radiochemical fCi/1 8/1 pCi/1 pCi/1 pCi/1 pCi/i g/1 g/1 pCi/1 Reporting Increments 1 pCi/1 1 pCi/1 1 pCi/1 .1 pCi/1 analysis) .1 fCi/1 10 g/1 1 pCi/1 1 pCi/1 1 pCi/1 1 pCi/1 .1 g/1 •1 8/1 1 pCi/1 Minimum Detectable Levels 5 pCi/l(c) 10 pCi/l(c) 10 PCi/l(c) .4 pCi/1 .4 fCi/1 10 g/1 10 pCi/1 10 pCi/1 10 pCi/l(c) 10 pCi/l(c) •12 g/1 .12 g/1 100 pCi/1 (a) The value in terms of nCi/m^ would be dependent on precipitation (mm) (b) This value in terms of pCi/m3 would be dependent on the air volume. (c) Activity as of the day of counting. ------- DATA - EPA ENVIRONMENTAL RADIATION AMBIENT MONITORING SYSTEM (ERAMS) SECTION I. Air Program Airborne Particulates and P re eip itat i on Gross beta radioactivity measurements and certain specific analyses are performed on air particulates and precipitation samples as indicator measurements in assessing the general (national) impact of all contributing sources on environmental levels of radiation. Airborne particulates are collected continuously at field stations representing wide geographic coverage, including present and potential sources of environmental radioactivity. Sampling sites are located throughout-the United States, Virgin Islands, and the Panama Canal. Filters ( 10-cm diameter synthetic fiber ) from air samplers are changed twice weekly and field measurements are made with a G-M survey meter at 5 hours and 29 hours after collection to allow for radon and thoron daughter product decay. Field estimates are reported to appropriate EPA officials by telephone or mail depending on the activity levels found. The filters are sent to EERF for more sensitive analyses in a low background beta counter. Gamma scans are performed on all filters showing laboratory gross beta counts greater than 1 pCi/tn^. The lower gross beta values reported for laboratory measurements are largely due to the decay of radionuclides which occurred between the times of the field estimates and laboratory measurements. Precipitation samples are collected at the field stations where air filters are collected. These samples are also sent to EERF where they are composited monthly for tritium, gross beta activity measurements and gamma scans. These locations also correspond to airborne particulate and drinking water sampling locations selected for plutonium analyses. Plutonium-238, -239, and uranium-234, -235, and -238 analyses are performed annually on precipitation samples collected during March - May. ------- Tables 2-4 present the monthly average gross beta concentrations in airborne participates for April - June 1983. Tables 5-7 present the monthly average gross beta concentration in precipitation April - June 1983. The tritium in precipitation samples for April - June 1983 at the selected stations are shown in Table 8. The specific gamma results will be published when they are available. A compilation of individual measurements is available from the EPA, EERF, Montgomery, AL 36193. ------- TABLE 2 AIRBORNE PARTICULATES GROSS BETA CONCENTRATION APRIL 1983 5-HR FIELD ESTIMATE EERF LAB MEASUREMENT LOCATION # SAM MAX MIN AVG MAX MIN AVG (pCi/m3) (pCi/m3) AL:MONTGOMERY CA:BERKELEY CA:LOS ANGELES CO:DENVER CT:HARTFORD DE:WILMINGTON FL:MIAMI HI:HONOLULU IA:IOWA CITY ID-.BOISE ID:IDAHO FALLS IL:CHICAGO IN:INDIANAPOLIS ME:AUGUSTA MI :LANSING MN:MINNEAPOLIS MO .-JEFFERSON CITY MS:JACKSON ND:BISMARCK NH:CONCORD NJ:TRENTON NM:SANTA FE NV:LAS VEGAS NY:ALBANY NY:NIAGARA FALLS NY:SYRACUSE NY:YAPHANK OH:COLUMBUS OHtPAINESVILLE OR:PORTLAND PA:HARRISBURG PA PITTSBURGH RI:PROVIDENCE SC:BARNWELL SC:COLUMBIA SD:PIERRE TN:KNOXVILLE TN:NASHVILLE TX:AUSTIN UT.'SALT LAKE CITY VAiLYNCHBURG WA:SEATTLE WA:SPOKANE WI:MADISON WV:CHARLESTON MINIMUM DETECTABLE MINIMUM DETECTABLE 11 9 9 8 8 8 9 8 7 8 8 8 8 8 8 9 9 1 9 9 3 1 8 9 8 7 7 8 9 9 8 8 5 2 9 8 8 15 8 5 7 9 8 8 7 ,1MT ,IMI' 0.6 0.1 0.8 0.0 0.2 0.3 0.1 0.5 0.5 0.3 0.0 0.3 1.0 0.2 0.2 0.5 0.3 0.2 0.6 4.2 0.0 0.2 0.5 0.1 0.2 0.1 0.0 0.7 0.3 0.0 0.7 0.1 0.1 0.0 0.9 0.2 0.8 0.0 1.5 0.2 0.4 0.0 0.6 0.6 0.2 r FOR C FOR 0.1 0.0 0.0 0.0 0.0 0.0 0.0 0.0 0.1 0.1 0.0 0.0 0.1 0.0 0.0 O.I 0.1 0.2 0.0 0.6 0.0 0.2 0.1 0.0 0.1 0.0 0.0 0.1 0.0 0.0 0.1 0.0 0.1 0.0 0.1 0.0 0.1 0.0 0.5 0.1 0.1 0.0 0.1 0.0 0.0 FIELD 0.3 0.1 0.3 0.0 0.1 0.1 0.0 0.2 0.2 0.2 0.0 0.1 0.3 0.1 0.1 0.2 0.1 0.2 0.3 1.3 0.0 0.2 0.3 0.1 0.1 0.0 0.0 0.2 0.2 0.0 0.2 0.1 0.1 0.0 0.3 0.1 0.3 0.0 0.9 0.1 0.2 0.0 0.3 0.2 0.1 0,01 0.02 0.01 0.05 0.01 0.01 0.01 0.01 0.02 0.02 0.01 0.04 0.01 0.01 0.01 0.04 0.02 0.01 0.02 0.01 0.01 0.01 0.02 0.02 0.01 0.01 0.01 0.02 0.02 0.01 0.02 0.01 0.01 0.01 0.02 0.02 0.03 0.03 0.02 0.01 0.01 0.01 O.OL 0.02 0.02 ESTIMATES - LAB MEASUREMENT - 0.00 0.01 0.00 0.01 0.00 0.00 0.00 0.00 0.00 0.00 0.01 0.00 0.00 0.00 0.00 0.01 0.00 0.01 0.00 0.00 0.00 0.01 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.01 0.01 0,01 0.01 0.01 0.00 0.00 0.00 0.00 0.00 0.01 0.01 0.01 0.01 0.02 0.00 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.00 0.01 0.01 0.01 0.01 0.01 0.01 0.00 0.00 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.00 0.01 0.01 0.01 0.00 0.02 0.02 0.02 0.02 0.02 0.01 0.01 0.00 0.01 0.01 0.01 .1 pCi/m3, .01 pci/nr ------- TABLE 3 AIRBORNE PARTICULATES GROSS BETA CONCENTRATION MAY 1983 LOCATION AL: MONTGOMERY CA: BERKELEY CArLOS ANGELES CO rDENVER CT:HARTFORD DE:WILMINGTON FL:JACKSONVILLE FL:MIAMI HI:HONOLULU IA:IOWA CITY ID:BOISE ID:IDAHO FALLS IL:CHICAGO IN:INDIANAPOLIS ME :AUGUSTA MI:LANSING MN: MINNEAPOLIS MO:JEFFERSON CITY ND:BISMARCK NH:CONCORD NJ:TRENTON NV:LAS VEGAS NY:ALBANY NY:NIAGARA FALLS NY .-SYRACUSE NY:YAPHANK OH:COLUMBUS OH:PAINESVILLE OR:PORTLAND PA:HARRISBURG PA:PITTSBURGH RI:PROVIDENCE SC:BARNWELL SC:COLUMBIA SD:PIERRE TN:KNOXVILLE TN:NASHVILLE TX:AUSTIN UT:SALT LAKE CITY VAtLYNCHBURG WA:SEATTLE WA:SPOKANE WI .-MADISON WV:CHARLESTON WY:CHEYENNE 5-HR FIELD ESTIMATE Ul MAX MIN AVG (pCi/m3) 9 9 9 8 9 8 1 9 9 9 9 9 8 9 9 9 9 9 10 9 4 9 9 9 5 5 9 9 9 9 9 5 2 9 9 9 7 9 9 9 8 9 2 9 1 tMIl IMI1 1.0 0.1 0.5 0.0 0.1 0.2 0.1 0.0 0.1 0.9 0.2 0.0 1.4 0.3 0.2 0.2 0.3 0.3 1.1 2.9 0.3 0.4 0.1 0.2 0.0 0.0 0.3 0.3 0.1 0.3 0.0 0.1 0.0 0.4 0.2 0.7 0.0 1.4 0.2 0.3 0.0 0.5 0.4 0.2 1.6 : FOR P FOR 0.1 0.0 0.2 0.0 0.0 0.0 0.1 0.0 0.0 0.1 0.1 0.0 0.0 0.2 0.0 0.0 0.0 0.1 0.0 0.3 0.0 0.1 0.1 0.1 0.0 0.0 0.1 0.1 0.0 0.1 0.0 0.0 0.0 0.1 0.0 0.1 0.0 0.2 0.0 0.1 0.0 0.2 0.2 0.0 1.6 FIELD 0.5 0.1 0.3 0.0 0.1 0.1 0.1 0.0 0.0 0.4 0.1 0.0 0.3 0.2 0.1 0.1 0.2 0.2 0.6 0.9 0.1 0.2 0.1 0.1 0.0 0.0 0.2 0.1 0.0 0.2 0.0 0.0 0.0 0.2 0.1 0.4 0.0 0.8 0.1 0.2 0.0 0.3 0.3 0.1 1.6 EERF LAB MEASUREMENT MAX MIN AVG (pCi/m3) 0.01 0.01 0.01 0.02 0.01 0.01 0.01 0.01 0.01 0.03 0.01 0.01 0.01 0.01 0.01 0.01 0.03 0.02 0.03 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.02 0.01 0.01 0.01 0.02 0.03 0.02 0.05 0.02 0.09 0.01 0.01 0.03 0.01 0.03 0.03 ESTIMATES - LAB MEASUREMENT - 0.00 0.00 0.00 0.01 0.00 0.00 0.01 0.00 o.oo 0.01 0.00 0.01 0.00 0.00 0.00 0.00 0.01 0.00 0.00 0.00 0.00 0.01 0.00 0.00 0.01 0.00 0.01 0.01 0.00 0.01 0.01 0.00 0.00 0.00 0.01 0.01 0.00 0.01 0.01 0.01 0.00 0.00 0.01 0.01 0.02 0.01 0.01 0.01 0.01 0.00 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.02 0.00 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.00 0.01 0.01 0.01 0.00 0.01 0.01 0.01 0.02 0.01 0.02 0.01 0.00 0.01 0.01 0.01 0.02 .1 pCl/m3 .01 pCl/m3 ------- TABLE 4 LOCATION AIRBORNE PARTICIPATES GROSS BETA CONCENTRATION JUNE 1983 5-HR FIELD ESTIMATE EERF LAB MEASUREMENT // SAM MAX MIN AVG MAX MIN AVG (pCi/m3) (pCi/m3) 14 8 8 7 8 8 8 8 9 .8 6 7 8 8 2 9 9 8 8 3 8 8 5 9 8 8 5 8 8 8 3 5 3 8 7 8 3 8 3 8 5 7 8 8 8 7 1.3 0.1 0.6 0.0 0.3 0.6 0.3 0.0 0.2 1.4 0.3 0.0 0.9 0.9 0.9 0.4 0.3 0.3 1.7 0.2 0.4 4,1 0.3 0.5 0.3 0.5 0.1 0.0 0.9 0.5 0.4 0.7 0.0 1.5 0.3 0.2 0.1 1.5 0.2 1.1 1.2 0.3 1.0 0.0 0.4 0.2 0.1 0.0 0.2 0.0 0.1 0.1 0.0 0.0 0.0 0.4 0.1 0.0 0.2 0.3 0.2 0.1 0.1 0.0 0.2 0.1 0.1 1.2 0.0 0.1 0.0 0.1 0.0 0.0 0.2 0.2 0.2 0.3 0.0 0.2 0.1 0.1 0.0 0.1 0.0 0.2 0.2 0.1 0.1 0.0 0.1 0.0 0.4 0.0 0.3 0.0 0.2 0.3 0.1 0.0 0.1 0.8 0.2 0.0 0.5 0.6 0.6 0.2 0.2 0.2 0.5 0.2 0.3 2.5 0.1 0.3 0.2 0.2 0.0 0.0 0.4 OV3 0.3 0.5 0.0 0.6 0.2 0.2 0.1 0.6 0.1 0.7 0.8 0.2 0.6 0.0 0.2 0.1 0.01 0.01 0.01 0.03 0.02 0.02 0.01 0.01 0.03 0.03 0.01 0.02 0.02 0.03 0.01 0.01 0.02 0.04 0.03 0.01 0.02 0.01 0.01 0.03 0.02 0.02 0.02 0.01 0.03 0.02 0.01 0.03 0.01 0.03 0.02 0.02 0.01 0.02 0.02 0.03 0.03 0.01 0.01 0.01 0.01 0.02 0.00 0.00 0.01 0.01 0.00 0.00 0.00 0.00 0.00 0.01 0.00 0.00 0.01 0.00 0.00 0.01 0.00 0.00 0.01 0.00 0.01 0.01 o.oo b.oi 0.01 0.01 0.01 0.00 0.01 0.01 0.01 0.01 0.00 0.01 0.01 0.01 0.01 0.01 0.00 0.02 0.01 0.00 0.00 0.00 0.00 0.01 0.01 0.00 0.01 0.02 0.01 0.01 0.01 0.00 0.01 0.02 0.01 0.01 0.01 0.01 0.00 0.01 0.01 0.01 0.02 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.01 0.02 0.01 0.01 0.02 0.01 0.01 0.01 0.01 0.01 0.02 0.01 0.02 0.02 0.01 0.01 0.00 0.01 0.01 AL:MONTGOMERY CA:BERKELEY CA:LOS ANGELES CO'.DENVER CT:HARTFORD DEtWILMINGTON FL:JACKSONVILLE FL:MIAMI HI-.HONOLULU IA:IOWA CITY ID:BOISE ID:IDAHO FALLS IL:CHICAGO IN:INDIANAPOLIS KS:TOPEKA ME :AUGUSTA MI: LANSING MN:MINNEAPOLIS MO:JEFFERSON CITY MS:JACKSON ND:BISMARCK NH:CONCORD NJ:TRENTON NV-.LAS VEGAS