r/EPA
             United States
             Environmental Protection
             Agency
              Office of Radiation Programs
              Las Vegas Facility
              P.O. Box 15027
              Las Vegas NV 891 14
ORP/LVF-79-1
November 1978
             Radiation
Radioactivity in Selected
Mineral Extraction
Industries
A Literature  Review

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                                                                Technical Note
                                                                ORP/LV-79-1
           RADIOACTIVITY IN SELECTED MINERAL EXTRACTION INDUSTRIES
                             A LITERATURE REVIEW
                               James D. Bliss*
                                November 1978
                     U.S. Environmental Protection Agency
                         Office of Radiation Programs
                              Las Vegas Facility
                           Las Vegas, Nevada 89114
*Now with the U.S. Geological Survey, 920 National  Center, Reston, VA 22092

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                                   PREFACE
    The Office  of Radiation Programs  of the Environmental  Protection  Agency
carries out  a national  program  designed to  evaluate  population exposure  to
ionizing and  non-ionizing radiation,  and  to promote development of  controls
necessary to protect the public health and safety.   This  literature  survey was
undertaken to identify  possible  sources  of ionizing radiation in the mineral
extraction  industries  (excluding  uranium and  phosphate).    The information
gathered during  the survey  is also  serving  as a  guide in planning  further
studies to meet  the  requirements  of the Clean  Air  Act  (as  amended  in  1977).
Readers  of this  report  are  encouraged  to  inform  the  Office  of  Radiation
Programs  of  any  omissions  or errors.    Comments  or  requests  for  further
information are also invited.
                                    Donald W.  Hendricks
                                    Director,  Office of
                                    Radiation  Programs, LVF
                                      2.2.

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                                   ABSTRACT
    The mining, milling, and processing of mineral  resources may cause varying
degrees of technologically  enhanced  natural  radioactivity  (TENR)  which is de-
pendent on the inherent uranium and thorium content of the target resource and
the details of the total extraction process.
    The objective of  this  review is  to  identify from the  available domestic
literature  possible  metallic  and nonmetallic  mineral  extraction  industries
(exclusive of  uranium, phosphate, and  fossil fuels)  which may  require  sub-
sequent assessment.   Certain industries such as phosphate and coal are already
identified as  potential sources  of  radioactivity;  hence,  they  are  excluded
from this overview.
    Uranium  and thorium  content  is a  useful  first  order measure  of  the
radioactivity a mineral commodity may contain.  This, in turn, is dependent on
the gross  geochemical  characteristics and geological history of  the  ore  body
of concern.   The observed  variability  of uranium and thorium  content is de-
pendent not only on mineral genesis  but also  on  the  local  geological  setting.
This along  with the  absence  of  many direct observations  prevents  confident
selection of mineral  commodities with consistently  large TENR.   However, the
following  metallic  commodities  should   be  subject  to  further  exploratory
inspection:   rare-earth elements, gold,  iron,  molybdenum,  copper,  aluminum,
and lead-zinc.   Among  these,  mining and  milling of molybdenum  and  gold  ores
have been associated with the  largest radiation  levels in air  and water, re-
spectively.  Placer deposits of any metal  should be inspected for radiation

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related  to  the  thorium  decay chain.   Similarly,  resources  which  are  the
residual  results of weathering should be evaluated.   Nonmetal  resources  which
appear to  have the  greatest  potential  of TENR  are fluorspar, granite,  and
clays.    Underground   operations   in  most  any  material  may  have  elevated
radioactivity  as  is  the  case  for caves  in limestone, which  consistently is
among the rocks having the lowest  associated radioactivity.   Radiation surveys
should involve the  uranium and   thorium  decay  chains and  other  naturally
occurring radioisotopes  as  applicable.   Secondly, each  operation should  be
surveyed, restricting  generalizations  to  the same geological  province and to
deposits  with similar local  geology,  mineralogy,  and  genesis.
                                      IV

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                       TABLE OF CONTENTS
                                                        Paqe
PREFACE                                                   ii
ABSTRACT                                                 iii
LIST OF TABLES                                           vii
ACKNOWLEDGMENTS                                         viii
INTRODUCTION                                               1
GEOCHEMISTRY OF URANIUM AND THORIUM                        4
  Introduction                                             4
  Igneous Rocks                                            6
  Residual  Igneous Rocks                                   8
URANIUM MINERALS IN METALLIC ORE DEPOSITS                 11
  Summary                                                 16
WEATHERING AND SEDIMENTARY CYCLE                          17
  Introduction                                            17
  Resistate Deposits                                      18
  Residual  Deposits                                       21
  Organic Matter Associations                             21
MINERAL EXTRACTION AND RADIOACTIVE BYPRODUCTS             23
RADIOACTIVITY MEASUREMENTS ASSOCIATED WITH
 MINING OPERATIONS                                        25
SUMMARY                                                   31
  Conclusions                                             31
  Recommendations                                         33
REFERENCES                                                35

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APPENDICES
  A.  Radiological  Data for Selected
      Metallic Commodities                                42
  B.  Radiological  Data for Selected
      Nonmetallic Commodities                             45
  C.  Glossary of Geological  Terms Used                   46
TABLES                                                    50
                                vi

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                       LIST OF TABLES
Number                                                  Page

  1  Uranium and Thorium Content of Minerals              50
     Found in Igneous Rocks

  2  Generalized Distributions of Uranium in              50
     Various Groups of Igneous Rocks

  3  Uranium and Thorium Content of Selected              51
     Sedimentary Rocks

  4  Summary of Radiological Information on               52
     Metallic Commodities Given in Appendix A

  5  Summary of Radiological Information on               53
     Nonmetallic Commodities Given in Appendix B
                               Vll

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                               ACKNOWLEDGMENTS

    I wish to  thank the staff  of the Office of Radiation  Programs-Las  Vegas
Facility  for  their  assistance,  criticisms,  and  suggestions  during   the
preparation of  this report.   I  am  appreciative  of the  help provided by  C.
Robbins, Office of Radiation Programs-Headquarters;  R.  Rock, Mining  and Safety
Administration  (now Mining  Safety  and  Health Administration);  A.  Goodwin,
Mining Safety and  Health Administration,  in supplying technical  information;
and  to  A. Tanner  and J.  Stuckless  of  the U.  S.  Geological  Survey and  R.
Kaufmann, ORP-LVF, for taking the time to review this  report and for providing
numerous criticisms and suggestions.   A special thanks to  Mr.  David  Ball  for
his graphic and artistic contribution particularly  in  preparation  of the  cover
illustration and to Mrs. Edith  Boyd  and  Ms.  Sandi Graves  for assisting in  the
typing.
                                    Vlll

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                                 INTRODUCTION
    In order to establish radiation  protection  guidance,  the Office of Radia-
tion Programs (ORP) of the U. S. Environmental  Protection Agency (USEPA) makes
a continuing  effort  to identify  source  categories of radiation.   An  area of
increasing interest involves the  identification  of enhanced  human  exposure to
ambient  radiation  and  radioactive   material   resulting   from  various  human
activities  that  concentrate or  redistribute   radioactive  material  in  the
earth's crust.

    This brief  review  is  intended as an overview  document which will  support
ORP efforts under the Clean Air Act as amended in 1977.  This review is not to
be considered inclusive and  primarily will  address readily available domestic
literature  only.    Secondly,  a  substantial  amount   of  current  information
germane  to  this  report  on  uranium and  thorium  concentrations   in  various
geological materials is unpublished.  Some of the observations given herein are
admittedly dated  but  are  included for lack of  more recent information.   This
report  primarily  provides  some  background  information  on  which  further
investigative activities can be based.

    Of the  approximately  one hundred naturally  occurring radionuclides, about
thirty (most of which are members of the uranium and thorium decay series) are
of interest due to their abundance and toxicity  (Conference of Radiation

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Control  Program  Directors,  1977).   Natural  radiation  is  by far  the  largest
source of  human  radiation exposure  to the  world  population (United  Nations
Scientific Committee  on the  Effects  of Atomic  Radiation,  1977).    The  major
portion  of this exposure is unavoidable.   However, as a result  of industrial
activities and  changes  in  modes  of  living due  to technological  advances,
increased  exposures  to  naturally occurring  radioactive materials  can  take
place.  This process has been designated  as  "Technologically Enhanced  Natural
Radiation" or TENR (Gesell  and Prichard, 1975).

    Extraction and processing of  mineral  commodities may enhance  exposure  of
humans to  natural radioactivity in several ways.   Workers  located  in or adja-
cent to mining sites  can be   exposed to gamma radiation  from the  ore  body  as
well as the surrounding  rocks.  Exhalation of radon gas  from exposed surfaces
can result in  an inhalation  hazard  to mine workers,  particularly  in  under-
ground  operations.    Beneficiation,   involving  such  operations  as  grinding,
washing, flotation, drying, or  chemical  extraction, can redistribute  or con-
centrate  radioactive  material in  tailings,  byproducts,  products,  or  wastes.
Tailings may become a  hazard  if used  in  construction  or reclamation.   Waste
water may  contaminate  surface water  or find its way  into ground water.   Pot-
able water supplies may be  contaminated and result in radiation  exposure  to
users.  If radioisotopes are  concentrated  in a  product  or  byproduct, exposure
can result when  this  material is  fabricated into  a consumer product  and  ul-
timately  located  in close  proximity  to  humans in  either   the  home or  work
place.   However,  this  facet  is not  within the  scope  of the study  presented
herein.

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    Occupational and public radiation exposures  as  a  result of uranium mining
and milling have been documented and were initially investigated in this coun-
try in the early 1950's.   Studies  of radiation  exposure associated with cer-
tain phosphate  mining  and  processing operations have been  conducted  by Spal-
ding  (1972),  Guimond and  Windham  (1975), and  the U. S.  Environmental  Prot-
ection Agency  (1973).   In  many  respects,  exposure  to  elevated  levels  of
radioactivity as  a result  of  phosphate  extraction  has  occurred in  a manner
similar to that from uranium extraction.  Exposure can occur via inhalation of
radon gas and its  radioactive  decay  products  in enclosed areas (USEPA, 1975),
direct exposure to gamma  radiation  from solid  waste and  byproduct  material
(Duncan et al., 1977), and  ingestion  of water from  supplies  which  have ele-
vated radioactivity (Kaufmann and Bliss, 1977).

