EPA-450/3-76-028b
December 1976
                      OPEN SPACE
                              AS AN
                   AIR RESOURCE
       MANAGEMENT MEASURE
VOLUME II: DESIGN CRITERIA
  U.S. ENVIRONMENTAL PROTECTION AGENCY
      Office of Air and Waste Management
   Office of Air Quality Planning and Standards
   Research Triangle Park, North Carolina 27711

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                                  EPA-450/3-76-028b
              OPEN SPACE
                   AS AN
            AIR RESOURCE
     MANAGEMENT MEASURE
VOLUME II:  DESIGN CRITERIA
                      by
           R.S. DeSanto, R.A. Glaser, W.P. McMillen,
              K.A. MacGregor, and J.A. Miller

                 COMSIS Corporation
                972 New London Turnpike
              ClaBlonbury, Connecticut 06033
                 Contract No. 6842-2350
            EPA Project Officer: Thomas McCurdy
                   Prepared for

          ENVIRONMENTAL PROTECTION AGENCY
            Office of Air and Waste Management
          Office of Air Quality Planning and Standards
          Research Triangle Park, North Carolina 27711

                   December 1976

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This report is issued by the Environmental Protection Agency to report
technical data of interest to a limited number of readers.  Copies are
available free of charge to Federal employees, current contractors and
grantees, and nonprofit organizations - in limited quantities - from the
Library Services Office (MD35), Research Triangle Park, North Carolina
27711;  or,  for a fee, from the National Technical Information Service,
5285 Port Royal Road, Springfield, Virginia 22161.
This report was furnished to the Environmental Protection Agency by
COMSIS Corporation, Glastonbury,  Connecticut 06033, in fulfillment
of Contract No. 68-02-2350.  The contents of this report are reproduced
herein as received from COMSIS Corporation.  The opinions,  findings,
and conclusions expressed are those of the author and not necessarily
those of the Environmental Protection Agency. Mention of company or
product names is not to be considered as an endorsement by the Environ-
mental Protection Agency.
                    Publication No. EPA-450/3-76-028b
                                    11

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                              ACKNOWLEDGEMENTS


We wish to thank Mr.  Thomas McCurdy,  the E.P.A.  project officer for this  study,
whose assistance and  advice was  most  valuable and greatly appreciated.
                                  STAFFING


Dr. Robert S. DeSanto was project manager and principal investigator for  this
study at COMSIS CORPORATION - Environmental Services.   Mr.  Richard A. Glaser,
of David A. Crane and Partners,  provided interpretations of the literature from
the point of view of the landscape architect.  He also provided all illustrative
material with the exception of the electron micrographs which were provided by
Dr. William H. Smith of the Yale University School of  Forestry and Environmental
Studies.  Mr. William P. McMillen and Mr. Kenneth A. MacGregor of COMSIS  CORPORATION
assisted in all aspects of this  study providing engineering and planning  overviews
and writing much of the text.  Dr. Joseph A. Miller, Head Librarian at Yale
University School of Forestry and Environmental Studies, executed all library
services and guided the numerous processing operations required for document delivery.

Ms. Dana Pumphrey of COMSIS CORPORATION assisted at all levels in the preparation
of the report.  Her help was broad and very important.

Mrs.  Joy Maxfield typed the manuscript entirely alone.  Her accuracy and  her
stamina were important to us and to our successful completion of this Volume.
We are grateful to her for her support.
                                      iii

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                                 •TABLE OF CONTENTS

Chapter                                Title                          Page



          LIST OF FIGURES	     v

          LIST OF TABLES	     viii

I         INTRODUCTION, APPROACH AND SUMMARY OF RESULTS 	     1-1

          A.  INTRODUCTION AND ORGANIZATION OF THE REPORT ....     1-1
          B.  SUMMARY OF THE RESULTS	     1-4

II        HIGHWAY BUFFER AND RELATED OPEN SPACE 	     II-1

          A.  POLLUTANT IDENTIFICATION	     II-1
              1.  Source Emissions  	     II-1
              2.  Transport Mechanisms  . . . . *	     II-5
              3.  Atmospheric Diffusion 	     11-10
          B.  LITERATURE SEARCH FINDINGS  	     11-18
          C.  POTENTIAL DESIGN ALTERNATIVES 	     11-42
              1.  Summary of Literature Search Findings 	     11-42
              2.  Design Configurations 	     11-54

III       REGIONAL OPEN SPACE	     III-l

          A.  POLLUTANT IDENTIFICATION	     III-l
              1.  Source Emissions   	     III-3
              2.  Pollutant Removal  	     111-12
          B.  LITERATURE SEARCH FINDINGS	     Ill-17
          C.  LAND USE/GREEN BELT ORGANIZATION  	     111-22
          D.  CONVERSION OF LEAF AREA TO GROUND AREA AND
                 WEIGHTED SINK FACTORS  	     111-28

IV        GLOSSARY	     IV-1

V         BIBLIOGRAPHY  	      V-l

VI        APPENDIX	    VI-1

          A.  HIGHWAY DIFFUSION MODELS  	    VI-1
          B.  SENSITIVE SPECIES LIST	    VI-20
          C.  CALCULATION OF LEAF AREAS FOR SELECTED TREES  ....    VI-46
          D.  HOLLAND STACK RISE EQUATION	    VI-52
                                         iv

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                                 TABLE OF FIGURES
Figure                                Title                           Page

1-1       SCANNING ELECTRON MICROGRAPH OF THE ADAXIAL SURFACE
            OF A LONDON PLANETREE LEAF...      	    1-5

1-2       SCANNING ELECTRON MICROGRAPH OF AGGREGATE PARTICLES ON
            THE ADAXIAL SURFACE OF A LONDON PLANTREE LEAF	    1-6

1-3       SCANNING ELECTRON MICROGRAPH OF A TRICHOME ON THE
            ADAXIAL SURFACE OF A LONDON PLANETREE LEAF...     ...    1-7

1-4       SCANNING ELECTRON MICROGRAPH OF AGGREGATE PARTICLE
            BLOCKING A STOMATE OF A LONDON PLANETREE LEAF	    1-8

1-5       SCANNING ELECTRON MICROGRAPH OF SUB-MICROMETER PARTICLES
            ON THE SURFACE OF A LONDON PLANETREE LEAF
            TRICHOME...     	    1-9

1-6       SCANNING ELECTRON MICROGRAPH OF POLLEN AND FUNGI ON THE
            ADAXIAL SURFACE OF A LONDON PLANETREE LEAF...     ...    I-10

II-1      THE INFLUENCE OF WIND SPEED ON GROUND LEVEL POLLUTANT
            CONCENTRATIONS	    II-6

I1-2      SOIL LEVEL OF LEAD QUEEN'S PARK AND SOIL LEVEL OF
            CADMIUM QUEEN'S PARK	    II-8

II-3      LEAD CONTAMINATION OF WHITE PINE TWIGS PLUS NEEDLES
            SAMPLED FROM TREES GROWING AT VARYING DISTANCES FROM
            INTERSTATE 95, CONNECTICUT...        	    II-9

I1-4      COORDINATE SYSTEM SHOWING GAUSSIAN DISTRIBUTIONS IN THE
            HORIZONTAL AND VERTICAL   	    11-11

IT-5      HORIZONTAL DISPERSION COEFFICIENT AS A FUNCTION OF
            DOWNWIND DISTANCE FROM THE SOURCE 	    11-14

I1-6      VERTICAL DISPERSION COEFFICIENT AS A FUNCTION OF DOWNWIND
            DISTANCE FROM THE SOURCE	    11-15

II-7      ALTERNATE SOLUTION CALIFORNIA LINE SOURCE CROSSWIND
            MODEL FOR CARBON MONOXIDE CONCENTRATIONS  	    11-17

I1-8      THE SHELTER PROVIDED BY A 16-METRE-HIGH SHELTERBELT
            OF DECIDUOUS TREES IN SUMMER AND WINTER	    11-33

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                         TABLE OF FIGURES (CONTINUED)

Table                                 Tltlfe                           Page

II-9      DESIGN PARAMETERS OF BUFFERS FOR SOUND ATTENUATION.  .  .  .    11-41

11-10     DENSITY OF BUFFER RELATED TO REDUCTION OF WIND VELOCITY .    11-46

11-11     EXTENT OF INFLUENCE OF WINDBREAK AND SHELTERBELT PLANTINGS  11-49

11-12     FORM OF BUFFER IS RELATED TO REDUCTION OF WIND VELOCITY .    11-50

11-13     INCREASED DIVERSITY WITHJN EDGE CONDITION MAXIMIZES
            SINK POTENTIAL	    11-51

11-14     CREATION OF THERMAL CHIMNEYS FOR VENTILATION OF
            FORESTS AND BUFFERS	    11-51

II-15     CO CONCENTRATIONS ADJACENT TO ROADS	    11-52

11-16     INCREASING BUFFER EDGES  	    11-55

11-17     INCREASING BUFFER VENTILATION	    11-55

11-18     CHEVRON HEDGEROW 	    11-56

11-19     PARALLEL HEDGEROW 	    11-56

11-20     MULTIPLE HEDGEROW 	    11-57

11-21     MANAGED NATURAL BUFFER   	    11-57

11-22     VENTILATING ROADWAY CUTS	    11-58

11-23     RECREATION FACILITY SETBACK  	    11-58

11-24     PLANTING EXISTING MEDIANS    .  .	    11-59

III-l     SCHEMATIC REPRESENTATION OF  THE  CHEMICAL PROCESSES
            INVOLVING ENVIRONMENTAL  SULFUR...      	   III-3

III-2     SECTION ALONG 79TH STREET, MANHATTAN  ISLAND  	   111-19

III-3     WEDGES	   111-20

III-4     GREENBELTS	   111-20

III-5     STREET TREE PLANTINGS ARE  ENCOURAGED  AS PART OF REGIONAL
            PLANTING AND BUFFER PROGRAM	   111-21
                                       vi

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                          •TABLE OF FIGURES (CONTINUED)

Table                                 Title                           Page

III-6     DISTANCE OF MAXIMUM CONCENTRATION AND MAXIMUM  XU/Q AS A
            STABILITY AND EFFECTIVE HEIGHT OF EMISSION	   111-25

III-7     TWO DIMENSIONAL RELATIONSHIPS BETWEEN SOURCE, SINK, AND
            RECEPTOR LOCATIONS	    111-26

III-8     IDEALIZED POINT SOURCE BUFFERS WITHOUT REGARD TO LAND
            CONSTRAINTS	    111-27

III-9     IDEALIZED POINT SOURCE BUFFER WITH LAND CONSTRAINTS. .  .    111-27
                                        vli

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                                 LIST OF TABLES

Table                               Title                             Page

II-l      KEY TO STABILITY CATEGORIES	   11-13

II-2      PLANTS KNOWN FOR THEIR CAPACITY TO RETAIN DUSTS 	   11-22

II-3      NUMBER OF KERNELS IN ONE CM3	    11-25

11-4      PROCESS OF SULFUR ABSORPTION BY PLANTS	    11-30

I1-5      ECOLOGICAL CHARACTERISTICS OF COMMERCIAL FORESTS AS
            CONTRASTED WITH PROTECTIVE GREENBELT VEGETATION ....   11-36

III-l     SUMMARY OF SOURCES AND ANNUAL EMISSIONS OF ATMOSPHERIC
            POLLUTANTS	   III-2

III-2     ESTIMATED CARBON MONOXIDE EMISSION SOURCES IN THE
            UNITED STATES IN 1970	   III-6

III-3     KEY TO STABILITY CATEGORIES 	   111-24

III-4     WEIGHTED SINK AND EMISSION FACTORS FOR AVERAGE SOIL AND
            AVERAGE VEGETATION...     	   111-30,31

III-5     SPECIES RELATIONSHIP OF GROUND AREA COVERED TO PLANT
            SURFACE AREA 	    111-32

III-6     SELECTED TREES AS POLLUTION SINKS	    111-32,33

VI-1      PLANT SPECIES SENSITIVITY LISTS
                                 FLUORINE	   VI-22

VI-2      PLANT SPECIES SENSITIVITY LISTS
                        GENERAL POLLUTION 	   VI-26

VI-3      PLANT SPECIES SENSITIVITY LISTS
                        HYDROGEN CHLORIDE 	   VI-33

VI-4      PLANT SPECIES SENSITIVITY LISTS
                        NITROGEN DIOXIDE  	   VI-35

VI-5      PLANT SPECIES SENSITIVITY LISTS
                                    OZONE	   VI-37
                                      viil

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                            LIST OF TABLES (CONTINUED)

Table                               Title                             Page
VI-6      PLANT SPECIES SENSITIVITY LISTS
                                      PAN	   VI-40

VI-7      PLANT SPECIES SENSITIVITY LISTS
                       PARTICULATES-SMOKE 	   VI-41

VI-8      PLANT SPECIES SENSITIVITY LISTS
                           SULFUR DIOXIDE 	   VI-42

VI-9      DATA CHARTS OF THE TREE SPECIES USED IN THE MODEL
            HECTARE	   VI-50
                                       ix

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I.    INTRODUCTION.  APPROACH AND SUMMARY  OF RESULTS

     A.   INTRODUCTION AND ORGANIZATION OF THE REPORT

         The work undertaken in this project has resulted in the preparation
of  three separate report volumes and one Appendix Volume.  Taken together,
they cite and attempt to interpret all of the pertinent and accessible literature
from the United States of America,  and elsewhere, relating to the potential use of
open space as a practical means to mitigate air pollution.

         Volume II, this Volume, is entitled Design Criteria and presents the essence of
this study in the form of a workbook. It reviews the primary biological and design
features which are crucial to the effective utilization of open space to mi-
tigate air pollution.  It presents generalized schemes for the design and
location of buffer strips and other forms of open space and also illustrates
air pollution mitigation by open space by identifying the mathematical pro-
cedures necessary in order to permit the incorporation of the appropriate sink
factors into four generally used carbon  monoxide diffusion models.

         Since this project concerns an investigation into the real and potential
use of  open  space, a rather abstract and loosely used phrase, the following
definition is given as the frame upon which our work is placed.  Open space is
an area with a natural cover of soil, water, and plants, where there are usually
minimal human activities, and where there are legal restrictions that limit
the development of facilities or structures.  In a limited sense, open  space may
be thought of as parks.  However, they may also be Resource Open Spaces where the land
or water is devoted to some form of non-structural production activity.  A forest,
range-lands, and water storage lakes or  rivers, are examples.  Flood control and
drainage lands,  lands used as waste disposal areas or borrow pits, wildlife refuges,
or lands reserved for future urban development, are all examples of Utility Open
Spaces.   Another major category may be  called Green Open Spaces where recreation,
or relatively non-structural uses, are sought and where the natural vegetation
tends to dominate the landscape.  Examples include; national park areas, urban
parks, buffers, and the associated greenbelts or green wedges, which may be
interspersed with urban development.  A  fourth major category consists of Corridor
Open Spaces  where space is allocated for the movement of people and material from
one point to another.  Examples include, rights-of-way such as highways and streets,
or  canals and railroads, and the areas associated with the terminals and/or
interchanges associated with those rights-of-way.
                                     1-1

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         These, and other categories of open space  are more fully described in
the literature.  DeChiara and Koppelman (1975)   include the above definitions and
others which may be useful should the reader seek detailed information from the
point of view of urban planning and design.   However,  as explored in this project,
open space is limited to those categories defined above.

         Open space, in its natural state or manipulated state,  can have a varied
and far reaching effect on regional air quality.  It has been well documented in
Volume I of this report that open spaces particularly when planted, as bare soil,
or as water bodies, can act as sinks for important  air pollutants.  Through the
natural process of adsorption, absorption,impingement,and deposition, pollutants
generated by urban land uses can be entrapped by these areas.  From a planning
point of view, open space has been used as a buffering device to contain the expansion
of urban development and its attendant generation of air pollution.  The characterization
of open space as land upon which there is minimal human activity makes' the phase an
antonym to urban type development.  The extent and  location of such open space has
varied effects on regional air quality.  For example, the use of an open space
adjacent to a transportation artery (i.e  a roadway,) reduces the ambient levels
of automobile generated pollutants.  Vegetation in  the path of air, laddened
with particulates, can serve to filter out some of  the particulates.  This capability
can reduce concentrations of particulates which would otherwise impact area residents.
The use and design of open space areas on a micro-scale can mitigate pollution
transport characteristics.  Through the break-up of tunnel or canyon effects,
vegetation canopies can encourage air current eddying and thus can cause mixing
and the sedimentation of particulates.

         The atmosphere should be looked upon as a finite sink for pollutants.   It
has a limit which we can try and set as an "acceptable" concentration of pollutants.
By reducing the density of urban development through  the use of open space,  the
loadings are reduced in a region.

         The possible negative effect of open space includes the natural emission
factors characteristic of particular plant species.   The generation of hydrocarbons
by plants  produce photochemical  oxidants.   Depending upon the amount of plant materials,
the hydrocarbons  emitted can intensify or create oxldant problems.  The use of

                                       1-2

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open space within a comprehensive land use plan can also have negative effects
on overall air quality if the entire community infrastructure is not evaluated.
For example, if large tracts of open spaces cause an increase in vehicular travel,
the associated generation of transportation related pollutants is Increased.
In addition, some open space uses are marked air polluters.  For example, open pit
mining and agricultural activities, such as plowing, can significantly increase
the particulate loadings in the ambient air.

         The knowledge obtained from the investigation of open space as an air
quality maintenance strategy should be used to re-evaluate the concept of the
atmosphere as a sink.  Historically, our view has been to dilute the pollutants
with the atmosphere.  However, vetetation and open space can be utilized as a sink
or filtering device.  It would be efficient to concentrate polluting emissions and
direct them through an appropriate open space so that they can be filtered.  This
seems contrary to present day thinking.  However, systems planning, value engineering
and resource recovery are also relatively new concepts gaining in their acceptance.
It is hoped that the information in this report may help make open space an air quality
management technique somewhat better understood than was previously the case.   It
should be actively implemented as an additional strategy available for environmental
management.

         Volume I  is entitled Sink Factors  and presents the data collected from
the manual and computerized literature searches.  Most of the information presented
in the other volumes was derived from the data contained in Volume I.  There-
fore, much cross referencing is made.  Volume I contains tables of sink and
emission factors which were developed based on the collected data, and it also
contains tables of pollution sensitive and pollution resistant plant species derived
from the surveyed literature.  The separate Appendix Volume for Volume I presents
abstracts of the pertinent literature.  It was decided to include as many abstracts
as possible in order that our work might find as broad a utilization as possible
by future researchers.

         Volume III is entitled Demonstration Plan and applies our findings in
a hypothetical manner to a test city, St. Louis, Missouri.  This demonstration
plan includes a cost/effectiveness analysis of the combined open space/AQMA
plan with that analysis based on the best available data which we were able to
secure.  It provides the reader with a realistic application and evaluation
of using open space as a practical part of the AQMA plan strategy.
                                    1-3

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     B.  SUMMARY OF THE RESULTS

         Of approximately eight thousand references examined, about two thousand
were used because they were directly or indirectly relevant to
determining the sink and emission factors of those pollutants under study.
Information was collected on: 1) Ammonia, 2) Carbon monoxide, 3) Chlorine,
4) Fluorine, 5) Hydrocarbons, 6) Nitrogen oxides,  7) Ozone, 8) Perbxyacetylnitrate
(FAN), 8) Particulates, and 9) Sulfur dioxide.  Sink and emission factors are
reported from the literature and, where possible,  the average factor is calculated
based on a subjective evaluation of the data.

         As a result of this study, it is clear that there are very little data
available that  quantitatively evaluate  the function of water bodies as a sink
and/or source of air pollutants.  Most of the data we reviewed dealt with soil and
vegetation relative to sinks and emissions and therefore, the imbalance of data
causes this report to make only very general statements concerning the importance of
water as a factor in open space mitigation of air pollution.  Future research should
focus on this area for both qualitative and quantitative analyses.

         The present literature is most clear in its conclusion that open space,
 vegetation in particular, is a filter for all manner of partlculates.  In
fact,  the air-pollution-mitigating-capacity of open space is graphically so
clear that this Summary of Results has been extended to include the following
series of electromicrographs prepared by the Yale University Laboratory of
Dr. William H. Smith, a co-author of Volume I - Sink Factors.

         Particles are intercepted by vegetation,and the literature also
reports absorption of various air polluting gases.  These are summarized in
Volume I and their conclusions are applied in this Volume.  Soil, as a sink for
carbon rronoxide, is the most effective element of open space in removing
noxious gas, as reported in the literature.

         With these two simple and well documented findings, it is clear  that
open space, carefully placed, can effectively function to filter particulates and
carbon monoxide from the air.  Furthermore, it can be demonstrated from the
literature that open space also functions to mitigate numerous other pollutants.
The use and predicted mitigation by open space as an air resource management

                                     1-4

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II.  HIGHWAY BUFFER AND RELATED OPEN SPACE
     This section of the study is concerned with the control of pollutants  from
a highway source.  It introduces the concept of  using highway  buffer strips  to absorb
pollutants transported to the edge of a highway.   Initially, a review of pollutants
emitted from motor vehicles is presented followed  by discussions on transport
methodology and diffusion modeling.  Next,  sink  factors are presented for  various
highway related pollutants.  Finally, the literature is reviewed on buffer strips
and design alternations.

     The section was written to allow the user  to  initially predict the type and
amount of pollutants that will be present adjacent to highways and highway
corridors.  Following this predictive methodology,  one can determine the amount
and type of buffer strips that would best absorb  these pollutants.

     It should be noted that the concepts  presented in  this  chapter are not
based on an exact science and should be used only as planning guidance*.  The
sink factors and design alternatives that  are presented are  based solely on a
review of the literature.  More practical  research  is needed on the effective-
ness of using these concepts.   In addition,  before  making  detailed predictions  of
the concentrations of pollutants near highways,  Jihe user should consult with
other publications to determine the best model to use for  the actual case with
which he is involved.

     A.  POLLUTANT IDENTIFICATION

         1.  Source Emissions.

             Before developing design concepts  for highway  buffer strips,  it
is necessary to review the type and quantities  of  pollutants that are emitted  from
a motor vehicle.  Air is polluted as a  result of combustion and the majority of
transportation systems today use the combustion  of fossil fuels as their main  source
of energy.  Carbon monoxide (CO), hydrocarbons  (HC), and  oxides of nitrogen  (N0x)
are the three major air pollutants released by motor vehicles. It has been
estimated that motor vehicles represent 98% of  the sources  for CO, 50% of  the  sources
for NO  and 60% of the sources for HC  (Willis ,'et al.,|1973).
                                      II-1

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             In addition to the above, motor vehicles emit a small percentage
of  two other pollutants usually considered in air pollution problems; sulfur oxides
(SO ) and total suspended particulates (TSP).  SO  is usually considered more of
   X                                             X
a regional problem associated with individual point sources and it will be discussed
in Section III of this study.  Although transportation sources are not responsible
for any significant portion of TSP emissions, their contribution,especially lead,
should and can be considered in designing buffer strips for highway corridors.

             Wolsko, et al., (1972) present a description of the  fuel combustion process
and how pollutants are formed.  The majority of emissions come from gasoline
powered motor vehicles.  When gasoline is mixed with air in proper proportions, a
combustible mixture is formed.  Because the combustion process is not complete, by-
products are formed which are considered pollutants.  This situation is character-
istic of any combustion process using fossil fuels  (electrical generating stations,
space heating, transportation).
                     Fuel Combustion Equation for Gasoline

         Gasoline . Air Combustion	_g^  Combustion Products + Pollutants
         (HC)m  w^tv/	^^» C02 + H20 + H9 + CO + NO
*   = many types

             The above equation depicts that carbon dioxide (CO.,) ,  water vapor
(H20), free hydrogen (HO, oxygen (02) and nitrogen (N2) make up the
bulk of the products of combustion, but carbon monoxide, oxides of nitrogen (NO,
N0_) and unburned hydrocarbons (HC)  are also produced.  More than 200 unburned
hydrogens (HC)  have been detected in vehicle exhaust.  (Note:  The above equation
is representative of the fuel combustion process and does not necessarily balance
in a chemical sense).

             The amount of each of the pollutants emitted on a highway is dependent
 on the number of vehicles using the highway as well as the relative efficiency
 of each automobile's  emission system.  Because of the many different types of
 vehicles and their different ages and degrees of operating efficiency, emissions
 vary widely from vehicle to vehicle,:-. In addition to differences in vehicle
 emission characteristics, the operating cycle is also an important determinant
                                    II-2

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of pollutant emissions from transportation sources.  Speed, cold starts, acceleration,
starts and stops,are factors of the vehicle operating cycle that effect emissions.

             The Environmental Protection Agency has published factors which
represent the weighted emissions for a standard distribution of vehicles.  Using
emission factors for each vehicle, it is possible to quantify the total pollutants
being emitted along a highway corridor.  The necessary data and procedures used to
calculate emission factors for motor vehicles are contained in "Supplement No. 5
for Compilation of Air Pollutant Emission Factors" (U.S. EPA, 1975).
             In  order to determine the total  emissions for a given  time period,
multiply  the emission factor obtained from Supplement No. 5 by the total number
of vehicles for  that same period.

              The amount of  particulates emitted from a  highway source Is more
 difficult to quantify than the gaseous pollutants.  Most of the particulate matter
 comes from two sources:  the  first being the salts formed in the exhaust and the
 second being rubber particles from tires and asbestos particles from brake linings.
 In addition to these sources,  the turbulence in the air from a moving vehicle causes
 dirt particles on the side of the road to be disturbed  and emitted into the air.

              The particulate from automobiles that has  been-given most attention
 is lead.   To reduce quantities of lead being emitted, all new cars are made
 to use lead free gas thereby eliminating the source of  the problem.  However, it
 will take years before all older vehicles are phased out and only lead free
 automobiles are allowed on the highway.

             Lead  is one  of the principal particulates emitted by motor vehicles.
Specific  estimates  of the amount  of  lead annually  introduced to  the atmosphere via
gasoline  combustion includes 98%  (National Academy of Sciences,  1972) and 95%
(Ewing and Pearson,  1974).  Atmospheric, terrestrial and aquatic environments
immediately adjacent to roadways  are contaminated  with lead by motor vehicles
combusting leaded  gasoline.  No controversy surrounds this observation.
                                    II-3

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             Most  of  the  gasoline  for  vehicles  sold prior  to  1975  in  the United
 States  contains  alkyl lead  compounds to  improve the antiknock quality of the  fuel.
 The  amount  of  lead in gasolines prior  to 1975 (in the form of lead alky Is) varied
 from 2  to 4 g/gal.  The average lead content is approximately 2.5  g/gal.
 (Ewing  and  Pearson,  1974).

             Not all  the  lead  combusted  in  automobile  engines is  released into
 the  atmosphere.  Hirschler  and Gilbertl( 1984)1, concluded  that  25%  of  the  lead
 combusted may  be held in  exhaust system  deposits or removed during changes of
 lubricating oil  and oil filters.   These  investigators  further found  that the
 percentage  of  lead burned in the engine, which  is discharged  to the  atmosphere,
 varies  with driving speed,  driving conditions,  vehicle age and fuel  employed
 among others.  Over many  thousands of  miles of  driving it  is  generally assumed
 that approximately 70-80% of the combusted  lead will eventually be released
 to the  atmosphere.  Assuming average and approximate conditions,  automobiles
 prior to  1975  may  release 130  mg of lead per mile per  car  (81 mg  Pb/km)  into  the
 roadside environment  (Smith, 1975).

                          2.5gPb/gal   x   0.80 emission    n  .,    _. , ...
                             "  ?,.—7;	;—;	  =  O.U g. Pb/mile
                                  15 miles/gal.

             An  average lead emission  rate  for  production  vehicles at 108 mg.
 of lead per mile has  been given by Cantwell, etal.,  (1972). A more conservative
 average emission rate of  40 mg. of lead  per mile has been  presented by Haar (1972).

             To determine  the amount of lead emitted from vehicles along a highway
corridor it is suggested that one use 130 mg.  Pb/mile and apply this  emission
rate to the percentage of  vehicles using the highway corridor that were manufactured
prior to 1975.   After 1975,  all vehicles are using no-lead gas and thereby, no
lead salts  are  being emitted.   The age distribution of vehicles in a particular
state is usually available from the local motor vehicle department.
                                      II-4

-------
         2.  Transport Mechanisms.

             The concentration of pollutants at a roadway edge (the receptor)
depends on more than just the quantity of pollutants emitted at the source.
The atmosphere is the agent that transports and dispenses pollutants between
sources and receptors and thus its state helps to determine the concentration
of pollutants observed at the receptor location.  The following paragraphs
have been adapted from Epstein, et al. (1974) and are used to briefly review
the phenomena of transport mechanisms for gaseous pollutants (CO,  HC, NO) from
                                                                        A
a highway source.

             In general,,three parameters are used to describe atmosphere
transport and dispersion;processes. These  are wind speed, wind direction and
atmospheric stability.  For a ground level pollutant (the general case for
a highway) the concentration of pollutants downwind from a highway source is
inversely proportional to wind speed.  This phenomenon is illustrated in
Figure II-1.

             Wind direction ±s perhaps the most important atmospheric
condition influencing the concentration at a given receptor location.  For a
given wind direction,nearly all the pollutant transport and dispersion will be
downwind.

             Atmospheric stability is a measure of the turbulent structure of
the atmosphere.  Epstein explains that "it may be defined in terms of the
atmospheric temperature  profile where ambient temperature is a function of
height above ground level.  When the temperature decreases rapidly with height,
vertical motions in the atmosphere are enhanced, and the atmosphere is called
unstable.   ...When the temperature does not decrease rapidly with height,
vertical motions are neither enhanced nor repressed and the stability is
described as neutral... When the temperature decreases very little, remains
the same, or increases with increasing height, the atmosphere is called stable."
                                    II-5

-------
                                      FIGURE II-l


          THE INFLUENCE OF WIND SPEED ON GROUND LEVEL POLLUTANT CONCENTRATIONS
Height
               Wind
              Direction
       Distance  Downwind

/
14.4
-Kilometers 	 +•
•S r-
                                   L_
                                     Kilo
   -7.2—*
Kilometers
                                                            .Volume of air
                                                             containing the
                                                            pollution emitted
                                                              In one hour
                                                            Wind  Speed •
                                                              4 Meten/Second
                                                  Volume of air
                                                    containing
                                                  the pollution emitted
                                                     in  one hour
                                                  Wind  Speed- 2 Motors / Second
                                    II-6

-------
              An unstable atmosphere is  the best type for dispersing  pollutants.
 A neutral atmosphere allows dispersion  of  pollutants in the horizontal direction,
 but not as rapidly in the vertical direction.   A stable atmosphere is  the worst
 for air pollutant dispersion as  it suppresses  the upward movement of rising air.
 It essentially forms a lid beneath which pollutants  can freely disperse horizontally
but not vertically.

              The available literature on the transport  of lead reveals that it
 is slightly affected by prevailing winds and that most  of this contaminant is
 contained in the particulate fraction of materials generated by the  traffic.
 The distance that the lead particles will  be transported depends on  size of the
 particle and the atmospheric conditions prevalent during the time period.
 Hirschler and Gilbert (1964),suggest that  one-half to two-thirds of  the lead
 exhausted in city type driving was in particles 5y in diameter or less.
 Only 4  to 12%  of the exhaust lead was  lu  or less.  Under cruise conditions
 and at  constant speed,  Mueller,  ec al. ,(1963),  found  that 62  to 80% of  the  particulate
 lead exhausted was less  than 2y  in diameter.   Of these  small particles,  68%
 were less than 0.3vi.

              The roadside environment receives lead  particles  of all size
 classes,  the large ones  by sedimentation and the smaller ones  by impaction,
 precipitation and inhalation.  Determining the amount of lead  at various distances
 from a  highway source is reflected in literature concerning  the lead content
 of soils and vegetation  near the highway.   Hutchinson, (1971),  has developed experimental
 data illustrating the soil level of lead adjacent to Queen's Park (Figure  II-2).
 Smith (1971),  has studied lead contamination of white pine  twigs in  Connecticut
 (Figure II-3),  and concluded that  the lead content drops drastically as  the perpendicular
 distance from the roadway increases.  This conclusion is supported by  numerous
 studies,  the finest being that of  Daines,  et al.,(1970), and Shuck ancTLocke (1970).
 Between 30 and 150m perpendicular  distance from the  highways in the  above
 studies,  the atmospheric lead rate per  30m was 32%and 23% respectively.   In the
 Daines  et al., (1970),study,  the  lead  content of the  air decreased 50%  between
 3  and 46m from the highway.  At  533 m perpendicular  distance,  50% of the lead
 containing particles greater than  6.5jj  settle  out of the air.   Little
 surface deposition,  however,  of  the less than  3.5y diameter  particles  occurred
 in this zone.
                                     II-7

-------
                         FIGURE II-2

            SOIL LEVEL OF LEAD IN QUEENfs PARK AND SOIL

                 LEVEL OF CADMIUM IN QUEEN's PARK
600
                                              Soil Depth
                                        	•  0-1/2 inches
                                        	• 2-3  inches
                                               5-6 inches
               6   8  10  12  14  16  18  20 22  24 26  28 30
                 DISTANCE FROM ROAD  (METERS)
                           II-8

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                                  FIGURE II-3


LliAD CONTAMINATION OF WHITE PINE TWIGS PLUS NEEDLES (GROWTH OF PREVIOUS YEAR)

SAMPLED FROM TREES GROWING AT VARYING DISTANCES NORTH AND SOUTH OF INTERSTATE

95 IN CONNECTICUT.  SAMPLES TOWARD THE ROAD WERE COLLECTED FROM THE TREE BRANCH

CLOSEST TO THE HIGHWAY WHILE SAMPLES AWAY FROM THE ROAD WERE COLLECTED FROM THE
OPPOSITE SIDE OF THE TREE, FARTHEST FROM THE HIGHWAY.
         E
         d
         o.
            250
            ZOO
            150
         (£
         O

         in
         ui
         _j
         O
         UJ
         UI
         z
         •f
         Ui
         o
         >   50
100
            25°
         z
         o
         t-
         z
         o
         o

         o
         <
         UJ
200
            I5O
IOO
             50
                 NORTH OF ROAD
                          •o—o- SAMPLES TOWARD ROAD



                          -•-—»• SAMPLES AWAY FROM  ROAD
                        •o   o o


                         -*L   r=-0.56
                 SOUTH OF ROAD
                      j_
                          00,

                           . ~~T

                          ••



                          •  '••••
                                       r=-0.57
                                                      = -0.33
                                                       •
                       5       10       15       2O      25      30

                         TREE DISTANCE FROM ROAD (METERS)
                                       II-9

-------
             In addition to distance from the road,  numerous other factors
influence the lead content of the atmospheric compartment of the roadway
environment.  Some of the important factors include traffic volume, proximity
Lo other roads,  prevailing winds, turbulence, season of the year and time of
day.  Urban atmospheres over streets may differ significantly from rural atmos-
pheres over roadways.  Edwards  (1974),has suggested that the canyons formed
by multiple story buildings may restrict ventilation and cause high increases
in atmospheric lead.

