EPA-600/4-7 7-001
January 1977                              Environmental Monitoring Series
       ENVIRONMENTAL RADIOACTIVITY LABORATORY
              INTERCOMPARISON  STUDIES PROGRAM
                                                FY 1977
                              Environmental Monitoring and Support Laboratory
                                     Office of Research and Development
                                    U.S. Environmental Protection Agency
                                          Las Vegas, Nevada 89114

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                RESEARCH REPORTING SERIES

Research reports of the Office of Research and Development, U.S. Environmental
Protection Agency,  have been  grouped into  five series. These five  broad
categories were established to facilitate further development and application of
environmental technology. Elimination of traditional grouping was consciously
planned to foster technology transfer and a maximum interface in related  fields.
The five series are:

     1.    Environmental Health Effects Research
     2.    Environmental Protection Technology
     3.    Ecological Research
     4.    Environmental Monitoring
     5.    Socioeconomic Environmental Studies

This report has been assigned to the ENVIRONMENTAL MONITORING series.
This series describes research conducted to develop new or improved methods
and  instrumentation  for the  identification and quantification of environmental
pollutants at the lowest conceivably significant concentrations.  It also includes
studies to determine  the ambient concentrations of pollutants in the environment
and/or the variance of pollutants as  a function of time or meteorological factors.
This document is available to the public through the National Technical Informa-
tion Service, Springfield, Virginia 22161.

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                                           EPA-600/4-77-001
                                           January 1977
         ENVIRONMENTAL RADIOACTIVITY
LABORATORY  INTERCOM?ARISON  STUDIES  PROGRAM
                    FY  1977
                        by

             Quality Assurance Branch
Monitoring Systems Research and Development Division
   Environmental Monitoring and Support Laboratory
             Las Vegas,  Nevada  89114
        U.S. ENVIRONMENTAL  PROTECTION AGENCY
        OFFICE OF RESEARCH AND DEVELOPMENT
   ENVIRONMENTAL MONITORING AND SUPPORT LABORATORY
             LAS VEGAS,  NEVADA  89114

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                                 DISCLAIMER
     This report has been reviewed by the Environmental Monitoring and Support
Laboratory-Las Vegas, U.S. Environmental Protection Agency, and approved for
publication.  Mention of trade names or commercial products does not constitute
endorsement or recommendation for use.
                                     11

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                                   PREFACE

     Quality assurance is an integral part of any viable environmental moni-
toring activity.  The primary goals of the U.S. Environmental Protection
Agency's (EPA) quality assurance program are to improve and document the
credibility of environmental measurements.  To achieve these goals, quality
assurance is needed in nearly all segments of monitoring activities and should
cover personnel, methods selection, equipment, and data handling procedures.

     Five major functions, each essential to an effective quality assurance
effort, comprise EPA's quality assurance program.

                • Promulgation of standardized methods of
                  measurement

                • Distribution of standard reference materials

                • Issuance of guidelines and procedures

                • Training and technical assistance

                • Evaluation and certification of monitoring
                  activities

     This manual has been prepared to assist laboratories involved with en-
vironmental radiation measurements in developing and maintaining a quality
control program and documenting the precision and accuracy of their data.
All EPA monitoring programs are requested to make use of this document in
planning their own radiation measurements and in assisting the States in
carrying out radiation monitoring activities.

     Comments concerning the utility of this document, along with any sug-
gestions for possible changes and revisions, are welcomed.  Questions on
matters related to quality assurance of environmental measurements in various
fields should be directed to the following person(s):

          Air Pollution

            Mr. Thomas Clark
            Quality Assurance Branch
            Environmental Monitoring and Support Laboratory
            Research Triangle Park, North Carolina  27711
                                     111

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          Pesticides

            Mr. Jack Thompson, Chief
            Analytical Chemistry Branch
            Environmental Toxicology Division
            Health Effects Research Laboratory
            Research Triangle Park, North Carolina  27711

          Radiation

            Mr. Arthur N. Jarvis, Chief
            Quality Assurance Branch
            Monitoring Systems Research and Development Division
            Environmental Monitoring and Support Laboratory
            Las Vegas, Nevada  89114

          Water

            Mr. John Winter, Chief
            Quality Assurance Branch
            Environmental Monitoring and Support Laboratory
            Cincinnati, Ohio  45268

     Periodically, manuals and documents will be issued which provide guide-
lines to be followed in all phases of monitoring activities.  Use of these
guidelines throughout the Agency will enable a uniform approach to be estab-
lished within EPA which ultimately can be implemented at the State level.
This should permit a significant improvement in the validity and reliability
of environmental data collected throughout the Nation.

