NATIONAL AIR TOXICS INFORMATION CLEARINGHOUSE NEWSLETTER 453N89003 A EDiA Office °' ^'r Quality Planning and Standards December 1989 Research Triangle Park, North Carolina 27711 ^crpry nET)rEr)/7\ fj /7\ ft M State and Territorial Air Pollution Program Administrators UZ-ALr u L-\ U i^liriZr-Au Association of Local Air Pollution Control Officials IN THIS ISSUE... NATICH IS NOW LINKED TO TRIS 1 HARDCOPY REPORTS USEFUL, ACCORDING TO NEWSLETTER QUESTIONNAIRE 2 STATE/LOCAL AGENCY SPOTLIGHT* LOUISIANA BEGINS TO IMPLEMENT NEW COMPREHENSIVE AIR TOXICS PROGRAM 2 STUDY TO EVALUATE ATMOSPHERIC DEPOSITION OF TOXIC CONTAMINANTS TO PUGET SOUND UNDERWAY 3 A CASE STUDY FOR CARBON DISULFIDE: VIRGINIA FINDS VIOLATION OF AIR TOXICS REGULATION EPA ISSUES GUIDANCE ON DATA QUALITY OBJECTIVES 5 CTC COMPLETES NEW AIR TOXICS REPORTS 5 NESCAUM RELEASES HEALTH EVALUATION OF GASOLINE VAPORS 6 EPA ISSUES POLICY DIRECTIVE ON AIR STRIPPERS AT SUPERFUND SITES 9 ALL STATES NOW ADDRESS AIR TOXICS, STAPPA/ALAPCO SURVEY FINDS 10 TAMS UPDATE: SYSTEM WILL REMAIN A RESEARCH VEHICLE 11 EPA MOVES TO REDUCE BENZENE AIR EMISSIONS 11 IMATICH IS NOW LINKED TO TRIS State and local agency users of the NATICH data base may now access industry emissions data located in the Toxics Release Inventory System (TRIS)* through a link that has been established between the NATICH and TRIS data bases. These data bases both contain a large volume of information related to air toxics. Thus, the computer link is seen as a major step in integrating information sources to the benefit of air pollution control agencies. TRIS was developed to make available information that was submitted by industry under the provisions of the Emergency Planning and Community Right to Know Act. The information covers releases of over 300 toxic chemicals to air, water, and land. Data include names and addresses of facilities that manufacture, process, or otherwise use the chemicals as well as amounts re- leased to the environment or transferred to waste sites. Data on stack and fugitive emissions to the air were reported on over 70,000 forms for the 1987 reporting year; data from the 1988 reporting year are currently be- ing added. Access to TRIS through NATICH is available only to individuals working for State, local, and Federal agen- cies. Public access to TRIS is available through the Na- tional Library of Medicine. Call the Library at (301) 496-6193 or (800) 638-8480. Once they have logged onto the NATICH system, all State and local agency personnel with a computer ac- count for NATICH are presented with a menu item that enables them to access TRIS. Users may elect to use programs that were developed by NATICH specifically for air program activities, or programs developed by the EPA Office of Toxic Substances to retrieve data from the TRIS files. Once queries to TRIS have been completed, the user is automatically returned to NATICH to enable access to the complementary information on air toxics contained there. While the link simplifies data access, some characteristics of the systems are slightly different. User assistance is available through an information screen describing these differences and steps to ensure NATICH users a smooth transition as they access TRIS. ' —» ****** ------- Additionally, NATICH users may contact the Clear- inghouse staff at (919) 541-0850 for assistance or to ob- tain information on setting up NATICH accounts. In addition to the TRIS link, a program has recently been added to NATICH that enables users to retrieve all of the information in the NATICH files on an individual pollutant, source type or agency. This streamlines the collection of information of interest, and sends the data to remote printers distributed throughout the country. An on-line option will be added soon to provide a list of the remote printer locations in the user's State. Until that op- tion is available, NATICH users not familiar with the remote printer facilities may contact the National Com- puter Center User Support group (919) 541-7862 on the Clearinghouse Staff for further information. * See related articles in May 1988 Newsletter, pp. 1 - 2,8. HARDCOPY REPORTS US El TO NEWSLETTER QUESTIO Despite a small rate of return of the questionnaires recently included in the NATICH Newsletter, certain prevailing opinions have emerged. The Newsletter is now sent regularly to approximately 2,000 subscribers; of these, 35 percent are affiliated with State or local agen- cies and another 32 percent are employed by industry or as independent consultants. More than 50 percent of those who returned the questionnaire are with State and local agencies, accounting for more than 70 percent of those who access the NATICH data online, and report- ing the highest frequency of NATICH use. Hardcopy reports of information were found useful across the FUL, ACCORDING iNNAIRE board, but particularly by consultants and various en- vironmental and special interest groups. Various other reports were also well received and the frequency of publication and/or updating was judged adequate for most needs. A majority of respondents have not used the NATICH help line. However, of those who have used it, most were satisfied with the assistance received. Many respondents took time to make suggestions for special reports. These have been tabulated and will be useful to staff in selecting topics for future issues of the Newsletter and for other publications. STATE/LOCAL AGENCY SPC LOUISIANA BEGINS TO IMI COMPREHENSIVE AIR TO> by Mike McDanlel, Assistant Secretary, Office off Louisiana Department of Environmental Quality Recognizing the magnitude of the air toxics prob- lem within the State and the inadequacies of its existing air toxics control program, the Louisiana Department of Environmental Quality (DEQ) drafted a toxic air pollutant emissions control bill, introduced in the 1989 regular ses- sion of the State Legislature. In response to comments from both industry representatives and environmen- talists, the bill was refined to a form that was generally acceptable to both, but still met the basic program ob- jectives of DEQ. The bill then won unanimous approval of both houses of the legislature and was signed into law as Act 184 on June 23rd by Governor Buddy Roemer. Act 184, The Comprehensive Toxic Air Emissions Control Act, borrows language and some of its approach from evolving Federal Clean Air Act legislation. It is designed to use the basic concepts of the Federal air tox- ics program while meeting the specific needs of the State program. Act 184 is unique among State programs in that its language is broad enough to address toxic emissions from industrial, mobile, and area sources. It #1 la PLEMENT NEW [ICS PROGRAM Air Quality and Nuclear Energy, r also sets a goal and a