NY:ALBANY NY:NIAGARA FALLS NY SYRACUSE NY:YAPHANK OH:COLUMBUS OH:PAINESVILLE OH:TOLEDO OK:OKLAHOMA CITY OR PORTLAND PA:HARRISBURG PA PITTSBURGH RI:PROVIDENCE SCtBARNWELL SC:COLUMBIA SD:PIERRE TN:KNOXVILLE TX:AUSTIN UTrSALT LAKE CITY VA:LYNCHBURG WA:SEATTLE WA:SPOKANE WV:CHARLESTON MINIMUM DETECTABLE LIMIT FOR FIELD ESTIMATES - .1 r MINIMUM DETECTABLE LIMIT FOR LAB MEASUREMENT - .01 pCi/mJ 5 ------- TABLE 5 GROSS BETA CONCENTRATION IN PRECIPITATION APRIL 1983 LOCATION AL:MONTGOMERY CA: BERKELEY COrDENVER CT:HARTFORD ID:BOISE ID:IDAHO FALLS IL:CHICAGO IN'.INDIANAPOLIS MI:LANSING MS:JACKSON NJ:TRENTON NV:LAS VEGAS NY:NEW YORK CITY NY:NIAGARA FALLS OH-.COLUMBUS OH:PAINESVILLE OR .'PORTLAND PA .'HARRISBURG SC:BARNWELL SC:COLUMBIA VA:LYNCHBURG DEPTH (mm) 270.0 88.1 37.8 246.3 24.8 21.8 67.9 25.0 111.8 311.8 60.0 3.7 60.0 136.0 116.3 83.8 108.3 108.0 82.5 162.5 177.2 ACT. ± 2s (nCi/m2) 0.15 0.09 0.05 0.37 0.10 0.03 0.06 0.02 0.12 0.11 0.10 0.01 0.12 0.13 0.06 0.13 0.17 0.04 0.21 0.27 0.11 0.12 0.04 0.02 0.14 0.02 0.01 0.03 0.01 0.05 0.12 0.03 0.00 0.04 0.06 0.05 0.05 0.06 0.04 0.05 0.08 0.08 SPECIFIC GAMMA ACT. (pCi/1) ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND NO GAMMA ACTIVITY DETECTABLE s SIGMA COUNTING ERROR ------- TABLE 6 GROSS BETA CONCENTRATION IN PRECIPITATION MAY 1983 LOCATION AL: MONTGOMERY CA:BERKELEY CO:DENVER CT:HARTFORD FL:JACKSONVILLE ID:BOISE IL:CHICAGO IN .-INDIANAPOLIS MI:LANSING MN.-MINNEAPOLIS MS:JACKSON ND: BISMARCK NJ:TRENTON NY:NEW YORK CITY NY:NIAGARA FALLS OH:COLUMBUS OH.-PAINESVILLE OH:TOLEDO OR:PORTLAND PA:HARRISBURG PA:PITTSBURGH SC: BARN WELL SC:COLUMBIA TX:AUSTIN WV:CHARLESTON DEPTH ACT. + 2s (mm) (nCi/m2) SPECIFIC GAMMA ACT. (pCi/1) 123.8 26.5 59.8 151.3 81.2 63.4 130.2 72.5 176.8 53.8 249.6 33.4 41.3 58.6 79.2 225.6 150.6 40.0 32.3 98.3 89.5 40.0 31.2 40.0 71.7 0.44 0.01 0.09 0.35 0.14 0.06 0.18 0.06 0.15 0.13 0.29 0.04 0.08 0.15 0.05 0.08 0.09 0.04 0.04 0.13 0.12 0.04 0.06 0.02 0.09 0.08 0.01 0.03 0.09 0.04 0.03 0.07 0.03 0.08 0.03 0.12 0.02 0.02 0.04 0.03 0.09 0.06 0.02 0.02 0.05 0.04 0.02 0.02 0.02 0.03 ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND NO GAMMA ACTIVITY DETECTABLE s SIGMA COUNTING ERROR ------- TABLE 7 GROSS BETA CONCENTRATION IN PRECIPITATION JUNE 1983 LOCATION AL: MONTGOMERY CO:DENVER CT:HARTFORD FL:JACKSONVILLE ID:IDAHO FALLS IL:CHICAGO IN:INDIANAPOLIS MI:LANSING MN: MINNEAPOLIS MS:JACKSON ND:BISMARCK NJ:TRENTON NY:NEW YORK CITY NY:NIAGARA FALLS OH .'COLUMBUS OH:PAINESVILLE OH:TOLEDO OK:OKLAHOMA CITY OR:PORTLAND PA:HARRISBURG PA .-PITTS BURGH SC:BARNWELL SC:COLUMBIA TX:AUSTIN WV:CHARLESTON DEPTH (mm) 115.0 23.5 75.0 130.6 24.0 29.6 22.5 107.5 417.5 86.8 40.8 25.3 20.0 346.2 99.0 66.3 35.0 36.5 103.7 37.3 75.3 130.0 20.0 42.5 35.1 ACT. ± 2s (nCi/m2) 0.17 0.03 0.36 0.08 0.03 0.03 0.05 0.09 0.56 0.07 0.02 0.05 0.02 0.44 0.11 0.06 0.03 0.05 0.17 0.02 0.17 0.12 0.02 0.03 0.04 0.06 0.01 0.05 0.06 0.01 0.01 0.01 0.05 0.23 0.04 0.02 0.01 0.01 0.17 0.05 0.03 0.02 0.02 0.06 0.02 0.05 0.07 0.01 0.02 0.02 SPECIFIC GAMMA ACT. (pCl/1) ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND NO GAMMA ACTIVITY DETECTABLE s SIGMA COUNTING ERROR 8 ------- TABLE 8 PRECIPITATION TRITIUM CONCENTRATION LOCATION AL:MONTGOMERY CA:BERKELEY CO:DENVER CT:HARTFORD FL:JACKSONVILLE ID:BOISE ID:IDAHO FALLS IL:CHICAGO IN:INDIANAPOLIS MI:LANSING MN:MINNEAPOLIS MS:JACKSON ND:BISMARCK NJ: TRENTON NV.-LAS VEGAS NY:NEW YORK CITY NY:NIAGARA FALLS OH:COLUMBUS OH:PAINESVILLE OH:TOLEDO OK:OKLAHOMA CITY OR:PORTLAND PArHARRISBURG PA .'PITTSBURGH SC:BARNWELL SC:COLUMBIA TX:AUSTIN VArLYNCHBURG WV:CHARLESTON APRIL - JUNE APRIL nCi/1 + 2s 0.2 0.2 0.1 0.2 0.3 0.2 0.1 0.2 NS 0.2 0.2 0.3 0.2 0.2 0.2 0.1 0.2 0.3 0.2 NS 0.2 0.2 NS 0.2 0.2 0.1 0.2 0.1 0.2 0.2 0.2 0.1 0.2 0.3 0.2 NS NS 0.2 0.2 0.2 0.2 NS 3.1 0.2 0.4 0.2 NS 0.3 0.2 NS 1983 MAY nCl/1 + 2s 0.2 0.2 0.2 0.2 0.2 0.2 0.3 0.2 0.3 0.2 0.2 0.2 NS 0.2 0.2 0.2 0.2 0.2 0.2 0.3 0.2 0.1 0.2 0.3 0.2 0.3 0.2 NS 0.3 0.2 0.3 0.2 0.1 0.2 0.2 0.2 0.2 0.2 NS 0.2 0.2 0.4 0.2 0.3 0.2 0.9 0.2 0.2 0.2 0.2 0.2 NS 0.3 0.2 JUNE nCl/1 + 2s 0.1 NS 0.2 0.2 0.3 NS 0.3 0.2 0.2 0.3 0.2 0.1 0.1 0.2 NS 0.3 0.4 0.2 0.3 0.2 0.2 0.1 0.2 0.2 0.4 0.4 0.2 NS 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 NS NO SAMPLE s SIGMA COUNTING ERROR ------- Plutonium and Uranium i_n Airborne Particulates Environmental radiation levels of plutonium and uranium are determined by the analyses of quarterly composite samples (air filters) collected from the continuously operating airborne particulate samplers. The number of continuously operating stations is being increased from the original 22 will eventually number 67 when all equipment is operational. Analyses of the composited filters consist of ashing, separating by liquid ion exchange, and coprecipitation of the plutoniura or uranium. Concentration of the specific isotopes of plutonium-238, -239, and uranium-234, -235, and -238 are determined by alpha spectroscopy. The volume of air analyzed normally ranges from 25,000 to 40,000 m3 for each quarterly composite. Plutonium and uranium in airborne particulates data for January - March 1983 are shown for the 42 stations operating during this period in Table 9. 10 ------- TABLE 9 PLUTONIUM AND URANIUM IN AIRBORNE PARTICULATES JANUARY - MARCH 1983 COMPOSITES 238 Pu 239 Pu 234 U 235 U 238 U LOCATION AL: MONTGOMERY CA:BERKELEY CA:LOS ANGELES CO:DENVER CT:HARTFORD DE:WILMINGTON FLrMIAMI HI:HONOLULU IA:IOWA CITY ID:BOISE ID:IDAHO FALLS IL:CHICAGO ME:AUGUSTA MI:LANSING MN:MINNEAPOLIS MO:JEFFERSON CITY MS:JACKSON ND:BISMARCK NH:CONCORD NJ:TRENTON NM:SANTA FE NV:LAS VEGAS NY:ALBANY NY:NEW YORK CITY NY:NIAGARA FALLS NY:SYRACUSE NY:YAPHANK OH .-COLUMBUS OHrPAINESVILLE OR:PORTLAND PA .-HARRISBURG PA:PITTSBURGH RI:PROVIDENCE SC:BARNWELL SC:COLUMBIA SD:PIERRE TN:KNOXVILLE TN:NASHVILLE TX:AUSTIN VA.-LYNCHBURG WA:SEATTLE WA:SPOKANE WI:MADISON WV:CHARLESTON aCi/m3 0 0 -0 0 0 0 0 0 0 0 2 0 0 0 0 0 -0 1 0 0 0 3 0 0 0 0 0 0 0 1 0 2 0 1 0 0 0 -0 0 0 0 1 0 1 .2 .1 .4 .1 .8 .1 .7 .1 .7 .1 .5 .6 .9 .3 .0 .3 .1 .2 .1 .5 .2 .2 .7 .9 .4 .8 .1 .3 .6 .8 .0 .1 .3 .0 .3 .9 .3 .1 .2 .3 .4 .6 .4 .0 0 0 1 0 0 0 0 0 0 0 1 0 1 0 0 0 1 0 0 0 0 1 1 0 0 0 0 0 0 0 0 1 0 2 0 0 0 0 0 0 0 1 0 1 + 2s aCi/m3+ .6 .6 .0 .5 .5 .2 .6 .2 .6 .5 .3 .5 .1 .4 .5 .3 .8 .6 .3 .4 .6 .8 .2 .8 .5 .8 .6 .4 .5 .5 .8 .6 .5 .7 .5 .7 .6 .5 .4 .5 .7 .5 .3 .2 0 1 1 1 2 1 1 1 1 1 2 0 1 4 1 0 1 0 0 2 2 5, 1, 0, 0, 1, 0, 0, 1, 3, 0, 0, 0. 0. 0. 1. 3. 1. 0. 1. 0, 0. 1. 1. .9 .6 .3 .1 .2 .0 .7 .1 .2 .5 .2 .9 .0 .5 .0 .9 .7 .6 .6 .6 .1 .3 .2 .6 .4 .8 .7 .5 ,0 .3 .9 .7 ,9 ,7 ,9 ,5 ,1 ,1 ,9 ,2 ,4 ,8 ,1 6 0 0 0 0 0 0 0 0 0 0 1 0 0 1 0 0 1 0 0 1 0 2 0 0 0 0 0 0 0 1 0 0 0 1 0 0 1 0 0 0 0 0 0 0 .6 .8 .9 .6 .8 .4 .7 .7 .6 .6 .1 .5 .8 .2 .6 .4 .4 .5 .3 .0 .9 .0 .9 .8 .4 .8 .5 .3 .5 .4 .6 .7 .7 .4 .5 .8 .0 .6 .5 .6 .3 .7 .5 .9 aCl/ 5.9 4.9 15.6 42.0 16.2 10.9 13.9 6.3 8.5 14.2 41.7 17.3 35.7 8.2 18.5 15.3 19.8 60.3 11.1 13.3 13.6 94.8 44.0 29.8 51.3 30.0 6.5 27.3 27.8 17.6 27.0 57.2 13.3 8.7 22.1 16.4 61.6 24.0 11.7 234.7 5.7 25.7 12.1 49.3 m3+ 2s 1.6 1.8 2.5 5.4 2.8. 1.9 2.7 1.8 1.8 2.5 7.4 3.4 5.8 1.8 3.1 2.6 5.0 8.9 1.9 2.9 3.2 13.0 6.5 5.6 8.1 5.2 1.7 6.6 4.9 3.6 4.2 8.9 1.8 3.7 3.0 3.5 8.3 4.1 2.2 23.9 1.5 5.4 2.3 8.2 aCi/m3+ 2s 0.5 0.4 0.1 0.5 1.3 0.6 1.5 0.7 0.5 0.4 0.8 0.4 0.5 0.5 0.8 0.6 0.8 0.5 0.7 0.5 1.3 1.2 1.0 0.6 1.7 1.0 0.4 0.3 1.0 0.6 0.5 0.4 1.2 1.1 1.6 0.9 1.2 0.5 0.5 0.4 3.1 1.4 5.9 2.2 2.8 1.3 1.4 1.0 2.9 1.3 1.8 1.0 0.6 0.5 1.0 0.9 0.5 0.5 0.9 0.7 0.9 0.6 4.0 1.7 0.5 0.4 0.0 0.0 1.6 0.6 0.3 0.4 10.1 2.3 0.9 0.6 0.5 0.4 7.2 1.4 0.7 0.5 0.4 0.8 0.3 0.4 0.4 0.5 aCi/ 4.8 4.9 14.4 45.7 15.8 10.3 8.9 7.0 13.7 11.3 42.6 12.6 30.6 9.5 18.5 13.0 9.7 57.3 9.8 12.1 13.3 47.4 33.9 22.0 45.8 24.0 7.4 28.3 28.3 15.8 27.8 53.2 14.9 7.2 19.0 14.8 45.9 20.1 9.2 10.8 6.9 28.0 11.5 32.8 m3+ 2 1.4 1.8 2.4 5.7 2.7 1.8 2.0 1.8 2.5 2.2 7.4 2.7 5.2 2.0 3.1 2.3 3.3 7.0 1.8 2.7 3.1 7.8 5.4 4.6 7.5 4.5 1.9 6.7 5.0 3.4 4.3 8.5 2.5 3.3 2.7 3.2 6.6 3.6 1.9 1.8 1.6 5.6 2.2 6.2 SIGMA COUNTING ERROR 11 ------- Krypton-85 Krypton-85 is a long-lived noble gas with a half life of 10.8 years. It is released into the atmosphere "by nuclear reactor operations, fuel fabrication, fuel reprocessing, and nuclear detonations. Krypton-85 also occurs naturally in minor quantities primarily from the neutron capture of stable krypton-84 as well as spontaneous fission and neutron-induced fission of uranium. Monitoring of krypton~85 in the atmosphere has been conducted to identify and establish baseline levels and long-term trends. Krypton-85 analysis began in January 1973 with sample collections and analyses being performed for 12 sampling locations. These locations were selected to provide atmospheric coverage of the United States with considerations being given to the proximity to fuel reprocessing plants, nuclear reactors, and wide geographic coverage. Dry compressed air samples, collected at each location, are purchased from commercial air suppliers annually and shipped to the EERF where the krypton-85 is cryogenically separated and counted in a liquid scintillation system. The Kr-85 results will be published when they are available. 