ANNUAL REPORT
FY 86

ENVIRONMENTAL MONITORING AND SUPPORT LABORATORY
OFFICE OF RESEARCH AND DEVELOPMENT
U.S. ENVIRONMENTAL PROTECTION AGENCY
CINCINNATI, OHIO 45268

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^\|/^ 1 UNITED STATES ENVIRONMENTAL PROTECTION AGENCY

OFFICE OF RESEARCH AND DEVELOPMENT
ENVIRONMENTAL MONITORING AND SUPPORT LABORATORY

CINCINNATI. OHIO 45268	S}

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DATE: December 15, 1986

SUBJECT: FY86 Environmental Monitoring and Support Laboratory - Cincinnati
(EMSL-Cincinnati) Annual Report

FROM: Robert L. Booth, Director	/.

Environmental Monitoring and Support /

Laboratory - Cincinnati

TO:	SEE BELOW

Merry Christmas and Happy New Year to all	of you!

The following pages summarize the purpose of our projects, approach used,

and accomplishments. If additional copies are	needed for distribution to other

key staff members, please call us at 684-7301.	Selected highlights from FY86
are:

° Published and distributed "Short-term Methods for Estimating the Chronic
Toxicity of Effluents and Receiving Waters to Freshwater Organisms" (EPA-
600/4-85-014).

0 Revised Chapter 8 and Chapter 9 of the "USEPA Manual of Methods for Virology"
The latter chapter has been divided into two new chapters, the first of which
was completed and has received Agency clearance, "Cell Culture Preparation
and Maintenance". The second part, "Cell Culture Procedures for Virus Assay"
is near completion and distribution will be made in FY87.

° Established a computer-based information exchange system (bulletin board)
to provide access by the user community to IBM PC-AT compatible versions of
a biological statistics package currently containing 45 programs.

o Prepared draft interim report on "Evaluation of a Microbial Test for Muta-
genicity of Wastewater" which describes preliminary precision and accuracy
determinations performed with the Ames test.

0 Forwarded the final report on the comparison of the hydrophobic grid membrane
filter (HGMF) with the standard membrane filter and submitted for journal
publication.

° Completed laboratory Performance Evaluation (PE) Studies Water Pollution
(WP) 015 and 016 and distributed reports to the participants on how they
performed on the unknown samples.

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2

0 Completed Water Supply (WS) 18 and WS19 PE studies for certification under
the requirements of the Safe Drinking Water Act (SDWA). Overall, 2000
laboratories participated in these studies for measuring the contaminants
near the maximum contaminant level (MCL).

0 Completed WSM07 and WSM08 microbiological PE studies. Approximately 100
regional and state laboratories participated in these studies for total
coliforms at two concentration levels.

0 Provided over 285,000 WP quality control (QC) samples to U. S. Environmental
Protection Agency (USEPA), regional, state, and USEPA contractors. Addition-
ally, distributed approximately 75,000 spiking/calibration solutions in
support of regulations under the Clean Water Act and Consent Decree for
Priority Pollutants.

0 Provided final report to each participating laboratory in the Discharge
Monitoring Report-Quality Assurance (DMR-QA) study 6 (approximately 7400
major National Pollutant Discharge Elimination System (NPDES) dischargers).

0 Prepared and distributed three special interlaboratory comparison studies to
evaluate Resource Conservation and Recovery Act (RCRA) contract laboratories.

0 Prepared and distributed special inorganic and organic PE samples for con-
tract laboratories involved in groundwater monitoring.

0 Provided full-volume natural wastewater samples spiked with organic toxi-
cants to Superfund contract laboratories on a quarterly basis as a measure
of their potential performance.

0 Completed a special project to develop a method for acid soluble metals and
presented an overview at the Society for Applied Spectroscopy Seminar on
Atomic Spectroscopy.

° Provided a "Report on Evaluation of Metals Dissolution for Chromium" to the
Office of Solid Waste (0SW).

0 Redrafted and forwarded final rule of the October 26, 1984, Interim rule on
priority pollutants to the Office of General Counsel and the Work Group for
comment. Maintained a continuing project to correct inadequacies of 304(h)
methods for application to specific matrices.

° Submitted a paper for publication entitled "A Universal Kriging Program for
the IBM-PC for Use in Monitoring Sediments 1n Lakes", as part of the Symposium
Proceedi ngs.

° Processed a total of 74 requests for alternate test procedures (ATPs), 51 of
which were related to NPDES and 23 to the SDWA requirements. Of the total,
34 were approved; 6, disapproved; 24 required additional data; 4, pending;
and 6 were not-germane (not ATPs).

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3

° Transmitted a revised manual entitled "Methods for Volatile Organic Chemicals"
to the Office of Drinking Water.

° Held two certification training courses for state and regional persons:
Drinking Water Chemical Laboratory Certification Course and Drinking Water
Microbiological Laboratory Certification Course.

° Made on-site visits to four regional laboratories during the fiscal year. At
the request of Regions 2 and 8, also evaluated the United States Geological
Survey laboratory in Denver, Colorado, for compliance with drinking water
regulations.

° Continued the evaluation and testing of several SW-846 methods.

° Participated in the National Inorganic and Radiological Survey by providing
analytical results for 37 elements on 475 samples totalling 22,191 analyses,
and analyzed 1176 radionuclide samples.

° Developed an enzyme linked immunosorbent assay technique for the measurement
of dioxins and furans. Plans are to field test this immunochemical method
in FY87.

° Provided methods manual report on "Standard Methods for Collection and
Analysis of Precipitation".