             The effect of traffic density is limited to a relatively narrow
zone (76m) along busy highways according to the data of Daines et al.,  (1970).
Numerous studies have shown if the prevailing wind direction is perpendicular
to the highway,  greater amounts of lead will be distributed to the lee side
of the road.  In seasonal studies, conducted in various United States locations,
the fall months consistently exhibit the highest air lead levels.  The increasing
fall concentrations are generally ascribed to favorable wind patterns and
atmospheric mixing occurring at this time of year.  Diurnal variations in
atmospheric lead burden close to the road generally follow the peak traffic
volumes of early morning and late afternoon.

             Without further refinement, no exact relationship can be constructed
for the amount of lead in the atmosphere versus the perpendicular distance
from the highway.  However it can be safely concluded that the majority of the
lead particles are deposited by some method close to the highway (50m ±).  The
lighter particles (< 3.5y) travel a further distance from the highway source
and generally would tend to accumulate on the leeward side of the highway.

         3.   Atmospheric  Diffusion.

             The  preceding  two  sections have described  the  quantities  of
 polLutants  emitted  from  a  motor vehicle and the transport  mechanisms  that
 influence their  dispersion from the source  to  receptor  location.   There are
 numerous mathematical  models that simulate  the  dispersion  of  CO from  a  highway
 source.   These models  are  generally classified  into the following  categories:
 Gaussian statistical,  box,  particle-in-cell,  and  mass  conservation.   This section
 will  describe the Gaussian model and its adaption to a  highway  line source for the
 prediction  of CO.

                                       11-10

-------
             The Gaussian plume dispersion model has achieved considerable
popularity among people attempting to describe the role of atmosphere dispersion.
The model is an adaption of the normal distribution curve as a predictive tool
to describe the concentration of gaseous pollutants at given distances from
a source.  The model was originally suggested for use by Pasquill(1961) and
modified by Gifford (1961).

             The concentration  (x) of gas or aerosols (particles less than about
20 v      diameter) at x,y,z from a continuous source with an effective emission
height, H, is given by equation 1 and the coordinate system used in the equation
is illustrated in Figure TI-4.
                                   FIGURE  II-A
               COORDINATE  SYSTEM  SHOWING GAUSSIAN DISTRIBUTIONS
                         IN THE HORIZONTAL AND VERTICAL
                                                                                     (1)
                                         11-11

-------
             The following assumptions are made in  equation  (1):

                 (1)   The plume  spread has a Gaussian distribution in both
                      the horizontal and vertical planes, with standard
                      deviations of plume concentration distribution in the
                      horizontal and vertical of ay and oz, respectively.
                 (2)   The mean wind speed affecting the plume is p.
                 (3)   The uniform emission rate of pollutants is Q.
                 (4)   Total reflection of the plume takes place at the earth's
                      surface.
             Any consistent set  of units may be used.  The most common is:

                 x (g nf3)
                 Q (g sec  )
                 y (g sec  )
             oy,oz,  H,x,y,  and z (m)

             For concentrations  calculated at ground level, i.e. z=Q, the
equation becomes:
                        x (x,y,0;H) = ^r^T exp
                                                            (2)
             [-•Hi-)1]
             Where the concentration  is  to be calculated along the center line
of the plume (y=0),  the equation  is simplified  to:
                                 IT
 §— -exp I — -i-f^Y 1

-------
             The values  of oy and oz  in the previous equations have produced the
major areas of investigation.  Turner (1972),  developed a procedure to relate
oy and oz to stability classes which  is in turn estimated from wind speed at a
height of about 10 meters and, during the day,  the incoming solar radiation or
during the night, the cloud cover.  Stability  classes are given in TableH-l-
                                   TABLE II-1
                          KEY TO STABILITY CATEGORIES

Day

Surface Wind — ; 	 — - — —
Speed (at 10 m). lncomin* Solar Radiallon
m sec~»
< 2
2-3
3-5
5-6
> 6
Strong
A
A-B
B
C
C
Moderate
A-B
B
B-C
C-D
D
Slight
B
C
C
D
D
Night
Thinly Overcast
or
^4/8 Low Cloud

E
D
D
D

^3/8
Cloud

F
E
D
D
                  The neutral class, D, should be assumed for overcast conditions during
                  day or night.
                           SOURCE:   (TURNER,  1972)

             Having  determined  the stability  classes, one can estimate ay and oz
as a function of  downwind distances from the source, x, using Figures  II-5  and II-6.

             The Gaussian  plume dispersion model can be applied to a continous
line source, such as a highway.  Federal Highway Administration (1972) suggests
that equation (5 )be used  to predict downwind ground level concentrations for at
grade highways and crosswind conditions:
                        c
                                    sin-0-
             where:
                        Q =  source  strength,  grains/meter-second
                        K =  empirical constant = 4.24
                        p =  wind  speed,  m/sec
                        •6- =  wind  angle with respect to road
                       oz =  vertical  dispersion parameter, meters
                                       11-13

-------
                                     FIGURE  I1-5
                    HORIZONTAL DISPERSION COEFFICIENT AS A  FUNCTION
                         OF DOWNWIND DISTANCE FROM THE SOURCE
10,000
                                1                           10
                                    DISTANCE DOWNWIND, km
                                            11-14

-------
                                    FIGURE  H-6
                   VERTICAL DISPERSION COEFFICIENT AS  A FUNCTION
                       OF DOWNWIND DISTANCE FROM THE SOURCE

  1,000
E

r~
b
                                1                           10
                                    DISTANCE DOWNWIND, km
                                           11-15

-------
             Using  a  technique  developed by  Noll,  et  al.,  (1975)  equation (5)  can
be  solved  for  CO using a nomograph (Figure  II-7).    Starting at  the left axis,
there  are  six  meteorology scales  labeled  A-F and  marked  off  in a wind speed scale
in  meters/second.  These meteorology scales reflect   allowable wind speed ranges
for each stability class as outlined in Table II- 1.   To  the  right of the meteorology
lines  are  next found a scale labeled jj 0z,  m2/sec and then x, normal distance from
the road,  meters.  Connecting  any distance  on the x-axis with the desired stability-
wind speed combination yields  the product y oz on the intermediate axis.

             The next axis is labeled, $,  the wind angle  with respect to the
road.   This axis represents sin ,  and a  line connecting the previously obtained
                                                              _            2
M oz,  through  the  appropriate  value for $ (yields  the product y oz sin <|>, m /sec
on  the next axis.)
             Having now evaluated the denominator  in equation (5), it is now left
 to  evaluate the line source strength, Q,  gms/m-sec.

                   Q = (VPH)  (EF)   (1.73 (10.7))             (6)
             where:

                           VPH = Traffic volume, veh/hr
                           EF  = emission factor,  gms/veh-m
                                                               3
                           Q   = pollutant concentration, gms/m

             The emission factor  (EF) is obtained from "Supplement No. 5  for
Compliance of Air Pollution Emission Factors",  (U.S. EPA, 1975).

             However, concentration in parts per million  (ppm), by volume is
required.  Assuming ideal gas behavior, yields  at 25 C for CO:

                         ppm CO = (875) (S^2)      (7)
                         ppm CO = 1.51 (10-4)              (8)
                                              oz v sin$     '
             Equation 8  is solved graphically by  the  last  four  lines of  the
nomograph in Figure II-7.          Connecting the previously described value
of {I oz sin<|> with a value of emission factor yields an intermediate value on the
pivot line.   Alignment of this pivot point with a value for traffic volume
and extending to the final line yields the desired result, ppm CO,
                                     11-16

-------
                          FIGURE H-7

     ALTERNATE SOLUTION CALIFORNIA LINE SOURCE CROSSWIND
           MODEL FOR CARBON MONOXIDE CONCENTRATIONS
M
C <






ft



A
3








2
















1
9


4





3~

'


2
•
1)
[" . 1 8
U 0) _
 _
a es o> -e- o
13 CL O
7
1
e


9

E
4



• 3
0

•2
C

•




.





1
9


4


3
F
3

,

s ;
' 2 '



1

1



H*1 •
0 v» C
190 *> 0» i- *g
"
l
0

^~ «
C.
(U

'so
40
30
20
. 10
i 8
: 6 1
' 4 !
1 3
2
* 1

•


,
t

,
•
.
.

.
.

O.
0.
rlOO
80
' 60

40

•30
20

10.
e.

6.

• 4.
3.

2.

1.0
.BO
• .60
.40
.30

.20


0.1

.08
.06

.04
.03

.02

0.01
stability wind
speed, u-m/sec
                               11-17

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     B.  LITERATURE SEARCH FINDINGS

         This section of Literature Search Findings is composed of those key
points which were extracted from the greenbelt literature utilized to derive the
landscape architectual information in this Volume.  These papers represent a
relatively small fraction of the literature obtained for the entire project.  An
overview of the main body of information about vegetation as sinks and emissions
may be gained by referring to the approximately two thousand abstracts appearing
in the bibliography of Volume I.  The majority of the papers cited in that
bibliography were located and read.  Those papers that were potentially valuable
for the purposes of the landscape architect were then selected.  The landscape
architect team member decided which were most relevant and most important in his
conceptualization of effective greenbelts.  Additional papers were sought which
augmented the Volume I bibliography.  The key bibliography used for this
Volume is presented here.

         Where possible, the exact words of the various authors are quoted in order
to insure accuracy.  In other instances, the author's words were paraphrased, but
most of the information appears without interpretation.  These papers are presented
as generally representative of a larger literature and they are interpreted in the
following order:

         1)  The value of forests in removing particulates
         2)  Plant mechanisms for absorbing and adsorbing pollutants.
         3)  Organization of plantings.
         4)  Maximizing buffer edges to increase sink potential.
         5)  Ventilation of buffers and woodlots to increase sink potential.
         6)  Importance of local adaptation of plants to local site conditions.
         7)  Ecological approach to roadside treatment.
         8)  Size of buffers.
         9)  Safety factors as design.
        10)  The sound absorbing qualities of buffers.
        11)  Idealized plant material.
                                       11-18

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          1.   The value of forests  in removing particulates.

              It  has been frequently stated that  plants,  in general,  forests
 especially,  are  excellent agents for reducing ambient air pollutant  levels.

              Excellent discussions of the  functions  of forests which produce
 this  phenomenon  are found in  Keller (1971) :

                      An essential factor for environmental protection, on
                      the other hand, is the filtering action of the forest
                      on dust-shaped  air pollution.  The most favorable effect
                      in  this  respect is from loosely  structured, step-like
                      forest stands,  as can be deducted from Nageli's
                      investigation of windbreak sectors  (1943), dense forest
                      stands deflect  the wind upwards which also leads to
                      precipitation of dust due to turbulence for irregular
                      trre roof tops.  Loosely structured forests, on the
                      other hand,let  the wind penetrate and brake it, thereby
                      permitting the  dust particles to sedimentate.  In
                      addition, it is well known that particles up to 80y can
                      on impact even  adhere to vertically located surfaces of
                      leaves and the  like.   Forest air is, therefore, especially
                      devoid of dust with the exception of blossom time when
                      noticeable amounts of pollen are discharged into the air.
                      The filtering action of the forest regarding dust can
                      manifest itself even in soil scientific studies.  In
                      this way, in the lee of an area of industrial concentration
                      where enormous  amounts of soft coal, rich in ash, were
                      burnt ,the pH value of the humus layer in pine forests
                      to a distance of about 30km was increased because the
                      tops filtered out alkaline fly ash.

             According to Warren (1973),  the best deciduous trees for reduction
of particulates (according to Russian literature) - are lilac, maple,poplar.
Conifers are best for all year filtering - apparently they may remove 34% of  the
submicroscopic particles  compared to  19% removed by deciduous trees.


              Bach  (1972), further  suggests that the best genera for adsorbing
 particulates are:

                 Lilac (Syringa)               2.33 g/mj
                 Maple (Acer)                  1.11 g/m.
                 Linden (Tilia)                0.61 g/m.
                 Poplar (Populus)               0.26 g/m

                 Also good:  sugar  maple,  sycamore and white  ash.
                                        11-19

-------
             According to Geiger (1950), studies have demonstrated that the
reduction of wind velocity by forests and shelterbelts is proportional to tree
height; one can expect a 10% reduction in wind speed within a distance equal to
three times the tree height on the windward side and twenty times the tree
height on the leeward side.  Dense plantings, however, seem to reduce this effect
due  to the turbulance that they create. (See Figure II- 11).

              Other studies on the characteristics of pp.iticulate distribution
within a forest indicate that temperature differential within and above the
forest canopy can provide convection currents which move the air (and the pollutants)

              Fritschen and Edmonds (date unknown) found:

                      Inversions in the crown during the daytime and above
                      the crown at night trapped the particles within the stem
                      space.   Particles released below the inversion were trapped
                      until they reached a thermal chimney (i.e.; less dense
                      vegetation where solar heating had penetrated to the forest
                      floor)  where they escaped above the forest.

              Hagevik (1974)  refers to:

                      A study by A.L. Page, et al. examined lead concentrations
                      in 27 varieties of vegetation along highways.  They
                      found a direct relation between lead content in the plants
                      and distance from the roadway, although the relationship
                      was most significant at distances less than 150 meters
                      from the highway.  Lead content was also found to be
                      influenced by prevailing winds.

             Although Warren (1973)  feels that this can be reduced by the
planting of hedgerows which essentially reduce the velocity of the air to a point
where the heavy metal precipitates.   In one study cited, a dense hedgerow was
responsible for an approximate 40% decline in the lead content behind it.

              The World Meterorological Organization (1964) indicated that:

                      ...the measurements of Woodruff & Zingg  (1955) with systems
                      of four belts in the wind tunnel show no accumulative
                      effects but an increased degree of turbulence in the air
                      flow after passing the first belt.  This indicated that when
                      several parallel belts are planted the interval between
                      them should not increase but should be the same.

              It follows then that increased spacing between parallel hedgerows will
create increased turbulence and therefore increase the amount of CO and particulates
removed.
                                       11-20

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         2.  Plant mechanisms for absorbing and adsorbing pollutants.

             To understand the functions of the plants to reduce various
pollutants, their mechanisms and responses to various pollutants must be understood.

             a.  Particulates

             Smith and Dochinger (1975)  state:

                      Much of the understanding of  the mechanics of  deposition
                      of particles on natural surfaces has been gleaned from
                      studies with particles in the size range l-50\i m and is
                      reviewed in the excellent papers of Chamberlain (1967)
                      and  Ingold (1971).  Basically.participates are deposited on
                      natural surfaces by three processes:  sedimentation under the
                      influence of gravity, impaction under the influence of
                      eddy currents and deposition under the influence of per-
                      cipitation.  Sedimentation usually results in the deposition
                      of particles on the upper surfaces of plant parts and  is
                      most important with large particles.  Sedimentation velocity
                      varies with particle density, shape and other factors.
                      Impaction occurs when air flows past an obstacle and the
                      airstream divides, but particles in the air tend to
                      continue straight due to their momentum and strike the
                      obstacle.  The efficiency of collection via impactation
                      increases with decreasing diameter of the collecting obstacle
                      and increasing diameter of the particle.  Chamberlain
                      (1967), suggested that impaction is the principal means of
                      deposition if;  1)   particle  size is of the order of tens
                      of microns or greater,  2)  obstacle size is of the order of
                      centimeters or less,  3)   approach  velocity is  of the order
                      of meters per second or more and 4)  the collecting surface
                      is wet, sticky,  hairy or otherwise retentive.   Ingold  (1971),
                      presented data indicating that leaf petioles are consid-
                      erably more efficient particulate  impacters than either twigs
                      (stems) or the leaf lamina.   For particles of  dimensions
                      l-5jj impaction is  not efficient and interception by fine
                      hairs on vegetation is  possibly the most efficient retentive
                      mechanism.   The  efficiency of washout of particles by
                      rain is high for particles approximately 20-30y m  in size.
                      The capturing efficiency of raindrops falls off very sharply
                      for particles of 5\i m or  less. Particulate removal  by
                      stomatal uptake  has been suggested (Jordan 1975),  but  is
                      of unclear significance.   The latter process would probably
                      involve small (< lym dia) particles.

             Heichel and Hankin  (1976)  found  that  the pattern  of  lead accumulation
on twigs is unrelated to  the pattern  or  quantity of precipitations falling  on a  site.
It appears that these particles are less easily dislodged  from the rough surfaces
of twigs than from the waxy, smooth surfaces of needles  or leaves.

             Wylie and Bell  (1973) concluded  that  the major deposition  of lead
particles along roadways  occurs  within the first 25 meters(m) away from the road edge.
                                        11-21

-------
           Berindan  (1969) remarks:

                    The property of leaves to retain dust is a function of
                     the roughness  of their surface.  Table III indicates some
                    of the species for which the retention has been  tested.
                    This ability is much less in winter.  To ensure  continuous
                    action,  the species in Table III must be combined with
                    Coniferae; yet, considering that the latter are  highly
                    sensitive, this combination is no longer effective in
                    cases of mixtures of dusts with SO., for example."
                    "Some air pollution studies have focused on the  third
                    aspect of dust retention by plants which is the  action
                    of swirl of suction, in view of their property for
                    directing pollutants from top to bottom at the level of
                    the respiratory tract.  This type of draught  is  made up
                    behind any barrier which is high enough to hinder the
                    main direction of the wind  (22, 39, 56) (Fig. 7).* It
                    is also  thought that by using this property,  it  is possible
                    for dusts carried by the wind behind strips to be drained
                    at the level of the land.  In cases of thick  clumps,
                    however, the reverse result may be obtained:  the current
                    brings the dusts on the targets that are to be protected.

                                   TABLE H-2

                    PLANTS KNOWN FOR THEIR CAPACITY TO RETAIN DUSTS
                          (Modified from Berindan,- 1969)
                          Plant                    Units of
                         Species                  Dust Removal

                      Abies	   30
                      Picca	   30
                      Pinus	   30
                      Ulmus	   '7.3
                      Syringa	    2.9
                      Betula	    2.5
                      Tilia	    2.4
                      Acer platanoides	     1.9
                      Populus 	     1
                      Platanus   	
                      Fraxinus   	
                      Morus	    -

              (Original units in  gr/rn.c)

              Smith and Dochinger (1975) observed:

                      Trees  may be  especially  efficient  filters  of airborne
                      particles because  of  their large  size, high  surface to volume
                      ratio  of  foliage,  and frequently hairy  or  rough leaf,
                      twig or bark  surfaces.

*  Number 22 refers to Halitsky  (1962);  number 39 refers  to Moses  (1964); and
number 56 refers to Warren Spring Laboratory (1966).   Figure  7  can be located on
page 15 of Berindan (1969).

                                       11-22

-------
                      Numerous investigations, reviewed by White & Turner (1970),
                      have indicated that trees catch airborne nutrient particles.
                      These authors found that their mixed deciduous forest was
                      capable of annually removing 125 kilogram/hectare (kg/ha)
                      sodium, 6 kg/ha potassium, 4 kg/ha calcium, 16 kg/ha
                      magnesium and 0.1 kg/ha phospherous from the atmosphere.
                      Degree of leaf hairiness was inversely correlated with
                      particle retention.  Apparently the small droplets employed
                      had insufficinet inertia to penetrate the stable boundary
                      layer created by the hairy leaves.  Small diameter
                      branches were more efficient particle collectors than
                      large diameter branches in all species examined.

             Monteith (1975) states:

                      Once particles  are at rest on a surface,  surface
                      tension and other forces hold them, and the drag of the
                      wind is reduced by the viscous sub-layer, so they are not
                      easily disturbed.

             Warcen (1973), says that concentration of particulates is reduced
by 40 - 50% within the first 65' - 85' of forest adjacent to the edge.

             Smith and Dochinger (1975) comment:

                      Many investigators,  for example,  Raynor et  al.  (1966),
                      have shown that the concentration of particles carried by
                      an air mass through a woodland decreases rapidly from
                      the edge.

             Keller (1971) mentions:

                      The  powerful filter  action of  the  forest in regards to
                      dust  makes itself  felt most  impressively, however, in
                      reports  of figures  (Handbuch der  Staubtechnik,  Handbook  of
                      Dust  Technology,  1955,  by Meldau)  according to  which
                       1  Hectare  (ha)  of  spruce  forest  can fix  32 tons, beech
                      forest even 68  tons  of dust  until  the  filtering capacity
                      has  been exhausted.   This means  that in  an extreme case
                      the  forest could  fix several times the weight of its tops;
                      however,  these  figures should  be  regarded as very maximum,
                      in a way, as the  potential dust  collecting capacity of
                      the  forest.

             Podgorow (1967) states:

                       ...considerable quantities  of  dust are deposited on
                      1m  of the region which is adjacent to  the  city.  Plantings
                      growing in the  vicinity of the  city (500  -  1,900m)  retain
                      80.1% of  the precipitation/surface of ground dust.  From
                      this quantity up to 40.2%  can be attributed  to  the
                      pine needles.   Our investigations thus  showed  that  the
                      pine is a good  retainer of dust.   It  is,  therefore,
                      necessary to  include them  in  the plantings  of parks and
                      wooded areas which are close  to industrial  centers.

                                       11-23

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             Haupt and Flemming (1973) investigated the efficiency with which dust
is filtered out of the air by forests.  It is dependent upon the leaf and needle
surfaces and their species specific collecting capacity.  It was observed that coal
dust deposition was less during calm and wet periods and more during turbulent and
dry periods.  For example, dust deposition during April was 207 times greater than
in July.  In addition, rates of deposition at any one time were virtually the same
whether the collecting surface was vertical or horizontal.

             Lampadius (1963) determined that spruce stands on 1 hectare(ha) absorb
67-114 kg of sulfate which reduces the S02 content of the air by 18-40 grams.
Similarly, a ha spruce stand absorbs 32 tons of dust, pine absorbs 36.4 tons and
beech absorbs 68 tons, but no time span is mentioned in this comparative study.

             Relative to pollen, Zinke (1967) found that dispersion into a forest
is reduced by interception in the canopy.  That filter may remove 30% of the pollen
grams compared to the concentration in the air over an adjacent open field.

             Raynor et al. (1966) concluded that pollen grains are removed from
forest air more rapidly at low wind speeds than at higher speeds.  Impaction seems
important in the first 10 meters of travel into a forest and along the upper canopy
surface.  Decreased wind speed within the forest allows pollen and other aerosols
to settle out by gravitation.

             Neuberger et al. (1967) studied concentrations of ragweed pollen
within a dense coniferous forest.  They found that 80% was removed within the
first 100 meters of trees.  The efficiency of Aitken nuclei removal by coniferous
material averaged 34% while deciduous material averaged 19%.

             Weisser  (1961) investigated dust contents of forests.  One hectare
plots of spruce can contain approximately 32 tons of dust, Scotch pine, 35.4 tons,
and beech, 45 tons.  The average dust settling on a 100 meter square (m2) plot
ranges between 3,000 grams per month near a fossil fuel power plant, 1,072 grams
per month in a city, and 340 grams per month in a large urban park.

             Smith and Dochinger (1975) point out that under controlled wind
tunnel conditions, the deposition of particulates on rough, pubescent sunflower
leaves was 10 times greater than on smooth.waxy, tulip poplar leaves.

             Bernatzky (1968)  states:

                      The air in a city is impregnated with a large number of
                       kernels which become  the  nuclei  about which  such matter
                       as  exhaust gases and  radioactive substances  gather;
                       eventually they will  get  into  the respiratory organs where
                       they will work havoc.   (The kernels which we refer  to  are
                       particles of pollution  of a size measuring from one
                       millionth to one five  thousandth of a millimeter.)
                                     11-24

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                            TABLE II-3
                   NUMBER OF KERNELS IN ONE CM"
Big cities
Small towns
Country places
Coastal areas
Mountains:
 500-1000m
 1000-2000m
 above 2000m
Ocean
                Average
147,000
 34,300
  9,500
  9,500

  6,000
  2,130
    950
    940
               Max.
                 of  average
379,000
114,000
 66,500
 33,000

 36,000
  9,830
  5,830
  4,680
Min.
ge
49,100
5,900
1,050
1,560
1,390
450
160
840
(A.
Absolute
Maximum
4,000,000
400,000
336,000
150,000
155,000
37,000
27,000
39,800
Landsberg)
   Average values of air pollution have been found by Reifferscheldt
   in Germany shortly after the end of the war to be
Kernels
Dust particles
       Big cities
       200,000
           270
                   Country
                   8,000 per cm3
                   7-10
                 Air pollution varies according to hours of the day and
                 to the seasons of the year as well as to the height
                 above ground.  We may distinguish three levels:

                                    Just above ground
                                    Roof level (domestic heating)
                                    Level of factory chimineys

                 This means that high blocks of flats which are much
                 higher than other houses might easily reach their upper
                 storeys into zones that are polluted to a far greater
                 extent and where the amount of pollution is continually
                 kept on a certain level by the factory chimneys as well
                 as the smoke from the houses.  The content of kernels and
                 dust particles leads to the formation of a dust dome which
                 is responsible for ultraviolet (U-V) poorness and dimness
                 of sunlight (loss of 20%) in the cities.

                 The higher the buildings of a city, the more they do
                 to counteract the natural flow of air.  To overcome
                 friction, energy is used up. the draught action slows
                 down and thus an air cushion is formed above the city.
                 Oncoming air currents have to rise above this cushion and
                 the result is poor ventilation of the city.
                                11-25

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             Smith and Dochinger (1975) comment:

                      The annual mean concentrations of suspended particulate
                      matter in the United States urban areas range from
                      60 micrograms/cubicmeters (mg/m3) to 200 ug/m^.  The maximum
                      24 hour average concentration is usually approximately
                      three times the annual mean.  Urban areas generally have
                      higher particulate loads in the winter than in the summer
                      (Spirtas and Levin, 1971).


             b.  Carbon Monoxide (CO)

                 Carbon monoxide is one of the primary pollutants produced by
automobiles.  Studies have shown that the most effective receptor for CO are
soil microorganisms which apparently metabolize the gas.

                 Summarizing the findings of a recent study by the General
Electric Company on the dispersion characteristics of carbon monoxide cited by
Hagevik (1974) it was found that CO exhibits exponential decay with distance as
long as the path of the pollution is not obstructed.  Also,the concentration
of CO at the level of the automobile exhausts is inversely related to traffic
speed.  As the speed of the traffic increases, the concentration of CO decreases
due to the increased efficiency of the vehicles and the increased turbulence.
Although the distance required for the removal or decay of CO has been studied,
the impact of turbulance and canyon effect on the dispersion of the gas is not
clear.  Also, the shape and size of surrounding buildings appears to have an effect
on dispersion irrespective of wind velocity.  The General Electric study indicates
that peak values occur at impermeable walls, and the magnitude of CO concentrations
are related to traffic volumes on each side of the highway.  The example of an
open roadway cut is given the maximum concentration occurs at the two walls and
the minimum concentration occurs at the center of the roadway.  In an example
where there is a wall (or cut) along one side of the road and an open area on
the opposite side, the maximum concentration occured along the wall; where both
sides of the road are open to ventilation, the maximum concentration occurs in the
center of the roadway and decreases in both directions. (See Figure 11-15).


             H.E. Heggestad is cited by Hagevik (1974) as indicating that soil,
apart from vegetation, is important in removing pollutants from the atmosphere,
especially gas such as CO and ethylene which are not absorbed by green plants.
Apparently, it is fungal microflora which are the primary absorbers of CO.  The
soil is also a sink for hydrocarbons, a major automotive pollutant.

             Inman and Ingersoll (1971) found that non-sterile potting soil
reduced CO concentrations in a chamber from 120 parts per million (ppm) to zero
within a three hour period.  When sterilized, the soil removed no CO.  Furthermore,
soil absorption of CO was apparently dependent upon high organic matter content and
low pH.


                                       11-26

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             ti.  Ozone  (03)

                 Aldaz  (1969) reported that bare, dry soil removes about 75%
more ozone than when it is moist while the opposite is true when vegetation is
present.  Relative to water bodies, it was reported that ozone is removed from
the atmosphere about 15 times faster over land areas than over sea water.

                 In 1970 Fesler reported that tobacco plants were generally most
sensitive to ozone concentrations coincident with low nitrogen fertilization levels
(60 Ibs./acre), and high levels least sensitive was found for plants treated with
an intermediate level of nitrogen fertilization (120 Ibs. N/acre).

                 Babich and Stotzky (1974) concluded that the removal of ozone
from the atmosphere by soil is directly dependent upon the moisture content and
surface texture of the soil.  Soil compaction and increasing moisture content both
decrease exposed soil surfaces and porosity and therefore, decrease the sink
capacity of that soil relative to ozone removal.  They also feel that the removal
process is essentially a physical and chemical process with soil micro-organisms
possibly serving as additional active decomposers of ozone.

                 Smith and Dochinger (1975) report that herbaceous species
absorb more ozone than do woody species and that as an example the deposition
velocity determined for a petunia species was about 9 times greater than an oak
species.


                 Turner et aj..(1974) investigated the dispersion and absorption
of ozone as it passes through forested areas.  They found a 10% decrease in
concentration as the ozone containing air passed through about thirty meters of
forest.

                 Davis  (1975) calculated that an average shade tree contains
4,300 square feet of leaf area and that if one assumes an average 8 hour 03
concentration of 0.17 ppm, and an 03 diffusion resistance of 0.33 min/cm,
about 27% of the ambient 03 would be removed if the air passed into the canopy
at a speed of less than 0.1 miles per hour.

                 Braun  (1974) found that the penetration of solutions under
natural conditions occurs mainly through the cuticle and not tnrough the stomata.
Therefore, foliar uptake is significantly affected by the chemical composition of
the cuticle of each species as well as by the mobility and solubility of the
pollutant in question.

                 Smith and Dochinger (1975) also point out that herbaceous species
absorb more ozone than do woody species.
                  Bennett and Hill.(date unknown) determined that under
 favorable growing conditions, air pollutants tend to be taken up by vegetation
 in the exposed and upper portions of dense canopies.
                                      11-97

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             d.  Sulfur Dioxide (S02)

                 Sulfur dioxide is a gas produced primarily by the burning of
fossil fuels, it is generally considered an industrial pollutant rather than
associated with vehicular traffic.  It is believed that S02 (and other water
soluble gases) pass into the plants through the stonata and go into solution within
the plant itself.

                 The following studies cited by Smith and Dochinger (1975)
illustrate these processes.

                      Speeding (1969) investigated the uptake of S02 by
                      barley leaves and found a 6-fold increase in average
                      deposition velocity with open stomata compared to closed
                      ones.  In related work, Rich and Associates (1970)
                      reported that uptake of ozone (03) by bean was regulated
                      by the same factors that control the exchange of water
                      vapor between leaves and the atmosphere.  This conclusion
                      is also supported by Thorne and Hanson (1972).  Once
                      inside the leaf gases probably become dissolved in water.
                      Hill (1971) compared the rates of uptake of pollutants by
                      alfalfa with the water solubility of the pollutants.
                      Fluorides had the highest water solubility and uptake.
                      As the rates of uptake of pollutants decreased, their water
                      solubility was also reduced.  Any factor that affects the
                      stomata influences the uptake rate of gaseous pollutants.
                      Some of the environmental factors that are important in
                      the action of stomata are light, humidity, temperature,
                      wind, and the available supply of soil water.

                      Atmospheric pollutants themselves are also reported to have
                      an effect on stomatal activity.  Majernik and Mansfield (1970)
                      and Unsworth et al. (1972) reported that SO2 caused stomata
                      to open faster in the light, to achieve a greater aperature,
                      and to close more slowly in darkness.  All of these would allow
                      for the absorption of more S(>2.