    These and other  findings  have  led  to this attempt  to  identify  potential
sources of radiation exposure  resulting from  mineral  commodity extraction and
production operations.  As  a first step, the present study  attempts  to indi-
cate, through an examination of  the  domestic  literature, those minerals which
may be expected to be  associated  with  increased concentrations  of  naturally
occurring radioactivity.  Emphasis  is on resource development (mining, proces-
sing) rather than on product or byproduct use by the consumer.

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                     GEOCHEMISTRY OF URANIUM AND THORIUM
INTRODUCTION

    The movement  of  uranium,  thorium,  and associated elements in the earth is
part of a natural  geochemical  cycle between rock, water,  and air.  While human
dose  assessment  is  one  of the  ultimate concerns,  the  understanding  of  the
enrichment  processes  of  radioactive elements  in the  lithosphere has  direct
application  in  defining  extractive  mineral   ore   bodies  which  may  show
preferential enrichment in radioactivity.

    The behavior  of  uranium and  thorium is dependent on  the outer  electron
configuration.  For  example,  thorium is  analogous  to the rare-earth  elements,
with an incomplete 5f shell.   A  valence state of 4+ is dominant with  3+ or
2+  states  occasionally  noted.    Only  the  tetravalent state is  observed  for
thorium  under  natural  surface conditions.    In  general,  thorium  compounds
exhibit low solubility.  The thorium ion in solution is small, highly-charged,
and forms  an extensive  number of complexes  (Ames  and  Rai, 1978).    In  the
tetravalent state the ionic radius is similar to U+ and Ce+.

    Uranium  has  been identified  as  forming  about  103  distinct  minerals.
Uraninite  is the most  commonly  identified  ore  mineral.    Many  secondary
minerals can be formed  including  sulfates,  silicates, phosphates, molybdates,

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and vanadates as well  as multiple oxides (Ames and Rai, 1978).  Generally, the
geochemistry of uranium is intimately associated with thorium, particularly in
the distribution  in igneous  rocks.   However,  significant  separation  between
the two  elements  does  occur  during  weathering, transport, and  deposition in
the sedimentary cycle (Rogers and Adams, 1969b).

    The overall similarity in size, electron configuration, and bonding nature
of thorium,  cerium,  uranium, and  zirconium promotes  geochemical  association
with  various  other elements  (Bayer,   1974).    These  associations  provide
valuable keys  to  defining  possible  ores and  products or  byproducts  wherein
there  is  enrichment  of  radioactive  elements.    Many  observed  elemental
assemblages  can  be   predicted   by   noting  similarity   in   outer   electron
configurations and other relevant properties as noted above.

    Two broad processes whereby radioactive elements relate to the geochemical
cycle  include  igneous   differentiation and  sedimentary  deposition.    Both
processes  can cause  reconcentration of radioactive  elements.    For  igneous
rocks, differentiation  by fractional crystallization  of  magma is one  of the
primary  processes  for  partitioning elements.    Certain  late  crystallizing
minerals, e.g., potassium and sodium feldspars  and  quartz,  may be enriched in
trace elements (including uranium  and thorium)  due  in  part to their increased
concentration in the magma  from which these minerals  crystallize.   Secondly,
gases and  fluids  expelled from  cooling magmas are thought to be responsible
for  the  formation  of  many  metallic  ore  deposits,  particularly  those  of
hydrothermal  origin.    Occasionally,   surface  or   ground  water  remobilizes
uranium and other metals and redeposits  them as secondary minerals or
secondary ore deposits.  Other concentrating mechanisms occur in the

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sedimentary cycle and particularly  involve minerals  containing  thorium.   Many
of these  minerals  are  resistates,  i.e., minerals  resistant  to chemical  and
physical weathering, as well as being characterized  by  high  specific gravity.
Because of  these  properties, thorium minerals,  when introduced into  dynamic
water bodies, may form  placer  deposits.  Another  site  of enrichment involves
the concentration of uranium by organic  or organically derived material.   This
accounts  for the  association  of  uranium  with  humates, coal  (particularly
lignites), oil,  and  peat.
IGNEOUS ROCKS

    While uranium and thorium are  observed  in  all  major rock forming minerals
(Table 1), the mechanics  of  location within the mineral  are  largely unknown.
Generally, the mafic minerals, i.e., those enriched in magnesium and iron, are
also  enriched  in  uranium  and  thorium;  but  there  are  many  exceptions.
Accessory minerals,  i.e.,  minerals occurring  in  small  quantities  in  a  rock,
are usually greatly enriched in uranium and thorium, particularly in granites.
Accessory minerals particularly enriched in thorium are allanite and monazite.
Xenotime is enriched  in  uranium.   The  common  accessory minerals,  zircon  and
sphene, generally  have  a  low Th/U  ratio  of 1 to 2 which  may be  either  an
expression of early magmatic composition or differential enrichment of uranium
(Rogers and Adams,  1969a).   The St. Francois  Mountains of Missouri are  noted
as  being  enriched   in  uranium  (10  to  30 ppm)  and  investigation  of  its
petrography by Mash  (1977,  p. 30)  revealed  that 80  percent  of the uranium is
located as rims about magnetite  crystals.   Lesser  amounts  are associated with
the biotite.   Stuckless  et  a!.,  (1977)  noted similar patterns  in magnetite

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crystals at  Granite Mountain,  Wyoming.   The  biotitic phase  is  particularly
enriched in  uranium.   They  calculate  an  average  uranium concentration  of
9.8 ppm but if suggested levels of uranium loss are correct, the rock may have
contained an average of as much as 30 ppm uranium.   The content  is  highest  in
the accessory  minerals zircon,  sphene,  and monazite  with lesser  amounts  in
epidotes, apatites  and biotitic/chloritic  alteration  products  (Stuckless  et
al., 1977).   They  also noted  that uranium was  not obvious in  either inter-
granular borders or in fractures.

    Before making  generalizations  on igneous  rocks,  it  should be  noted  that
some geographic  areas  have an  overall  elevated  concentration of  uranium and
thorium  regardless  of  rock type or  geological age.   Such areas  include the
Rocky Mountain  Front  (Phair and Gottfried,  1964)  in Colorado  and  part of New
England  (Rogers  and Adams, 1969a).   Portions  of  central  Wyoming  as  well  as
parts  of the Colorado  Plateau may  also  fall  into  this  category  (Stuckless,
written communication, 1978).  Putting such  geographic variability aside,  ura-
nium content increases  as  the  silica  content  increases.   This  property is the
result  of  uranium  exclusion  from  early minerals and  rocks  formed  in  the
processes of  magmatic differentiation.   Whether  intrusive or extrusive, ig-
neous rocks tend to show similarity in uranium and silica  distribution.  While
individual  rock  suites commonly exhibit uranium enrichment  in  later members,
it is not universal (Rogers and Adams, 1969a).   Thorium generally exhibits the
same  geochemical  trends   in  petrological   evolution  as  uranium (Rogers  and
Adams,  1969b).   Thorium is also closely tied  to  potassium with a  K/Th  ratio
"nearly  constant...in  a large  variety of  igneous rocks"  (Heier  and  Rogers,
1963).

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RESIDUAL IGNEOUS ROCKS

    Pegmatites, possibly the last residual  portion  of  a  magma  to crystallize,
often move some distance from the parent  magma.   Enriched in a  wide  range  of
elements not  easily  incorporated into common  minerals of the  cooling  magma,
pegmatites have been used as a  source of many rare metals  including  lithium,
beryllium,  scandium,  rubidium,  yttrium,  zirconium, molybdenum,  tin,  cesium;
the rare-earth elements, columbium (niobium), tantalum, tungsten, thorium, and
uranium.    Industrial   minerals  produced  from  pegmatites  include  feldspar,
muscovite, phlogopite, tourmaline, and quartz (Mason,  1966;  Bates, 1960).

    Pegmatites are a  complex  group  of rocks containing  diverse mineralogical
and  compositional  members.   The largest pegmatite mines  and the only ones
which have  operated  on  a more or less  continuous basis  are those  extracting
feldspar  (Bates,  1960).  Mica,  spodumene,  and beryl   are often important by-
products.   Production  is greatest in North  Carolina with substantial  produc-
tion  also  in  California,  South  Dakota,  and  Colorado.   Usually,  domestic
pegmatites  are not  considered  a commercial  source of  uranium  and  thorium.
However,  pegmatites   having  significant  amounts of  uranium  stimulated  some
interest  in  the past (Lang,  1952;  Page, 1950)  and Charbonneau  and  Jonasson
(1975) more recently referred to "radioactive pegmatites" in Ontario.
Garside  (1973)  indicates that uranium, thorium,  and  rare-earth  minerals are
common  accessory  minerals  in  pegmatites.    He  noted 33 so-called  radioactive
pegmatites occur  in  Nevada.  Similar  occurrences  of radioactive minerals were
observed in pegmatites  around Kingman, Arizona (Peirce et al.,  1970).
                                       8

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    Uranium content appears to  be  strongly  related  to potash feldspar content
of the pegmatites (Page, 1950).  This appears to be  a logical  continuation  of
the geochemical  behavior  of uranium and  potassium  as observed  in  common  ig-
neous rocks.   Radioactivity  in pegmatites can  have  a broad regional  impact.
DalTAglio (1971) examined the  uranium content  of water  in the Italian Alpine
range and found anomalous  areas.  Subsequent radiometric  surveys  revealed that
the source was  pegmatites  which contain 3 to 10 times the background uranium
content.

