LENA VALLEY, 110HTANA,

AREA ENVIRONMENTAL POLLUTION STUDY


              SUMMARY
  Environmental Protection Agency
         Washington, D.C.

             June 1971

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U. S. ENVIRONMENTAL PROTECTION AGENCY

                                                 *t,.y-'

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HELENA VALLEY,
           ,  AREA
POLLUTION  STUDY
        ENVIRONMENTAL PROTECTION AGENCY
             Washington, D. C.
               June 1971

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                              PREFACE

     The Helena Valley,  Montana,  Area  Environmental  Pollution Study was
a cooperative undertaking between the  Federal  Government  and the State
of Montana.

     Because it had been alleged  that  pollutants  are contributing  to the
endangerment of health and welfare in  the  Helena  Valley,  this study was
undertaken to provide factual  information  bearing on the  allegations and
to aid in delineating the solution of  any  observed problem.

     The investigation concerned  contamination of the  environment  by
arsenic, cadmium, lead,  zinc,  and sulfur dioxide  from  the industrial
smelting complex in the  city of East Helena.

     Since the atmosphere was  suspected as being  the major pollutant-
transport mechanism in the area's environment, the National Air Pollution
Control Administration*  was designated to  lead and coordinate Federal
participation in the study.

     The study included  the investigation  of  in-plant  air quality
and lead accumulation in smelter  workers.   However,  since right-of-entry
to the plants was gained under Montana State  law, which prohibits  pub-
lication or public release of any information gathered during in-plant
surveys, such material is not included in  this report.  Results were
furnished to the Montana State Department  of  Health  for such use as it
may deem appropriate.

     For the purpose of  the Helena Valley, Montana,  Area  Environmental
Pollution Study, the findings  of  the many  individual investigations are
integrated and summarized in this report.   The remainder  of the report,
to be published as a companion document, provides baseline data and guidance
for future research activities.
 *Presently the Office of Air Programs of the Environmental  Protection Agency.

                                 Ill

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                      ACKNOWLEDGMENTS
     Mr.  Benjamin  F. Wake, Director, Division of Air Pollution,
State Department of Health, and Mr. Earl  V.  Porter, Director,
Region VIII,  Office of Air Programs, Environmental Protection
Agency, served as  the respective State and Federal Co-Directors
of the study.
     Mr.  Norman A. Huey, Assistant Director, Region VIII, Office of
Air Programs, Environmental Protection Agency, was principal technical
coordinator and editor for the study.
     Mr.  William H. Megonnell, Compliance Officer, Office of Air
Programs, Environmental  Protection Agency, assisted with the over-
all study direction and  report preparation.

     This document has  been compiled from technical  reports con-
tributed by authors affiliated with the Environmental  Protection
Agency, Food and Drug Administration, University of Montana, and
the U.S. Geological  Survey.   Principal authors are:   Mr. Francis  M.
Alpiser, Mr. Marius  J.  Gedgaudas,  Dr. C. C.  Gordon,  Dr. Douglas I.
Hammer, Dr.  Ibrahim J.  Hindawi,  Mr. Norman A. Huey,  Mr. Paul A.
Humphrey, Dr. Trent R.  Lewis, Mr.  A. T. Miesch, Dr.  Samuel  I.  Shibko,
and Mr. Albert V. Soukup.
                                iv

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                              CONTENTS

RESULTS AND RECOMMENDATIONS	.'	   1
INTRODUCTION	   3
    BACKGROUND INFORMATION	   7
        History 	   7
        Topography.	   7
        Climatology  	   8
        Population Statistics  	   9
        Employment	   9
        Industry	   9
        Agricultural  Activity  	   10
        Property Evaluation  	   10
    REVIEW OF PREVIOUS  POLLUTION STUDIES	11
        A Study of Air  Pollution in Montana, July 1961 to July 1962 ..   11
        A Study of Air  Pollution in the Helena - East Helena
          Area, October 1965 to October  1968	11
        Pollution Study in East Helena,  December 1968   	   12
ENVIRONMENTAL EVALUATION  	   13
    SULFUR DIOXIDE	13
        Annual Mean  Concentrations	13
        Daily Concentrations	14
        Hourly Concentrations  	   14
        Maximum Concentrations	15
    ARSENIC	15
        Contamination of Air	16
        Contamination of Water	16
        Contamination of Soil	16
    CADMIUM	17
        Contamination of Air	17
        Contamination of Water  	   18
        Contamination of Soil	• •   I8
    LEAD	i	19
        Contamination of Air  	  19

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        Contamination of Water	20
        Contamination of Soil	20
    ZINC	21.
        Contamination of Air	21
        Contamination of Water	21
        Contamination of Soil	22
EVALUATION OF POLLUTANT EFFECTS 	   23
    VEGETATION	   23
        Damage from Sulfur Dioxide	   23
        Arsenic Contamination 	   23
        Cadmium Contamination 	   24
        Lead Contamination	   24
        Zinc Contamination	   24
    ANIMALS	   24
        Acute Effects on Health	   25
        Heavy-Metal Accumulation In Hair	   25
        Heavy-Metal Accumulation in Organs	   25
        Heavy-Metal Accumulation in Animal Foodstuffs 	   26
    HUMANS	 .   26
        Heavy-Metal Accumulation in Hair	   26
        Body Burden	   26
POLLUTANT SOURCES  	   29
    SULFUR DIOXIDE EMISSIONS	   30
        Lead Smelter	   31
        Zinc Recovery Plant	   32
        Source-Receptor Relationships 	   32
    PARTICULATE EMISSIONS 	   33
    LEAD SMELTER	   33
        Zinc Recovery Plant	   34
        Source-Receptor Relationships 	    34
    WASTE WATER EMISSIONS	    34
        Lead Smelter	    34
        Zinc Oxide Plant	    35
    SOLID WASTE DISPOSAL  	    35
        Lead Smelter	    35
        Z1nc Oxide Plant	    35

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     HELENA  VALLEY, MONTANA,  AREA

    ENVIRONMENTAL POLLUTION STUDY


            RESULTS AND  RECOMMENDATIONS

    Atmospheric concentrations  of sulfur dioxide in the Helena
Valley exceed Montana air quality standards and levels reported  in
Federal criteria to be associated with deleterious effects on human
health, vegetation, and materials.   Industrial operations of American
Smelting and Refining Company and Anaconda Company in  East Helena
are the responsible sources.

    Air, water, and soil in the Valley are contaminated with heavy
metals from the East Helena smelting complex.  Water in Prickly
Pear Creek is contaminated by the American Smelting and Refining
Company plant.  Arsenic, cadmium, and lead, which are  emitted as
air pollutants from both plants, settle and accumulate in soil
and on vegetation to an extent surpassing levels that  are toxic  to
grazing farm animals.  Furthermore, evidence indicates that sub-
clinical effects could be occurring  in humans.

    Threshold-limit values have been established for  industrial
exposure of healthy adults for 8 hours per day, 40 hours per week,
during a normal working life; knowledge is insufficient, however,
to establish limits below which  heavy metals may be considered harm-
less to humans in various states of  health who are exposed to heavy
metal contamination from birth or, through parental contact with
heavy metals in the environment, even before birth. Calculations
of total body burden of lead and cadmium from air, food, and drink,
plus evidence of heavy-metal accumulation in human hair, are
sufficient cause for concern and action to control pollution
from the smelting complex in East Helena.
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     Heavy-metal particulates are not prone to  significant  dispersion,
and tall stacks will not change the impact of these particles  on  the
Helena Valley.   Increasing the height of emissions  is  not emission
control, in that it removes no pollution; tall  stacks  merely spread
gaseous pollutants and fine particles for wider consumption.