time period for reductions in toxic emissions, provides a means for measuring progress toward attaining the goal, establishes reporting re- quirements so that the public is informed of DEQ's prog- ress, and provides a funding mechanism for the pro- gram. Some of the more notable provisions of Act 184 are described below. The new act defines "toxic air pollutant" in broader terms than the old hazardous air pollutant definition, reflecting contemporary definitions seen in developing Federal legislation. According to Act 184, " 'toxic air pollutant' means an air pollutant which, based on scien- tifically accepted data, is known to cause or can reasonably be anticipated to cause either directly or in- directly through ambient concentrations, exposure levels, bioaccumulation levels, or deposition levels, adverse effects in humans, including but not limited to: (i) cancer; (ii) mutagenic, teratogenic, or neurotoxic effects; (iii) reproductive dysfunction; (iv) acute health effects; and (v) chronic health effects." 2 ------- Act 184 requires the development of an initial list of not more than 100 toxic air pollutants to be published by December 31,1989. The DEQ is currently developing the list, working from Superfund Amendments and Reauthorization Act (SARA) industrial emissions data to which mobile and area sources will be added. The list will take into account relative toxicity, the populations ex- posed, and environmental fate/effect information. The list is to be ranked or classified according to level of concern based on such criteria as emission levels, human health effects, population exposure, and persistence or accumulation in the environment. The list must be re- viewed at least every 3 years and may be modified by additions or deletions. Any person may petition to modify the list. The act addresses both new and existing sources. Existing sources affected by the regulation will be placed on compliance schedules. After completing the pollutant list, DEQ will decide how to define a major source, how to rank area sources, and what stationary, mobile, and area sources to include. The goal of the toxic air pollutant control program is to reduce emissions of toxic air pollutants from all sources by 50 percent from 1987 levels by December 31, 1994. It is an aggressive goal, but one that DEQ feels is attainable without unreasonable economic impacts. A guiding principle in the emissions reduction plan will be to target those areas offering the greatest aggregate reduction of health risks associated with populations ex- posed to toxic air pollutant emissions. To provide a benchmark or baseline against which to measure progress in reducing emissions of toxic air pollutants, Act 184 requires DEQ to conduct studies to estimate emissions of toxic air pollutants from industrial, area, and mobile sources, and publish a report summarizing the baseline 1987 emission levels by April 30, 1990. In April of each year thereafter, DEQ must publish a report summarizing changes in emission levels from the previously reported year and from the 1987 baseline levels, and documenting measures taken and progress made toward reducing toxic air pollutant emissions levels. Act 184 requires that initial regulations for the con- trol of toxic air pollutant emissions be proposed by July 1, 1990. The initial regulations will identify toxic air pollutants to be regulated and establish a schedule for the development of control measures for those pollutants. The regulations will also seek to prevent sud- den, accidental releases and minimize consequences of any such releases. The act requires monitoring of toxic air pollutants "at locations and times deemed necessary" to further develop information concerning sources and levels of ex- posure to toxic air pollutants. In several instances, Louisiana's new act directs that information developed as a result of program efforts "shall be made readily available to the public by the Office of Air Quality and Nuclear Energy in an easily accessible manner". Finally, Act 184 provides DEQ with the authority to levy and collect fees sufficient to fund the toxic air pollu- tant emission control program and supporting ambient air monitoring efforts. The DEQ is at work now outlining a fee and permit system using Federal Clean Air Act legislation as a guide. For further information on the Louisiana air toxics program, write Mike McDaniel at P.O. Box 44096, Baton Rouge, LA 70804-4096, or call him at (504) 342-1201. STUDY TO EVALUATE ATM* TOXIC CONTAMINANTS TO by Naydene Maykut, Puget Sound Water Quality An atmospheric deposition study is currently in progress in the Commencement Bay watershed (near Tacoma, Washington). The objective of this study is to evaluate the importance of atmospheric deposition of toxic contaminants to Puget Sound. Whether at- mospheric deposition contributes toxic materials in con- centrations high enough to harm the biota of Puget Sound is an important scientific question and of poten- tial regulatory interest. Knowledge of the toxic chemical deposition pathway to Puget Sound will help direct future research and management programs. It is considered possible that the atmospheric deposition of certain contaminants such as lead, arsenic, polycyclic aromatic hydrocarbons (PAHs), and other organic compounds may represent an important source of pollutants to the Sound. Both lead and PAHs have OSPHERIC DEPOSITION OF PUGET SOUND UNDERWAY Authority, Seattle, WA been measured at levels of concern in both the sediments and the sea-surface microlayer in several ur- ban bays. More extensive studies in other parts of the country have shown that atmospheric deposition is an important source of particulate metals and PAHs in the southern California Bight; a source of metals, polychlorinated biphenyls, DDT, and other pesticides in the Great Lakes region; and a source of nitrogen com- pounds that contribute to serious eutrophication prob- lems in Chesapeake Bay. A sampling network was set up in Commencement Bay consisting of five aerosol and deposition sites. Two air deposition samples per month are being col- lected at each of these five sites from July 1 to December 31,1989. A sixth sampler is collocated at various times at each of the five sites to help verify the quality of the 3 ------- sampling data. The aerosol sampling protocol is divided into two different regimes: intensive and nonintensive. There are two 5-week intensive sampling periods during the study; one during primarily dry weather (July - August) and the second during primarily wet weather (November - December). Aerosol data are collected at three of the sampling sites during the nonintensive parts of the study. During the two intensive periods, aerosol sampling takes place at all five primary