    Carbonatites  are   particularly enriched  in  a  wide  range  of  elements
including rare-earth elements (lanthanides and yttrium).   Deposits at Mountain
Pass, California, constitute a major reserve of  these materials.   This deposit
also contains the thorium minerals thorite and bastnaesite and  less  frequently
monazite and allanite  (Staatz,  1974).  The  vein was  initially  investigated  as
a  result  of elevated  radioactivity.   Nininger (1955) noted  that  thorium  is
found in a number of rare-earth minerals and identified Mountain Pass among  13
important thorium-bearing vein  deposits in  the  United States.   Association  of
rare-earth elements, uranium,  and  thorium has  been observed in  vein deposits
in the  Bokan Mountains of Alaska.  Geological  investigations  by M. H. Staatz
(1977)  revealed  that some  of these veins are traceable  for about  2.8  km  and
that  uranium  content   varies   from  0.005  to  2.8  percent  while  rare-earth
elements and thorium concentrations vary between a  few hundredths of a percent
to over 10  percent.   Enrichment of barium,  beryllum,  niobium, strontium,  and
zirconium has  also been  noted  in these  deposits.    Because  of  the  common
associations of  rare-earths  and thorium,  extraction of one  could involve  the
extraction  of  the  other   as   a   byproduct  or possible  enrichment  in  the
processing of wastes.

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    While of minor  importance,  another radiation  source may be  from  several
rare-earth  elements   which  have   radioisotopes   including   lanthanum-138,
neodymium-144,  samarium-147, and lutetium-176 (Lowder  and Solon, 1956).

    In summary, residual rocks  like pegmatites may  be enriched  in uranium and
thorium,  particularly  if the potassium  content  is high.    Carbonatites  with
substantial  rare-earth content appear to be somewhat radioactive.
                                        10

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                  URANIUM MINERALS IN METALLIC ORE DEPOSITS

    Two approaches can  be  taken in analyzing uranium  distribution  in  mineral
deposits.   One  is  to observe associations in uranium  ore  deposits.   This can
help to define  geochemical  affinities  which  may be applicable  to  other types
of commodities  and ore deposits.   The second is  to observe  uranium minerals
which  occur  in  other  types  of  ore  deposits  and thereby  define  potential
radioactive hazards in other mineral extraction operations.

    Many major metallic deposits  are believed to  have  been generated by gases
and  liquids  moving away  from  cooling  magmas.    Deposition  of minerals  from
these fluids involves complex processes with definite geochemical  associations
among  resulting  mineral and element  assemblages.   In examining  uranium ore
deposits,   several  classifications have  been developed based  upon persistent
mineralogical and  chemical  associations.   McKelvey (1955) classified  uranium
vein deposits  into three principal mineral  groups:   (1)  nickel-cobalt-native
silver-pitchblende,   (2)   pyrite-galena-pitchblende,   and  (3)   uraniferous
fluorite veins.  Everhart (1956) also identified three  types  of deposits:   (1)
siliceous-pyrite-galena (a type of major importance),  (2)  nickel-cobalt-native
silver, and  (3) gold bearing  pyrite.   Everhart and Wright  (1953)  noted  that
epigenetic  uranium deposits are  more  likely  in  veins  containing  either  a)
cobalt, nickel, and silver or b) copper, lead, zinc, and silver.

    Direct mineral  associations with uranium deposits may occur within the ore
body or on a regional basis.   In  the  Coeur d'Alene mining  district,  uranium
                                        11

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deposits are  spatially associated with  silver  and base metal  ores  but exact
genetic association  is uncertain  (Butler and  Schnabel,  1956).   Uranium  de-
posits occur  as  part  of the  metal  assemblage of ore deposits  in  the central
mineral belt of Colorado (King et al., 1953), whereas those in the Front Range
of  Colorado  are usually  associated  with molybdenum.   Within  this  province,
molybdenum is  used as  a  geochemical indicator  of possible  uranium deposits
(Ferris and Bennett,  1977).   A similar  relationship  has  been observed in the
Marysvale, Utah, district (McKelvey et al., 1955).

    McKelvey et al. (1955) noted that the list of metallic minerals found with
uranium vein deposits  is extensive.   In  their judgment, iron minerals are the
most "nearly universal and conspicuous"  association.   The  iron  mineral may be
pyrite or marcasite but finely dispersed hematite is considered to be poten-
tially  indicative  of  uraninite  association.    Magnetite  is  found  associated
with  pitchblende  at Maryvale,  Utah, whereas some  magnetite deposits  in  New
Jersey and New York have trace amounts  of  uraninite.  In  general,  "...large
magnetite  iron  ore  bodies   of  the  world  are  not  abnormally  radioactive"
(McKelvey et al., 1955).

    The second most common metallic element  associated with uranium deposits
is copper.  Most common copper  minerals  have  been observed with uraninite ore
types.   Uranium minerals are  also  commonly  associated with  those containing
cobalt  which   is  an  important  geochemical  indicator, particularly  for  the
Ni-Co-Ag uranium ore type (McKelvey et al., 1955).

    Lead  is  the next  metal  in  abundance in  uranium deposits.   Galena is the
principle  mineral   observed,  but   "...lead-bearing   veins   are  singularly
                                       12

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nonradioactive"  (McKelvey  et  al.,  1955).   After lead in  abundance  is  nickel
which,   when   associated   with   uranium,   is   generally   restricted   to
cobalt-nickel-silver  ore  types.   Nickel  deposits not  characterized by  the
cobalt-silver association are not usually observed to  be  particularly radioac-
tive.

    Minerals containing silver tend to  coexist with uraniferous  veins but  are
zoned in  such  a  fashion  that the  association  is more  regional  than  local.
Although  zinc  is  also  found  in  uraniferous veins,  "...many rich  zinc  ores
throughout the world are nonradioactive" (McKelvey et  al., 1955).

    Other  metal lies  of note  are molybdenum,  native  bismuth,  titanium,  and
vanadium.   Molybdenum minerals are observed  in  the Marysvale district,  Utah
and in other mining districts.  Occurrence  is more likely  in  the  Si-Fe-Pb  ore
type.    Native  bismuth  is generally  restricted  to  the  Co-Ni-Ag   ore  type.
Bismuth  ores  tend  to  be slightly  radioactive.    Titanium  occurrence   is
localized  and   tends  to  occur together  with uranium  in  the  same  mineral,
davidite.  Vanadium is sporadically present and  most  common in low temperature
uranium deposits.  Carnotite, a potassium-uranium vanadate, is the most
common mineral  (McKelvey et al., 1955).

    Uranium minerals  have  been observed  in  a  variety  of  hydrothermal metallic
ore  deposits.  Butler and  Schnabel  (1955)  indicated  that  uranium  was  found
associated  with  base metal  sulfides  and precious metals  in several  western
states and Michigan.  Usually reserves of uranium are  low,  typically  less than
1000 tons  of uranium  ore  (of  unspecified  grade).   Traces  of uranium  have been
found with  gold  and  zinc  minerals (Leonard,  1952).   Investigation of mercury
                                        13

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deposits in the  McDermitt  caldera in Nevada-Oregon by  Rytuba  (1977)  revealed
that associated opalitic material  contained up to 520 ppm uranium.

    Uranium is also observed  in  iron formations.  Everhart  (1956)  noted  that
uraninite is associated with  various  iron  minerals  in the iron-bearing strata
and quartzite  of upper Huronian  age metasediments in  Michigan.    Uranium  in
iron formations  is  often associated  with  copper, lead,  and zinc  (Butler and
Schnabel, 1956).  While uranium may occur with iron minerals, thorium has  been
observed as detrital grains of monazite in the associated metasediments as ob-
served  in  rock dumps of  abandoned iron mines  in Marquette County,  Michigan
(Vickers, 1956).   The Old  Bed  Mine, a magnetite deposit  near Mineville, New
York,  has  thin  seams  of  fluorapatite  "usually rich  in thorium  and  rare-
earths." Similar type  deposits  exist  elsewhere in  the area  (Twenhofel  and
Buck, 1956).

    Uranium minerals  in the  Camp  Smith area of  New  York occur in  a  complex
sequence of  Precambrian metamorphic  rocks.   Uraninite  occurs  in  association
with several lithologies as well as with a massive strata-bound Cu-Ni ore  body
(Grauch  and  Campbell,  1977).     Popenoe  (1966)  noted  that   a  major  aero-
radioactivity   anomaly   was  associated  with   a  mine  positioned   on   the
sulfide ore body.

    The  strongest  association  of  uranium  with  gold  tends  to  occur  in
metasediments,  particularly  conglomerates.    Vein deposit  associations   are
infrequent  but  have  been  observed   in  the  Front   Range   of   Colorado.
Metasediment deposits  include the Missisagi  Conglomerate of the Blind  River
District,  Ontario  and  the  Witwatersrand  Conglomerates  in  South  Africa.
                                       14

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The occurrence of uraninite  in  the  Witwatersrand gold deposits of Precambrian
age was first noted  by  Cooper  (1923).   Subsequently  it was  determined  that a
frequently   observed   ore   component   referred  to   as   "carbon"  was   an
uraninite-carbon aggregate (Davidson and Bowie,  1951).   The  average ore grade
in terms of  uranium  is  approximately  0.03  percent.   Generally, mine operators
considered gold to be enriched when "carbon" occurred in greater amounts (Park
and MacDiarmid, 1970).  Substantial  uranium has been recovered as part of gold
processing in  South Africa  beginning  near  the  conclusion  of World War  II.
Uranium, in fact, has become more important than gold production in some parts
of the Witwatersrand district  (Nuclear  Fuel, 1977b).   In  some cases, defunct
gold  mines  are being  re-evaluated  in  terms  of potential uranium production
(Nuclear Fuel, 1977a).

    Uranium  minerals  have been  observed in  a  variety of fluorite  deposits.
Brown et al.  (1954)  noted that  uranium  minerals  occur in fluorite deposits in
Illinois, and Wilmart et  al.  (1952)  observed that in the  Rocky  Mountain area
uranium can  either be  disseminated  as   discrete mineral  grains  or  contained
within the host mineral of the fluorite  ore bodies.   Secondary uranium mineral
coating in  fractures and vugs  in  both  fluorite ore  bodies  and  adjacent wall
rock was also recorded.  Butler and Schnabel (1956)  noted that 20 fluorite
deposits or "fluorite-bearing ores"  had  noticeable uranium.

