vyEPA
         United States
         Environmental Protection
         Agency
          Industrial Environmental Research
          Laboratory
          Research Triangle Park NC 2771 1
EPA-600/7-78-193
October 1978
Particle Collection
by a Venturi
Scrubber Downstream
from an Electrostatic
Precipitator

Interagency
Energy/Environment
R&D Program Report

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                 RESEARCH REPORTING SERIES


Research reports of the Office of Research and Development, U.S. Environmental
Protection Agency, have been grouped into nine series. These nine broad cate-
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    1. Environmental Health Effects Research

    2. Environmental Protection Technology

    3. Ecological Research

    4. Environmental Monitoring

    5. Socioeconomic Environmental Studies

    6. Scientific and Technical Assessment Reports  (STAR)

    7. Interagency Energy-Environment Research and Development

    8. "Special"  Reports

    9. Miscellaneous Reports

This report has been assigned to the  INTERAGENCY ENERGY-ENVIRONMENT
RESEARCH AND DEVELOPMENT series. Reports in this series result from the
effort funded under the 17-agency Federal Energy/Environment  Research and
Development Program. These studies  relate to EPA's mission to protect the public
health and welfare from, adverse effects of pollutants associated with energy sys-
tems. The goal of the Program is to  assure the rapid development of domestic
energy supplies in an environmentally-compatible manner by providing the nec-
essary environmental data and control technology. Investigations  include analy-
ses of the transport  of energy-related pollutants and their health and ecological
effects;  assessments of, and development of, control technologies for energy
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This report has been reviewed by the participating Federal Agencies, and approved
for publication. Mention of trade names or commercial products does not con
stitute endorsement or recommendation for use.

This document is available to the public through the National Technical Informa-
tion Service, Springfield, Virginia 22161.

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                                 EPA-600/7-78-193

                                     October 1978
Particle Collection  by a Venturi
Scrubber  Downstream  from an
     Electrostatic  Precipitator
                       by

             L E. Sparks, G. H. Ramsey, and B. E. Daniel
                Environmental Protection Agency
               Office of Research and Development
             Industrial Environmental Research Laboratory
             Research Triangle Park, North Carolina 27711
                 Program Element No. EHE624
                     Prepared for

             U.S. ENVIRONMENTAL PROTECTION AGENCY
               Office of Research and Development
                  Washington, DC 20460

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                                ABSTRACT
     The results of pilot plant experiments of participate collection by
a venturi scrubber downstream from an electrostatic precipitator (ESP)
are presented.  The data, which cover a range of scrubber operating
conditions and ESP efficiencies, show that particle collection by the
venturi scrubber is not affected by the upstream ESP; i.e., for a given
scrubber pressure drop, particle collection efficiency as a function of
particle diameter is the same for both ESP on and ESP off.  The experi-
mental results are in excellent agreement with theoretical predictions.
Order of magnitude cost estimates indicate that particle collection by
ESP scrubber systems is economically attractive when scrubbers must be
used for SO  control.
           A
                                   ii

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                                TABLE OF CONTENTS


                                                                       Page
Abstract                                                                i i
List of Figures                                                         iv
List of Tables                                                          iv
Nomenclature                                                            v
Introduction                                                            1
Conclusions                                                             2
Recommendations                                                         2
Experimental Equipment                                                  3
Test Program                                                            5
Experimental Results                                                    5
   ESP Scrubber System Performance                                      11
Theoretical Analysis of Combined ESP Scrubber Systems                   11
Discussion                                                              16
Cost Analysis                                                           19
Plume Opacity                                                           24
References                                                              28

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                                   FIGURES

Number                                                                     Page
  1       Scrubber system added to ESP outlet                                4
  2       Graded penetration curves for venturi  scrubber
             - phase 1 experiments                                           8
  3       Graded penetration curves for venturi  scrubber
             - phase 2 experiments                                           9
  4       Average graded penetration curves for venturi  scrubber
             - phase 2 experiments                                          10
  5       Graded penetration curves for ESP scrubber system                 12
  6       Graded penetration curves for ESP scrubber system                 13
  7       Graded efficiency curve for ESP with penetration
             of 0.0771                                                      17
  8       Penetration versus particle diameter for scrubber with
             pressure drop = 23 cm HLO, density - 2.4 g/cc                  18
  9       Graded penetration curve for ESP scrubber system
             - ESP penetration = 0.0771; scrubber pressure drop =
               23 cm H20                                                    20
 10       Parameter K as a function of the log-normal size
             distribution parameters for a white aerosol                    25
                                    TABLES

Number                                                '                     Page
  1       Experimental Conditions for ESP Scrubber Experiments               6
  2       Summary of Calculated Results for ESP Scrubber System             15
  3       Estimated Light Transmission and In-Stack Plume Opacity
             for ESP Scrubber Systems                                       26
                                       IV

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                              NOMENCLATURE