sites. All aerosol samples will be weighed for determination of total mass. A selected number of aerosol and deposition samples will be analyzed for metals and PAHs. A modeling analysis will be used to correlate the aerosol and deposition sampling results and to provide a basis for future use of the results and methodology throughout the Sound. Following are some important areas that the modeling efforts will address: - Deposition of pollutants: the modeling effort will produce maps of estimated target chemical deposition in Commencement Bay and its watershed; - Mobilization coefficients: estimates will be made of toxic concentrations present in storm- water runoff due to atmospheric deposition; - Chemical mass balance: estimates will be made of the ratios of toxicants in the aerosol samples contributed by the various air emission sources, and the ratio of the air versus nonair contribution of toxics to the sediments in Commencement Bay; and - Synthesis of the data for final reporting. Focusing efforts in the manner described above will result in information and methodologies that can lead to understanding the complexities involved in this research area. For example, based on the results of this study, and an institutional/regulatory analysis that will be included in the final report, the Puget Sound Water Quality Authority may decide to include programs in the 1991 Puget Sound Water Quality Management Plan that ad- dress atmospheric deposition of toxic contaminants. The Puget Sound Air Pollution Control Agency may also use the results of this study to modify its air toxic program. The final report is expected to be complete in May 1990. For additional information, please call Naydene Maykut at (206) 464-6893. A CASE STUDY FOR CARBC FINDS VIOLATION OF AIR by Charles Holmes, Air TdxIcs Program Coordlnat The Virginia Department of Air Pollution Control (the Department) recently performed an exhaustive evalua- tion of the air emissions from Avtex Fibers Front Royal, Inc., and found the emissions of carbon disulfide to be in violation of the Commonwealth's regulations* Before the Department began its action, Avtex was the world's largest manufacturer of rayon and the only source of a carbon yarn used by NASA and the Department of Defense in rocket motor nozzles. Carbon disulfide is used as a solvent in the fiber-forming process and is emitted to the air without any reduction from control devices. The emissions of carbon disulfide to the air were reported at 49 million pounds per year, or 5,600 pounds per hour. Emissions of hydrogen sulfide, dimethyl amine, ammonia, sulfuric acid, and lead were also reported, but at much lower rates than carbon disulfide. The magnitude of the emissions from Avtex resulted in this facility being ranked number two in the nation on the basis of total pounds of air emissions reported for calendar year 1987, under SARA 313. In ad- dition to the violation of air pollution regulations, Avtex has been cited for water pollution and worker safety violations, and this facility is an active Superfund site. Virginia's existing Source Rule 4-3, Emission Stan- dards for Noncriteria Pollutants, was the basis for the en- forcement action against Avtex. This regulation provides )N DISULFIDE: VIRGINIA TOXICS REGULATION or, Virginia Department of Air Pollution Control for acceptable ambient limits (AAL) that are calculated as a fraction (1/60 in this case) of the workplace guidelines threshold limit values (TLVs) recommended by the American Conference of Governmental Industrial Hygienists. Virginia's AAL for carbon disulfide is 500 ug/m3 (0.167 ppm) averaged over a 24-hour period Ex- tensive modeling was performed, including runs with both Industrial Source Complex, Short-term (ISCST) and COMPLEX I models. Over 50 release points were fac- tored into the models; based on 5 years of meteorolo- gical data, the predicted concentrations were calculated. The models predicted concentrations of carbon disulfide as high as 6,000 ug/m3 (24-hour averaging time), with exceedances of the 500 ug/m3 AAL out to distances of 5 kilometers. The predicted exceedances of the AAL trig- gered a requirement of one or more of the three options available to the facility under this regulation. These three options were: (1) Demonstrate that the facility does not and will not cause or contribute to an exceedance of the AAL, (2) Demonstrate that the AAL for the substance in question is inappropriate by showing that the emissions from the facility do not endanger human health, or 4 ------- (3) Reduce emissions from the facility to a level which does not result in an exceedance of the AAL. Avtex chose to demonstrate option two, no en- dangerment of human health. Health effects testimony on carbon disulfide was presented by consultants hired by Avtex. For the Department, testimony was provided by the State Health Department and the EPA's Air Risk Information Support Center (Air RISC). The support pro- vided by Air RISC was particularly useful, resulting in an inhalation Risk Reference Dose for carbon disulfide. The reference dose for carbon disulfide is 10 ug/m3, much lower than Virginia's AAL of 500 ug/m3. While the reference dose was not adopted as a revised AAL, it was the single most important piece of health effects evidence presented. The State Air Pollution Control Board, a five- member citizen board, held a formal hearing to consider the hundreds of pages of testimony provided by Avtex and the Department. In a 16-hour session, the Board upheld the Department's recommendation and ordered Avtex to submit a compliance plan within 2 months and to achieve and demonstrate compliance within 1 year. Avtex has filed an appeal to this Order in the Circuit Court for the City of Richmond. This enforcement action received national attention since it coincided with the announcement of SARA 313 data by Representative Henry Waxman. The fact that Avtex was the second most serious emitter of toxic air pollutants in the nation also emphasized the importance of this case. The company's strategic position as the sole supplier of carbonized yarn to NASA and the Department of Defense caught the attention of the national media. Despite the threat of a significant loss of employ- ment in Front Royal, there was widespread support for the action of the State Air Pollution Control Board from local citizens' groups, physicians at the community hospital, and the Front Royal Town Council. Virginia's air toxics regulations are currently undergoing revisions that will result in a more efficient and streamlined procedure. The Department is also looking to incorporate a more widespread use of risk assessment in its decision-making process. The Depart- ment would welcome any ideas from other regulatory agencies on what