12 ------- DATA - EPA ERAMS SECTION II. Water Program The ERAMS water program provides ambient radiation data to assess the effects of the nuclear power industry, the natural radiation environment, and other nuclear sources on the nation's rivers, streams and drinking water supplies. Surface Water Grab samples are taken quarterly at 58 stations located downstream from operating or future nuclear facilities. Surface water monitoring consists of tritium analyses quarterly and gamma scans annually. Tritium is the primary radioactive pollutant from nuclear power plants. Tritium concentrations are determined by liquid scintillation counting of distilled samples. Gamma scans are performed annually to determine if there is a buildup of other contaminants. Tritium concentrations for surface water samples for April - June 1983 are given in Table 10. 13 ------- TABLE 10 SURFACE WATER TRITIUM CONCENTRATION APRIL - JUNE 1983 LOCATION AL:DECATUR ALrDOTHAN ALrSCOTTSBORO CA:CLAY STATION CA:DIABLO CANYON CA:EUREKA CA:SAN ONOFRE CO:GREELEY CTrEAST HADDAM CTrWATERFORD FL:CRYSTAL RIVER FL:FT. PIERCE FLrHOMESTEAD IA:CEDAR RAPIDS ID:BUHL IL:E. MOLINE IL:MORRIS ILrOREGON IL:ZION LA:NEW ORLEANS MA:PLYMOUTH MA:ROWE MD:CONOWINGO MD:LUSBY ME:WISCASSET MI:BRIDGMAN MI:CHARLEVOIX MI:MONROE MI:SOUTH HAVEN MN:MONTICELLO MN:RED WING MS:PORT GIBSON NC:CHARLOTTE NC:SOUTHPORT NE:RULO NJ:BAYSIDE NJ:OYSTER CREEK NV:BOULDER CITY NY:OSSINING NYrOSWEGO NY:POUGHKEEPSIE OH:TOLEDO OR:BRADWOOD PA:DANVILLE SOURCE TENNESSEE RIVER CHATTAHOOCHIE RIVER TENNESSEE RIVER FOLSOM S. CANAL PACIFIC OCEAN HUMBOLDT BAY PACIFIC OCEAN SOUTH PLATTE RIVER CONNECTICUT RIVER LONG ISLAND SOUND GULF OF MEXICO ATLANTIC OCEAN BISCAYNE BAY CEDAR RIVER SNAKE RIVER MISSISSIPPI RIVER ILLINOIS RIVER ROCK RIVER LAKE MICHIGAN MISSISSIPPI RIVER CAPE CODE BAY DEERFIELD RIVER SUSQUEHANNA RIVER CHESAPEAKE BAY MONTSEWAY BAY LAKE MICHIGAN LAKE MICHIGAN LAKE ERIE LAKE MICHIGAN MISSISSIPPI RIVER MISSISSIPPI RIVER MISSISSIPPI RIVER CATAWBA RIVER ATLANTIC OCEAN MISSOURI RIVER DELAWARE RIVER OYSTER CREEK COLORADO RIVER HUDSON RIVER LAKE ONTARIO HUDSON RIVER LAKE ERIE COLUMBIA RIVER SUSQUEHANNA RIVER DATE COLLECTED 4/ 4/83 4/ 7/83 5/27/83 4/ 8/83 4/14/83 4/ 7/83 6/ 4/83 4/22/83 5/11/83 5/10/83 4/ 4/83 4/ 5/83 4/13/83 4/ 5/83 4/19/83 5/ 5/83 5/13/83 4/15/83 4/12/83 4/ 8/83 4/ 6/83 6/ 1/83 4/19/83 4/ 5/83 4/ 4/83 4/ 5/83 4/10/83 4/11/83 4/ 4/83 4/ 7/83 4/20/83 4/21/83 4/ 5/83 4/ 6/83 4/12/83 4/ 6/83 4/ 7/83 4/ 1/83 4/20/83 5/15/83 4/ 6/83 4/ 1/83 5/29/83 4/20/83 .1 .1 .2 .2 .1 .1 .1 .2 .1 nCi/1 0.2 0.1 0.3 0.1 0.2 0.1 0.2 0.2 0. 0. 0. 0. 0. 0. 0. 0. 0. 0.3 0.3 0.1 0.2 0.2 0.2 0.2 0.3 0.2 0.1 0.2 0.4 0.1 0.2 0.2 0.4 0.2 0.2 0.2 0.1 0.4 0.2 0.4 0.3 0.3 0.2 0.3 + 2s 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0. 0. 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 .2 .2 14 ------- LOCATION SCtALLENDALE SC:BROAD RIVER SC:HARTSVILLE TN: DAISY TN KINGSTON TX:EL PASO TXrMATAGORDA VTrVERNON WA:NORTHPORT WA:RICHLAND WI:VICTORY WVrWHEELING TABLE 10 (CONTINUED) SURFACE WATER TRITIUM CONCENTRATION APRIL - JUNE 1983 SOURCE SAVANNAH RIVER BROAD RIVER LAKE ROBINSON TENNESSEE RIVER CLINCH RIVER RIO GRANDE COLORADO RIVER CONNECTICUT RIVER COLUMBIA RIVER COLUMBIA RIVER MISSISSIPPI RIVER OHIO RIVER DATE COLLECTED 4/21/83 4/27/83 4/11/83 5/17/83 4/26/83 4/20/83 4/ 5/83 4/ 5/83 5/27/83 4/19/83 4/ 4/83 4/14/83 nCi/1 1.0 0.2 0.4 0.1 1.2 0.1 0.1 0.3 0.3 0.2 0.2 0.1 + 2s 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 s SIGMA COUNTING ERROR 15 ------- Drinking Water The drinking water program provides ambient radiation monitoring relevant to the effects of the nuclear power industry, natural environmental levels, and other pertinent sources. These data serve to assess trends and anomalies in concentrations, and to compare with standards set forth in the EPA "National Interim Primary Drinking Water Regulations." These regulations provide for approval of supplies when the combined radium-226 and radium-228 levels do not exceed 5 pCi/1, when the gross alpha (excluding radon and uranium) levels do not exceed 15 pCi/1, when tritium levels do not exceed 20,000 pCi/1, when the strontiura-90 levels do not exceed 8 pCi/1, and when the gross beta levels do not exceed 50 pCi/1. Grab samples are taken at 78 sites which are either major population centers or selected nuclear facility environs. The analyses include (a) tritium on a quarterly basis (b) gross alpha, gross beta, strontiura-90 and gamma on annual composites. Radium-226 analyses are performed if the gross alpha exceeds 2 pCi/1; and radium-228 analyses are performed if the radium-226 activity falls between 3 and 5 pCi/1) (c) specific iodine-131 is performed on one quarterly sample per year for each station (d) an annual composite for plutonium-238, -239, uranium-234, -235, -238, for stations which demonstrate gross alpha levels greater than 2 pCi/1. Tritium analyses are performed by scintillation counting of the distilled samples, gross beta, and gross alpha by evaporating an aliquot on stainless steel planchets for counting, and radiura-226 by the standard emanation technique. Strontium-90 is determined by beta counting a strontium carbonate precipitate isolated by ion exchange. The results of tritium in drinking water analyses for April June 1983 are shown in Table 11. All samples were taken as either a single grab sample or composite samples taken over 12 to 14 days. 16 ------- TABLE 11 DRINKING WATER TRITIUM CONCENTRATION APRIL - JUNE 1983 LOCATION AK:FAIRBANKS AL:DOTHAN AL:MONTGOMERY AL:MUSCLE SHOALS ALrSCOTTSBORO CA:BERKELEY CA:LOS ANGELES CO:DENVER COtPLATTEVILLE CT:HARTFORD FL:MIAMI FL:TAMPA GA:SAVANNAH HI:HONOLULU IA:CEDAR RAPIDS ID:IDAHO FALLS IL:MORRIS IL:W. CHICAGO KS:TOPEKA LA:NEW ORLEANS MA:LAWRENCE MD:BALTIMORE MD:CONOWINGO ME:AUGUSTA MI:DETROIT MIrGRAND RAPIDS MN:MINNEAPOLIS MN:RED WING MS:JACKSON MS:PORT GIBSON MT:HELENA NC:CHARLOTTE NC:WILMINGTON ND:BISMARCK NErLINCOLN NH: CONCORD NJ:WARETOWN NM:SANTA FE NV:LAS VEGAS NY:ALBANY NY:NEW YORK CITY NY:NIAGARA FALLS OH:CINCINNATI OH:COLUMBUS DATE COLLECTED 4/ 1/83 4/ 7/83 4/ 5/83 4/ 4/83 5/27/83 4/ 1/83 4/ 1/83 4/22/83 4/22/83 4/ 4/83 4/ 1/83 4/11/83 4/20/83 4/ 1/83 4/ 3/83 5/ 2/83 4/ 4/83 4/ 1/83 4/ 1/83 4/ 4/83 4/ 5/83 4/ 5/83 4/19/83 4/ 7/83 4/ 5/83 4/ 7/83 4/ 4/83 4/20/83 4/ 1/83 4/ 7/83 4/ 8/83 4/ 5/83 4/ 7/83 4/ 1/83 5/23/83 4/ 1/83 4/ 7/83 4/ 4/83 4/ 1/83 4/ 1/83 4/11/83 4/ 6/83 5/16/83 4/ 1/83 nCi/1 0.3 0.2 0.3 0.3 0.2 0.1 0.2 0.3 0.4 0.2 0.2 0.0 1.6 0.2 0.2 0.2 0.1 0.2 0.2 0.4 0.2 0.1 0.4 0.2 0.4 0.3 0.2 0.1 0.2 0.2 0.3 0.3 0.2 0.3 0.2 0.2 0.1 0.1 0.3 0.3 0.2 0.1 0.1 0.1 ± 2s 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 17 ------- TABLE 11 (CONTINUED) DRINKING WATER TRITIUM CONCENTRATION APRIL - JUNE 1983 LOCATION OH:EAST LIVERPOOL OH:PAINESVILLE OH:TOLEDO OK:OKLAHOMA CITY OR:PORTLAND PA:COLUMBIA PA:HARRISBURG PA PITTSBURGH PC:ANCON RI:PROVIDENCE SC:BARNWELL SC:COLUMBIA SC:HARTSVILLE SC:JENKINSVILLE SC:SENECA TN:CHATTANOOGA TN:KNOXVILLE TX:AUSTIN VA:DOSWELL VA:LYNCHBURG VA:VIRGINIA BEACH WA:RICHLAND WA:SEATTLE WI:GENOA CITY WI:MADISON s SIGMA COUNTING ERROR DATE COLLECTED 4/13/83 A/ 1/83 4/ 1/83 A/ 1/83 4/ 4/83 4/21/83 4/15/83 4/13/83 A/ 6/83 4/ 4/83 4/21/83 A/ 1/83 4/11/83 4/ 8/83 4/19/83 4/29/83 A/ 1/83 A/ 1/83 4/22/83 A/ 1/83 A/ 6/83 4/19/83 A/ 1/83 A/ 5/83 A/- 5/83 nCi/1 0.1 0.3 0.4 0.2 0.1 0.2 0.2 0.1 0.1 0.2 0.1 0.4 0.1 0.2 0.2 0.4 0.2 0.3 0.2 0.3 0.1 0.4 0.2 0.1 0.1 ± 2s 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 0.2 18 ------- R^don-222^ in Drinking Water Radon-222 in drinking water has previously been considered a source of radiation exposure primarily from an ingestion standpoint. The Office of Radiation Programs (ORP) of the U.S. Environmental Protection Agency (EPA) is investigating radon in water supplies to evaluate the possibility that a major pathway from inhalation exposure may exist in addition to the ingestion pathway. As an inert gas, radon is not chemically bound to the water and consequently can be released during any operation that aerates or agitates water. Depending upon the initial concentration of radon in water, significant quantities of radon could be released in a home or to the general environment. To determine the scope of this potential problem, a national ground water sampling program has been initiated by the Eastern Environmental Radiation Facility (EERF) to obtain data on radon concentrations in water supplies throughout the country. Sampling kits have been assembled by EERF and distributed to various state health departments. The kit is designed so that state personnel can collect samples from potable water supplies and ship them, without loss of radon other than radioactive decay, to EERF for analysis. The selection of water supplies to be sampled is handled by two separate methods. Method 1 in which each state collects samples from all groundwater supplies serving at least 1000 people and Method 2 in which the choice of sampling locations and the number of supplies to be sampled is left to the discretion of the state programs. Each state is asked to obtain a representative sampling of ground water supplies within its boundaries. The extent of the sampling efforts and how representative the data are for a given state is determined primarily by the amount of time each state devotes to the program. The concentrations of radon in water are determined at the EERF by liquid scintillation counting. The limit of detection for this technique using a 50-minute count and a 10-ml sample is 0.16 pCi or 16 pci/1. The sampling kits are being provided to the various states on a rotating schedule. This schedule is designed to cover the U.S. within approximately two years. Summaries of the data for Arizona, Illinois, Rhode Island, South Carolina, Tennessee, Virginia, Vermont and Wyoming are shown in Tables 12-19. All radon concentration and counting error results are computer generated resulting in numbers that are less accurate than what is presented (i. e., up to five significant figures are Implied). All results should be rounded off to no more than three significant figures when using these results. 