AC         - Annualized cost, $
C          - Cunningham correction factor
CC         - Capital cost, $
CCESp      - Capital cost of ESP, $
CC
  scrubber - Capital cost of scrubber, $
d          - Particle diameter, ym
d.         - Aerodynamic particle diameter, ymA
E          - Fan efficiency
H          - Number of operating hours per year
I          - Intensity of light transmitted through aerosol
I          - Intensity of light source
                                           32
K          - Light scattering parameter,  cm /m
K          - Cost of electric power, $/kW-hr
L          - Optical path length
L/G        - Liquid to gas flow rate ratio, m /m
PtESP      " Overa11 penetration through  ESP
Ptrrnq     - Overall penetration through  ESP scrubber
Pt(d)ESp   - Penetration of  particles with diameter d through ESP
pt(d)ESps  _ penetration of  particles with diameter d through ESP scrubber
Pt(d)      - Penetration of  particles with diameter d through scrubber
     s                   3
Q          - Flow rate, m /hr
r          - Geometric mass  mean particle radius
 gw                                    23
SCA        - Specific collector area, m /Am /s
                                               23
SCAmin     - Minimum specific collector area, m /Am /s
W          - Mass concentration of particles
AP         - Pressure drop,  cm of water
p          - Density, g/cc
a          - Geometric standard deviation

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INTRODUCTION

     There is considerable interest in using electrostatic precipitator
(ESP) scrubber systems for particulate collection in coal fired utility
boilers. At least one utility plans to use a moderately efficient ESP
followed by a scrubber to meet emission standards for a new boiler.  The
recent amendments to the Clean Air Act which require SO  removal for
                                                       /\
most plants are likely to increase interest in ESP scrubber systems.

     There are numerous undocumented reports that a scrubber downstream
from an ESP works better than expected.  Theoretical and experimental
studies of particle collection by drops indicate that there is no reason
to expect a scrubber downstream from an ESP to have different performance
characteristics than a scrubber alone.   But data on ESP scrubber combinations
are insufficient to allow one to determine if the results from drop
collection theory apply to scrubbers.

     The experimental study  discussed  in this report was undertaken  to
provide the necessary data.  Also a theoretical study was conducted  to
determine what ESP scrubber  configurations are capable of meeting  the
possible particulate New Source Performance Standard for utility  boilers
of 13  ng/J  (0.03 lb/106 Btu).  Order of magnitude cost estimates
were also made.

     The objectives of the program were  to:

     1.   Determine the effect  of  an  ESP  on  the  particle penetration
           (1  minus efficiency)  of  a  venturi  scrubber  as  a  function of
          particle diameter  characteristics.

     2.    Determine  the  overall  mass  penetration and  particle
           penetration  as  a function  of particle  diameter
           for the  ESP  scrubber system.

      3.    Determine,  with the aid  of mathematical  models,  the ESP
           scrubber configurations  capable of meeting  an emission
           standard for fly ash of 13 ng/J.

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     4.   Estimate order of magnitude costs for the systems in 3 above.

CONCLUSIONS

     The results of the experimental and theoretical studies support the
following conclusions:

     1.   The performance of a venturi scrubber is not affected
          by the ESP; i.e., the particle penetration versus particle
          diameter characteristics of the scrubber are the
          same whether the ESP is on or off.

     2.   The performance of the scrubber is adequately modeled
          by the SR-52 programmable calculator model described
                    2
          by Sparks.

     3.   An ESP scrubber system can achieve an emission of
          13 ng/J.

     4.   Annualized costs of an ESP scrubber system are attractive
          when compared to costs for an ESP alone for many cases.

     5.   Plume opacity from an ESP scrubber system may be much
          higher for a given mass emission than the plume
          opacity from an ESP alone.

RECOMMENDATIONS

     1.   Detailed  cost studies of  ESP scrubber sytems should  be
          conducted to determine their economics.

     2.   Experimental and theoretical studies of  plume opacity
          from ESP  scrubber systems should  be  undertaken.

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EXPERIMENTAL EQUIPMENT

     The scrubber system tested in conjunction with the ESP system
consisted of a venturi scrubber, an entrainment separator, and a blower
and motor.  The venturi scrubber had a round cross section with a throat
length of 25.4 cm.  The throat section could be removed so various
throat diameters could be tested.  The ESP scrubber tests involved only
two throat diameters:  7.62 and 10.16 cm.  Larger diameters could not be
installed due to the limiting size of the opening at the throat bottom
flange.  The water was added tangentially at two points at the top of
the scrubber.  The water flow rate could be varied up to a maximum of
         -2  3
6.43 X 10   m /min.  The scrubbing water was not recirculated.  Maximum
gas flow was about 28 m /min.

     Following the venturi scrubber, the gas stream entered  a  cyclonic
entrainment  separator.  The separator had a diameter of  50.8 cm and was
1.22 m in height.  The gas entered the separator at the  bottom and
exited tangentially  near the top.  The gas was  moved through the  system
by a blower  powered  by a 15 hp motor.