works and what does not. If you have questions about the program or information on possible improvements, please contact Charles Holmes, Air Tox- ics Program Coordinator, Virginia Department of Air Pollution Control, P.O. Box 10089, Richmond, Virginia 23240. *Note: As of November 10, Avtex ceased all operations in Front Royal as a consequence of revocation of its National Pollution Discharge Elimination System water discharge permit by the Virginia State Water Control Board on November 8. EPA ISSUES GUIDANCE ON I An EPA document entitled "Guidance on Applying the Data Quality Objectives Process for Ambient Air Monitoring Around Superfund Sites (Stages I and II)" is now available. This document should help readers design an ambient air monitoring system that will be ade- quate for the intended use of the data. It is intended to serve as a bridge between the Quality Assurance Management Staff's data quality objectives (DQO) guidance and actual application of the DQO process at Superfund sites. Specifically, this document was written to aid the Remedial Project Managers, Enforcement Project Managers, and the EPA Regional and Superfund contractor personnel responsible for ambient air >ATA QUALITY OBJECTIVES sampling and analysis at Superfund sites to carry out their duties efficiently and effectively. This document gives an example of Stage I (preliminary definition of the decision) and Stage II (refinement of the decision and requirements) for monitoring ambient air quality during remedial action at a hypothetical Superfund site. Stage III of the DQO pro- cess, to be completed in February 1990, involves the design of an ambient air monitoring data collection system for the case study presented in this document. For further information or a copy of the document, call Jane Leonard, EPA Technical Support Division at (919) 541-5653, (FTS) 629-5653. CTC COMPLETES NEW AIR The EPA's Control Technology Center (CTC) has recently completed several projects dealing with estimating air toxic emissions and evaluating control techniques for a wide range of source categories. The resulting documents cover surface impoundments, in- tegrated steel plants, and waferboard plants. The Surface Impoundment Modeling System (SIMS) is a user-friendly PC program that can be a TOXICS REPORTS valuable tool when estimating emissions of volatile organic compounds (VOCs) and air toxics. It can be used on all types of surface impoundments or function- ally similar wastewater treatment processes, including biological treatment units. The program allows entry of specific source information, but also provides industry- based default values. Details of SIMS are included in a user's manual and a technical support document that 5 ------- accompany the software. In response to a request from the State of Utah and EPA Region VIII, the CTC evaluated potential air toxics emissions from integrated steel plants. The resulting CTC report provides a comprehensive set of criteria and toxic pollution emission factors for all source types com- monly found at steel plants. It includes information on process, fugitive, and nonpoint source emissions. A new project to provide similar information for iron foundries has been initiated and should be completed within 6 months. A number of State agencies and EPA Regional Offices asked the CTC to evaluate emission controls from wood chip dryers and press vents at waferboard manufacturing plants. These processes emit particulate matter, formaldehyde, wood decomposition products, and VOCs. The final report focuses on wet electrostatic precipitator and electrified filter control systems and their ability to adequately reduce these emissions. The EPA and State and local air pollution control agency staff should call the CTC HOTLINE at (919) 541-0800 or (FTS) 629-0800 for more information on these new reports or to request CTC service. Others may call Bob Blaszczak at (919) 541-5432 or Chuck Darvin at (919) 541-7633 for more information. NESCAUM RELEASES HEAI OF GASOLINE VAPORS by Margaret Round, Northeast States for Coordli The Northeast States for Coordinated Air Use Management (NESCAUM) has completed a report en- titled "Evaluation of the Health Effects from Exposure to Gasoline and Gasoline Vapors." This report was initiated in response to the growing concern in the Northeast over the known and potential health effects of gasoline, especially as related to ex- posure from gasoline service station operations and from leaking underground storage tanks. This document was developed as a tool for assisting States in their management of gasoline-related health risks, and with the expectation that its findings will be modified to ac- commodate the various risk assessment and risk management approaches that exist among the States in the region. The evaluation estimated exposure of service sta- tion attendants, self-service customers, and nearby residents to gasoline vapor emissions associated with service station operations. Estimates were also deter- mined for residents exposed to gasoline-contaminated drinking water and gasoline vapors which have migrated below ground into their houses from leaking underground storage tanks. A review of the toxicological data was conducted to assess the health significance of these exposures. Because limited data exist regarding the health effects from exposure to gasoline, the evalua- tion also assessed the health impacts associated with three constituents: benzene, toluene, and xylene. Health criteria for cancer and noncancer effects were based on the U.S. EPA cancer potency factors for gasoline and benzene, and the most sensitive non- cancer health effects identified by NESCAUM associated with exposure to gasoline, benzene, toluene, and xylene. These toxicity data were evaluated relative to the six human exposure scenarios associated with en- vironmental releases of gasoline in order to estimate the .TH EVALUATION nated Air Use Management corresponding public health impacts (Table 1). Based on this assessment, all scenarios pose cancer and non- cancer risks from exposure to gasoline and/or three of its constituents. The document presents a qualitative discussion of the major assumptions, uncertainties, and limitations of this quantitative risk assessment. These considerations must be taken into account when applying these data to site-specific cases of exposure to gasoline vapors and in the development of regulatory programs. Report Approach Described Standard risk assessment methods were adopted, although it was necessary to modify them because of limited toxicological data on the mixture and the variabili- ty of the composition of the mixture after it is released into the environment. This assessment of gasoline in- cluded (1) studies on the entire mixture, (2) particular fractions of the mixture, and (3) specific components (benzene, toluene, and xylene) that were considered to have the greatest health impacts. The primary sources of data for refueling exposures were monitoring studies of self-service customers and service station attendants during refueling operations. The exposure assessment accounted for exposure to gasoline vapors both during refueling operations and other time spent at the service station. In the case of residential exposure, dispersion modeling was used to estimate ambient concentrations from service station emissions. Because conditions associated with leaking underground storage tanks can vary significantly from case to case, quantification of exposures was based on limited case study information. Therefore, NESCAUM points out that estimates for exposure and associated risks for any given site need to be determined on a site- specific basis. 