     The implementation of a total and meaningful national environmental
quality assurance effort cannot succeed without the full support of all moni-
toring programs.  Your cooperation is appreciated.

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                                 CONTENTS

                                                                      Page

Preface	ill

The Laboratory Intercomparison Studies Program  	     1

Types of Environmental Samples Distributed  	     2

Analysis of Data	     3

Participation in the Laboratory Intercomparison
Studies Program 	     3

Statistical Calculations  	     4


Tables

  1.   Summary of Cross-check Programs  	     9

  2.   Cross-check Sample Distribution Schedule 	    10

  3.   Laboratory Precision:  One Standard Deviation
       Values for Various Analyses  	    11


Figures

  1.   Results report form	    12

  2.   Sample analysis and report of participant's data 	    14

  3.   Control chart	    16

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           THE LABORATORY  INTERCOMPARISON  STUDIES PROGRAM

     Environmental measurements of radiation are made daily by many Federal,
State, local, and private agencies.  The data from these measurements are
used for a wide variety of purposes including assessment of health effects,
the establishment of standards and guides,  and for enforcement activities.
It is therefore imperative that the precision and accuracy of the data be
assured in order that policy decisions concerning environmental quality are
based on valid and comparable data of known reliability.

     In order to attain this goal, an Agency-wide quality assurance program
has been implemented within the U.S. Environmental Protection Agency (EPA).
In the area of radiation, quality control responsibilities have been assigned
to the Quality Assurance Branch at the EPA's Environmental Monitoring and
Support Laboratory-Las Vegas which carries out a program designed to en-
courage the development and implementation of quality control procedures for
sample collection, laboratory analysis, and data handling and reporting.

     A major objective of this program is to assist laboratories involved in
environmental radiation measurements to develop and maintain both an intra-
laboratory and an interlaboratory quality control program.  In part, this is
accomplished through an extensive laboratory intercomparison study  ("cross-
check") program involving environmental media (milk, water, air, food, soil,
and gases) and a variety of radionuclides with activities at or near environ-
mental levels.

     Simulated environmental samples, containing known amounts of one or more
radionuclides, are prepared and routinely distributed to all laboratories
upon request.  These laboratories perform the required analyses and return
their data to the Quality Assurance Branch for statistical analysis and
comparison with known values and analytical values obtained by other partici-
pating laboratories.  A report and a control chart are returned to each
participant.  The program thus enables each laboratory to document the pre-
cision and accuracy of its radiation data,  identify instrument and procedural
problems, and to compare its performance with that of other laboratories.

     Each laboratory making environmental measurements for radiation should
have an internal quality control program in operation to insure that all
instrumentation is calibrated and functioning, and that analytical procedures
are being carried out properly.  Such a program includes continual monitoring
of instrumentation, the plotting of instrument control charts, frequent
analysis of replicate samples to check precision, and the regular measurement
of samples to which known amounts of activity have been added to check the
accuracy of systems.

     Participation in a laboratory intercomparison study does not automatical-
ly assure the precision and accuracy of a laboratory's data and should not be

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considered as a substitute for a continuous quality control program within a
laboratory.  Intercomparison data may be useful for documenting precision and
accuracy, and helping to indicate instrument or procedural problems.  Par-
ticipation in intercomparison studies is useful in augmenting a laboratory's
quality control program by serving as a check on its internal quality control
program.

     You are encouraged to have your laboratory participate or expand par-
ticipation in the cross-check program of the Quality Assurance Branch of the
EMSL-LVs Monitoring Systems Research and Development Division.
             TYPES OF ENVIRONMENTAL  SAMPLES DISTRIBUTED

     The current laboratory intercomparison studies program covers the analy-
sis of a variety of media containing various levels of radioactivity.  These
include:

     Milk:     Four-liter milk samples containing potassium, strontium-89,
               strontium-90, iodine-131,  cesium-137, and barium-140 are
               distributed on a bimonthly basis.

     Water:    Water containing several different mixtures of radioactive
               materials is included in the cross-check program.

               •  Four-liter samples for the analysis of gross alpha and
                  gross beta activity are sent bimonthly to participating
                  laboratories.