     The  installation  of the scrubber to the outlet of the  ESP involved
removing  a  3 m section of duct  from  the  ESP system and rerouting  the  gas
stream through the scrubber system and back to  the original  ESP  system
duct, as  shown in Figure 1.  A  transition  section  was  added to the  ESP
duct to reduce the duct diameter  from 30.48 to  15.24 cm  to  accommodate
the scrubber. Flexible duct was  used to  connect the transition section
to the scrubber.  The gas was exhausted from the entrainment separator
through a 15.24  cm duct to  the  fan and through  a  flexible duct (30.48 cm
diameter) to connect the fan to  the  original  ESP exhaust system.

     Pressure taps were added  to  the duct  at  the entrance to the  scrubber,
between the  scrubber and separator,  and  at the  exit of the  separator.
The pressure taps allowed  for  measurement  of  pressure  drop  over  the
scrubber  and separator.

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    ORIGINAL ESP
    EXHAUST DUCT
ROTA-
METER
          TRANSITION DUCT
(30.48 cm DIAMETER TO 15.24 cm DIAMETER)
                                                                                                                                      ORIGINAL
                                                                                                                                    ESP EXHAUST
                                                                                                                                       DUCT
\
                                                      15.24 cm FLEXIBLE DUCT
                                                        20.32cm SQUARE
                                                           SECTION
                                                Figure 1. Scrubber system added to ESP outlet.

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     The ESP used for the experiment is a one lane wire duct ESP and is
fully described by Lawless et al.

     The aerosol generator consisted of two sand blast guns which were
fed fly ash by a vibrating screw feeder.  Preliminary experiments were
conducted with fly ash fed directly to the sand blast guns.  These
experiments showed that significant fly ash settled in the inlet duct. A
cyclone was placed in the line  between the feeder and the sand blast
guns, to prevent dust fallout in the inlet duct.  Previous experience
showed that this aerosol generator was stable.  Additional information
can be found in Lawless et al.  The particle size distribution was
approximately log-normal with a geometric mass mean diameter of about
5.5 ymA and geometric standard  deviation of 2.3 when the cyclone was
used.

     All size distribution measurements were made with Meteorology
Research,  Inc.  (MRI) cascade  impactors with greased substrates.  The
impactors  were  calibrated by  personnel of  EPA  Industrial Environmental
Research Laboratory's Particulate Technology Branch  (PATB),  using the
                                     4
procedure  described  by  Calvert  et al.

TEST PROGRAM

     The experimental program was divided  into two  phases:   Phase  1  was
a  preliminary  study, and  Phase  2 was a  systematic study  with replication.

     The variables  studied  in the Phase 2  experiments  were:

                ESP  on or off
                ESP  penetration  1  to 0.037  (efficiency 0 to 96.3%)
                Liquid/gas ratio 6.65 x 10"4 to 2.66 x 10~3 m3/Am3

     The experimental  conditions  for all tests are shown in Table 1.

  EXPERIMENTAL RESULTS

     The overall  penetrations  for the ESP, the scrubber and the ESP
 scrubber system are shown in Table 1.   Since the particle size distribution

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Table 1.  EXPERIMENTAL CONDITIONS FOR ESP SCRUBBER EXPERIMENTS
Date
12/17/77
12/18/77
12/19/77
1/16/78
1/17/78
1/19/78
1/23/78
1/24/78
1/25/78
1/26/78
1/27/78
2/3/78
2/6/78
2/7/78
2/6/78
2/14/78
2/16/78
2/21/78
2/23/78
ESP
Penetration
0.05
ESP off
0.034
0.382
0.34
ESP off
ESP off
ESP off
ESP off
0.328
0.516
ESP off
ESP off
0.257
0.256
ESP off
ESP off
0.733
0.0375
Scrubber Parameters
Throat
Diameter, cm
10.16
10.16
10.16
10.16
10.16
10.16
10.16
10.16
10.16
10.16
10.16
7.62
7.62
7.62
7.62
10.16
10.16
10.16
10.16
L/G, m3/m3
1 X 10"3
1 X 10"3
1 X 10"3
1.2 X 10"3
1.2 X 10"3
1.2 X 10"3
1.2 X 10"3
2.3 X 10"3
2.3 X 10"3
2.3 X 10"3
2.3 X 10"3
1.2 X 10"3
1.2 X 10"3
1.2 X 10~3
1.2 X 10~3
5.32 X 10"4
5.32 X 10"4
5.32 X 10"4
-4
5.32 X 10
AP,cm H20
31.1
31.1
31.1
39.6
39.6
39.6
39.6
68.3
68.3
68.3
68.3
62.2
62.2
62.2
62.2
26.7
26.7
26.7
26.7
Penetration
0.0226
0.022
0.024
0.0129
0.0165
0.0106
0.010
0.0022
0.0020
0.0034
0.004
0.0041
0.0048
0.0072
0.0079
0.0235
0.019
0.0138
0.0911
Overall
Penetration
for System
0.00113
0.022
0.000816
0.0049
0.0056
0.0106
0.010
0.0022
0.0020
0.0011
0.0021
0.0041
0.0048
0.0018
0.0020
0.0235
0.019
0.010
0.0034

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into the scrubber depends on the penetration through the ESP, the overall
penetration results shown in Table 1 must not be used to determine the
effect of the ESP on scrubber performance.  Instead, the particle penetration
as a function of particle diameter (the graded penetration) curves for
the scrubber must be used to determine the effect of the ESP.  (The
graded penetration curve for a scrubber is independent of the inlet
particle size distribution.)