       Industrial sources should abate emissions to the lowest practicable
  levels by application of modern technology.


      Residents of Helena Valley should be informed of possible toxic
  effects from consumption of vegetables or other food items that might
  be contaminated either from the soil or from dustfall.   All locally
  grown vegetables should be washed to remove surface contamination
  before consumption.

       Ranchers  within about  5 miles  of  the smelting complex should
  be advfsed of  the  danger  to  low-grazing  farm animals like  horses  and
  sheep.  Such animals should  not graze  in fields 1n the  vicinity of
  East Helena.

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                        INTRODUCTION

     In 1888 the Helena &  Livingston  lead  smelter was built at East

Helena.  The American  Smelting  and  Refining Company purchased this

operation in 1899.   Anaconda  Company,  in 1927, built a plant adjacent
to the lead smelter to recover  zinc from the latter's waste slag.
In 1955 The American Chemet Corporation constructed a nearby paint

pigment plant whose raw material  is zinc oxide from the Anaconda zinc

plant.

     As early as 1901, the American Smelting and Refining Company

began protecting itself against claims for damages to the neighboring

premises with indentures releasing  them from such claims.

     Lead contamination of the  soil has been acknowledged by the
management of American Smelting and Refining Company, as stated by
this quotation from a  1963 letter sent to  a neighboring rancher

by the plant manager:

    I have finally received  the results of the soil samples
    and must report that your soil  is highly contaminated with
    lead.  Following are comments on  the  samples:

    Under some circumstances, it  is risky  to pasture horses
    op land, the surface portions of  the  soil of which contain
    oVer 200 parts per million  of lead.  This risk is great
    when grass is grown in soil with  a content of 1000 ppm
    lead.  During the  times  the grass is  lush and the animals
    can graze in the pasture  without  cropping low, or without
    picking up some soil,  I  should  say the danger would be
    minimized.

    I cannot imagine a very  luxuriant growth of vegetation
    in a pasture which contains such  high  concentrations of
    metals unless the  soil is quite calcareous.  Certainly,  in
    this particular area,  it would  not be "up  to the stirrups"
    of an ordinary size horse.  My  advice, therefore, is that
    you discour§ge the use of this  pasture for animals, especially
    for horses.

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     Contamination of the air with sulfur dioxide  also  was  acknow-
ledged by letter from management to a neighboring  rancher:
    During the spring of 1967 and the spring  and summer
    of 1968, your property south of the smelter has  experienced
    considerable exposure to S02.  Under the  present state  of
    knowledge, it is not likely that the condition can  be im-
    proved for a matter of years.
    Because of this unfortunate situation, it would  appear
    advantageous to all concerned if you were to move out of that
    location.  Possibly you can find another  location in the
    countryside and your house could be moved there.
    Please let me know if you are interested  so that we can
    negotiate terms of sale.

     An allegation of heavy-metal contamination of garden vegetables
was brought to the attention of the Food and  Drug  Administration's
Regional Inspector in Helena on September 20, 1968.   This information
was relayed from the Food and Drug Administration  to the Consumer
Protection and Environmental Health Service.   Discussions between
Montana Health Officials and Consumer Protection  and Environmental
Health Service led to an environmental pollution  study of the Helena
Valley, Montana, area.
     In May 1969, the Memorandum of Agreement on the following page
was signed by Federal and state officials.

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                   MEMORANDUM OF AGREEMENT

                           BETWEEN

             THE MONTANA STATE DEPARTMENT OF  HEALTH

                             AND

       THE NATIONAL AIR POLLUTION CONTROL ADMINISTRATION

                THE FOOD AND DRUG ADMINISTRATION

           THE ENVIRONMENTAL CONTROL ADMINISTRATION

     (CONSUMER PROTECTION AND ENVIRONMENTAL HEALTH SERVICE,

                      PUBLIC HEALTH SERVICE,

      U. S. DEPARTMENT OF HEALTH, EDUCATION,  AND  WELFARE)
Authority;  Under provisions of Section 301  of the Public Health
Service Act, as amended (Public Law 78-410), and Section 103 (a)
(3) of the Clean Air Act, as amended {Public Law 90-148), the
National Air Pollution Control Administration, the Food and Drug
Administration, and the Environmental  Control Administration of
the Consumer Protection and Environmental  Health Service, Public
Health Service, U. S. Department of Health,  Education, and Welfare,
and the Montana State Department of Health agree to cooperate in
the conduct of a study of environmental pollution as enumerated
in the terms of this memorandum.

Title of Project:  Helena Valley, Montana, Area Environmental
Pollution Study.

Purpose of Project;  To conduct a study of the types, amounts,
sources, distribution and effects of environmental pollution in the
Helena Valley, Montana area, with a view to recommending solutions
of any problems that are found.

Need for Project:' It has been alleged that pollutants arising from
man's activities in the area are contributing to health and welfare
endangerment.  This study will provide factual information bearing
on the allegations and aid in delineating solution of any observed
problem.

Location of Project:  Helena Valley, Montana; specific geographical
boundaries to be determined during field work.

Direction of the Study:  Administrative co-direction of the study
shall be the responsibility of Mr. Benjamin F. Wake for the State
of Montana, and Mr. Earl V. Porter for the Federal government.

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    Arrangements  for  and coordination of participation by State and
    Federal  agencies  not parties to  this agreement shall be the respon-
    sibility of the respective co-directors.  Technical direction of
    each  party's  personnel  shall be  by  the designee of each individual
    agency.


    Duration of Federal Participation:  Approximately six months' field
    work, plus such time as necessary for data analysis and report
    'preparation,  unless extension of the study is agreed to by the
    parties  concerned.


    Sharing  of Data:   Data  gathered  during the study, because of its
    possible research value, shall be freely  accessible to all partici-
    pating agencies.   However, data  especially created by the activities
    of this  study, prior to submittal of the  final report, shall be
    released only after consultation with the Montana State Department
    of Health.


    Final Report: A  report of findings and recommendations will be
    prepared by  the Federal participants,  in  consultation with the Montana
    State Department  of Health,  Any of the parties  to this agreement
    may disseminate copies  of the final report in accordance with  their
    regulations  and normal  procedures.


    Special  Provisions;  Details  concerning conduct  of various
    phases of the study and the  roles of  individual  agency participants
    will  be  developed jointly by  the Federal  and State parties to  this
    agreement and will be  appended,  as  developed, to become parts  of
    this agreement.
     Investigations for this study were conducted between July 1969

and July 1970.

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BACKGROUND INFORMATION
History
    In 1864, four prospectors in the  hostile  reaches of Montana
Territory came upon a gulch that they considered to be their "last
chance" in their search for gold.   Gold  was found  in such abundance
that a city sprang into existence.  Within 1  year  this mining
community numbered over 100 cabins  and was known as "Last Chance."
The main street, running north and  south through the center of town,
became "Last Chance Gulch."

    In 1882, shortly after the coming of the  railroads,  Helena  became
a corporate city with over 600 citizens  voting for a charter.

    With the enormous loads of gold being mined in the area,  Helena
was fast becoming  the banking capital of the territory.   The  city
soon enjoyed the reputation of being  the wealthiest city per capita
in the world.

    When Montana Territory was created by Congress in May 1864,
the city of Bannock was the seat of the  territory  legislature.   In 1865,
the capital was moved to Virginia City,  another booming miners'  town 200
miles to the south of Helena.  By 1875 Helena was  the uncontested center
of wealth and culture in the Montana  Territory.  Shortly  thereafter
Helena became the capital city.