               •  Four-liter samples containing chromium-51, zinc-65,
                  cobalt-60, ruthenium-106, cesium-134, and cesium-137 are
                  distributed bimonthly for analysis of gamma emitters.

               •  Fifty-milliliter samples for tritium analysis are dis-
                  tributed on a bimonthly basis.

               •  Four-liter water samples containing plutonium-239 are
                  shipped to laboratories twice a year.

               •  Four-liter samples of well water containing radium-226
                  and/or radium-228 are distributed four times a year.

     Air:      Three 2-inch-diameter air filters are sent out on a quarterly
               basis for gross alpha, gross beta, plutonium-239,  cesium-137,
               and strontium-90 analysis.

     Soil:     Thirty-five-gram soil samples, containing plutonium-239 and
               plutonium-238 or thorium-228, thorium-230 and thorium-232,
               are distributed twice each year.

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     Food:     Two 4-liter food slurries containing strontium-89, strontium-90,
               iodine-131, cesium-137, barium-140, and potassium are sent to
               participants quarterly.

     Urine:    Fifty-milliliter urine samples containing tritium are shipped
               on a quarterly basis.

     Gases:    One-liter, steel, gas cylinders, containing 10 liters (S.T.P.)
               of krypton-85 , are distributed four times each year .

     Sample size, approximate activity levels, type of analysis, and other
pertinent information concerning the cross-check samples are summarized in
Table 1.  The distribution schedule is outlined in Table 2.

     A laboratory may participate in any one or all of the studies described.


                             ANALYSIS  OF DATA

     Each participating laboratory is expected to carry out three independent
determinations for each radionuclide included in a particular cross-check
study and to report its results on a form (Figure 1)  provided with the
sample.

     Upon receipt of the reports from all participating laboratories, the
data are transferred to punch cards for computer analysis.  As indicated in
the sample calculations, this analysis includes determination of the labora-
tory standard deviation, calculation of the normalized range, normalized
deviation, sample standard deviation, and the grand average of all labora-
tories.  The analytical precision values, used as a basis for judging labora-
tory performance for specific nuclides, are summarized in Table 3.

     A report is generated containing data reported by participating labora-
tories, listed according to their identity code, along with the results of
the analysis (Figure 2) .  In addition, a control chart is generated  and re-
produced for each radionuclide included in the sample (Figure 3) . The
control charts are updated each time a laboratory participates in a  particu-
lar cross-check study, thus giving each laboratory a continuous record of its
performance.
     A letter giving the known v^iue for each radionuclide is mailed to
participants approximately 2 weeks after the report due date.  This is
followed by a complete report which includes a copy of the computer printout
and control chart.
                          PARTICIPATION IN  THE
             LABORATORY INTERCOMPARISON STUDIES  PROGRAM

     Any laboratory involved in, or concerned with, environmental radiation
monitoring and surveillance is eligible to participate  in any one or all of
the cross-checks described.   Moreover,  dependent upon personnel available and

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their workload, a laboratory may elect to receive samples on a less frequent
basis than indicated on the distribution schedule (Table 2).

     To become a participant in the laboratory intercomparison studies pro-
gram, complete one of the forms included at the end of this publication and
return to:

               U.S. Environmental Protection Agency
               Environmental Monitoring and Support Laboratory
               Quality Assurance Branch
               P.O. Box 15027
               Las Vegas, NV  89114

     Should the laboratory require additional types of cross-check samples at'
some later date, a second form indicating the samples desired should be
submitted.
                        STATISTICAL  CALCULATIONS

     To illustrate the computations performed by the computer, example calcu-
lations are given using data for three samples analyzed at one laboratory
(Laboratory D, see Figure 2).

     The experimental data are listed and the mean, experimental sigma and
range are computed.  These statistics provide measures of the central ten-
dency and dispersion of the data.

     The normalized range is computed by first finding the mean range, R,
the control limit, CL, and the standard error of the range, aR.  The nor-
malized range measures the dispersion of the data  (precision) in such a form
that control charts may be used.  Control charts allow one to readily compare
past analytical performance with present performance.  In the example, the
normalized range equals 0.3 which is less than 3, which is the upper warning
level.  The precision of the results is acceptable.

     The normalized deviation is calculated by computing the deviation and
the standard error of the mean, am-  The normalized deviation allows one to
readily measure central tendency (accuracy) through the use of control charts.
Trends in analytical accuracy can be determined in this manner.  For this
example, the normalized deviation is -0.7 which falls between +2 and -2,
which are the upper and lower warning levels.  The accuracy of the data is
acceptable.