6 ------- TABLE 1. POTENTIAL NONCANCER RISKS ASSOCIATED WITH EXPOSURE TO GASOLINE AND SELECTED INDICATOR CONSTITUENTS Estimated Exposure a NESCAUM Margin of Safety Exposure (mg/kg/dayj Reference Dose (ref. dose/exp. dose) Scenario mean maximum (mg/kg/day) mean maximum Scenario 1: self-service customer at gas station exposed via inhalation1,3 gasoline 9.4 x 10 1.0 x 10 0.003 0.32 0.03 benzene 7.3 x 10"5 7.2 x 10"4 0.004 55 5 toluene 5.7 x 10"6 4.9 x 10"4 0.0014 25 3 xylenes 2.2 x 10"5 2.6 x 10"4 0.034 1545 131 Scenario 2: gas station attendant exposed via inhalation1,3 gasoline 1.8 0.003 0.002 benzene 2.1 x 10"2 1.4 x 10"1 0.004 0.19 0.03 toluene 3.8 x 10'2 0.0014 0.04 xylenes 1.5 x 10'2 0.034 2 Scenario 3: resident living downwind of gas station exposed via inhalation1,3 gasoline 3.1 x 10 1.6 x 10 0.003 0.97 0.19 benzene 2.6 x 10"5 1.1 x 10"4 0.004 154 36 toluene 6.2 x 10"5 2.9 x 10'4 0.0014 23 5 xylenes 2.7 x 10'5 1.3 x10"4 0.034 1260 262 Scenario 4: resident inhaling vapors from nearby leaking underground storage tank1,4 gasoline 0.003 - - benzene 3.6x10"' 1.9 0.004 0.01 0.002 toluene 6.2 x 10"1 5.9 0.0014 0.002 0.0002 xylenes 4.2 x 10"1 3.6 0.034 0.08 0.0009 Scenario 5: resident exposed to gasoline via ingestion of contaminated well water2,4 gasoline 1.7x10 2.9 0.003 0.02 0.001 benzene 1.4 x 10"2 7.0 x 10"2 0.004 0.29 0.06 toluene 8.0 x 10'3 5.0 x 10"2 0.0014 0.18 0.03 xylenes 8.6 x 10"3 4.0 x 10"2 0.034 4 0.85 Scenario 6: resident exposed via inhalation and dermal contact during showering1,4,5 gasoline 1.7x10' 3.4x10 0.003 0.02 0.009 benzene 1.4 x 10"2 2.8 x 10'2 0.004 0.29 0.14 oluene 8.0 x 10'3 1.6 x10"2 0.0014 0.18 0.09 xylenes 8.6 x 10'3 1.7 x 10"2 0.034 4 2 a These calculations are presented in the report's exposure assessment chapter. Assumes inhalation of 14.4 cu M/day, 24 h/day. 2 Assumes ingestion of 2L water/day. Based upon arithmetic means of monitoring studies described in the report's exposure assessment chapter. Based upon limited case-study information. Estimated risks for any given site need to be determined on a site-specific basis. 5 Assumes mean values equal mean drinking water exposures, and upper limits equal twice drinking water maxima. Health Effects Identified studies after protracted exposure to gasoline vapors Acute exposure to gasoline and its components were pulmonary toxicity and nephrotoxicity. Reproduc- benzene, toluene, and xylene has been associated with tive and developmental effects were among the most skin and sensory irritation, central nervous system sensitive noncancer toxic endpoints for benzene, depression, and effects on the respiratory system. Pro- toluene, and xylene exposures. These effects includ- longed exposure to these compounds also affects these ed increased resorptions, reduced fetal body weight, organs as well as the kidney, liver, and blood systems. and delayed skeletal development, and in the case of In general, the effects that have been identified follow- benzene, induced bone marrow suppression in off- ing gasoline exposure were also identified for one or spring. more of the components of gasoline evaluated in this With respect to carcinogenic effects, one adequate assessment. For example, all substances have been carcinogen bioassay for gasoline vapors was identified shown to be neurotoxic and studies that indicated that that reported statistically significant increases in kidney gasoline is hematotoxic were supported in the assess- tumors in male rats and hepatocellular tumors in mice. ment by the abundant literature on benzene hematotox- Major uncertainties were (1) the vapor composition in icity. The primary effects reported in several animal this study was different from the ambient human 7 ------- environment and (2) the kidney tumors observed in male rats may be the result of a mechanism specific to the male rat and not female rats or other species. Sufficient evidence, however, was not available on the mechanism of male rat kidney tumors to discount the positive car- cinogenicity data from this bioassay. With respect to benzene, an association between benzene exposure and hematopoietic tumors has been found in epidemiology studies. Thus, carcinogenicity of gasoline and benzene was corroborated in more than one study, by multiple routes of exposure, and in at least two species of laboratory animals. It was the finding of NESCAUM's evaluation that the animal and human data provided sufficient evidence for presuming gasoline to be a probable human carcinogen. Risk Assessment Conducted In NESCAUM's quantitative assessment for non- cancer effects, critical studies were identified in the areas of general toxicity, reproductive and developmen- tal toxicity, and genetic toxicity. After the most sensitive toxicological responses were identified, the studies most appropriate for risk assessment based on study design and toxicological relevance were selected for the risk assessment. The most sensitive health effects associated with gasoline, benzene, toluene, and xylene were kidney toxicity (gasoline); developmental effects (benzene); neurotoxic effects (toluene); and reproduc- tive and fetotoxic effects (xylene). Comparisons of human equivalent doses for the lowest effect levels observed in animal studies showed that sensitive toxicity endpoints for each substance reviewed in this assessment (gasoline, benzene, toluene, and xylene) are associated with fairly definable dose ranges. For gasoline, kidney toxicity is associated with human equivalent doses in the 2 to 4 mg/kg/day dose range. For benzene, hematotoxicity occurs in the dose range of 0.1 to 1.0 mg/kg/day. For toluene, thresholds for sensitive neurobehavioral, hematological, and immunological effects occur in the dose range of 0.5 to 1.5 mg/kg/day. Risk Characterization Procedures Explained Estimated cancer and noncancer risks for each