    From a  broader geochemical  viewpoint,  Van  Alstine  and  Shawe  (1976)  ob-
served that  fluorine has a  tendency to  be  associated  with  beryllium,  man-
ganese, columbium (niobium), tin, tungsten,  uranium,  yttrium,  lead,  and zinc.
McKelvey  et   al.  (1955)  noted  that  fluorite   is  a  persistent,  but  minor,
constituent  of  a  majority  of  uranium  vein  deposits.    While  uranium  is
                                        15

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associated with fluorspar  deposits  in the western United  States,  deposits in
the  central  and  eastern  United  States, outside  of  the  Illinois-Kentucky
district, exhibit thorium  minerals  as  a  possible associated constituent (Heyl
and  Van  Alstine,  1976).     It  would  appear  that  fluorspar  may  exhibit
radioactivity either from the uranium series or thorium series.  Griffitts and
Van  Alstine (1976)  suggest  that  radioactivity may  be  a useful  tool  for
exploration of fluorspar-uranium  deposits similar to those seen in the Thomas
Range, Utah, which  contains  "the largest known  uraniferous  fluorspar  deposit
in  the United States"  (Staatz  and Osterwald,  1956).   The  extreme  case  of
uranium  mineral  association  with fluorite  is  the Marysvale,  Utah ore  body
which  is  an  important  source of  uranium.   Currently,  exploration for  uranium
has  been  planned  for  fluorspar claims  in  Utah {Engineering  Mining Journal,
1978; p. 149).

SUMMARY
     In summary, uranium ore  deposits  are associated with  a wide  variety of
metallic and nonmetallic elements.   In  vein deposits,  McKelvey (1955) ranked
the  following  metallic  elements found  with  uranium  vein  deposits   (in  de-
scending order of uranium abundance):  iron, copper, cobalt, lead, nickel,
silver,  zinc.   Gold  is occasionally  noted.    Important nonmetallic elements
include silica and  fluorine.   Precambrian iron  and magnetite  deposits on the
U.S.  east  coast  contain uranium  minerals.   Gold and uranium  are  observed in
metasediments.     Fluorite  deposits  can  contain either  uranium  or  thorium
minerals.

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                       WEATHERING AND SEDIMENTARY CYCLE

INTRODUCTION

    It is during  weathering  and the  sedimentary cycle that major  separation
occurs between  uranium and  thorium.   This  is  due in  part because  uranium
oxidizes  to a  relatively  soluble uranyl  ion compared  to the thorium  form.
Uranium deposition is occasionally difficult to explain due in  part  to the ob-
vious  absence  of  reducing  agents  of  any  sort  to act  on the  uranyl  ion.
Krauskopf (1976)  suggests  that under conditions  of alkalinity and  carbonate
ion availability, highly soluble uranium carbonate complexes may form and con-
tribute to uranium mobility.   Experimentation conducted by Naumov  and Mironova
(1969) substantiate  this  suggestion  as well  as  showing that  carbonate com-
plexes may also play a role  in  uranium  mobility  even with  temperatures in the
range of  100  to 200°C.  Uranium deposits appear to be related  to  reduction in
carbonate content  by  either  carbon  dioxide  degassing  or  wall  rock  inter-
action.

      When rocks are  subject  to weathering,  thorium either remains  tied  up in
resistate minerals or is "...strongly adsorbed by clay particles or present as
insoluble oxides  and hydroxides"  (Ames and  Rai,  1978).    Thorium  resistance
to  chemical   mobility  is   well   exhibited  in  extremely  weathered  soils.
Bauxites, which are  one  end  product  of intense weathering, may  have thorium
concentrations  up to 50 ppm  or more  (Adams and Richardson, 1960).   In summary,
uranium  is  moved  into the environment  of  sedimentary  deposition  in solution;

                                        17

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thorium  is  moved into  the  depositional  environment associated  with  discrete
grains.  This fundamental behavioral difference  effectively  decouples  the two
elements (Table 3).

RESISTATE DEPOSITS

    In  igneous  rocks,  trace  minerals  bearing significant amounts  of  thorium
are usually resistant to surface  and near  surface chemical  weathering  proces-
ses.   Such  minerals will  largely be mobilized only  when the grains are phys-
ically  transported  in  a high energy environment  typified  by  fluvial  and/or
beach  settings.    Due to their higher  specific  gravity than  the  associated
quartz and clay particles,  these mineral  grains may become concentrated.  Such
deposits have been  subject  to extensive study,  particularly  in Brazil  (Roser
et al., 1964; Penna-Franca, 1975).  Some of  these beach deposits are  utilized
as a source of thorium.  Other mineral  resources (e.g.  rutile) concentrated by
similar  processes may also  contain substantial concentrations  of radioactive
resistates.

    Placer  deposits generated  by  streams  and rivers as  well  as by shoreline
processes could contain a variety of deposits of economic importance including
gold,  platinum,  and  inert  oxides  and   silicates  of zirconium,  tin,  chrome,
tungsten, and titanium  (Park  and  MacDiarmid,  1970).  The radiation  hazard, if
any, from such deposits is  dependent on  the  geology of the source area, posi-
tioning  of  the  deposit  relative to the  land  surface,  and a  host of variables
relating to land and water use by man or segments of the human food chain.
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    Because of elevated radioactivity,  placer  deposits  along  streams  in Idaho
have been investigated.  Mackin and Schmidt  (1956) concluded  that  most  of the
radioactive minerals found in the  placer was derived  from quartz monzonite, a
component of the Idaho batholith.   The placers  in Bear Valley are particularly
enriched with these minerals.   In  some  areas,  monazite, and euxenite occur in
the ratio (by weight) of about  1:2 with approximately  0.5 pounds monazite per
cubic yard  (Mackin and Schmidt, 1956).  During the interval of 1955 to  1960 a
plant 20 miles to the  south  at  Lowman,  Idaho processed about  200,000 tons of
placer  material  from  Bear  Valley.    Minerals  extracted  include  columbite,
euxenite,  monazite,  magnetite,  ilmenite,   zircon, and  garnet.    Subsequent
inspection  of  the  plant  site  was made to assess potential  radiation  hazard
(Ford, Bacon, and Davis,  Inc., 1977).   While thorium  is an  obvious portion of
the ore  mineralogy,  no attempt was made  to quantify  the potential  radiation
hazard from the thorium-232 decay scheme.   The  uranium-238 decay chain was ad-
dressed, however.

    Placers  of  various ages may  contain thorium.   Twenhofel  and  Buck  (1956)
observed Precambrian age quartzites which  contain  thorium minerals.   Previous
discussion  touched on  the fact  that detrital  grains  of monazite in metasedi-
ment  of  possible placer  origin  are adjacent stratigraphically  to  Precambrian
age iron  formation.   The Witwatersrand gold deposit  is accepted by  some  as a
placer deposit.  Overall,  gold  placer deposits  have  been the  subject  of ex-
tensive  exploitation.   There also  has  been substantial  interest  in  titanium
deposits in eastern  Florida  beach deposits  (Lynd, 1960;  Park and  MacDiarmid,
1970).   The two principal  deposits are located at  Trail  Ridge and east  of
Jacksonville with  monazite  being  identified among the mineral  assemblage of
the former.  Numerous  occurrences  of  titaniferous  sands are common in Florida
                                        19

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but are  usually  less than commercial  grade.   Sand sampled from  Venice Beach
was found to contain between 0.05 and 1.5 percent monazite (Florida Department
of Health  and Rehabilitative  Services,  1976).    In  general,  Florida  "black"
sand contains 250 to 1000 ppm thorium with an average of  300  ppm  and  about  an
order of magnitude less uranium (Osmond, 1964).

    Processing of  heavy sands  has  created some  radioactivity  problems.   In
Albany,  Oregon there has been  extensive processing  of  zirconium as well  as
other  rare metals  including  columbium, tantalum, and  hafnium (Boly,  1977).
Ore of these  metals usually contains substantial radioactivity,  which  in  the
Wan Chang  operation is concentrated in  a  "flour-like mineral  residual" which
is radioactive.   Leachate water  associated  with wastes  buried  on the plant
site  contained  on  the  order of 45,000  pCi/1  of radium-226  (State of  Oregon
Health Division  as  cited  in Boly,  1977).   Approximately  4000  tons  of  this
waste material are  located at the plant site with similar material disposed of
at  several  locations  outside  the  plant  site,  including the  Coffin  Butte
landfill  near Adair Village.

    In summary,  placer  deposits  of  any type have  a  potential   for  elevated
radioactivity during mineral extraction and processing.   The thorium-232 decay
series   is  especially,  but   not   exclusively,  the  source  of  activity.
                                        20

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RESIDUAL DEPOSITS

    While soil can  be  expected to reflect some  properties  inherited  from the
underlying  bedrock, significant  deviations  are  observed  in  radioactivity
levels between the two.  Soils are the result of complex chemical, biological,
and physical processes  which alter the concentration of certain elements.
This is  particularly true when conditions  involve  extensive,  long-term chemi-
cal weathering and minimal physical transport.   For  example,  Pinkerton et al.
(1964) found  that  the  soil  over  limestone in Maryland was  quite radioactive
despite the low activity of  limestone.   This  is  due in part  to  selected  con-
centrations of  radioactive elements  in  the  parent  rock  as  it  weathers  into
soil.  Bauxites, the  principal aluminum ore,  are  complex aggregates  of  iron
and aluminum  minerals  which  form  as residual deposits, often over limestone,
under  tropical  climatic  conditions  (Park  and MacDiarmid,  1970).  They  have
been  observed to  have substantially  higher  levels of  uranium  and  thorium
(Polanski, 1965) than the parent  limestone  (Table  3).   Although  not signific-
ant  in the continental United States,  important  residual  ores  include  man-
ganese  oxides in  India  and  nickel  in  New  Caledonia  (Park  and  MacDiarmid,
1970).