     Finally, the experimental error of all laboratories, the grand average,
and the normalized deviation from the grand average are calculated in order
to ascertain the performance of all the laboratories as a group.  Any bias in
methodology or instrumentation may be found from these results.

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EXAMPLE CALCULATIONS  (Laboratory D Data, see Figure 2)




Experimental data:



     Known value = y = 3273 pCi 3H/liter urine on September 24, 1974


     Expected laboratory precision = a = 357 pCi/liter



               Laboratory     Sample         Result



                    D           xi       3060 pCi/liter


                    D           x2       3060 pCi/liter


                    D           x3       3240 pCi/liter


     Mean = x



                        N


                           "
                                        =  3120 pCi/liter
where      N = number of results = 3



     Experimental sigma = s
        S
                /(3060)2 + (3060)2 +
               v	
                             (3240)2 - (3°6° + 306° + 3240)2

s  =	            3
           =  103.9 pCi/liter



     Range  =  r



               r  =  |maximum result - minimum result]



                  =  |3240 - 3060|   =  180 pCi/liter

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Range Analysis  (RNG ANLY)*




     Mean range = R




          R  =  d2O




             =  (1.693) (357)




             =  604.4 pCi/liter




     Control limit = CL




         CL  =  R + 3a
                      K




             =  Di*R




             =  (2.575) (604.4)




             =  1556 pCi/liter




     Standard error of the range = CR





         aR  =  (R + 3aR - I) v 3
                                             where d2*  =  1.693 for N = 3
                          where
                          - R) T 3




                  =  (1556 - 604.4) v 3




                  =  317.2 pCi/liter




     Let range  =  r  =  wR + xaR  =  180 pCi/liter




     Define normalized range  =  w + x




          for  r > R,  w  =  1




          then         r  =  wR + xO   =  R + xa
                 R
                                                R
                                                        =  2.575 for N = 3
          or
                       x  =
                             r - R
therefore
w+x  =  1+x  =  1+
                                           r ~ R

                                           -

                                             aR
* Rosenstein, M., and A. S. Goldin, Statistical Techniques for Quality Control

of Environmental Radioassay, AQCS Report Stat-1, U.S. Department of Health,

Education and Welfare, PHS, Nov 1964

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          for  r < R,  x  =  0
          then         r  =  wR + xn   =  wR
                                    K
          or
     therefore     w+x  =  w+0  =  —

                                       R



          since   r < R   (180 < 604.4)


                                      180

                           W + X  =
                                  =  0.30




Normalized deviation of the mean from the known value = ND



     Deviation of mean from the known value = D



                            D  =  x - V


                               =  3120 - 3273



                               =  - 153 pCi/liter



     Standard error of the mean = 
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Experimental sigma  (all laboratories) - s    (See Figure 2)
                                              N    ^2
                                 N
                                        2

                                                N
                             -*/ 1=1
                      s
                                162639133 -
                                         14
                          =  149 pCi/liter

Grand average = GA

                              N
                               N

                             49345
                              15

                          =  3290 pCi/liter

Normalized deviation from the grand average = ND1

     Deviation of the mean from the grand average = D1

                      D1  =  x - GA

                          =  3120 - 3290

                          =  - 170 pCi/liter

     »•  -  g^
              m

             - 170
             206.1

          =  - 0.8

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                                  TABLE 1.   SUMMARY OF CROSS-CHECK PROGRAMS*
j SAMPLE
Milk
Water
Gross a, 8*
Gamma
3H
239PU*
Radium
Air
Gross a, B*
239Pu*
Soil*
Diet
Urine
Gas
ANALYSIS
89Sr, 90Sr, 131I,
137Cs, '""Ba, K

Gross a, 6
60Co, 106Ru, 13*Cs,
137Cs, 51Cr, 65Zn
3H
239PU
226Ra, 228Ra

a, B. 9°Sr, 137Cs
239Pu
238Pu, 239Pu
228Th/ 230Thf 232Th
89Sr, 90Sr, 131I,
137Cs, i*»Ba, K
3H
85Kr
ACTIVITY
PER ISOTOPE
< 200 pCi/liter