of the six scenarios were based upon comparison of health criteria with estimated exposure doses. The health criteria for cancer effects were cancer potency values; the health criteria for noncancer effects were NESGAUM reference doses. Several uncertainties were associated with quantifying cancer and noncancer risks to humans based upon data from animal bioassays and epidemiological studies. These uncertainties included: (1) estimates may exclude gasoline components of potential concern; (2) inaccuracies in the assumptions about the intensity and duration of exposure; (3) lack of information on interactive effects among constituents in the complex mixture, and (4) uncertainties associated with exposure of sensitive individuals, including preg- nant women, the very young, and the old or infirm, as well as individuals who may suffer from chronic respiratory, immunological, or other predisposing illnesses. These and other uncertainties warranted the adoption of conservative assumptions, when possible, so that any errors were made on the side of caution. A reflection of these uncertainties was provided in the assessment by both average and upper limit exposure doses and health criteria. Noncancer health risks associated with gasoline ex- posure are presented in Table 1. Both mean and worst- case exposure assumptions yield estimates of exposure doses that are greater than reference doses derived in this assessment. Some margins of safety, however, ex- ist with regard to specific indicator substances under all scenarios. Potential individual lifetime (70 years) cancer risks associated with exposure to unleaded gasoline and benzene were presented in the assessment. These cancer risks were based on a cancer potency value of 0.0035 per mg/kg/day for gasoline and 0.026 mg/kg/day for benzene. The exposure doses corresponding to one in a million cancer risk for gasoline and benzene were estimated to be 2.8 x 10"4 mg/kg/day and 3.8 x 10 s mg/kg/day, respectively. Based upon an evaluation of available data, toluene and xylene were assigned cancer potency values of zero. Maximum individual lifetime cancer risks associated with gasoline and/or benzene are estimated below. SCENARIO MAXIMUM INDIVIDUAL LIFETIME RISK(1> Scenario 1 3.5 x 10"4<2) Scenario 2 3.6 x 10'3(1) Scenario 3 5.6 x 10"5(2> Scenario 4 4.9 x 10'2(1) Scenario 5 1.0 x 10"2(Z) Scenario 6 1.1 X 103(z> (1) Maximum individual lifetime risks based on max- imum exposure to benzene. (2) Maximum individual lifetime risks based on max- imum exposure to gasoline (see Table 1 for exposure doses). It should be noted that although the exposure doses for scenarios 4,5, and 6 were based on data from limited case studies, significant risks may be associ- ated with such exposures. Estimated risks for any given site, however, need to be determined on a site-specific basis. Copies of the document are available from the NESCAUM office. The price is $90.00 ($35.00 for government or nonprofit agencies). For details, please call Margaret Round, Toxics Coordinator, NESCAUM, at (617) 367-8540. 8 ------- EPA ISSUES POLICY DIRECTIVE ON AIR STRIPPERS AT SUPERFUND SITES Approximately 35 percent of the Superfund Records of Decision signed to date have involved the use of a pump-and-treat technique to either partially or fully remediate ground-water contamination. Almost 45 per- cent of these pump-and-treat sites have chosen air strip- ping, a technique that uses volatilization to remove volatile organic compounds (VOCs) from the ground water. One known side effect of air stripping is that the VOCs, many of which are toxic, are released to the am- bient air. Control devices such as vapor carbon adsorp- tion and incineration are used on 60 percent of the air strippers to control these emissions, according to analyses by EPA's Office of Emergency and Remedial Response (OERR) and the Office of Air Quality Plan- ning and Standards (OAQPS). Despite a trend toward increased control of air emis- sions from air strippers at Superfund sites, EPA remains concerned with the control of these VOC emissions. This concern is underlined by the vigorous efforts by EPA, State, and local agencies, and industries across the country to control air toxics and reduce VOC emissions in ozone nonattainment areas. As a result of this con- cern, OERR and OAQPS issued an OERR policy direc- tive on June 15,1989, to provide guidance to the Super- fund program on the control of VOC emissions from air strippers at Superfund sites. The policy directive states that for sites in ozone at- tainment areas, the EPA Regions should continue to im- plement Applicable or Relevant and Appropriate Requirements (ARARs) which include State regulations, risk management (i.e., protectiveness) guidelines, and other requirements of Section 121 of the Comprehensive Environmental Response, Compensation, and Liability Act. In ozone nonattainment areas, however, the adoption of controls is more likely to be indicated even if the controls are not mandated by current Federal or State regulations or indicated by a cancer risk analysis. Aside from their contributions to cancer risk, most constituents of VOC emissions are precursors to the formation of ozone. Consideration of these impacts during remedy selection generally will show that Superfund air strippers, except those with the lowest emission rates, generally merit controls in nonattainment areas. In determining the need for air stripper controls at a particular Superfund site in a nonattainment area, the guidance indicates that the sources most in need of controls are those with actual VOC emission rates in excess of 3 pounds per hour, 15 pounds per day, or a potential (i.e., calculated) rate of 10 tons per year. The calculated rate assumes 24-hour operation, 365 days per year. Control limits are applied on a facility basis. For the purposes of this directive, "facility" is defined as a contiguous piece of property under common ownership. The potential for applicability of the directive to other VOC sources at Superfund sites is recognized. General- ly, the guidelines described for air strippers are suitable for VOC emissions from other vented extraction tech- niques (e.g., soil vapor extraction) but not from area sources (e.g., soils excavation). The policy directive applies to future remedial deci- sions at Superfund sites. It is not designed explicitly for actions taken by the removal program in the case of emergency or time-critical removal actions. However, where time and other response circumstances permit, such as for nontime-critical actions, adherence to the directive is expected. The control levels referred to in the directive serve as guidelines only if ARARs do not exist or are less stringent. They are not intended to preclude or replace