Attachments (66):

Annual Report for Each Project

ADDRESSEES:

Vaun Newill, Assistant Administrator, Office of Research and Development (RD-672)
Donald Ehreth, Deputy Assistant Administrator, Office of Research and Develop-
ment (RD-672)

Courtney Riordan, Director, Office of Acid Deposition, Environmental Monitor-
ing, and Quality Assurance (RD-680)

H. Matthew Bills, Deputy Director, Office of Acid Deposition, Environmental

Monitoring, and Quality Assurance (RD-680)

Alan Neuschatz, Special Assistant to the Director, Office of Acid Deposition,

Environmental Monitoring, and Quality Assurance (RD-680)

Paul Palm, Chief, Program Operations Staff, Office of Acid Deposition, Environ-
mental Monitoring, and Quality Assurance (RD-680)

Stanley Blacker, Director, Quality Assurance Management Staff, Office of Acid

Deposition, Environmental Monitoring, and Quality Assurance (RD-680)

Gary Foley, Director, Acid Deposition and Atmospheric Research Division, Office
of Acid Deposition, Environmental Monitoring, and Quality Assurance (RD-680)
Charles Brunot, Director, Environmental Monitoring Systems Division, Office of
Acid Deposition, Environmental Monitoring, and Quality Assurance (RD-680)

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4

Richard Nalesnik, Special Assistant to the Director, Environmental Monitoring
Systems Division, Office of Acid Deposition, Environmental Monitoring, and
Quality Assurance (RD-680)

Charles Plost, Chemist, Environmental Monitoring Systems Division, Office of
Acid Deposition, Environmental Monitoring, and Quality Assurance (RD-680)

Vernon Laurie, Program Analyst, Environmental Monitoring Systems Division,

Office of Acid Deposition, Environmental Monitoring, and Quality Assurance
(RD-680)

John Koutsandreas, Environmental Scientist, Environmental Monitoring Systems
Division, Office of Acid Deposition, Environmental Monitoring, and Quality
Assurance (RD-680)

Michael Dellarco, Environmental Scientist, Environmental Monitoring Systems
Division, Office of Acid Deposition, Environmental Monitoring, and Quality
Assurance (RD-680)

David Graham, Environmental Monitoring Systems Division, Office of Acid Deposi-
tion, Environmental Monitoring, and Quality Assurance (RD-680)

Jack Puzak, Acting Director, Environmental Monitoring Systems Laboratory - Research
Triangle Park

Erich Bretthauer, Director, Environmental Monitoring Systems Laboratory - Las
Vegas

Alfred Ellison, Director, Atmospheric Sciences Research Laboratory - Research
Triangle Park

Thomas Hauser, Director, Hazardous Waste Engineering Research Laboratory -
Cincinnati

Francis Mayo, Director, Water Engineering Research Laboratory - Cincinnati
Lowell Van Den Berg, Director, Technical Support Division, Office of Drinking
Water

Herbert Brass, Chief, Drinking Water Quality Assessment Branch, Technical Sup-
port Division, Office of Drinking Water
Calvin Lawrence, Director, Center for Environmental Research Information
Frank Princiotta, Director, Air and Energy Engineering Research Laboratory -

Research Triangle Park
Lester Grant, Director, Environmental Criteria and Assessment Office - Research
Triangle Park

Jerry Stara, Director, Environmental Criteria and Assessment Office - Cincinnati
Rosemarie Russo, Director, Environmental Research Laboratory - Athens
Clinton Hall, Director, Robert S. Kerr Environmental Research Laboratory - Ada
Thomas Murphy, Director, Environmental Research Laboratory - Corvallis
Norbert Jaworski, Director, Environmental Research Laboratory - Narragansett
Gilman Velth, Acting Director, Environmental Research Laboratory - Duluth
Henry Enos, Director, Environmental Research Laboratory - Gulf Breeze
F. Gordon Hueter, Director, Health Effects Research Laboratory - Research
Triangle Park

Rebecca Hanmer, Deputy Assistant Administrator for Water (WH-556)

Joseph Cotruvo, Director, Criteria and Standards Division, Office of Drinking
Water (WH-550)

Arthur Perler, Chief, Science and Technology Branch, Criteria and Standards
Division, Office of Drinking Water (WH-550)

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5

Irwin Pomerantz, Quality Assurance Officer, Science and Technology Branch,

Criteria and Standards Division, Office of Drinking Water (WH-550)

Maria Gomez-Taylor, Chemist. Health Effects Branch, Criteria and Standards

Division, Office of Drinking Water (WH-550)

Paul Berger, Microbiologist, Health Effects Branch, Criteria and Standards

Division, Office of Drinking Water (WH-550)

Arnold Kuzmack, Director, Program Development and Evaluation Division, Office

of Drinking Water (WH-550)

Marian Ml ay, Director, Office of Ground-Water Protection (WH-550G)

Tudor Davies, Director, Office of Marine and Estuarine Protection (WH-556M)
Michael Quigley, Director, Office of Municipal Pollution Control (WH-546)

James Elder, Director, Office of Water Enforcement and Permits (EN-335)

J. William Jordan, Director, Enforcement Division, Office of Water Enforcement

and Permits (EN-338)

Martha Prothro, Director, Permits Division, Office of Water Enforcement and
Permits (EN-336)

William Brandes, Permits Division, Office of Water Enforcement and Permits
(EN-336)

Geoffrey Grubs, Permits Division, Office of Water Enforcement and Permits
(EN-336)

Marcia Williams, Director, Office of Solid Waste (WH-562)

Jeffery Denit, Deputy Director, Office of Solid Waste (WH-562)

David Friedman, Manager, Methods Program, Characterization and Assessment

Division, Office of Solid Waste (WH-562B)

Paul Friedman, Characterization and Assessment Division, Office of Solid Waste
(WH-562B)

Florence Richardson, Quality Assurance Officer, Characterization and Assessment

Division, Office of Solid Waste (WH-562B)

Stanley Kovell, Chief, Analytical Support Branch, Hazardous Response Support

Division, Office of Program Management (WH-548A)

William Garetz, Environmental Results Branch, Management Systems Division,

Office of Management Systems and Evaluation (PM-222A)

R. Augustus Edwards, Deputy Assistant Administrator, Office of External Affairs
(A-100EA)

Hugh McKinnon, Co-Chairperson, Consolidated Water Research Committee (RD-682)
Curtis Harlin, Office of Regulatory Support (RD-672)

Victoria Price, Office of Water (WH-556)

William Whittington, Director, Office of Water Regulations and Standards (WH-551)
Devereaux Barnes, Director, Industrial Technology Division, Office of Water

Regulations and Standards (WH-552)