ORGANIC MATTER ASSOCIATIONS

    While it  is  beyond the scope of this  report to detail  the relationships,
organic matter can play an important role  in  uranium deposition.   Much of the
radioactivity in sedimentary rocks is found to be related  to organic residues.
Breger and Deul (1956)  note that the close association  between carbonaceous
                                        21

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material  and  uranium may  be the  result  of  three mechanisms:    (1)  organic
matter acts directly as  a reducing agent converting the soluble uranyl  complex
to insoluble uranous  ion,  (2)  sulfide ubiquitously present  in organic debris
acts  as the reducing agent  and,   (3)  the carbonaceous  material  acts as  a
chemical  precipitant  in  some unknown fashion.  Jennings  and Leventhal (1977)
proposed a structural  model of humic-acid type material which identifies sites
for uranium attachment.

    Organic materials which can exhibit substantial uranium enrichment include
coal  (esp.  lignite),  humate, black  shale, asphalt, and  oil.   Armstrong  and
Heemstra  (1973)  noted that  as  oil  becomes more  oxidized  or asphaltic, total
uranium  content  increases.    Rocks  with  unusually  high  levels of  organic
residue  or  asphalt-bearing   rocks   also  tend  to  exhibit  higher levels  of
radioactivity.   Hail  et  al.,  (1956)  found  that ash of the  extracted  oil  con-
tained  from  0.028 to 0.376  percent uranium.   Uranium is  clearly confined to
the organic  fraction  of material  and not  in  the  confining rock.   Uranium is
enriched  in lignite,  particularly in deposits in the upper Great Plains (Vine,
1956).   Denson  et al. (1960) analysed  275 surface and 1000  core  samples  and
found uranium content to vary between 0.005 and 0.02 percent.

    Living  organic  matter  may  even  have  a  more  active  role  in  uranium
deposition.   Jensen  (1958)  suggests that anaerobic  bacteria may  act as  a
source  of hydrogen sulfide which in turn promotes uranium precipitation.

    In  summary,  organic matter  is  an  important  agent which  can concentrate
uranium in  the   sedimentary  cycle.    In  contrast,  thorium  is   enhanced  in
residual  or resistate deposits such as placers and soil.
                                        22

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                MINERAL EXTRACTION AND RADIOACTIVE BYPRODUCTS

    A specific  mining  operation  may  involve elevated (relative to background)
radioactivity if  the  principal  ore  material  contains  or  is  associated  with
uranium and/or  thorium  and their daughters.   Obviously, the  potential  for  a
radiological   health  hazard   depends   on   whether  significant   amounts   of
radionuclides are  present  and  benefaction  results in sufficient radioactivity
to be of concern in the product, waste, or  environs.   Radioactivity levels  so
created may  increase occupational  and/or  general  population exposure.   The
occurrence of  radioactivity in  byproducts is  also cause  for  concern.    In
certain instances,  uranium is, or soon will  be, recovered as  a  byproduct  of
phosphate, copper,  and gold  extraction.    For  example,  the  Central  Florida
Land-Pebble Phosphate District was initially  identified as  having significant
amounts of uranium (Cathcart, 1963a;  1963b; 1963c; 1964; 1966) yet large scale
byproduct  extraction  during  phosphate processing  only  began  in late  1975
(Finch, 1977).   The potential  radiological  hazard posed by  phosphate  mining
and  processing   has  only  recently  been   evaluated,  partly   in  response  to
increased local  population and  competition for land and water.

    Byproduct production  of uranium  is being implemented  as part of  copper
extraction in Utah.  Another operation proposed in Utah involves extraction  of
uranium from beryllium ore (Engineering and Mining Journal,  1978; p. 149).   In
the Witwatersrand district of  South Africa,  uranium minerals  were reported  as
part of the  ore mineralogy  as early  as  1923 (Cooper,  1923).    However,  by-
product recovery of uranium was not attempted until the latter part of World
                                        23

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War II.  In some cases uranium has become the principal  metal  of economic
interest.   As  the demand for  uranium increases, other mining  industries  are
likely to  become  potential  sources  of  uranium  or thorium.    As  these  new
resource materials are  identified,  a need will develop to  identify  potential
radioactivity problems they  may pose.

    In summary,  uranium  byproduct   extraction  has  been  made  in  phosphate,
copper,  and gold  ore  processing.   Similar extraction  operations  have  been
suggested for beryllium ore  in Utah.
                                       24

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         RADIOACTIVITY MEASUREMENTS ASSOCIATED WITH MINING OPERATIONS

    A limited amount of information concerning radiation and ratiation dose is
available in and adjacent to non-uranium mining operations.   Included  in  this
category is  information  defining  trace concentrations of  uranium  and  thorium
in ore bodies and surrounding terrain.   The Mine Safety and Health  Administra-
tion (MSHA) is the principal  Federal  Agency concerned with radiation levels in
underground mine  air and the  principal  source of the  information  presented
herein   (Rock,   1977,   written   communications;    Goodwin,   1978,   written
communications).    Radioactivity   measurements  made  to  date  in  mines   are
primarily concerned with the assessment of  potential  hazard to miners  and may
not or may  only indirectly  relate to ore geochemistry.   Radon  in  some mines
has been attributed to sources  other than  the ore, as in the case  at the  Pine
Creek tungsten mine, California where ground water  is believed to  be the radon
source  (Rock,  1977,  written   communication).     Secondly,  the  presence  or
absence of ventilation may play an important role  in mine  air radioactivity.
Clearly, an underground operation  which for a variety of reasons  has excellent
ventilation can  have  low concentrations  of airborne radioactivity but a  high
overall radioactivity potential.  Procedural variability in atmospheric radia-
tion  measurements  made  by  MSHA  is  also   present  (Andrews,  personal   com-
munication, 1978).   In  general  the available data  are  very limited and  vary
from  qualitative  to quantitative.   It  includes observations from  both water
and air measurements.  It is  unknown how representative  these numbers are.  It
is  also  unknown how the  available observations on activity  levels  relate  to
water  and  air  outside  the   mine  or how  they  interrelate  to other  possible

                                       25

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radiological source terms of the mining  operation.   Radium-226 levels in mine
related water are expressed as picocuries per liter (pCi/1).  For the purposes
of  this  report  they  are compared  to the  5 pCi/1  limit of  radium-226  plus
radium-228  set by  the  national  interim  primary  water regulations  (USEPA,
1976).  Selected ores  or mines  will  be noted  if  radon/radon  daughters  are
thought to be elevated (subjective experience of Rock, personal communication,
1977) but  exact values  are  not  available.   Otherwise,  radon/radon daughters
are  expressed  as working levels  (WL).   All the  quantitative data  from  MSHA
were taken  from  a  list of  observations  of 0.1  WL or greater.  Therefore,  they
may  not  be typical of the  vast  majority  of  operations in  a  given  mineral
industry.   (A  WL  is defined  as  any  combination  of short lived radon daughters
in  1 liter of  air which will  produce  1.3  x  10^  million  electron  volts  of
potential alpha energy.)   MSHA regulations require corrective action when mine
atmosphere levels exceed 1.0 WL.

     Substantial effort has  been  made to  investigate  radioactivity associated
with ore bodies.   In  part, this  is  to  determine whether radioactivity may be
helpful in exploration and ore definition.   Gross (1952) inspected gold mines
located in  igneous stocks  in  Canada  and  found  that  elevated radioactivity was
a pervasive feature.   Moxham  et  al.  (1965)  observed that uranium was enriched
about four  times that of  the  surrounding country  rock  in  tiie  Bagdad Copper
Mine, Arizona.   However  Moxham  et  al.  (1965) also conducted radiation surveys
of  three  Precambrian  age  massive  sulfide deposits  in  North-Central  Arizona:
1)  United  Verde/United Verde Extension Mine at Jerome,  a massive copper-zinc
deposit; 2) Iron King Mine, a massive lead-zinc deposit; 3)  Old Dick Mine  near
Bagdad, a massive  copper-zinc mine.   No  significant systematic dependency was
observed  between  uranium  or  thorium  content  in  either  the  alteration  or
                                       26

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mineralized  configuration  of  any  of  the  mines.   Gangadharam et  al.  (1963)
similarly  noted  that  the  copper   and   uranium  content  were   essentially
independent  in  the  environment of a massive  sulfide  ore body at  the Mosaboni
Copper Mine, India.

       Fitzgerald  (1976)  reviewed  the literature  concerning  radioactivity
associated with low grade  copper deposits.   One of the principal  contributors
he notes is  Still (1962) who observed  the  uranium content of various porphyry
copper deposits  in  the Miami  District  of Arizona.   The geometric mean of 140
observations by Still  (as  given by Fitzgerald, 1976) at  the  Copper City Mine
is about 50  ppm uranium.   A second mine in the district, the Castle Dome, had
a geometric  mean of approximately  10 ppm.   Apparently  within  the same mining
district, the uranium content of similar ore body types may vary considerably.
The enrichment  of  potassium is a  common  feature of  porphyry  copper deposits
and  attributed  to  a  variety  of  processes  (Davis  and  Guilbert,  1973).
Potassium-40 is  a  radioisotope which  makes  up about 0.01  percent  of natural
potassium  and   may  contribute to  the  overall  radioactivity  of  an  ore  body
(Davis and Guilbert, 1973).  They note that others in the area of theoretical
crystal chemistry have suggested that  uranium as well as thorium could also be
enriched along  with  potassium.   However, investigation  by  Davis  and Guilbert
(1973)  of  four  porphyry   copper   mines  and   adjacent   geologically  similar
features without copper  mineralization revealed that uranium  and  thorium are
not  systematically enriched  as a result  of or  in  association  with  copper
mineralization.     A   weighted  average  uranium  content   from   mineralized
occurrences  is  0.95 ppm (Data taken from Table 1; Davis and Guilbert, 1973;
p. 157).  For barren sites the weighted average uranium content is 0.63 ppm.
                                        27

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    Analysis by  the U.S.  Bureau  of Mines  of 4 copper,  1 molybdenum, and  5
lead-zinc tailing  samples revealed  less than  30  ppm  0303.   One  lead-zinc
tailing  sample  contained  60 ppm  U^QQ  and  a phosphate  tailing  sample  con-
tained 150  ppm  1)303  (written  communication, K. Dean,  U.S.  Bureau of Mines
to R.  Snelling,  1970).   Addressing the  problem from a mineralogical  point  of
view, trace amounts of uranium in  pyrite, sphalerite,  and  galena have been
observed to  vary from  one to several  thousand parts  per million  (Wright  et
al., 1960).  They  suggest that in samples with greater than 80 ppm,  uranium
appears to be irregularly  distributed  and, therefore, not  strongly  related  to
the fluid which  deposited the metal sulfide.   Stuckless  (written commu-
nication, 1978)  suggests  that this may  even be true for  concentrations  even
greater than 8 ppm.  Apparently trace  amounts of  uranium  in sulfides  are re-
lated to secondary processes or microcrystalline minerals  not directly tied  to
sulfide deposition.  Secondly, uranium  content appears to  be dependent more  on
regional  availability than on mineral  genesis.

