EPA 520/5-73-007
        AN  INTEGRATING DEVICE FOR  USE WITH
         PRESSURIZED IONIZATION CHAMBERS
U.S. ENVIRONMENTAL PROTECTION AGENCY

   Offici of Ridiition Progtimi

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                                          EPA 520/5-73-007
AN INTEGRATING DEVICE FOR  USE WITH
PRESSURIZED  IONIZATION  CHAMBERS
                S. T. Windham
               J. E.  Partridge
      Eastern Environmental Radiation Facility
                P. 0. Box 3009
           Montgomery, Alabama 36109

                K. L. Kelley
     National Environmental Research Center
               P. 0.  Box 15027
           Las Vegas, Nevada 89114
                December 1973
        ENVIRONMENTAL PROTECTION AGENCY
          Office of Radiation Programs
             Waterside Mall East
             401 M Street, S. W.
           Washington, D. C. 20460

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The  mention of commercial products,  their source,
or their  use in  connection with material  reported
herein is  not to be construed  as  either an  actual
or implied endorsement of such products  by the
U. S. Environmental Protection  Agency.

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                                  PREFACE
      The Eastern Environmental Radiation Facility participates in the identification
of solutions to problem areas as defined by the Office of Radiation Programs. The
Facility  provides laboratory  capability for evaluation and assessment of radiation
sources through environmental  studies and surveillance and analysis. The  EERF
provides technical assistance  to  the State and local health  departments in  their
radiological health programs  and  provides special  laboratory support for EPA
Regional Offices and other federal governmen^ageiicies as requested.
                                         Charles R. Porter
                                          Acting  Director
                          Eastern  Environmental Radiation Facility

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                An  Integrating  Device for Use with  Pressurized
                            lonization Chambers
Introduction

      The proposed AEC Regulation  10CFR50 Appendix  I limits radiation dose
equivalent at the site boundary of light water power reactors to a maximum of 5
millirem  per  year (mrem/yr) above  natural background. A dose equivalent of 5
mrem/yr added to a natural background dose equivalent of 100-120 mrem/yr is
virtually impossible  to measure using  monitoring devices such as film badges or
thermoluminescent dosimeters. The Health and Safety Laboratory (HASL) of the U.
S. Atomic Energy Commission describes  in HASL-260 a high pressure ionization
chamber designed to accurately measure ambient environmental radiation exposure
rates. A commercial instrument similar to the HASL chamber is now available from
Reuter Stokes (Model RSS-111). This instrument has gained  rather  widespread
acceptance in the nuclear power field. Several of the instruments have been used by
the EERF for over a year with very satisfactory results.

      The basic RSS-111 pressurized ionization chamber (PIC) as marketed by Reuter
Stokes is equipped with a panel meter  readout and a strip chart recorder. For short-
term  or real  time  measurements these forms of data presentation  are entirely
satisfactory. However, for long-term field monitoring which we routinely perform for
periods from 1-3 months duration, visual reduction of the voluminous strip chart data
using a planimeter is quite time consuming. An optional magnetic tape recorder is
to be offered by Reuter Stokes. After storing data the magnetic tape is read into a
computer for data processing. This system of data handling, however, is  rather
expensive (~ $4,000) and it requires the user to have a computer available for data
retrieval.

      As an option to the readout methods described above, the EERF has adapted
a low cost, commercially available integrator module to work in conjunction with the
recorder and panel meter which are standard on the RSS-111, making a very versatile
arrangement. The  integrator may  be  disengaged  when  real-time or short-term
measurements only are necessary. When using the integrator in conjunction with the
strip chart recorder for long-term measurements, the readouts provide total exposure,
and the time and exposure rates of intermittent exposures. This report describes the
integrator and provides details for its use in conjunction with RSS-111.

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 2

 General Description

       The integrator adapted for use with the RSS-111 is manufactured by Curtis
 Instruments, Inc. Integration of current is performed with a mercury microcoulometer.

       The microcoulometer consists of a glass capillary tube containing two columns
 of mercury separated by an electrolyte. Wire electrodes are inserted into the mercury
 columns through the ends of the capillary for electrical connection (Figure 1).
 When a direct current is passed through the coulometer, mercury is deposited across
 the electrolyte gap which causes the gap to move toward the anode. The movement
 of the electrolyte is directly proportional to the current/time integral.*

       A metal sheath is positioned around the exterior of the capillary such that the
 length of either mercury columns can be determined electronically by measuring the
 capacitance between the sheath and the column of mercury, which varies in length
 as the gap moves.