             Berindan (1969) describes the process in the following excerpt:

                      As regards  the action  of  green  spaces  on  gaseous
                      pollutants, it is much less known since research aiming
                      at determining it has been more restricted and more
                      recent..."

                      So far the  retention of sulphurous gas, fluorine,hydrogen
                      sulphide, and nitrogen oxides has been established.  Or
                      all of these mechanisms of action, S02 is very well known,
                      its diagram is shown on Table II-4.  This table explains the
                      absorption process of sulphur by plants, wherein it can
                      pile up to a given level, which once exceeded, entails the
                      deterioration of the plant.
                                        11-28

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                 Blum  (1965) in a review of the literature found that a  mature
beech stand served  to  filter S02 from the air in the vicinity of a smeltery.
This beech stand protected an adjacent, enclosed stand of spruce which died in
response  to removal of the beech trees.

                 Davis (1975) reported that the use of fertilizers can increase
the resistance of plants  to S02 damage, but that they do not necessarily relate
to the  rate of S02  uptake by this vegetation.

                 Murphy et pi.  (1975) determined that the diurnal pattern of
S02 uptake by plants reflect changing sun light patterns and temperature as they
affect  stomatal functioning and S02 solubility.  Seasonal changes in day length
and leaf  area are key  variables and the  formation  of dew and the vegetation can
form a  very sizable sink  for the transient absorption of SC^.

             e.   Gases - General & Miscellaneous

                 Smith & Dochinger (1975)

                       In  the  case  of  gaseous  pollutants, much  of  the  evidence
                       comes from controlled environmental studies  with non-woody
                       species.   We do not have adequate information to document the
                       ability of trees to remove "meaningful" quantities of
                       pollutants from actual urban atmospheres.  Trees have yet to
                      be shown to be capable of reducing a  particular air
                      contaminant below a significant threshold of effect for any
                       urban area.

                      The  primary method  of vegetative  removal  of  gases  from
                       the atmosphere is via uptake through  the stomates.   Minor
                      methods by which plants remove gaseous pollutants from the
                       atmosphere may include uptake by plant surface microflora,
                       uptake through bark pores and absorption of  gases to the
                      surfaces of plant parts.

                      The  processes  of  transpiration  and photosynthesis  require
                       that plants exchange gases with the ambient  atmosphere
                       through leaf,  branch and stem pores.   Contaminant gases
                      present in the atmosphere in the vicinity of a plant may be
                      absorbed when the stomates of lenticels are  open.

                  Shclterbelts  and windbreaks  have  traditionally been  used  to
alter microclimate in various  ways,  primarily by slowing down wind speed and reducing
evapotranspiration.


                 World Meteological Organization (1964)  cites:

                       ....in  Canada,  after experiments at  the Soil Research
                      Laboratory,  Dora.  Exper.  Sta., Swift Current,  Saskatchewan,
                      as by Matjakin (1952)  and Panfilov in the U.S.S.R.  (1937).
                      According to  these  two  an impermeable belt of woodland
                      hardly lets  the  wind through  at all Immediately behind the
                      wind is  almost completely calm and when it returns to earth
                      in the lee it  is  very turbulent.   A belt  of  medium permiability
                      with numerous  small holes distributed evenly over  the entire
                      belt acts as  a sieve,  preventing  turbulence  to a large
                      extent.


                                       11-29

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                                        TABLE  11-4

                               PROCESS  OF  SULFUR ABSORPTION  BY  PLANTS
so2
sterna tes
SO-
sulphites—fr absorption and transformation
             in sulphates (the decrease by
             30 times of the toxicity as a
DEPOSITS of sulphites
gradual increase
                                     .result of the slow process of oxidation)
                                                                           localized chronic lesions
closed          opened
-darkness       -heavy light
                -increased relative humidity
                -humidity reserve
                -moderate temperature
                                      incomplete metabolism
                                      in organic sulphur

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                 Thus,  by using plant materials to break up the winds, a great amount
of exposure of the air currents to the leaf surfaces occurs.  This results not only in
slowing  down  the wind and allowing particulates to  settle  out but enables  the gaseous
pollutants to be taken up by the leaves.  Furthermore,  the turbulance created by
the air passing through the shelter belt forces the air current down toward the
ground where CO can become engaged by soil microorganisms.

                 Turner  et  al.  (1974)  investigated  the  dispersion and absorption
of 03 as it passes  through  forested  areas.  They  found  a  10% decrease in
concentration as  the 03  containing air passed  through about thirty meters  of
pores.

                 Davis  (1975)  calculated  that  an  average  shade  tree  contains
4,300 square  feet  of leaf area and that if  one assumes  an average 8  hour 03 concen-
tration  of 0.17 parts per million (ppm),  and on 03  diffusion resistance of 0.33 m
minute per centimeter  (min/cm),  about  27% of the  ambient  63 would be removed  if
this  air passed into the canopy at a speed  of  less  than 0.1 miles per hour.

                 Makarov and Dokuchayev (1970) found that there is a considerable
variation in  the  liberation of nitrogen dioxide  (N02> during the growing   season.
Reduced  generation rates are associated with treatments which  suppress miceobial
metabolism.
         3.  Organization of plantings

             Factors effecting the efficiency and functioning of buffers are
similar  to windbreaks and shelterbelts.  In both cases the importance of
breaking up and slowing down air currents is essential.

             World Meterological Organization (1964)states:

                      Windbreaks and shelterbelts alter 'the air flow primarily
                      according to strength, direction, and degree of turbulence.

                      We can for the moment forget whether a windbreak be artificial
                      or of natural growth.  Effective protection and the
                      influence on the windy area are not directly dependent on
                      this.

                      The deciding factor for wind reduction with shelterbelts
                      is the belts*s density permeability.

                      Immediately behind very dense belts wind reduction is
                      at its greatest; with increased permeability it becomes
                      less.  At wind minimum, wind reduction is also a function
                      of permeability, called "covering degree" by Tanaka  (1956).
                      With dense belts the position of greatest wind reduction is
                      very close to the belt; yet it is furthest away when the
                      belt is of medium density.  According to George  (1960)
                      maximum wind reduction occurs immediately in the lee of a belt
                      of 10 rows, shifting to 2.4 x H with 5 to 7 - row belts.
                      Similarly the distance behind belts where wind reductions
                      are still at least 20% is  greatest behind belts  of medium
                      density and  least for very dense and very loose belts.
                                       11-31

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The different density belts show different curves of wind
speed on their leeward side.  So it is not permissible to
judge the sheltering effect of belts,  as Den  uyl did (1936)
only on measurements taken at small distances.  From the curves
it can be concluded that where wind reduction extending far
behind the belts is required, more than sharp reduction,
high belts of medium density are the best (Naegeli, 1946;
van der Linde, 1958).  The smaller extent of wind reduction
with dense belts is a consequence of the stronger displacement
flow and the greater power of recovery that this gives
the surface wind.  The wind recovers speed behind denser
belts more quickly than it was reduced.

Blenk & Trienes  (1955) also studied the effect of different
shapes of belt with four impermeable models 30 millimeters  (mm)
high in the wind tunnel.  One of them was 1 mm wide, the
other three 15 mm, of which one was right-angular in cross-
section, with sharp edges; the other two were rounded off
in different degrees.  The model most rounded off on the top
edge had the least extent of wind reduction; the one with
less had a little greater extent, and the best proved to be
the sharp-edged sheet 1 mm wide. (See Figure II- 12).

In the Russian terminology a permeable belt is a wood
plantation with large gaps running right through.
These belts in the U.S.S.R. mostly have bare, 1 to 2 inch
thick trunks without undergrowth or stunted threes.

With such belts eddies would be prevented particularly
near the surface by the wind penetrating the lower parts.

A permeability of 40 to 50% can be obtained by various
sizes and shapes of opening.  According to Naegeli  (1946),
Nffkkentved (1938), Konstantinov (1950), many small
openings are especially effective.  Blenk and Trienes (1955)
compared three strips 30 mm high with a permeability of
50%, but with different sizes of opening, in the wind tunnel.
The wind distribution behind those with openings of 2 and 5 mm
diameter was almost equal.  The strips with openings of 8 nun
reduced wind for a considerably shorter distance.

In the open, where the degree of permeability is hard to
estimate, van der Linde (1958) classes well cared for leafy
blackthorn or yew hedges as dense, counting belts of Lombardy
poplar among those of medium density.  Eucalyptus makes
equally good belts of medium density in warm, semi-arid areas,
but according to Duncan (1950) belts of "thin cottonwood"
20 m high belong to the very loose and least effective.

Shelterbelts of  deciduous  trees vary in  density with the
season.  According to Flensborg and N^kkentved (1940)
the seasonal differences with loose belts in Denmark were
slight; in the autumn dense belts assume the character of
medium, and medium that of loose.  The protective effect
of leafless belts is not to be neglected, however.  Figure II-8
shows the wind conditions at a belt of medium density 16m
high with and without foliage  (Naegeli, 1946).
               11-32

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                    FIGURE II-8


THE SHELTER PROVIDED BY A 16-METRE-HIGH SHELTERBELT OF
DECIDUOUS TREES IN SUMMER AND WINTER (NAEGELI, 1946)
    wsw
                                                        WSW - Wind
                                                        Summer
                                                        Winter

                                                        ENE -Wind
                                                        Winter
         According to Jensen (1954) and N^kkentved (1938) leafless
         belts generally gave 60% of the shelter with folage.  In
         northwest Germany, Franken & Kaps (1957) found about 50%
         less wind reduction at three, four and seven belts when
         without leaves.  Similar evaluations were made by von
         Eimern (1957) at a two row belt of maple 12m high with
         undergrowth.

    Berindan (1969) states:

          ...some guiding concepts may be defined for the planting
         of green spaces for sanitary protection:

           a)  The necessity of a correlation between the type and
         the concentration of the pollutant and the degree of resistance
         of plants;

           b)  The necessity, in some countries, of checking, through
         research and experimentation the findings on the resistance of
         plants, since the uncontrolled inplementation of the findings
         could lead to erroneous or inefficient solutions;

           c)  For each situation, the degree of toxicity of the
         pollutant or the mixture of pollutants must be known in
         order to select species which have adequate specific resistance;

           d)  In so far as the height of the plantings are concerned,
         in the first place, it must be recommended to plant trees, shrubs
         and/or to plant some turfs only to supplement their retention
         capacity.  In the last analysis, flowers are used for
         decorating roads.  The same applies to fruit trees, provided
         however that they are resistant and are not exposed to
         accumulation of toxics, otherwise planting them will be useless,
         costly and sometimes even dangerous;
                          11-33

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                        e)   Aerated structure plantings, obtained by grouping
                      curtains or rows of trees can better retain dust or even
                      gaseous pollutants, than compact clumps, due to the filtering
                      action of the former.  To this end, the form and composition
                      of cross sections of green barriers, function of the effects
                      desired and resulting from the draughts generated are to be
                      closely studied;

                        f)   It is necessary to place dust collecting plants by order
                      of capacity: those that retain large particles are to be placed
                      close to the source; and further off, those which stick to
                      the smallest particles.

         4.  Maximizing buffer edges to increase sink potential

             It is clear that the most diverse and most important part of forests
 (and buffers) for the purposes of reducing pollutants is the area within the buffer,
adjacent to the edge. Warren (1973) previously cited, indicates that the most effec-
 tive and efficient zone for this purpose lies within 65 - 85 feet of the edge.
This is due to the greater diversity of plant materials within this area.  Generally
 the canopy occurs at all elevations not only at the top as it is further into the
 forest interior  (See Figure  II- 13).

             Obviously  in the design of effective buffers,  techniques to Increase the
edges are of great importance.   This is true not only for newly planted installations
but for existing forests and woodlots as well.

         5.   Ventilation of buffers and woodlots to increase sink potential

             As previously indicated,  thermal chimneys within a forest can
increase deposition of  particulates and absorption of gases by increasing ventilation,
and exposing pollution laden air to leaf surfaces high in the interior canopies.   Such
a phenomenon can be built into buffers or existing forest areas by the creation of
openings in the interior forest canopy. (See Figure  11-14).


         6.  Importance of local adaptation of plants to local site conditions

             World Meteorological Organization  (1964)states:

                      As the extent of the protective effect of belts is
                      proportional to  their height, it is often  (in the U.S.S.R.
                      for example) considered an advantage to plant belts which
                      reach a maximum  height dependant on soil and climate, for
                      which purpose the types of tree and bush particular  to
                      that landscape are selected.

                      Width and shape  of belts are not always decided from the
                      aspect of best wind reduction;  forestry also plays a
                      large part.  Because of maintenance, care  and  their possible
                      use  for other purposes, wider belts of more than 5 -10m
                      are preferred in many climates.  In such belts part  of the
                      wood can be  used elsewhere without appreciable harming
                      the wind reducing effect, and  they are often.'capable of
                      reducing themselves; filling  gaps  left by  dead wood with new
                      growth.  In  any  case they seldom leave such large  gaps that
                      harmful nozzle effects evolve...

                                   11-34

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Smith and Dochinger (1975)  state:

          1.   Trees selected or bred to provide this  amenity function
         must be tolerant of acute,  adverse influences or air pollution.
         Clearly if the tree is severely damaged or killed by one or
         an interaction of  contaminants       utility as  a sink will
         be short-lived.   In addition to air pollution tolerance,
         suitable tree varieties should be capable of withstanding other
         urban stresses,  such as poor soil aeration and drought,  nutrient
         deficiencies and microclimate extremes.  A suitable variety
         should be able to grow vigorously.  Vigorous growth will
         require maximum stomatal aperture and ensure maximum uptake
         of gaseous pollutants.

          2.   Coniferous  species retaining their foliage  year round
         may appropriately  be favored over deciduous  species.   The
         atmospheric burden of both  particulates and  gases is generally
         higher in the winter than in the summer for  most urban areas.
         It is important,  therefore,  to have maximum  plant surface
         available for absorption and adsorption during winter months.
         Since the time of  persistence of foliage of  evergreens is
         longer than deciduous foliage, the opportunity for pollutant
         removal is correspondingly  longer.  The morphology of coniferous
         foliage (for example; pine,  spruce,  fir) results in a high
         surface to volume ratio which may be instrumental in more
         efficient removal rates.
          3.  Since petioles are especially efficient  particle receptors,
         species with long petioles  (for example; ash, aspen,  maple)
         may be favored.
          4.  Surface hairiness on plant parts (leaves, twigs, petioles,
         buds), may be especially effective for retention of particles.
         Those species processing these hairs(for example; oak,birch,
         sumac) should be considered.
          5.  Species with small diameter branches and twigs should be
         selected or bred over species with large diameter branches
         or twigs as the former are  more efficient particle collectors.
          6.  Since gases are removed from the atmosphere  primarily by
         the stomates, species should be selected or  bred with maximum
         stomatal capacity for absorption.  This ability  may be related
         to absolute stornate number  per unit of leaf  surface, size of
         stomatal capacity number per unit of leaf surface, size of
         stomatal aperature and length of time the stomates are open.

          7. Species should be selected or bred that  have maximum
         resistance to stomatal closure occasioned by environmental
         variables such as moisture availability, temperature, wind,
         light intensity and air pollution.
          8. Selection and breeding should consider one relative ability
         of tree species to utilize pollutant gases as partial sources
         for required nutrients.

                          11-35

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         7.  Ecological approach to roadside treatment.

             Using natural succession as a basis for roadside management.
resulting in increased sink potential, reduced maintanence costs.
             Odum (1971)
                                   TABLE II-5
               ECOLOGICAL CHARACTERISTICS OF COMMERCIAL FORESTS AS
               CONTRASTED WITH PROTECTIVE GREEN BELT VEGETATION
Features

Species diversity

Age structure

Annual growth increment

Stratification



Mineral cycles



Selection pressure
Maintenance costs  (re-
   planting, fertiliza-
   tion, pest control,
   thinning, etc.)

Stability  (resistance to
   outside perturbations
   such as storms, pest
   outbreaks, etc.)

Overall function
Commercial Forest

Low (usually monoculture)

Even-aged

High

One-layered (mostly
  canopy trees)
More open (losses from
  leaching and run off)
For rapidly growing, sun-
  adapted species  (often
  softwoods)
High  (requires "manage-
  ment")
Low

Production of    '-rket-
  able products
Green Belt Vegetation

High (mixed species)

Multi-aged

Low

Multi-layered (under-
  story, and ground
  cover well developed)

More closed (retention
  and recycling within
  stand)

For slower-growing,
  shade tolerant spe-
  cies  (more hardwoods)
Low  (self-maintaining)
High

Protection  of  the  qual-
   ity  of man's envi-
   ronment
             Use  of mixed  plantings  - mixed  canopy  trees,  and  shrubs - deciduous
 and  evergreen  to  increase  sink potential,  screening headlights of oncoir'.ng cars,
 reducing maintanence  costs,  protecting wildlife,  etc.
                                       11-36

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 Rich (1972) comments:
          Many species of roadside trees suffer moderate to severe
          injury from sodium chloride applied to the highways in
          winter to prevent ice formation and to aid in snow and ice
          removal.   Trees within 30 feet of the edge of the highway are
          affected most frequently and most severely..." Canadian
          hemlock,  balsam fir,  white and red pine,  and sugar and red
          maple, basswood and American elm are among the most sensitive.

          Tolerant species include: red oak,white oak,  white ash,  black
          locust,  quaking aspen,  black cherry,  black birch,  grey birch,
          paper birch,  yellow birch,  Norway maple and red cedar.

 Odum (1971)  states:

          The first and most  important  consideration in planning and
          managing  the  urban  greenbelt,  then is diversity.

          Too often tree plantings in urban and suburban areas  end up
          as  even-aged  monocultures with no provision for understory
          young trees that could  replace the old ones as they die
          or  become diseased.
          A second  important  ecological consideration involves  careful
          selection of  species  and varieties  that are naturally disease
          resistant,  and adapted  to soil, water,  light,  topographic
          and other conditions  of the microhabitat.   When trees are
          planted outside of  their preferred  habitat (bottomland trees
          planted on dry uplands,  or  vice versa,  for example)
          a lot of  maintenance  (watering, fertilizing,  etc.)  may be
          required.

          Also, the metabolic cost of adapting  to the suboptimum
          condition makes the tree vulnerable to disease or  drought.

 Williston (1971)  comments:

          Trees will lower right  of way maintenance costs.   Grasses
          need to be periodically fertilized to maintain good cover
          on  roadbanks; trees do  not,  and yet they  control erosion
          well. Trees  eliminate  the  need for weed  control and  for
          maintenance mowing, which can cost $10. or more per acre
          per year.  (Costs are  1971 - add 10%/year).

Odum (1971) states:

Shrubs in the buffers are important.

          1.   Shrubs, and leafmold they produce, enhance soil
         moisture, encourage useful soil decomposer organisms,  and
         help in self-fertilization of nutrient recycling.
                          11-37

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                       2.   Shrubs,  especially evergreen ones,  are very effective
                      noise barriers.   Robinette (1969),  for example,  points out
                      that a band of dense shrubs backed by several rows of
                      trees along a highway or street can reduce noise of traffic
                      or garbage collection ten-fold.   In such a case  sound is
                      not only absorbed by twigs and foliage of shrubs,  but it is
                      reflected upward (away from hearer)  by trees. Trees alone
                      would have very little value in noise abatement  at close
                      range.  Since noise pollution is rapidly becoming critical,
                      it could well be that plantings structured to mimic a
                      multi-layered natural forest could be more valuable for noise
                      abatement than for any other purpose.


                       3.   Shrubs and other understory vegetation are  absolutely
                      essential for songbird populations.   I think we  will all
                      agree that pleasant sights and sounds of songbirds are a
                      desirable point of the urban landscape.   Among desirable
                      birds only the robin thrives in habitats containing the
                      only tall trees and grass or other ground cover.  Most
                      songbirds (mockingbirds,  brown thrashers,  thrushes,  towhees,
                      song sparrow, etc.)  require shrubs  or understory vegetation
                      for  nesting and escape shelter.  Contrary to most people's
                      ideas very few songbirds nest high in trees.  In a study of
                      bird nesting heights,Preston and Norris  (1947) found that
                      80% of bird nests were between 3 and 18  feet above ground
                      with the median height being 7 feet.  For more about the
                      dependency of songbirds on the understory see Odum and Davis
                      (1969).

         8.  Size of buffers.

             Warren (1973) feels that greenbelts should be a minimum of 100 to
120m. wide and should channel the wind to provide a maximum dispersion for the
gaseous pollutants.  The width must depend on the pollutants and local conditions
and could range up to 2,000 feet.

             Buffers adjacent to highways should be planted with trees and shrubs
as close to the highway as safely possible.  Also, forested or planted medians
should be provided.  They should be at least 15-30m. wide and average  10-20m. tall.

             Hagevik (1974) states:

                      Peter Rydell and Gretchen Schwarz cite a Russian study
                      which concludes1that the concentration of pollution decreases
                      by about half over 500 meters of planted land1.   I.A. Singer
                      also notes a 75% reduction in dust particle count over a 600
                      foot wide strip of open space.
                                     11-38

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                      Frank Cross  determined  the size  requirements  for  a  buffer
                      zone to protect citrls  groves  from fluoride emitted from
                      a phosphate  plant gypsum pond.   Based  upon a  standard where
                      75 parts per million of fluoride in citrus leaves was considered
                      to be evidence of pollution a  one half mile buffer  strip was
                      established  around the  pond to alleviate the  fluoride effect.
                      In another case,  Cross  defined a zone  for suspended particles
                      emitted from a dolomite processing plant, and concluded that
                      to reduce the adverse impact of  settling particles  upon
                      nearby residents, a buffer of  1,500 feet radius around  the
                      plant site would be required.  A third study  by Cross inves-
                      tigated the  buffer width needed  to restrict ambient air
                      particulate  concentrations from  a hot  mix asphalt plant to
                      100 micrograms per cubic meter.   Results indicated  that a
                      buffer zone  of one mile radius reduced particulate  concentration
                      to the determined level.


             Bernatzky (1968) in West Germany feels  that to  reduce  gases  the
stands need to be 5 times deeper than their height on  the windward  side and 25
times deeper than their width on the leeward.

             Corn (1968) comments:

                      Numerous studies have found that particulate  dispersion
                      is directly  related to  the source and  receptor.  It is
                      difficult, however, to  establish a specific  distance as a
                      guideline for buffer width, since dispersion  depends upon
                      factors other than distance alone.

                      The acutal direction of transport is determined by  large
                      scale circulation in the atmosphere as well  as by the local
                      influences of breezes,  the surface features  of a  specific area,
                      heat sources (such as the higher temperature  observed over
                      urban areas) and air masses of differing densities."

         9.  Safety factors as design considerations.

             Williston (1971) states:

                      Planting areas must be  carefully selected lest they
                      interfere with the drivers' safety.  Trees growing to a
                      diameter breast height(d.b.h.) of at least 4 inches or
                      larger should be planted 30 feet or more from the edge of
                      the pavement, smaller trees at least 20 feet.  Care must
                      be taken that as the trees grow they do not  form a tunnel,
                      causing drivers to crowd the centerline.  On cut sections,
                      plan at least 6 to 8 feet up the slope from the edge of the
                      ditch and do not plant fills.

                      Screening headlight glare by planting  trees  on the median
                      strip is most needed on level ground.
                                       11-39

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             According to Everett (1974) there is a very real danger in exercising
in areas of heavy traffic.  Many cyclists ride along crowded roads and joggers
running along arterials are common.   Also many other types of active recreation
facility are initially located along roads which are later improved to accommodate
high volumes of traffic.

             Studies indicated that levels of pollutants in air along such corridors
may be as much as 10 times higher than ambient pollution.  Heavy exercise in these
zones can cause particulates and other harmful pollutants such as lead, and asbestos
can be pulled deep into the lungs and deposited there.  Also, as a greater volume
of gaseous pollutants are pulled over the particulates, the possiblity of synergistic
reactions is increased.

             Buffer strips intended to be used in conjunction with active recreation
areas should separate such facilities from heavily traveled roads with heavy planting.
Although no specific dimensions have been identified for this purpose, Warren (1973)
indicated that 40-50% of concentration of particulates is removed by the first 65 -
80 feet of forest.  An 80 foot minimum would probably be reasonable.
         10.  Sound absorbing qualities of buffers.

              It has  been adequately shown that plant materials acting as
buffers can effectively absorb sound.  Hagevik states that, generally,  intensities
greater  than 120 d 6(A) may cause pain to the human ear and that physical damage
may result at  160 d B(A) especially if the  exposure is prolonged.

             There apparently are conflicting opinions as to the importance of
the sound frequency  (cycles per second or o.p.s.) but Embelton  (1963) suggests
that attenuation is independent of frequency tange of 200 -  2000 c.p.s. for
all tree types  including deciduous trees in full leaf.  Gerhard Reethof  (1972)
indicates that  trees 40-50 feet tall planted in a buffer 100' wide can  reduce
noise by 5-8 dB. His data supported Embleton's conclusions.

             Reethof (1972) states:

                       ...other studies point out the difficulty in making
                      definitive statements concerning the value of trees in
                      reducing noise.  For instance, assuming that noise reduction
                      in the 300 - 800 c.p.s. range is desirable and  that a
                      25 d B(A) reduction is required, based upon Embelton's
                      data, a dense, coniferous growth, approximately 400 feet wide
                      would be needed; data compiled by F.M. Weiner and
                      D.N. Keast (1959) indicate that a 1,900 foot wide belt
                      would be necessary for the same reduction.

             Hagevik (1974) cites two recommendations of Cook and Haverbeke (1971)
which indicates the possibility of reducing noise levels to 5-15 dB.   Specifically,
for high speed  vehicular noise, they recommend planting a 65 -  100 foot wide belt
of shrubs and  trees with the edge of the belt within 50 - 80 feet of  the middle
of the traffic  lane nearest the buffer.  Trees in the center of the buffer should
be at least 45  feet high.
                                         11-40

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                                 FIGURE  I1-9

                        DESIGN PARAMETERS OF BUFFERS
                            FOR SOUND ATTENUATION
                        - AFTER COOK AND HAVERBEKE,(1971)
               (£Road
                        20-50'        20-50'
              For  moderate speed  traffic
             <£ Road
                       50-80'         65-100'
              For  high  speed  traffic
             In cases where the  traffic speed is moderate,  the belts need only
be 20 - 50  feet wide with shrubs along the edge.  This should be placed 20 - 50
feet from the middle of the nearest  lane of traffic.  The shrubs should be 6 - 8
feet tall with trees being 15 -  30 feet high.  See Illustration  II-9.

            The characteristics of  plantings upon which sound attenuation is
dependent are height, density, and width.  Hagevik cites a study by Peter Durk
which indicates that a 50 meter(m) wide buffer or park can result  in a 20 - 30 dB
reduction of noise level.  Odum (1971) also  references the use of  vegetation as
a buffer for noise  (See page 11-37).
                                      11-41

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     C.  POTENTIAL DESIGN ALTERNATIVES

         After reviewing the available literature,  certain guidelines for
establishing and maintaining healthy, efficient greenbelts become evident.
Examples of the authors' recommendations and data may be located in the Liter-
ature Search Findings section and also, Sections III and IV of Volume I.
The information for creating greenbelts that are efficient sinks of airborne
contaminants is summarized below and this material is the basis for the
design alternatives of highway buffers.

         Summary of Literature Search Findings:

         1.  Evaluation of the environment -La necessary before selecting or
breeding plant species that will compose the greenbelt which functions in the
improvement of air quality.

             Two factors which dictate plant growth are climate and soil.  The
degree of the protective effect of greenbelts is dependent on the amount of
growth which is expressed by the vegetation, particularly in terms of height.
Vegetative buffers which attain maximum height asre generally mare efficient
in the role of sinks for air pollutants.  Since climate and soil greatly influence
whether vigorous growth will occur, both of these elements of the environment
should be analyzed before determining the most suitable woody plants for a
greenbelt.  Plant species that are unable to adapt adequately to both the
climate and soil will not sufficiently remove airborne pollutants.

             Poor soil conditions will cause harmful stresses on even the most
tolerant plant species.  To alleviate the primary detrimental effects produced
by poor soil in terms of plant growth is to relieve any deficiencies in water
or nutrients and also, to provide proper aeration of the soil.  By taking
such measures, the general health of the vegetation may improve and the plants
may be capable of more than merely existing; active growth may actually occur.
Vigorous growth requires maximum stomatal aperture which ensures optimum uptake
of atmospheric pollutants.

             However, the energy expended in improving the soil will not
produce satisfactory  results if  the plants are not growing in their preferred
habitats.  Plants surviving in a suboptimum environment will not significantly
                                 11-42

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participate in the removal of air pollutants.   Also,  the metabolic cost of
adapting to less than favorable conditions may cause  the plants to become more
susceptible to disease and drought.

         2.  Selection or "breeding of plant species that can withstand the adverse
effects of the air pollutants that are present in their potential habitats is
essential to contribute to the health of the greenbelt.
             A woody plant that is extremely sensitive to one or a combination
of pollutants will be a poor sink due to irreversible damage and even death
of that particular plant.  The degree of resistance of plants is correlated with
the type and the concentration of the pollutant.  The Plant Species Sensitivity
List, which is located in Volume I and also, in Volume II, this Volume, as
Appendix B, provides lists of plant species which are either relatively tolerant
or sensitive to some of the primary types of air pollutants:  fluorine, hydrogen
chloride, nitrogen dioxide, ozone, PAN, particulates - smoke, sulfur dioxide.
Since vegetation is usually exposed to a combination of pollutants instead
of a single pollutant, lists of relatively resistant and sensitive plants
for general pollution also have been developed.
         3.  Removal rates of air pollutants by vegetation and soil types
should be considered in attempting to increase the efficiency of roadside
forests and buffers as air pollutant sinks.

             General estimates of the removal and emission rates of air pollutants
by vegetation and soil types are given in Volume I.  These values are arranged
in tables headed by the pollutants ammonia, carbon monoxide, fluorine,
hydrocarbons, nitrogen oxides, ozone, PAN, particulates, lead, and sulfur dioxide.
By reading the literature about air pollution and natural elements and extracting
the pertinent information from the research papers, the data was carefully
evaluated and limitations of the presently available information were observed.

                                    11-43

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These limitations of the literature are discussed in the introduction of Section III
in Volume I.  Therefore, it is essential to recognize that the removal and emission
rates are general estimations which are based on information that is very limited.

             However, the tables provide some guidelines for mitigating air
pollution problems by the utilization of soil and vegetation.  A utility factor of
1,2 or 3 was assigned to each given value.  The utility factor of 1 means that
the research team attempted to measure field conditions and the methods for
obtaining the data seemed appropriate.  Results that were less applicable to the
tables were given utility factors of 2 and the least applicable data was designated
as being 3.

             Table III-ll on page 111-40 of Volume I is a summary table which
was developed by selectively averaging the sink and emission factors for each
pollutant.  The purpose of this table was to find figures which roughly approximate
the data obtained from the reviewed publications.

             The tables of the section on Sink and Emission Factors for Natural
Elements are tools for landscape design in terms of natural removal of air pollution.
By referring to these tables and the Plant Species Sensitivity List, the effectiveness
of a particular natural element for removing a specific pollutant may be estimated.
Also, Table III-ll of Volume I, which provides very rough estimates for absorbing
and emitting specific pollutants by vegetation and soil, displays much larger
concepts of the effectiveness of natural elements in removing airborne contaminates.

         4.  Plants that have certain morphological characteristics are
relatively more efficient particle and gas receptors.

             In addition to selecting or breeding tree  and shrub species  that
are  relatively resistant to the types and concentrations of air pollutants present
in  their potential habitats, the morphological aspects  of these species should
also be considered.  Certain physical characteristics  that are especially
efficient  pollutant receptors have been identified  in  the literature, particularly
                                       11-44

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in Smith and Dochinger (1975).   These characteristics are listed below
and species with several of the features should be selected or bred over
species that lack most of the advantageous characteristics.

                 a.    Petioles are effective in the retention of particles and
there is a correlation between the length and the collection.'capacity of the
petiole.
                 b.    Surface hairiness on leaves, twigs, petioles, etc.  trap
the particles more readily than the plant parts that are smooth in texture.
                 c.    Generally, more particulates are deposited on small
diameter branches and twigs as compared to large diameter branches and twigs.
                 d.    Maximum stomatal capacity for absorption is a significant
characteristic in plants potentially used in greenbelts since the primary
mechanisms for removal of gaseous pollutants are by stomatal processes.
                 e.    Species having maximum resistance to stomatal closure
caused by environmental variables are preferred for removal of airborne pollutants
than species in which stomatal closure occurs due to slight changes in temperature,
moisture, light, or air pollution.
                 f.    Plants that more readily metabolize substances extracted
from the atmosphere may be considerably more suitable for greenbelts than
plants that lack the capacity to utilize contaminated air as a partial source
for essential nutrients.

         5.  Multi-layered stratification is a characteristic of an efficient
roadside forest for absorption and adsorption of air pollutants.

             A stratified forest, formed by developing the understory and
ground cover as well as the upper tree layer, is a more effective receptor of
air contaminants than an unstratified forest.  However, if the strata of a
forest, particularly at the edge, grow to such an extent that dense overlapping
results, this "natural wall" may drastically hinder the passage of the wind through
the forest and the exposure of the air pollutants to the vegetation is reduced.
Therefore, the degree of effectiveness of a forest in removing air pollutants
is partially dependent on the permeability of that forest.  As the diagram on the next
page illustrates, moderate permeability is the most favorable condition of a forest
                                     11-45

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since more vegetative surface  area comes  in  contact with  the  flow  of air  than
in a forest of maximum permeability and also, less wind deflection occurs than
in a forest of minimum permeability.
                                 FIGURE   II-10
            DENSITY  OF  BUFFER RELATED TO REDUCTION OF WIND VELOCITY
              impermeable
 moderate
permeability
 maximum
permeability
         6   There are other advantages of maintaining a multi-layered forest
in addition to improving air quality.