    Metallic  commodities   and  associated   radioactivity   observations  are
summarized  in  Table  4.   Radium-226  data  are taken  from  Supplement B-13,
radiological data,  Calspan  Corp.  (1975) and air  sampling  data  supplied  by
MSHA.  Working levels  shown are derived from a  list  which  notes  underground
mines  with  at  least one  sample of 0.1  WL or greater.   For  commodities  with
three  or  more  maximum  WL observations  available,  the  rank  from  highest  to
lowest  is  1)  molybdenum,  2)  iron,  3)  lead/zinc,  and  4)  gold.    If all
commodities are  pooled,  the  average maximum  WL is  0.54.   Only molybdenum  is
greater  (0.83) in  terms of average maximum  WL and  iron has approximately the
same  value  as the  pooled  average.    For  commodities  with  only  one  or two
observations  the  highest was  antimony  followed   by  copper,  tungsten,  and
                                       28

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silver. The single available maximum WL observation  for  antimony  is 0.91;  the
average for two copper values is 0.70; the average for two  tungsten values is
0.61 and  for  silver  is 0.24.   When analyzed  in terms  of WL and  rejecting
single values, the commodities with.possibly  the greatest air concentration of
radon-222 progeny are:  1)  molybdenum,  2)  copper, 3}  tungsten, and 4) iron.

    The radium-226 data base from  water samples  is  extremely incomplete.   For
all commodities  pooled,  the  average  radium  content  is  17.3  pCi/1.   If  the
extremely  high value in a gold mine  is  excluded  (81.7 pCi/1),  the  average
radium content is 9.2 pCi/1.   Data values appear to  be extremely high or  low
(see Appendix A).  If observed radium-226  activity in water from various  parts
of the metallic mineral  extraction  industry are indicative, radium-226  content
of water sampled is elevated and in general would exceed  the 5 pCi/1  standard.
Such  a  direct  comparison  is  probably  not   strictly  valid  particularly
considering that the waters tested  are not intended  for potable use.
Nevertheless there is some possibility  that  a radiological  health  hazard  may
exist in process water associated with metallic mineral  extraction operations.
Radium-226 data  ranked in  decreasing concentration for these commodities with
observations greater than 9.2 pCi/1 are:   1)  gold, 2) iron, 3) molybdenum,  and
4) aluminum.

    Among the  nonmetallic commodities,  fluorspar appears  to have significantly
greater concentrations (1.2 WL)  in mine atmospheres  (Table  5),  although  these
are  associated with  low  ventilation rates.   The  Federal   Radiation  Council
(1967)  reported  that radon  in a  fluorspar mine in  Newfoundland  in areas  of
restricted  ventilation exceeded  1000  pCi/1.   Also,  tailings  from a fluorspar
operation  near Golden,  Colorado have gamma  radiation levels on  the order of
                                        29

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1 mR/h (USEPA, 1976).  The pooled average maximum WL for nonmetallics was 0.56
which is very close to 0.54 observed for the metal lies.  The highest number
reported was  1.6  WL for  a  phosphate mine, but  since  phosphates  are excluded
from this  discussion,  this  value  will   not  be  used.    Outside  of  these  two
observations maximum working levels are much  lower,  possibly indicating that
fewer  nonmetallic  mine and  milling  operations  bear  much additional  study.
Robbins  (written  communications,  1977)  noted that MSHA  also  reported signif-
icant  amounts  of  radon-222  in  fluorspar related mines  with  about  500  pCi/1
reported.   Similarly,  about  100  pCi/1  radon-222  was  noted in  underground
granite, marble, and limestone operations.
                                       30

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                                   SUMMARY

CONCLUSIONS
1.    The overall  geochemical  properties of uranium and thorium  suggest  that
cerium, zirconium, and the rare earth elements should be associated.

2.     Uranium  and thorium content  of igneous rocks generally  increases  with
increasing silica  and with  increasing  potassium.   Some  mafic and  accessory
minerals are much more enriched than  the felsic  minerals.   Thorium content of
igneous rocks closely follows the potassium content.

3.     Certain  areas  such as  the Front  Range  in  Colorado  and portions  of New
England are broad regions of overall enrichment in uranium and thorium.

4.     Pegmatites may  be enriched  in  uranium, particularly  if the potassium
content is elevated.

5.     Carbonatites  can be enriched in  uranium  and thorium, particularly  if
rare-earth content is high.

6.     Some  rare-earth  elements have  radioisotopes which  may contribute  to
overall radioactivity of an REE ore body.
                                       31

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7.     Hydrothermal  mineral  deposits  exhibit  a broad  spectrum  of geochemical
and mineralogical association with thorium and uranium.  The three principal
metals  observed  in  vein  type  uranium  deposits are  iron,  copper,  and  lead.
Uranium minerals have been found in many different  types of deposits including
ores for gold, silver, and iron.

8.     The  distribution of trace amounts  of uranium  is homogeneous in pyrite,
sphalerite,  and  galena at  concentrations less  than  8 ppm  uranium.    Trace
amounts of uranium greater than this are irregularly distributed and
presumably not strongly related to the deposition of the host minerals.

9.     Fluorspar  deposits  appear to be more radioactive than most  other  non-
metallic  ores.   Both  thorium  and  uranium minerals  have been  observed  with
fluorite.
       Fluorspar deposits have  been  noted as  having  significant radioactivity
in associated underground  mine atmosphere and  mine  tailings.  Radioactivity of
fluorspar deposits has been suggested as a useful exploration tool.

10.   Uranium is generally soluble and mobile  in the sedimentary cycle.
Uranium may be stabilized by  organic matter.   Thorium  minerals  are resistant
to  surface  weathering  and tend to  be concentrated in  placers  or in residual
soil (such as bauxite).

11.    Byproduct recovery  of uranium  from phosphate,  copper,  and gold  ore
processing is underway and is proposed for beryllium ore.
                                       32

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12.   With  the  exception of uranium and phosphate ore bodies  and  to  a lesser
extent in the case of placer deposits of resistate minerals,  no persistent
pattern  of  radioactivity is associated  with ore  bodies.    Radioactivity  may
vary  substantially  between  ore bodies  with similar  mineralogy and  genesis.
Mines of gold, copper, and iron have been observed with  elevated
radioactivity.

13.    Observations  on radioactivity of  mine atmospheres are  of  questionable
validity.  Preliminary information suggests that higher  working levels are
associated with molybdenum,  copper,  tungsten, and iron.

14.   Radium-226 observed in various types  of  mine related water tends to  be
elevated.  The highest concentrations observed,  in descending order,  are gold,
iron, molybdenum, and aluminum.

RECOMMENDATIONS
1.     Radiological  surveys  of various  mining  industries need to be  made  for
both the  uranium  and thorium decay  series.  Rare-earth  element  radioisotopes
and potassium-40 may be important  in certain situations,

2.    Atmospheric radioactivity levels  in  underground mines  may  be poorly re-
lated to ore geochemistry.  Radon  levels have been found to  be  substantial  in
limestone caves despite the  fact that limestone  has low  concentrations of  both
uranium  and thorium  (see Table  3).    Detailed  information is  required  on
ventilation before valid conclusions can be attempted.
                                       33

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3.    Mineral extraction appears to enhance  radium-226  concentrations  in  mine
related water.  Further investigation  is appropriate in  this  area.
                                       34

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radiochemical   pollution  from  phosphate rock  mining and milling;  Office  of
Enforcement, National Field Inv.  Center-Denver, Colorado, 46 pp.
                                       40

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	}  1975}  Preliminary  findings  - radon daughter  levels  in  structures
constructed  on reclaimed Florida phosphate land; Office of Radiation Programs,
Tech. Note ORP/CSD-75-4, 7 pp.

	1  1976,  Radiological  quality  of the environment:  Office  of Radia-
tion Programs, Report No. EPA-5201 lr-76-010, 247 pp.

Van Alstine, R. E., and D. R. Shawe, 1976, Element association, j_n Geology and
resources of  fluorine  in  the  United States:   D.  R.  Shawe,  ed.,  U.S.  Geol.
Survey Prof. Paper 933, p. 14-15.

Vickers, R.  C., 1956, Geology and monazite content of the Good  Rich  Quartzite,
Palmer area,  Marquette County, Michigan,  in  Contributions to  the  geology  of
uranium and thorium  by  the United States Seblogical Survey  and  Atomic Energy
Commission for the United Nations International Conference on peaceful  uses of
Atomic Energy 1955,  Geneva,  Switzerland:   U.S. Geol.  Survey Prof.  Paper 300,
p. 593-596.

Vine, J. D., 1956, Uranium bearing coal  in the United States, in  Contributions
to the geology of  uranium and  thorium by the  United States  Geological  Survey
and  Atomic  Energy Commission for the United  Nations  International  Conference
on peaceful  uses of Atomic Energy 1955,  Geneva, Switzerland:   U.S. Geol.
Survey Prof. Paper 300, p. 405-411.

Wilmarth, V. R.,  H.  L.  Bauer,  M.  H. Staatz, and D. G.  Wyant, 1952,  Uranium in
fluorite deposits:  U.S. Geol.  Survey Circ. 220, p. 13-18.