19 ------- TABLE 12 RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s AZ:APACHE JUNCTION AZ:ARIZONA CITY AZ:AVONDALE AZrBISBEE AZ:BUCKEYE AZ:BUCKEYE AZ:CAREFREE AZrCASA GRANDE AZ:CAVE CREEK AZ:COOLIDGE AZ:COOLIDGE AZ:DOUGLAS AZ:EL MIRAGE AZ:ELOY AZ:FLORENCE AZ:FLORENCE AZ:FLORENCE AZ:FOUNTAIN HILLS AZ:GILA BEND AZ:GLENDALE AZ:GLOBE AZ:GOODYEAR AZ:HAYDEN AZ:HUACHUCA AZ:KEARNEY AZ:LITCHFIELD PARK AZ:LITCHFIELD PARK AZ:MAMMOTH AZ:MIAMI AZ:NOGALES AZ:NOGALES AZ:ORACLE AZ:PARADISE VALLEY AZ:PARKER AZ:PAYSON AZ:PHOENIX AZ:PHOENIX AZ:PHOENIX AZ:PICACHO AZ:PINE AZ:PINE AZtPRESCOTT AZ:SCOTTSDALE AZ:SIERRA VISTA AZ:SIERRA VISTA AZ:SIERRA VISTA AZ:SIERRA VISTA 4/15/81 5/29/81 6/ 4/81 4/28/81 4/30/81 4/30/81 3/18/81 3/10/81 3/18/81 3/10/81 3/10/81 4/ 7/81 3/17/81 3/19/81 3/18/81 3/18/81 3/18/81 3/18/81 5/22/81 3/17/81 3/13/81 4/30/81 4/ 9/81 4/ 2/81 4/ 9/81 3/18/81 4/30/81 4/ 9/81 3/13/81 4/21/81 4/21/81 4/ 9/81 3/18/81 6/ 2/81 4/28/81 3/17/81 3/17/81 3/17/81 5/ 7/81 4/27/81 4/27/81 4/27/81 3/18/81 3/17/81 4/14/81 4/14/81 7/15/81 10000 1200 6550 12000 1800 3300 1200 14900 1450 6711 1000 17300 7200 7000 3200 1300 2500 3500 1800 80500 8500 2000 1400 2380 3000 3500 1200 1300 11456 13500 1363 3000 11000 6000 7000 880000 1200 20100 2500 1600 4169 3256 53000 6130 1295 1505 4543 135.8 308.6 251.3 487.4 1005.5 372.9 2228.5 544.2 1356.5 249.1 241.9 369.1 128.1 195.2 197.8 236.0 251,1 728.1 279.6 386.8 310.5 203.6 113.7 0.0 310.9 64.2 194.0 580.9 259.5 396.4 253.2 210.8 242.5 463.4 6118.5 311.9 233.9 335.3 137.5 -51.6 226.3 859.9 433.3 608.2 313.3 1153.0 535.9 107.9 77.8 110.1 78.4 140.8 130.3 111.4 54.4 95.0 48.6 49.6 51.5 110.4 61.7 42.3 42.3 43.0 97.3 133.3 107.7 92.7 123.7 90.2 650.2 92.8 91.6 156.9 95.8 90.8 72.8 67.5 90.7 114.4 155.2 123.0 143.3 104.8 105.0 93.0 83.6 88.2 98.7 121.1 48.7 81.4 92.2 80.4 20 ------- TABLE 12 (CONTINUED) RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s AZ:SIERRA VISTA AZ:SOMERTON AZrSUN CITY AZrSUN CITY AZ:SUN CITY AZ:SUPERIOR AZrTOLLESON AZ:TUCSON AZ:TUCSON AZ:TUCSON AZ:TUCSON AZ:TUSCON AZcTUSCON AZcTUSCON AZ:TUSCON AZ:TUSCON AZ:YUMA 7/15/81 5/22/81 3/10/81 3/17/81 3/17/81 3/13/81 4/30/81 4/ 9/81 5/ 7/81 9/28/81 9/28/81 3/ 2/82 3/ 2/82 3/ 2/82 3/ 2/82 3/ 2/82 5/22/81 5425 3500 1200 2400 48000 5000 4000 443680 121140 22750 15000 1700 3200 3245 3200 3100 3500 743.8 265.1 561.1 708.5 310.1 30.9 57.2 201.8 434.3 460.7 416.2 19.7 326.4 246.9 262.1 53.1 68.7 81.9 126.4 56.1 113.1 142.5 89.3 153.2 88.8 101.0 78.3 78.9 60.3 63.6 62.7 72.5 60.5 124.9 s = SIGMA COUNTING ERROR ( pCi/1 ) 21 ------- TABLE 13 RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCl/1 + 2s ILcADDISON IL:ARLINGTON HEIGH IL:AURORA IL:AURORA IL:HARRINGTON IL:BARTLETT IL:BATAVIA IL:BATAVIA ILiBEARDSTOWN IL:BELLWOOD IL:BELVIDERE ILrBENSENVILLE ILtBETHALTO IL:BLOOMINGDALE IL:BOLINGBROOK IL:BOLINGBROOK IL:BUFFALO GROVE IL:BUSHNELL IL:CAROL STREAM IL:CAROL STREAM IL:CARPENTERSVILLE IL:CHICAGO HEIGHTS IL:CHILLICOTHE IL:CLARENDON HILLS IL:CLINTON IL:COAL VALLEY IL:COLLINSVILLE IL:COUNTRY CLUB HI IL:CREST HILL IL:CREVE-COURE IL:CRYSTAL LAKE IL:CUBA IL:DARIEN IL:DEKALB IL:DES PLAINES IL:DES PLAINES IL:DIXON IL:DOWNERS GROVE IL:E. CHICAGO HEIG IL:EAST ALTON IL:EAST PEORIA IL:EDWARDSVILLE IL:ELGIN IL:ELK GROVE IL:ELMHURST IL:FLOSSMOOR IL:FOX LAKE 9/17/82 8/25/82 1/22/81 7/20/82 8/ 6/82 8/26/82 1/21/81 7/26/82 7/14/82 8/24/82 8/ 5/82 9/17/82 7/20/82 9/17/82 7/27/82 7/27/82 8/27/82 1/19/81 1/22/81 9/ 7/82 8/ 2/82 9/ 1/82 6/17/82 8/ 4/82 8/10/82 1/20/81 7/20/82 8/18/82 11 2/82 8/18/82 7/29/82 1/19/81 7/27/82 8/ 5/82 8/26/82 8/26/82 8/ 3/82 7/27/82 9/ 1/82 7/20/82 8/18/82 7/20/82 8/ 2/82 8/27/82 9/ 3/82 8/27/82 8/20/82 29759 65000 75000 82000 9029 13254 10000 12800 6500 23000 15000 16124 16103 13000 15000 28000 22684 3500 > 10000 15500 23000 37026 6500 6857 7400 3500 19567 14676 8000 6851 18590 3500 12000 35500 6237 54000 15650 42500 5347 8750 23500 15400 67000 28907 44251 8300 6300 150.4 438.1 123.9 265.1 -2.0 167.1 47.0 209.6 138.8 112.6 160.8 92.9 47.2 210.3 486.1 373.7 45.9 180.0 -47.5 241.7 7.9 338.6 315.3 148.7 45.9 130.5 55.8 296.0 268.6 550.8 97.4 302.8 324.9 127.4 91.1 81.1 144.8 647.2 256.6 30.9 439.9 2.9 76.1 72.3 189.4 218.3 18.1 96.0 112.2 75.6 76.8 80.5 93.8 88.4 74.3 56.9 56.5 101.8 96.3 59.8 96.5 147.3 67.1 68.3 57.6 73.1 72.4 40.3 62.2 86.0 124.9 58.0 47.0 115.1 104.5 94.9 104.7 101.6 57.5 142.3 98.8 85.6 85.9 73.1 145.0 61.5 61.0 101.0 58.3 56.8 69.5 95.2 78.6 64.4 22 ------- TABLE 13 (CONTINUED) RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s IL:FREEPORT ILrGALESBURG IL:GENESEO IL:GENEVA IL:GLEN ELLYN IL:GLEN ELLYN IL:GLENDALE HEIGHT IL:GLENVIEW IL:GLENWOOD ILrGRAYSLAKE ILrGURNEE IL:HANOVER PARK IL:HARVARD ILrHINSDALE IL:HOFFMAN ESTATES IL:HOMEWOOD IL:HOOPESTON IL:ITASCA IL:JERSEYVILLE IL:JOLIET IL:JONESBORO IL:KEWANEE IL:LA GRANGE IL:LA GRANGE HIGHL IL:LA SALLE IL:LAKE COUNTRY IL:LAKE IN THE HIL IL:LAKE ZURICH IL:LAWRENCEVILLE IL:LEMONT IL:LEMONT IL:LIBERTYVILLE IL:LINCOLN IL:LISLE IL:LISLE IL:LOCKPORT IL:LOMBARD IL:LOVES PARK IL:MATTESON IL:MCHENRY IL:MENDOTA IL:METROPOLIS IL:MILAN IL:MINONK IL:MOMENCE IL:MONMOTH IL:MONTGOMERY 8/ 4/82 8/25/82 8/23/82 7/26/82 7/30/82 9/20/82 9/ 7/82 8/25/82 8/31/82 8/ 7/82 8/ 9/82 8/26/82 7/26/82 8/16/82 8/27/82 9/ 1/82 7/27/82 9/ 7/82 7/14/82 6/30/82 8/ 5/82 8/23/82 8/12/82 8/12/82 8/26/82 8/ 7/82 7/29/82 8/ 9/82 8/10/82 1/22/81 7/ 2/82 8/ 9/82 7/14/82 8/ 4/82 8/ 5/82 7/ 2/82 9/20/82 8/ 9/82 8/18/82 7/29/82 8/26/82 8/ 5/82 8/25/82 1/21/81 8/ 9/82 8/25/82 7/20/82 30000 35300 6450 9880 8650 23649 24000 32000 10437 5260 6300 28719 5126 18000 37000 19724 6500 7129 8627 78000 10000 14500 17100 4700 10800 2027 5651 8225 9200 5500 5600 16520 19000 9000 9500 10000 37295 13000 10282 10908 7100 7000 6300 2500 3300 12100 13800 59.2 183.8 237.7 68.7 261.9 111.8 83.0 58.6 352.2 95.8 98.0 196.8 21.9 34.1 278.6 86.7 57.6 92.7 70.1 129.8 66.2 340,2 54.5 55.8 599.0 995.0 185.0 66.8 7.4 88.3 230.8 62.8 118.0 543.5 160.6 219.3 90.8 96.4 360.1 156.4 55.0 549.7 101.0 71.0 598.1 85.8 98.7 58.2 63.1 59.4 69.7 86.1 55.9 69.1 111.0 73.9 70.6 59.3 92.1 62.7 56.0 75.1 57.6 57.1 68.6 55.7 57.1 97.5 74.1 78.5 77.7 98.8 84.4 101.5 56.6 58.9 74.2 92.1 69.9 54.9 130.2 121.9 93.5 56.8 134.5 104.5 100.2 80.2 109.5 62.5 87.4 68.7 62.2 120.5 23 ------- TABLE 13 (CONTINUED) RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s IL:MORRIS IL:MORTON IL:MOUNT PROSPECT IL:MT. PROSPECT IL:MUNDELEIN IL:N. AURORA IL:NAPERVILLE IL:NEW LENOX IL:NORMAL IL:NORTH PARK IL:NORTH TAZWELL IL:OAK BROOK IL:ORLAND PARK IL:OTTOWA IL:PALATINE IL:PALATINE IL:PARK FOREST IL:PARK FOREST SO. IL:PAXTON IL:PEKIN IL:PEORIA HEIGHTS IL:PERU IL:PLANO IL:PRINCETON IL:RANTOUL IL:RICHTON PARK IL:RIVERSIDE IL:ROCHELLE IL:ROCK FALLS IL:ROCKFORD IL:ROLLING MEADOWS IL:ROMEOVILLE IL:ROSELLE IL:ROUND LAKE BEAC IL:S. ELGIN IL:SANDWICH IL:SAUK VILLAGE IL:SCHAUMBURG IL:SILVIS IL:SO. CHICAGO HEI IL:SPRING VALLEY IL:ST. CHARLES IL:STEGER IL:STERLING IL:STREAMWOOD IL:SYCAMORE IL:THORNTON 6/30/82 6/21/82 8/25/82 8/26/82 8/ 9/82 7/26/82 7/30/82 11 2/82 8/10/82 8/10/82 8/30/82 9/ 3/82 8/16/82 8/27/82 8/25/82 8/25/82 8/18/82 8/ 9/82 7/27/82 11 1/82 6/18/82 8/26/82 7/20/82 8/26/82 7/27/82 8/18/82 8/12/82 8/ 5/82 8/ 3/82 8/ 9/82 8/25/82 11 2/82 9/ 7/82 8/20/82 8/ 2/82 8/ 5/82 8/31/82 8/27/82 8/23/82 8/27/82 6/22/82 8/ 6/82 8/27/82 8/ 3/82 8/27/82 8/ 5/82 1/22/81 8835 14000 20000 39100 17573 5300 47600 6265 34800 18500 10000 14300 23045 19500 32166 7600 26222 6300 4500 34000 8500 13000 5000 7300 13500 9403 9236 9100 60640 150000 20167 15500 16948 13600 6218 5600 10906 52000 8300 3775 5800 17500 10000 19500 23400 9000 3700 22.9 73.9 107.8 149.4 188.7 69.2 337.5 225.0 25.4 171.6 10.2 138.8 207.4 108.0 366.3 105.6 97.3 226.1 137.2 348.0 302.7 111.1 381.9 16.3 40.4 273.4 226.0 29.4 63.5 81.2 152.1 60.5 64.5 235.2 178.4 95.2 334.3 261.0 99.3 15.5 181.8 288.4 188.9 150.6 155.1 -14.4 176.6 56.6 57.3 104.7 88.4 73.0 71.9 87.7 105.8 56.5 60.1 54.2 100.4 57.4 69.8 111.7 106.9 97.6 84.1 59.2 115.2 