Frederic Leutner, Acting Director, Monitoring and Data Support Division, Office

of Water Regulations and Standards (WH-553)

Timothy Stuart, Chief, Monitoring Branch, Monitoring and Data Support Division,

Office of Water Regulations and Standards (WH-553)

Edmund Notzon, Director, Criteria and Standards Division, Office of Water

Regulations and Standards (WH-585)

James McDermott, Scientific and Technical Advisor, Criteria and Standards
Division, Office of Water Regulations and Standards (WH-585)

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6

David Davis, Deputy Director, Office of Federal Activities (A-104)

Robert Wolcott, Director, Regulatory and Economic Analysis Division, Office of

Policy Analysis, Office of Policy, Planning, and Evaluation (PM-221)

Samuel Bryant, Program Analyst, Budget Division, Office of the Comptroller
(PM-225)

Richard Frank, Program Analyst, Planning Staff, Office of Research Program
Management (RD-674)

Brenda Washington, Management Analyst, Program Coordination Staff, Office of

Research Program Management (RD-674)

Michael Deland, Regional Administrator, U. S. Environmental Protection Agency,

Region 1, Attention: Lester Sutton, Research and Development Contact
Paul Keough, Deputy Regional Administrator, U. S. Environmental Protection
Agency, Region 1

Christopher Dagget, Regional Administrator, U. S. Environmental Protection
Agency, Region 2, Attention: Barbara Metzger, Research and Development
Contact

William Muszynski, Deputy Regional Administrator, U. S. Environmental Protection
Agency, Region 2

James Seif, Regional Administrator, U. S. Environmental Protection Agency,

Region 3, Attention: John Ruggero, Research and Development Contact
Stanley Laskowski, Deputy Regional Administrator, U. S. Environmental Protec-
tion Agency, Region 3
Jack Ravan, Regional Administrator, U. S. Environmental Protection Agency,

Region 4, Attention: David Hopkins, Research and Development Contact
Lee DeHihns, Deputy Regional Administrator, U. S. Environmental Protection
Agency, Region 4

Valdas Adamkus, Regional Administrator, U. S. Environmental Protection Agency,
Region 5, Attention: William Sanders, III, Research and Development Contact
Frances Phillips, Acting Regional Administrator, U. S. Environmental Protection
Agency, Region 6, Attention: Oscar Ramirez, Jr., Research and Development
Contact

Morris Kay, Regional Administrator, U. S. Environmental Protection Agency,

Region 7, Attention: Ralph Hazel, Research and Development Contact
William R1ce, Deputy Regional Administrator, U. S. Environmental Protection
Agency, Region 7

John Welles, Regional Administrator, U. S. Environmental Protection Agency,

Region 8, Attention: Denis Nelson, Research and Development Contact
Alexandra Smith, Deputy Regional Administrator, U. S. Environmental Protection
Agency, Region 8

Judith Ayres, Regional Administrator, U. S. Environmental Protection Agency,

Region 9, Attention: Arnold Den, Research and Development Contact
John Wise, Deputy Regional Administrator, U. S. Environmental Protection Agency,
Region 9

Robbie Russell, Regional Administrator, U. S. Environmental Protection Agency,

Region 10, Attention: Carolyn Wilson, Research and Development Contact
Ralph Bauer, Deputy Regional Administrator, U. S. Environmental Protection
Agency, Region 10

Edward Conley, Director, Environmental Services Division, U. S. Environmental
Protection Agency, Region 1

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Barbara Metzger, Director, Environmental Services Division, U. S. Environmental

Protection Agency, Region 2
Greene Jones, Director, Environmental Services Division, U. S. Environmental

Protection Agency, Region 3
James Finger, Director, Environmental Services Division, U. S. Environmental

Protection Agency, Region 4
William Sanders, III, Director, Environmental Services Division, U. S. Envi-
ronmental Protection Agency, Region 5
Russell Rhoades, Director, Environmental Services Division, U. S. Environmental

Protection Agency, Region 6
John Wicklund, Director, Environmental Services Division, U. S. Environmental

Protection Agency, Region 7
James Lehr, Director, Environmental Services Division, U. S. Environmental

Protection Agency, Region 8
David Mowday, Deputy Director, Office of Policy and Management, U. S. Environ-
mental Protection Agency, Region 9
William Schmidt, Acting Director, Environmental Services Division, U. S. Envi-
ronmental Protection Agency, Region 10
Michael Mastracci, Director, Regional Services Staff, Office of Research Program

Management (RD-675)

Robert Booth, Director, Environmental Monitoring and Support Laboratory -
Cincinnati

Thomas Clark, Deputy Director, Environmental Monitoring and Support Laboratory -
Cincinnati

Terry Grady, Chemist, Equivalency Staff, Environmental Monitoring and Support

Laboratory - Cincinnati
Robert Graves, Technical Advisor, Environmental Monitoring and Support Laboratory -
Cincinnati

Daniel Bender, Quality Assurance Management Staff Liaison, Environmental Monitoring

and Support Laboratory - Cincinnati
Teresa Firestone, Budget Analyst, Environmental Monitoring and Support Laboratory -
Cincinnati

James Llchtenberg, Chief, Physical and Chemical Methods Branch
James Longbottom, Chief, Organic Analyses Section, Physical and Chemical Methods
Branch

Gerald McKee, Chief, Inorganic Analyses Section, Physical and Chemical Methods
Branch

William Budde, Chief, Advanced Instrumentation Section, Physical and Chemical
Methods Branch

Joseph Roesler, Environmental Engineer, Sampling and Field Measurements Section,

Physical and Chemical Methods Branch
John Winter, Chief, Quality Assurance Branch

Edward Berg, Chief, Project Management Section, Quality Assurance Branch
Harold Clements, Chief, Evaluation Section, Quality Assurance Branch
Cornelius Weber, Chief, Biological Methods Branch
Robert Safferman, Chief, Virology Section, Biological Methods Branch
Robert Bordner, Chief, Microbiology Section, Biological Methods Branch
William Horning, Chief, Aquatic Biology Section, Biological Methods Branch

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FY-86 OUTPUT PLAN
AQUATIC BIOLOGY SECTION, BMB, EMSL-CINCINNATI

WATER QUALITY-MONITORING SYSTEMS AND QUALITY ASSURANCE, BIO

Page J	of 76

PE#

OUTPUT Reference Biological Methods - Water Quality

ORD Contact
Name W.B. Horning

rTc 		778-8-350

FIS No.