Wright, H. D., M. S. Chester, and J. J. Hutta,  1960, Role of trace  amounts  of
uranium  in  some  base  metal  sulfides  from vein  deposits,  jji  International
Geological  Congress  Report of  the  Twenty-First  Session,  Part XVI:   Theodor
Sorgenfrei,  ed., p. 248-260.
                                        41

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                               APPENDIX A.   RADIOLOGICAL  DATA FOR SELECTED METALLIC COMMODITIES
Commodity
Al uml num
Antimony
Copper
Gold
State - Mine
Arkansas
Bauxite
Montana
Babbitt
Arizona
Mammoth Mt.
Bagdad
Copper Queen
(& Silver) Red Rover
Michigan
White Pine
Montana
Butte
Tennessee
Boyd
Colorado
Brooklyn
Nevada
(& Silver) Gooseberry
Oregon
Buckeye
Bald Mountain
South Dakota
Homestake
Water Type
Mine
Wastewater
Basin c(?)
300 Level, Mine
Pit Mine
Discharge #1
Discharge #2
Discharge #3
Mine
Mine
Mine
Input to emergency
pond
Mine
Radium -226 Atmospheric Radioactivity*
pCi/1 WL Observed
32.2 +
2.15 +
4.6 +_
2.6 +
1.6 +
27.3 +
4.18 +
13.6 +
4.79 +
1.52 +
2.95 +
1.72 +_
81.7 +
2.3
.22
.62
.26
.16
2.7
.46
1.4
.48
.15
.53
.17
8.2
.47 (.91)
Yes**
- (1.2)
.089(.207)
.15 (1.15)
.17 (.2)
.13 (.13)
.17 (.32)
Footnotes - See end of Appendix

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                       APPENDIX A.  RADIOLOGICAL DATA FOR SELECTED METALLIC COMMODITIES (Continued)
Commodity
Iron
(Magnetite)
Lead/Zinc
(Lead/Silver)
(Zinc Only)
(Zinc Only)
(Zinc Only
(Lead Only)
(Lead Only)
(Lead Only)
(Lead & Silver)
State - Mine
Michigan
Mather B
Sherwood
Missouri
Pilot Knob
Pea Ridge
Pennsylvania
Grace
Colorado
Leadville Unit
Idaho
Kellogg
Muldoon Barium
Silver Empire
Horseshoe
Tamarack
Star
Bunker Hill
Missouri
Bixby
Indian Creek
Viburnum #27
Viburnum #28
New York
Balmat
Oklahoma
Eby
Pennsylvania
Central Valley
Utah
Deertrail
Washington
Pend Oreille
Radium-226
Water Type pCi/1
Mine 16.6 + .7
Mine 3.01 _+ .30
Mine/Mill (treated) <1
Pond Effluent <1
Mine Drainage 27.8 _+ 2.8
Mine <1
Atmospheric Radioactivity*
WL Observed
.21 (.49)
.51 (.9)
- (.26)
- (.642)
.14 (.14)
.21 (.42)
- (.23)
.37 (.37)
(.18)
•2 (.7)
.08 .2)
.07 (.2)
^ (.17)
- (-11
- (.15)
Yes**
- (.25)
.70 (1.4)
Footnotes  - See end of Appendix

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                       APPENDIX A.  RADIOLOGICAL DATA FOR SELECTED METALIC COMMODITIES (Continued)
Commodity
Molybdenum
Nickel
Silver
Tungsten
Vanadium
State - Mine Water Type
Colorado
Climax Mine
Henderson
Idaho
TFompson Creek
Oregon
Nickel Mountain Slag
Idaho
Sunshine Mine
Silver Empire
Crescent
California
Pine Creek
Nevada
Emerson
Arkansas
Garland Operation Mine
Radium -226
pCi/1
15.8 ± 1.6
8.23 + 83
4.47 + .45
2.44+ .5
Atmospheric Radioactivity
WL Observed
.24 (.38)
.21 (1.56)
- (.54)
.37 (.37)
.04 (.10)
.31 (.72)
.1 (.5)
"*Underground operations, Average WL followed by maximum WL in brackets.
     Yes  - R. Rock, MSHA, 1977, indicated that significant atmospheric radiation was observed but no
     quantitative measurements are available.
**

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                           APPENDIX B.   RADIOLOGICAL DATA FOR SELECTED NONMETALLIC COMMODITIES
Commodity
Clay
Fluorspar
Gypsum
Limestone
Phosphate
Silica Sand
Talc
State - Mine Water Type
Pennsylvania
Kitanning
Continental Clay
Ohio
Dando
Irondale
Strong Creek Brick
West Virginia
Globe Clay
Arizona
Western Fluorspar
Colorado
Burlington
Nevada
Crowell Fluorspar
Texas
Paisano Underground
Virginia
No. 6 Mine
Illinois
Alton
Montana
Brock -Warm Springs
Wisconsin
Bay City Sand
Vermont
Windham
Radium-226 Atmospheric Radioactivity*
pCi/1 WL Observed
**
Yes
.4 (.4)
.37 (.46)
.10 (.13)
.18 (.24)
.3 (.3)
.9 (2.2)
Yes
.9 (1.0)
.3 (.41)
.28 (.30)
.05 (.16)
.75 (1.6)
.13 (.19)
•18(-)
*   Underground Operations, Average WL followed by maximum WL in brackets
**  Yes - R. Rock, MSHA, 1977, indicated that significant atmospheric radiation was observed

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                APPENDIX C.  GLOSSARY OF GEOLOGICAL TERMS USED


ALLANITE - A mineral  of variable composition of the epidote group with general
formula  (Ca,   Ce,  La)£(Al ,  Fe,  MgJ3(Si04)3  (OH);  may  contain Th  as  much
as 3.2 percent.

APATITE -A mineral group with the general  formula 035^04)3
(OH,   F,C1).     Fluorapatite  [Cas(P404)3F]   is   by  far  most  common   and
apatite is used synonymously with fluorapatite.

BASE METAL - Metal  of less value than gold  or  silver;  generally considered to
be one of the following:  copper, lead,  zinc, tin, or mercury.

BASTNAESITE - A complex  fluorcarbonate  of  the  rare-earth elements principally
cerium and lanthanum  and usually less  than  one percent uranium  and  thorium;
occur in metamorphic contact zones.

BATHOLITH  - A  body of intrusive rock at least  40  square miles  in surface ex-
posure.

BAUXITE - A rock composed of aluminum hydroxides and impurities  in the form of
free silica, clay, silt and iron hydroxides; the principle ore of aluminum.

BERYL  -  A mineral  with  the  formula  Be3Al2(Si60is)  but may  also  contain
Na, Li, Cs and occasionally Rb.

BIOTITIC  -Containing biotite, an iron rich tri-octahedral  mica.

CARBONATITE - An intrusive igneous  rock of  high carbonate  content and usually
enriched in a wide range of rare elements.

CENOZOIC ERA - The time  interval covering the last 60 million years.

CHLORITIC  - Containing  chlorite, a mica-like mineral  of the  formula  (Mg, Al,
Fe)12 [(S1,A1)80203 (OH)16.

CLAY  -Crystalline fragments of minerals that are essentially hydrous  aluminum
silicates or hydrous magnesium silicate.

COLUMBITE  - A  mineral,  the Nb  - rich end  member of the columbite - tantalite
series (Fe,Mn) (Nb,Ta)206.

CONGLOMERATE  - A rock made  up of  pebbles  and  other  rock  fragments  (usually
rounded) cemented together.

DETRITAL  - Consisting of mineral or rock fragments.
                                        46

-------
EPIGENETIC - Refers  to  a process in which  minerals  undergo  changes  as result
of external  processes usually at or near the earth's  surface.

EPIDOTE - A mineral  of the formula Ca2(Al, Fe+3)3(Si04)3(OH).

EUXENITE  - A complex oxide mineral  containing thorium,  rare-earths,  niobium,
tantalum,  calcium  and titanium;  occurs as an  accessory mineral  in  granitic
rocks.

FELDSPAR  -A group of minerals commonly in most rocks with the general  formula
XA1(A1 ,Si)30s  where  X  =  K,  Na, Ca  as  the  major  ions,  and Ba,  Rb, Sr  as
trace ions usually less than 1500 ppm.

FLUORAPATITE   -  A   mineral    of   the   apatite   group   with   the   formula
Ca5(P04)3F.

FLUORITE  - See Fluorspar below.

FLUORSPAR - A mineral, CaF2, the principal ore of fluorine.

FLUVIAL - Of, or pertaining to, rivers; produced by river action.

FRACTIONATION  - The process by which a  mixture is broken down into components.

GALENA - A mineral with formula PbS.

GARNET - A mineral group, with a general formula X3Y2(Si04)3  where
X = Ca, Mg,  Fe+2, and Mn+2; Y = Al , Fe+2. ,Mn+2, and  Cr.

GRANITE - A  silica  rich igneous rock  with  minerals  discernible to the  naked
eye consisting  of alkali  feldspar  and quarts with  minor  muscovite,  biotite,
and hornblende.

HURONIAN  -  A  subdivision  of Precambrian  rocks  identified   in  the  Canadian
Shield which range from about 800 to 1200 million years in age.

IGNEOUS - Formed by solidification from a molten or partly molten state.

ILMENITE  -  A mineral with  the formula FeTi03; accessory mineral  in  many  ig-
neous and metamorphic rocks.

LIGNITE - Brownish -black  coal  composed of  a  plant  residue more  altered  than
peat but  less than bituminous coal; less than 8300 BTU.

LIMESTONE - Sedimentary rock consisting mainly of calcium carbonate (CaC03).
MAGNETITE  -  A magnetitic  iron  mineral,  FeFe*,   occurring  as  an  ac-
cessory mineral in igneous rocks and as an iron ore.