       Unlike electronic integration which  depends upon the state-of-charge  of a
 capacitor, the mercury microcoulometer does not undergo leakage and loss of  data
 over a long storage period. This characteristic is very important since  long-term
 integration with maximum stability is essential in this application.

       It was desired to  obtain an integrator which would require no electronic
 modifications to the RSS-111.  After learning of our specific  requirements, Curtis
 mstruments was able to produce a unit which was compatible with the  RSS-111.
 Ranges of current to be integrated, type of  data readout, and characteristics of the
 RSS-111 were taken into account when adapting the integrator for our application.

       Data from the integrator are presented on two devices, a panel meter and a
 mechanical register. As current flows and the electrolyte gap moves in the capillary
 its position  is indicated on the panel meter. Total range movement of the  gap
 corresponds to full scale deflection of the meter and to an integrated exposure of 50
 microroentgens, depending on the calibration. When the electrolyte gap reaches the
 end of its travel the  polarity of the electrodes is automatically reversed, the panel
 meter is reset to zero, and one count is registered on the mechanical register. For each
 50 microroentgens exposure  integrated, one count will be recorded. Thus, with a
 mechanical register having five decades, it is possible to integrate large exposures
over a  long period of time with no data overflow and at the same time very small
exposures are easily  and accurately recorded.
* C.C. Beusman, "Electrochemical Devices for Timing and Switching Applications,"
IEEE International  Convention Record, March 1964.

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                        Figure 1.   Mercury Microcoulometer
                 MERCURY COLUMNS
METAL SHEATH
                           ELECTROLYTE GAP
                                                     ELECTRODE
 Installation

       In keeping with our desire to perform no electronic modifications to the RSS-
 111, the integrator derives its input signal from the output jacks which are present
 on the front panel of the RSS-111. Power to operate the integrator ±  12 volts  DC,
 is obtained from the RSS-111, however, to obtain (+) 12 volts with respect to ground
 it is  necessary to ground the negative side of the recorder motor supply. This is the
 only modification  necessary to the RSS-111, and it  does not  detract from  the
 instrument's independent performance in any way.

       The RSS-111 is designed to operate from 110 volts AC or from an internal,
 rechargeable battery pack for up to 200 hours. The integrator, however, requires too
 much current to operate from this battery pack for extended periods, and for this
 reason the integrator is designed to operate from 110 volts AC only. The RSS-111,
 when operating from 110 volts AC, will automatically  switch to the battery pack
 power supply should the AC source be interrupted. During field testing  of  the
 integrator it was found that when this automatic changeover occurs and the integrator
 is no longer receiving its ±12 volt DC supply voltage (due to excess battery drain)
 damage will occur-to the integrator. This damage occurs since the signal from  the
 RSS-111 is still present and driving the coulometer, however the  polarity reversing
 circuitry is inoperative thus driving the coulometer beyond its capacity. This may be
 prevented by using  a three pole relay as shown in (Figure 2). When 110 volts AC is
not present, the supply voltages and signal are disconnected from the integrator.

      Two versions of the integrator have been obtained from Curtis Instruments.
In the first version which cost $425, the integrator circuitry and readout units are all

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mounted within a metal case (Figure 3). Signal and power connections to the RSS-111
are made using appropriate cables from a terminal strip on the back of the integrator
case. This version  is quite easy  to put into operation  and requires no  major
modifications to the RSS-1 1 1. Also, this arrangement allows the integrator to be used
alternately with several PIC's since it is easily connected  and disconnected through
the use of jacks on the front panel of the PIC.

       In the second version of the integrator, which cost  $380, the components are
supplied without a case. These components include a printed circuit board, a panel
meter, and a mechanical register  (Figure 4). These  components  can be installed
directly in the case of the PIC, (Figure 5). This arrangement produces a very compact
and rugged arrangement. Both versions work equally well.
 110 VOLT AC RELAY
                 110 VAC
  ENERGIZED
-+12 VDC SOURCE

-+12 VDC TO INTEGRATOR

--12 VDC SOURCE

 -12 VDC TO INTEGRATOR

  SIGNAL FROM FRONT PANEL JACKS

-  SIGNAL TO INTEGRATOR
                                                             Figure  2.
                                                             Protective
                                                             Circuit  for
                                                             Integrator
      Figure 3.
      Integrator Mounted
      in  External Case

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                                                          Figure 4.
                                                          Components
                                                          of Integrator
          Figure  5.  Components
          Installed in  PIC Case
Laboratory Calibration

       Prior to use  of the  integrator it is necessary to establish  the  exposure
relationship between the  recorder and the integrator. It is assumed that the recorder
has been previously  calibrated either by  Reuter  Stokes or by the user. A high
resolution potentiometer  is provided on the integrator so that it can be adjusted to
minimize the scaling error between the recorder and the integrator proper adjustment
5 the potentiometer, following the  instructions provided by  Curt.s Instruments,
should result in errors less than ± It%.