    Prickly Pear Junction, a  "way station" on the stage  coach route
from  Ft. Benton to Helena  and other gold camps, became  East Helena
with  the building  of a  lead  smelter in  1888.    In 1899,  the American
Smelting and Refining Company purchased the old Helena  & Livingston
plant.   In  1927,   the Anaconda Company  installed a zinc  plant,  and
other industries  that use  smelter by-products  settled  in the vicinity.

Topography
    The  Helena  Valley in western Montana is an intermountajn valley
                                                                      .7

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bounded on the north and east by the  Big  Belt Mountains and on the
west and south by the main chain of the Continental  Divide.  The
valley is approximately 25 miles in width from  north to south, and
35 miles long from east to west.  The average height of surrounding
mountains above the valley floor (elevation  3700  feet) is  about 3000
feet.

    The city of Helena, with an average  elevation of 4100  feet, is
located on a slope at the south side  of  the  valley.   The southern
parts of the city have elevations of  about 4300 feet, and  the  northern
parts are at elevations of about 3800 feet.

    The city of East Helena is located about 4  miles east  of Helena
at an elevation of about 3900 feet.  The ground slope is much  less
evident in East Helena than it is in Helena.   The ground  south of
East Helena, where the smelting operations are  located,  is 30  to  50
feet higher than the city.

    The valley floor continues to slope gently  to the north and
northeast to Lake Helena, which is located about 10 miles  northeast
of East Helena.  Lake  Helena  is the lowest point in the valley with
an elevation of 3650 feet.

Climatology
     The climate of  the Helena Valley may  be described as modified
continental.

     As may  be  expected in  a  northern  latitude, cold waves may
occur  from  November through  February, with  temperatures occasionally
dropping  well  below zero.  Summertime temperatures  are moderate, with
maximum readings  generally under  90°  F and  very  seldom reaching 100°.

     Total  precipitation varies  widely throughout the valley, from a
semiarid  total  of 9 to 10 inches  in  the  drier  northern and eastern
portions  of the  valley,  to a subhumid 30 inches  along the Continental
 B

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Divide to the southwest.   Most of the precipitation  falls from April
through July from frequent showers or thundershowers, with  some Steady
rains in June, the wettest month of the year.   Late  summer,  fall, and
winter months are relatively dry.  Snow can  be  expected  from September
through May.  During the winter months snow  may remain on the ground
for several weeks at a time.  Amounts during the spring  and  fall are
usually light.

    Strong and persistent temperature inversions are common to the
Helena Valley.  The surrounding mountains shelter the area  from the
winds.  At night, cold air drains into the valley from the  surrounding
mountain slopes.

Population Statistics
    Population statistics for the Helena Valley can  be estimated
from Helena and East Helena statistics.  There  are 125 farms in the
valley.  These people may not be included in the city  statistics.
Table 1 gives population estimates for Helena and East Helena.
    Table  1.  ESTIMATED POPULATION OF HELENA AND EAST HELENA
           Year	Helena	East Helena
           1950               17,581               1,216
           1960               20,227               1,490
           1969	26.602	2.079

Employment
    The  largest  employer  in the  Helena Valley is the State of Montana.
Helena  is  the state capital.  Retail  trade and professional services
make  the greatest  remaining contribution to employment.

Industry
     Heavy  industrial  manufacturing companies have located within the
city  of  East  Helena.  American  Smelting and Refining Company operates
a  custom lead smelter that  employs 180 workers.  Anaconda Company

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 operates a zinc recovery  plant  that  employs 80 workers.  American
 Chemet manufactures  paint pigments and  employs 10 people.  Several
 miles southwest of the  city of  East  Helena, the Kaiser Cement and
 Gypsum Company operates a cement  plant  that employs 75 workers.

     About 20 light industrial manufacturing companies* in the city of
Helena employ about 400  people.

 Agricultural Activity
     There are approximately 220,000  acres  of agricultural land on
 the valley floor, valued  at about $10 million.

     Most farming in the valley  is by dry-land practices.  The soil
 is seeded 1 year, left  fallow the next, and seeded again the third
 year.  A total of 20,000  acres  of wheat and barley is planted each year.
 The yearly gross income is estimated to be $300,000 and $200,000 from
 wheat and barley, respectively.   Four thousand acres of alfalfa is
 grown on irrigated land with  the  estimated worth being about $2 million.
 Two hundred acres is planted  in either  corn, oats, or potatoes, with
 an approximate value of $9,000.   Three  thousand acres is used as
 seeded or improved pasture, and about 200,000 acres is used as range-
 land pasture.

     About 700 private gardens are planted  in the valley to produce
 tomatoes, beets, carrots, corn,  beans,  peas, onions, radishes, and
 cabbage.
     There are 15,000 cows and calves in the valley; their market value
 1s $3 million.  Also present  are  5,000  sheep and lambs, 5,000 chickens,
 1,000 hogs, and 800 horses,  the combined worth  of  which  is  estimated
 at more than $300,000.

 Property Evaluation
     Value of properties within  the Helena  Valley can be estimated
 from the biennial reports of  the State  Board of Equalization for
 Lewis and Clark County.

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          Table 2.  HELENA VALLEY  PROPERTY EVALUATION
                           (dollars)
Lewis and Clark County
Assessed valuation
Personal property
All real estate, including
improvements, town lots
Agricultural lands and
improvements
Grazing lands
All livestock
All timber
June 30, 1960
80,000,000
30,000,000
40,000,000
6,000,000
3.000,000
2,000,000
70,000
June 30, 1968
100,000,000
30,000,000
60,000,000
7,000,000
3,000,000
3,000,000
80,000
REVIEW  OF PREVIOUS POLLUTION STUDIES
A Study of Air Pollution in Montana, July 1961 to July  1962
    There was a study of air pollution conducted by  the Montana State
 Board  of Health from July 1961 to July 1962 with assistance  from  the
 Division of Air Pollution, Public Health Service, U.S. Department of
 Health,  Education, and Welfare.  Limited air quality measurements were
 made  in  seven Montana cities.

    Total suspended particulate loadings in the city of  Helena were
 reported to average 72 micrograms per cubic meter (ug/m^) of air.
 Arsenic, lead, and fluoride were reported to average 0.08, 0.34,
 and 0.10 ug/m » respectively.

 A Study of Air Pollution in the Helena -  East Helena Area,
 October 1965  to  October 1968
     Another study of air pollution,from October 1965 to  October 1968,
was conducted  by  the Montana  State Department of Health.   The objective
was to define  the  quantity and  quality of certain air pollutants in the
Helena - East  Helena area.

     Monthly average  sulfur  dioxide  (SOg) concentrations  up to 0.055 part
per million (ppm), hourly averages up to 0.4 ppm, and 5-minute average
concentrations up  to  6  ppm were reported.   Suspended particXilate loadings
averaged 76 pg/m3  in  East Helena and 50  to  60 pg/m3 at various sampling

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locations in Helena.   Arsenic  and  lead concentrations were higher in East
Helena than in Helena.   The  contribution of the smelter complex in East
Helena to air pollution was  demonstrated by the decline in sulfation,
dustfall, and lead content of  dustfall during a smelter strike.

    The  study recommendations called for reduction in sulfur dioxide
and dust emissions from the East Helena smelting  complex, prohibition
of open  burning, and elimination of street dust through paving.

Pollution Study in East  Helena, December 1968
     In December 1968,  a study of pollution in East Helena, financed by
the Montana State Board of Health, was conducted  by Dr. C. C.  Gordon,
Associate Professor of Botany, University of  Montana, Missoula, Montana.
The study objective was to determine the severity and extent of  sulfur
dioxide  damage to vegetation.  The study scope was extended  to include an
Investigation of the effects of lead and cadmium on the ecosystem.