     The graded penetration curves for Phase 1 are shown in Figure 2 as
a plot of penetration versus aerodynamic particle diameter, dA.   (dA = d
/P C where d is the physical particle diameter, p is the density of the
particle, and C is the Cunningham correction factor.)  The predicted
graded penetration curve is also shown in Figure 2.

     The results of all the Phase 2 tests are shown in Figure 3.  The
average graded penetration curves for each of the Phase 2 tests are
shown in Figure 4.

     It is obvious from the data shown in Figures 2 and 4 that scrubber
performance is dominated by the pressure drop across the scrubber and
that the ESP has no effect on the performance of the scrubber.  It is
also clear from Figure 2 that the predicted graded penetration curve is
in excellent agreement with the experimental data.

     Statistical analysis of the data showed that:

          1.   There was no effect on scrubber performance due
               to the ESP.

          2.   Particle  collection  in the venturi was  dominated
               by pressure drop.

          3.   Changes in throat diameter  (i.e., changes  in  gas
               velocity  in the  throat) had more  effect than  changes
               in L/G.

          4.   The estimated standard deviation  in  the experimental
               graded  penetration  curves  was  about  20%.

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   1.0
                  1    I   I
T    I   I   I  I  I
1    I   I
I    I   t  I  I
o
H
  0.10
    01
             O MEASURED • ESP ON 12/17/77
                ESP PENETRATION = 0.05
               SCRUBBER Ap = 31.1 cm H20


             D SCRUBBER PENETRATION-PREDICTED
               SCRUBBER Ap= 31.1 cm H20


             A ESP OFF -MEASURED 12/20/77

               Ap=31.1cmH20


             • ESP ON-12/19/77

                ESP PENETRATION = 0.034
               SCRUBBER Ap = 3i.ic
                   I    1   1
 L   1   I  I   I  I  I
     0.1                                         1.0
                             AERODYNAMIC PARTICLE DIAMETER, micrometers

             Figure 2.  Graded penetration curves for venturi scrubber - phase 1  experiments.
                                                           10

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  0.10 —
o
t-
oc
                                                                                21 6/78
                                                                                21 7/78
                                                                                21 8/78
                                                                                2/14/78
                                                                                2/15/78
                                                                                2/21/78
                                                                                2/23/78
  0.010
  0.001
                                    1.0                            10

                                AERODYNAMIC PARTICLE DIAMETER, micrometers

              Figure 3.  Graded penetration curves for venturi scrubber - phase 2 experiments.

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   1.0
F 0.10
   0.01
                  1    I   r
                                           i    I   r
                                           I    I   I   IT
                                                      O ESP ON
                                                      D ESP OFF
                                                      • ESP ON
                                                        ESP OFF
                                                        ESP OFF
                                                        ESP ON
             I
I    I   I
                                                10.16 cm THRO AT
                                             - SCRUBBER AP =  39.6cmH20
                                             • SCRUBBER AP =  39.6 cm H20
                                             - SCRUBBER AP =  68.3 cm H20
                                             - SCRUBBER AP =  68.3cmH20
                                                 7.62 cm THROAT
                                             - SCRUBBER AP =  62.2cmH20
                                             - SCRUBBER AP =  62.2 cm H20
I    I   I  I   I  I  I
III     I    I   I   I   I  I
     0.1                                         1.0                                         10
                             AERODYNAMIC PARTICLE DIAMETER, micrometers
       Figure 4. Average graded  penetration curves for venturi scrubber - phase 2  experiments.
                                                10

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     ESP Scrubber System Performance

     The overall  mass penetration of the ESP scrubber system for each
run is summarized in Table 1.   Note that in all  cases the overall  mass
penetration is quite low; i.e., the overall mass collection efficiency
is quite high.

     Typical graded penetration curves for the ESP scrubber system are
shown in Figures  5 and 6.  These curves indicate that the ESP scrubber
system is capable of meeting the proposed revised New Source Performance
Standard.  In other words, a particle collection system operating with
the characteristics shown in Figures 5 and 6 can collect fly ash with a
typical size distribution with penetrations less than 0.003 (efficiencies
greater than 99.7%).

THEORETICAL ANALYSIS OF COMBINED ESP SCRUBBER SYSTEMS

     The data presented in previous sections clearly show that particle
collection by a scrubber is adequately modeled by Calvert's venturi
scrubber model.  ESP particle collection data show that the EPA/SoRI ESP
     5
model  adequately predicts ESP performance.  Therefore, the performance
of a combined ESP scrubber system should be adequately predicted by a
combination of the two models.

     The predictions of the two models were combined to obtain order of
magnitude estimates of the performance and economics of using an ESP
scrubber system as opposed to either an ESP or a scrubber alone.   In
essence such a system represents a tradeoff between scrubber pressure
drop and ESP plate area.