70.8 82.8 129.8 81.1 57.8 101.1 84.0 94.4 69.1 69.1 111.8 89.9 68.0 69.2 57.6 96.9 74.5 338.6 56.5 73.4 59.1 125.2 75.9 70.5 82.1 95.6 74.2 24 ------- TABLE 13 (CONTINUED) RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s IL:TROY IL:URBANA IL:VILLA PARK IL:W. CHICAGO IL:WASHINGTON IL:WATSEKA ILrWAUCONDA IL:WESTERN SPRINGS IL:WESTMONT IL:WHEATON IL:WHEELING IL:WINFIELD IL:WINTHROP HARBOR IL:WOOD DALE IL:WOOD RIVER IL:WOODRIDGE IL:WOODSTOCK 7/21/82 7/27/82 9/20/82 9/21/82 6/17/82 8/25/82 8/ 6/82 8/12/82 8/ 4/82 9/20/82 8/25/82 9/21/82 8/ 9/82 9/17/82 7/20/82 7/27/82 7/26/82 6650 135000 23185 12550 9500 5543 5688 12876 16700 44075 23266 4600 5428 11251 16275 2300 11725 25.1 39.1 174.2 183.2 105.4 243.9 220.4 119.2 -88.7 170.1 174.0 40.5 118.7 142.4 138.1 491.4 21.8 62.7 57.9 59.1 58.8 80.6 63.4 85.9 81.5 121.8 56.1 107.2 55.9 59.9 97.0 62.6 148.0 62.2 s = SIGMA COUNTING ERROR ( pCl/1 ) 25 ------- TABLE 14 RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s RI:BRIARCLIFFE RI:BRIARCLIFFE RI:BRIARCLIFFE RI:BRIARCLIFFE RI:BRIARCLIFFE RI:BURRILLVILLE RI:BURRILLVILLE RI:BURRILLVILLE RI:BURRILLVILLE RI:BURRILLVILLE RI:BURRILLVILLE RI:BURRILLVILLE RI:BURRILLVILLE RI: BURRILLVILLE RI:CHARLESTOWN RI:CHARLESTOWN RI:CHARLESTOWN RI:CHARLESTOWN RI:CHARLESTOWN RI:CHARLESTOWN RI:CHARLESTOWN RI:CHEPACHET RI:CHEPACHET RI: CHEPACHET RI:CHEPACHET RI:COVENTRY RI:COVENTRY RI:CUMBERLAND RI:CUMBERLAND RI:GLENDALE RI:GLENDALE RI:GLENDALE RI:GLOUCESTER RI: GLOUCESTER RI:GLOUCESTER RI GLOUCESTER, RI GLOUCESTER, RI:GLOUCESTER RI GLOUCESTER RI:GLOUCESTER RI:GLOUCESTER RI:HARRISVILLE RI:HARRISVILLE 5/14/82 5/14/82 5/14/82 5/14/82 5/14/82 ! 4/21/81 5 4/21/81 ! 7/15/81 I 4/21/81 ! 4/21/81 ! 4/21/81 5 4/21/81 ! 4/21/81 I 4/21/81 8/14/81 8/14/81 8/14/81 8/14/81 8/20/81 8/20/81 8/20/81 5/ 1/81 5/ 1/81 4/16/81 5/ 1/81 12/17/80 8/26/81 9/ 1/81 9/ 1/81 4/16/81 4/16/81 7/15/81 4/16/81 5/ 1/81 5/ 1/81 WES 5/ 1/81 WES 5/ 1/81 8/26/81 8/26/81 8/26/81 8/26/81 1/14/81 1/14/81 >UTH1 1/25/80 IUTH11/25/80 IUTH 4/30/81 >UTH 8/20/81 550* 550 550 550 550 < 100 550 550 550 550 550 < 100 550 550 550 550 550 550 550 550 550 550 550 550 550 70000 < 100 550 550 550 < 100 550 550 550 550 550 550 550 550 550 550 3000 3000 3200 3200 550 550 206200.0 248850.0 185550.0 233200.0 265600.0 809.5 418.2 1267.0 2430.0 4351.0 5186.0 2050.0 6151.5 3076.5 2040.5 3536.0 2098.0 2129.0 15510.0 8019.0 3742.0 1180.5 690.2 2765.5 1184.0 1719.0 1826.5 1496.5 1514.5 13400.0 1120.5 5108.0 692.7 1020.0 873.8 377.4 1602.0 2074.0 420.9 1658.0 898.9 747.3 809.3 2255.0 3038.5 587.0 2516.0 0.0 ** 0.0 ** 0.0 ** 0.0 ** 0.0 ** 97.1 93.5 139.4 121.5 130.5 155.6 111.6 123.0 123.1 102.1 106.1 104.9 106.5 155.1 160.4 149.7 130.0 123.9 138.4 135.9 103,4 127.9 92.6 90.9 134.0 106.4 204.3 103.9 142.8 125.6 118.6 135.8 134.1 106.4 124.1 116.1 74.8 76.7 90.2 91.2 117.2 125.8 26 ------- LOCATION TABLE 14 (CONTINUED) RADON IN GROUND WATER SUPPLIES COLLECTION DATE POPULATION Rn~222 CONCENTRATION SERVED pCi/1 + 2s RI:KINGSTON, SOUTH 8/20/81 RI:KINGSTON, SOUTH 1/15/81 RlrKINGSTON, SOUTH 3/17/81 RI .-KINGSTON, SOUTH 8/20/81 RI KINGSTON, SOUTH 4/30/81 RlrKINGSTON, SOUTH 8/20/81 RlrLINCOLN 2/25/81 RI:LINCOLN 2/25/81 RI:LINCOLN 2/25/81 RI-.LINCOLN 2/25/81 RI:LINCOLN 2/25/81 RI:NO. SMITHFIELD 9/ 4/81 RI.-NO. SMITHFIELD 9/ 4/81 RI:NO. SMITHFIELD 9/ 4/81 RI:NORTH KINGSTOWN I/15/81 RI:NORTH KINGSTOWN 1/27/81 RI-.NORTH KINGSTOWN 1/27/81 RI:NORTH KINGSTOWN 1/27/81 RI .-NORTH KINGSTOWN 1/27/81 RI:NORTH KINGSTOWN 1/27/81 RI:NORTH KINGSTOWN 1/27/81 RI .-NORTH KINGSTOWN 1/27/81 RI:NORTH KINGSTOWN 1/27/81 RI-.NORTH KINGSTOWN 1/27/81 RI:NORTH KINGSTOWN 5/20/81 RI:NORTH KINGSTOWN 5/20/81 RI:PASCOAG 1/14/81 RI:PASCOAG 1/14/81 RI:SMITHFIELD 7/15/81 RI.-TIVERTON 5/19/81 RI-.TIVERTON 5/19/81 RI:TIVERTON 5/19/81 RI:W. KINGSTON 4/30/81 RlrWAKEFIELD 11/25/80 RI:WARWICK 1/12/81 RlrWARWICK 1/12/81 RI:WARWICK 1/27/81 RI:WARWICK 1/27/81 RI:WEST GREENWICH 12/17/80 RI:WEST GREENWICH 12/17/80 RI.-WEST GREENWICH 12/17/80 RlrWESTERLY 12/18/80 RI:WESTERLY 12/18/80 RI:WESTERLY 12/18/80 RI:WESTERLY 12/18/80 550 2100 500 550 550 550 13500 13500 13500 13500 13500 550 550 550 1500 22000 22000 22000 22000 22000 22000 22000 22000 22000 550 550 5200 5200 550 100 550 550 550 28000 6000 6000 70000 70000 70000 70000 70000 20000 20000 20000 20000 7788.0 1113.5 2757.0 32590.0 16745.0 2524.5 312.8 845.4 924.6 415.4 830.9 360.6 3533.5 23145.0 118.9 1294.5 1656.0 1455.0 1656.0 1455.0 1656.0 1455.0 1905.5 2394.5 10315.0 2585.0 1175.0 565.7 119.5 3098.0 22045.0 17985.0 2101.0 1948.5 2605.0 3132.0 2205.5 2034.0 930.4 1093.0 955.8 958.5 843.9 1195.0 1161.5 155.8 72.0 55.2 325.9 167.5 126.4 89.1 97.0 96.8 89.3 95.4 77.2 176.7 231.7 62.0 64.7 66.2 58.2 66.2 58.2 66.2 58.2 57.2 71.9 206.3 181.1 82.4 79.2 118.9 217.5 440.9 359.7 147.1 97.5 117.2 125.8 66.2 70.6 97.7 98.4 94.6 85.6 83.6 83.7 87.0 * 550 REPRESENTS 100-1000 PEOPLE SERVED ** 0.0 REPRESENTS LESS THAN + 0.005% COUNTING ERROR s = SIGMA COUNTING ERROR ( pCi/1 ) 27 ------- TABLE 15 RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s SCtAIKEN SCtAIKEN SC:ALLENDALE SC:ANDREWS SC:BAMBERG SC:BARNWELL SC:BATH SCrBATH SC:BEACH ISLAND SC:BELVEDERE SC:BENNETTSVILLE SC:BISHOPVILLE SC:BLACKVILLE SC:BLENHEIM SC:BOWMAN SC:BRANCHVILLE SC:BREEZY HILL SC:BUFFALO SC:BULLS BAY SC:BURNETTOWN SC:CASSATT SC:CHERAW SC:CLIFTON SC:CLOVER SC:CLOVER SC:COLUMBIA SC:COLUMBIA SC:COLUMBIA SC:CONWAY SC:DARLINGTON SC:DENMARK SC:DILLON SC:ELLOREE SC:ESTILL SC:FAIRFAX SC:FLORENCE SC:FORT MILL SC:GARDEN CITY SCrGASTON SC:GEORGETOWN SC:GILBERT SC:GLOVERVILLE SC:GOOSE CREEK SC:GRAY COURT SC:HAMPTON SC:HARDEEVILLE SC:HARTSVILLE 7/27/81 7/27/81 7/28/81 8/ 3/81 7/14/81 7/19/82 7/27/81 7/27/81 7/27/81 7/27/81 5/24/82 4/27/82 7/19/82 5/24/82 7/14/81 7/14/81 7/27/81 7/20/82 7/29/81 7/27/81 8/10/81 5/24/82 7/20/82 4/20/82 4/20/82 11 8/81 7/ 8/81 11 8/81 8/ 4/81 8/10/81 7/14/81 5/31/82 7/14/81 7/28/81 7/28/81 4/27/82 4/20/82 8/ 3/81 7/13/81 8/ 3/81 7/ 8/81 7/27/81 7/29/81 7/20/82 7/28/81 7/25/81 8/10/81 2000 1250 5134 3800 4900 6500 1560 1239 4500 6800 11900 4000 2975 1383 2056 1330 7000 1260 3150 1200 1558 4725 1365 5075 2030 1228 1412 1435 11000 10150 4550 3500 2000 3010 1973 44000 2600 2650 2000 5500 1850 1440 4648 1250 4300 2222 11000 216.3 454.0 227.3 98.2 -15.5 339.0 131.0 150.3 196.3 58.6 298.1 381.8 341.1 455.5 32.8 34.8 191.4 5653.0 51.0 79.5 203.9 52.2 75.5 4092.0 45.8 722.9 943.8 -126.5 118.1 126.6 210.7 152.2 105.1 37.2 73.9 -21.3 3618.0- 85.6 262.8 155.7 989.8 18.6 -5.2 16135.0 154.7 -24.2 252.1 82.1 86.3 74.6 77.3 81.9 81.4 81.2 81.6 82.8 79.6 60.9 63.0 80.1 63.8 82.5 83.0 114.0 113.2 110.4 80.1 78.2 56.4 64.5 81.8 57.4 68.5 75.5 56.7 71.2 76.7 86.3 58.1 83.5 84.8 86.2 54.7 108.5 76.3 61.7 77.7 73.9- 56.1 76.4 161.4 86.8 143.8 78.2 28 ------- TABLE 15 (CONTINUED) RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s SC:HEMINGWAY SC:HILTON HEAD SCrHOLLY HILL SC:HOWLANDVILLE SC:INMAN SC:ISLE OF PALMS SC:JACKSON SC:JOHNSONVILLE SC:KINGSTREE SCrLAKE CITY SC:LAKE VIEW SC:LAMAR SCtLANGLEY SC:LATTA SCrLAURENS SCtLEESVILLE SCiLITTLE MOUNTAIN SCtLORIS SC:MANNING SC:MARION SC:MARION SC:MCBEE SCiMCCALL SC:MONCKS CORNER SC:MT. PLEASANT SC:MULLINS SC:MURRELL'S INLET SC:MYRTLE BEACH SC:MYRTLE BEACH SC:NEW ELLENTON SC:NORTH SC:OUTLAND SC:PACOLET MILLS SC:PAMLICO SCrPAWLEY'S ISLAND SC:PINOPOLIS SC PROSPERITY SC:RIDGELAND SC:SANGAREE SCrSEABROOK SC:SHAW AFB SCrSPARTANBURG SC:SPRINGFIELD SC:ST. GEORGE SC:ST. MATTHEWS SC:ST. STEPHEN SC:SULLIVAN'S ISLA 8/ 4/81 7/28/81 7/14/81 7/27/81 7/20/82 7/29/81 7/27/81 8/ 4/81 8/ 3/81 8/ 4/81 8/ 4/81 8/10/81 7/27/81 5/31/82 7/20/82 11 8/81 7/13/81 8/ 4/81 7/20/81 8/ 4/81 8/ 4/81 8/10/81 5/24/82 7/29/81 7/29/81 8/ 4/81 8/ 3/81 8/ 3/81 8/ 4/81 7/27/81 7/14/81 8/ 3/81 7/20/82 8/ 4/81 8/ 3/81 7/29/81 7/13/81 7/28/81 7/29/81 7/28/81 7/20/81 7/20/82 7/19/82 7/14/81 7/14/81 8/ 3/81 7/29/81 1400 2922 1600 1232 1068 5250 3152 3500 6300 8750 1230 1575 1330 2450 2636 3400 1420 2540 5282 2625 10000 1190 3115 3500 11900 9450 1200 20000 6000 4000 1918 1050 2268 1680 3800 1200 1035 2013 3381 8724 6975 3000 1120 2835 4200 1900 2660 30.8 -17.0 131.5 73.6 45.2 88.9 394.5 42.2 190.8 138.2 82.5 536.9 73.2 274.7 39.4 236.4 303.8 74.6 150.4 1244.0 221.2 240.3 387.5 132.1 32.5 67.4 133.6 102.9 72.1 154.6 331.8 117.0 45.3 89.9 152.9 83.7 3882.5 -35.6 17.0 137.1 95.1 96.2 314.8 258.2 500.0 54.3 -13.0 69.7 83.3 85.2 79.9 63.6 111.2 85.3 69.5 78.6 76.5 70.0 83.1 80.8 60.3 63.2 64.3 62.4 70.1 62.4 87.1 73.0 78.2 62.0 111.6 109.1 70.4 77.9 76.7 75.1 82.5 87.6 77.4 63.6 101.1 77.5 110.9 116.5 81.7 109.6 91.8 61.3 64.0 79.4 86.5 89.7 77.0 108.5 29 ------- TABLE 15 (CONTINUED) RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCl/1 + 2s SClSUMMERTON 7/20/81 2100 SCtSUMTER 7/20/81 2325 SC:SUMTER 7/20/81 40859 SCtSURFSIDE BEACH 8/ 3/81 5500 SC:SWANSEA 7/13/81 1364 SCrTALATHA 7/27/81 1300 SC:TIMMONSVILLE 4/27/82 2615 SC:VARNVILLE 7/28/81 1760 SC:WAGENER 7/27/81 1400 SC:WATERBORO 7/28/81 12000 SCsWILLISTON 7/27/81 3800 SC:WINDJAMMER MHP 8/ 3/81 1386 194.5 65.9 85.1 33.8 303.9 373.4 122. 222. 