     Dr.  Gordon reported that local farmers had stated that raising of
horses had not been  feasible  for  several decades.  American Smelting
and  Refining  Company plant  management reportedly has been of the opinion
 that residents of East Helena should not eat local garden vegetables
 because of metal  contamination.

     Sulfur dioxide effects  were found on pine seedlings  as  far as
 4 miles south of  the East Helena  smelter complex.  Elevated lead
 and cadmium levels were reported  in garden vegetables and in animal
 tissues.

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               ENVIRONMENTAL EVALUATION

    A1r, water, and soil were examined for contamination by arsenic,
cadmium, lead, and zinc.   In addition, airborne sulfur dioxide was
measured.

SULFUR DIOXIDE
    Sample averaging  time  is important in the evaluation of sulfur
dioxide pollution of  the air.  Unlike generalized air quality deterio*-
ration from myriad emission sources in urban areas, a single source
or a few sources  in close  proximity will cause a heterogeneous pollutant
distribution usually  characterized by infrequent but severe levels.
The Helena Valley is  subjected to this type of pollutant distribution,
as demonstrated  by the range in  annual, daily, hourly,  and 1-minute
average sulfur dioxide concentrations.

Annual  Mean Concentrations
    The Environmental Protection Agency's Office of Air Program's
best judgment of effects  that  occur when various levels of pollution are
reached  is reported in AP-50.  Air Quality Criteria for Sulfur
Oxides.  This document states  that:
    1.  At concentrations  of 0.04 ppm,  frequency of lung disease
        may increase and mortality  from bronchitis and lung cancer
        may occur.
    2.  At concentrations of 0.03 ppm,  chronic plant injury and
         excessive leaf drop may occur.
    3.   At concentrations of 0.12 ppm,  the  corrosion rate of steel
         may increase by 50 percent.

    The Montana  State Board of Health adopted 0.02 ppm sulfur dioxide
 maximum annual average as a state-wide ambient air quality standard
 on May 27,  1967.

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     The city of Helena  experienced  0.01  ppm from June 1969 to June
1970.  Residents of East Helena  were exposed to 0.0] to 0.08  ppm,
depending upon their location within the city.  Throughout most of
East Helena, levels varied between 0.02 to 0.04 ppm, but a small
center-city portion was  exposed  to levels between 0.04 and 0.08 ppm.
A 20-square-mile area adjacent to and southeast of  the city of East
Helena had levels greater than 0.02 but less than 0.04 ppm.   The
remainder of the Helena  Valley was not exposed to levels greater  than
the State standard of 0.02 ppm.

Daily Concentrations
    Air Quality Criteria for Sulfur Oxides states that:
    1.  At concentrations of 0.1 ppm, absenteeism from work  and
        .increased hospital admissions of older persons for
        respiratory disease may occur.
    2.  At concentrations of 0.2 to 0.3 ppm,  patients with chronic
        lung disease may experience accentuations of symptoms, and
        the general population may experience  increased  mortality.
    Montana's state-wide sulfur dioxide standard  is 0.10 ppm, 24-
hour average, not to be exceeded over 1 percent  of  the days  in any
3-month period.

    The concentration equaled or exceeded 0.1  ppm on 4  of the 129
days sampled  (3  percent) in Helena, on 5 of the 128 days sampled
(4 percent)  in East Helena, on  15 of the 136 days sampled (11 percent)
in the Helena Valley 0.5 mile southeast of the smelter,  and  on 10 of
the  123 days  sampled (8 percent) in the Helena Valley 2.5 miles
southeast of  the smelter.

     Concentrations  equaled or exceeded 0.2 ppm on 4 days 0.5 mile
southeast of  the smelter and on 1 day  at  2.5 miles southeast.

Hourly Concentrations
     Air Quality  Criteria for Sulfur Oxides reveals that at concentration?
of 0.10 ppm  sulfur  dioxide, in  the presence of particulates, visibility
 may be reduced to about 5 miles.
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    Montana's standard is 0.25 ppm, not to be exceeded  more than 1
hour in any 4 consecutive days.  In approximately 140 days  of sampling
1n the summer of 1969, 0.25 ppm was exceeded during 41  hours in  Helena,
47 hours in East Helena, 126 hours in the Helena Valley 0.5 mile
southeast of the smelter complex, and 74 hours in the Helena Valley
2.5 miles southeast of the smelter complex.

Maximum Concentrations
    While the effects of short-term peak concentrations are not
discussed in the Air Quality Criteria Document and  although limits
are not included in the Montana State standards, at concentrations
greater than 1 ppm the air usually is so fouled as to cause nausea  and
coughing in the normal population.  The taste threshold occurs at
0.3 ppm.

    The instruments used during the 140-day sampling period to measure
sulfur dioxide had an upper limit of detection of 4 ppm. The monitor
located in Helena registered greater than 1 but less than 2 ppm  for 48
minutes.  The monitor in the city of East Helena registered greater
than 2 but less than 4 ppm for a total of 41 minutes.  In the Valley
0.5 mile southeast of the smelter, a monitor registered greater  than
4 ppm for about 2 minutes.

ARSENIC
    Arsenic compounds are toxic to humans, animals, and plants.
Most arsenic compounds, when heated in air, are converted to arsenic
trioxide, a tasteless, toxic, white powder.  Arsenical  dusts can
produce dermatitis, bronchitis, and irritation to the upper respira-
tory tract.  Ingestion of arsenic can produce keratosis and cancer
of the skin.  The relationship of arsenic to other types of cancer,
particularly lung tumors, is strongly suggestive.  Herbivorous animals
have been poisoned from eating plants contaminated with arsenic.  Seventy
milligrams of arsenic trioxide has been reported as a fatal dose for
man.

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Contamination of Air
    Maximum permissible atmospheric concentrations have not been
adopted in the United States.  A  24-hour standard of 3 pg/m  has
been recommended in the U.S.S.R.  and Czechoslovakia.

    During the summer and fall of 1969, an average 24-hour concentra-
tion of 0.005 yg/m3 was found  in  Helena.  Maximum 24-hour concentrations
did not exceed 0.07 yg/m3.   East  Helena was exposed to an average of
0.08, although the maximum reached 0.3 pg/m3.  These values represent
the highest found in the Helena Valley.

    The concentration of arsenic  in the particulates that settle
in the vicinity of the East Helena smelter is  200 to 1000 ppm.  Each
month, 1 to 4 milligrams (mg)  of  arsenic settle  on each square meter
of surface area within a 1-mile radius of the  smelter.

Contamination  of Water
    Arsenic concentrations of 2 to 4 mg  per  liter are  reported not
to interfere with the self-purification  of streams.  The Montana
water quality criteria are consistent with the Public  Health  Service
Drinking Water  Standards that state  that the concentration of arsenic
in drinking water should not exceed  0.01 mg  per liter  and concen-
trations in excess of 0.05 mg per liter  are  grounds  for rejection of
the  supply.

     Sampling of waters in the Helena Valley  revealed arsenic  in  the
surface waters  in Prickly Pear Creek,  downstream from  the smelting
complex.  On October 25, 1969, and on April  4, 1970, the  surface water
in Prickly Pear Creek, which is 2.5 miles  northwest of East Helena,
contained 0.01  mg per  liter.  On  the same dates, Missouri River  water
at the  Helena City Water Plant intake contained 0.02 mg  per liter.