Resources:

$(000) 417 K PFT

OPFT

PFTE6.9 OPFTE

Project 01

ANNUAL REPORT - FY86

The manual, "Short-Term Methods for Estimating the Chronic Toxicity of
Effluents and Receiving Waters to Freshwater Organisms,"
(EPA-600/4-85-014) was published and distributed.

A manuscript, "Toxicity Reduction by Municipal Wastewater Treatment in
Ohio," was completed for submission to the Journal of the Water Pollution
Control Federation. This report was the result of a cooperative study
between EMSL-Cincinnati, the Water Engineering Research Laboratory -
Cincinnati, and the Ohio Environmental Protection Agency. The reduction
of toxicity by municipal waste treatment plants was determined by
measuring influent and effluent toxicity.

A computer-based information exchange system (bulletin board) was
established to provide access by the user community to IBM PC-AT
compatible versions of a biological statistics package (BSP) at the
EMSL-Cincinnati Newtown Facility, which currently contains 45 programs.
Approximately 80 requests have been received for the BSP, and 57
individuals have downloaded the BSP directly from the IBM PC.

The Aquatic Biology Section participated in a 10-laboratory study of the
precision of the seven-day fathead minnow larval survival and growth test
sponsored by the American Petroleum Institute and the Electric Power
Research Institute in cooperation with the USEPA and the Chemical
Manufacturers Association. The study was coordinated by thev
Battelle-Columbus Laboratories, and involved testing of seven reference
materials, including effluents, over an eight-month period. The
EMSL-Cincinnati Newtown Facility provided test animals for five of the
participating laboratories.

The annual review of the literature on "Effects of Pollution on
Freshwater Organisms," was completed for publication in the Journal of
the Water Pollution Control Federation, as part of a joint effort with
the Environmental Research Laboratory - Duluth.

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Page 2 of Project No. 01	Page 2 of 76

A report, "Taxonomy of Ceriodaphnia (Crustacea: Cladocera) in U.S.
Environmental Protection Agency Cultures," was completed.

The manuscript, "Short-term Fish and Amphibian Embryo-larval Tests for
Determining the Effects of Toxicant Stress on Early Life Stages and
Estimating Chronic Values for Single Compounds and Complex Effluents,"
based on research funded by EMSL-Cincinnati under a cooperative agreement
with the University of Kentucky, Lexington, was published by Dr. Wesley
Birge and associates in the journal, Environmental Toxicology and
Chemistry. Funding for a new cooperative agreement with the University of
Kentucky, Lexington, entitled "Improvements in Methods for Toxicological
Monitoring of NPDES Effluents with Emphasis on Short-Term Chronic
Procedures," was also approved.

A formal paper, "A Short-term Chronic Toxicity Test Using Daphnia magna,"
was presented at the Tenth ASTM Aquatic Toxicity and Hazard Assessment
Symposium. A poster session, "Comparative Evaluation of Two Short-term
Fathead Minnow Tests for Measuring Chronic Toxicity to Three Reference
Toxicants," was also presented. Both will be submitted to peer-reviewed
publications.

Cultures for four marine species have been established using "Forty
Fathoms" artificial sea salts. These species are: Mysid shrimp
(Mysidopsis bahia), sea urchin (Arbacia punctulata), sheepshead minnow
(Cyprinodon variegatus) and the red macro-alga Champia parvula.

Short-term chronic toxicity tests with these species are being evaluated.

The Aquatic Biology Section supplied 192,000 fathead minnows (in various
life stages) to other USEPA and state laboratories, universities, USEPA
grantees or contractors, and other Federal agencies performing toxicity
tests with effluents or pure compounds in USEPA-related activities.

A meeting of the EMSL-Cincinnati-sponsored Agency Biological Advisory
Committee was held in Cincinnati. The meeting was attended by biologists
from the regional programs, research laboratories, and headquarters
program offices.

Aquatic Biologists participated in on-site visits to the Environmental
Services Division, Region 3, Wheeling Office, and Regions 5 and 6, to
determine compliance with methodology and quality assurance practices for
NPDES and other biomonitoring activities.

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FY-86 OUTPUT PLAN
MICROBIOLOGY SECTION, BMB, EMSL-CINCINNATI

WATER QUALITY - MONITORING SYSTEMS AND QUALITY ASSURANCE

Page __3	of 76

PIt B101

ORO Contact

OUTPl/T Reference Biological Methods - Water Quality

Name

R. Bordner

FTS Ho.

68fl-J31

Resources:

5(000) 265.6Kppj 4.8 QPFT 0.0 PFTE 4.8 OPFTE

0.0

Project 02

ANNUAL REPORT - FY 86

The final report on the comparison of the hydrophobic-grid membrane filter
(HGMF) with the standard membrane filter (MF) and most probable number (MPN)
procedures was forwarded to the Office of Water and submitted to Applied and
Environmental Microbiology for publication. The standard MF and HGMF
procedures did not produce significantly different results.

A draft interim report on "Evaluation of a Microbial Test for Mutagenicity of
Wastewater" was prepared. The report describes preliminary precision and
accuracy determinations performed with the Ames test, and confirms the inhousc
capability to run this test. The test will be used as a reference method for
evaluation of other proposed short-term tests for microbial mutagenicity.
Successful practice trials using resin-packed glass and stainless steel
columns were completed as the initial step in the task to compare the
efficiency of mutagen recovery by three methods of sample preparation used in
performing the Ames Test.

A draft of the interim report entitled "Precision and Relative Accuracy of th(
Membrane Filter and Most Probable Number Total Coliform Methods with Several
Water Types" was completed and awaits typing of several tables. The positive
tube MPN data from this project were tabulated and given to the Computer
Services and Systems Division to calculate the MPN values using the upgraded
computer program developed for EMSL-Cincinnati under the statistical services
contract. A separate report will be prepared describing the application and
availability of the computer program for calculating MPN results.