225, 298.8 345.1 239.4 .5 .7 .7 .3 ,1 62.8 60.2 61.0 75.9 62, 85, 57.6 89.0 80.9 88.0 86.1 80.2 s - SIGMA COUNTING ERROR ( pCi/1 ) 30 ------- TABLE 16 RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCl/1 + 2s TN:ALAMO TNrBARTLETT TN:BARTLETT TN:BOLIVAR TN:BROWNSVILLE TN:CHATTANOOGA TN:COVINGTON TN:COVINGTON TN:DECHERD TN:DRESDEN TN:DYERSBURG TN:DYERSBURG TN:EAGLEVILLE TN:ELIZABETH TN:ELIZABETHTON TN:ERWIN TN:HALLS TN:HENDERSON TN:HIXSON TN:HOENWALD TN:HUMBOLDT TN:HUNTINGDON TN:JACKSON TN:JACKSON TN:JEFFERSON CITY TN:LAFAYETTE TN:MARTIN TN:MCKINZIE TN:MEMPHIS TN:MILAN TN:MILLINGTON TN:MILLINGTON TN:MOUNTAIN CITY TN:NEW TAZWELL TN:NEWBURN TN:OLIVER SPRINGS TN:PARIS TN:PIKEVILLE TN:RIPLEY TN:RIPLEY TN:SAVANNAH TN:SEMLER TN:SIGNAL MTN. TN:SO. FULTON TN:SOMERVILLE TN:TAFT TN:TRACY CITY TN:TRENTON TN:UNION CITY TN:WOODBURY 7/28/82 7/27/82 7/27/82 7/26/82 7/27/82 8/ 5/82 7/27/82 7/27/82 8/ 5/82 7/28/82 7/28/82 7/28/82 9/14/82 8/24/82 8/24/82 8/24/82 7/27/82 7/26/82 8/ 6/82 9/16/82 7/28/82 7/28/82 7/26/82 7/27/82 8/25/82 9/15/82 7/28/82 7/28/82 7/27/82 7/28/82 7/27/82 7/27/82 8/24/82 8/25/82 7/28/82 8/25/82 7/28/82 9/15/82 7/27/82 7/27/82 7/26/82 7/26/82 8/ 5/82 7/28/82 7/26/82 9/14/82 10/12/82 7/28/82 7/28/82 9/15/82 3000 2800 3300 8000 10000 7643 4631 8000 1045 3000 1430 15143 500 8800 3835 3500 3900 5000 14000 4000 10000 4000 50000 50000 10000 2500 9585 2000 655320 10270 9500 15000 5492 7500 6183 5295 4200 800 2500 7500 4000 8503 1510 2500 4070 2400 3538 5000 6000 1500 83.3 -4.5 -58.3 40.9 -5.1 211.0 9.4 -10.2 587.8 27.3 -33.7 3.1 165.3 210.6 980.8 208.1 -4.2 -1,7 23.8 694.1 85.0 32.5 11.0 24.8 33.3 164.1 62.5 62.1 -37.0 46.4 3.4 -33.4 276.3 -5.6 65.2 277.4 9.1 166.8 3.4 -17.8 185.4 119.8 241.2 28.6 46.3 148.6 -56.4 33.7 -10.4 297.5 112.2 39.4 65.9 69.9 67.2 104.2 67.6 47.2 116.8 102.1 59.7 60.9 142.9 71.1 83.3 70.7 66.6 65.6 89.4 111.1 102.5 102.3 65.8 55.5 108.4 117.7 103.2 102.4 67.0 101.9 67.9 66.9 68.1 108.0 103.2 111.3 101.8 120.1 66.9 66.6 68.5 67.7 108.0 102.2 66.4 140.4 166.8 101.9 101.3 122.0 s = SIGMA COUNTING ERROR ( pCi/1 ) 31 ------- TABLE 17 RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s VA:ALEXANDRIA VA:ALTAVISTA VA:ALTAVISTA VA:APPOMATTOX VAtAVONDALE VA:BOWLING GREEN VArBOYKINS VA:BOYKINS VA:BOYKINS VA:BRACEY VA:3RANCHVILLE VA:BUCHANAN VA:BUENA VISTA VA:BURKEVILLE VArCAPE CHARLES VA:CHASE CITY VA: CHESAPEAKE VA:CHESAPEAKE VA:CHILHOWIE VA:CHINCOTEAGUE VA:COLLINSVILLE VA:COLONIAL BEACH VAiCOURTLAND VA:DAHLGREN VA:DAHLGREN VA:DANTE VA:ELKTON VA:FAIRLAWN VA:FERRUM VA.-FORK UNION VA:FRANKLIN VA:GLASGOW VA:GLOUCESTER VA:GLOUCESTER VA:GROTTOES VA:GRUNDY VA:HONAKER VA:HOT SPRINGS VA:INDEPENDENCE VA:IRVINGTON VA:JONESVILLE VA:KILMARNOCK VA:LA CROSSE VA:LANEXA VA:LAUREL PARK VA: LEBANON VA:LEESBURG VA:LOUISA VA:LOUISA 6/23/81 4/27/81 3/31/81 3/31/81 5/13/82 7/15/81 5/20/82 6/30/82 6/30/82 4/ 8/81 5/20/82 6/24/82 5/ 7/81 4/14/81 8/12/82 4/14/81 6/15/82 8/11/82 6/17/81 8/12/82 4/17/81 7/28/82 4/14/82 5/14/81 5/14/81 6/12/81 5/ 4/81 8/ 3/82 4/21/81 4/ 9/81 11/23/81 5/ 7/81 7/22/82 7/22/82 5/ 4/81 6/12/81 6/12/81 5/ 6/81 6/23/81 5/18/82 6/29/81 7/22/82 4/ 8/81 6/15/81 4/17/81 6/12/81 5/15/81 6/ 5/81 5/22/81 1200 1000 1200 2500 1300 1000 800 1000 790 300 1000 1700 7000 800 1550 3400 2000 2240 3600 4000 7008 2500 1500 1000 3394 3600 1600 1600 1700 1000 9600 1350 1500 800 1400 1800 2500 2200 1000 1110 1190 1100 900 1194 1270 4000 11000 932 1100 303.3 2475.5 2012.5 1956.5 306.8 216.9 113.7 154.4 226.6 1255.0 187.8 148.3 474.0 7890.5 248.8 680.6 279.6 214.9 331.0 239.8 655.5 226.1 111.9 424.6 207.4 152.3 188.4 21.4 293.6 4743.5 184.9 109.9 255.8 207.0 120.7 -13.8 480.5 10.9 342.8 152.3 114.8 236.4 650.2 276.2 2098.5 537.7 247.7 9195.0 4543.0 64.8 99.0 100.7 97.8 89.0 77.0 85.9 60.2 61.8 181.8 83.1 86.4 101.8 236.7 88.5 135.8 61.4 59.0 66.2 86.2 144.2 64.1 97.0 101.7 97.3 78.5 170.9 67.1 88.1 142.3 64.2 97.2 90.2 89.5 165.4 75.1 86.5 114.7 65.1 71.5 72.5 90.3 165.7 66.2 168.0 86.0 81.0 183.9 136.7 32 ------- TABLE 17 (CONTINUED) RADON IN GROUND WATER SUPPLIES LOCATION' COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s VA.-LURAY VArMARION VA:MARTINSVILLE VAtMAYFIELD FARMS VArMCCLURE VArMCCLURE VA.-MCKENNEY VA:KECHANICSVILLE VA:MINERAL VA:NEW CASTLE VA:ONANCOCK VArPARKSLEY VA.-PEARISBURG VA:PEMBROKE VA: PETERSBURG VA:POTOMAC SHORES VA:PURCELLVILLE VA:RAINBOW FOREST VA:RICH CREEK VA:RICHMOND VA:RICHMOND VA:RICHMOND VA:RIDGEWAY VA:ROUND HILL VA:RURAL RETREAT VA: SALEM VArSALEM VArSALEM VA:SALEM VA:SALEM VA: SALEM VA:SALEM VA:SALEM VArSALTVILLE VA.'SMITHFIELD VA:SPRING MEADOWS VA:STANLEY VA:STANLEYTOWN VA:SUFFOLK VA:SUGAR GROVE VA:SURRY VA:TAPPAHANNOCK VA:VERONA VA:VIRGINIA BEACH VA:VIRGINIA BEACH VA:WAKEFIELD VA .'WARSAW 3/25/81 6/17/81 4/17/81 5/13/82 6/12/81 6/12/81 6/30/82 6/22/82 6/ 5/81 4/22/81 8/12/82 8/12/82 5/20/81 5/20/81 6/30/82 7/28/82 5/27/82 4/22/81 5/20/81 12/ 3/81 5/13/82 6/22/82 4/17/81 6/ 9/82 6/23/81 11 8/82 11 1/82 7/ 1/82 7/ 1/82 7/ 1/82 If 1/82 11 1/82 7/ 1/82 6/17/81 11/23/81 5/13/82 3/25/81 4/17/81 11/23/81 6/23/81 6/15/81 7/28/82 5/ 4/81 8/11/82 6/15/82 6/30/82 7/28/82 4000 2500 1450 1550 1800 1500 1312 3200 2800 1100 1700 1000 3500 500 1022 1364 1600 1450 1500 2300 1150 6000 227 1100 1500 2280 4200 6000 1452 5850 2476 2480 2224 3350 3600 2450 1208 1850 1100 1000 525 1800 3500 1860 2000 1100 1500 14.0 222.9 705.1 184.9 -4.6 6.3 4712.5 238.3 928.5 87.2 341.0 206.5 31.7 269.6 313.4 145.8 43.7 234.4 130.7 182.8 777.6 523.8 4975.0 9.2 213,8 -1.0 964.0 650.2 547.9 75.4 -52,5 67.5 316.2 316.1 168,8 190.9 138.0 732.2 193.2 52.6 -1.7 145.3 -57.7 379.7 368.1 214.6 235.5 51.9 63.5 150.9 85.5 74.5 74.3 188.8 76.2 102.1 69.8 88.8 87.7 60.2 64.6 63.9 58.1 177.0 70.0 62.0 94.5 93.3 67.5 199.0 60.5 63.1 81.8 120.4 116.6 115.1 105.5 102.0 104.6 111.3 66.4 66.4 85.7 38.6 150.2 64.1 59.7 71.7 63.9 157.2 62.6 76.4 62.3 65.1 33 ------- TABLE 17 (CONTINUED) RADON IN GROUND WATER SUPPLIES LOCATION COLLECTION POPULATION Rn-222 CONCENTRATION DATE SERVED pCi/1 + 2s VArWAVERLY 6/30/82 2500 172.5 62.7 VA:WAYNESBORO 5/ 6/81 19000 92.4 113.9 VA:WEST POINT 7/22/82 2726 230.7 90.7 VA:WINDSOR 11/23/81 1600 203.A 65.0 VA:WINTERGREEN 4/ 9/81 1000 146.6 94.0 s = SIGMA COUNTING ERROR ( pCi/1 ) 34 ------- LOCATION TABLE 18 RADON IN GROUND WATER SUPPLIES COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s VT:ARLINGTON VT:BETHEL VT.-CASTLETON VT:HARDWICK VTrLUDLOW VT:LYNDONVILLE VT:MORRISVILLE VTrPITTSFORD VTtQUECHEE VT:RANDOLPH VT:WINDSOR 6/1L/82 4/ 6/82 10/19/82 9/ 1/81 6/22/82 3/15/82 9/ 1/81 6/25/82 4/19/82 3/31/82 4/ 8/82 1200 1030 1900 1500 1250 3200 4100 1380 2000 2500 3700 396.0 841.3 650.0 388.6 773.6 1317.0 628.0 227.1 621.5 329.6 624.0 75.2 84.1 68.1 79.6 69.6 79.0 81.7 76.1 86.5 98.9 93.6 s - SIGMA COUNTING ERROR ( pCi/1 ) 35 ------- LOCATION TABLE 19 RADON IN GROUND WATER SUPPLIES COLLECTION DATE POPULATION Rn-222 CONCENTRATION SERVED pCi/1 + 2s WY:CASPER WY:DUBOIS WY:GILLETTE WY:GLENROCK WY:JACKSON WY:JEFFREY CITY WYtLUSK WY:LYMAN WY:MILLS WY:MILLS WY:MOORCROFT WY:NEWCASTLE WY:POWELL WY:RIVERTON WY:S. SUPERIOR WY:SHOSHONI WY:SUNDANCE WYrUPTON 7/30/82 8/24/82 7/13/82 8/ 5/82 8/ 8/82 9/15/82 7/ 8/82 6/18/82 7/30/82 7/30/82 7/14/82 11 7/82 9/ 2/82 8/25/82 9/25/81 8/24/82 7/14/82 11 7/82 3000 850 16603 2700 5000 500 1600 2284 3000 2500 1500 4500 5300 9288 700 879 1250 1100 131.6 306.0 54.1 307.9 556.4 93.8 379.5 1428.0 612.6 600.5 592.0 114.2 278.9 938.9 1729.5 1294.0 288.0 155.6 78.9 74.6 55.7 107.3 89.0 56.3 90.5 85.7 85.4 83.6 65.1 98.2 114.1 70.3 146.5 70.9 61.1 59.1 s = SIGMA COUNTING ERROR ( pCi/1 ) 36 ------- SECTION III. External Gamma Ambient Monitoring Program The external gamma monitoring program, which began in October 1978, provides a continuous measurement of ambient gamma exposure rates, including cosmic, at selected sites throughout the continental United States. Data from this program will be used to evaluate fluctuations in natural background due to variations in environmental conditions and to provide a means of monitoring any significant increases in ambient gamma levels due to weapons fallout, reactor operations, etc. Initially, the program will consist of approximately 22 sites representing a wide geographic coverage throughout the country. Hopefully, at some later date additional sites will be added to the program. Although exposure measurements at these few sites are not totally representative of nationwide exposures, they will be indicative of national trends. The jj program utilizes CaF2:Mn thertnoluminescent dosimeters (TLD's). These dosimeters are commercially available glass-bulb type dosimeters with energy compensating shields. A group of four TLD's is located at each station or site. Dosimeters are annealed by the station operator prior to positioning in the field. The dosimeters are returned to EERF for readout on an approximate one-month cycle. Several dosimeters are annealed by the station operator as controls and returned with the exposed field dosimeters to correct for any exposures accumulated during shipment. Results from the period April - June 1983 are shown In Table 20. 