Contamination  of  Soil
     The arsenic content of  soils  ranges from 1 to 50 ppm and  averages
about 5 ppm.    The  soil outside,  but adjacent to, the Helena  Valley
contains  6 ppm.
16

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    The concentrations of arsenic  in the  soil  decrease with distance
from the smelting complex.  At distances  of 1  and  2 miles, respectively,
the upper inch of uncultivated soil  contains 140 and 23 ppm and the
upper 4-inch layer of cultivated soil contains 40  and  20  ppm.

CADMIUM
    Cadmium is recognized as an element with high  toxic potential.
Children have been made sick by consuming a frozen dessert containing
13 to 15 mg of cadmium per liter.

    Cadmium is absorbed without regard to the level of existing body
concentrations, which indicates a lack of homeostatic  mechanisms  for
the control of cadmium levels.  It has been reported that the  feeding
of 0.1 mg of cadmium per liter causes accumulation of  cadmium  in  the
liver and kidney tissues of rats.

    Epidemiological evidence associating  cadmium with  renal arterial
hypertension in humans is conflicting.

Contamination of Air
    When inhaled, cadmium can produce pulmonary emphysema and  bron-
chitis, kidney damage resulting in proteinuria, and  gastric and  intes-
tinal disorders.  In one epidemiological  study, air  cadmium levels
have been associated with cardiovascular mortality rates, but  this
relationship is very tenuous and has not been confirmed  in other  studies
to date.

    Maximum permissible atmospheric concentrations for cadmium have
not been suggested or adopted  in the United States.   In 1963,  the
National Air Sampling Network reported that the nation's  air contained
an average 24-hour concentration of 0.002
    The maximum reported individual annual concentration was 0.028
 vg/m3.  A maximum 24-hour concentration of 0.18 vg/m3 was reported in
 East St. Louis, Illinois.

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    During the summer and  fall  of  1969,  the city of Helena was
exposed to an average 24-hour concentration of 0.03 and a maximum
24-hour concentration of 0.11  ug/m3.  The  residents of East Helena,
depending upon their location within  the city, were exposed to an
average 24-hour concentration between 0.06 and 0.29 ug/m3 and to a
maximum 24-hour concentration of 0.7
    The concentration of cadmium in the particulate matter  that
settles in the vicinity of the East Helena smelter is  200 to  1000  ppm.
Each month, 1 to 4 rog of cadmium settles on each square meter of surface
area within a 1-mile radius of the smelter.

Contamination  of Water
    Recognition of the toxic potential of cadmium when it is  taken by
mouth is based on the occurrence of poisoning from cadmium-contaminated
food and beverages, epidemiologic evidence that cadmium may be asso-
ciated with renal arterial hypertension, and long-term oral toxicity
studies in animals.

    According to the Public Health Service Drinking  Water Standards,
a drinking water supply containing in excess of 0.01  mg cadmium  per
liter should be rejected.

    Water was sampled from Prickly Pear Creek (downstream of the
smelting complex) on July 1, 1969; October 25, 1969; and April 4,
1970.  The cadmium content was 0.006, 0.001, and 0.007 mg per liter,
respectively.  Limited sampling of other Helena Valley waters suggests
that  the concentration of cadmium generally is less  than 0.001 mg
per liter.

Contamination of Soil
    The expected  cadmium content  of  soils  is 0.5 ppm.  The concen-
tration in  the  soil  outside,  but  adjacent  to, the Helena Valley ranged
from  less  than  0.5  to  2  ppm.

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    The concentration of cadmium in the soil  of  the Helena Valley
decreases with distance from the smelter.  At a  distance of 1 , 2, and
4 miles, respectively, the upper inch of uncultivated soil contains 68,
17, and 4 ppm and the upper 4-inch layer of cultivated soil contains
21, 9, and 3 ppm.

LEAD
    Lead can be seriously injurious to health as a result of  accumu-
lations in the body.   Long-term daily intake  of  less than 0.6 mg
by healthy adults may cause small  increases in body burden, but no
clinical disease.  An intake in excess of 0.6 mg per day may  result
in the accumulation daring a lifetime of a dangerous quantity of lead
In the body.

Contamination  of Air
    Because maximum permissible atmospheric concentrations have not
been established in the United States, judgment  regarding the .
significance of lead contamination must be related to permissible
body burden.  Intake from the air can be approximated by assuming 20
percent retention of what is inhaled and a daily intake of 20 cubic
meters of air.

    During the summer and fall of 1969, the city of Helena was ex-
posed to an average daily concentration of 0.1 yg/m  , with maximum
daily concentrations up to 0.7 pg/m3.  The residents of East  Helena,
depending upon location within the city, were exposed to an average
daily concentration of 0.4 to 4 yg/m3, with maximum daily exposures
up to 15
    Daily respiratory intake in Helena is calculated to be 0.5 micro-
gram  (yg).  In East Helena, the daily respiratory intake varies from
2 to  20 yg, depending upon location within the city.

    Particles that settle from the air in the vicinity of the smelter

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contain 6,000 to 28,000 ppm.   Ingestion of 0.007 to 0.04 ounce of
these participates may exceed  the daily body-burden limit.

    Within a 1-mile radius  of  the East Helena smelter, 30 to 140 mg
of lead settles in particulate form  each month on each square meter of
surface area.  Accordingly, each 0.5 to 2 square feet of surface area
is contaminated each month  by  an amount equivalent to the daily body-
burden limit for lead.

Contamination of Water
    The lead concentration  in  drinking water supplies ranges from
traces to 0.04 mg per liter, averaging 0.01 mg per liter.  At con-
centrations of 0.1 mg per liter, bacterial decomposition of organic
matter is inhibited and some fish are susceptible to lead poisoning.
Adults consume 1 to 3 liters of drinking water per day.


    The Public Health Service  Drinking Water Standards state that
0.05 mg of lead per liter constitutes grounds for rejection of the
water supply.

    Helena Valley waters contain  less than 0.001 to 0.04 mg per liter.
The water in Prickly Pear Creek contained 0.044, 0.000, and 0.042 on July
1, 1969, October 25, 1969, and April 4,  1970, respectively.  Missouri
River water at the Helena City Water Plant intake contained 0.033,  0.000,
and 0.019 on those respective  dates.

Contamination of Soil
    The expected lead content  of  soil  is  16  ppm.  The concentration
in soil outside, but adjacent  to,  the  Helena Valley is 15  ppm.  The
concentration in the soil of the  Helena  Valley decreases with distance
from the smelting complex.  At distances  of  1, 2, and 4 miles, respec-
tively, the  upper  inch of uncultivated  soil  contains 4000,  600, and
100 ppm and  the upper 4-inch layer of cultivated  soil contains 700,
250, and 90  ppm.

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ZINC
    Zinc is a normal constituent of the human body.   It  is taken
Into the body in the diet or by inhalation,  and is  eliminated  by
processes of excretion and perspiration.   Excessive body intake,
however, can result in zinc poisoning.

Contamination of Air
    Inhalation of zinc does not represent a  significant  health risk  to
the general population, but it is of concern in the field of occupational
health.  Exposure to air containing milligram quantities per cubic
meter has resulted in metal-fume fever, a malaria-like illness that
lasts about 24 hours and has never been known to be fatal.

    Maximum permissible atmospheric concentrations  for zinc have  not
been established.  The 1967 American Conference of  Governmental Industrial
Hygienists adopted the value of 5 milligrams per cubic meter (mg/m  )  for
zinc oxide fumes in occupational exposures.

    During the summer and fall of 1969, airborne zinc in the Helena
Valley, depending upon location, averaged less than 0.1  to 3 ug/m ,
with maximum 24-hour values up to 8 yg/m3.