             Trees are considered  to be efficient  filters  of  airborne  pollutants
because of their large dimensions.  Some  trees  are capable of growing  to  sub-
stantial heights which increases the protective effect of  greenbelts.  Another
important aspect of most trees  in  terms of the  uptake of pollutants  is their
high surface area to volume ratio.

             Although the large dimensions of  trees provide greater  vegetative
surface for absorption and adsorption  than other life forms,  a forest  with  a
poorly developed understory is  less efficient  in the removal  of pollutants
than a stratified forest.  Therefore,  developing the understory (primarily  by
opening the tree canopy which will stimulate the growth of the lower plants or
by planting shade tolerant species) will  increase  the effectiveness  of the  forest.

             Also, a stratified forest is valuable in the  abatement  of noise.
Sound may either be absorbed by the twigs and  foliage of shrubs or reflected
upward by trees.  A forest composed of primarily mature trees located  near  a
source of noise pollution,  such as adjacent to  a highway,  is  incapable of trans-
ferring the sound upward, away  from the hearer.

             In addition to their  role in noise abatement,  shrubs can  improve
the habitat.  The leaf matter produced by shrubs as well as trees enhances  soil
moisture and maintains the populations of the  soil decomposer organisms which
are essential components of nutrient recycling.  Also, wildlife require  shrubs
                                     11-46

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 and other understory plants for shelter and food.   Many songbirds utilize the
 understory vegetation for nesting and protection from predators.

          7.  The use of mixed plantings for reducing levels of pollution should
ecrtf'nly include trees and shrubs which contain deciduous and coniferous plants.

              To ensure continuous filtering action, conifers should be planted
 with the deciduous trees.  Compared to deciduous woody plants,  conifers possess
 a longer time of foliage retention which provides  a correspondingly greater
 opportunity for pollutant removal.  Another morphological characteristic of
 conifers that promotes the removal of air pollutants is the high  surface area
 to volume ratio.  Both the persistent foliage and  the consistently -high surface
 to volume ratio of conifers become increasingly important in urban areas, and
 possibly along highways,  as the winter progresses.   Urban areas generally have
 higher concentrations of atmospheric particulates  and gases in the winter as
 compared to the ambient pollutant concentrations of the summer.

              Although conifers may be preferred over deciduous species in terms
 of absorption and adsorption of pollutants, coniferous species are generally
 more vulnerable to the adverse effects of atmospheric pollutants  than most
 deciduous trees due to the greater concentrations  of pollutants in the foliage
 of the conifers.  Since deciduous trees lose their leaves after the termination
 of each growing season,  the pollutants have less time to accumulate in the living
 deciduous leaves as opposed to coniferous foliage.   In other words, deciduous
 species have a more rapid mechanism for the disposal of lethal levels of pollutants
 in their foliage than conifers.  That is seasonal leaf senescence.

              As a result,  mixed plantings of deciduous and coniferous species
 are recommended since the deciduous trees will protect the conifers by extracting
 a substantial amount of  airborne contaminants present in an area  which will
 Jower the pollutant load  in the vicinity of the conifers.
                                      11-47

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         8.  A high number of plant species with varying ages is important for
developing healthy, efficient greenbelts.

             Many  urban plantings are even-aged monocultures in which regeneration
is negligible.  Since understory young trees are virtually absent, the older,
mature trees as they die or become diseased cannot be replaced.  Also, in these
situations of extremely low plant diversity,  the dominant tree species is
more susceptible to disease.  Two recommendations for improving such urban greenbelts
are to increase the diversity index, especially for tree species, and to maintain
representatives of all age groups.

         9.  Moderate density is the optimum density for the removal of air
pollutants.

             Moderate density is achieved when more surface area of the vegetation
is exposed to the flow of air through a greenbelt than in a low density condition
and when less deflection of the wind occurs than in a high density condition.

        10.  There are numerous factors influencing the determination of the minimum
width of greenbelts necessary for maximum dispersion of atmospheric pollutants.

             The minimum width of a particular greenbelt which causes maximum
dispersion of air pollutants is dependent on numerous factors in addition to that
of the distance from the source to the receptor.  The large scale circulation
of the atmosphere determines the general direction of pollutant transport and
deviations may be caused by local breezes, topographical features of a specific area,
varying densities of air masses, etc.'

             Warren (1973) estimates that the minimum width of greenbelts is
100 to 120 meters in which maximum dispersion of airborne pollutants results.

        11.  The speed of the wind passing through or over a greenbelt may be
influenced by the dimensions and density of that particular greenbelt.

             Decreasing the wind speed by natural barriers allows the ambient
substances to settle out onto the vegetation and soil by gravitation.  The
extent of wind disruption resulting in the deposition of particulates is partly
dependent on the height, shape, and permeability of forests and buffers.
                                11-48

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             The reduction of wind velocity by a greenbelt  is  correlated to tree
height.   According  to Geiger (1950), the wind speed is  reduced 10% within a
distance equal to three times the tree height on the windward  side and twenty
times the tree height on the leeward side.   The diagram that follows may
illustrate this phenomenon more clearly.

                                 FIGURE II-ll

          EXTENT OF  INFLUENCE OF WINDBREAK AND SHELTERBELT  PLANTINGS
           windward
                3h
leeward
   20h
      WIND
                           Area of Wind  Shadow
                                                            V=Velocity
                                                            h=Unit of Length
             Wind  reduction occurs in the lee of  greenbelts  regardless of the
degree of permeability; however, the location of  the  area  of greatest wind
reduction is  a function of permeability.   Immediately behind a dense greenbelt
is the area of greatest wind reduction whereas the position  of greatest wind
reduction is  further away from the boundary of a  greenbelt of medium density.

             The extent of wind reduction caused  by greenbelts of medium density
is greater than that caused by dense greenbelts.   Also,  a  natural barrier of
medium permeability with openings distributed evenly  throughout  the greenbelt
prevents turbulence in the lee to a larger extent than an  impermeable forest or
buffer does.
             Blenk and Trienes (1955)created models of impermeable plant belts which
varied in shape.  The rounded model that was devoid of any  sharp  edges was the
least efficient  in wind reduction whereas the model that  exerted  the greatest
effect in wind reduction was right-angular in cross section.   The diagram on the
following page  displays three  of the models and their differing degrees of wind reduction.

                                    11-49

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 Buffers which are permeable to wind  are more efficient in reducing wind velocity
 than those buffers which are not  as  permeable.
                                   FIGURE H-12
            FORM OF BUFFER IS RELATED TO REDUCTION OF WIND VELOCITY.
                 maximum
                 reduction
moderate
reduction
  least
reduction
              In  conclusion,  during the process of developing plant belts, there
should be some consideration of  the conditions influencing wind reduction.  The
dimensions  and permeability  of a greenbelt are factors that cause disruption of
the air flow which may  lower the velocity to such an extent that pollutants filter
out of the  air onto  the vegetation and soil surface.

        12.  Increasing the  sink potentials of roadside forests and buffers
can be accomplished by  expanding the length and increasing the diversity of the
edge.

             According  to Warren (1973),  the initial 65 to 85 feet from the edge
of a forest can reduce  the concentration of particulates by as much as 50%.   By
increasing  the diversity and thereby,  increasing the density of the plant species
within the first 65 to  85 feet of the greenbelt,  the rate of removal of airborne
particulates by vegetation composing the edge can be enhanced.  The following
diagram shows the relative efficiency of the first 65 to 85 feet of a forest
for depositing particulates.


             Another method  for increasing the sink potential of buffers or
roadside forests is by  clearing to create additional edge.   (Figure 11-16 on page 11-55
of the Design Alternatives demonstrates a pattern for clearing the vegetation
to increase the length  of edge).
                                    11-50

-------
                                 FIGURE 11-13
     INCREASED DIVERSITY WITHIN  EDGE CONDITION MAXIMIZES SINK POTENTIAL
           Line
           or Source
           Pollution
                                65-85    L particulates reduced
                              maximum
                              efficiency
40-50%
        13.   Thermal  chimneys within the forest aid  -in increasing air circulation
which causes more exposure of polluted air to the upper leaf surfaces in the
interior canopies.

             The installation of  thermal chimneys in the forest will allow the
airborne particles trapped below  the forest canopy to become dispersed in the
crowns of the trees since the openings in the canopy will promote the movement
of air that  will escape  above the forest.  The diagram below illustrates how a
thermal chimney can increase the  ventilation of a forest.
                            FIGURE  II-14
                       CREATION OF THERMAL CHIMNEYS FOR
                      VENTILATION OF FORESTS AND BUFFERS
                                  clear cut
                                     11-51

-------
        14.  Poor ventilation along  highways may be caused by steep banks or
dense buffers and this adverse condition aan be partially removed by alleviating
the effect of the natural and artificial barriers.

             Steep roadside banks promote  localized areas of high carbon monoxide
concentrations,  especially in areas  of high traffic volumes.  If the flow of air
containing carbon monoxide is not obstructed, the amount of carbon monoxide
fallout corresponds to increasing distance from the highway.  The dispersion
characteristics  of carbon monoxide in situations in which the highway is
bordered on each side by steep banks are that the maximum concentrations occur
in the vicinity  of the impermeable walls and the minimum concentrations of
carbon monoxide  are found at the center of the highway.  The peak values of
carbon monoxide  also occur along the wall  in a situation where there is a
barrier along one side of the roadway and  an open space area on the opposite
side.  If the sides of the road are  open to ventilation, the center of
the highway will have the highest content  of carbon monoxide while the
concentration of carbon monoxide will decrease in both directions.  The
diagram below displays the three dispersion patterns of carbon monoxide due to
the presence or  absence of barriers  adjacent to the highway.
                                 FIGURE  H-15
                      CO CONCENTRATIONS ADJACENT TO  ROADS
                              ««
                       increasing concentration of CO
                increasing   44         ^ ^ decreasing
                concentration                 concentration
                         decreasing concentration

                                      11-52

-------
             Also, Figure 11-22 on page 11-58 of the Design Alternatives shows a
method for increasing ventilation of a roadway originally bordered by steep banks.

             In some instances, dense buffers may hinder adequate ventilation
and high concentrations of carbon monoxide may occur.  By cutting through the
vegetation, the carbon monoxide concentration values will be reduced due to
the increased dispersion of this pollutant caused by more ventilation.  The
technique of increasing buffer ventilation is illustrated in Figure 11-17 on page 11-55
of the Design Alternatives.

        15.  Safety measures that should be included in tine design of greeribelts
near highuays or in urban areas.

             The minimum distance from the edge of the pavement for safely
planting trees growing to a diameter breast height (d.b.h.) of 4 inches or larger
is 30 feet and for smaller trees is 20 feet.

             Persons vigorously exercising near areas of high traffic volumes
may be jeopardizing their health.  To avoid some of the potentially dangerous
effects, it is recommended to establish a buffer which separates areas of high
traffic volumes from active recreation sites.  This buffer should be at least
65 to 80 feet wide since the percentage of particulate removal as indicated
by Warren (1973) is 40 to 50%.  Figure 11-23 of the Design Alternatives on page II-5g
shows the protection of a recreational facility by the use of a buffer that
is at least 65 feet wide.

             Width is not by any means the only consideration for developing
a vegetative barrier that effectively shields actively exercising individuals
from the potential dangers of air contaminants emitted by motor vehicles.  The
buffer should be high enough to hinder the prevailing winds coming from the
polluting source.   Also,  a barrier of high density may cause an adverse effect
since the wind will be unable to sufficiently penetrate the thick clumps of
vegetation and the deflected current may bring the harmful pollutants in contact
with the people that are to be protected.
                                      11-53

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     2.   Design Configurations.

         The preceding text was a summary primarily concerning the methods for
increasing the sink potential of greenbelts.   The information can also be found
in the Literature Search Findings of Volume II,  the Plant Species Sensitivity
List in the appendix of Volume II, and the Sink and Emission Factors for Natural
Elements of Volume I.  This material provided the guidelines for developing the
design alternatives which follow.

         Each of the designs illustrate ways for increasing the removal rate
of atmospheric pollutants by vegetation resulting in the improvement of air
quality.  Some of the designs for enhancing the sink potential of natural
elements involve compiling plants into hedgerows and the most effective
arrangement of these hedgerows depends on the direction of the prevailing
wind, location of the polluting source, variations in topography, etc.  By
correctly placing the hedgerows, the wind may be disrupted to such an extent
that the airborne particulates settle out onto the vegetation and soil.

         In situations where the dense buffers along highways cause inadequate
ventilation to such a point that high localized accumulations of carbon
monoxide occur, one of the solutions is to divide the vegetation into hedgerows.
The design on page 11-55 (Figur,e  II-17)shows that gaps in the dense vegetation will
channel the polluted air away from the highway.  Also, by cutting through the
thick vegetation, the edge length will be increased.

         Another method for enhancing the edge effect is demonstrated in Figure II-16
on page  IT-55 which  involves  cutting gaps at  least  65 feet back  from  the  original
edge of the buffer.  The additional edge will increase the deposition of
pollutants by the greenbelt.

         The rest of the designs range from improving the sink capacity of a
grassy median to ensuring  the adequate protection of individuals vigorously
exercising in the vicinity of a heavily traveled highway.  All of the designs
have at least one common characteristic which is increasing the efficiency of
highway buffers in extracting harmful air pollutants emitted by motor vehicles.
                                     11-54

-------
Increasing

Buffer

Edges

In cases where buffers or road-
side forest cover exist, the
sink potential of the vegeta-
tion can be increased by
clearing to create additional
edges.  As the first 65 to 85
feet of forest is the most
valuable as a receptor for
pollutants, this technique will
greatly increase the efficiency
of the existing buffer,
especially for the removal of
particulates.
Section
65'  min.
                  FIGURE   11-16
 Plan
Increasing

Buffer

Ventilation

Dense buffers along high volume
arterials can create high con-
centrations  of CO (as shown in
Figure 11-15.  To reduce CO con-
centration,  cuts through the
vegetation will allow ventila-
tion of the  roadway and dis-
persion of CO.  This technique
also provides increased forest
edge thus aiding in the removal
of particulates as well as
soluble gases.
 Section
                    FIGURE   II-

                          11-55
 Ran

-------
Chevron

Hedgerow
The alignment of  discontinuous
hedgerows in a chevron pattern
will provide a large area of
leaf surface contact for adsorp-
tion of particulates and absorp-
tion of soluble gases.  The gaps
between the plantings provide
adequate ventiliation for CO
dispersion.  The  belts should be
oriented at a 45  degree angle
to the road; in the direction
of the prevailing winds.  A 30'
safety setback should be main-
tained .
                                                              Wind
                     FIGURE   11-18
Plan
Parallel

Hedgerow
In situations where existing
woodlots or buffers are para-
llel to the road and relatively
perpendicular to the prevailing
winds, the placement of a dis-
continuous hedgerow windward
of the edge of vegetation, as
shown, will increase wind tur-
bulence and decrease wind speed
thereby causing particulates to
drop out.  The polluted air is
forced closer to the soil sur-
face where CO can be metabo-
lised by soil organisms.  The
increased exposure of leaf
surfaces further reduces par-
ticulates and allows for the
absorption of soluble gases.
Openings in the hedgerows are
located at intervals to limit
the buildup of CO. A 30' safety
setback should be maintained.
Section
                      FIGURE 11-19
Plan
                            11-56

-------
Multiple

Hedgerow

In areas of sloping terrain or
where  roads are  located on fill,
an arrangement of multiple
hedgerows, parallel to the road
and perpendicular to the pre-
vailing winds are recommended.
This arrangement provides a
maximum disruption of the wind
which  results in the deposition
of particulates  as well as
maximum exposure of polluted
air to leaf and  soil surface
which  reduces CO and soluble
gases.  The increased spacing
between rows will increase
turbulence thereby decreasing
particulates.
Section
                      FIGURE 11-20
Plan
 Managed
 Natural
 Buffer
Management of rights of way
along roads to stimulate
natural plant succession to
occur is a useful technique
for providing buffers.   The
development of old fields and
forests, or woodlot conditions,
will provide increased  pollu-
tant sink potential by  first
reducing wind speed through
increased turbulence and by
exposure of leaf and twig sur-
face for adsorption of  par-
ticulates and absorption of
soluble gases.
                                  Section
                                                8' Manage as  as
                                                    old field  forest
                      FIGURE 11-21  Plan
                           11-57

-------
Ventilating

Roadway

Cuts

Steep roadside cuts become areas
of high concentrations of CO,
particularly in areas of high
traffic volume (as illustrated
in Figure 11-15).  Cutting
back steep banks to more
shallow slopes provides better
air ventilation to reduce CO
levels.  Covering the exposed
banks with legumes (such as
crown vetch) provides soil
stability as well as increased
sink potential.  It also may
improve the visual quality of
the road experience.
             •original
             grade
Section
                    FIGURE  11-22
Plan
Recreation
Facility
Setback
                                                         Foot or
Because of  the potential dangers
of vigorous exercise adjacent
to high traffic volumes, it is
recommended that active recre-
ation facilities be located at
least 65 feet behind the buffer
edge.
Section
*    bike
     path
                     FIGURE  11-23

                          11-58

-------
Planting
Existing
Medians
Roads with medians now planted
in maintained grass could
greatly reduce the level of
pollution by installing a
moderately dense mixed planting
of trees and shrubs, both ever-
green and deciduous.  This
would also reduce headlight
glare and ambient noise levels.
                                Section
                   FIGURE  11-24
Plan
                         11-59

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JTI. REGIONAL OPEN SPACE

     This section of the study is concerned with  the  regional control of
pollutants.  Initially, a review of pollutants  from both natural and anthropo-
genic sources is presented including sulfur compounds, nitrogen compounds,
carbon monoxide, organic gases (eg. hydrocarbons),  asbestos, lead and fluorocarbons.
Next, removal processes are discussed to illustrate how regional pollutants
interact with the environment.  Finally, the  literature is  reviewed on using
open spaces to reduce regional pollutants and several planning concepts are
presented.

     A.   POLLUTANT  IDENTIFICATION

          Regional scale air pollution problems are generally associated  with point
sources  of pollutants.  However,  there  are numerous  natural sources of air
pollutants that can be  the major  cause  or that can contribute to regional pollution
problems. Ultimately, all air pollutants  are from  natural  sources.  However  most
problems  occur when the natural  compound  is  transformed by man  into an  air
polluting compound.  As an example,  the major  source of air polluting sulfur is
hydrogen  sulfide  (H_S) which, in  itself,  is  not  injurous.   However, tUS  is rapidly
oxidized  to sulfur  dioxide (S02>,  sulfur  trioxide  (SOO, and sulfuric acid  (H_SO,)
which are all considered air  pollutants.  In the combustion process, S0_ is
produced  from elemental sulfur.   It  is  also  important to recognize that  while sulfur
in the form of SCL may be considered an air  pollutant in industrial areas, crops  of
various kinds are dependent upon atmospheric sources for a large proportion  of
their sulfur needs.

         Table 1II-1 is a summary  of the  annual  emissions  of various atmospheric
pollutants.  Careful attention should be  directed  to the proportion of natural
emissions by the anthropogenic sources.
                                      III-l

-------
            TABLE III-l
SUMMARY OF SOURCES & ANNUAL EMISSIONS
      OF ATMOSPHERIC POLLUTANTS
POLLUTANT
so2

H S
£,
N20
NO



N0_
2

NH


CO



°i
J

non-
reactive
hydrocar-
bons
reactive
hydrocar-
bons
asbestos
MAJOR SOURCE
ANTHROPOGENIC NATURAL
combustion of coal
and oil
chemical processes;
sewage treatment
none
combustion



combustion


coal burning;
fertilizer; waste
treatment
auto exhaust;
and other
combustion
processes
none


auto exhaust;
combustion of
oil

auto exhaust;
combustion of
oil
insulation,
i shipbuilding,

lead




f Luorocar-
bons




brake linings
auto exhaust,
combustion of
coal, refuse &
sludge incener-
ation
aluminum, fertili-
zer, fuel combus-
tion, steel indus-
tries


volcanoes

volcanoes ;
biological decay
biological decay
bacterial action
in soil; photo-
dissociation of
NO and N02
bacterial action
in soil; oxidation
of NO
biological decay


oxidation of methane;
photodissociation
of CO ; forest fires;
oceans
tropospheric reactions
and transport from
stratosphere
biological processes
in swamps


biological processes
in forests

mining


mining






ESTIMATED EMISSION KILOGRAM
ANTHROPOGENIC NATURAL
65 x 109

3 x 109

none
53 x 109
combined with
N07




4 x 109


360 x 109



	


70 x 109



27 x 109


(?)


143 x 106




(?)

2 x 109

100 x 109

590 x 109
768 x 109






170 x 10^


3000 x 109
(?)


(?)


300 x 109



175 x 109


(?)


(?)




(?)



SOURCE: Rasmussen, et al, 1974
m_2 (Adapted by COMSIS CORP. 1976)

-------
          1.  Source Emissions.

              a.  Sulfur Compounds

                  The element sulfur (S) occurs in a variety  of  stable compounds
 that are derived from both the natural environment and from  air pollution sources.
 Among the more common compounds are: hydrogen sulfide  (H.S),  sulfur dioxide (SO.),
 sulfur trioxide (SO.) and sufuric acid (H.SO,).  H.S has not, in itself,  been
 considered a pollutant.  However, it oxidizes rapidly to S0_  and further  to SO. and
 H2SO,.  This chemical reaction is represented in Figure  III-l    (Kellogg,  et al.,
 1972).
                                 FIGURE III-l
         SCHEMATIC  REPRESENTATION OF THE CHEMICAL PROCESSES INVOLVING
         ENVIRONMENTAL SULFUR,  WITH INDICATIONS OF THE MEAN LIFETIME
                   OF EACH COMPOUND IN THE LOWER ATMOSPHERE
                                            (hours or days;
                            Anaerobic bacteria   *(aster'" solutlonl
                            in soil, marshes,   «
                            and tidal flats       3
                                                  XSO/
             Robinson  &  Robbins,  (1968),  have suggested that on an annual basis,
220 x 10  tons of sulfur are discharged into the atmosphere with about one  third
coming from air pollution sources,  mostly in the form of SO., and the rest  from
natural processes.  Kellogg,  et al.,  (1972), estimated that man is contributing
about one half as much as nature, but  that by AD 2000 he will be contributing about
                                      III-3

-------
 as  much,  and  in  the Northern Atmosphere  alone he will more  than match  the
 natural  generation rate.

              Most of  the S being emitted by natural sources is in  the  form of
 H-S.   It  is estimated that H_S represents one half of the total sulfur now being
                                    6
 released  to the  atmosphere, 100 x  10   tons  (Robinson & Robbins,  1968),  The primary
 sources  for this natural emission  are decaying vegetation in swamps, bogs and
 other  land areas.  Estimates of the annual emissions from natural  sources vary.
                                                                       9
 Erikson,  (1960), suggests decaying vegetation is the source of 112 x 10  kg H_S
                                                       9                     L
 per year.  Robinson &  Robbins, (1968), estimate 70 x 10  kg per year.

              The oceans have also been suggested as a source of H_S.  Erikson,
                                                                 *•         c
 (1960), speculated that the annual H?S emission from the oceans is 202 x 10  tons.
                                    *•                   e.
 Robinson & Robbins, (1968), suggest that it generates 10  tons.  Kellogg, et al.,
 (1972), dispute both  these figures saying that undoubtedly some H-S is liberated
 from tidal flats, but  probably very little is emitted from the open ocean.  Active
 volcanoes are another  source of H«S, however,  no estimates are known of the amount
 of H S emitted.  Only  small quantities of H^S are emitted from anthropogenic sources.

             Most of  the SO. and SO, compounds in the air are from anthropogenic
 sources and their contribution to pollution problems can be linked with industrial
 growth.  A good example of this is illustrated by the fact that in 1940 there was
                    9
 an estimated  78 x 10   kg/yr of SO. emitted on a global basis (Katz,  1956).
 Robinson & Robbins, (1968), in Rasmussen et al., (1974), estimated anthropogenic
                                          9
 activity in 1968 as the source of 146 x 10  kg SO- each year,  70% of which they
 estimated was due to  the combustion of coal, 16% from the combustion of petroleum
 products, primarily residual fuel oil.  The remaining emissions resulted from
 refining operation ( 4%) and non-ferrous smelting ( 10%).  Kellogg et al.,(1972),
                                      9
 believes an estimate of about 100 x 10  kg SO- per year would be reasonable for
 the same period.

             In terms  of regional areas, Prince and Russ, (1972),  have estimated that
                                                              _2
 S0_ emissions in Britain have increased from 9.1 to 11.4 mg km   from 1950 to 1970,
                        —2
an increase of 2.3 mg km"  in 20 years.  On the  same basis,  they estimated emissions
                                             _2
 in the United States were approaching 2 mg km   in 1970 and are expected to reach
         _2
 3.3 mg km   by 1980 if the fossil fuel becomes available and no steps are taken to
 reduce emissions.
                                     III-4

-------
             Most of the natural sources of SO- is from volcanic activity.  Kellogg,
et al.,(1972), estimated that the quantity released by volcanoes is about 1.5 x 109
kg/yr. Stoiber and Jepsen (1973), estimated annual volcanic emissions of S00 to be
       9                                                                    a
15 x 10  kg. Rasmussen, et al., (1974), determined an average to be 2.0 x 10  kg/yr.

         b.  Carbon Monoxide

             Carbon monoxide (CO), is the most abundant and widely distributed air
pollutant found in the atmosphere.  CO emissions generally exceed that of all other
pollutants combined (excluding carbon dioxide CO.) particularly in urban atmospheres.
Practically all of the CO formed is due to man's technology with more than 90%
of the total CO emitted from combustion of fossil fuels being derived from motor vehicle
emissions (Jaffe,  1973).

             Rasmussen,et al., (1974), has written an excellent review of
natural and anthropogenic sources of CO.  The following is a synopsis of that
material.

             By far the largest single anthropogenic source of CO is motor vehicle
exhaust.  Jaffe (1973), estimated that of a total anthropogenic CO emission
                                                 9              9
source in the United States in 1970 of 132.6 x 10  kg, 96.9 x 10  kg resulted from
the burning of gasoline by motor vehicles alone.  Other significant contributions
                                                                  9
to this man-made CO burden are from solid waste disposal (6.5 x 10 kg), industrial
                       9                                       9
process loss (10.3 x 10 kg) and agricultural burning (12.5 x 10  kg).  On a global
                                                                                9
basis, for 1970 Jaffe(1973), estimated CO emissions to be approximately 360 x 10  kg.
(See Figure III-2).

             The most widely recognized natural source of CO is forest fires
                                              9
which have been estimated as releasing 11 x 10  kg CO into the atmosphere each year
(Robinson & Robbins, 1968).  Minor amounts of CO have been found to be released
from volcanoes and marshes (Flury and Zernik, 1931).  CO can also be formed
during electrical storms (White, 1932), and by the photo dissociation of C0?
in the upper atmosphere (Bates and Witherspoon, 1952).  Calvert, et al.,(1972) has
suggested the photo dissociation of fonneldehyde as a possible source of CO
and recently, Swinnerton, et al.,(1971) found CO to be present in rain water in
high concentrations.

                                   II1-5

-------
                                    TABLE  IH-2

                     ESTIMATED  CARBON MONOXIDE EMISSION SOURCES
                           IN THE UKITED  STATES IN  1970
                                                            Enissions,
                         Source Category                       10' "erne ton*


                                              Han-Kade Sources
                Fuel coabustion in stationary sources                   0.7
                 Steam and electrical                               0-1
                 Industrial                                       0.1
                 Commercial and institution*!                         ".2
                 fcesidential                                      0.1
                Transportation, mobile sources                        J0ff.fi
                 Motor vehicles, gasoline                            8b.9
                 Motor vehicles, diesel                              0-7
                 Railroads                                       0-1
                 Kaiercrafl                                       !-J
                 Aircraft                                        2-7
                 Oihei nonhighway use                               • •*
                Solid waste disposal                                 *•*
                 Municipal incineration                              0.3
                 On-site incineration                               "•*
                 Open burning                                     *•!
                 Conical burning                                   *••
                Industrial process losses                             J0-3
                Miscellaneous                                      **•*
                 Structural fires                                  0.2
                 Coal refuse burning                                0-3
                 Agricultural burning                               12.S
                 Preicribed burning                                 '-^
                Total all ean-oadc categories                        732.fi

                                              Matural Sourcei
                 Forest fires (wild)                                Z.J


                                                Source:   Jeffe,  1973

              The  ocean was first  suggested  as a major source  of CO by  Swinnerton,
                                                                      9
et  al.,(1970), who estimated that  it can produce  up to 220 x  10  kg  each year.

Robinson o Moser,(1971)  suggested  that plants could indirectly be the  source  of
              q
about 54 x 10  kg CO  by  the oxidation of released terpenes.   Finally,  McConnell,
                                                          o
et  al.,(1971), suggested that approximately 900 x 10  kg  CO are produced each

year by the oxidation  of methane.



              Rasmussen,et al., (1974), also points.out that Stevens  et al.,O972)

believes that natural  sources of  CO could yield about 10  times more  CO than

all  anthropogenic sources in the northern hemisphere.  Using  that conclusion  they
                                                                 9
estimate  the total CO natural emissions to be  3000 kg x  10   per year.



              On a regional basis,  the emissions from anthropogenic sources far

exceed any natural sources.  The  concentration  of this pollutant is  well corelated

with can's activity and  predominantly with  the  flow of vehicles on urban streets.


                                     III-6

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           c.  Nitrogen Oxides

               The photochemical smog reaction involving nitrogen oxides,  hydrocarbons
  and sunlight was identified in the early 1950s as the basic mechanism for the
  characteristic air pollution problem found in Los Angeles.  Since that time photo-
  chemical smog has been identified as a significant air pollution factor in a
  number of large urban areas and has focused attention on the role of nitrogen
  oxides in urban air pollution (Robinson & Moser,  1971).
               The main source of  N.O is believed to be the  result of  bacterial
  decomposition of other nitrogen  compounds  in the soil.   On a  global  basis,
  the  quantity  of  N_0 and NO  produced naturally has been estimated as  786 x  10
  tons by  Robinson &  Moser,  (1971).  Goody &  Walshaw,  (1953)  estimated
                                                12
  a  global NO  production rate of  about  100  x 10   kg/year and  Robinson  & Robbins
  (1968) suggested that soils produce about  59.2 x 10    kg N20  each year by  biological
  action;  and of  this about 55.4 x 1010  kg  (35.3 x 1010kg NjO-N)  are reabsorbed by
  the  soil and  about  3.8 x 1010 kg N20 (2.4  x 1010 kg  N^-N) travels  up to  the
  stratosphere  where  it is destroyed.  Schutz   et al.,  (1970),  cited in Rasmussen, et  al.,
  (1974) showed a  flux of NjO in the order of 10~8 g NjO/m2  sec,  a level which, if
  maintained  globally,  would  necessitate on N?0 cycle  of  about  70 years.

               Nitrogen (N) is  one of  the most  abundant elements  constituting
  78%  of our  atmosphere.  There are  a  number  of compounds  of  nitrogen, but only 2
  are  considered pollutants - nitric  oxide (NO)  and  nitrogen  dioxide (N0_).  Most
  other compounds are  from anthropogenic  sources.  Another compound, nitrous oxide
  (N?0), is predominantly from  natural sources; however it oxidizes to NO  compounds
   »                                                                    X
  and  therefore should be considered in air pollution calculations.  In pollution
  estimates,  the NO and NO. are usually  considered  together and expressed as NO-.
  It is estimated that natural  emission of nitrogen as N_0 are approximately 15
                                                 9                   9
  times greater than pollutant  emissions  (768 x  10  kg NO. vs. 53 x 10 kg NO.,
 Robinson & Robbins,  1970).

             Production rates of  N0 and N02 by soils  are much  more difficult to
 predict.   McConnell  (1973)  in Rasmussen, et al.,(1974) recently  summarized a
 few of the problems  involved in appraising  the amount of nitrogen oxides  generated
 by soil.   He contends that the soil source  is  small compared to  that  produced as
 a result  of  the gas  phase oxidation of  atmospheric ammonia  (NH ) by oxides  of
nitrogen.   He  believes  this  source  produces  7  x 1010  kg  NO^N/year.   He offers
 alternative  reaction  sequences for  NH3  in the  atmosphere.   One reaction sequence
 provides a constant source of  NO, the other  a  sink.   If  the  later occurs in the
atmosphere an additional source of NO must be  found in order to  account for the
amount of NO known to be in  the atmosphere.  In  this case, McConnell  concedes
                                      III-7

-------
 that the soil might actually  constitute  a significant  source  of NO  , generations
         11                                                        x
 above 10   kg/year.