37 ------- TABLE 20 ENVIRONMENTAL GAMMA AMBIENT MONITORING PROGRAM INTEGRATED EXPOSURE LOCATION DATE RANGE EXPOSURE RATE MR MICRO R/HR + 2 s * AL:MONTGOMERY AL: MONTGOMERY AL:MONTGOMERY CA:BERKELEY CA:BERKELEY CA:BERKELEY CO:DENVER CO :DENVER CO:DENVER FL:ORLANDO FL:ORLANDO FL: ORLANDO ID:BOISE IL:CHICAGO IL: CHICAGO IL: CHICAGO ND:BISMARCK ND:BISMARCK ND:BISMARCK NJ:TRENTON NJ:TRENTON NJ:TRENTON MM:SANTA FE NM:SANTA FE NM:SANTA FE NV:LAS VEGAS NV:LAS VEGAS NV:LAS VEGAS NY:NEW YORK NY:NEW YORK NY:NEW YORK OH:COLUMBUS OH:COLUMBUS OH:COLUMBUS OK:OKLAHOMA CITY OK:OKLAHOMA CITY OK:OKLAHOMA CITY OR:PORTLAND OR:PORTLAND OR .-PORTLAND PA:HARRISBURG PA:HARRISBURG PA:HARRISBURG PA:PITTSBURGH PA PITTSBURGH PA:PITTSBURGH 40183- 50283 50283- 60283 60283- 70583 40183- 50483 50483- 60283 60283- 70583 33183- 51683 51683- 60283 60283- 70583 40183- 50283 50283- 53183 53183- 70683 50983- 71283 40583- 51083 51083- 60883 60883- 70883 40483- 50483 50483- 60183 60183- 70883 40483- 50283 50283- 60383 60383- 71283 40483- 51783 51783- 61683 61683- 71983 33183- 50283 50283- 60283 60283- 63083 41383- 50583 50583- 61583 61583- 71183 40183- 50483 50483- 60183 60183- 70183 41183- 50683 50683- 60683 60683- 70883 40883- 50383 50383- 60283 60283- 71183 33083- 50283 50283- 53183 53183- 70183 40483- 50383 50383- 60383 60383- 70583 5.2 5.3 4.8 6.0 3.8 4.1 15.3 6.4 10.0 4.2 3.8 4.2 17.2 6.3 4.6 4.2 6.4 5.9 7.0 7.2 7.8 8.0 15.0 10.1 9.8 5.2 5.0 4.0 4.3 7.4 3.6 5.4 4.6 4.0 4.5 5.6 5.3 4.7 5.6 5.6 6.0 4.5 3.7 8.1 8.9 7.8 7.0 7.1 6.0 7.5 5.5 5.1 13.9 15.6 12.6 5.6 5.5 4.9 11.2 7.6 6.7 5.8 9.0 8.8 7.8 10.8 10.1 8.6 14.5 14.1 12.4 6.8 6.7 5.9 8.1 7.5 5.8 6.8 6.9 5.6 7.5 7.6 6.9 7.9 7.7 5.9 7.1 6.5 5.0 11.7 12.0 10.2 15.3 15.4 9.0 14.0 10.8 11.7 8.6 5.3 8.1 16.1 8.2 13.8 10.0 28.0 18.8 9.7 5.9 5.1 11.5 4.2 21.0 6.2 20.3 10.1 11.3 12.9 14.2 9.9 7.1 7.8 7.2 4.6 7.3 6.6 8.1 10.8 31.5 9.9 13.0 7.2 17.6 10.2 14.6 7.6 7.0 13.1 38 ------- TABLE 20 (CONTINUED) ENVIRONMENTAL GAMMA AMBIENT MONITORING PROGRAM INTEGRATED EXPOSURE LOCATION DATE RANGE EXPOSURE RATE RI:PROVIDENCE RI:PROVIDENCE RI:PROVIDENCE SC:BARNWELL SC:BARNWELL SC:BARNWELL SC:COLUMBIA SC:COLUMBIA SC:COLUMBIA TN:KNOXVILLE TN:KNOXVILLE TN:KNOXVILLE VA:RICHMOND VA:RICHMOND VT:MONTPELIER VT:MONTPELIER VT:MONTPELIER MR 41283- 51683 51683- 60883 60883- 70783 33183- 50583 50583- 60283 60283- 80583 40183- 50383 50383- 53183 53183- 70183 33083- 50283 50283- 53183 53183- 63083 33183- 60183 60183- 70783 40183- 50683 50683- 60283 60283- 70283 8.2 5.5 6.4 7.0 4.2 9.9 6.6 5.7 6.3 7.3 6.8 5.7 10.5 5.2 6.3 4.7 5.0 MICRO R/HR + 2 s * 10.1 10.0 9.1 8.3 6.2 6.5 8.6 8.5 8.4 9.3 9.7 7.9 7.0 6.0 7.5 7.3 7.0 8.1 4.7 25.1 20.9 14.0 8.2 4.6 22.3 4.6 7.1 .11.5 20.0 6.5 5.4 12.2 7.5 4.9 SIGMA ERROR (IN PERCENT) 39 ------- SECTION IV. Milk Program Pasteurized Milk This is a cooperative program of the EPA, ORP and the Dairy and Lipid Products Branch, Milk Sanitation Section, Food and Drug Administration. Milk is a reliable indicator of the general populations intake of radionuclides since it is consumed by a large segment of the population and contains several of the biologically important contaminants resulting from environmental releases from nuclear activities. A primary function of this program is to obtain reliable monitoring data relative to current radionuclide concentrations and determine any long-term trends. Monthly samples are collected at 65 sampling sites with one or more located in each state, Puerto Rico, and the Panama Canal. These are composite samples representing more than 80 percent of the milk consumed in a given population center. These samples are analyzed for iodine-131, barium-140, cesiura-137, and potassium. All 65 samples are analyzed annually in July for strontium-89, and strontium-90. Also, for the first month of the three quarters beginning January, April and October, 10 regional composite samples of milk made up from the states within each of EPA's 10 regions are analyzed for strontium-89 and strontium-90. Iodine-131, barium-140, cesium-137 and potassium are determined by gamma spectral analysis. Strontium-89 and strontium-90 are determined by beta counting a total strontium precipitate which has been chemically separated by ion-exchange. The values from the pasteurized milk samples for April - June 1983 are shown in Tables 21-23. Strontium values from regional composite samples collected April - June 1983 are shown in Table 24. Tritium In Milk It was previously proposed to analyze all 65 milk samples for tritium in the aqueous and organic phases, on an annual basis (on the April sample). The EERF is currently evaluating alternative analytical techniques anticipating that these analyses will begin during the coming year. 40 ------- TABLE 21 CONCENTRATIONS OF RADIONUCLIDES IN PASTEURIZED MILK APRIL 1983 LOCATION AL:MONTGOMERY AR:LITTLE ROCK AZ:PHOENIX CA:LOS ANGELES CA:SACRAMENTO CA:SAN FRANCISCO CT:HARTFORD DC:WASHINGTON FL:TAMPA GA:ATLANTA HI:HONOLULU IA:DES MOINES ID:IDAHO FALLS IL:CHICAGO IN:INDIANAPOLIS KS:WICHITA KY:LOUISVILLE LA:NEW ORLEANS MA:BOSTON MD:BALTIMORE ME:PORTLAND MI:DETROIT MI:GRAND RAPIDS MN:ST PAUL MOrKANSAS CITY MO:ST LOUIS MS:JACKSON NC:CHARLOTTE ND:MINOT NE:OMAHA NH:MANCHESTER NJ:TRENTON NV:LAS VEGAS NY:BUFFALO NY:NEW YORK CITY NY:SYRACUSE OH:CINCINNATI OH:CLEVELAND OK:OKLAHOMA CITY PA:PHILADELPHIA PA:PITTSBURGH PCrANCON PR:SAN JUAN SC:CHARLESTON DATE COLLECTED 4/ 7/83 4/ 4/83 4/ 8/83 4/11/83 4/ 4/83 4/ 6/83 4/ 3/83 4/ 1/83 4/11/83 4/18/83 4/ 5/83 4/11/83 4/18/83 4/ 4/83 4/ 4/83 4/13/83 4/ 4/83 4/26/83 4/ 5/83 4/ 8/83 4/ 5/83 4/ 7/83 4/ 7/83 4/ 6/83 4/ 8/83 4/ 6/83 4/ 4/83 4/11/83 4/18/83 4/ 8/83 4/ 6/83 4/ 7/83 4/19/83 4/12/83 4/ 4/83 4/ 4/83 4/ 4/83 4/11/83 4/ 4/83 4/ 4/83 4/ 5/83 4/19/83 4/29/83 4/25/83 K g/l+2s 1 1 1 1 1 1 1 1 1 1 1 1 1 0 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 .61 .60 .57 .74 .62 .77 .47 .57 .47 .55 .66 .60 .84 .76 .60 .54 .53 .59 .52 .67 .64 .53 .64 .59 .50 .56 .58 .98 .66 .53 .56 .51 .60 .59 .61 .57 .60 .63 .52 .56 .57 .60 .56 .68 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 .13 .13 .13 .18 .13 .25 .12 .12 .12 .12 .13 .13 .25 .11 .13 .12 .12 .13 .12 .13 .09 .12 .13 .13 .12 .12 .09 .25 .13 .08 .12 .08 .13 .13 .13 .12 .09 .13 .12 .09 .12 .13 .12 .24 137Cs pCi/l+2s 1 4 -4 -11 5 -4 -4 -1 5 5 1 3 6 0 3 7 3 2 6 0 7 1 3 -2 -1 0 3 1 3 0 2 2 4 -1 6 -1 0 0 0 5 3 19 0 -3 7 7 7 11 7 16 7 7 7 7 7 7 16 7 7 7 7 7 7 7 5 7 7 7 7 7 5 16 7 5 7 5 7 7 7 7 5 7 7 5 7 7 7 16 UOBa pCi/l+2s 0 -3 1 11 -1 3 -2 -2 7 0 5 -3 1 0 2 4 1 5 4 2 0 3 -3 3 -1 -5 -3 -6 -4 0 -3 -1 0 4 -2 -8 0 8 -1 0 -4 5 0 9 9 9 9 15 9 20 9 9 9 9 9 9 20 9 9 9 9 9 9 9 6 9 9 9 9 9 6 20 9 6 9 6 9 9 9 9 6 9 9 6 9 9 9 21 131r pCi/l+2s 2 -2 5 -3 1 -8 1 0 -1 2 -6 4 -3 -2 -4 -2 -3 -2 -2 2 2 -1 1 -1 -2 -1 4 -1 3 -2 2 0 -2 0 4 3 3 -5 1 1 1 1 J. -4 -8 7 7 7 10 7 14 7 7 7 7 7 7 14 7 7 7 7 7 7 7 5 7 7 7 7 7 5 14 7 5 7 5 7 7 7 7 5 7 7 5 7 / 7 / 7 14 41 ------- TABLE 21 (CONTINUED) CONCENTRATIONS OF RADIONUCLIDES IN PASTEURIZED MILK APRIL 1983 LOCATION SD:RAPID CITY TN:CHATTANOOGA TN:KNOXVILLE TX:AUSTIN UT:SALT LAKE CITY VA:NORFOLK VT:BURLINGTON WA:SEATTLE WA: SPOKANE WV:CHARLESTON WY:LARAMIE DATE COLLECTED 4/ 5/83 4/ 4/83 4/11/83 4/ 6/83 4/ 4/83 4/20/83 4/11/83 4/ 4/83 4/ 3/83 4/11/83 4/ 4/83 K g/l+2s 1 1 1 1 1 1 1 1 1 1 1 .49 .50 .46 .60 .67 .59 .59 .51 .73 .62 .58 0 0 0 0 0 0 0 0 0 0 0 .12 .12 .12 .09 .09 .13 .24 .12 .17 .13 .13 137 140™ u/Cs 1HUBa pCi/l+2s -2 1 6 0 5 -3 7 3 3 0 2 7 7 7 5 5 7 16 7 11 7 7 pCi/l+2s -1 2 -2 -5 5 -1 8 -1 7 3 -2 9 9 9 6 6 9 20 9 15 9 9 13 lt pCi/l+2s 1 -1 0 2 1 -1 -4 -1 4 -3 ~2 7 7 7 5 5 7 14 7 10 7 7 SIGMA COUNTING ERROR 42 ------- TABLE 22 CONCENTRATIONS OF RADIONUCLIDES IN PASTEURIZED MILK MAY 1983 LOCATION AL:MONTGOMERY AR:LITTLE ROCK AZ:PHOENIX CA:LOS ANGELES CA:SACRAMENTO COrDENVER COrDENVER CT:HARTFORD DC:WASHINGTON GA:ATLANTA HI:HONOLULU IA:DES MOINES ID:IDAHO FALLS IL:CHICAGO IN:INDIANAPOLIS KS:WICHITA KY:LOUISVILLE LA:NEW ORLEANS MA:BOSTON MD:BALTIMORE ME:PORTLAND MI:DETROIT MI:GRAND RAPIDS MN:MINNEAPOLIS MN:ST PAUL MO:KANSAS CITY MO:ST LOUIS MS:JACKSON NC:CHARLOTTE ND:MINOT NE:OMAHA NH: CONCORD NJ:TRENTON NM:ALBUQUERQUE NY:BUFFALO NY:NEW YORK CITY NY:SYRACUSE OH CINCINNATI OH:CLEVELAND OR:PORTLAND PA PHILADELPHIA PA PITTSBURGH PC:CRISTOBAL PR:SAN JUAN DATE COLLECTED 5/ 5/83 5/ 2/83 5/ 5/83 5/12/83 5/ 4/83 5/31/83 5/ 1/83 5/ 2/83 5/ 6/83 5/ 4/83 5/ 3/83 5/ 9/83 51 4/83 5/ 2/83 5/ 9/83 5/ 5/83 5/ 3/83 5/12/83 5/ 2/83 5/ 6/83 5/ 3/83 5/ 5/83 5/ 3/83 5/ 2/83 5/ 3/83 5/ 6/83 5/ 4/83 5/17/83 5/ 2/83 5/ 2/83 5/ 6/83 5/ 2/83 5/ 5/83 5/ 2/83 5/ 9/83 5/ 1/83 5/ 4/83 5/ 2/83 5/ 9/83 5/ 2/83 5/ 2/83 5/ 4/83 5/23/83 5/19/83 K g/l+2s 1.56 1.57 1.50 1.53 1.53 1.50 1.59 1.54 1.57 1.49 1.65 1.62 1.80 1.51 1.55 1.55 1.55 1.57 1.46 1.65 1.59 1.48 1.58 1.59 1.57 1.63 1.47 1.55 1.73 1.64 1.50 1.71 1.52 1.60 1.65 1.50 1.59 1.48 1.46 1.65 1.53 1.56 1.46 1.54 0.09 0.12 0.08 0.12 0.12 0.12 0.13 0.09 0.09 0.12 0.13 0.13 0.25 0.12 0.12 0.08 0.12 0.09 0.12 0.13 0.13 0.12 0.13 0.09 0.13 0.13 0.12 0.12 0.25 0.13 0.12 0.13 0.12 0.13 0.13 0.12 0.13 0.12 0.12 0.13 0.12 0.12 0.12 0.08 j.j / Cs pCi/l+2s 4 2 0 0 -3 5 1 3 0 3 5 3 -6 7 5 4 1 0 0 2 5 -2 3 2 -3 -4 1 4 9 0 -4 -4 5 -1 -3 5 3 0 5 0 1 0 14 0 5 7 5 7 7 7 7 5 5 7 7 7 16 7 7 5 7 5 7 7 7 7 7 5 7 7 7 7 16 7 7 7 7 7 7 7 7 7 7 7 7 7 7 5 J-tV. Ba pCi/l+2s -2 -4 -2 -2 2 2 -1 1 0 -6 -1 -1 3 0 1 -2 -3 2 -2 -6 -1 0 7 2 4 1 0 2 -2 -1 5 0 -2 -1 -2 4 -2 -3 1 1 -2 -5 1 -1 6 9 6 9 9 9 9 6 6 9 9 9 20 9 - 9 6 9 6 9 9 9 9 9 6 9 9 9 9 20 9 9 9 9 9 9 9 9 9 9 9 9 9 9 6 j.