Contamination  of Water
    Zinc salts act as gastrointestinal  irritants.  Although the
Illness may be acute, it is transitory.  The emetic concentration in
water is 1 gram per liter.  Communities have used waters containing
up to 27 mg per liter without harmful effects.

    Concentrations of about 30 mg per liter  impart  a milky appearance
and a metallic taste.  Concentrations below  4 mg per liter generally
are not detectable by the human sense of taste.

    Inasmuch as zinc in water does not cause serious effects on health
but produces undesirable esthetic effects, it is recommended that con-
centrations of zinc be kept below 5 mg per liter.
                                                                     21

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    Water supplies  within the  Helena Valley were found to contain
0.003 to 0.2 mg per liter.

Contamination  of  Soil
    The expected content of the soil is  44 ppm.  The concentration
in soil outside, but adjacent  to,  the  Helena Valley is 58 ppm.  The
concentration of zinc in the soil  of the Helena Valley decreases
with distance from the smelting complex. At a distance of 1 mile,
the upper inch of uncultivated soil and  the upper 4-inch layer of
cultivated soil contain 1100 and 300 ppm, respectively, whereas at a
distance of 2 miles from the complex both soils contain 200  ppm.
22

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            EVALUATION  OF  POLLUTANT EFFECTS

VEGETATION
     Leaf damage and  contamination can be attributed  to specific pollutants
Suppression of growth rate may occur as a result of pollution.  From
studies conducted during  the surmer of 1969, it was concluded that the
vegetation growth rate was suppressed 15 percent in the vicinity of the
city of East Helena.

Damage  from Sulfur Dioxide
     Within 1 mile of the smelter complex, sulfur dioxide  leaf damage to
Indigenous alfalfa, corn, sweet  potato, lettuce, tomato, grape, apple,
and plum occurred during  the summer of 1969.

     Sulfur dioxide damage was identified historically on pine trees
growing within 1/2 mile of the smelter complex during 1969.  In 1968,
this type of damage was found at distances up to 4 miles from the
smelter complex.

•Arsenic  Contamination
     The tolerance for arsenic on sprayed fruits and vegetables set by
the Food and Drug Administration is 3.5 ppm.  Lettuce, carrot,  beet,
pinto  bean, and alfalfa grown  in the  city of Helena in 1969 had an
average arsenic content of 0.4 ppm.

     Concentrations  in edible  portions of unwashed vegetables and crops
grown  in 1969 within a 4-mile  radius  of East Helena varied from 0.05
 to 14  ppm on a wet basis.  Pasture  grass, barley straw, and alfalfa
contained 0.4 to  14  ppm.  Barley, wheat, and oat kernels contained  0.05
 to 0.9 ppm.  Onion,  lettuce, carrot,  and cabbage had maximum concentra-
 tions  of 0.9 to 3 ppm.  Apple,  beet,  kohlrabi,  potato, radish, rutabaga,
 string bean, and  garden peas had maximum concentrations of 0.05 to  0.5
 ppm.
                                  -23

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Cadmium Contamination
     Lettuce,  carrot, beet, bean, and alfalfa grown in the city of Helena
during 1969 had an  average cadmium content of 0.7 ppm.

     The concentration  in edible portions of unwashed vegetables and
crops grown in 1969 within a  4-mile radius of East Helena varied from
0.05 to 10 ppm.  Pasture grass, alfalfa, and barley straw contained
0.1 to 10 ppm.  Barley, wheat, and oat kernels contained 0.1 to 1.5 ppm.
Lettuce and beet maximum concentrations were 3.4 and 2.5 ppm, respectively.

Lead Contamination
     Lettuce, carrot,  beet,  bean,  and  alfalfa grown in the city of Helena
during 1969 had an average  lead  content of 1 ppm.

     Concentrations in edible portions of unwashed vegetables and crops
grown in 1969 within a 4-mile radius  of East Helena varied  from 0.1  to
100  ppm.   Pasture grass,  barley  straw, and alfalfa contained 1.4  to  100
ppm.  Barley, wheat, and oat kernels  contained 0.1 to  10  ppm.  Lettuce,
beets, and cabbage had maximum concentrations of 17,  15,  and 9 ppm,
respectively.

Zinc Contamination

      Lettuce,  carrot,  beet, bean, and alfalfa grown  in the  city of  Helena
in 1969  had an average zinc content of 12 ppm.

      Concentrations in edible portions of •unwashed  vegetables  and  crops
grown in 1969 within a 4-mile radius of East Helena  varied  from 0.5 to
 230 ppm.  Pasture  grass, barley straw, and alfalfa contained 23 to 124
 ppm.  Barley, wheat, and oat kernels contained  23 to 86 ppm.  Beet,
 lettuce, carrot, and garden  peas had maximum concentrations of 68,  36,
 36, and 22 ppm, respectively.

 ANIMALS
      Systematic investigation of health abnormalities caused by air
 pollutants was not feasible  during this study.   Accumulation of heavy
 metals  in hair, in organs,  and  in edible animal  tissue was  investigated.

  2*

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Acute Effects on Health
     Horses are more susceptible than other species of farm animals to
the environmental toxicants that occur within  the Helena Valley.  The
1969 post-mortem report on a 3-year-old bay mare reads:
     10/12 - about 4 pm on horse reported to have clinical signs of
     "smoked" horse syndrome.  Frothy nasal exudata, congestion and
     consolidation in lungs with varying degrees of hepatization,
     grossly; not the severity of lung damage  as seen  in some  previous
     cases on ranch.  All  other systems (no nervous exam)  appeared
     grossly normal.
This report is consistent with chronic lead and/or cadmium exposure,
pneumonia primary or secondary to heavy-metal  exposure, and/or heart
disease primary or secondary to heavy-metal exposure.  The presence of
toxic  levels in the kidney  (300 ppm cadmium and 3  ppm  lead)  and in the
liver  (80 ppm cadmium and 4 ppm lead) but not  in the mane, indicates
an  acute rather than a long-term or chronic exposure.

Heavy-Metal Accumulation in Hair
      Hair is a depot for arsenic, cadmium, and lead  during long-term
exposure to  these metallic  toxicants.   Increasing levels  of  arsenic,
cadmium, and lead  in the manes of horses of the Helena Valley correlate
with  proximity to  the smelter complex.  Older horses,  horses residing in
 the Valley  for the  longest  duration,  and chronically impaired horses
 have  the highest concentrations of lead and cadmium.   A significant
 percentage  of  the  horses exhibit lead and  cadmium levels that are two
 to five  times  the  usual concentrations  of  cadmium and lead in horse
mane hair.

Heavy-Metal Accumulation in Organs
      Livers and  kidneys of uncaged domestic rabbits living within
 0.5 mile of the smelter complex contained  elevated levels of  cadmium
 and lead.   Cadmium content of the  livers  from different rabbits varied
 from 4 to 9 ppm, and content of the  kidneys varied from 20 to 60 ppm;
 the usual cadmium content is approximately 0.1 ppm for liver  and 0.3
 ppm for kidney.  Lead content of the livers varied from 3 to  8 ppm, and
 content of the kidneys varied from 2 to 19 ppm;  the usual lead content
 is less than 0.1 ppm.
                                                                       25"

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     Liver and kidney tissues of mice living in the Helena Valley also
contain increased levels  of  cadmium and lead.  The average cadmium
content of liver tissue varied  from 0.4 to 5 ppm, and the content of
kidney tissue ranged  from 1.5 to 14 ppm.  Liver and kidney tissue of
similar animals caught outside, but adjacent to, tbe Valley averaged
0.2 and 2 ppm cadmium, respectively.  Jn liver tissue, the average
lead content varied from  2 to 15 ppra and in kidney tissue, from 2 to
110 ppm.  Liver and kidney tissue of similar animals caught outside,
but adjacent to, the  Valley  both averaged 0.5 ppm leaoU

Heavy-Metal  Accumulation  in Animal Foodstuffs
     Delayed opening  of a local slaughterhouse limited the evaluation
of the hazard of foodstuffs  derived from the animal population to
samples that could be collected from local farms.  Beef, swine, chicken,
and rabbit muscle within  2 miles of the smelting complex contained
maximum concentrations of 0.6 ppm arsenic, 0.4 ppm cadmium, 0.5 ppm
lead, and 70 ppm zinc. Whole milk was found to contain a trace quantity
of arsenic, 0.02 ppm of cadmium, 0.06 ppm of lead, and 5 ppm of zinc.