Two cases were examined:

          A low current density case which corresponds to a
          fly ash with high electrical resistivity  (^ 5 x 10
          ohm cm) such as produced by  low  sulfur coal (<1% S).
                                     11

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    0.10
                     I    I    I
   0.010
tu
z
tu
   0.001
       0.1
                     I  I  I  I  I
IIII\I   I   I  l_
                                                                         DATE OF RUN

                                                                         O 1/26/78

                                                                         n 1/27/78

                                                                         A 2/23/78
                     III     I    I   I   I   I  I  I
                               1.0


           AERODYNAMIC PARTICLE DIAMETER, micrometers


Figure 5.  Graded penetration curves for the ESP  scrubber system.
                              10
                                                    12

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  0.10
                                 I    I   I   I   I  1  I
                                                     I   I
I    I   I  I  I  L
F 0.010
  0.001
                                                                      DATE OF RUN
                                                                      O 2/7/78
                                                                      Q 2/8/78
I     111     I    I   I  I  I  I  I	|	I	LJ	I	I   I   I  I  I
                                   1.0                                          10
      0.1
                               AERODYNAMIC PARTICLE DIAMETER, micrometers

                    Figure 6. Graded penetration curves for the ESP  scrubber system.
                                                  13

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          A moderate current density case which corresponds
          to a fly ash with moderate electrical  resistivity
          (^3 x 10   ohm cm)  such as produced by moderate
          sulfur coals (^1.5-2% S).

The following assumptions were made:

     1.    The fly ash size distribution was log-normal  with
          mass mean diameter of 20 ym and geometric standard
          deviation of 4.5.

     2.    Fly ash density was  2.4 g/cc.

     3.    Gas flow distribution in the ESP was characterized
          by a normalized standard deviation of 0.25.

     4.    The factor for sneakage and nonrapping reentrainment
          in the ESP was 0.1.
                                                               5
     5.    Rapping losses were typical as described by McDonald.

The results of the calculations are summarized in Table 2.

     The results summarized in Table 2 show that the scrubber pressure
drop, AP, is a function of the penetration through the ESP,  T^fpcp*
and is essentially independent of the current density.  The  pressure
drop to PtpSp  relationship is:

                          AP = 85~PtESp                                (1)

where  AP is in cm water and H     is a fraction.
     Because the specific collector area, SCA, required to give a given
PtESP *s a funct^on °f tne current density, the relationship between AP
and SCA is different for the two current densities:
                                     14

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Table 2.  SUMMARY  OF  CALCULATED  RESULTS  FOR  ESP  SCRUBBER SYSTEM
Configuration
ID Number
ESP Parameters
SCA
m2/Am3/s Ft Resistivity
ScrubDer Parameters
P 	
cm water Pt
Overall
Penetration
1
2
3
4
5
6
7
8
9
10
11
156.1
78.04
33.93
16.43
8.214
74.32
35.47
15.30
7.094
3.393
0
0.0024 high
0.0165
0.0771
0.187
0.330
0.002 moderate
0.0164
0.0762
0.186
0.331
_ _
-
9.1
24.0
34
43
-
8
24
34
43
67
-
0.182
0.0389
0.016
0.009
-
0.183
0.0394
0.016
0.0091
0.0029
0.0024
0.003
0.003
0.003
0.003
0.002
0.003
0.003
0.003
0.003
0.003
                               15

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          For the high current density case,

                    AP = exp (3.94 - 0.0536 SCA)                             (2)

          For the low current density case,

                    AP = exp (3.90 - 0.0220 SCA)                             (3)

                                           2   3
For both,  P is in cm water and SCA is in m /Am /s.

     The calculated results show that the SCA can be reduced by about a
factor of 2 for both moderate and high resistivity cases, for a scrubber
AP of about 10 cm water.

DISCUSSION

     The initial reaction to the calculated and experimental results is
one of disbelief.  It does not appear reasonable to expect a fairly
inefficient ESP and a moderate to low pressure drop scrubber to perform
as well as both the experimental data and the calculated results
show. An examination of the particle penetration versus particle diameter
curves (the graded penetration curve) for both devices acting alone and
the combined graded penetration curve can explain  the results.

     The calculated graded penetration curve for an ESP with a penetration
of 0.0771 is shown in Figure 7.  Note that the ESP curve has a broad
peak from about 0.4 to 1 ym and then drops fairly  rapidly on both sides
of the peak.  On the other hand the graded penetration curve, Figure 8,
for a scrubber needed to produce an emission of 13 ng/J in combination
with the ESP drops rapidly from essentially 1.0 at 0.1 ym to less than
0.01 at 3 ym.  The scrubber is seen to be efficient in particle diameter
regions where the ESP is inefficient and the ESP is efficient in particle
diameter regions where the scrubber is inefficient.  The two devices
complement each other.