The project plan and quality assurance plan for the project entitled
"Evaluation of Improved MF methods for Fecal Coliforms in Chlorinated
Effluents" were prepared, and cultures of Escherichia coli and several other
fecal positive organisms were isolated and characterized for use in evaluating
the fecal coliform media.

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Page 2 of Project No. 02

Page 4 of 76

The task to develop, evaluate, and standardize methods for the detection and
enumeration of salmonellae in sludges, wastewater, and leachates was initiated
with an on-line literature search of several data bases. A feasibility study
was conducted to determine if the HGMF could be used in a quantitative
technique for salmonellae. The procedure shows promise based on preliminary
results from a raw primary sludge sample.

In collaboration with the Quality Assurance Branch, EMSL-Cincinnati, and the
Toxicology and Microbiology Division, Health Effects Research Laboratory -
Research Triangle Park, descriptions of two agency test methods for
recreational waters, "Test Methods for Escherichia coli and Enterococci in
Water by the Membrane Filter Procedure" were prepared for publication, and
round-robin testing was conducted to determine the precision, bias,
specificity, and upper counting range of the methods.

Two abstracts were prepared and submitted to the American Society for
Microbiology for presentation at the Annual Meeting in Atlanta, Georgia, March
1987. The abstracts describe research on development of a new screening test
to determine the acceptability of 0.45 um MFs for water analyses, and a
comparison of three selective media for isolation and enumeration of
Staphylococcus aureus in swimming pool waters.

In line with EMSL-Cincinnati1s lead role in analytical quality assurance
for the Agency, quality control checks were run on several lots of MFs.
Problems with colony spreading, non-wetting, ink grid toxicity, and other
unacceptable effects were observed. Procedures were initiated to study these
deficiencies with the electron microscope.

A comparison of commercially-available, disposable dilution bottles containing
phosphate buffer (PB) and 0.1 percent peptone buffer with inhouse prepared
dilution blanks containing the same two buffers was conducted in response to a
request for approval through the Equivalency Program. The contents of>both
commercially-available buffers were sterile. Inhouse and commercially
prepared PB dilution blanks recovered Escherichia aerogenes equally well and a
comparison of peptone waters showed similar results. However,
commercially-prepared peptone blanks contained less peptone than specified.

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FY-86 OUTPUT PLAN
VIROLOGY SECTION, BMB, EMSL-CI NCINNATI

WATER QUALITY-MONITORING SYSTEMS AND QUALITY ASSURANCE, B101

Page 5 of 76_
PE#

OUTPUT Reference Biological Methods - Water Quality

ORD Contact

^tineR.S. Safferma
FTS No. 684-7337

Resources:

$(000) 332,6 K PFT 4-° OPFT T-8 PFTE 4-0 OPFTE^-8

Project 03

ANNUAL REPORT FY86

The report, "Optimization of the BGM Cell Line Culture and Viral Assay
Procedure for Monitoring Viruses in the Environment", was published in
the April issue of "Applied and Environmental Microbiology". Presented
in this report are standardized procedures for cultivating the Buffalo
green monkey (BGM) kidney cell line and for its use in assaying
waterborne viruses. Also reported were the superiority of the cell line
for virus isolations when compared to nine other cell types and the
finding that certain media and additives tended to increase BGM cell
sensitivity to a specific group of viruses.

The report, "Recovery of Viruses from Water by a Modified Flocculation
Procedure for Second-Step Concentration", was published in the June issue
of "Applied and Environmental Microbiology." The study was undertaken
because a change in the commercial processing of beef extract had
resulted in a reduction in virus recovery efficiencies. Investigation of
the problem led to the finding that the addition of Celite analytical
filter-aid corrected this deficiency.

The operational capacity of a fluid proportioner currently used in virus
concentration systems was compared with that of a recently developed
in-line injector system. The in-line injector system proved to be much
less cumbersome and much more economical.

The revised Chapter 8 of the "USEPA Manual of Methods for Virology" was
prepared for distribution. This new chapter provides improved
methodology that can be applied to the recovery of viruses from samples
of sewage, effluents and waters found toxic to mammalian cells used for
the assay of enteroviruses, and can also be used to remove deeply colored
samples which, if left on the cell monolayers, would result in inaccurate
plaque counts. Chapter 9 of the manual is now in the process of being
revised. The original chapter has been divided into two chapters, and
the first of these chapters, "Cell Culture Preparation and Maintenance",
was completed and has received Agency clearance.

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Page Z of Project No. 03

Page 6 of 76

Round-robin tests involving nine laboratories were completed with
methodology for detecting viruses in soil, under the jurisdiction of the
Task Group on Viruses in Solids, American Society for Testing and
Materials.

An internal report, "Method for Mammalian Cell Toxicity Test", was
prepared which describes a technique to determine the threshold
cytotoxicity of water and wastewater .

Draft reports on the optimization of the suspended cell technique for
virus enumeration, and for recovery of viruses from sewage sludges, were
prepared and are in internal review and revision.

Virus analyses were performed for the Water Engineering Research
Laboratory - Cincinnati (WERL-Cincinnati) using outputs from a
feed-and-draw sludge operation at the USEPA's Test and Evaluation
Facility in Cincinnati. Samples were also analyzed for WERL-Cincinnati
to determine whether retrofitted anaerobic and aerobic wastewater sludge
digesters would meet the pathogenic bacteria and enteric virus reduction
requirement of USEPA Criteria 40 CFR, Part 257, Appendix 11(A). Results
thus far indicated good reproducibi1ity of data sets and a pronounced
difference in the virus removal efficiency between the conventional and
modified systems.

Technical support was provided to the South Carolina Department of Health
and Environment Control concerning enteric virus monitoring of secondary
sewage effluents at Hilton Head.

Nine water samples collected from the New York Bight by Region 2 were
analyzed for viruses.

A guest worker in the Virology Section was awarded a Master of Science
degree from the University of Cincinnati. Her thesis, entitled "The
Evaluation of Reconcentration Methods in Monitoring for Human Enteric
Viruses in Environmental Samples," was based on research conducted in our
laboratory under the guidance of the Virology Section staff.