HUMANS
     Investigation of air-pollution-related health impairment in the
residents of the Helena Valley  was not within the scope of this study.
Investigations were made, however, of  heavy-metal accumulation in human
hair and body burdens of  heavy  metals.

Heavy-Metal Accumulation  in  Hair
     The exposure of the  residents of  the Helena Valley to heavy metals
was reflected by elevated concentrations of arsenic, cadmium, and lead
in the hair of fourth-grade  school boys.  Elevated levels of these
metals in hair have not been associated with any clinical illness in
these children.

     Average  and maximum heavy-metal  levels  in  hair are listed by city
in Table  3.

Body  Burden
     Acceptable daily  intake of trace metals  is based  upon  analysis  of
common foodstuffs, air, and water and upon excretions. Estimated
 2$

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          Table 3.   HEAVY-METAL  LEVELS  IN  HAIR FOR THREE CITIES


East Helena
Helena
Bozemana
Arsenic
Average
5.2
0.8
0.4
Maximum
30
1
1
Cadmi urn
Average
2.0
1.3
0.9
Maximum
6
6
3
Lead
Average
43
12
8
Maximum
175
75
22
aBozeman, a neighboring city not believed to be influenced  by  contamina-
 tion, is listed for the sake of comparison.

maximum daily intake levels for arsenic, cadimum,  lead,  and zinc  are  0.9,
0.2, 0.4, and 13.0 milligrams, respectively.

     The diet represents the major source of body  intake of these heavy
metals; however, in areas of high contamination, ingestion  of  soil or dirt
also may be a consideration.  In East Helena, ingestion  of  10  milligrams
(0.0004 ounce) of the airborne settleable particulates will double the
acceptable daily intake of lead.  The ingestion of 200 milligrams of such
particulate matter will result in an intake of cadmium that is double the
acceptable level.

     Assuming that garden vegetables contain heavy-metal contaminants
equivalent to the maximum measured and  that garden vegetables  provide the
entire dietary  source of vegetables on  a continuing basis,  calculations
Indicate that the body  burden will be exceeded for cadmium and lead.
Tissue accumulation  is  to be expected.   Although  no acute  health
hazard is  indicated, concern must be given  to  the effects  that might occur
following  continuous exposure  to these  levels  of  cadmium and lead.
                                                                       27

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                      POLLUTANT SOURCES

     Annually,  industrial  processes  in the Helena Valley are the source
of approximately 80,000 tons  of sulfur dioxide and 6,000 tons of partic-
ulate matter.  Additional  particulates are also emitted from unpaved
roads.

     Industries of the East Helena smelting complex contribute the bulk
of air pollution found in  the Helena Valley.  This complex consists of
the lead smelter of the American Smelting and Refining Company, the zinc
oxide plant of the Anaconda Company, and the paint pigment plant of the
American Chemet Corporation.

     The East Helena smelter  of the  American Smelting and Refining
Company converts mineral ore  to usable metal.  Lead concentrates and
crude ore are brought to the  plant by rail.  Ore concentrates contain
50 to 70 percent lead and  10  to 30 percent sulfur.  Gondola cars (about
8 per day) are unloaded with  a backhoe onto moving belts that carry
the material up to receiving  bins.   Crude ore is put  through a crusher
before being put into a bin.   Concentrates are mixed  with zinc residues,
limestone, and siliceous ore; the material is pellitized and then
delivered by belt conveyor to the sintering plant, where the mixture is
fused by burning off the sulfur.  The resulting  sintered ore concentrate
1s mixed with coke and charged into  the  top of a blast furnace.  The
charge, about 1,000 tons of material per day, 1s ignited, melted,  and
reacted to form lead bullion and slag.   Lead  and slag flow  from  the
furnace continuously into  a brick-lined  settler.   Slag overflows the
settler into slag pots and is transferred  by  rail  either to the  Anaconda
Zinc Oxide plant or to the slag pile.  Lead  bullion  is tapped  into pots
and transferred by rail to the dressing  plant.   In the dressing  plant,
the lead is  poured into one of several  large  (90-ton) kettles  and  allowed
to cool.  Copper, having a higher melting  temperature, crusts  or drosses.
The dross floats on top and is skimmed off;  after  being mixed  with soda
ash and coke breeze, the dross is transferred to a reverber»atory furnace
where it is  smelted for further separation of zinc and lead according  to
                                 29

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density.  Molten lead flows to the bottom and  a  layer of  slag floats  to
the top.  Just under the slag, copper matte (metal  sulfides) forms, and
copper speiss (metal arsenides and antimonides)  settles just over  the
molten lead.  The matte and speiss are cooled  and  shipped out of the
area to a copper recovery plant.   Molten lead  is recycled to the dressing
kettles.  Lead in the dressing kettle is further purified by the addition
of sulfur and by cooling, which results in further removal  of copper  as
matte.  The lead is then cast into 10-ton ingots and shipped out of the
area to a lead refinery.

     The zinc oxide plant of the Anaconda Company  recovers  zinc from  the
lead smelter slag.  Daily, 100 tons of zinc oxide  is recovered  from
approximately 500 tons of smelter slag.  Molten slag received directly
from the lead smelter or from cold storage is  transported by rail  in
large pots and dumped into the top of a furnace.  Pulverized coal  and
air forced into  the bottom of the slag bath heat the mixture to 2,200° F.
Zinc is vaporized, oxidized, and drawn from the furnace through a  flue-
and-cooling system, where the oxides solidify.  The air stream  bearing
the solid oxides is forced through a baghouse that collects the zinc
oxide.  Molten slag, drawn from the bottom of the furnace into  pots,  is
taken by rail and dumped on the waste slag pile.

     The paint pigment  plant of the American Chemet Company modifies
zinc and copper  oxides.  Daily, 15 tons of zinc oxide from the  zinc
fuming  plant  is  heated  with natural gas in rotary kilns to improve the
whiteness quality by removing traces of coal and by reacting any remain-
ing sulfur.   This product  is  then pulverized and packed in bags for
outside distribution.   Additionally, up  to 100  tons per day of zinc  oxide
from a  different source can be pulverized.  This plant also has the
capacity  to  produce 150 tons  per day of cupric  oxide pigments.   Crude
cupHc  oxide  is  reduced in a  closed retort, milled, and packaged for
distribution.

SULFUR DIOXIDE EMISSIONS
      The  East Helena lead  smelter and  zinc recovery plants collectively
account for 99 percent of  the Helena  Valley sulfur dioxide emissions.