< 100 pCi/liter
< 500 pCi/liter
< 3500 pCi/liter
< 10 pCi/liter
< 20 pCi/liter

< 200 pCi/sample
< 2 pCi/s ample
< 50 pCi/sample
< 200 pCi/kg
< 3500 pCi/liter
< 20 pCi/ml
QUANTITY
SUPPLIED
^ 4 liters

^ 4 liters
a- 4 liters
^ 50 ml
^ 4 liters
^ 4 liters

3 - 2"-diam.
air filters
3 - 2"-diam.
air filters
^35 grains
2 - 4-liter
samples
^ 50 ml
10 liters
PRESERVATIVE
Formalin

0 . 5N HNO 3
DISTRIBUTION
Bimonthly

Bimonthly
!
0.5N HNO 3 Bimonthly
none • Bimonthly
0 . 5N HNO 3
0 . 5N HNO 3

none
none
none
Formalin
Formalin
none
Semiannual ly
Quarterly

Quarterly
Quarterly
Semiannual ly
Quarterly
Quarterly
Quarterly
TIME FOR
ANALYSIS
& REPORT
6 weeks

4 weeks
4 weeks
4 weeks
8 weeks
— 1
6 weeks

6 weeks i
	
6 weeks ;
8 weeks
8 weeks
4 weeks
6 weeks
* Laboratories are required to have the necessary licenses before receiving these samples.

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TABLE 2.  CROSS-CHECK SAMPLE DISTRIBUTION SCHEDULE
        (Numbers indicate week of the month)
Month
in
FY-77
1976
Oct
Nov
Dec
1977
Jan
Feb
Mar
Apr
May
Jun
Jul
Aug
Sep
Milk
Sr,Y


1


1

1

1

1

1

Gross

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TABLE 3.  LABORATORY PRECISION:  ONE STANDARD DEVIATION VALUES FOR VARIOUS ANALYSES
Analysis
Gamma Emitters
Strontium-89
Strontium-90
Pocassium
Gross Alpha
Gross Beta
Tritium
Radium-226,
Radium-228
Plutonium,
Thorium Isotopes
Kry~con-85
Level
5 to 100 pCi/liter or kg
>100 pCi/liter or kg
5 to 100 pCi/liter or kg
>100 pCi/liter or kg
2 to 30 pCi/liter or kg
>30 pCi/liter or kg
> 0.1 g/liter or kg
420 pCi/liter
> 20 pCi/liter
4100 pCi/liter
>100 pCi/liter
<4000 pCi/liter
>4000 pCi/liter
> 0.1 pCi/liter
>0.1 pCi/liter, gram or sample
5 to 100 pCi/ml (S.T.P.)
Standard Deviation
Single Determination
5 pCi/liter
5% of known value
5 pCi/liter
5%
1.5 pCi/liter
5%
5%
5 pCi/liter
25%
5 pCi/liter
5%
Is (pCi/liter) = 169.85 x (known)'0933
10%
15%
10%
10%

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          U.S.  ENVIRONMENTAL  PROTECTION AGENCY
                                              ENVIRONMENTAL MONITORING AND
                                                  SUPPORT LABORATORY
                                                      P.O. BOX  15027
                                                  LAS VEGAS. NEVADA 89114
                                                       702/736-2969
                      QUALITY ASSURANCE BRANCH
                         ANALYSIS-RESULTS
                TRITIUM IN URINE CROSS-CHECK PROGRAM
Laboratory  	
Contact Person

Phone
Collection  Date
IMPORTANT:   Report  results corrected for decay as  of  the collection date.

            Please  refer to instructions on  back of page.






1

1,
A


i

C

0
I)

E
2

DO NOT

USE
THIS

SPACE
3 4
i
i

6

7
1
I
g


E

3H
ANALYSIS #1
ii

12

13

14

M

.»./»
ll
19
LJ
2b
•


ANALYSIS #2


71

22
.
23
._
24

23

26

37

38

29

3C
.


ANALYSIS #3


31

32

13

14

35

19 37J33
1
w|«
i.


UNITS



pCi/1
     In order  to be  included in the final  report,  please send your results
no later than                         to:
               U.S. Environmental Protection  Agency
               Environmental Monitoring and Support  Laboratory
               Quality Assurance Branch (MSQ)
               P.O. Box 15027
               Las Vegas, NV  69114
                 Figure  1.   Results report form
                                  12

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                          REPORT SHEET INSTRUCTIONS
1.   Legibly type or print numbers and letters in the proper squares.  Use
     only capital letters.