     The graded penetration of the ESP scrubber system can be obtained
by multiplying the two  separate graded penetration curves; i.e,.
                                        16

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    10
                             1—I   I   I  I  11
                                          i   r~i—i—i    iiiu
oc 0.10
  0.01
                              I    I   I   I  I  I  I
                                      I
I    i   I
I    I   I   I  I  I
     0.1
                              1.0
             PHYSICAL PARTICLE DIAMETER, micrometers
Figure 7.  Graded efficiency curve for ESP with penetration of 0.0771.
                                                                                     10
                                            17

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   1JJ
F0.10
  OKI
n — i    i   i   i   i
                                                                   rn — i    i   i  i  i  u
                                    J   1  I
                                            I   I
I   I  I  I
     0.1
                          1.0

         PHYSICAL PARTICLE DIAMETER, micrometer*
                                                                                            10
    Figures.  Penetration versus particle diameter for scrubber with pressure drop = 23 cm
    density - 2.4 g/cc.
                                                18

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             Pt(d)ESps = Pt(d)ESp x Pt(d)s                                  (4)

where

            Pt(d)ESps, Pt(d)ESp and Pt(d)s are the penetrations of
particles with diameter d for the ESP scrubber system, the ESP alone,
and the scrubber alone, respectively.  The resulting graded penetration
curve is shown in Figure 9.  Note the curve has a sharp peak at about
0.3 ym and drops rapidly on both sides.  This sharp peak  is characteristic
of the ESP scrubber system and, as is discussed in the section on plume
opacity, may cause problems with respect to plume opacity  limits.  (Note
that the curves in Figures 7, 8, and 9 are for penetration versus physical
particle diameter, not aerodynamic particle diameter as in Figures 2,  3,
4, 5, and 6.)

     The experimental graded penetration curves for the ESP scrubber
system do not  show the peak in  penetration because data for particle
diameters less than about  0.7 micrometers are not available.

COST ANALYSIS

     A detailed cost  analysis  is necessary to determine  if the trade  off
between  pressure drop and  SCA  is justified.

     The order of magnitude  cost analysis  involves  the following assumptions:

           1.   The  total  turnkey capital  cost of  a  cold-side  ESP is
               $30/m2 plate  area.   (A rough  range of  total turnkey
               cost is  $270  to $370  per m .)

           2.   There  is  no capital  cost of the  scrubber because it  is
               needed for SO  control.
                             A

           3.    Fan  efficiency is 60%.

           4.    Electricity cost is $0.03/kW hr.
                                         19

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 1.0
0.10
0.01
T—i—n—i—rr
                                                     T—i—n—\—i   i   i  i  L
          j	i	«   i     i
                                                            J	i   i  i   i  L
   0.1
                                                                                       io!
                             PHYSICAL PARTICLE DIAMETER, micrometers
Figure 9. Graded penetration curve for ESP scrubber system - ESP penetration = 0.0771 scrubber
pressure drop = 23 cm fO.
                                           20

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          5.    Annualized capital  charges are 15% of total  turnkey
               capital  cost.

          6.    Plant operates 6100 hrs per year (<\70% capacity).

          7.    ESP operating and maintenance costs are insignificant
               compared with capital costs of ESP and can be
               neglected.

          a.    Scrubber maintenance and liquid loop costs are not
               included because they are needed for the SO  system.
                                                          A

          9.    Costs are for 1 MW which produces 5440 Am /hr of
               flue gas.

With these assumptions the total annualized cost per MW is given by:

     AC = Q [4.38 x 10"3 HK  	Af_  ]   +0.15 CC                         (5)
                             15.8E
where AC is the annualized cost
       Q is the flow rate in Am /hr,
       H is the number of operating hours per year
      K  is the cost of electric power in $ per  kW hr
      AP is the scrubber pressure drop in cm ^0
       E is the fan efficiency
      CC is the capital cost in $
      4.38 x 10   and 15.8 are unit conversion constants

For a 1 MW plant:

       Q = 5440 Am3/hr
       H = 6100
      Ke = $0.03
       E = 0.60
      CC = 320 x  SCA x  Q
              3600
                                      21

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                                             2   3
where SCA is the specific collector area in m /Am /sec,  and 3600  is

                       3         3
necessary to convert Am /hr to Am /sec.





For the moderate resistivity case





          AP = exp (3.94 - 0.0536 SCA)





and for the high resistivity case





               AP = exp (3.90 - 0.022 SCA)





The cost equation for the moderate resistivity case is:





     AC = 5440 {[ 4.38 x 10"4 x 6100 x 0.03 exp (3.94 -  0.0536)]          (6)

                              15.8 x 0.6



               + 0.15 x 320  SCA}

                     3600



The SCA for minimum cost can be obtained from dAC/dSCA = 0.  For  the


moderate resistivity case:





_dAC  =  5440 [8.46 x 10"3 exp (3.94-0.0536 SCA) x - 0.0536 + 1.33 x 10"2]

dSCA



      =  4.53 x 10"4 exp (3.94 - 0.0536 SCA) + 1.33 x 10"2 = 0           (7)





 4.53 X 10"4 exp (3.94 - 0.0536 SCA) = 1.33 x 10"2           .            (8)





    3.94 - 0.0536 SCA^ - In frg * ftf                              (9)





     SCA.  = 3.94 - In 29                                               (10)

       ^"n     0.0536	



            =10.7 m2/Am3/sec





For the high resistivity case the only change is in the exponential  term


and


                 = 3.90 - In 71.4 =  - 0.37 m2/Am3/sec                   (11)
                                      22

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In other words the scrubber alone is the minimum cost option.   The cost
for the moderate resistivity case is:

          $2.1 x 103/year/MU

The cost for the high resistivity case is

          $2.3 x 103/year/MW

The maximum cost for the high resistivity case is for the ESP alone and
           2
is $11 x 10 /year/MW.  The maximum cost for the moderate resistivity
case is also for the ESP alone and is $5 x 103/year/MW.