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APPROACH
Water Quality - DU B107

Page 7 of j$_
PE# AAPB1A

Complete semi-annual
OUTPUT and report on USEPA,
A.

performance evaluation studies
state and local laboratories.

C. ORD Contact

Name Harold Clements
FTS No. 684-7325

Resources

B.	$(000) 50 PFT 0.8 OPFT 0.2 PFTE	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 04

Inhouse Task: Develop Performance Evaluation (PE) Samples.

Purpose:	Provide a system for evaluating the skills of USEPA, USEPA

contractor, state, and local laboratories analyzing samples as
required under the Clean Water Act.

Approach:	As part of the Mandatory Quality Assurance (QA) Program, PE samples

are designed, developed, produced, and verified by repeated
analyses. These stable, homogeneous sample concentrates with known
true values are then used in formal studies to evaluate 500-900
USEPA, state, and local laboratories, based on on requests from
regional QA coordinators, states, and USEPA project officers.

Accomplishments: New PE ampuls were prepared for total phenolics (3,000 ampuls),

total residual chlorine (6,000 ampuls) and minerals (24,000 ampuls).
Analyses of the above samples verified that the theoretical
concentrations and the analyzed values agree. Final verification
analyses were completed for all samples before distribution in Water
Pollution (WP) Studies 16 and 17. Samples were sent to 546
laboratories in WP Study 16 and 830 laboratories in WP Study 17.

Most of these laboratories participated in the organic and the
inorganic portion of the tests which comprised 73 parameters/
analytes at two separate concentrations.

Status:

Annual Report on Design, Development,
and Distribution of PE Samples

Completed
(12/85)

-------
Page 2 of Project No. 04

~	Page 8 of 76

APPROACH	PE# MFB1A

	 			 Water Quality - DU B107			

Complete semi-annual performance evaluation studies C. ORD Contact
OUTPUT and report on EPA, state and local laboratories.	Name Paul Britton

A	.	FTS No. 684-7325

RpQrturrp^

B.	$(000) 255 PFT 4.1 OPFT 0 PFTE	 OPFTE	

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 04

Task:	Conduct Water Pollution (WP) Laboratory Performance Evaluation

Studies.

Purpose:	To provide an objective measure of the ability of the USEPA, USEPA

contractor, state, and local laboratories that generate water
quality data to demonstrate acceptable performance.

Approach:	Samples are designed, prepared, and distributed in interlaboratory

studies offered twice each year to USEPA, state, USEPA contract
laboratories, and additional laboratories elected by the USEPA
Regions. These studies cover a broad group of ambient monitoring
analytes including: 21 trace metals, 12 minerals, 5 nutrients, 3
demands, 2 polychlorinated biphenyls (PCBs), 8 pesticides, 11
volatile organics, 6 aromatic purgeables, total cyanide, non-
filterable residue, oil and grease, total phenolics, and total
residual chlorine. Analytical results are compared with acceptance
and warning limits based upon the known true concentrations and
results from the current and past studies. Performance in these
studies is used to identify problems so they can be investigated and
resolved.

Accomplishments: During the year, reports were generated for studies WP015 and WP016,
with 525 and 381 participating laboratories, respectively. Study
WP017 was initiated and will be completed next year. There were 73
parameters offered for analyses, most at two separate concentrations
in each study.

Status:	Individual Laboratory Performance Evaluation	Completed

Reports Distributed to Participants in Study	(7/86)

WP015 and Study WP016

-------
Page 3 of Project No. 04

APPROACH
Water Quality - DU B107

Page 9 of 76
PE# TOFB1A

OUTPUT QA Sample Repository
A.

C. ORD Contact
Name Harry Kolde
FTS No. 684-7325

Resources

B. R/D $30K $(000) 39.7 PFT 0.2 OPFT

PFTE

OPFTE

Extramural Task;
Purpose:

Approach:
Accomplishments:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 04

USEPA Repository for Toxic and Hazardous Materials, Produce and
Distribute Calibration Standards and Surrogates.

The USEPA Repository for Toxic and Hazardous Materials provides
spiking/calibration solutions of organic compounds in support of
regulations under the Clean Water Act and Consent Decree for
Priority Pollutants.

Compounds of interest to the 304(h) and priority pollutant
regulations are purchased or synthesized, then purified, dissolved
in the appropriate solvent and dispensed in 5 mL ampuls. The verity
of pure compounds and concentrations of the compounds in the ampuls
are verified by referee laboratories. Upon verification, spiking/
calibration solutions are distributed to USEPA, USEPA contractor,
state, and local laboratories monitoring the environment.

1.	Spiking/calibration solutions for 110 of 111 organic priority
pollutants under the Consent Decree are available for use by
USEPA, USEPA contractor, regional, state, and local
laboratories. The remaining one is now being analyzed by
referee laboratories.

2.	In FY86 75,200 spiking/calibration solutions were distributed to
1553 USEPA, regional, state, and local laboratories engaged in
environmental monitoring. Compounds available for distribution
are listed in USEPA Quality Assurance Newsletter.

3.	Of the 16 gas chromatograph/mass spectrometer (GC/MS) surrogates
specified in USEPA Methods 624 and 625, all are now available
for use as calibration standards.

4.	Native and 13c-iabeled 2,3,7,8-tetrachlorodibenzo-p-dioxin
(TCDD) are available as calibration standards.

Status:

Annual Report on the Repository

Completed
(12/85)

-------
Page 4 of Project No. 4



APPROACH
Water Quality - DU B107

Page 10 of 76
PE# TOFB1A

OUTPUT QC Sample Program
A.



C. ORD Contact

Name Ray Wesselman
FTS No. 684-7325

Resources

B. R/D $20K $(000) 29.7 PFT 0.2 OPFT	 PFTE 	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 04

Extramural Task: Develop, Analyze, and Distribute Quality Control (QC) Samples for
Water-related Analytes.