2.   Record lab code in columns 1 and 2 for each isotope  (one isotope per
     line).  For a code of only one letter, use column 1.

3.   Slash the letters 0 and E.  Do not slash any numbers.

4.   Do not use columns 3-7; they are for internal use only.

5.   Data entry:  (columns 11-40)

     a.   All numbers must be right justified  (entered to far right of
          field) .

     b.   For statistical purposes, it is important that each laboratory
          report three results for each radionuclide.  If, for some un-
          avoidable reason, less than three values are reported, record
          the data starting with the columns reserved for analysis #1
          and work to the right.

     c.   Report results to the nearest whole number with the exceptions
          of tritium and potassium (each recorded to multiples of ten)
          and radium-226  (recorded to one decimal place).  Decimal points
          are provided on the report forms.

     d.   Each line of the coding form contains the name of the isotope
          and its unit of activity, preprinted for your convenience.
          Each line should contain information pertaining to just that
          one isotope.

     e.   If a value is less than (LT) the minimum detectable activity
          (MDA), record LT, space, then the MDA value (right justified).
                 Figure 1 (continued).  Results report form
                                     13

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EMSL-LV TRITIUM IN URINE  CROSS-CHECK  PROGRAM  	 SEPTEMBER 1974

                09/20/74            SAMPLE - A        3H
     EXPECTED LABORATORY  PRECISION
                     KNOWN  VALUE
           [IS,  1  DETERMINATION)
LAB
AN
CF
CF
CF
CM
CM
CM
CO
D
D
D
J
J
J
RESUL
NO D,
3269
3522
3632
3261
3373
3362
NO D,
3060
3060
3240
3255
3247
3294
                    EXPERIMENTAL
                       SIGMA
                       186.1
                        61.7
                       103.9



                        25.1

           NO DATA  PROVIDED
           3240
           3340
           3190
76.4
           RNG ANLY
           (R = SR)
               .60
               .19
                                       .30
               .08
.25
          AVERAGE
            3474
            3332
                           3120
                           3265
3257
                   -   3273
                       357
                  PCI/L
                  PCI/L
         NORMALIZED DEVIATION
        (GRAND AVG)     (KNOWN)
             .9
                                                               .2
                       -.8
                       -.1
-.2
             1.0
                         -.7
                                                   -.0
-.1
EXPERIMENTAL SIGMA  (ALL  LABS)
             149
        GRAND  AVERAGE  -
                  3290
      Figure 2.  Sample analysis and report of participant's  data

                                      14

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Explanation of terms in Figure 2:
     Title:
     Column 1:
     Column 2:
     Column 3:
     Columns 4
      and 5:
     Column 6:
     Column 7:

     Column 8:
     Bottom of
      Chart:
Program name, sample collection date, sample code letter,
analysis type, known concentration of radionuclide, expected
standard deviation of analysis - single determination.
Laboratory identification code (A, B, c, etc.).
Laboratory results (0-25 results listed down column).
Is (standard deviation) of the experimental results.
Normalized range value in "mean range + standard error of
the range" (R + a )  units for comparability.  (See
                 R
Statistical Techniques for Quality Control of Environmental
Radioassay, AQCS Report Stat-1, November 1964, pages 4-8.)
(S  = a  for printing purposes.)
  K    R
Average value.
Normalized deviation from the grand average value of all
laboratories expressed in a  units.
Normalized deviation from the known value expressed in OM
units.
Is experimental error of all laboratories, and the grand
average of all laboratories.
                                     15

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10
9
8
7
6
5
4
3
2
* 1
o 0
5 -1
-2
-3
-4
-5
-6
-7
-8
-9
-10
R+3
R+2
R+l
ft+0
0
EMSL-LV TRITIUM IN URINE CROSSCHECK PROGRAM
LAB - D 3H
NORMALIZED DEVIATION FROM KNOWN
1973 W74








^-A r— 	
^^ v 	

















\ ^-» 	 .








