A EPA United States Environmental Protection Agency EPA/540/M5-89/006 April 1989 SUPERFUND INNOVATIVE TECHNOLOGY EVALUATION Demonstration Bulletin Organic Extraction Utilizing Solvents CF Systems Corporation TECHNOLOGY DESCRIPTION: This technology utilizes liquified gases as the extracting solvent to remove organics, such as hydrocarbons, oil and grease, from wastewater or contaminated sludges and soils. Carbon dioxide is generally used for aqueous solutions, and propane is used for sediment, sludges and soils (semisolids). Contaminated sediments are fed into the top of the extractor (Figure 1). Solvent (condensed by compression at 70 °F) flows upwards through the extractor, making non-reactive contact with the waste. Typically, 99 percent of the organics are dissolved out by the solvent. Then, clean material is removed from the extractor. A mixture of solvent and organics leave the extractor, passing to the separator through a valve where pressure is partially reduced. In the separator, the solvent is vaporized and recycled as fresh solvent. Finally, the organics are drawn off from the separator, recovered for disposal, or reused off-site in industrial processes. The difference in the mobile units for aqueous solutions and semisolids can be found in the extractor. For example, mixing variations can exist in the extractor whereby aqueous solutions can go through one type of mixer having a series of trays while semisolids can go through a "cement-type" mixer. WASTE APPLICABILITY: This technology can be applied to a wide variety of organics such as the following: carbon tetrachloride, chloroform, benzene, naphthalene, gasoline, vinyl acetate, furfural, butyric acid, higher organic acids, dichloroethane, oils and grease, xylene, toluene, methyl acetate, acetone, higher alcohols, butanol, propanol, phenol, heptane, PCBs and other complex organics. Figure 1. Solvent extraction unit process diagram. STATUS: Currently, a pilot-scale system has been tested on PCB-laden harbor sediments from the Massachusetts New Bedford Harbor Superfund site during September 1988. During the test, PCB concentrations (ranging from 300 ppm to 5000 ppm) and the number of passes through the unit were varied for each of the four separate test runs. About one-half drum (30 gallons) of sediments, with additional water added to obtain the appropriate consistency, was processed for each run. Results of the demonstration will be available in several months. DEMONSTRATION RESULTS: Demonstration of this technology was conducted on PCB- contaminated harbor sediment from New Bedford, Massachusetts. The pilot-scale commercial unit (PCU), rated at 20 bbl/day, was utilized at the site. The PCU was a trailer mounted organic extraction system for non-aqueous materials that used a ------- Table 1. New Bedford Test Results Initial Final Number PCB PCB Test of Concentration" Concentration" Percent No. Passes (ppm) (ppm) Reduction 2 10 350 10 '97 3 3 292 73 75 4 6 2,450 96 96 "Mean PCB concentrations, ppm dry weight basis. propane/butane mixture as the extraction solvent. To obtain information for a commercial-scale unit, the same waste was processed through the unit a number of times. • The demonstration was active during September 1988. • The process successfully removed PCBs. • Harbor sediments containing 350 ppm PCB were extracted to 10 ppm after ten passes through the unit. A PCB concentration reduction of 97% and a mass reduction of 99% were achieved. • Sediments containing 2,250 ppm PCB were reduced to a 96 ppm level after six passes through the extractor. • Equipment and material handling problems became apparent with the pilot-scale unit and only operation of a full-scale unit will be able to answer scale-up questions. • A full-scale aqueous unit (400 bbl/day) has been constructed, and a full-scale solids unit should be available in March 1989. FOR FURTHER INFORMATION: EPA Project Manager: Richard Valentinetti U.S. EPA (RD-681) 401 M Street, SW Washington, DC 20460 202-382-5753 (FTS: 382-5753) BULK RATE POSTAGE & FEES PAID EPA PERMIT No. G-35 Official Business Penalty for Private Use $300 EPA/540/M5-89/006 United States Center for Environmental Research Environmental Protection Information Agency Cincinnati OH 45268 ------- |