QC samples are provided to USEPA, USEPA contractors, regional,
state, and local laboratories as a check on the technique and
analytical methodology. Such checks are necessary to measure
quality of data being generated in carrying out mandates of the
Clean Water Act and Consent Decree for Priority Pollutants.

Bionetics, Inc., the technical service contractor, develops,
produces, and distributes QC samples. Development of new sample
types requires chemicals of the highest purity which are obtained
from best sources including the USEPA Repository for Toxic and
Hazardous Materials. The methodology for the compounds of interest
are selected, retention time studies are conducted, and finally
combining groups of organic compounds to minimize overlapping gas
chromatography (GC) peaks. Zero, 45-, and 90-day stability studies
are conducted. Those compounds proven stable are produced at one
concentration level in lots of 5,000. Random samples are withdrawn
during production and sent to referee laboratories for verification
analyses. Upon verification, the new sample series is listed in the
USEPA Quality Assurance (QA) Newsletter and distributed to
requesters.

Accomplishments: A total of 285,167 water pollution QC samples were distributed for
all programs containing such analytes as trace metals for atomic
absorption (AA) and inductively-coupled plasma (ICP) analyses,
demands, nutrients, suspended solids, minerals, 109 priority
pollutants for USEPA 600 series methodology, GC/mass spectrometer
(MS) base neutrals, acids and purgeables, natural matrix samples
such as polychlorinated biphenyls (PCBs) in oil and fish, metals and
pesticides in fish, phenols, cyanide, and crude oils. Samples
listed in the USEPA QA Newsletter are distributed to USEPA, USEPA
contractor, state, and local laboratories.

A total of 181,000 ampuls were produced to replenish depleted
inventories and included such QC series as trace metals, cyanide,
PCBs in oil and acetone, pesticides, demand, nutrients, and seven
volatile organic series.

Purpose:

Approach:

-------
Page 5 of Project No. 04

APPROACH
Mater Quality - DU B107

Page n ot~7?
PE# TOPB1A

Extramural Task:

Accomplishments:
(continued)

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 04

Develop, Analyze and Distribute Quality Control (QC) Samples for
Water-related Analytes (continued).

Chlorophyll (Spectrophotometry and Fluorometric), ATP, Reference
Toxicants (cadmium chloride, sodium lauryl sulfate, and sodium
pentachlorophenate), simulated plankton and natural plankton for
counting, Algae for Identification (two samples), and five bacterial
indicator cultures have been developed and 5,091 ampuls were
distributed. A new reference toxicant, sodium pentachlorophenate,
was produced. Several pure cultures and natural collections of
algae for use in identification samples were obtained. A
chlorophyll extract was prepared from natural periphyton to provide
a source of chlorophyll £ in future samples. A new algae for sample
identification was prepared. A new procedure involving high
performance liquid chromatography (HPLC) analysis of algal pigments
is being investigated, which provides information on several
chlorophyll degradation products and other accessory pigments. A
calibration sample for this HPLC analysis is also under development.

Status:

Annual Report on QC Sample Program

Completed
(12/85)

-------
Page 6 of Project No. 04

APPROACH
Water Quality - DU B107

Page 12 of /b
PE# OTB1A

OUTPUT Referee Analytical Services
A.

C. ORD Contact
Name Harry Kolde
FTS No. 684-7325

Resources

B. R/D $5K $(000) 14.7 PFT 0.2 OPFT

PFTE OPFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 04

Extramural Task: Referee Laboratory Services.

Purpose:	Usage of large numbers and types of quality control (QC),

performance evaluation (PE) and spiking/calibration samples in all
USEPA programs to assess the quality of monitoring data necessitates
that true or reference values associated with the samples are in
fact, valid. Otherwise poor decisions will result which could
adversely impact the environment. Therefore, referee laboratories
are used to establish the veracity of all samples.

Approach:	Referee laboratories are selected through the competitive procurement

process upon the basis of PE and cost for the analytes of interest.
These analytes include trace metals, nutrients, minerals, sodium and
corrosivity, demand, priority pollutants in samples designed for gas
chromatograph (GC) and GC/mass spectrometer (MS), polychlorinated
biphenyls (PCBs) in oil, and synthetic organic contaminants
specified in the Clean Water Act and in the Consent Decree.

Accomplishments: Referee laboratories conducted a total of 2,318 analyses: (1) 90
neat organic analyses to establish purity of materials in USEPA's
Repository for Toxic and Hazardous Materials, (2) 1,876 analyses on
QC and PE samples produced inhouse and on contract, (3) 320 analyses
on spiking/calibration solutions from USEPA's Repository for Toxic
and Hazardous Materials, (4) No analyses on neat surrogates related
to USEPA Methods 624 and 625, and (5) analyses on 32 neat surrogate
solutions.

Status:

Annual Report on Referee Analytical Services

Completed
(12/85)

-------
Page 7 of Project No. 04

APPROACH

Page 13 of 76
PE# MPB1A

Water Quality - DU B107





C. ORD Contact

OUTPUT Continue NBS Traceability

Name John Winter

A.

FTS No. 684-7325

Resources



B. R/D $20K $(000) 29.7 PFT 0.2 OPFT

PFTE OPFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 04

Extramural Task: Establish Traceability of Quality Control (QC) and Performance
Evaluation (PE) Samples to National Bureau of Standards (NBS).

Purpose:	The QC and PE samples utilized throughout the United States and

internationally in water/wastewater-related monitoring programs must
be of high quality since they are involved in many important
decisions. As such, there is a stringent quality assurance program
to assure the veracity of the QC and PE samples including
traceability to the NBS.

Approach:	An interagency agreement (IAG) was signed with the NBS to develop a

protocol for traceability of QC and PE samples, and then to implement
the protocol for those analytes/samples of interest to the Agency
for which NBS has expert analytical capabilities.

Accomplishments: NBS verified, thereby establishing traceability for pesticides

(lindane, endrine and methoxychlor) for Water Supply (WS) Studies 19
and 20, two herbicides (2,4-D and Silvex), and 14 volatile organic
contaminants (VOCs) (trans and cis 1,2-dichloroethylene, dibromo-
chloropropane, o-dichlorobenzene, ethylbenzene, chlorobenzene,
sytrene, toluene, xylene, ethylene dibromide, chloroform, bromodi-
chloromethane, dibromochioromethane and bromoform). Seven sludges
which are to be used in an interlaboratory method validation study
are currently being analyzed.