MAGMATIC DIFFERENTIATION  -  Operation  by which various types of  igneous  rocks
are separated from a single molten mass.
                                       47

-------
MARBLE  - A  rock,  metamorphosed limestone  or  dolostone  with  more or  less
course -grained crystalline structure.
MARCASITE  - A  mineral  of the  formula  Fe$2;  pyrite  is  a  different  crystal
form of the same chemical composite.
MICA -A mineral group of phyllosil icates with sheet -like structures.
MINERAL  -A naturally occurring chemical element or compound having a definite
range in chemical composition and characteristic crystal structure.
MONAZITE  -  A  mineral  (Ce,La)P04 commonly containing  thorium as well  as  rare
earth elements.
MUSCOVITE  - A mineral  of the mica  group (which  are characterized  by a sheet-
like structure) of the general formula KAl£
OPALITIC  -A material consisting of opal, with amorphorus hydrated silica
PHLOGOPITE - A mica mineral with the formula K2(Mg, Fe+2)6
            (OH,F)4.
PITCHBLENDE - Another term for uraninite when massive.
PRECAMBRIAN -All geologic time previous to about 600 million years ago.
PYRITE  - A mineral of the formula Fe$2 the most abundant sulfide.
QUARTZ  - A mineral, $104.
QUARTZITE - A rock of quartz grains bonded by metamorphism.
QUARTZ  MONZONITE  - An  igneous  rock  (with minerals identifiable with the naked
eye) which contains plagioclase (Na/Ca feldspar), orthoclase (K feldspar), and
quartz  with biotite and/or hornblende and accessory apatite, zircon and opaque
oxides.
RESISTATE MINERALS - Those undecomposed residues of weathering.
ROCK  - Any  natural   aggregate  of  mineral  matter  (or  single mineral)  con-
stituting an essential part of the earth's crust.
RUTILE  - A mineral, Ti02.
SPECIFIC GRAVITY  - Ratio of  the  mass  of a body to the mass of an equal volume
of water at a specified temperature.
SPHENE  - A mineral with the formula
SPODUMENE - A mineral with the formula LiAlSi206.
THORITE - A mineral with the formula ThSi04.
                                       48

-------
TOURMALINE - A  mineral,  a complex borosllicate containing varying  amounts  of
Na, Mg, Fe, Mn, Li, and Al.
URANINITE  - A  mineral, primarily U02  but also may  contain Th,  rare-earths,
Ra, and Pb.
VEIN  DEPOSIT  - A  mineralized zone  long in  two  dimensions and  thin in  the
third.
WEATHERING - Chemical  and physical processes  operating at the  earth's surface
on rocks  resulting  in  change in  character,  decay, and finally crumbling  into
soi 1.
XENOTIME  - A mineral YP04 also containing rare-earths,  Th  and U.
ZIRCON  -  A  mineral,  ZrSi04, a  common  accessory  mineral,  particularly  in
silica enriched plutonic rocks.
Principal Sources:
American Geological  Institute,  1962,  Dictionary of geological terms;  Dolphin
Books, Garden City, NJ, 545 pp.
American Geological  Institute;  1976,  Dictionary of  geological  terms;  Anchor
Press, Garden City, NJ, 472 pp.
Deer, W. A.,  Howie, R.A., and  J.  Zussman,  1966,  An introduction to the  rock
forming minerals; John Wiley and Sons, New York, 528 pp.
Leet, L. D.,  and S. Judson, 1965, Physical Geology; Prentice-Hall,  Englewood
Cliffs, NJ, 406 pp.
Moore, R. C., 1958, Introduction to Historical  Geology,  McGraw-Hill,  New York,
656 pp.
                                       49

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               TABLE  1.   URANIUM AND  THORIUM CONTENT OF MINERALS
                             FOUND  IN  IGNEOUS ROCKS *
Major Mineral



Quartz

Feldspar

Biotite

Muscovite

Hornblende

Pyroxene
Uranium  ***

 Mean  (ppm)

    1.7

    2.7

    8.1



    7.9  (?)

    3.6

    0.05
                                               Uranium       Thorium

                                               Normal  Range  (ppm)**
0.1-10
0.1-10
1.0-60
2-8
0.2-60
0.1-50
0.5-10
0.5-10
0.5-50
-
5-50
.
                                                               0.02
01ivine
(mean)
  * Summarization  of tables given  in Rogers  and Adams  (1969a;  1969b)

 ** Normal  range excluding extreme values

***  Recent  work  suggests  that  the quartz  and  feldspar  values are too  high,
biotite  is low  by order of magnitude  and pyroxene high  by order  of magnitude
(Stuckless, 1978 written communication)
           TABLE   2.   GENERALIZED DISTRIBUTIONS OF URANIUM IN VARIOUS
                       GROUPS OF  IGNEOUS ROCKS
                    Ultramaflc rocks
                    (dunltes, serpenUnites,	
                    ecfogfles, etc.)
                    Mafic rocks (basalts, gabbros etc.)
                    Intermediate rocks (andesites, dacites,
                    rhyodacites, diorltes, quartz diorites,
                    granodiorites, etc.)
                    Silicic rocks (quartz latites, rhyolites,
                    quartz monzonites, granites)
                              0.001     0.01      0.1      1.0

                                    Uranium (ppm)

                       (Taken from Rogers and  Adams, 1969b)

                                           50
                                         10

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              TABLE 3.   URANIUM AND THORIUM CONTENT OF SELECTED
                        SEDIMENTARY ROCKS*
     Rocks
Sandstones
    Orthoauartzite
         (North American Avg.)
    Graywacke (Est. Avg.)
    Arkose
Thorium (ppm.)  Uranium (ppm)
     1.7

     2.8
     5
0.45

2.1
1.5
Shale
    Common Shale, Gray, Green, etc.
         (North American Avg.)
         Black Shale
Bauxites
Bentonites
Limestones (North American Avg.)
Dolomites (Range)
Phosphate Rock (Range)
Evaporites**
13.1
Low
48.9
24.0
1.1
-
1-5
3.2
8
11.4
5
2.2
0.03-2.0
50 -300
               generally less
               than 0.1
 * Summarization of tables given in Rogers and Adams (1969a, 1969b)
** Some evaporites can be important ore deposits particularly those found in
  Africa and Australia (Stuckless, 1978, written communication).
                                       51

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Ln
tN)
                          TABLE 4.   SUMMARY OF RADIOLOGICAL  INFORMATION ON METALLIC COMMODITIES
                                    GIVEN  IN APPENDIX A
Commodity
Aluminum
Antimony
Copper(3)
Gold(4)
Iron(5)
Lead/Zinc(6)
Molybdenum
Nickel
Silver
Tungsten
Vanadium
                                    Average Maximum(l)   Number of
                                      WL Observed
Observations
Radium-226(2)
     pCi/1
                                                                                  (2.44)(8)
Number of
Observations
-
.91
.70
.20
.48
.37
.83
-
.24
.61
-
1
2
4
5
12
3
-
2
2
13.0
-
6.7
81.7
16.7
(6.46)(7)
15.8
8.34
4.47
«.
3
-
9
1
1
5
1
1
1
„
        (1)   Underground operation, Goodwin, MSHA, written communication, 1978; (2) Calspan Corporation,
             1975,   (3) Includes  a copper and silver mine;   (4)  Includes a gold and silver mine;  (5)
             Includes  a magnetite mine;  (6)  Includes 3 zinc only mines, 3 lead only mines and a lead/
             silver  mine;   (7)  Less than 1 pCi/1 replaced with  .5 pCi/1 in calculation;  (8) Composite
             of two  samples.

-------
         TABLE 5.   SUMMARY OF RADIOLOGICAL INFORMATION ON NONMETALLIC
                   COMMODITIES GIVEN IN APPENDIX B
                             Average Maximum*         Number of
    Commodity                  WL Observed           Observations
  Clay                           0.3                      5
  Fluorspar                      1.2                      3
  Gypsum                         0.30                     1
  Limestone                      0.16                     1
  Phosphate                      1.6                      1
  Silica Sand                    0.19                     1
  Talc                          (0.18)**                  1
 * Underground operation, Goodwin, MSHA, written communication, 1978
** Average WL, maximum value not available
                                        53

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                                    TECHNICAL REPORT DATA
                             (Please read Instructions on the reverse before completing!
1. REPORT NO.
   ORP/LV-79-1
                                                             3. RECIPIENT'S ACCESSION NO.
4. TITLE AND SUBTITLE
   Radioactivity in Selected Mineral Extraction
   Industries - A Literature Review
              S. REPORT DATE

               Nnvpmher 1
              6. PERFORMING ORGANIZATION CODE
7. AUTHOR(S)

   James  D.  Bliss
                                                             8. PERFORMING ORGANIZATION REPORT NO,
9. PERFORMING ORGANIZATION NAME AND ADDRESS
                                                             10. PROGRAM ELEMENT NO.
   Office  of Radiation Programs - Las Vegas  Facility
   U.S. Environmental Protection Agency
   P.O. Box 15027
   Las Vegas,  NV  89114
              11. CONTRACT/GRANT NO.
12. SPONSORING AGENCY NAME AND ADDRESS
                                                             13. TYPE OF REPORT AND PERIOD COVERED
                                                                Final
   Same as  above
              14. SPONSORING AGENCY CODE
15. SUPPLEMENTARY NOTES
16. ABSTRACT
        The  mining, milling,  and processing  of mineral resources may cause  varying
   degrees  of technologically enhanced natural radioactivity  (TENR) which is  de-
   pendent  on the inherent  uranium and thorium content of  the target resource and
   the  details of the total  extraction process.
        [The  objective of  this review is to  identify from the  available domestic
   literature possible metallic and nonmetallic mineral extraction industries
   (exclusive of uranium, phosphate, and fossil fuels) which  may require sub-
   sequent assessment.! Certain industries  such as phosphate  and coal are already
   identified as potential  sources of radioactivity; hence, they are excluded from
   this overview.
17.
                                 KEY WORDS AND DOCUMENT ANALYSIS
                  DESCRIPTORS
b.lDENTIFIERS/OPEN ENDED TERMS  C.  COSATI Field/Group
          Geology and mineralogy
          Radioactive materials
          Mineral deposits
                                0807
                                1808
                                0807
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