     The cost picture is changed somewhat if a scrubber has to be purchased
for particulate removal.  In this case Equation 6 becomes

     AC = 5440 [ 8.46 x 10"3 exp (3.94 - 0.0536 SCA) + 1.33 x 10"2 SCA]   (12)

          + °'15 CCscrubber

for the moderate resistivity case and

     AC = 5440 L 8.46 x 10"3 exp (3.90 - 0.022 SCA) + 1.33 x 10"2 SCA]    (13)

          + °'15 CCscrubber

for the high resistivity case.  ccscruDber is tne capital cost of a
scrubber.  Ensor et al.  reported that the turnkey capital cost of a
particulate scrubber system is $50/kW or $50,000/MW.  The annualized
cost of the scrubber is 0.15 x $50,000 = $7,500 which must be added to
the minimum costs calculated earlier.  The annualized cost for the
moderate resistivity cases becomes $9,600 per MW per year, which
exceeds the cost of ESP alone. The annualized cost for the high resistivity
case becomes $9,800/MW/year which is still less than the cost of
the ESP alone.

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     It must be noted that the cost calculations above are based on
general cost data which have a great deal of uncertainty in them.
However, the cost calculations do show that once the decision to install
scrubbers for SO  control is made, the particulate collection job should
                A
be shared by the ESP and the scrubber.

PLUME OPACITY

     Theoretical calculations of in-stack light transmittance (1 minus
the plume opacity) as measured by a transmissometer are inexact due to
lack of data on particle refractive index and other parameters, especially
the particle size distribution.  However, useful estimates can be made
based on the work of Ensor.

     The in-stack plume opacity is a function of the particle size
distribution, the refractive index of the particles, the particle concen-
tration, and the optical path length.  Ensor has shown that the in-stack
light transmittance is given by

                    In (I/I ) =  WL                                         (14)
                                 KP
where I is the intensity of the light transmitted through the aerosol
      I  is the intensity of the light source  (I/IQ is the transmittance)
      W is the mass concentration of particles
      L is the optical path length which is usually the stack diameter
      K is a parameter which depends on the particle size distribution,
        the particle refractive index, and the wavelength of light
      p is the particle density

     A plot of K for a log-normal particle size distribution versus
geometric mass mean radius with geometric standard deviation as a parameter
for wavelength of light = 550 run and a refractive index = 1.50 is shown
in Figure 10.

     The graded penetration curves for the ESP, scrubber, and ESP scrubber
system can be used to estimate the log-normal  parameters for various system
                                       24

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                                       I    I  I I I III)
                                   REFRACTIVE INDEX = 1.50

                                   WAVE LENGTH OF LIGHT = 550 nm
                                       I'll ""I      1   I  I  I  II
                GEOMETRIC MASS MEAN RADIUS, rgw (microns)

 Figure 10. Parameter K as a function of the log-normal size distribution
 parameters for a white aerosol.
(§} D.S. ENSOR USED BY PERMISSION OF COPYRIGHT OWNER
                                25

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     Table 3.  ESTIMATED LIGHT TRANSMISSION  AND  IN-STACK PLUME OPACITY
              FOR ESP SCRUBBER SYSTEMS
Configuration*
ID Number
1
2
3
4
5
11
System
ESP alone
ESP & Scrubber
ESP & Scrubber
ESP & Scrubber
ESP & Scrubber
Scrubber alone
Transmission
'"o
0.85
0.63
0.70
0.73
0.76
0.80
Opacity
1-I/I0
0.15
0.37
0.30
0.27
0.24
0.20 ^
Configuration ID number refers to Table 2.

All systems produce outlet emission of 13 ng/J.
                                     26

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configurations that meet the 13 ng/J emission limit.  These log-normal
parameters can then be used to estimate K from Figure 10.  The light
transmittance can then be calculated from

               I/I0 = exp (-WL/Kp)                                     (is)

We will assume W = 0.02 g/Am3 (roughly equivalent to 13  ng/J)
               L = 10 m
               P = 2.4 g/cc

The estimated light transmittance for each of the system configurations
in Table 2 is shown in Table 3.  Because the particle size distributions
of the ESP scrubber system are essentially the same for  both the moderate
and high resistivity cases when the ESP penetration is constant, only
results for the high resistivity cases are shown in Table 3.