             Estimation of  the anthropogenic  emissions of NO  and NO  are lumped
 together as emission data which rarely distinguishes between the two  forms.  Robinson
 and  Moser,  (1971), estimated that annual production is  about 53 x  10  kg with 31%
 of the  total due to coal combustions and  41%  due  to petroleum production and the
 combustion of petroleum products.  Within the petroleum class, combustion of gasoline
 and  residual fuel oil are the major contributors  of NOj.  For the coal combustion
 category, power generation and industrial users account for most of  the NO.
 emissions.  Robinson and Robbins  (1970),  suggest  using the same anthropogenic
                         9                                    Q
 emission rate of 53. x 10  kg of NO  but  convert  it to 16 x 10 kg NO -N.

             Although the natural sources of  nitrogen compounds are greater
 than  the  anthropogenic sources, the anthropogenic  sources are concentrated in
 industrial sections and thus their contribution is more significant in a±T pollu-
 tion  problems. There is more than one reason  for  the build-up of NO  in urban
 areas.  First, the soil serves as the main sink for NO  and in urban areas the
                                                      X
 anthropogenic sources of NO  usually exceed the capacity of the soil to absorb
 NO .   Secondly,  although the soil releases great  quantities of N00, the release
  x                                                             Z
 occurs at the ground surface thus the same soil can serve as  a sink in a dynamic
 equilibrium.

             Most of the anthropogenic sources of NO. are released 20-50 meters
 in the air.   Because a soil - gas interface is necessary,  the soil has less of
a chance  to serve as a sink for NO. released  at height.  Therefore, NO. remains
 in the air for a longer period and can contribute  to the photochemical smog
problem.  It is  recognized that if the NO- were released at the ground level
 there would be higher concentrations; however the  soil could  then better serve
as a  sink and absorb more of the NO..

         d.   Organic gases (hydrocarbons)

             This group of gases represents a major factor contributing to air
pollution.  It includes all classes of hydrocarbons including  those
formed when some of the hydrogen of original  compound is replaced by other
                                   III-8

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substituent groups including  nitrogen, sulfur or oxygen (Rasmussen, et al.,  1974).
There are two classifications of  organic gases, reactive and non-reactive.
In areas where photochemical  air  pollution is a serious problem, a major concern
is with the olefins and  other reactive hydrocarbons rather than with the total
organic emissions.  Using factors derived by the Bay Area Air Pollution
Control District in San  Francisco, Robinson & Moser, (1971) estimated that
approximately one-third  of the total hydrocarbon emissions are classed as reactive,
or about 27 x 106 tons out of the 88 x 10  total tons of organic materials.   The
major natural source of  reactive  hydrocarbons is decaying vegetation and plant
metabolic processes.
             Since the analytical work of F.W.  Went  in  1960, an  increasing base of informa-
tion has been developing related to the emissions of air polluting hydrocarbons
by vegetation.  Particular  focus has been made on the presence of aromatic
ethers,  and some unsaturated material which generally is found in air and  is
among the prime determinants of  our perception of the 'freshness*  of the air
(Turk and D'Angio, 1962).

             The primary volatile organic compounds  emitted  are  the monoterpenes which
contain  ten  carbon atoms  and include a-pinene,  B-pinene, and limonene and the
hemiterpene  isoprene which contains five carbon atoms  (Rasmussen, 1970, 1972).
Other naturally  occurring hydrocarbons include  Camphene,6-phellandrene,
1, 8-Cineal,  Camphor, P-Cymena,  Terpinene and A3-Carene.   In effect, these
substances serve as  tracers for  a larger group  of  lower molecular weight
organics which provide material  available for reaction  with  ozone to generate
smog through  the photochemical reaction of these chemicals.

          It  has  been estimated that  1.7 x 108 tons of volatile hydrocarbons
  are generated each  year by all  of  the vegetation of the earth as compared with
  0.27 x 108  tons of  reactive hydrocarbons generated from anthropogenic sources
  (Eschenroeder,  1974).  However,  natural emissions from vegetation, because  of
  the low emission densities involved, are not believed to be present in
  sufficiently high ambient  concentrations to result in significant quantities
  of photochemical oxidants—especially  in comparison with ozone levels resulting
  from anthropogenic precursors.

          A cursory examination of the literature reveals that the synthesis  of
  aromatic carbon compounds by  plants is  an  integral part of their cellular

                                      III-9

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 activities.   It  is  logical to anticipate  the release of  these biosynthetic
 products  in proportion to the potential metabolic activity of the plant
 species under consideration  (Beytia, et.al., 1969).  Certain species are far
 more  efficient hydrocarbon generators than others and variations may even be found
 between clonal variations of the same species  (Gerhold and Plank, 1970; Rodwan
 and Ellis, 1975).

              On  the other hand, a single  species of plant may show marked fluctuation
 in the generation of hydrocarbons in apparent  physiological response to a very
 wide  array of environmental alterations.  These alterations include, at a
 minimum,  injury such as from elevated ozone levels (Craker, 1971) or insect
 attack (Shain and Hillis, 1972).  Other alterations include temperature,
 humidity, nutrient level and any other factor  contributing to the cellular
 environment of the plant under study (DeSanto, personal  communication).

             There are numerous pollutant sources of reactive hydrocarbons.
 On a  global basis, Robinson and Myers,(1971),  have estimated an emission rate of
 88 x  10   tons per year.  Of this total, 66% is from petroleum usuage, 34 x 10
 tons  from gasoline usage, 6.3 x 10  tons  from  refinery uperections; 7.8 x 10
 tons  by transfer losses;  petroleum evaporation, and 10 x 10 tons from solvent
 usage.  Other sources of  hydrocarbons include  incineration and coal combustion.

         e.  Other pollutants

             There are numerous other pollutants emitted by both natural
 and anthropogenic sources including asbestos,  lead and flourocarbons.  Most of
 the sources of these pollutants can be considered minor when compared to the
 pollutants previously discussed.  A brief description of each pollutant is contained
 below.

              1)  Asbestos

                 Asbestos is a generic term covering several fibrous silicate
minerals  that are found in almost every country in the world.  These minerals
are classified into two groups:  (1) Serpentine - chrysotile and (2) Amphiboles
encompassing actinolite,  amosite, anthophyllite, crocidolite and tremolite.
Chrysotile - the fibrous  form of serpentine, the so called white asbestos -
 is the most widely used type of the mineral, constituting more than 90% of the
                                    III-10

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 world's production.   Within the second group,  anthophyllite,  amusite,  and crocidolite
 are of commercial importance  (Hammons and Huff,   1974).

                  Hammons  and Huff,  (1974),  have reported  that in  the  last 60 years
 global use  of  asbestos  has  increased more than. 100 fold-from  30,000  tons  to four
 million tons.   The same authors stated that asbestos  is used  in more  than 3,000
 products -  cement, textiles,  yarns  and cords,  boards  and  papers,  sealing  and packing
 materials,  plastics,  thermal insulants and fire proofing  and  friction material for
 brake  linings  and many  other devices.

                 Anthropogenic  sources of  asbestos  are mostly industrial  that use it
 as  part of  their  final  product.   These include ship building,  insulation,  construction,
 iron foundries, pharmaceutical  and  brake  lining industries.   Natural  sources of
 asbestos include mineral  production, weathering of  mineral outcrops,  and
 release during farming  of asbestos  - containing soil.  No information could be
 found  on quantities of  asbestos  being  emitted  on either a global  or regional level.

             2)  Lead

                  Lead is  a  heavy metal that is naturally  present   in  small amounts
 in  soil,  rocks, surface waters  and  the atmosphere.  Due to its unique properties,
 it  has  been an element  widely used  by  man.   This  utility  has  resulted in  greatly
 elevated lead  concentrations  in  certain ecosystems.

                 The  primary  source  of lead in urban  areas is the combustion of
 gasoline containing lead  additives.  Specific  estimates of the amount  of  lead annually
 introduced  to  the atmosphere  via gasoline  consumption includes 98% (National
Academy, of Science. 1972),  and 952,  {Ewing  and Pearson, 1974).  Approximately 136 x
 10  kg  of lead were released  in  automotive  exhausts in 1970 ( U.S. Bureau  of Mines,
 1971).    Since  1970 no-lead  and  low-lead gasolines have become increasingly available
and in  1974 all new cars  in the  United States  were  required to use no-lead gasoline.
Other sources  of lead include coal combustion,  refuse and sludge  incineration, burning
or attrition of lead-painted  surfaces  and  industrial processes.

                 Lead is  a  naturally occurring element and therefore  small amounts
are present in  the environment from non-anthropogenic  sources.  In studies to
determine the  impact of lead  from highways  on  vegetation  it has been  reported that
                                     III-ll

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 the background lead content of twigs and foliage of shrubs  and  decidous  trees
 is generally within the range of 1-4 pg/g dry weight of  tissue  (Smith,  1975).

                  Other studies have reported that the lead  content  of  the  upper
 soil horizons of  unmineralized and uncontaminated areas  is  approximately 10-20 vg/g,
 dry weight  (Smith,  1975).   These statistics indicate the amount  of  lead occurring
 naturally in the  environment.

              3)   Fluorocarbons

                  Atmospheric fluorides  may be placed into four major categories;
 gaseous, particulate,  soluble  and insoluble.   The major form of  fluorine is
hydrogen flouride (HF)  and is  given off by aluminum, steel and fertilizer  processing
 industries.   Coal and  shale contain up  to 120 - 550 ppm fluorine respectively
 (Crossley,  1944), and  during the  combustion process a proportion of this is
released as  hydro fluoric  acid, silicon tetra fluoride and as a  form associated
with particulate  matter (Davison,  et al.,  1973).

         2.   Pollutant Removal.

             There are numerous mechanisms  for removing air pollutants from  the
 atmosphere by natural phenomena.   A review of  these mechanisms was performed by
 Rasmussen, et al., 1974, which was based on work by Robinson and Robbins, 1968, and
 Hidy, 1973.   The  important mechanisms include:

              (1) Precipitation scavenging in which the pollutant is removed
 by  two modes.  The first is "rainout" which involves  the absorption of gases and
 aerosols by  clouds.  The second is "washout" which involves both gas absorption and
 particle capture  by falling rain drops;
              (2)  Chemical reactions in the atmosphere, including  the stratosphere,
 which produce either aerosols or oxidized products such as carbon  dioxide and water
 vapor.
              (3)  Dry deposition which involves absorption  by  aerosols and subse-
 quent deposition  on the earth's surface; and
              (4)  Absorption by various substances  at the earth's  surface including
 vegetation,  soil  and water bodies.
                                     111-12

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              The  remainder  of  this section will  discuss how  each  of  these
 processes  affects the  removal  of  each  of  the previously mentioned atmospheric
 pollutants.   Particular  attention will be given  to  those  processes that  contribute
 to the removal of pollutants using open space  measures.

              a.   Sulfur  Compounds

                  S07  is  very soluble in water  and very reactive either photochemically
 or catalytically  in dilute  concentrations in  the atmosphere.   Accordingly,  the  main
 processes  for the removal of SO,  from the atmosphere  are:  (1)   precipitation scavenging
 (2)   chemical conversion and  (3)  absorption by  soil, water,  rock and plants.

                  In precipitation scavenging,  the S02 will undergo a series of
 reactions,  some catalytic,  to  ultimately  form HjSO^  drops or a sulfate salt. In
 the chemical conversion  processes, dry S0«  in  the daytime  under  low humidity condition,
 will react with N02 and  hydrocarbons in the transformation of S02 to form  a H2SO^
aerosol.  At night and under high humidity a process involving  the absorption of SO.
by alkaline water droplets and a reaction to form SO, within the  drop is a well-documented
process and can occur at an appreciable rate which  removes S0_  from the atmosphere
 (Robinson and  Robbins, 1968).

                  In terms of open space measures, SO. can be absorbed from the
atmosphere directly by vegetation, soil, rocks and water.   This technique can be
thought of separately or in combination with dry deposition and precipitation
scavenging.  Vegetation needs elemental sulfur for metabolic processes and much of
that sulfur can be obtained from S02  especially in areas where  the soil is sulfur
deficient.   Soils readily absorb SO  although the removal process is  not fully
understood.  Smith, et al.,  1973,  suggests that S02  absorbed is oxidized  to
sulfate which may then be subject to  leaching and uptake by plants.  Thus the
soil can remain a   renewable sink for SOj.  Limestone rocks react with H-SO, to
form gypsum, thus  serving as a sink for SO..  Table  111-10 of Volume  I of this  study is
a synopsis  of sink factors for SO-.
                                      111-13

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             b.  Carbon Monoxide

                 For all practical purposes carbon monoxide is insoluble in water.
Therefore, the processes of washout and rainout are insignificant in removing it
from the air.  Gas-phase reactions in the troposphere serve as chemical sinks for
CO.  In these reactions, CO interacts with the hydroxyl radical to form C02
(Rasmussen, et al., 1974).  However, there is much debate about this removal process
as well as its technical accuracy.  It is believed that most of the CO that enters
the stratosphere is destroyed (Pressman,  et al.,  1970).

                 Soil, and vegetation to a lesser degree, serve as sinks for CO
and thus can be utilized in mitigation techniques.  Based on laboratory results, it
has been proven that soil can act as a significant sink for CO.  There are two
schools of thought on the subject; Inman and Ingersoll, 1971, believe that the CO
is removed by biological activity while Smith, et al., 1973, using sterilized soil
in their laboratory concluded that soil could act as a sink by a definitely non-
biological pathway.  It is evident from the literature that practical research
is needed  to determine  the ability of in situ soils to serve as a sink for CO.
Vegetation can reduce CO from the atmosphere but not as effectively as soil.  The
results of the ability  of both to serve as a sink are summarized in Table III-2
of Volume  I.

              c.   Nitrogen  Compounds

                  Of  the major nitrogen compounds, N.O  is  slightly soluble  in water
and  under  normal  troposphere conditions,  is  chemically inert.  Therefore there  are
no significant removal  processes.   NO  is  rather  insoluble in water  and  is  either
oxidized  to  NO™  or photolyzed  to N~  in  the atmosphere.   The N02  is  then removed
primarily by precipitation in  the form of nitric  acid  (HNO.j).  It can also be
removed by vegetation and soils.   The main removal  mechanisms  for NO  and NO^ are
precipitation scavenging,  chemical reactions and absorption by plants and  soil.
                                        111-14

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                 The main removal mechanism for NO  is precipitation.   There is
                                                  X
no disagreement with this conclusion. However,  there are many theories as to the
exact chemical reactions involved.  With hydrolysis,  the outcome is the same and
the nitric acid formed by the reaction of NO with rain is absorbed onto hygroscopic
particles or it reacts with atmospheric ammonia to form nitrate salt aerosols
(Rasmussen,  et al.,  1974).

                 NO  can also be removed by chemical reactions in the atmosphere.
                   A
The primary reaction is its oxidation by ozone  to form N02<  It can also be
photolyzed to form N which can then react with  other NO molecules to.form N .  N0_
can also react with ozone to form N0_ or with the hydroxyl to form nitric acid.

                 In polluted atmospheres, NO and NO. react with SO. and hydrocarbons
to form aerosols.  The most important aerosols  formed is atomic oxygen which is
free to react with molecular oxygen to form ozone.

                 In terms of open space techniques for air pollution mitigation,
vegetation and soil can serve as a sink for NO  and N0_.  There is no valid evidence
of the exact methodology by which vegetation absorbs N02, but from laboratory work
it is evident that it serves as a sink for both NO and NO-.  Soil has long been considered
a natural emission for N20, but recently it has been discovered that it also can
absorb NO and N0_.  It is believed that the N0_ absorbed will ultimately be oxidized
to nitrate (Nelson and Bremner, 1970).  The nitrates eventually decompose'and result
in the production of N0?.  NO. is also produced from the absorption of NO from the
atmosphere, but the reaction is almost instantaneous.  However, certain alkaline
earth cations can retard this NO- production Sundareson, et al., 1967, found that
alkaline earth zeolites readily absorb NO and release it as NO  and HNO_.  Much
                              '                               x        3
research is needed on the exact mechanisms involved in the use of soil as a sink
for NO  and especially on the rule of organic material in the soils to halt or
      J\
hinder the production of NO-
                           f, m

             d.  Organic Gases (Hydrocarbons)

                 Reactive hydrocarbons are completely insoluble in water and there-
fore cannot be removed by washout or precipitation.  The main removal mechanism is
chemical reaction where some of the gases are transformed in the troposphere to
other gases.  For instance, methane has been shown to react with the hydroxyl ion
to form CO (Rasmussen, et al., 1974).

                                      111-15

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                 In terms of open space techniques,  there have been recent
laboratory experiments that show that vegetation may be a sink for hydrocarbons
and that soil may use them in bacteriological processes. It is also suggested
that vegetation may serve to retard the natural release of hydrocarbons to the
atmosphere.  For instance, tree canopies may prevent sunlight from filtering to
a roadway edge where  the light would otherwise cause the reactive hydrocarbons to
form smog.  This is a theoretical possibility but the principal is sound.

             e.  Other Pollutants

                 There are numerous papers that discuss the capacity of vegetation
and soil to act as sinks for numerous particulates including asbestos,  lead and
fluorine (inits particulate form).  The photographs in the introduction to this
volume illustrate this phenomenon.

                 Lead is introduced into the atmospheric compartment of the
roadside environment from exhaust emissions and then transferred  to the soil, plant
or animal compartment, via sedimentation, impaction, precipitation or inhalation.
The roadside environment receives lead particles of all classes,  the larger ones
by sedimentation and the smaller  ones by the latter three processes (Smith, 1975).

                 Sedimentation and precipitation (washout and washoff) act to
deposit lead particles, primarily in the relatively soluble halide form, on the
soil surface in the roadside environment.  Once the lead enters the soil surface,
it is speculated that it may react with soil anions, or with some soil organic
or clay complex  (Singer and Hanson, 1969 in Smith, 1975).  These reactions would
indicate  that  the lead is insoluble in the soil and thus preclude its rapid
mobility and restricts plant or microbial uptake.

                   Lead may also react with sulfuric acid in the atmosphere to
form lead sulfate (Pb SO,).  This reaction could also occur at the soil-atmosphere
interface.  Reaction with the sulfate anion may occur in the soil in contact with
ground water (Skogorbee,  1974 in Smith, 1975).
                                     111-16

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                 Vegetation has been proved (see especially Smith, 1975) to be
an effective agent to adsorb lead particulates in the atmosphere.  It is accumulated
by the vegetative component of roadside ecosystems from both the atmospheric and
soil compartments.  Contamination of above ground plant parts from the atmospheric
compartment may be via gravity settling, impaction (kinetic capture/ or precipitation)
Contamination from the atmospheric compartment is also generally considered to
be topical (superficial) in nature and largely susceptible to removal by washing
(National Academy, 1972 in Smith, 1975).

                 We found no literature on removal of asbestos from the atmosphere.
However, it can be speculated that in the particulate form, it can be removed
from the atmosphere in the same manner as lead.  Reaction in the soil compartment
has not been studied so no conclusions can be made relating to this agent serving
as a sink.

                 There is some evidence that vegetation can serve as a sink for
fluorine.  The results indicate that fluorine from the air can be adsorbed to the
surface of leaves (in its particulate form) as well as accumulated internally
(in its gaseous form) and that fluorine in leaves can be translocated outward to
the surface as well as upward to the tips.  Fluorine remains in a soluble form in
plant leaves and maintains the chemical properties of free, inorganic fluorine.
The solubility and mobility of fluorine and the ease of removal from plant tissue
indicate that irreversible binding to cellular components does not occur
(Jacobson, et al., 1966).

     B.   LITERATURE SEARCH FINDINGS

         While there are a number of articles on town planning and buffers
to control air qulaity, relatively little work has been done to quantify these
planning proposals.   The criteria developed for highway buffers are also applicable
to larger (i.e.  regional) open space systems.   Essentially,the purpose of both is
similar and the  differences are generally those of scale and proximity to
pollutant source.
                                   111-17

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         Berindan (1969) states:
                      Numerous authors recommend,  at present,  the necessity
                      of a zone which separates air polluting  industries from
                      other urban sectors.   This zone is compulsorily provided for
                      in the management plans of towns of certain countries.
                      The idea of planting this zone is to increase its protective
                      efficiency  and, consequently, to reduce  its surface area,
                      an essential advantage in view of the crisis of urban areas
                      which has become generalized in our time.

         An example of such a town in the U.S.S.R. is Volgograd, a new town

proposed by Milijutin, considered to be one of the best examples of urban zoning.

The plan of the town locates residential, industrial, railroad access, and park

land in linear bands perpendicular to the prevailing wind and  separates industrial
and transportation corridors from residential areas with wide  bands of "planted

protection zones."


         1.  Urban parks play an important role in the reduction of pollutant levels.


         Sherman (1972) comments:
                      Dr. Davidson studied the atmospheric concentration of
                      sulphur dioxide (S0_) in mid-Manhattan,  going from the
                      Hudson River to the East River along 79th Street downwind.
                      Remember that this is a single component of the air pollution
                      load, but an important one associated with the burning of coal
                      and oil.  The significant feature of this study is the
                      dramatic drop in the S02 level created by the presence of
                      Central Park in mid-Manhattan.  There are no belching stacks
                      in the park, so being pollution-free itself, it provides
                      an important, perhaps indispensable, dilution of the rest
                      of the community's air pollution load.  See Figure III-2.


         Bach  (1972) states:


                      For Hyde Park, a recreation  area of only one square
                      mile in size in the center of London, an average reduction
                      in the smoke concentration of 27% was found.

         Stanley Tankel  (1963) advocates the use of green wedges as opposed to
greenbelts due primarily to the  in flexibility of  the greenbelt concept in response  to

urban growth.  Green wedges, radiating from the urban center, can grow with the
demand  for urban development.  Also, they can respond to regional transportation
systems and provide access to regional open space.  See Figure  III-3.


                                   111-18

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                                FIGURE III-2
                SECTION ALONG 79th STREET, MANHATTAN ISLAND
                           (AFTER SHERMAN, 1972)
       '§
       b  2-
       CO
                         !40% dilution of S<
                          at Central  Park
              Hudson
              River
              WEST
Central Park
   East
  River
EAST
         There  are apparently no established minimum widths for such wedges.  They
are generally dependant upon local physiographic  features such as river valleys,
escarpments,  flood plains, etc.  However,  in Hagevik  (1974).literature is cited
which observes  that a 75% reduction of dust particles occurred within a 600  foot
wide greenbelt.  Hagevik also cites a study concluding that the concentration of
pollutants is decreased by half as they pass over 1500 feet of planted land.

         Work was also reported which demonstrated  that the pollutants from  a
phosphorous plant required a buffer of 2540 feet  in order to protect a citrus grove
from fluoride.   In another study, it was determined that suspended particles
from a dolomite  plant required a buffer of 1500 feet  in order to minimize impact.
                                    111-19

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Wedges
Primary open space:
available natural
features; i.e.
valleys
            FIGURE III-3
               WEDGES
rivers.
Secondary open space:
transportation related
                         FIGURE III-4
                          GREENBELTS
Greenbelts
 To contain growth and
 separate land use
 functions.
                           111-20

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                                   FIGURE III-5
                    STREET TREE PLANTINGS ARE ENCOURAGED AS
                  PART OF REGIONAL PLANTING AND BUFFER PROGRAM
Tt was also proposed that a buffer one mile wide be used around a hot mix asphalt
plant in order to minimize particulate pollution.
         Such  guidelines imply that a great amount of land be used for the
regional buffer systems.  If the minimum width for such sinks is established between
600 feet and one mile, depending upon the pollutant source and local conditions
and opportunities many hundreds of square miles would be involved.
system.
However, there are opportunities for other land uses within the buffer
Aside from its function as a pollution sink, the following are all compatible:
         2.
    .Recreation/Parks
    .Cemetaries/Memorial Parks
    .Education/Agriculture
    .Wildlife Protection
    .Protection of Natural Resources
        (flood plains, steep slopes, archeological sites,
        historic sites, etc.)
    .Sanitary Landfill
    .Spray Effluent Fields
    Planning design criteria for regional buffer systems resulting
    from overall consideration of the literature.
             a.  Radial wedge system based upon natural land features as primary
wedges and planted buffers along major transportation radials augmenting the
system.
                                    111-21

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             b.  Size of wedges determined by local conditions including pollutant
sources and prevailing winds.  Minimum width to be set at 600 - 5,000 feet.

                 Hagevik (1974) feels:

                      ...that the economics of providing buffer zones
                      to improve environmental quality do not justify locating
                      them in the most densely populated urban areas.  However,
                      several practical approaches to providing additional
                      sink potential to a region inlcude:
                 (1)  Thinning existing forest areas to increase turbulance and
increase leaf surface area.  Creating openings in dense canopies in order  to provide
thermal chimineys and increase exposure of pollution laden air to leaf surface.
Clear cutting edges of existing forests to provide additional edge areas.

                 (2)  Urban street tree programs in order to reduce ambient
pollutant levels.  According to Geiger (1950).streets with trees had 1000  - 3000
dust particles/litre; streets without trees had 10,000 - 12,000 dust particles/litre.
                      Commonly, in areas where street trees are doing poorly, such
as on many city streets, the plants are allowed to die and are not replaced.
Instead, additional trees should be planted to reduce the pollutant burden on the
existing trees by providing  adequate  leaf surface area to  bring pollutant levels
down to a level that can be tolerated by the trees.

     C.   LAND USE/GREENBELT ORGANIZATION

         The literature search findings indicates that the  use of greenbelts in
urban areas can have multiple benefits. Planners and engineers have,  to date,
recognized the positive contributions  of soil retention, physical separations
between non-compatible land uses, climatology,  etc.  It is  now evident that
greenbelts can contribute to the air cleansing process or urban pollutants.
                                      111-22

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             The land use planning process has utilized many techniques in order
to prepare plans which best serve the interests of the community.  Deciding on the
amount of acreage and the location of lands to be used for residences, commercial
establishments and industries, is a fairly straight forward process.  Open space
has usually been assigned to serve a recreational need, buffers between different
land uses, or it has been identified as land that does not or is not expected to
experience developmental pressures.

             Now that it is recognized that vegetative plantings within a buffer
area can trap particulates and remove other pollutants, the open space land use
takes on an increased level of importance.  Within current planning processes,
sufficient quantities of land are reserved to serve population and development
pressures.  Ideally, such lands are located in a manner which best serves the
interest of the community, e.g. industrial areas near transportation and utility
arteries; commercial plots near residential centers, etc.  Planners can reserve
grecnbelt open space lands using comparable planning design criteria.  The particular
technique that would be utilized requires considerable investigation to allow
planners to rationally quantify required areas for greenbelts and to locate  them
so that they tend to balance urban pollutant loadings.

             Planning design in the previous section calls for urban tree programs
to reduce ambient pollutant levels.  Such programs have usually been haphazardly
undertaken based upon vague civic Interest.  It should be considered that
rights-of-way along streets systems be put into an active use by being planted.
Such rights-of-way have been used for utility line placement and access, sidewalks,
etc.  Street plantings for pollution control should be inventoried and planned
for just as any other land use.

             The planning design criteria also calls for the use of radial
wedges to be utilized in consort  with major transportation arms and natural land
features.  The planners should now look to reserving such lands and, more
specifically, assign a value  to  them that  is comparable with that normally
associated with some of  the more dominant  land uses.

             The value of open space and greenbelts take on added dimension when
land use planners specifically identify their use as air pollution sinks.
Preservation of open space can significantly contribute to the maintenance of air
quality which elevates the value of open space above the historically associated
benefits of aesthetics and recreation.
                                     111-23

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             The objectives  of  this strategy is to locate an open space  area within
the influence area associated with maximum ground level air pollutants generated
from existing stationary  sources.   The information required in  order  to  establish
these areas includes:

             a.  The  effective  height of the emission source (H)
             b.  The percentage distribution of 'wind directions experienced at
the given point source  of pollution over a period of time (wind rose  showing
prevailing wind direction).
             c.  The  Stability  Class of the atmosphere - the degree of  turbulence
that is experienced during the  hours of operation of the source of  pollution.
             The coordinate  system in the Figure II-4 is used  in  the  analysis
of air pollution dispersion. The point identified as (x, 0, 0) is  located where
the maximum concentration of pollutants occurs most of the  time.given the
prevailing winds and  the  dominant stability class.

             In order to  determine point (x,0,0) the following  must be known:

             a.  Effective stack height obtained from area air  pollution central
agencies or calculated  using the Holland stack rise equation as defined  in Appendix D.
             b.  Prevailing  wind direction obtained from area meteorology stations
of published reports.
             c.  The  dominant stability classes obtained from area  meteorology
stations  are  determined from the following  table:
                                  TABLE  III-3

                              KEY TO STABILITY CATEGORIES
                 Surface W,nd
                Speed (at 10 m),  lncominS Solar Radiation  Thinly Overcast
m sec-1
< 2
2-3
3-5
5-6
> 6
Strong
A
A-B
B
C
C
Moderate
A-B
B
B-C
C-D
D
Slight
B
C
C
D
D
Ul
^4/8 Low Cloud

E
D
D
D
— J/8
Cloud

F
E
D
0
                The neutral class, 0. should be assumed for overcast conditions during
                day or night.
              One  may start the analysis by selecting the  prevailing wind direction
and stability class for the period of time during which the source usually operates.
With  these  inputs,  Figure 111-6,  may be used  in order to  determine x Max (x,0,0).
                                      111-24

-------
                               FIGURK IH-6
    DISTANCE OF MAXIMUM CONCENTRATION ANb MAXIMUM xu/Q AS A FUNCTION OF
STABILITY (CURVES) AND EFFECTIVE HEIGHT (METERS) OF EMISSION  (NUMBERS)
                                    111-25

-------
          The point x Max merely provides a centroid of pollutant concentrations.
 Naturally, the pollutants spread downwind and in a crosswind direction around
 this point.  The task of designing the  actual buffer involves many inputs.  As a
 starting point, an idealized configuration is as shown in Figure III-7.
                                  FIGURE III-7
                 TWO DIMENTIONAL RELATIONSHIPS BETWEEN SOURCE,
                           SINK, AND RECEPTOR LOCATIONS
source
                                                                    receptor
          Under ideal circumstances, theta (•&)  should represent  a  sweep
  angle  of predominating winds for the site.   Where consistent winds  are  encountered,
     will be  smaller than where the winds are less limited in their  directions.
           The  land use planner would need to locate all point  sources  and  determine
  x Max  for each  case.  The position of sensitive land uses relative to the point
  sources,  would  be plotted and the buffer configuration ideally expanded  to shield
  the  receptor.

           If available open space were not at a premium in an  urban area,  the
  logical  buffer  design would be a series of concentric belts,  each with an inside
  radius equal  to the  particular x Max, around each point source.
                                      111-26

-------
                                  FIGURE III-8
                       IDEALIZED POINT SOURCE BUFFERS WITHOUT
                            REGARD TO LAND CONSTRAINTS
           This seems hardly ever  feasible.  Therefore, we end up with configurations
  such as shown in Figure III-9 where the  open  space  is designed as arcs.
                                   FIGURE  III-9
               IDEALIZED POINT SOURCE BUFFER WITH LAND CONSTRAINTS
»
     I
    *
source
4
b
                       *
                       a
                  *
                  c
           The estimation of horizontal dispersion  of  the pollutants is necessary
  in order to determine the arc length of  the  buffer.  The  Gaussian dispersion in a
  y axis helps determine this arc length of  the  greenbelt as do variations in prevailing
  wind directions (6-).   Finally,  the space available for placing  these buffers will
  determine final configurations.

           Planning the location of greenbelts can  only be  done within the
  context of the comprehensive land use planning process.   The input variables are
  of such a magnitude that no generalization can be made other than those outlined
  in the foregoing procedures.
                                        111-27

-------
     D.  CONVERSION OF LEAF AREA TO GROUND AREA AND  WEIGHTED  SINK FACTORS

         The sink and emission factors for soil are reported  in this project
relative to the surface area of the soil as a unit of measure.  Therefore, the
relative removal rate or the emission rate for soil is reported as micrograms/
square meter/hour.  The removal rate or the emission rate, reported for various
types of vegetation is also given in units of micrograms/square meter/hour.  However,
in the case of vegetation, square meters refers to the surface area of the leaves
and not the ground area over which the vegetation grows.  Therefore, in order to
estimate the gross removal rate, or emission for an open space, it is necessary
to convert to square meters the canopy area (that is, the ground area shaded by the
covering vegetation) to leaf surface area.  This requires that one knows the height
and canopy diameter of each species of tree growing on the site.  It also requires
knowledge of the relationship between the particular species  of vegetation involved
and its leaf area at various stages in its life history.  We  used the following
process in making required adjustments which allow us to draw general conclusions
from the available literature.  In addition to determining the relationship
between canopy area and leaf area, it is also necessary to determine average removal
and emission rate for various general types of vegetation. This is important because
the literature does not contain much specific information about more than a few
species of plants.  Taken together then, determination of a typical leaf surface
area for an open space, in combination with a typical removal or emission rate
for the same area, will allow us to estimate the rate of removal for certain
specified pollutants.  Table III-ll,entitled SUMMARY OF SINK AND EMISSION FACTORS
FOR NATURAL ELEMENTS , appeared in Volume I and it has been used here as the basis
for a further modification, adapting it more directly to an integrated use in
conjunction with estimation of leaf surface areas.  That Summary Table is based
upon selective averaging of the sink and emission factors for each pollutant under
consideration.  It was meant as a first rough approximation of the broadest inter-
pretation of the reviewed literature and must be utilized with that caution in mind.
It reflects the factors associated with both deciduous and coniferous trees as well
as shrubs and various ground covers treated by the literature.  Therefore, in order
to make the summary table more applicable to an evaluation of woody plants in open
spaces, it was determined to modify the Summary Table slightly in the following way.
                                     111-28

-------
The average value for vegetation or soil serving as a sink for each of the
pollutants, was taken directly from the Table.  The detailed tables of emission
and sink factors, which also appear in Volume I, Section III, were reviewed and
where specific or general averages were available relating to the specific
pollutants, these figures were also considered in creating a new average sink rate
as shown on Table III-4   in this Volume.  The end result is that based on the
available literature,the average sink or emission rates are weighted toward the
vegetation or soil which we would most likely expect to find in an open space
project in St. Louis, Missouri.  This project area is further defined
in Volume III of this report.