30

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Lead Smelter
     During the normal production rate of 1,200 tons  of  feed  per day,
the smelter emits 330 tons of sulfur dioxide.   The charge  stock  contains
up to 30 percent sulfur, of which 89 percent is released during  the
sintering operation, 4 percent is released from the blast  furnace,  and
7 percent remains with the slag.  Small amounts are released  from the
slag dump, the dressing plant, and the reverberatory furnace. Off-gases
from the sintering operation pass through an electrostatic precipitator
for dust removal and are discharged to the atmosphere from a  400-foot
stack.  Off-gases from the blast and reverberatory furnaces are  combined,
pass through a baghouse, and are discharged into the atmosphere  at an
elevation of 117 feet.

     No attempt is made to curtail emissions by either recovery  or
removal of sulfur from the gaseous emissions.  In July 1970,  the Montana
State Board of Health adopted an emission standard stating that within
3 years the amount of sulfur that may  be released into the atmosphere in
gaseous form must be  less than  10 percent of the amount contained in
the  process raw material.

      The  400-foot stack is used to reduce the  impact of emissions from
the  sintering operation at ground level near the smelter.  In the spring
of 1970,  an induced draft fan and stack heater were added to reduce such
impact further.  Three ground-level  suTfur  dioxide monitoring stations
are  operated  In  the smelter area by  the American Smelting and Refining
Company.   Reportedly,  if  a monitor detects  a concentration of 0.7 ppra
that persists  for 15  minutes, the sintering plant  is shut down  and  is
not  started up until  the  monitor indicates  a concentration of less  than
0.5  ppm  for 15 minutes.

      Sulfur dioxide emissions from  the sintering  operation can  be reduced
by conversion to and  recovery as sulfuric  acid, by conversion to and
recovery as  sulfur, or through  removal by  scrubbing.  Sulfur dioxide
emissions from the  baghouse can be  reduced by  a limestone scrubber.

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Zinc Recovery Plant
     Operating at a production rate of 100 tons  of product per day,  the
plant emits 13 tons of sulfur dioxide.  The raw  material  is 2 percent
sulfur, and the resulting waste slag is 1  percent sulfur.   Sulfur
dioxide is emitted from the charging of the furnace,  from the baghouse,
and from the slag pile.
     Sulfur dioxide emitted from the baghouse  and  from furnace  charging
can be reduced by cleaning the effluent with a limestone-type scrubber.
Emissions from the slag-dumping operation can  be eliminated by  the  use
of a granulating-type operation in which the molten residue slag is
quenched by a stream of water, inside an enclosure, and the effluent
gases are vented to a limestone scrubber.
Source-Receptor Relationships
      Estimates of contributions from individual sources to the ambient
pollutant concentrations were made using sulfur dioxide emission data
and  meteorological measurements of air movement.  Sources considered
were the zinc fuming  plant baghouse, the smelter baghouse, and the 400-
foot stack  from  the smelter.


      Depending upon atmospheric stability,  the  point of maximum impact
 of the baghouses generally will occur at distances of  0.2 to  2 miles
 from the  source.  The maximum 1-hour sulfur dioxide concentrations '
 expected  are 0.6 to 0.9 ppm  from  the Anaconda  baghouse and  1  to 3 ppm
 from the  smelter baghouse.   The maximum point  of  impact from  the 400-
 foot stack can  occur  at distances of 0.4  to 31  miles,  and respective
 1-hour values of 5 and 0.2  ppm can be expected.  The maximum  point of
 impact from the  400-foot stack when heater  and fan  are operating will
 occur at distances of 0.5 to 43 miles,  and  concentrations of  2  and  0.1
 ppm, respectively, can be expected.
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     Aerodynamic downwash of the baghouse  emissions is expected to cause
concentrations in excess of 8 ppm within the  city  of East Helena.

     Diffusion calculations of annual mean concentrations, neglecting
downwash phenomena, throughout the Helena  Valley predict that:  75
percent of the atmospheric sulfur dioxide  in  Helena originates from the
400-foot stack (with fan and heater); 85 percent of the atmospheric
sulfur dioxide in East Helena originates from the  baghouses;  and  50
percent of the atmospheric sulfur dioxide  in  the area  southeast of the
city of East Helena originates from the 400-foot stack.

PARTICULATE EMISSQftS
     Industrial processes and fuel use  account for 98  percent of  the
estimated particulate emissions.  Unpaved  streets  in the area emit an
unknown quantity of particulates; the seriousness  of these emissions
is compounded by the number of unpaved  streets in  use  and by  the
cadmium and lead contamination of road  dirt in East Helena.

LEAD SMELTER
     When operating at  a normal production rate of 1,200  tons of  feed
per day, the smelter is estimated to emit 1,000 pounds of  particulate
matter that contains substantial concentrations of arsenic,  cadmium,
lead, and zinc.  Known  points of emission include the  material-receiving
area during unloading of concentrates,  the outside yard area used for
storage of concentrates, and  the baghouse through which off-gases from
the sintering furnace pass  to the atmosphere.

     Only minimal  efforts  have  been made by the company to control
emissions from material  handling.  Particulates in the off-gases  of the
blast and reverberatory furnaces are estimated to be 99 percent controlled
by the baghouse.   Particulates  in the off-gases of the sintering  furnace
are controlled  by  an electrostatic precipitator reported to be  97 percent
efficient, but  the reported efficiency is questionable because  of the
age of  this  precipitator.
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Zinc Recovery  Plant
     Quantitative estimates  of  emissions are not available; but known
points of emissions  are  the  furnace,  the baghouse, the slag dump, and
the coal pulverizer.   When slag is  charged  into the furnace, copious
emissions of white fumes,  believed  to contain high concentrations of
cadmium, lead, and zinc, are emitted  at the charging door.  The product,
zinc oxide, is collected by  a baghouse with a high collection efficiency.
Disposal of slag is  estimated to emit in excess of 1 ton per day of
particulate matter,  and  coal crushing emits a sizable but undetermined
quantity of coal dust.

     The company has made  no efforts  to control particulate emissions
from the charging of the furnace and  from  the dumping of slag.  A bag-
house has been installed to  control emissions from the coal crusher.

Source-Receptor Relationships
     Neither the amounts nor the physical  and chemical properties - such
as size, shape, density, and chemical content - of particles  emitted  by
industrial sources in East Helena are known.  Quantitative estimates
cannot  be made, therefore, of the distribution of particles and heavy
metals  at ground level.   Unlike gases, particulates attain some downward
settling velocity.  Accordingly, maximum  ground-level airborne particulate
and heavy-metal concentrations  occur  closer to the sources  than do  the
maximum concentrations predicted for  sulfur dioxide.

WASTE WATER  EMISSIONS

Lead Smelter
      Plant effluent, consisting of cooling water  and  process  wash water,
1s discharged into holding  ponds that connect with Prickly Pear  Creek.
Cooling water is cycled at  a rate of 1,450 gallons per minute between
the plant and the retention ponds.  Water from  the washing of speiss  is
discharged into  the ponds for  a period of 1 hour  per  day at a rate  of
600 gallons  per  minute.
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     Speiss wash water is  high  1n heavy metal content.  Analysis by the
State of Montana of the pond  discharge into the creek indicates the
following metals and their concentrations in parts per million:  arsenic,
0.8; copper, 1.1; lead, 0.6;  and iron, 1.1.

Zinc Oxide Plant
     Process and cooling water  from this facility is held in ponds for
recirculation, with no discharges being made into Prickly Pear Creek or
any other portion of the Valley's drainage system.

SOLID  WASTE DISPOSAL

Lead Smelter
     Process slag from past operations  is stored on plant property near
Prickly Pear Creek.  Upon  demand,  this  slag  is  taken  to the zinc oxide
plant  for further processing.

Zinc Oxide Plant
     The waste slag is taken in pots by rail and dumped on the  large
waste-slag  pile located between the smelting complex  and the city of
East Helena.
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