     The estimates of transmittance show that the ESP scrubber system
can have considerably lower transmittance (higher opacity) than either
the ESP-only system or the scrubber-only system.

     It must be noted that these calculations of transmittance are subject
to large uncertainties; e.g., the calculated outlet size distributions
are not exactly log-normal.   The ESP computer model predictions of graded
penetration curves are not well confirmed with experimental data.  Slight
changes in the non-ideal  factors in the ESP model can have a large effect
on the predicted outlet size distribution, which will affect the calculated
transmittance.

     In spite of the uncertainties in the calculations,  the fact that ESP
and scrubbers operate on the particle size distribution  differently will
tend to make the outlet particle size distribution finer and more monodisperse.
This tendency to make a fine monodisperse outlet particle size distribution
should cause higher opacities for a given mass emission.
                                      27

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REFERENCES

     1.   Sparks, L. E., "The Effect of Scrubber Operating and Design
Parameters on the Collection of Particulate Air Pollutants."  Ph.D.
Dissertation, University of Washington, 1971.

     2.   Sparks, L. E., "SR-52 Programmable Calculator Programs for
Venturi Scrubbers and Electrostatic Precipitators," EPA-600/7-78-026
(NTIS PB 277-672/AS), March 1978.

     3.   Lawless, P., G. Ramsey,  and B. Daniel, "Characterization  of
the IERL/RTP Pilot Scale Electrostatic Precipitator."  EPA report in
press, 1978.

     4.   Calvert, S., C. Lake, and R. Parker, "Cascade Impactor Calibration
Guidelines," EPA-600/2-76-118 (NTIS PB 252-656/AS), April 1976.

     5.   McDonald, J. R., "Modeling and Programming the Electrostatic
Precipitation Process."  EPA report in press, 1978.

     6.   Ensor, D. S., B. S. Jackson, S. Calvert, C. Lake, D. V. Wallon,
R. E. Nilan, K. S. Campbell, T. A. Cahill, and R. G. Flocchini, "Evaluation
of a Particulate Scrubber on a Coal-Fired Utility Boiler."  EPA-600/2-
75-074 (NTIS PB 249-562/AS), November 1975.

     7.   Ensor, D. C., "Smoke Plume Opacity Related to the Properties
of Air Pollutant Aerosols."  Ph.D. Dissertation, University of Washington,
1972.
                                       28

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                                TECHNICAL REPORT DATA
                          (Please read Instructions on t/ie reverse before completing)
. REPORT NO.
EPA-600/7-78-193
                           2.
             3. RECIPIENT'S ACCESSION NO.
. TITLE AND SUBTITLE
Particle Collection by a Venturi Scrubber Downstream
from an Electrostatic Precipitator
             5. REPORT DATE
              October 1978
             6. PERFORMING ORGANIZATION CODE
 AUTHOR(S)

 j.E.Sparks, G.H.Ramsey, andB.E.  Daniel
                                                       8. PERFORMING ORGANIZATION REPORT NO.
              IERL-RTP-612
. PERFORMING ORGANIZATION NAME AND ADDRESS
                                                        10. PROGRAM ELEMENT NO.
                                                        EHE624
See block 10
              11. CONTRACT/GRANT NO.

              NA (Inhouse report)
 2. SPONSORING AGENCY NAME AND ADDRESS
 EPA, Office of Research and Development
 Industrial Environmental Research Laboratory
 Research Triangle Park, NC  27711
              13. TYPE OF REPORT AND PERIOD COVERED
              Final; 12/77 - 2/78
              14. SPONSORING AGENCY CODE
               EPA/600/13
15.SUPPLEMENTARY NOTES Coauthor Sparks'  mail drop is 61; his phone is 919/541-2925.
             repOrt gjves results of pilot plant experiments of particulate collection
   a venturi scrubber downstream from an electrostatic precipitator (ESP). The data,
covering a range of scrubber operating conditions and ESP efficiencies, show that
particle collection by  a venturi scrubber is not affected by the upstream ESP; i. e. ,
for a given scrubber pressure drop, particle collection efficiency (as a function of
particle diameter) is the same whether the ESP is on or off. The experimental  results
are in excellent agreement with theoretical predictions.  Order of magniture cost
estimates indicate that particle  collection by ESP scrubber systems is economically
attractive when scrubbers must be used for  SOx control.
17.
                              KEY WORDS AND DOCUMENT ANALYSIS
                 DESCRIPTORS
                                           b.lDENTIFIERS/OPEN ENDED TERMS
                           c.  COS AT I Field/Group
Air Pollution
Dust
Scrubbers
Venturi Tubes
Electrostatic Precipitators
Sulfur Oxides
  Air Pollution Control
  Stationary Sources
  Particulate
  Venturi Scrubbers
13B
11G
07A,13I
14B

07B
18. DISTRIBUTION STATEMENT

 Unlimited
  19. SECURITY CLASS (This Report)
  Unclassified
21. NO. OF PAGE?
    34
  20. SECURITY CLASS (This page)
  Unclassified
                           22. PRICE
EPA Form 2220-1 (9-73)
29

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