         In order to estimate the sink capacity of some representative vegetation,
it is necessary to relate total leaf area to canopy diameter.  This relationship
can be made for several representative trees based upon information provided by
Rich (1970) and Monteith (1976).  They have reported ratios of the surface area of
certain trees to their height and canopy diameters.  The logic of our approach
to this analysis, and the use of Leaf Area Indexes, is detailed in Appendix C of
this Volume.  Here, the conclusion of that interpretation has been used to create
Table III-5.
                                   111-29

-------
                                         TABLE III-4
                   WEIGHTED SINK AND EMISSION FACTORS FOR AVERAGE SOIL AND
                   AVERAGE VEGETATION BASED ON DATA REPORTED IN VOLUME  I
     POLLUTANT
 ECOSYSTEM ELEMENT
                                 REMOVAL RATE
REFERENCE
CARBON MONOXIDE
Vegetation
Vol.1 (Table III-11)
Average Unspecified
    Weighted Average
                               2.5 x 10  yg m
                               2.75 x 103 yg m"
                                       3     -2-1
                               2.6 x 10  yg m  hr
                                                                       1  rBidwell & Fraser, 1972
                                                                       '1 \Ziegler, 1975
                     Soil
                     Vol. I (Table III-11)Average
                     Forest soil - Charlton
                     Forest/field soil
                     Columbia, Mo.
                     Mt. Olive, Miss.
                         Weighted Average
                               2.0 x 104 yg m 2hr l
                               2.2 x 104 yg nf^r'1
                               8.0 x 10  yg m^hr"1
                               3.82 x 104 yg m~2hr~L
                               1.52 x 10  yg m~ hr~
                                       4     -2-1
                               1.9 x 10  yg m  hr
                                                     rHeichel,1973a
                                                     LHeichel,1973b
                                                      Heichel,1973b
                                                      Ingersoll, 1972
                                                      Ingersoll, 1972
NITROGEN OXIDES
Vegetation
Vol. 1 (Table III- 11) Average  2 x 1C3 yg nf
Unspecified
Unspecified
    Weighted Average
                               7.42 x 1Q  yg nhr"
                                        3     -2  -1
                               4.09 x 10  yg m  hr
                                       3     -2  —1
                               2.3 x 10  yg m  hr
                                                                           Heggestad, 1972
                                                                           Dochinger, 1974
                     Soil
                     Vol. 1 (Table 111-11) Aver age   2.0 x 102 yg
OZONE
Vegetation
Vol. 1 (Table III-11)Average
white oak
white oak
sugar maple
sugar maple
Ohio buckeye
Ohio buckeye
sweet gum
sweet gum
                                                    8.0 x 10  yg nfr"
                                                    6.35 x 104 yg m'^r"1
                                                    1.32 x 105 yg nf^r'1
                                                    3.71 x 10  ug m  hr
                                                    8.63 x 104 yg nf^r'1
                                                    3.62 x 104 yg nf^r""1
                                                    9.27 x 104 ug m"2^"1
                                                      Townsend, 1974
                                                      Townsend, 1974
                                                      Townsend, 1974
                                                      Townsend, 1974
                                                      Townsend, 1974
                                                      Townsend, 1974
                                                      Townsend, 1974
                                                    2.78 x 10  ug m 'hr
                                                             4     -2-1
                                                    8.54 x 10  ug m  hr    Townsend, 1974
                                               111-30

-------
     POLLUTANT
 ECOSYSTEM ELEMENT
                                 REMOVAL RATE
REFERENCE
OZONE (cont.)
Vegetation
red maple
red maple
white ash
white ash
    Weighted Average
                                                    2.72 x 10  yg
                                                    5.55 x 10* yg
                                                    2.39 x 104 yg
                                                    5.62 x 104 yg
                                                    6.2 x 104 yg n
                                                      Townsend, 1974
                                                      Townsend, 1974
                                                      Townsend, 1974
                                                      Townsend, 1974
                     Soil
                     Vol. 1(Table I11-11)Average
                                       Q    -2-1
                               1.0 x 10 yg m  hr
PAN
PARTICULATES
Vegetation
Vol.(Table III-11)Average

Vegetation
Vol. 1 (Table III-11)Average
hardwood canopy
conifer canopy
chestnut
tuliptree
    Weighted Average
                                                            ,      _   .  /-Jenson, 1973
                                                    1.2 x 10  yg m  hr   j^Hill, 1971
                                                    4.0 x 10  yg nT
                                                    1.79 x 103 yg nf
                                                    6.28 x 103 yg n
                                                    2.74 x 103 yg m'
                                                    3.0 x 102 yg m'
                                                    2.5 x 103 yg m'
                                                      Dochinger, 1972
                                                      Dochinger, 1972
                                                      Chasseraud,1958
                                                      Wedding,et al.,1975
SULFUR DIOXIDE
Vegetation
Vol. 1 (Table III-11)Average
forest(unspecified)
vegetation (unspecified)
vegetation (unspecified)
    Weighted Average
                                                    5.0 x 10  yg nfr"
                                                    3.33 x 103 yg m'^r"1
                                                    1.47 x 104 yg tn'^r"1
                                                    ] .45 x 10  yg m  hr
                                                    4.1 x 104 yg n^hr"1
                                                      Davis, 1975
                                                      Dochinger, 1974
                                                      Jensen, 1973
                     Soil
                     Vol. 1 (Table III-11)Average
                     oolitic limestone
                     acid soil (unspecified)
                         Weighted Average
                               1.15 x 10  yg
                               1.68 x 105 yg
                               1.15 x 107 yg
                               7.7 x 106 yg n
                                                      Spedding, 1969
                                                      Bohn, 1972
                                              111-31

-------
                                TABLE III-5
      SPECIES RELATIONSHIP OF GROUND AREA COVERED TO PLANT SURFACE AREA
       SPECIES
HEIGHT
GROUND AREA COVERED
PLANT AREA
Maple
(Acer plantano-ides)
Oak
(Quercus robur)
Poplar
(Populus tremula)
Linden
(Tilia cordate)
Birch
(Be tula vevrufiosa)
Pine
(Pinus sp.)
6m
6m
6m
5m
5m
3m
7
7
7
4
4
1
. 1m
. 1m
. 1m
.5m2
.5m
.8m
36.8m2
36.1m2
52.5m2
23.0m2
27.2m2
4.2m2
Having weighted sink factors and a relationship of total leaf area to ground area,
we can develop the following table:
                                TABLE III-6
                     SELECTED TREES AS POLLUTION ' SINKS
                                            ug/hr
                                       TYP ftons/vr)
One maple tree (6 m high)
sulfur dioxide
participates
carbon monoxide
nitrogen oxides
ozone
PAN
One oak tree (6 m high)
sulfur dioxide
particulates
carbon monoxide
nitrogen oxides
ozone
PAN

1.5 x 19*
9.4 x 10*
9.6 x 1CK
8.5 x lo£
2.3 x 10°
4.4 x 10

1.5 x lOJj
9.0 x 10J
9.4 x lo£
8.3 x HT
2.2 x 10°
4.3 x 10^

1.0 x 10~2
9.0 x 10~7
9.0 x 10"?
8.0 x 10";
2.0 x 10 ,
«£L
4.0 x 10 *

1.0 x 10"?
9.0 x 10~£
9.0 x 10~^
8.0 x 10,
2.0 x 10 7
— /*
4.0 x 10
                                      111-32

-------
                                TABLE III-6(cont)
*Conversion of pg/hr to tons/yr.
 pg/hr x gm/106PB x lb/453.59 gm
  x T/2000 Ibs x 24 hrs/day
  x 365 days/yr  =  T/yr
                                              ug/hr
TYP (tons/yr)
One poplar tree (6m high)
sulfur dioxide
particulates
carbon monoxide
nitrogen oxides
ozone
PAN
One linden tree (5 m high)
sulfur dioxide
particulates
carbon monoxide
nitrogen oxides
ozone
PAN
One birch tree (5 m high)
surfur dioxide
particulates
carbon monoxide
nitrogen oxides
ozone
PAN
One pine tree (3m high)
sulfur dioxide
particulates
carbon monoxide
nitrogen oxides
ozone
PAN

2.2 x 10^
1.3 x 103
1.4 x 103
1.2 x 10£
3.3 x 10
6.3 x 10

9.4 x 10^
5.8 x 107
6.0 x 10?
/i
5.3 x 107
1.4 x 10°
2.8 x 10

1.1 x 10?
6.8 x 107
7.1 x 10,
6.3 x 10^
1.7 x lo£
3.3 x 10

1.7 x HTJ
1.1 x 10J
1.1 x 107.
9.7 x 105
2.6 x 10-
5.0 x 10J

2.0 x 10"
i.o x io~;r
1.0 x 10 ^
1.0 x 10~2
3.0 x 10"
6.0 x \0

9.0 x 10"^
6.0 x 10 ~7
^£l
6.0 x 10 7
5.0 x 10~2
1.0 x 10~
3.0 x 10

1.0 x 10"
7.0 x 10 7
7.0 x 10~7
mm/I
6.0 x 10_2
2.0 x 10~,
3.0 x 10

2.0 x 10~,
1.0 x 10~*
1.0 x 10"^
9.0 x 10"
3.0 x 10"
5.0 x 10"3
                                    111-33

-------
GLOSSARY
 IV-1

-------
AIR POLLUTION - Contamination of the air by liquids, solids and/or gases at
 unexceprably high levels (except water in its several phases) or in unnatural,
 anthropogenic forms.  Typical natural contaminants are salt particles from
 the oceans or dust and gases from active volcanoes.  Typical anthropogenic pollutants
 are waste smokes and gases formed by industrial,  municipal, household, and
 automotive combustion processes.

BUFFER - Used here to mean land used to separate one land usage from another.
 Especially relating to open space used to insulate one land use from a contiguous
 land use.

CONIFEROUS - Refering to cone bearing trees.  Generally, evergreen needle-leaved
 vegetation.

D.B.H. - diameter breast height - The diameter of the trunk of a tree measured at
 approximately 4.5 feet above the ground.

DECIDUOUS - Refering to those plants which shed their leaves seasonally.  Generally,
 plants other than evergreens.

GLABROUS - Smooth, without fuzz or hair.

GREENBELT - In this report, an open space land use within, or around, urban growth
 and separating one land use from another.  Usually, an open space band at least
 a few hundred feet wide and of variable length.

LENTICLES - Corky spots on young bark, corresponding in function to stomata on
 leaves (i.e. relating to gas exchange).

LEAF LAMINA - The flattened body of a leaf.  A leaf consists of a stem  (stalk or
 petiole) and a lamina.

OPEN SPACE - In this report, a park or natural area unoccupied by formal structures
 and generally unspoiled and permitting the natural processes of animal and plant growth.

PARTICIPATES - Minute and separate particles which may be viable (e.g.. pollen,
 bacteria, viruses, protozoans, etc.) or non-viable, (e.g. mineral dust, metals, etc.)
 and which are readily transported.  Generally, sizes of particulates range between
 0.0005 and 500 micrometers in diameter.

PHOTOSYNTHESIS - The process by which green plants convert water and carbon dioxide
 into sugars and oxygen.

PETIOLE - The stem of a leaf.

SHELTER BELT - A linear planting of shrubs and trees generally parallel to
 agricultural fields to protect  them from winds (i.e. a windbreak).

STOMATES-(vernacular; sing, stoma; pi. stomata) - A microscopic opening generally
 on the lower surface of leaves, through which there is a gaseous interchange
 between  the atmosphere and the  interior of the leaf.

TRANSPIRATION - The movement of water from the internal circulation of  a plant
 through  its surfaces  (such as the leaves) into the atmosphere as water vapor.
                                       IV-2

-------
BIBLIOGRAPHY
   V-l

-------
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Bernatzky, A.   1968- "Protection plantings for air purification and improvement
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                                      V-2

-------
Caborn, J.M.  1957.  "Shelterbelts and microclimate."  Forestry Commission, Bulletin
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                                      V-4

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Ewing, B.B., and J.E. Pearson.  1974. "Lead in the environment."  Advan. Environ.
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    catch  of airborn particles by a woodland  canopy."  Jour. Appl. Ecol.,7:441-461.
                                     V-13

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White, J.J.  1932, "Carbon monoxide and its relation to aircraft."  U.S. Nav.
   Med. Bull.. 30;151.

Willis, B.H., J.R. Mahoney, and J.C. Goodrich.  1973. "Hackenaack Meadowlands
   air pollution study - air quality impact of land use planning."  EPA Contract
   No. EH3D 71-39, Research Triangle Park, North Carolina, 139 pp.

Williston, Hamlin L.  1971. "Guidelines for planting and maintaining Loblolly pine
   and other cover for roadbank stabilization."  Tree Planter's Notes,22(2);14-17.

Wolsko, T.D., M.T. Matthies., and R.E. Wendell.  1972. "Transportation air
   pollutant emissions handbook."  Argonne National Laboratory, Argonne, Illinois.
   (No page numbers).

Woodruff, N.P., and A.W. Zingg.  1953. "Wind tunnel studies of shelterbelt
   models."  J. of Forestry. 51(3);173-178.

World Meterological Organization.   1964. "Windbreaks and shelterbelts."  Tech.
   Note No. 59, Geneva, Switzerland, 188 pp.

Wylie, P.B., and L.C. Bell.  1973. "The effect of automobile emissions on the lead
   content of soils and plants in the Brisbane area."  Search, 4(5) -.161-162.

Young, W.C.  1968. "Ecology of roadside treatment."  Jour, of Soil and Water
   Conservation. 23:2.

Ziegler,  L.  1973. "The effect of air-polluting gases on plant metabolism."
   Environon. Oual.  Saf..  2: 182-208.

Zinke, P.J.  1967. "Forest interception studies in the United States."  In:
   Int. Sym. on Forest Hydrology. W.E. Sopper and H.W. Cull, ed., Pergamon Press,
   Oxford, England,  pp. 137-161.
                                    V-14

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       APPENDIX A



HIGHWAY DIFFUSION MODELS
         VI

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I.   INTRODUCTION

     The purpose of Appendix A is to investigate the possibilities of incorporating
vegetation sink factors for air pollutants into four(4) atmospheric dispersion models
that predict carbon monoxide (CO) concentrations from highway sources.  These models
include 1) the EPA HIWAY model,2) the California Line Source Model,3) the SRI Street
Canyon model and, 4)Emp 1, an emperical model.

     These models are reviewed by Noll et al.(1975), and a discussion of each
follows,

     A.  EPA MODEL

         The EPA HIWAY computer program serves to estimate nonreactive air pollutant
concentrations downwind from a highway line source of some specified finite length.
Concentration is calculated not as the result of a continuous line source as such, but
rather by the approximation of the line source by a finite number of evenly spaced
continuous point sources of strength equal to the total line source strength divided
by the number of sources used to simulate the line.

         The model itself considers each lane of traffic as an individual line
source.  Thus, traffic estimates for each lane are required.  Total concentration
is calculated using superposition, i.e., concentrations from the separate line
sources are additive.

         Because of the physical significance of mechanical mixing above the
roadway, some initial values of vertical and horizontal dispersion parameters must
be assumed to allow the plume to conform to the actual plume shape encountered.  To
accomplish this, the point sources are displaced by some virtual distance to the rear
such that sigma z and sigma y have an initial value at roadside.

         With the exception of receptors directly on the highway or within
the cut, the model is applicable for any wind direction, highway orientation, and
receptor location.  The model was developed for situations where horizontal wind flow
occurs.  The model cannot consider complex terrain or large obstructions to the flow
such as buildings or large trees.

                                      VI-1

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         The EPA HIWAY model simulates a highway with a finite number of point sources
and calculates the downwind concentration from each point using the Gaussian point
source diffusion equation.  The total contribution of all points Is calculated by
a numerical integration of the Gaussian point source equation over a finite length.
The coordinates of the end points source equation over a finite length.  The coordinates
of the end  points of a line source of length L, representing a single lane, extending
from point A to B (see Figure VI-1) are R., S , and RR, SB-  The direction of the
line source from A to B is 3.  The coordinates R, S of any point alcng the line at the
arbitrary distance I from point A are given by:
                             R  =  R  +  I  Sin 8
                    S = SA + £ cos B                        (2)
 Given a receptor at R. ,  S, ,  the  downwind distance,  x,  and the crosswind
,  y,  of the receptor from the point R,  S for any wind direction 9 Is given by
                             S  =  SA +  £  cos  B

distance, y, of the receptor

                   x  =  (S - Sk) cos 0  +  (R - Rk) sin 9              (3)
                   y =  (S = Sk)  sin 9 - (R - Rk) cos 9
Since R and S are functions of £, x and y are. also functions of SL.  The concentration,
X from the line source is then given by:
                         /
                                                                     (5)
where for stable conditions or if the mixing height is greater or equal to 5000 meters:
                                        VI-2

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                                 FIGURE VI-1

                  LINE SOURCE AND RECEPTOR RELATIONSHIPS
                          FOR EPA HIWAY MODEL
NORTH
                                              WIND
                                        RECEPTOR
                                        (
                                                                (RB,SB)
                                                                    EAST
                                                 SOURCE:   (Noll,  et  al.,  1975)
                                  VI-3

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!
2iro o exp
y z
~-i~M
_ 2 I',/
7
s
r^
exp
                                                     exp
  lfz-»-Hl    V  ,fiv
- ^ -r-l    f  (6)
where         H = height of the road above ground level, m
              z = height of the receptor above ground level, m
       a  & a   = horizontal and vertical dispersion parameters,
        '         respectively, m.
In unstable or neutral conditions, if a  is greater than 1.6 times the mixing height,
                                       Z
L, the distribution below the mixing height is uniform with height regardless of
source or receptor height provided both are less than the mixing height:
                                                                   (7)
         In the above equations, a  and a  are evaluated for the given stability class
                                  y      z
and the distance x + b for a  and x + a for a .  A and b are the virtual distances
required to produce the initial a  and a  respectively.

         The value of the integral (Eq. 5) is approximated by use of the trapezoidal
rule.  Let A2, = L/N.  Then the trapezoidal approximation gives:
                    X =
                                            N-l
                                                                    (8)
where f. is evaluated from  the appropriate Equation 6 or  7 for Si +  iAfc.  x and y
are functions of   £.

         For a given initial choice of the interval length, A£, the calculation is
then successively  repeated  with  twice the number of intervals, that is, with  At/2,
M/4..., until the concentration estimates converge to within 2 percent of the previous
estimate.  This value then  represnets the true value of the integral.
                                        VI-4

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         The above evaluation of the Integral is repeated for each lane of traffic
and the resulting concentrations summed to represent the total concentration from
the highway segment.

     B.  CALIFORNIA MODEL

         The California model calculates pollutant concentrations generated by
motor vehicles within a microscale highway corridor.  The mathematical model, which
is based on the Gaussian infinite line source diffusion equation, calculates hourly
concentrations of pollutants within a turbulent mixing cell above the highway as
well as at receptor points at given distances downwind.

         In the crosswind case, the mixing cell concentration is determined by the
wind speed and pollutant emission rate of the vehicles.  Dispersion downwind is
dependent on the atmospheric stability classification.  In the parallel wind case,
the California model accumulates pollutants within the mixing cell to account for
downwind buildup.   Pollutants are then dispersed latterally at a rate dominated by
stability class.  The computerized model is capable of estimating pollutant concentrations
where the winds are either parallel or at an angle to the highway alignment and where
the highway section may be at grade, elevated or in a cut.

         The California model uses separate equations for calculating pollutant
concentrations under crosswind and parallel wind conditions.  The most general form
of the crosswind equation has the form of the Gaussian line source equation:
              2 K az Us1n *
                             exp -   (        + exp -
(9)
where         C = concentration of pollutant gm/m
              Q = emission source gm/sec-m
                = wind speed m/sec (1 mph = 0.447 m/aec)
              K = empirical coefficient = 4.24
              ij> = angle of wind with respect to highway alignment
             a z = vertical dispersion parameter, in meters
              H = height of highway above surrounding terrain, in meters
              z = height of receptor above surrounding ground surface, in meters

                                        VI-5

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         For the parallel wind case, the California model accounts for a buildup
of pollution concentration within the mixing cell.  The estimated concentrations
within the mechanical mixing cell for aprallel winds, where the ratio of 30.5/W is
less than or equal to one, can be determined from the following equation:

                           C- A  & 1  30.6                       (10)
                                  U  *    w
where         C = concentration of pollutant (gm/m3) within the mechanical mixing
                  cell
                = wind speed (m/sec)
              K = empirical coefficient 4.24
              W = width of roadway from edge of shoulder to edge of shoulder,
                  in meters
              A = downwind concentration ratio for parallel winds (accumulation
                  term) is defined as C K     W .
                                       Q    30.5

          30.5  = the initial width  (meters) of the highway used for  the finite
                  element of area in developing the model for parallel winds
              Q = source emission strength  (gm/sec)

         For parallel winds, the source emission  strength (Q) is calculated using
the following equation:
              Q = {emission factor}  x {vehicles/hour} x  {5.26 x  10~  }    (11)
Where  the numerical constant is a factor  to convert units of the product (vph)
(gm/mi)  to gm/sec for a length of highway of  100  feet.

         To estimate the ground level pollutant concentration at a distance away
from the highway  (when the wind is  parallel to the alignment) the following equation
is used.
                                   exp - j- (=5-
(12)
                                         VI-6

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where  ppm    = concentration of CO at the highway within the mechanical mixing
           me     , ,
                cell
            Y = normal distance in meters from receptor to near edge of highway
                shoulder
        o ,o  = horizontal and vertical dispersion parameters in meters.  These
         y  Z   values are obtained from empirical data depending on the receptor's
                normal distance (Y) from the highway and on the stability class.

         The California model reduces to two simpler equations when one solves for
at-grade cases.  For mixing cell concentrations with crosswinds, equation (9) reduces
to:

         Cmc = *    .Q  , grams/cubic meter                 (13)
               K, 1 11 sin 4p

where    Q = source strength, grams /meter-second
         K = empirical constant = 4.24
         y - wind speed, m/sec
         <() = wind angle with respect to road (90° for winds perpendicular to the road)

For downwind ground level receptors and at grade highways for crosswinds, equation
(13) reduces to:
             K a zy sin (j»
where   az = vertical dispersion parameter, meters

     C.  MAJOR DIFFERENCES IN THE MODELS

         The major differences in the two models are outlined

         California's model uses a Gaussian line source equation while EPA uses
an integrated point source equation.  As a result, the California model requires
separate equations for predicting under crosswind and parallel wind conditions while
EPA's model needs only one equation.  The California model uses a wind angle of
12.5° with respect to the road as the boundary separating the two regions within
which different equations are used.  As a result, a discontinuity occurs at 12.5
between the concentrations predicted by the two equations.

                                        VI- 7

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         EPA's HIWAY model requires separate traffic and emission data for each
lane of the highway.  Downwind concentrations are calculated by superimposing the
separate pollutant contributions of each traffic lane.  California's model uses the
total traffic volume and emission rate for all lanes combined, assuming that all
emissions are initially dispersed from a uniform "mixing cell" extending from road
shoulder to shoulder (for medians <30 ft.).

         Initial dispersion of pollutants at the roadside edge is handled differently
in the two models.  The EPA model uses a virtual source correction providing an
initial a  =1.5 meters.  The California model assumes a "mixing cell" with initial
         z
az = k meters. (See Figure VI-2).

         Downwind dispersion  is described by the empirical dispersion coefficients,
a  and a .  Both models use different dispersion coefficients.
 y      z

     D.  MODEL ASSUMPTIONS

         The following basic assumptions are common to both models.

         1)  The mass of pollutants is conserved throughout the downwind length
of the plume.  No material is lost by reaction or by sedimentation.
         2)  The ground surface, when encountered, is a perfect plume reflector.
         3)  There exists no wind shear in the vertical direction.  The wind velocity
used should be representative of the average wind velocity between ± sigmaz from
the plume centerline in the vertical sense.
         4)  Dispersion occurs only by turbulent diffusion which varys according
to Pasquill's atmospheric stability categories.
         5)  Atmospheric stability is constant within the mixing layer containing
both sources and receptor.
         6)  There exists no mixing of material in the x axis (i.e., longitudinal
mixing).
         7)  Emissions are from continuous sources.
         8)  The dispersion parameters sigma  and sigma  are good for modeling
                                            y          z
atmospheric dispersion over flat, grassy terrain with no significant aerodynamic
roughness nor any artifical vertical instability induced by heat island effects
associated with urban areas.
                                      VI-8

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                     FIGURE VI-2

     DISPERSION FROM VIRTUAL IMAGE  (EPA MODEL)
         AND MIXING CELL (CALIFORNIA MODEL).
Virtual
 Image
  of
 Plume
                       EPA Model
                      Htxlng Cell
                 /=A
                 (00          OCA
                 yEEz^E^
                                              Plume
                     California Model
                                           SOURCE:  Noll, et al., (1975)
                       VI-9

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      E.   SRI STREET CANYON SUBMODEL

         Stanford Research Institute's (SRI) Street Canyon Submodel was  determined
from an experiment conducted by Stanford Research Institute in San Jose, California
in 1971  to estimate the dispersion of vehicular carbon monoxide emissions within a
city street canyon.  For this work air motion within the canyon was believed to be a
single-helical circulation.   As shown in Figure VI-3, this helical air circulation
gives substantially higher concentrations to receptors on the leeward side (right
side of the figure) than on the windward side (left side of the figure) because of the
reverse flow component across the street, near the surface.  This model assumes that
the measured concentration,  C, at the receptor is derived from two components.  One
components is contributed from a background concentration, C.. , in the air entering
the canyon from above, and the other concentration component, AC, is supplied from
locally generated vehicular pollutant emissions, Q, in the street.Hence, we have

                                C = Cfek + AC                   (15)

         This model calculates the concentration component fron the vehicular
emissions  at a given receptor location by three different equations.  Different
equations are used depending on whether the wind directions are parallel or crosswind
with respect to the road angle and whether receptor locations are on the leeward or
windward side of a canyon.

         1.   Leeward Case.

              A leeward case equation is employed to calculate concentrations,
AC, from local vehicular emission for crosswinds (wind directions greater than 30
with respect to the road) and the receptor side of the highway where reverse air
movements within the canyon transports vehicular emissions directly to the receptor.
This equation can be represented by a simple box model form.
                                ACL = Q/UgY                   (16)
                                        VI-10

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                                   FIGURE VI-3

                          SRI STREET CANYON DESCRIPTION
   Canyor
   Walls
                       Windward
                         Side
                                                                Mean Wind
                                      Leeward
                                        Side
                                                          Canyon
                                                          Walls
where
               U
                s
                Y =
                                     SOURCE:  (Noll et al.,  1975)

       concentration component from the vehicular emissions
       for a receptor on the leeward side of the highway

       rate of vehicular pollutant emissions

       mean wind speed near the street

       depth of mixing volume
The leeward case model was then determined by SRI to be as follows:
                                     K x Q
where

where
Q

U
                          (U + 0.5) x (X2
                                     LQ)
                                                                     (17)
rate of vehicular pollutant emissions in the street (gm/ (m-sec)).

rooftop wind speed (m/sec.), 0.5 m/sec. is due to the influence
of the vehicles forward motion.  Therefore, U  of the box
model - k!(U + .5).                          s
                    horizontal distance from the receptor to the center of the nearest
                    lane (m) .

                    vertical distance from the road to the receptor (m) .
                                     VI-11

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where         L  =  two meters, the dimension where vehicular emission was assumed
                    completely mixed.  Therefore,  the depth of mixing volume (Y)
                    from a box model  . kz((x2 + Z2)% +
         2.   Windard Case.

              A windward case equation is for crosswind directions and for receptors
located on the windward side.  Similar to the previous leeward case, a box model concept
was also used for fomulation of this equation, where the depth of mixing volume is
considered to be constrained by the canyon's size.

                      AC  =       K x Q         (H - Z)                  (18)
                              W x (U + .5)  " X     H

where         AC  =  vehicular emissions concentration component for receptors
                     on the highway's windward side.

               W  =  width of canyon (m).
               H  =  average  building height or depth of depressed highway (m).

         3.   Parallel Case.

              A parallel case equation was determined for wind directions within
- 30° of the highway angle and for prediction of concentrations at receptor locations
on either  highway side.  This equation predicts parallel wind concentrations by taking
an average of the leeward and windward equation.

                             AC.J.  = JS(ACL  +  ACW)                   (19)

where         AC   =  the parallel wind concentration component from the vehicular
                      emissions.

     F.  EMPRICAL MODEL

         As  a result of the  work accomplished by Noll, et al.,  (1975) an empirical
model was  developed to predict CO concentrations from a highway source.  This empirical
model,  called EMP-1, was derived from simple dimensional analysis and has  the form:
                                      VI-12

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                              C a _ k Q                    (20)
                                    U  (X/sin 0)a

where         C  =  concentration at ground level from an at-grade highway, ug/m
              Q  =  pollutant emission rate, ug/m-sec
              U  =  mean wind speed normal to the road, m/sec
              X  -  distance from center of the road to the receptor
              0  =  the angle of the wind with respect to the road, degrees,
          K & a  =  empirical coefficients

         A regression analysis was performed on In (CD /Q) versus In (X/sin 0)
using 524 measurements during perpendicular and oblique wind conditions by Noll,
et al., (1975).  The values obtained for the slope of the regression line a = -1.106
and the intercept k = 8.18 were used to calibrate the model.  The final equation
for EMP-1 was

                               C           8.18Q
                                    U  (X/sin 0) 1.106
II.  INCORPORATION OF SINK FACTORS IN MODELS

     The following discussion and calculation are an attempt to incorporate sink factors
into the four models previously discussed.  A few words of caution are needed before
presenting these ideas.  First, it should be noted, that the state of the art of
using sink factors is not advanced to the point where one can confidently predict
the amount of pollution that will be adsorbed or absorbed by a given species of
vegetation.  Much more research is needed in this area.  Secondly, using buffer strips
near highways, changes the aerodynamics of the plume generation by the highway.
Most of the models discussed in the previous section are valid only for flat terrains
with no interference.  By using buffer strips, the models themselves are not accurate.
Thirdly, once the plume enters the buffer strip area, its characteristics will change
drastically.  The vegetation will create changing flow patterns as the plume travels
amongst  the trees.  Thermal chimney produced by gaps in the buffer strip will produce
additional changes in the plume.  Therefore, it is almost impossible to predict the
exact characteristics of the plume and its interaction with the vegetation.  Given the
above considerations, it is easy to conceptualize that incorporating sink factors into
mathematical algorithm to predict concentration of CO from highways is no easy task.
                                       VI-13

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     The methodology discussed in the remainder of this section for incorporating
sink factors into the four models is an initial attempt to perform this task.  The
models should only be used for planning purposes and not to predict exact concentrations
of CO.  Further research is needed to colaborate these proposed model modifications.

     A.  GENERAL THEORY

         For the California Line Source Model, the EPA HIWAY Model, and the
Empirical Model EMP 1,   there are two modifications that must be discussed.  The
first modification is the determination of the portion of the plume that will enter
the buffer.  The second modification is the development and incorporation of a
pollution sink factor into the  highway emission rate.

         To determine the portion of the plume that will be effected by the planting
of vegetation, it can be seen from the following illustration that Area A of the plume will
be unaffected where as Area B will be affected.
               mixing   If
                cell
     Area A

     Area B
TOTAL AREA
4L
                                 0       0   z
                                 0 (62-H)
                                           (5-4)-4L0 - JjL0 (H-4)
4L
4L
                                           (H-4)
                                           (6z-4)
                           .    *     ,P   . u
Fraction of Pollution Entering Trees if az> H =
                                                             (H-4)
                    4L0 +
                                              (oy-4)
                                                                           (22)
         The quantity of pollution leaving the buffer (Q2) can be determined by the
inclusion of the buffer sink factor (SLA) into that portion of the highway emission
rate  (Q) that is affected by the buffer strip
                                       VI-14

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                                  4L,  +  !*„ (H-4)
                        «2-«l   4L°  +  ^ (T.-4)  -   (SLA)
                                             2
where         S = Buffer sink rate - gm/sec-m  of vegetation
              L = Depth of Buffer, m
              A = Canopy Area Index, m^ canopy area/nr land

         In other terms SLA is the quantity of pollution absorbed by a buffer,
of a specific depth (L), per length of highway.  Essentially, Q2 is the quantity
of pollution remaining in the air as the air leaves the buffer strips.

     B.  EXAMPLE OF CALIFORNIA MODEL, EPA MODEL AND EMPIRICAL MODEL

         The EPA HIWAY Model, the California Line Source Model and the Empirical
Model will be evaluated using a hypothetical 2 lane highway with a peak hour traffic
volume is 2,000 vehicles.  The meteorological conditions used are a 6m/sec wind
approaching the highway 22*5° adjacent to the road with a stability classification
of D.