J FMAMJJAS ONDJ FMAMJ JA SOND
NORMALIZED RANGE
1973 1974




i . . , 1 , - i




1 . i
CL
WL
WL
CL
CL
WL


J FMAMJJASONDJFMAMJJASOND
Figure 3.  Control chart





           16

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Explanations of terms used in the control chart  (Figure 3).
     Title:
     Upper Graph:
     Lower Graph:
Name of program, laboratory code letter, and type of
analysis.
"Normalized deviation from known versus the month
of analysis."   [The 95.0% (y ± 2CJ ) and the 99.7%
(M ± 3aM) confidence levels were chosen as the warning
levels and control limits respectively.]
"Normalized range values (R + aD) versus the month of
                               R
analysis."  [The 97.5%  {R + 2n ) and ^100% (R + 3n)
                              R                   R
confidence levels were chosen as the warning levels
and control limits respectively.]
                                     17

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SUBJECT:  Participation in Intercomparison Studies Program

     TO:  U.S. Environmental Protection Agency
          Environmental Monitoring and Support Laboratory
          Quality Assurance Branch
          P.O. Box 15027
          Las Vegas, NV  89114

     Please include our laboratory in the cross-check studies we have
indicated below.  All samples are to be shipped to:
     Contact Person
     Title
     Laboratory
     Address
     NRC License
       and/or
Type(s)
     State License  Number(s)	
NOTE:  When requesting participation in a study containing either
       nuclear byproducts or special nuclear materials, a copy of
       the NRC license(s) must accompany the request.
       If your laboratory prefers participation other than the pub-
       lished frequency, please indicate months samples are desired.
            FREQUENCY DESIRED
                         FREQUENCY DESIRED
SAMPLE TYPES
Milk: Sr, y
Water :
Gross a, 3
Y
3H
239pu
226Ra, 228Ra
Diet: Sr, y
BIMONTHLY
QUARTERLY
D D
1 1
n n
a n
a
a
SEMIANNUALLY
ANNUALLY
a a
a a
n n
nnnn
nnnn
SAMPLE TYPES
Air Filter:
Gross a* (3
239pu
Soil:
Pu Isotopes
Th Isotopes
Urine: 3H
Gases: 85Kr
QUARTERLY
a
a
n
n
SEMIANNUALLY
a
n
D
|
nnnn nn
I certify this laboratory is authorized to receive the samples requested.
Date
     Signature
         Title

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                                   TECHNICAL REPORT DATA
                            (Please read instructions on the reverse before completing)
1. REPORT NO.
  EPA-600/4-77-001
                              2.
                                                           3. RECIPIENT'S ACCESSION NO.
4. TITLE AND SUBTITLE
 ENVIRONMENTAL RADIOACTIVITY LABORATORY INTERCOMPARISON
 STUDIES PROGRAM, FY 1977
                                                           5. REPORT DATE
                                                             January  1977
             6. PERFORMING ORGANIZATION CODE
7. AUTHOR(S)
  Quality Assurance Branch
  Monitoring Systems Research and Development Division
                                                           8. PERFORMING ORGANIZATION REPORT NO.
9. PERFORMING ORGANIZATION NAME AND ADDRESS
 Environmental Monitoring  and Support Laboratory
 Office of Research and  Development
 U.S.  Environmental Protection Agency
 Las Vegas, NV  89114
             10. PROGRAM ELEMENT NO.

               1HD621
             11. CONTRACT/GRANT NO.
12. SPONSORING AGENCY NAME AND ADDRESS
 Same  as above
                                                            13. TYPE OF REPORT AND PERIOD COVERED
                                                             interim  (FY-77)
             14. SPONSORING AGENCY CODE
             2PA-ORD, Office  of Monitoring
             ind Technical  Support
15. SUPPLEMENTARY NOTES
16. ABSTRACT

  The  U.S.  Environmental  Protection Agency's  intercomparison studies  program for
  laboratories involved in  environmental radiation measurements is  described.  The
  types of environmental  samples distributed,  the analysis required for each sample,
  the  distribution schedule,  and the statistical analysis and reporting of results
  are  discussed.  Instructions and application forms are included for laboratories
  desiring to participate in  the program.

  This document is not a  research report.   It  is designed for use by  laboratories
  participating or desiring to participate  in  this quality assurance  program.
17.
                                KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
b.IDENTIFIERS/OPEN ENDED TERMS  C. COS AT I Field/Group
  quality assurance
  quality control
  quantitative analysis
  radioactivity
  statistical quality control
                             07  B,  E
                             12  A
                             14  D
18. DISTRIBUTION STATEMENT
  RELEASE UNLIMITED
                                              19. SECURITY CLASS (ThisReport)
                                                 UNCLASSIFIED
                           21. NO. OF PAGES

                              28
20. SECURITY CLASS (Thispage)
  UNCLASSIFIED
                                                                         22. PRICE
EPA Form 2220-1 (9-73)

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