-» i I pCi/l+2s -2 1 0 -3 -2 — 1 2 -1 -1 5 1 0 -11 1 0 0 3 2 1 -3 1 1 -1 -2 -3 -3 -1 -2 -3 -2 -7 -1 2 3 3 -6 3 3 0 -1 -2 2 -5 -3 5 7 5 7 7 7 7 5 5 7 7 7 14 7 7 5 7 5 7 7 7 7 7 5 7 7 7 7 14 7 7 7 7 7 7 7 7 7 7 7 7 7 7 5 43 ------- TABLE 22 (CONTINUED) CONCENTRATIONS OF RADIONUCLIDES IN PASTEURIZED MILK MAY 1983 LOCATION SC:CHARLESTON SD:RAPID CITY TN:CHATTANOOGA TN.-KNOXVILLE TN:MEMPHIS TNrMEMPHIS TX:AUSTIN UTrSALT LAKE CITY VA:NORFOLK VT:BURLINGTON WA:SEATTLE WA:SPOKANE WV:CHARLESTON WYrLARAMIE DATE COLLECTED 5/18/83 5/ 5/83 5/ 2/83 5/ 9/83 5/ 1/83 5/26/83 5/ 5/83 5/ 1/83 5/20/83 5/ 5/83 5/ 2/83 5/ 1/83 5/16/83 5/ 2/83 K g/l+2s 1 1 1 1 1 1 1 1 1 1 1 1 1 1 .60 .60 .51 .58 .46 .57 .79 .56 .59 .74 .72 .50 .51 .50 0 0 0 0 0 o 0 0 0 0 0 0 0 0 .13 .13 .12 .13 .12 .12 .25 .12 .13 .13 .17 .12 .12 .08 137Cs pCi/l+2s 7 2 1 1 5 5 10 3 0 4 -4 2 -3 2 7 7 7 7 7 7 16 7 7 7 11 7 7 5 140Ba pCi/l+2s 2 ~5 -2 0 0 -7 3 -4 -2 -2 3 2 -6 -2 9 9 9 9 9 9 20 9 9 9 14 9 9 6 131j pCi/l+2s -5 -2 2 -3 -3 3 -10 1 -2 -3 -3 2 0 1 7 7 7 7 7 7 14 7 7 7 10 7 7 5 SIGMA COUNTING ERROR 44 ------- TABLE 23 CONCENTRATIONS OF RADIONUCLIDES IN PASTEURIZED MILK JUNE 1983 LOCATION AL:MONTGOMERY AR:LITTLE ROCK AZ:PHOENIX CArLOS ANGELES CA:SACRAMENTO CA:SAN FRANCISCO CO:DENVER CO:DENVER CT:HARTFORD DC:WASHINGTON GA:ATLANTA GA: ATT, ANT A HI .-HONOLULU IA:DES MOINES ID:IDAHO FALLS IL:CHICAGO IN:INDIANAPOLIS KS:WICHITA KYrLOUISVILLE LA:NEW ORLEANS MA:BOSTON MD: BALTIMORE ME:PORTLAND MI:DETROIT MIrGRAND RAPIDS MN:MINNEAPOLIS MN:ST PAUL MO:KANSAS CITY MO:ST LOUIS MS:JACKSON MT:HELENA NC:CHARLOTTE ND:MINOT NE:OMAHA NH:MANCHESTER NJ:TRENTON NVrLAS VEGAS NY:BUFFALO NY:NEW YORK CITY NY:SYRACUSE OH:CINCINNATI OH:CLEVELAND OK:OKLAHOMA CITY OR:PORTLAND DATE COLLECTED 6/ 9/83 6/ 6/83 6/ 8/83 6/ 8/83 6/ 2/83 6/ 2/83 5/31/83 6/28/83 6/ 6/83 6/ 3/83 11 1/83 6/ 1/83 6/ 9/83 6/ 6/83 6/ 9/83 6/ 6/83 6/ 6/83 6/ 6/83 6/ 6/83 6/ 7/83 6/ 7/83 6/ 3/83 6/ 7/83 6/ 9/83 6/ 6/83 6/ 6/83 6/ 1/83 6/10/83 6/ 8/83 6/ 6/83 6/ 6/83 6/ 6/83 6/20/83 6/10/83 6/ 6/83 6/ 6/83 6/ 6/83 6/13/83 6/ 6/83 6/ 6/83 6/ 6/83 6/ 7/83 6/ 6/83 6/ 6/83 K g/l+2s 1 1 1 1 1 1 1 1 1 1 1 1 1 1 2 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 .46 .55 .61 .77 .64 .53 .50 .43 .56 .56 .66 .53 .57 .56 .01 .59 .52 .55 .57 .46 .68 .58 .63 .55 .54 .73 .54 .48 .50 .58 .58 .60 .58 .31 .53 .58 .63 .57 .65 .57 .65 .61 .68 .53 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 .12 .08 .09 .25 .09 .12 .12 .12 .12 .12 .24 .08 .12 .09 .25 .13 .12 .12 .12 .12 .13 .13 .13 .12 .12 .13 .09 .12 .12 .13 .09 .24 .12 .12 .12 .13 .13 .13 0.13 0.08 0.24 0.13 0.13 0.06 137P 140D Cs Ba pCi/l+2s 1 3 0 -5 0 -1 5 -2 5 9 -2 -1 9 2 3 -1 -1 5 -3 9 2 -1 4 4 -2 1 4 -1 0 4 0 -3 0 1 2 1 -1 0 3 0 5 2 0 1 7 5 5 16 5 7 7 7 7 7 16 5 7 5 16 7 7 7 7 7 7 7 7 7 7 7 5 7 7 7 5 16 7 7 7 7 7 7 7 5 16 7 7 4 pCi/l+2s 2 -2 0 0 -2 -3 2 -1 -3 -2 -9 0 -1 2 -7 -1 0 0 0 -3 0 6 -5 -3 2 -3 -4 -3 1 -2 -6 12 -2 -4 -3 2 -4 2 -6 -4 -3 -1 -1 0 9 6 6 20 6 9 9 9 9 9 20 5 9 6 20 9 9 9 9 9 9 9 9 9 9 9 6 9 9 9 6 21 9 9 9 9 9 9 9 6 20 9 9 5 131I pCi/l+2s -3 -2 -2 5 4 -1 -7 -2 £> 1 -4 7 1 1 -2 -1 J_ -3 -1 A. -2 o -2 5 2 4 0 -2 2 -11 -2 -4 -2 -1 0 -2 2 2 -4 -8 -2 -3 7 5 5 14 5 _/ 7 7 / 7 7 / 7 14 c J 7 I 5 14 7 7 / 7 / 7 7 i 7 7 i 7 7 7 7 5 7 7 7 5 14 7 7 7 7 7 7 7 5 14 7 7 4 45 ------- TABLE 23 (CONTINUED) CONCENTRATIONS OF RADIONUCLIDES IN PASTEURIZED MILK JUNE 1983 LOCATION PA:PHILADELPHIA PArPITTSBURGH PC:CRISTOBAL PR:SAN JUAN SC:CHARLESTON SD:RAPID CITY TN:CHATTANOOGA TN:KNOXVILLE TN:MEMPHIS TXrAUSTIN UT:SALT LAKE CITY VA:NORFOLK VT:BURLINGTON WA:SEATTLE WA:SEATTLE WA:SPOKANE WI:MILWAUKEE WI:MILWAUKEE WV:CHARLESTON WYtLARAMIE DATE COLLECTED 6/ 6/83 6/ 7/83 6/ 6/83 6/16/83 6/15/83 6/30/83 6/ 6/83 6/20/83 6/29/83 6/ 6/83 6/ 6/83 6/15/83 6/13/83 6/ 6/83 11 1/83 6/ 6/83 6/ 1/83 7/ 1/83 6/28/83 6/ 6/83 K g/l±2s 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 .46 .59 .59 .61 .66 .60 .52 .72 .43 .61 .65 .62 .53 .52 .52 .58 .70 .56 .48 .45 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 .12 .13 .13 .13 .13 .13 .12 .24 .12 .13 .13 .13 .08 .12 .12 .13 .13 .09 .12 .12 137Cs pCi/l+2s 3 0 20 4 -1 -3 -1 1 — 1 -2 4 5 4 2 -2 -1 1 -1 0 5 7 7 7 7 7 7 7 16 7 7 7 7 5 7 7 7 7 5 7 7 UOBa pCi/l+2s 3 -4 0 -2 -6 3 6 -5 -4 5 -8 -1 -1 -5 -1 0 -8 0 -8 -1 9 9 9 9 9 9 9 20 9 9 9 9 6 9 9 9 9 6 9 9 131j pCi/l+2s -6 0 •"1 0 4 -3 -5 -6 -1 -8 2 -2 0 0 -6 -2 -2 -3 -3 -3 7 7 7 7 7 7 7 14 7 7 7 7 5 7 7 7 7 5 7 7 SIGMA COUNTING ERROR 46 ------- TABLE 24 STRONTIUM-90 AND STRONTIUM-89 IN PASTEURIZED MILK EPA REGIONAL COMPOSITES APRIL - JUNE 1983 EPA Sr Sr REGION pCi/1 + 2s pCi/1 + 2s* I 3.1 0.4 -1 1 II 2.3 0.7 1 2 III 3.3 1.0 -1 3 IV 3.3 1.0 -2 3 V 2.9 1.2 0 4 VI 3.1 0.9 0 3 VII 2.0 0.5 1 1 VIII 2.3 0.5 0 1 IX 0.7 0.3 1 1 X 2.0 0.6 2 2 SIGMA COUNTING ERROR ANALYTICAL ERROR TERM WHICH CLOSELY APPROXIMATES THE COUNTING ERROR 47 ------- Carbon-14 in Milk Nine stations, chosen for wide geographical distribution, contribute milk samples for annual analysis for carbon-14. These samples have monitored the carbon-14 levels in the food chain resulting from nuclear testing. Analysis consists of combusting the samples and measuring released carbon dioxide through liquid scintillation. Data will be published as it becomes available. 48 ------- DATA - STATE AGENCIES Radiological Healtli Laboratory^ Indiana State Board of Health Indiana Milk Analysis Program In order to evaluate the fallout on Indiana pasturelands, the State has implemented a program whereby monthly milk samples from five geographical areas are sent to the Radiological Health Laboratory of the State Board of Health. The milk in these samples is bottled on the same date in all five areas to provide uniform time from pasture to the lab. Once in the laboratory, the milk is first analyzed by gamma spectroscopy for iodine-131, barium-140, cesium-137, and potassiura-40. A one gallon sample is analyzed on a 3" x 3" Nal(Tl) scintillation crystal for 4800 seconds. A background sample of 48,000 seconds is also run. The data are analyzed to give pCi/1 for each radionuclide. A quarterly composite sample is saved and run for strontium-89 and -90 by ion exchange method. Data will be published as it is received. 49 ------- Radiological Health_ Division State Hygienic Laboratory of_ Iowa Iowa Water Sampling Program The radiological Health Division of the State Hygienic Laboratory of Iowa with the assistance of the State Department of Environmental Quality (DEQ) maintains a state-wide water sampling program of community drinking waters, surface waters and precipitation. All analyses with the exception of the sequential Ra-226, -228 analyses are performed according to "Standard Methods for the Examination of Water and Wastewater", 14th edition. The sequential analyses for radiums are performed according to the EPA publication, EPA-600/4-75-008, "Interim Radiochemical Methodology for Drinking Water." The drinking water samples are collected by DEQ regional personnel and sent to the State Hygienic Laboratory where they are preserved with HC1. These waters are analyzed for gross alpha and gross beta radioactivity as a screening process. Subsequent analyses for Ra-226, Ra-228, Sr-90 are performed if screening levels are exceeded. Radium levels are of primary concern in Iowa drinking waters as those levels are elevated in deep geologic aquifers within the state. Surface waters are collected at eleven sites throughout the state with site selection being determined by proximity upstream and downstream to nuclear power plants in Iowa or those plants discharging into rivers which are natural borders with adjoining states. Gross alpha, gross beta, and tritium are the routine radionuclide analyses for these samples. Strontium is of interest when gross beta screening levels are exceeded or if nuclear weapons testing necessitates monitoring to determine its impact on the environment. Data will be published as it is received. 50 ------- ENVIRONMENTAL RADIATION DATA (ERD) is published quarterly (January, April, July, October) by the U. S. Environmental Protection Agency's office of Radiation Programs. Requests for information concerning publication and distribution of ERD should be directed to: Charles M. Petko Technical Support Branch Eastern Environmental Radiation Facility P. 0. Box 3009 Montgomery, Alabama 36193 Requests for information concerning the operation of ERAMS should be directed to: H. Michael Mardis, Chief Monitoring and Analytical Services Branch Eastern Environmental Radiation Facility P. 0. Box 3009 Montgomery, Alabama 36193 or to: Lewis Battist, Chief Environmental Studies and Statistics Analysis and Support Division (ANR-461) IT- R. Environmental Protection Agency Waterside Kail East 401 M Street, SW Washington, DC 20460 *** ------- |