         The buffer of trees used to demonstrate their effectiveness in removing
carbon monoxide from the atmosphere will start 10 meters from the highway shoulder
and continue to a depth of 100 meters.  The receptor will be located 110 meters from
the shoulder of the highway.

         For the sake of analysis, the make-up of the buffer will consist of 344
deciduous (oak, maple, poplar, birch,linden) and 700 pine trees for every hectare.
The absorptive capacity of such a planting for carbon monoxide has been determined to
be 6.328 x 10~6 gr/sec-m2 vegetation.

         As the plume leaves the highway, part of the plume will escape the influence
of the buffer and the remainder of the plume will be trapped by the buffer.  To
calculate the fraction of the pollution captured by the buffer, the equation (23) and
the following data will be used.
                      L  = 10m       H = 6m       T_ = 7m
                       o                           z
                                       VI-15

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         By dividing the areas of the two trapazoidal areas between the mixing cell
and the buffer, the fraction of entrapment can be calculated.
                                   10m x 4m + h x 10m2 x 2m     _50_  _
         Fraction of entrapment =  i0m x 4m + J* x 10m  x 3m  "  55

         For these specific meterological conditions, approximately 91% of the
pollution being emitted by the highway is being entrapped by the buffer.

         Once part of the plume reaches the buffer, the trees start to absorb
the carbon monoxide at a hypothetical rate of SLA.  For this buffer arrangement
(S) has a value of 6.328 x 10~6 gr/sec-m2.  The buffer depth (L) is 100m and the
Canopy Area Index has a value of 1.5 m2/m2.  Combining these three parameters yields
a value for SLA of 9.49 x 10"^ gr/m-sec.

         As previously mentioned the example highway is carrying 2000 vehicles/hour
and if each car is emitting 42.8 gr/veh-km, the highway emission rate, Qi, will be
0.024 gr/m-sec. Since the Q,, SLA, and the fraction of entrapment have been calculated,
the emission rate after the buffer (0.2) can be calculated.

                               Q2 =  .910.J - SLA                     (24)

         Substituting previously defined values of Q]_, SLA, 0.2 can be calculated
to be:
                       Q2  =  .91 (.024) - 9.49 x  10~4 gr/m-sec
                       Q-  =  .0209  gr/m-sec

         To summarize,the following  parameters have been defined for the
hypothetical situation:

  U  =  6m/sec            QL  =  .024 gr/m-sec.        SLA  = 9.49 x 10~4 gr/m-sec
  (ft  =  22*5°              Q2  =  -0209  gr/m-sec.

          1.    Solution  of California Line  Source Model.

               By determining the vertical  dispersion coefficient  (QZ)  at .11 km normal
    the road to be 13 m,  the concentration of carbon monoxide for  a bare road side can
 to
                                       VI-16

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be calculated by using equation ( 14 ) .

                          C  =1.06 Qj  (4)
                                           >

                                           <*>
                               4.24 U sin 4> az
                                                 804.
                               4.24 (6)(.382)(13)

              If Q2 is substituted for Qj, the concentration 100m deep in the
buffer can be calculated.

                         C  =  1.06 Q2 4
                               4.24 u sin <>TZ
                            =  1.06 (.0209)(4)
                               4.24 (6)(.382)(13)

              As can be noted, a significant hypothetical reduction can be accomplished
by 100 meters buffer.

         2.   Solution of EPA HIWAY Model.

              The EPA HIWAY Model was graphically solved for the proposed hypothetical
situation.  The resultant concentration for an unforested highway is 4000 ugr/m3
where a forrested highway yields 3483 Mg/m3.

              Similar answers could be achieved through the numerical integration
of the EPA HIWAY equations presented in Section I of this Appendix A.

         3.   Solution of Empirical Model.

              By applying the values of Qp U and 6 to equation (21),the concentration
110 metiers (x) from non buffered highway can be calculated,

                          C  =8.18 Qj
                               U (x/sln 9)1'106
                          C  • 8.18 (.024), ._,     _..     . 3
                               emo/.zss)1-106   ' 344  M8/m

                                     VI-17

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              For a buffered highway, the value of Cv is substituted for Qj which
yields,
                                  C  =8.18 Q,
                                       „ ,  . L. ax 1.106
                                       U (x/sin8)
                                  C  = 8.18(.Q209) = 39  g/m3
                                       6(1107.283)1.106

         4.   Solution of SRI Street Canyon Model.

              Instead of the open highway, the SRI Street Canyon Model is applicable
to a street surrounded by tall buildings.  The tree configuration is also
different  for this model.  There will be a tree every 30 feet on each side of  the
highway.  If 20 ft. maples were used with a canopy area of 7.1 m2/tree, the
applicable sink rate(s) could be calculated;
          S  =  Sink rate x canopy area/tree x I/distance between  trees      (25  )
          S  =  6.328 x 10-6_gr     x 7.1 m2   x tree    =  2 4fi x 1Q-6
                            sec mz     tree      4.57m        '          T-—
                                                                        S6C in
              The configuration of the street canyon is shown  in  Figure VI-2.
The dimensions of the canyon are chosen to be Z =  1m, Lo =  2m, W  =  15m, X = 5m,
H = 10m. When these dimensions and the data from the previous example  are  entered
into equations (17 ) and  (  18) the leeward and windward concentrations can be
calculated for an unplanted street.

                   AC leeward  =  7 Q
                                  (U +.5)((X* + Z2)** + L0>

                               =  7 (.024)            =
                                                2)
                    AC windward  =  7  Q  (H-Z)
                                  W (U+.5)H
                                  7 (.024) (9)
                                                    1550.7 pg/tn3
                                       VI-18

-------
              The concentrations for a planted street can be determined by subtracting
S from Qjto determine a new emission rate.  Subsequently the revised emission rate
Q2 equal .02399  g/m sec.  By substituting this revised value into equations ( 1?)
and (18) the leeward and windward concentrations can be calculated to be:
                  AC  leeward  =  7
                                  (U +.5)((X2 +Z*)  +L0)
                  AC windward   =  7 Q (H-Z)
                                   W (U +.5) H

                                   7 (.02399)(9)
                                   (15)(6.5)(10)
                                   VI-19

-------
      APPENDIX B
SENSITIVE SPECIES LIST
         VI-20

-------
The Plant Species Sensitivity Lists contained in Volume I have been duplicated and
placed in this Appendix for convenience.  Both the Table and Page numbers which
appear in Volume I have been changed, where appropriate, to follow the numerical
order of this Volume.  Numbers in the Reference column of this list refer to the
literature citations listed in Volume I.
                                      VI-21

-------
                                 TABLE VI-1

                       PLANT SPECIES SENSITIVITY LISTS
 Fluorine
 TOLERANT -  Trees/Deciduous
                                                         Reference

 Apple Malus sp.                                           733
 American elm   Ulrnus americana                            1164,  536
 American linden  (Basswood)  Tilia americana              1164,  536
 American mountain ash  Sorbus domestica                    536
 American sycamore  Platanus occidental-is                   733
 Basswood (American linden)  Tilia americana              1164,  536
 Cornelian cherry  Cornus mas                             1164,  536
 Cutleaf  birch  Betula pendula var. gracilis                536
 European black alder  Alnus glutinosa                      536,  1164
 European elder Sambucus nigra                             536
 European larch Larix decidua                            1687
 European mountain ash  Sorbus aucuparia                  1164,  536
 European red elder  Sambucus racemosa                      536
 Flowering dogwood  Cornus florida                          733
 Flowering plum Prunus cerasifera                        1164,  536
 Hackberry Celtis sp.                                      733
 Litte leaf linden   Tilia cordata                          536
 Modesto  ash  Fraxinus velutina                           1164,  536
 Norway maple  Acer platanoides                             733
 Oleaster (Russian Olive)  Eleagnus angustifolia            536
 Oriental  cherry  Prunus eerrulata                          536
 Pear  Pyrus conmunis                                     1164
 Russian  olive  (Oleaster)  Eleagnus angustifolia            536
 Sugar maple  Acer saccharum                              1164
 Tree of  heaven  AilantTms altissima                        536
 Willow  Salix sp.                                           536,  1164
 White birch  Betula alba                                   733
 White mulberry  Morus alba                                 733

 TOLERANT  - Trees/ Coniferous

 American  holly  Ilex opaca                                 733
 Austrian  pine  Pinus nigra                               1164
 Canadian  hemlock (Hemlock)  Tsuga canadensia               733
 Eastern  red cedar  Juniperus virginiana                    525
 Hemlock  (Canadian hemlock)  Tsuga canadensiB               733
 Juniper  Juniperus sp.                                    1164,  536
Magnolia  Magnolia sp.                                     733
Western hemlock  Tsuga heterophylla                      1687
White spruce Picea glauca                               1164,  536

 TOLERANT  - Shrubs

 Bridal wreath spirea  Spirea prunifolia                  1164
 Currant   Ribes sp.                                       1164
 Firethorn  Pyracantha sp.                                1164

 TOLERANT - Herbaceous

Alfalfa  Medicago  sativa                                    16
                                    VI-22

-------
 Fluorine (Con't)

 TOLERANT -  Herbaceous
                                                         Reference
 Apricot  - vine  Passiflora ep.                            886C
 Celery  Spermolepsis sp.                                   16
 Cotton  Gbssypiwn sp.                                     136, 16, 269
 Cucumber Sicyos sp.                                       16
 Eggplant Solarium melongena                                16
 Fescue  Festuca elatar                                    890N
 Geranium Geranium  sp.                                     16
 Gladiolus                                                 886C
 Grapevine   Vitis sp.                                      886C
 Kentucky bluegrass  Poo. pratensis                         890N
 Red Fescue  Festuca sp.                                   890N
 Sweet  clover  Melilotus sp.                                16
 Tobacco  Nicatiana  sp.                                     16

 INTERMEDIATE  - Trees/Deciduous

 Apple  Malus  sp.                                           16
 Black  locust  Robinia pseudoacacia                       1164, 536
 Black  walnut  Juglans nigra.                               536
 Cut leaf  birch  Betula pendula var. aracilis                 16
 English  oak   QuercuB rdbor                   m             536
 English  walnut (Persian walnut)  Juglana regia          1164, 536
 Eugene poplar Populus canadeneis var. jugenci            1164, 536
 European ash  FTOxinus excelsior                         1164, 536
 European beech  FaguB sylvatica                           536
 European filbert  Corylua avellana                        536
 European hornbeam   Carpinus "betulus                       536
 European white birch  Betula pendula.                     536
 Green  ash   Fraxinus pennsylvanica lanceolata             536, 1164
 Hedge maple   Acer ocanpestre                               536, 1164
 Japanese larch  Larix leptolepsis                        1074
 Little leaf linden  Tilia cordata                        1164, 536
 Lombardy poplar  Populue nigra var.  italiea             1164, 536
 Oriental cherry  Primus serrulata                        1164
 Oriental plane tree  Platanus orientalie                  536
Persian  walnut (English walnut)  Juglans regia          1164, 536
Quaking  aspen Pcpulus tremuloidea                        1164, 536
Red mulberry  Morus  rubra                                  536
 Serviceberry  Amelanchier canadensie                      1164
 Silver maple  Acer saecharinum                            1164, 536
 Smooth sumac  fihus   glabra                                 536
 Spanish  chestnut Castenea sativa                          536

 INTERMEDIATE - Trees/ Coniferous

Aborvitae   Thuja sp.                                      536, 1164
Austrian pine  Pinus nigra                                525
Douglas  fir   Pseudotsuga menziesii                       1074
English holly Hex  aquifolium                            1164, 536
Lodgepole pine  Pinus contarta                           1074
                                        VI-2 3

-------
 Fluorine (Con't)

INTERMEDIATE - Trees/ Coniferous
                                                         Reference
Noble fir  Abies procera                                 1074
Ponderosa pine  Pinus ponderosa                          1074
Spruce  Picea sp.                                        1074
Western hemlock  Tsuga heterbphylla                      1074
Western red cedar  Juniperus scopulorum                  1074
Western white pine   Pinus monticola                     1074
White fir  Abies concolor                                1074

INTERMEDIATE - Shrubs

Common lilac  Syringa vulgaris                           1164
Japanese yew  Taxus cuspidate.                            1164, 536
Rhododendron  Rhododendron sp.                            1164
Rose  Rosa sp.                                            1074, 1164, 16

INTERMEDIATE - Herbaceous

Buckwheat  Fagopyrum                                       16
Iris  Iris sp.                                              16

SENSITIVE - Trees/Deciduous

Apricot (Flowering apricot)  Primus armeniaca             536, 1&» ^&°
Box elder  Acer negundo                                   536, 1164
Bradshaw plum  Prunus domestica 'Bradshau'                536, 1164
Empress tree Paulownia tomentosa                         536
Flowering apricot (Apricot)  Prunus armeniaca             536, 16, 460
Hop hornbeam Carpinus betulus                             765
Italian prunes   Prunus sp.                                269
Japanese apricot  Prunus name                             363
Maple  Acer sp.                                           765
Moorhead apricot                                          363
Paulownia (Empress tree)  Paulownia tomentosa             536
Plum  Prunus sp.                                           16
Western larch  Larix occidentalie                         536

SENSITIVE - Trees/ Coniferous

Cascades fir  Abies amabilis                             1074
Colorado spruce  Picea pungens                           536,1164
Douglas fir  Pseudotsuga menziesii                       525, 536, 1074, 1164
                                                         1687
Eastern white pine  Pinus strobus                         536
Engelmann spruce  Picea engelmannii                      1687
Loblolly pine  Pinus  taeda                               1164, 536
Lodgepole pine  Pinus contorta                           536, 525
Noble fir  Abies procera                                  1687
Nordman's fir  Abies  nordmanniana                        1074, 1687
Norway spruce  Picea  abies                               1074, 1687
Ponderosa pine  Pinus ponderosa                           536
Scotch pine  Pinus sylvestris                             525, 1164, 536, 1074

                                     VI-24

-------
Flourine (Con't)


SENSITIVE - Trees/Evergreen
                                                         Reference
Serbian spruce  Pioea omorika                            1074, 1687
Silver fir Abies peotinata                               1687
White fir  Abies ooncolor                                1687

SENSITIVE - Shrubs

Blueberry Vaooiniwn sp.                                  1164
Common barberry Berberis vulgaris                         765
Dwarf alps honeysuckle Lonicera alpigena                  765
Dwarf mugo pine Pinus mugo mughus                         536
St. Johnswort Hypericum maculatum                        1010, 765
St. Johnswort Jupericum perforation                        765

SENSITIVE - Herbaceous

Amaranthus Amaranthus retroflexus                         765
Annual blue grass Poa annua                               765
Catchfly  Silene inflata                                  765
Colchis (Fall crocus) Colchicum autumale                  765
Common chickweed Stellaria media                          765
Corn  Zea mays                                             16
Fall crocus (Colchis) Colchicum autumale                  765
Gladiolus                                                 990, 363, 318, 886C,
                                                           16, 136, 269
Goosefoot Chenopodiim alba                                765
Goosefoot Chenopodiim murale                              765
Grape Vivis vinifera                                      765
Iris Iris sp.                                             990
Mustard  Sinapsis arvenis                                 765
Oat grass Arrhenatherum elatius                           765
Orchard grass Daatylis glomerata                          765
Oregan grape Vitis sp.                                    363
Tulip                                                     318
                                    VI-25

-------
                                 J/MJLfc Vl-Z

                       PLANT SPECIES SENSITIVITY LISTS
 General Pollution
 TOLERANT - Trees/Deciduous
Alder  Alnus sp.
Almond tree  Prunus amygdalus
American beech (Red beech)  Fagus grandifolia
Apple  Malus sp.
Ash  Fraxinus sp.
Balsam poplar  Populus balsamifera
Birch  Betula lento.
Box elder  Acer negundo

Canadian poplar (Carolina poplar)  Populus canadensis
Carolina poplar (Canadian poplar)  Populus canadensis
Cherry  Prunus sp.
Eastern poplar  Populus deltoides
Elder  Sarribucus sp.
Elm  Ulmus sp.
European mountain ash  Sorbus aucuparia
Flowering dogwood  Cornus florida
Gingko (Maidenhair tree)  Gingko biloba
Goat willow  Salix caprea
Hawthorn  Crataegus sp.
Honey locust  Gleditsia triacanthos
Japanese larch  Larix leptolepsis
Japanese pagoda tree  Sophora japonica
Juneberry  Amelcnchier sp.
Larch  Larix sp.
London plane tree  Platanus acerifolia
Maidenhair tree (Gingko)  Gingko biloba
Oak  Quercus sp.
Oleaster (Russian olive)  Elaeagnus angustifolia
Ornamental apple   Malus floribunda
Peach  Prunus persica
Pear  Pyrus communis
Plum  Prunus sp.
Poplar  Populus sp.
Red ash  Fraxinus pennsylvanica
Red beech (American beech)  Fagus grandifolia
Rcdhaw hawthorn  Crataegus mollis
Russian olive (Oleaster)  Elaeagnus angustifolia
Scarlet elder  Sarribucus pubens
Silverberry  Elaeagnus  commutata.
Tree of heaven  Ailanthus altissima

TOLERANT - Trees/ Coniferous

Arborvitae  Thuja sp.
Austrian pine  Pinus nigra
Cedar (Eastern red cedar) Juniperus virginiana
Colorado spruce  Picea pungens
Eastern red cedar (Cedar) Juniperus virginiana
Eastern white pine  Pinus strobus
Sitka spruce  Picea sitchensis
Western red cedar  Thuja plicata
                                                         Reference
  39,
 407
  39
 787
 890Q,
 890 J,
 889 A,
 886K,
 890L,
 890L
 890L
 890Q,
 886N
 890Q
 886K,
 890Q
 890Q
1358
 890L
 889B
1976
 787
1976
8900
1400
1976
1358
 889A
 886K,
 890Q
 407
 809Q
 407
 889A,
 890
  39
 890Q
 886K,
 889B,
 890L
1358
1400
 39
 886K, 889A
8861,8900,1400
890L.890J,
8861
 1501, 407


889A.890J.890Q
890J,890,889A
 890Q
890J.890.889A
 890L
 886N
  41, 787
 890Q
 886N, 787
 890Q
 889A
 787
 787, 890Q

-------
 General Pollution (Con't)

 TOLERANT - Shrubs
                                                         Reference
 Alder buckthorn  Rhamnus frangula                        8861
 Alpine currant  Ribes  sp.                                 890Q
 Blueberry  Vacciniion sp.                                  407
 Common lilac  Syringa  vulgaris                            886K
 Hedgerow rose   Rosa  sp.                                   890Q
 Lilac  Syringa  sp.                                        890Lf  890Q
 Mentor barberry  Berberis mentorensis                    1501, 8861,  890Q
 Spindletree Euonymus  sp.                                 890L
 Snowberry  Symphoricarpos albua                           890L
 Sweetbriar  Rosa  eglantaria                               890Q
 Tatarian honeysuckle  Lonicera tatarioa                   890L
 Viburnum Viburnum sp.                                    890Q

 TOLERANT -  Herbaceous

 Annual bluegrass  Poa  annua                               407
 Barley  Uordeum sp.                                       407
 Bean   Phaseolus                                          407
 Benoite  Geum   sp.                                        407
 Blanketflower Gaillardia sp.                             1513
 Cabbage Brassica  napolerassiaa                            407
 Cauliflower                                              407
 Chickweed   Cerastium triviale                              38
 Chrysanthemum   Chrysanthemum                              407
 Corn   Zea mays                                            407
 Dandelion   Taraxacum platicardum                           38
 Day lily   Hemerocallis  fulva                              38
 Hawksbeard  Crepis japanica                                38
 Onion   AlHum japonica                                    38
 Peas   7t0wa sp.                                           407
 Pepper                                                   407
 Pink satin  petunia   Petunia ep.                           797
 Potatoes  Solatium jarnesii                                 407
 Radish  Raphanus  sp.                                      407
 Rhubarb Rheum  rhaponticwn                                407
 Roth   Athyrium  nipponicum                                  38
 Siberian pea shrub                                        886K,  890
 Spurge  Euphorbia helioscopia                              38
 Spurge  Euphorbia sieboldiana                              38
 St. Johnswort   Hypericum sp.                              407
 Starwort  Stellaria media                                  38
 Strawberry  Fragaria sp.                                  407
 Tickseed  Coreopsis  tinotoria                              38
Wheat  Triticum  aestivum                                   407
Woodbine  Lonioera periclymenum                           890Q
Wormwood  Artemis vulgaris                                 38

 INTERMEDIATE -  Trees/Deciduous

 Alder   Alnus sp.                                          886C,  889A
                                        VI-27

-------
 General Pollution (Con't)

 INTERMEDIATE - Trees/Deciduous
                                                         Reference
 American linden (Basswood)  Tilia americana              886, 733
 Apple  Mains sp.                                         1332
 Apricot  Prunus armeniaca                                407
 Ash  Fraxinus bungeana                                    38
 Ash  Fraxinus longicuspis                                 38
 Aspen (Hybrid poplar)   Populus sp.                        886L, 890E, 886C
 Balsam poplar  Populus balsamifera                       890E, 886L
 Basswood (American linden) Tilia americana               886, 733
 Black poplar  Populus  nigra                              890E
 Box elder  Acer negundo                                  889A
 Canoe birch (White birch)  Betula papyrifera              886L, 890E
 Chestnut oak  Quercus  dentata                             38
 Chokecherry  Prunus virginiana                           733
 Elder  Sarribucus                                          886C
 Elm  Ulmus  sp.                                            889A
 English oak  Quercus robor                                886N
 European larch Larix  decidua                            787, 886
 Fig  Fious  carica                                         733
 Gladbearing oak Quercus glandbearing                      38, 886C
 Grapefruit   Citrus sp.                                    407
 Green ash  Fraxinus pennsylvanica var. lanceolata         890E
 Hawthorn Crataegus                                      886C, 733
 Hornbeam Carpinus sp.                                    886C
 Hybrid  poplar (Aspen)   Populus sp.                        886L, 890E,  886C
 Little  leaf linden  Tilia  oordata                        886N
 Lombardy poplar  Populus nigra var. italica               733
 Maple Acer sp.                                           889A
 Mountain ash Sorbus americana                           890E
 Mulberry Morus sp.                                       886C
 Norway maple Acer platanoides                           501
 Pubescent birch  Betula sp.                               886N
 Red ash   Fraxinus  pennsylvanica                          886N, 501,  890L
 Sawtooth  oak Quercus acuta                                38
 Silver maple Acer saccharinum                           501
 Tulip poplar (Yellow poplar)   Liriodendron tulipifeva     501
 Walnut   Juglans sp.                                       407
 White birch (Canoe birch) Betula papyrifera               886L, 890E
 Willow   Salix sp.                                          886C
 Yellow poplar  (Tulip poplar)  Liriodendron tulipifeva      501

 INTERMEDIATE -  Trees/Coniferous

 Arborvitae   Thuja  sp.                                     889A
 Canadian hemlock   Tsuga  canadensis                        787
 Colorado spruce  Picea pungens                            733
Eastern white pine  Pinus strobus                         886N, 787
 Engelmann's spruce  Picea engelmanni                     889A
 False cypress  Chameocyparis  sp.                          889A
 Fir  Abies  sp.                                            787
 Japanese  red pine  Pinus densiflora                        38
 Lodgepole pine  Pinus contorta                            889A


                                        VI-28

-------
 General Pollution (Con't)

 INTERMEDIATE -  Coniferous
 Norway pine (Red pine)  Pinus resinosa
 Pitch pine  Pinus rigida
 Red pine (Norway pine)  Pinus resinosa
 Serbian spruce  Picea omorika
Reference

 886N
 733
 886N
 889A
 INTERMEDIATE - Shrubs
 Common lilac  Syringa Vulgaris                           890J
 Filbert  Copylus sp.                                      890L
 Forsythia  Forsythia  intermedia                          733, 501
 Hedgerow rose  Rosa sp.                                    890E
 Japanese barberry  Berberis thunbergii                   890L
 Juniper   Juniperus sp.                                   889A
 Spirea   Spirea  sp.                                       733
 Tatarian honeysuckle   Lonicera tatarioa                  501, 890J
 Weigela  Weigela florida                                 501

 INTERMEDIATE - Herbaceous

 Ageratum  Eupatorium  coelestimm                         407
 Bean   Phaseolus  sp.                                       407
 Bluegrass  Poa matsumural                                 38
 Carnation  Dianthus sp.                                   407
 Celery  Spermolepsis  sp.                                  407
 Chrysanthenum  Chrysanthenum sp.                          407
 Common plantago   Plantago major                           38
 Cudweed   Gnaphalium multiceps                             38
 Daisy  fleabane   Erigeron strigosus                         38
 Endive  Cichorium endivia                                407
 Grape   Vitis vinifera                                     733
 Groundsel   Senecio nikoensis                              38
 Heat lettuce  Lactuca sp.                                 407
 Knotweed  Polygonum virginianum                           38
 Lucerne  Medicago sativa                                 407
Maidenhair  Adiantwn pedatum                              38
Nasturtium   (Yellow cress)   Nasturtium indicum            38
Oat  Danthonia sp.                                        407
Onion  Alliumsp.                                           407
Petunia  Petunia  sp.                                      407
Rape seed  (Turnip)  Brassica rapa                         407
Siberian pea tree                                         889A, 890J, 890L
Sorrel  Rwnex acetosa                                      38
Sudan  grasses                                             407
Sweet  coltsfoot  Petasites japonioa                        38
Turnip  (Rape seed)  Brassica rapa                         407
Violet  Viola sp.                                          38
Yellow cress (Nasturtium)  Nasturtium  indicum              38
Zinnias   Seliopsis elegans                               407
                                        VI-29

-------
 General  Pollution  {Con't)

 SENSITIVE - Trees/Deciduous
                                                        Reference
Alder  Alnus multinervis                                  38
Apple  (Siberian crabapple)  Mains baccata                886L,  311
Ash  Fraxinus sp.                                        889A
Beech  FagitS sp.                                         889A
Birch  Betula sp.                                        8861,  311, 425
Black  oak  Quercus velutina                              733
Box elder  Acer negicndo                                  890E
Buckeye  Aesculus turbinata                               38
Catalpa  Catalpa speciosa                                311, 425
Chestnut oak  Quercus prinus                             733
Chokecherry  Prunus virginiona                           733
Elm  Ulmus sp.                                           811, 425, 1501
Japanese maple  Acer paimatwn                             38, 425
Judas  tree  Cercis siliquastrum                         1501
Larch  Larix sp.                                         890K,  311, 38, 890E
Lichen                                                  1490
Linden  Tilia sp.                                        889A
Lombardy poplar  Populus nigravap.  italiaa              311, 425
Mahogany  Melia japonica                                  38
Mulberry  Moms microphylla                              311
Oak  Quercus sp.                                         425
Orange  Citrus sp.                                       727
Peach  Primus persica                                   1332, 733
Pear  Pyrus comtunis                                     311
Pumila Arborea (Turkestan elm)  Ulmts turkestanica       890E
Siberian crabapple (Apple)  Malus baccata                886L,  311
Tree of heaven   Ailanthus altissima                    1501
Turkestan elm (Pumila arborea)  Ulmus turkestanica       89°E
White oak   Quercus alba                                 733
White poplar  Populus alba                                38
Wild black cherry  Prunus serotina                      1332

SENSITIVE - Trees/ Coniferous

Austrian pine  Pinus nigra                               733
Colorado spruce  Picea pungens                           733
Douglas fir  Pseudotsuga menziesii                       425, 733
Eastern white pine  Pinus strobus                        733, 311
Fir  Abies sp.                                           890E»  886N>  886C»
                                                         889A
Norway spruce  Picea abies                               733
Ponderosa pine  Pinus ponderosa                          311
Scotch pine  Pinus sylvestris                            733, 886K, 890J,
                                                         787, 889A
Spruce  Picea sp.                                        425> 889A» 886N»
                                                          39, 890E
                                      VI-30

-------
 General Pollution (Con't)

 SENSITIVE - Shrubs
 Common lilac  Syringa vulgaris
 Oregon holly-grape  Mahonia aquifplium
 Yew  Taxus  sp.

 SENSITIVE - Herbaceous

 Aconite  Aconitum japonicum
 Agrimony  Agrimonia  pilosa
 Alfalfa  Medicago sativa
 Aster  Aster bigelobii
 Bachelor's button  Centaurea ayanus
 Barley  Hordewn vulgare
 Bean  Phaseolus vulgaris
 Bedstraw  Galiwn strigoswn
 Beet  Beta vulgaris
 Bindweed  Convolvulus arvensis
 Bluegrass  Poo. sp.
 Broccoli  Brassica oleraccea
 Brussel sprouts Brassica aleracea var. geimrifera
 Buckwheat  Fagopyrum sagittatum
 Careless  weed  Amaranthus palmeri
 Carrot  Daucus carota
 Catbriar  Smilax racemo&a
 Chickweed Stellaria  media
 Cinquefoil  Potentilla chinensis
 Clover  Melilotus sp.
 Clover  ,frifolium\ sp.
 Corn  Zea mays
 Cosmos  Cosmos bipinnatus
 Cotton  Gossypium sp.
 Curly clock Rumex crispus
 Endive  Cichorium endivia
 Fleabane  Erigeron canadensis
 Four o'clock  \Mirabilis\jalapa
 Galinsoga  Galinsoga parvifolia
 Goosefoot   Chenapodium album
 Green beans  Phaseolus sp.
 Gypsy petunia  Petunia sp.
 Horsetail  Equisetum arvense
 Huckleberry  Gaylussacia sp.
 Lettuce   Lactuca  sativa
 Lettuce,  prickly   Lactuca scariola
 Lima bean  Phaseolus limensis
Mallow  Malva parvifolia
Morning glory  Ipomoea purpurea
Mosses  Commelina sp.
Oat  Avena sativa
Okra  Hibiscus esculentus
Pea  Vigna sinensis
Peanut  Arachis sp.
Reference

 733
 733
 889A
  38
  38
 727, 311
 311
 311
 311
 311

 311, 407
 311
 886C
 311
 311
 311, 1332
 311
 311
 733
 407
  38
 311
 311
1332
 311
 311
 311
 311
 311
 311
 407
 407
 727
 797
  38
 733
 311
 311
 727
 311
 311
1490
 311
 311
 890K
 727
                                       V-I-31

-------
 General  Pollution (Con't)

 SENSITIVE -  Herbaceous
                                                         Reference
 Pear  tree                                                 889A
 Pepper bell,  chili   Capsicum prutescens                  311
 Pinto beans                                               727
 Plantain   Plantago major                                 311
 Pumpkin  Cucurbita pepo                                   311
 Radish  Raphanus  sativus                                 311,  407
 Ragweed  Ambrosia artemisifolia                           311
 Rape  seed  (Turnip) Brassica rapa                          311
 Rhubarb  Rheum rhaponticum                               311
 Rye   Secale cereale                                       311
 Solomon's  seal  Polygonatum latifolium                    38
 Sorrel   Rumex sp.                                        407
 Soybean  Glycine  max.                                     311,  727
 Spinach  Spinacia oleracea                                727,  311,  407
 Squash  Cucurbita maxima                                 311
 Sunflower  Helianthus                                      311
 Sweet corn                                               727
 Sweet potato   Ipamoea batatas                            311
 Swiss chard Beta vulgaris var. cicla                      311,  407
 Thistle  Cirsium  inconiptum                               38
 Tomato   Lycopersicium esculentum                        1332,  727
 Turnip (Rape  seed)  Brassica rapa                         311
 Velvet-weed   Gaura parvifolia                            311
Vervain  Verbena  canadensis                              311
 Violet  Viola sp.                                         311
 Wheat  Triticum sp.                                       311
 Wild potato   Solanum jamesii                            727
 Wood nettle Laportea bulbifera                             38
 Zinnia  Zinnia elegans                                    311
                                        VI-32-

-------
                                 TABLE  VIi3

                       PLANT SPECIES SENSITIVITY LISTS
 Hydrogen Chloride

 TOLERANT - Trees/deciduous
 Birch  Betula sp.
 Black Cherry  Prunus serotina
 Cherry  Prunus sp.
 English walnut (Persian walnut)   Juglans regia
 Maple  Acer sp.
 Oak  Quercus sp.
 Oleaster (Russian  olive)  Eleagnus  angustifolia
 Pear  Pyrus comrmaiis
 Persian walnut (English walnut)   Juglans regia
 Red oak  Quercus borealis
 Russian olive (Oleaster)  Eleagnus  angustifolia

 TOLERANT -  Trees£oniferous

 Arborvitae   Thuja sp.
 Austrian pine Pinus nigra
 Balsam fir   Abies balsamea
 Canadian hemlock  Tsuga aanadenaia
 Eastern  white pine   Pinus  strobus
 Jack  pine  Pinus banksiona
 Loblolly pine Pinus taeda
 Norway spruce Picea dbies
 Short  leaf  pine  Pinus  echinata

 TOLERANT -  Shrub

 Yew  Taxus  sp.

 TOLERANT -  Herbaceous

 Carrot   Daunts carota
 Grapevine   Vitis sp.