State proposals for more stringent levels of control in pur- suit of the Clean Air Act goals as part of SIP revisions in nonattainment areas. The remedial investigation/feasibility studies of Superfund sites should generate the data needed to sup- port control decisions for both attainment and nonattain- ment areas. At a minimum, the five major types of infor- mation needed are: - Estimated cumulative uncontrolled air emis- sions rate from all air strippers at the site, - Consideration of health risks from the execution of the remedy as well as from the uncontrolled site, - Control alternatives and their costs, - Ozone attainment status, and - Air ARARs. For purposes of the policy directive "nonattainment area" means any county included in a formal post-1987 ozone SIP deficiency notification (SIP call) or any other county where the ozone National Ambient Air Quality Standard (NAAQS) was exceeded during the previous three-year period. EPA's initial SIP calls were issued pur- suant to Section 110(a)(2)(H) of the Clean Air Act and were described in the September 7, 1988, Federal Register. Questions concerning the policy directive should be directed to Joe Padgett, U.S. EPA, OAQPS, at (919) 541-5589 or (FTS) 629-5589. 9 ------- ALL STATES NOW ADDRESS AIR TOXICS, STAPPA/ALAPCO SURVEY FINDS Many State and local air pollution control agencies have developed or are now developing regulatory pro- grams, which go beyond implementation of Federal rules, to address toxic air pollutants. STAPPA/ALAPCO, in a collaborative effort with the EPA's Air Quality Management Division, recently surveyed 50 State and 220 local air pollution control agencies to determine the extent of each agency's existing or planned program for controlling toxic air pollutants. This survey updates one conducted in 1984. The results of the 1989 survey are compiled in a report entitled "Toxic Air Pollutants: State and Local Regulatory Strategies - 1989." The survey solicited information on all aspects of the agencies' air toxics programs, including enabling legisla- tion and administrative rules, program scope, control ap- proaches, implementation mechanisms, collection of toxic emissions data, level of agency effort, EPA assistance, and the effect of SARA Title III on their pro- grams. All 50 States and 40 local agencies responded to the survey. Since all 50 States also responded to the 1984 survey, it is possible to assess the progress in State air toxics program development that has occurred over the past 5 years. Air toxics control activity in the States has increased significantly in the past 5 years. In 1984 only 19 States had policies or regulations in place, and 23 had plans to develop programs. Today, every State addresses air toxics, either through a regulatory program (12 States), comprehensive policy (22 States), or more informally through New Source Review (16 States). Of the 40 local agencies that responded to the survey, 16 have air tox- ics programs in place for new sources and 11 are plan- ning programs. In addition, four local agencies have regulatory programs for existing sources and three have comprehensive policies. Most State and local agencies noted several reasons for having a control program, the most common being agency and public concern about health effects. Many agencies also cited the need for prevention of potential adverse health effects and EPA policy as reasons for developing a program. Not surprisingly, State and local agencies are spending more time and money on their air toxics con- trol programs than they were in 1984. Figure 1 illustrates the number of work-years that States devoted to air tox- ics activities in the past year compared to 1984. The me- dian number of work-years States spent on air toxics is 5.4, compared to a median of 1 work-year in 1984. Local agencies spent a median of 1.8 work-years on air toxics in the past year. Out of six types of activities addressed in the survey, most agencies spent the most amount of time on permitting activities, and the least on enforce- ment. In 1984, the median annual spending level for State agencies was $52,500. The 1989 survey indicated a me- dian funding level of $330,000. Figure 2 illustrates the in- crease in State funding from 1984 to 1989. The local agencies that responded to the 1989 survey reported an annual median funding level of $51,000. State agencies reported spending the most money on monitoring ac- tivities, while local agencies reported spending the most on permitting. Typically, most State and local programs are supported through a combination of their own funds and Federal grants. Several agencies reported receiv- ing a portion of their funding from operating permit fees or inspection fees. The agencies were also asked what type of assistance they wished to receive from EPA for their air toxics programs. The three highest priority areas cited by both State and local agencies were the need for health effects information, acceptable emission levels, and control techniques. More detailed information on these and many other topics can be found in the complete compilation of the survey results. In addition, a summary of the air toxics program of each of the agencies that responded to the survey is included in the document. For more informa- tion on obtaining a copy of "Toxic Air Pollutants: State and Local Regulatory Strategies-1989," contact STAPPA/ALAPCO at (202)624-7864. Figure 1. Comparison of State Agency Work Years Devoted to Air Toxics -1984 versus 1989 Years (37) 5-10 Years (5) 1984 1989 Note: Number of Agencies Shown in Parentheses Figure 2. Comparison of Annual Funding for State Air Toxics Programs Number of States 1984 Number of States 1989 10 ------- TAMS UPDATE: SYSTEM Wl A RESEARCH VEHICLE Experience gained in Volatile Organic Compounds (VOC) monitoring through the Toxic Air Monitoring System (TAMS) has enabled other programs such as the Urban Air Toxics Monitoring Program (UATMP) to pro- vide routine monitoring to further the goals of urban air toxics assessment. With the growth of the UATMP, the TAMS was recently reassessed to consider the need for field evaluation of polar compounds, semivolatiles, and ozone precursors. Upon evaluation, it was concluded that the TAMS should remain a research vehicle, and that an orderly phase-out of some of the sites would be necessary in order to explore monitoring methods for these other pollutants. To accomplish these goals, the LL REMAIN number of sites was reduced from 10 to 4. Presently, the TAMS consists of two sites each in Houston and Boston where VOCs, polar compounds, semivolatiles, for- maldehyde, and ozone precursor monitoring methodologies can be explored. Further information on the TAMS is available in the form of status reports that are distributed