       Having made this  adjustment the error may be determined in the laboratory
by using a small radioactive source to expose the ionizati^n  chamber at a cor
rate wUh both the recorder and the integrator operating. The total exposure should
be a  least several hundred  microroentgens. At the  end of the exposure penod  the

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6

"true" exposure is determined by integrating the area under the curve produced by'
the recorder. This may then be compared to the integrator readout which should be
the same if the scaling adjustment is correctly set.

Field Testing

      Testing in the field has provided comparative results between the recorder and
the integrator. Tests were run at exposure rates ranging from 6 microroentgens/hour
up to 165  microroentgens/hour and for both short and long  integration periods.
Results of these tests are presented  in Table 1.

          Table 1.  Comparison of  Total Exposures  as  Determined
                   by the Recorder  and by the  Integrator
                               in  Field  Tests
             Integration  of                Integrator              Percent
   Test       Recorder  Tape                 Reading             Difference
           (microroentgens)            (microroentgens)

     1             1271                     1295                 1.9%
     2             1465                     1411                 2.7%
     3             3048                     3035                 0.4%
     4             1645                     1655                 0.6%
     5             1236                     1250                 1.1%
     6             1226                     1237                 0.9%

      Differences between the recorder and the integrator are seen to be quite small.
A likely source of these differences arises from the inaccuracy of using a planimeter
on a long recorder tape.
Summary

      The integrator described has been used with good results and no malfunctions.
The low cost makes the integrator particularly appealing compared to other methods
of data  integration which  are available. No major modifications to the RSS-111
ionization chamber are required for use of the integrator.

      Field and laboratory testing of the integrator have shown the  unit to produce
good results at both high and low exposure rates for extended periods of time.

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. REPORT NO.
EPA-520/5-73-007
                                   TECHNICAL REPORT DATA
                           (Please read Instructions on the reverse before completing)

                             \2.
            3. RECIPIENT'S ACCESSION-NO.
. TITLE AND SUBTITLE

AN INTEGRATING  DEVICE FOR USE WITH  PRESSURIZED
   IONIZATION CHAMBERS
            5. REPORT DATE^
              December 1973
            6. PERFORMING ORGANIZATION CODE
 AUTHOR(S)
                                                           8. PERFORMING ORGANIZATION REPORT NO.
 S.  T. Windham,  J.  E. Partridge,  H.  L.  Kelley
. PERFORMING ORG \NIZATION NAME AND ADDRESS
Office of Radiation Programs
 Eastern Environmental Radiation  Facility
 P. 0. Box 3009
 Montgomery, AL  36109
 2. SPONSORING AGENCY NAME AND ADDRESS


 Same as #9
             10. PROGRAM ELEMENT NO,
                  2F6120
             11. CONTRACT/GRANT NO.
             13 TYPE OF REPORT AND PERIOD COVERED
                   Final
             14. SPONSORING AGENCY CODE
15. SUPPLEMENTARY NOTES
16. ABSTRACT
   integrating  th^area under a  lengthy strip chart curve.

        Use  of  the integrator with  the RSS-111 is quite simple and requires
         •5!  mLJfiration of the  ionization chamber.   Field  and laboratory  tests
   Sf Se0in?egrIlSr  ave"shown   t  to produce consistent results over both short
   and long  integration times, and  at both high and low exposure rates.
17.
                                KEY WORDS AND DOCUMENT ANALYSIS
   - electronic circuit
   - exposure integrator
18. DISTRIBUTION STATEMEN I
        Release Unlimited
       .——.«•—
EPA Form 2220-1 (9-73)
 - PIC integrator  .  .  .
 - integrating environ-
     mental radiation
     levels .  .  .
19. SECURITY CLASS (ThisReport)
   unclassified
20. SECURITY CLASS (TMS page)
   unclassified
                                              b.lDENTIFIERS/OPEN ENDED TERMS
18.  Nuclear
     Science &
     Technology

 D.  Nuclear
     Instrumenta
   	:ion
21. NO, OF PAGES
       14

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