 INTERMEDIATE  - Trees/Deciduous

 Black  Cherry  Prunus  serotina
 Black  gum   Nyssa sylvatica

 INTERMEDIATE - Trees/ Coniferous

Jack Pine  Pinus banksiana
Short  leaf pine  Pinus  echinata

SENSITIVE - Trees/Deciduous

Apple  Mains sp.
Box Elder  Acer negundo
Cherry  Prunus sp.
Horsechestnut  Aesculus  hippoaastanum
Larch  Larix sp.
Reference

 536
 536
 886C
 886C
 536
 536
 536
 536
 886C
 536
 536
 536
 536, 1104
 536
 536
 536
 536
 536
 536
 536
 536
 187
 88 6 C
 536
 536
 536
 536
 536
 536
 536
 536
 536
                                       VI-33

-------
Hydrogen Chloride (Con't)

SENSITIVE - Trees/Deciduous
                                                         Reference
Pin oak  Quercus palustris                                536
Sassafras  Sassafras albi&um                             536
Sugar maple  Acer saccharum                               536
Sweetgum  Liquidambar styraciflua                         536
Tree of heaven  Ailanthus altissima                       536
                                      VI-34

-------
                                 TABLE vi-4
                       PLANT SPECIES SENSITIVITY LISTS

Nitrogen Dioxide

TOLERANT - Trees/Deciduous


Beech  Fagus sp.
Gingko  (Maidenhair tree)  Gingko biloba
Maidenhair tree (Gingko)  Gingko biloba
Oak  Quercus sp.

TOLERANT - Trees/Evergreen

Austrian pine  Pinus nigra

TOLERANT - Herbaceous

Cabbage  Brassiaa sp.
Gladiolus
Onion Allium sp.

INTERMEDIATE - Trees/Evergreen

European larch  Larix decidua

SENSITIVE - Trees/Deciduous

Apple  Malus sp.
Black locust  Pobinia pseudoaoaaia
European beech  Fagus sylvatioa
European hornbeam  Carpinus betulus
European red elder  Sambucus racemosa
Gingko (Maidenhair tree)  Gingko biloba
Japanese maple  Acer palmatum
Large leaf linden  Tilia grandiflora
Little leaf linden  Tilia cordata
Maidenhair tree (Gingko)  Gingko biloba
Norwary maple  Acer platanoides
Pear  Pyrus comnrunis

SENSITIVE - Trees/Evergreen

Austrian pine  Pinus nigra
Colorado spruce  Pioea pungena
Eastern white pine  Pinus strobus
White spruce  Picea glauoa

SENSITIVE - Shrubs

Dwarf raugo pine  Pinus mugo mughus

SENSITIVE - Herbaceous

Barley  Hordeum sp.
Begonia  Rumex sp.
Carrot  \paucus caroto.
Kidney beans  Phaseolus sp.
Reference

  16
  16
  16
  16
  16
  16
  16
  16
 536
 536
 536
 536
 536
 536
 536
 536
 536
 536
 536
 536
 536
 536
 536
 536
 536
 536
  16
  16
  16
  16
                                    VI-35

-------
Nitrogen Dioxide (Con't)

SENSITIVE - Herbaceous
                                                         Reference
Lettuce  Lactuca sp.                                      1849, 16
Red clover  Trifolium pretense                             16
Sweat peas  Lathyrus odoratus                              16
Tobacco  Niaotiana sp.                                     16
                                     VI-36

-------
                       PLANT SPECIES SENSITIVITY LISTS

 Ozone

 TOLERANT -  Trees/Deciduous
                                                         Reference
Acacia  Acacia sp.
Alder  Alnus  sp.                                         1164
American  sycamore  Platanus occidentalie                 1074, 1164, 990
Ash  Fraxinus sp.                                         181
Basswood  (Linden) Tilia sp.                              1137
Black walnut   Juglans nigra                              1164, 536
English oak   Quercus  robor                               536, 1164
European mountain ash  Sorbus aucupafia                   536
European white birch  Betula pendula                      536, 1164
Fig  Ficus carica                                         181
Flowering dogwood Cornus florida                          536, 1164
Giant sequoia  Sequoia gigantea                           536
Linden (Basswood)  Tilia sp.                             1137
Little leaf linden  Tilia  cordata                        1164
Maidenhair tree Gingko biloba                            181
Norway maple   Acer platanoides                            536, 1164
Plum  Prunus  sp.                                          181
Red maple  Acer rubrum                                    536, 1164
Red oak  Quercus borealis                                1164
Redwood  Sequoia sempervirens                             536
Shingle oak   Quercus imbricaria                           536. 1164
Sugar maple   Acer sacchanm                               536, 1137
Weeping willow Salix babylonica                         1164
White birch   Betula papyrifera                           1137

TOLERANT - Trees/ Coniferous

Arborvitae  Thuja sp.                                     774, 1164, 536
Balsam fir  Abies balsamea                               1137, 536, 1164, 774
Black hills spruce  Picea glauca densata                  774, 1164, 536, 1137
Colorado spruce Picea pungens                           1137, 536, 1164, 774
Digger pine  Pinus sabiniana                              536
Douglas fir  Pseudotsuga menziesii                        774, 1137, 536, 1164
Eastern red cedar  Juniperus virginiana                   181
Jack pine  Pinus banksiana                               1074
Norway pine (Red pine)  Pinus resinosa                   1137, 1164, 774, 536
Norway spruce  Picea abies                               1137, 774, 1164, 536
Red pine  (Norway pine)  Pinus resinosa                   1137, 1164, 774, 536
Singleleaf pinyon pine  Pinus monophylla                  536
Sugar pine  Pinus lambertiana                             536
Torrey pine  Pinus torreyana                              536
Virginia pine  Pinus virginiana                          1074
White fir  Abies concolor                                 774, 1164, 1137
White spruce  Picea glauca                                536, 1164

TOLERANT - Shrubs

Ivy  Hedera sp.                                           181

TOLERANT - Herbaceous

Bugleweed (Carpet bugle)  Ajuga sp.                       181

                                     VI-37

-------
 Ozone (Con't)

 TOLERANT - Herbaceous
                                                          Reference
 California poppy Esahscholtzia California                 181
 Carpet bugle  (Bugleweed)   Ajuga  sp.                       181
 Lady's slipper  Cypripedium sp.                            181
 Leadwort  Ceratostigma plwnbaginaides                      181
 Petunia  Petunia sp.                                      1015,  1074

 INTERMEDIATE - Trees/ Coniferous

 Big cone Douglas fir  Pseudotsuga macrocarpa               536
 Coulter pine  Pinus coulteri                               536
California:  Incense-cedar  Libocedrus decurrens            536
 White fir   Abies concolor                                  536

 SENSITIVE - Trees/Deciduous

 Alder  Alrcus sp.                                           536
 American elm  Ulmus americana                             1164
 American sycamore Platanus occidentalis                  1074
 Black locust  Robinia pseudoacacia                        1164,  536
 Boxelder  Acer negundo                                     536,  1164
 California sycamore  Platanus racemosa                    1074
 Catalpa Catalpa  speciosa                                 1164
 European larch Larix decidua                              990,  1164, 1137, 536
Gambel  oak  Quercus gambellii                             1164,  536
Green ash  Fraxinus pennsylvanica lanceolata               536,  1164
Honeylocust  Gleditsia triacanthos                        1164,  536
Hybrid  poplar  Populus sp.
Japanese larch  Larix leptolepsis                         1164,  536, 77
Judas tree   Cerois siliquastrum                            536
Little  leaf  linden  Tilia cordata                          536
Mapleleaf mulberry (White mulberry) Morus alba             536
Pin oak Quercus palustris                                 536,  1164
Quaking  aspen  Populus tremuloides                         536,  1164
Scarlet  oak  Quercus coccinea                             1164,  536
Siberian crab apple  Malus  baccata                         536,  1164
Silver maple  Acer saccharinum                             536,  1164
Sweetgum  Liquidambar styraoiflua                         1164,  536
Thornless honeylocust  Gleditsia triacanthos inermis      1074
Tulip poplar  (Yellow poplar)  Liriodendron tulipifera      990,1164,536,1074,1137
Weeping willow  Salix babylonica                           536
White ash  Fraxinus  americana                              990,1137,1074,536,1164
White mulberry (Mapleleaf mulberry) Morus alba             536
White oak  Quercus alba                                   1164,  536, 1137
Yellow poplar  (Tulip poplar)  Liriodendron  tulipifera      990,1164,536,1074,1137

SENSITIVE - Trees/ Coniferous

Austrian pine  Pinus nigra                                 1164,  536, 774, 1137
                                      VI-38

-------
 Ozone  (Con't)

 SENSITIVE - Trees/ Coniferous
                                                         Reference
Canadian hemlock  Tsuga canadensis                        536, 1137
Eastern white pine  Pinus strobus                         536, 774, 1137,  532
                                                          990, 1164
Jack pine  Pinus banksiana                                774, 536, 1164
Jeffery pine  Pinus jeffreyi                              536
Monterey pine  Pinus radiata                              536
Pitch pine  Pinus rigida                                 1164, 1135, 774,  536
Ponderosa pine  Pinus ponderosa                           536
Scotch pine  Pinus .sylvestris                             774, 536, 990
Virginia pine  Pinus virginiana                           536, 774, 1137

SENSITIVE - Shrubs

Bridal wreath spirea  Spirea pmmifolia                  1164
Camellia  Cornelia sp,                                       2
Common lilac  Syringa vulgaris                            990, 1164
Common privet  Ligustrum vulgare                         1164
Snowberry  Symphoricarpos aibus                           536

SENSITIVE - Herbaceous

Aster  Aster sp.                                           990
Sage  Salvia sp.                                           990
Tobacco  Nicotiana sp.                                     599
                                     VI-39

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                                 TABLE VI-6

                       PLANT SPECIES  SENSITIVITY LISTS

 Pan

 TOLERANT - Trees/Deciduous
                                                         Reference

 European larch  Larix  decidua                             536
 Japanese larch  Larix  leptolepsis                         536
 Sugar maple  Acer saccharum                               536

 TOLERANT - Trees/ Coniferous

 Austrian pine  Pinus nigra                                536
 Canadian hemlock  Tsuga canadensis                        536
 Colorado spruce  Picea pungens                            536
 Eastern white pine  Pinus strobus                         536
 Jack pine  Pinus banksiana                                536
 Pitch pine  Pinus rigida                                  536
 White spruce  Picea glauca                                536

 SENSITIVE - Trees/Deciduous

 Little leaf linden  Tilia cordata                ^        536
 Tulip poplar (Yellow poplar)  Liriodendron  tulipifera    536
 Yellow poplar (Tulip poplar)  Liriodendron  tulipifera    536

 SENSITIVE - Herbaceous

 Aster  Aster sp.                                          990
Chrysanthemum  Chrysanthemum sp.                          990
 Lettuce  Laotuca sp.                                     1849
 Petunia  Petunia sp.                                      990
 Primrose  Primula sp.                                     990
 Sage  Salvia sp.                                          990
 Snapdragon  Chaenorrhinum sp.                             990
                                     VI-40

-------
                                 TABLE  VI-7

                       PLANT SPECIES  SENSITIVITY LISTS
Particulates - Smoke

TOLERANT - Trees/Deciduous
                                                         Reference
American Elm  Ulmus americana                             547
European larch  Larix deaidua                            1604
Scarlet elder  Sambuaus pubens                           1390

TOLERANT - Shrub

Cranberry  Vacoinium sp.                                  187

TOLERANT - Herbaceous

Knotweed  Polygonum cilinode                             1390

INTERMEDIATE - Trees/Deciduous

Alder  Alnus sp.                                         1604
American beech  (Red beech) Fagus grandifolia            1604
American hornbeam  Carpinus oaroliniana                  1604
Birch Betula sp.                                         1604
English oak  Querous robor (formerly called penduaulata) 1604
Maple  Acer sp.                                           1604
Poplar  Populus sp.                                      1604
Raceme oak  Quercus racemosa                             1604
Red beech  (American beech) Fagus grandifolia            1604
Red oak  Quercus borealis                                1604
White alder  Alnus rhombifolia                           1604

INTERMEDIATE - Trees/ Coniferous

Austrian Pine  Pirate nigra                               1604
Eastern white pine  Pinus strobus                        1604
Scotch pine  Pinus sylvestris                            1604

SENSITIVE -Trees/Deciduous

Quaking aspen  Populus tremuloides                       1390
Single-seeded hawthome  Crataegus monogyna              1675

SENSITIVE - Trees/Coniferous

Black Spruce  Picea maricna                              1390
Eastern white pine  Pinus strobus                        1390
Fir  Abies sp.                                           1604
Norway spruce  Picea abies (exaelsa)                     1604
White spruce  Picea glauaa                               1390

SENSITIVE - Herbaceous

Annual bluegrass  Poa annua                               269
                                     VI-41

-------
                                 TABLE VI-8
                       PLANT SPECIES  SENSITIVITY LISTS
Sulfur Dioxide

TOLERANT - Trees/Deciduous
                                                        Reference

American sycamore  Platanus occidentalis                1164
Ash  Fraxinus sp.                                        88 6C
Basswood (Linden)  Tilia sp.                             369
Beech  Fagus sp.                                        1187, 886C
Birch  Betula sp.                                         64, 523, 1187
Black gum  Nyssa sylvatica                              1169, 536
Black locust  ftobinia pseudoaaacia                       536
Cottonwood (Eastern poplar)  Populus deltoides          1164, 536
Eastern poplar  (Cottonwood)  Populus deltoides          1164, 536
English oak  Quercus robor                              1164, 536
European ash  Fraxinus excelsior                         369
European beech  Fagus sylvatica                          536
European hornbeam  Carpinus betulus                      536
European mountain ash  Sorbus aucuparia                  369
Flowering dogwood  Cornus florida                       1164, 536
Gingko (Maidenhair tree) Gingko biloba                  1164, 369
Green ash  Fraxinus pemsylvanica lanceolata             536, 1164
Hedge maple  Acer campestre                              536, 1164
Hornbeam  Carpinus sp.                                  1187
Larch  Larix sp.                                          ^
Linden (Basswood)  Tilia sp.                             369
Maidenhair tree  (Gingko)  Gingko biloba                 1164, 369
Mountain maple  Acer spicatum                           i16^
Oak  Quercus sp.                                          **
Oriental plane  tree  Platanuo orientalis                1164
Persian walnut Juglans regia                             8®^C
Pin oak  Quercus palustris                              H64
Poplar  Populus sp.                                      369
Red berried elder  Sambucus pubescene                   1074
Red maple  Acer rubrum                                   536, 1164
Red oak  Quercus borealis                               1164, 44
Smooth elm  Ubnus glabra                                 369
Sourwood  Oxydendrum arboreum                            369
Sugar maple  Acer saccharum               _        H°4
Tulip poplar (Yellow poplar) Liriodendron ftulipif&ra      16, 1164,  369
White ash  Fraxinus americana              ~             138
Willow  Salix sp.
Yellow poplar (Tulip poplar)  Liriodendron tulipif era      16, Ho4,

TOLERANT - Trees/ Coniferous

Arborvitae  Thuja occidentalis                          1JJJ
Austrian pine  Pinus nigra                               525, 1164,  536
Canadian hemlock  Tsuga canadensis
English holly  Ilex aqui folium
Lawson false cypress  Chamaecyparis  lawsoniana
Spruce  Picea sp.
Western red cedar  Thuja plicata
White spruce  Picea glauca
                                       VI-42

-------
Sulfur Dioxide  (Con't)

TOLERANT - Shrubs
                                                        Reference
Dwarf mugo pine  Pinus mugo mughus                       536
Juniper  Juniperus sp.                                  1164, 536

TOLERANT - Herbaceous

Alfalfa  Medioago sativa                                 886C
Corn  Zea mays                                            16
Fringed bindweed  Polygonum cilinode                    1074
Galleta  Hilaria jamesii                                1365
Grama grass  Bouteloua barbata                          1365
Heliotrope  Heliotropium sp.                             886C
Meadow fescue  Festuca elatior                           136
Oats  Avena sp.                                          88^c
Orchard grass  Daatilus glomerada                        136
Primrose  Primula sp.                                    88&c
Sweetpea  Lathyrus odoratus                              886C
Woodwaxen                                                886c

INTERMEDIATE - Trees/Deciduous

Apple  Malus sp.                                          16
Apricot  Prunus armeniaca                                 16
Balsam poplar  Populus balsamifera                      116^» 536
Bigtooth aspen  Populus grandidentata                   116*
Norway maple  Acer platanoides                          1164

INTERMEDIATE - Trees/ Coniferous

Balsam fir  Abies balsamea                               536, 1164, 525
Douglas fir  Pseudotsuga menziesii                      1164, 525, 536
Lodgepole pine  Pinus cantorta                           536, 525
Scotch pine  Pinus sylvestris                           1164
Silver fir  Abies pectinata                              536

INTERMEDIATE - Shrubs

Rose  Rosa sp.                                            16

INTERMEDIATE - Herbaceous

Gladiolus                                                 Jj?
Cotton Gossypitan sp.                                      16
Iris  Iris sp.                                            *6

SENSITIVE - Trees/Deciduous

Alder  Alnus                                             JJ5, 732
American elm  Ulmus americana          ^                 1164
American sycamore  Platanus occidentalis                1164
Apple  Malus sp.
                                      Vl-43

-------
 Sultur  Dioxide

 SENSITIVE - Trees/Deciduous
                                                        Reference

 Aspen (Poplar) Populus sp.                               732,  1187
 Birch   Betula sp.                                       1164,  1119
 Blueberry elder  Scaribucus coerulea                       732
 Canoe birch (White birch)  Betula papyrifera             732
 Catalpa Catalpa speoiosa                               1164
 Cherry  Prunus sp.                                       732
 Chokecherry  Prunus virginiana                           938
 English walnut (Persian walnut)  Juglans regia          1164
 European mountain ash  Sorbus auouparia                  732,  1187
 Horse chestnut  Aesculus hippocastanum                    44
 Hornbeam  Carpinus sp.                                    44
 Larch   Larix sp.                                         732,  1164
 Lombardy poplar  Populus nigra  var.  italica             1164
 Maple   Acer sp.                                         1187
 Mazzard cherry  Prunus avium                             886C
 Mountain ash  Sorbus americana                          1164
 Mountain maple  Acer spicatum                             44
 Narrowleaf cottonwood  Populus angustifolia             1365
 Pear  Pyrus comnunis                                    1164
 Persian walnut (English walnut)  Juglans regia          1164
 Poplar  (Aspen)  Populus sp.                              732,  1187
 Quaking aspen  Populus tremuloides                      1164,  119
 Scarlet hawthorn  Crataegus oxyacantha                   990
 Serviceberry  Amelanchier sp.                           1164
 Texas mulberry  Morus microphylla                       1164
 Utah serviceberry  Amelanchier utahensis                1164
 White ash  Fraxinus americana                            773
 White birch (Canoe birch)  Betula papyrifera             732
 Willow  Salix sp.                                       1164,  732

 SENSITIVE - Trees/Coniferous

 Black spruce  Picea mariana                             1164
 Canadian hemlock  Tsuga canadensis                      1164
 Douglas fir  Pseudotsuga menziesii                       990
 Eastern white pine  Pinus strobus                        990,  1164, 1074,
                                                         563,732,773,119
 Engelman's spruce  Picea engelmannii                    1164
 Fir  Abies sp.                                           119
 Jack pine  Pinus banksiana                              1164
Mountain hemlock  Tsuga mertensiana                     1164
 Norway  pine (Red pine)  Pinus resinosa                    16
 Ponderosa pine  Pinus ponderosa                         1164,  1007
 Red pine (Norway pine)  Pinus resinosa                    16
 Scotch  pine  Pinus sylvestris                           1074,  525
 Sitka spruce  Picea sitchensis                           732
 Virginia pine  Pinus virginiana                          773
 Western red cedar  Thuja plicata                        1°74
 Western white pine  Pinus monticola                     1164
                                       VI-44

-------
 Sulfur Dioxide (Con't)

 SENSITIVE - Shrubs
                                                         Reference
 Mountain laurel  Kalmia latifolia                       1164
 Ninebark  Physocarpus oapitatus  .                       1164
 Snowberry  Symphoricarpos aerophilus                    1365
 Wild rose  Rosa uoodsii                                 1365

 SENSITIVE - Herbaceous

 Alfalfa  Medicago sativa                                 938, 732
 Begonia  Rumex venosus                                   990, 1009
 Buckwheat  Fagopyrum sp.                                  16
 Celery  Spermolepsis sp.                                  16
 Cotton Gossypiwn sp.                                      16
 Cucumber  Sicyos angulatus                                16
 Eggplant  Solarium melongena                               16
 Evening primrose  Oenothera sp.                         1365
 Geranium  Geranium                                        16
 Globe mallow  Sphaeralcea munroana                      1365
 Goosefoot  Chenopodiwn ofrenonti                        1365
 Grape  Vitis sp.                                          938
Hound's tongue  Cynoglossim officinale                   1365
 Hungarian brome  Bromus inpermis                         136
 Indian rice grass Oryzopsis  hymenoides                 1365
 Lettuce  Lactuaa sp.                                     1844
 Locoweed    Astragalus utdhensis                         1365
 Lucerne   Medicago sativa                               1007
 Petunia  Petunia sp.                                     1009
 Potato   Solarium -tuberosum                              1007
 Red  clover  Trifolium pratense                           136
 Scarlet Gilia  Cilia agregata                           1365
 Squash  Cucurbita sp.                                     938
 Sunflower  Helianthus sp.                                 886C
 Sweet clover  Melilotus sp.                               732, 16
 Tobacco  Niootiana sp.                                     16
Vervain  Verbena sp.                                       990
 Violet  Viola sp.                                         990
 Wheat Tritioum aestivum                                 1007
                                      VI-45

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                 APPENDIX C




CALCULATION OF LEAF AREAS FOR SELECTED TREES
                    VI-46

-------
A one hectare forested unit of open space ±e proposed in Volume III.  It was developed
in order to estimate the amount of pollutants removed from the air by the natural
elements of such a standardized forest.  The tree species composing this model
forest are red oak (Quereus robur), Norway maple (Acer platanoides"), linden (Tilia
cordata), poplar (Populus tpemula ), birch (Betula vewntcosa) and pine (Pinus sp.).
The estimated height and diameter of the canopy for each tree species at age eight
(that is, five years after planting three-year-old saplings) were used in calculating
the surface area for each tree species.  The two dimensions of height, and diameter
of the canopy, for each tree species, may be found on Table VI-9.

By knowing the diameter of the canopy of a tree, the canopy area or ground area
can be calculated.   For example, uncrowded red maple, six meters high, may have
a canopy diameter of three meters.  Next, it is assumed that the area of a circle,
having the diameter of three meters, adequately estimates the ground area covered
by that red maple.

                                  diameter  =  3
                                  radius    =  1.5

Therefore, the area of the circle =  r2  =  (1.5)2  = 7.1 m2 and the estimated ground
                          2
area of this maple =7.1 m .  The total surface area of the plant, however, is much
greater.  One method for calculating that plant surface area, for a particular tree,
is to use its ground area and also, the area index of the tree.  That index, is the
ratio of total plant surface area to ground area.  Monteith (1976) has developed
an area index for each of the deciduous tree species used in the model hectare.
From that paper, the area index for a seven meter high maple is 5.18.  However,
the height dimension for the maple growing in the model hectare is six meters.
Since the nature of an extrapolation from a seven meter tree to a six meter tree
in unknown, the area index we used is unchanged from the literature.  It is assumed
that the area index for the seven meter maple may be directly used to estimate the
area index for the six meter maple.  One advantage for not extrapoliating the area
index given by Monteith is that the calculations we derived can be more easily recon-
structed.  Once the ground area and area index ratio for the tree is known, the plant
surface area can be computed.
                                      VI-47

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                        ground area for maple  =  7.1 m^
                        area index for maple   =  5.18
                        area index   =   surface area/ground area
                        5.18         X
                                 7.1 m^
                        surface area of maple  =  36.8 nr

                                                              -2   i
In multiplying the weighted average sink rate (reported as ug m hr  )of a pollution
by vegetation,by the surface area of a tree, the result  is the amount of pollutant
removed by that tree during one hour.  For instance, the surface area of a maple
as been calculated as 36.8 m2  and the weighted average sink rate for SO2
                         4     -2-1
by vegetation is 4.1 x 10  ug m- hr  . When these two values are multiplied, the
average amount of SO^ removed by a maple tree is 1.5 x 10^ ug/hr.

One problem with this procedure for determining the amount of pollutant removed
by a tree stems from the weighted average sink rate for that pollutant.  The
removal rates reported in the tables of Volume I were primarily obtained based
on studies of the rate of pollutant uptake by foliar material.   That is, the
pollutant removal rates by woody tissue were usually not considered during the
measurements of pollutant removal by vegetation.  As a result,  the weighted average
sink rate for a specific pollutant was primarily obtained from data based on foliar
uptake,exclusive of woody tissue uptake.

The area indices reported by Monteith (1976) involve both the foliage and woody
areas of the trees.  As a result, when the total surface area of a tree is calculated
by using the area index and ground area of the tree,  the woody surface area is
included in the total surface area of the tree.  When the latter value is multiplied
by the weighted average sink rate of the pollutant, in order to determine the
amount of pollutant removal by the tree, the calculation is generally lower than
if the surface area were all leaf.  The removal rate of the pollutant by the woody
surface area is assumed to be comparable to that by foliar surface area.  In truth,
the uptake rate of gaseous pollutants by the woody surface area  is apparently less
efficient than the removal rate by a comparable surface area of foliage.  The
opposite seems to be true when particulates are considered.  However, the removal
rates  for particulates by vegetation may have been primarily obtained from studies
                                     VI-48

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in which the entire plant was evaluated and as a result, the weighted average sink
rate for particulates may be more accurate than the other pollutant removal rates
since both the foiliage and woody areas are considered.  Therefore, when the total
surface area of a tree is multiplied by the weighted average sink rate for a
gaseous pollutant (which primarily defines the foliar uptake), the resulting amount
of pollutant removed from the air by the tree may be slightly off.  However, if one
considers the ratio of the total woody area indices of the five deciduous trees used
by Monteith (1976) to the total foliar area indices of the same five species, the
amount of woody surface area to that of the foliar surface area is relatively small
(0.08:1).  Because this ratio  is small, any error which it may cause is felt to also
be small.
                                     VI-49

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                                     TABLE VI- 9
              DATA CHARTS OF THE TREE.SPECIES USED IN THE MODEL HECTARE
  Maple (Acer platanoides )
     Height of the tree used in the model hectare
     Diameter of the canopy  of the 6.0 meter tree
     Canopy area or ground area of the 6.0 meter tree
     Height of the tree used in Monteith's area index
     Area index of the 7.0 meter tree
     Estimated plant surface area of the 6.0 meter tree
 6.0m
 3.0m
 7.1m2
 7.0m
 5.18m*
36.8m2
  Oak (Quercus robur}
     Height of the tree used in the model hectare
     Diameter of the canopy of the 6.0 meter tree
     Canopy area or ground area of the 6.0 meter tree
     Height of the tree used in Monteith's area index
     Area index of the 6.5 meter tree
     Estimated plant surface area of the 6 meter tree
 6.0m
 3.0m
 7.1m2
 6.5m
 5.08m**
36.1m2
  Poplar (Populus
     Height of the tree used in the model hectare
     Diameter of the canopy of the 6.0 meter tree
     Canopy area or ground area of the 6 meter tree
     Height of the tree used in Monteith's area index
     Area Index of the 10.5 meter tree
     Estimated plant surface area of the 6.0 meter tree
 6.0m
 3.0m
 7.1m2
10.5m
 7.4m***
52.5m2
  *The area index for the 7.0 meter maple is assumed to adequately estimate the
   actual area index of the 6.0 meter maple used in the model hectare.
 **The area index of the 6.5 meter oak is assumed to adequately estimate the actual
   area index of the 6.0 meter oak used in the model hectare.
***The area index of the 10.5 meter poplar is assumed to adequately estimate the
   actual area index of the 6.0 meter poplar used in the hectare.
                                       VI-50

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    Linden ( Tilia cordate)
       Height of the tree used in the model hectare
       Diameter of the canopy of the 5.0 meter tree
       Canopy area or ground area of the 5.0 meter tree
       Height of the tree used in Monteith's area index
       Area index of the 11.5 meter tree
       Estimated plant surface area of the 5.0 meter tree
 5.0ra
 2.4m
 4.5m2
11.5m
 5.1m*
23.0m2
    Birch (Betula verrueosa)
       Height of the tree used in the model hectare
       Diameter of the canopy of the 5.0 meter tree
       Canopy area or ground area of the 5.0 meter tree
       Height of the tree used in Monteith's area index
       Area index of the?.6 meter tree
       Estimated plant surface area of the 5.0 meter tree
    Pine (pinus sp. )
       Height of the tree used in the model hectare
       Diameter of the canopy of the 3.0 meter tree
       Canopy area or ground area of the 3.0 meter tree
       Leaf area index used by Rich (1970)
       Estimated woody area index
       Total estimated area index
       Estimated plant surface area of the 3.0 meter tree
 5.0m
 2.4m
 4.5m2
 7.6m
 6.04m**
27.2m2
 3.0m
 1.5m
 2.1m***
 0.2m****
 2.3m
 4.2m2
    *The area index of the 11.5 meter linden is assumed to adequately estimate the actual
     area index of the 5.0 meter linden used in the model hectare.
   **The area index of the 7.6 meter birch is assumed to adequately estimate the actual
     area index of the 5.0 meter birch used In the model hectare.
 *** The leaf area index used by Rich (1970) does not cite any height specification.
     As a result, it is assumed that the leaf area index does adequately define the ratio
     of leaf surface area to ground area of a 3.0 meter high pine.
**** The woody area index for the 3.0 meter high pine was estimated by comparing the
     surface area measurements of a 12 meter high white pine which were published by
     Stevens (1976).  He found that the foliage surface area of the pine was 15 x lO^cm2
     or 150m2 and the non-foliage or woody surface area was 15 x lO^cm2 or 15m2 (about
     10% of the foliage surface area).  In order to estimate the woody area index of
     the 3.0 meter pine, it was assumed that the woody surface area was 10% of the leaf
     surface area and this same percentage could be applied to determine the woody area
     index.
                                          VI-51

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          APPENDIX D
HOLLAND STACK RISE EQUATION
            VI-52

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The Holland stack rise equation is:
                   v  d                          AT
              AH = — - -  1.5  +  2.68 X 1(T3 p= - a
                     u                          Ls

where              AH  =  the rise of the plume above the stack  (meters)
                   v   =  stack gas velocity  (m/sec)
                    s
                    d  =  the inside stack diameter (meters)
                    u  =  wind speed (m/sec)
                    p  =  atmospheric pressure (mb)
                   Ts  =  stack gas temperature (°K)
                   AT  =  as in equation (1)  and
                          2.68 X 10" 3 is a constant having units of  (m"1 mb   )
                                     VI-53

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                                  TECHNICAL REPORT DATA
                           (Please read Instructions on the reverse before completing)
1  REPORT NO
                             2.
                                                          3 RECIPIENT'S ACCESSION-NO.
4 TITLE AND SUBTITLE
 Open Space as an Air Resource Management Measure -
 Design Criteria - Volume  II
                                       5 REPORT DATE
                                       December 1976
                                       6. PERFORMING ORGANIZATION CODE
7 AUTHOR(S)
 Robert S.  DeSanto, Richard A.  Glaser,  Joseph A. Miller
 William P. McMillan, Kenneth A.  MacGregor.	
                                       B. PERFORMING ORGANIZATION REPORT NO.

                                        H800-II
9 PERFORMING ORGANIZATION NAME AND ADDRESS
 COMSIS CORPORATION -  Environmental Services
 972 New London Turnpike
 Glastonbury, Connecticut  06033
                                                           10. PROGRAM ELEMENT NO.
                                       11 CONTRACT/GRANT NO.

                                        68-02-2350
12 SPONSORING AGENCY NAME AND ADDRESS
 Strategies and Air Standards Division Office of Air
 Quality Planning and  Standards Environmental
 Protection Agency
 Research Triangle Park. North Carolina    27711
                                       13 TYPE OF REPORT AND PERIOD COVERED

                                       TT-lnal	
                                       14. SPONSORING AGENCY CODE
15 SUPPLEMENTARY NOTES
16 ABSTRACT
This  report is a workbook which presents the primary biological and design features
which are crucial to the effective utilization of open space  to mitigate air
pollution.   It presents generalized schemes for the design and  location of buffer
strips and other forms of open  space.   It also illustrates air  pollution mitigation
by  open space by identifying  the mathematical procedures necessary in order to
permit incorporation of appropriate sink factors into four generally used carbon
monoxide diffusion models.
Directions and tables are given which may be used to estimate the air pollution
removal capacity of various  types of vegetation and open space.  Leaf area indices
are used in order to convert  canopy areas to total leaf areas and the associated
rates of pollution filtering  capacities by selected common  tree species.
17
                               KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
                                             b.lDENTIFIERS/OPEN ENDED TERMS  C.  COSATI Field/Group
Plants
Trees
Recreation Areas
Forests
Soils
Highways
Topographic Interactions
Air Resource Management
Open Space
Sanitary Zones
Air Pollutant Removal
Sinks
Highway Buffer  Strips
Greenbelts
18 DISTRIBUTION STATEMENT
                          19 SECURITY CLASS (ThisReport)
                             Unclassified
                                              20 SECURITY CLASS (THISpage)
                                                 Unclassified
                                                                        22. PRICE
EPA Form 2220-1 (9-73)

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