on a regular schedule. Additionally, a statement of the quality of data needed to support specific programs, known as the data quality objective, has been prepared for the TAMS. For further information, call Jane Leonard, OAQPS, Technical Support Division, at (919) 541-5653 or (FTS) 629-5653. EPA MOVES TO REDUCE Bl In September, EPA finalized rules* expected to result in 20,000 tons of reductions in emissions of benzene** from industrial sources. The final regulations require 97 percent emissions reductions from coke byproduct recovery plants and also significant reduc- tions from benzene storage tanks. In addition to its final rules, EPA also proposed requirements for other major benzene sources*** expected to result in an additional reduction of 14,000 tons per year. In all, benzene emis- sions would be reduced by 90 percent from current levels. A known human carcinogen, benzene is a major in- dustrial chemical that has been linked to adult leukemia. Benzene is used to manufacture a wide variety of prod- ucts including plastics, insecticides, and polyurethane foam. Benzene emissions are also present in automobile exhaust, automobile refueling operations, cigarette smoke, and many consumer products. Exposure to emissions of benzene from these two industrial sources represents an important long-term health concern, particularly for those who live close to major emitting facilities. Half the U.S. population is ex- posed to these sources, which account for 20 percent of the benzene emissions in this country. The procedure used to establish the level of the benzene emissions standards resulted from a 1987 court decision (Natural Resources Defense Council v. EPA) remanding to EPA earlier hazardous standards for vinyl chloride. The court held that EPA should use a two-step standard-setting process. First, the Agency must establish a level of emissions that is considered safe or acceptable based only on consideration of the potential health impacts of exposure. In the second step, this level may be reduced further upon consideration of control cost or technical feasibility to provide an ample margin of safety. For the benzene source categories, EPA estab- EIMZENE AIR EMISSIONS lished a presumptive health benchmark for an unaccep- table exposure level at a maximum individual lifetime risk of developing cancer of 1 in 10,000. Although other health risk measures and the inherent scientific and technical uncertainties are considered in the decision of what level of emissions is acceptable, the EPA's policy is to ensure that few, if any, members of an exposed population are exposed to levels at or above those associated with a 1 in 10,000 lifetime risk. A secondary goal is to ensure that as much of the exposed popula- tion as possible does not face a lifetime risk greater than one chance in one million. With the application of the benzene rules, over 99 percent of the exposed popula- tion would be below the one in one million lifetime risk. In addition to the rules promulgated in September, rules were proposed for several additional categories. The proposed rules will achieve a 94 percent cut in benzene emissions from railroad tank cars, trucks, boats, and other transfer operations; a 95 percent reduction from process vents in pharmaceutical manufacturing; a 75 percent reduction from rubber tire manufacturing; as well as reductions from benzene waste operations and reductions from gasoline terminals, plants, and service stations. The final and proposed rules represent EPA's first hazardous air pollutant rulemaking since the landmark 1987 vinyl chloride ruling. * National Emission Standards for Hazardous Air Pollutants (NESHAP) 54 FR 38044, September 14, 1989. ** See related articles in September 1987 and May 1988 Newsletters. *** Benzene waste operations including waste water treatment; waste treatment, storage, and disposal facilities; gasoline transfer operations; gasoline marketing operations; and solvent use. 11 ------- CALL NEW CONTACT FOR SECTION 313 RISK SCREENING GUIDE The September issue of the Newsletter an- nounced that EPA's Section 313 "Toxic Chemical Release Inventory Risk Screening Guide" is available. The contact for the document has now changed. For ad- ditional information on the Guide, write Lawrence S. HELPFUL NUMBERS Air Risk Information Support Center (Air RISC Hotline): (919) 541-0888 (FTSJ 629-0888 Control Technology Center (Hotline): (919) 541-0800 (FTS) 629-0800 NATICH Clearinghouse Staff: (919) 541-0850 (FTS) 629-0850 The National Air Toxics Information Clearinghouse Newsletter is published six times a year by the National Air Toxics Information Clear- inghouse to assist State and local agencies making decisions on noncriteria pollutant emissions. The first issue appeared in December 1983. The Clearinghouse is being implemented by the U.S. Environmental Protection Agency, Emission Standards Division, Pollutant Assessment Branch as part of a joint effort with the State and Local Air Pollution Control Officials (ALAPCO). The National Air Toxics Information Clearinghouse Newsletter is prepared by Radian Corporation under EPA Contract Number 68-D8-0065, Work Assignment 21. The EPA Project Officer is Scott Voorhees, EPA Office of Air Quality Planning and Standards, Research Triangle Park, North Carolina 27711, Telephone: (919)541-5348. The Radian Project Director is Caroline Brickley, P. O. Box 13000, Research Triangle Park, North Carolina 27709, (919)541-9100. The Newsletter is prepared primarily for State and local air pollution control agencies and is distributed free of charge. Those wishing to report address changes may do so by writing Meredith Haley, Radian Corporation, P. O. Box 13000, Research Triangle Park, North Carolina 27709. Please contact the Project Officer either with any comments you might have pertaining to this newsletter or with suggestions for future newslet- ters. Articles in the newsletter are written by Radian Corporation or EPA staff unless otherwise indicated. The views expressed in the National Air Toxics Information Clearinghouse Newsletter do not necessarily reflect the views and policies of the Environmental Protection Agency. Mention of trade names or commercial products does not constitute any endorsement or recommenda- tion for use by EPA. Rosenstein, Acting Director, Regional Risk Guidance Staff, U.S. Environmental Protection Agency, (TS-778), 401 M Street S.W., Washington, DC 20460, or call (202) 382-3628, (FTS) 382-3628. Scott Voorhees Pollutant Assessment Branch U.S. Environmental Protection Agency MD-13 Research Triangle Park, NC 27711 FIRST CLASS MAIL U.S. Postage Paid E.P.A. Permit No. G-35 L:i tarar y EPA, Regi on II t'J <_¦ o d b r :i. d q e A v e n u e [I d i s a n N J M ' iiiinliitiiiil'iill'l'"!''"" ------- |