Status:

Annual Report on Traceability to NBS

Completed
(12/85)

-------
Page 8 of Project No. 04



Page 14 of 76

APPROACH

PE# AAPB1A

Water Quality - DU B107





C. ORD Contact

OUTPUT Externalization of QA Programs.

Name John Winter

A.

FTS No. 684-7325

ftesources

B. R/D $ OK $(000) 9.7 PFT 0.2 OPFT	 PFTE 	 OPFTE

Inhouse Task:

Purpose:

Approach:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 04

Externalization of Quality Assurance (QA) Programs.

Recover costs of production, distribution, and administration of
quality control (QC) and performance evaluation (PE) sample programs
associated with the drinking water, industrial waste, and water
quality program.

Promulgate a cost recovery rule for the preparation and distribution
of QC and PE samples, set up a mechanism for collecting such fees
through the USEPA Financial Management Office, and begin the
externalization process for these sample types.

Accomplishments: An externalization task force was formed of USEPA personnel from the

Comptroller's Office; Office of General Counsel; Office of Program
Management; Office of Acid Deposition, Environmental Monitoring and
Quality Assurance (OADEMQA); operating program offices; the regional
offices; and the three EMSL laboratories to study and recommend the
best option for externalization of QA support services. Concur-
rently, EMSL-Cincinnati prepared a white paper on costs for
consideration by the Task Group. Discussions were also held between
the Contracts Management Division and EMSL-Cincinnati to explore the
best means to charge and collect user fees for these services and to
expedite return of funds to EMSL-Cincinnati for maintenance of the
QA program.

Based on these deliberations and discussions, OADEMQA prepared a
draft of a proposed rule: Proposed User Charges for Certain Quality
Control and Performance Evaluation Samples Under the Clean Water Act
and the Safe Drinking Water Act which was subsequently published in
the Federal Register on September 16, 1986. Comments are due by
October 31, 1986.

Status:	Report on the Externalization QA Program	Completed

(5/86)

-------
Water Quality Research Committee

Paqe 15 of 76
PE No. APTjTTT

A.	OUTPUT: Monitoring Measurements and Quality Assurance C. ORD Contact

Reference Chemical Methods - Water and Name: J. J. Lichtenberq
	Sediment Analysis	FTS No. 684-7306

B.	RESOURCES: 3384.0 k	FTE 7.0

FY 86 ANNUAL REPORT	Project No. 05

Purpose and Approach

The purpose of this project is to evaluate and standardize sample collection
and chemical measurement methods for pollutants in water and sediments.
In-house and under contract, single laboratory accuracy and precison data and
method detection limits will be obtained for organic and metal analytes in
environmentally contaminated water, sludge, sediment, and dredge material
matrices using standardized extraction, cleanup and determination procedures
and, when required, development of new techniques and procedures.

Progress and Accomplishments

Work on the project for "Identification and Determination of Metal Ions and
Their Organometallic and Metal Chelate Compounds by High Performance Liquid
Chromatography (HPLC)" continued throughout the year. A report, "Speciation
of Inorganic and Organometallic Mercury by High-Performance Liquid
Chromatography with Reductive Amperometric Electrochemical Detection", has
been submitted for journal publication. It was submitted to the program
office in May 1986. Investigations will continue in this area in FY 87 with
the application of HPLC to 2-mercaptoethanol complexes of three organomercury
compounds, i.e., methyl-, ethyl-, and phenylmercury.

A special project to develop a method for acid soluble metals was completed
this year. An overview of the technical findings resulting from the
"Evaluation of Method 200.1 Determination of Acid Soluble Metals" was
presented at the Society for Applied Spectroscopy (SAS) Seminar on Atomic
Spectroscopy, April, 1986. An abridged version of a report on this topic was
submitted to the U. S. Environmental Protection Agency (USEPA) Industrial
Technology Division for incorporation into the proceedings of the Ninth Annual
(1986) Analytical Symposium.

The project to evaluate procedures for digestion and extraction of inorganic
pollutants from biological fish tissue was begun in the second quarter.
Initially, two techniques for extraction and solubilization of the tissue,
microwave digestion and chemical treatment with tetramethylammonium hydroxide,
are being investigated. A report on this project is planned for mid-FY 87.

-------
Page of Project No. 05	Page 16	 of 76

Work to develop methods for nonvolatile hazardous substances using a liquid
chromatography/mass spectrometry (LC/MS) interface was begun early in FY 86.
The unit connects the effluent from a HPLC to a Finnigan Model 4500 quadrupole
mass spectrometer. Emphasis is on methods for carbamate, amide, urea, and
triazine pesticides that are not amenable to gas chromatography/mass
spectrometry (GC/MS) and for which no generic methods exist. This project is
in the quantitative analysis stage including preliminary assessments of
precision, accuracy, and detection limits.

The project to develop design criteria for mechanical construction of a fiber
optic chemical analyzer is continuing at Battelle Columbus. Analysis of the
fiber optics technique determined that interferometry measurements of the
sensitized fiber and the use of an elliptical fiber optics core provides the
greatest sensitivity. However, since the system is extremely sensitive to
temperature, compensatory techniques are being explored. In-house studies
including electron microscope photographs of the fiber optics coated with
3-cyanopropyl silane showed excellent bondage and large surface area which
should result in more sensitivity to polar compounds.

-------
Industrial Wastewater Research Committee

Page 17 of 76
PE No. BETO

A. OUTPUT: New and Improved Analytical Test Procedures	C. ORD Contact

for Pollutants in Industrial Wastewater Name: J. J. Lichtenberg

FTS No. 684-7306

B. RESOURCES: $638.6K	FTE 10.1

FY 86 ANNUAL REPORT	Project No. 06

Purpose and Approach

The purpose of this project involves development of improved priority
pollutant 600 series methods to correct deficiencies identified by users of
the methods and to improve state-of-the-art flow measurement techniques.
Liaison will be maintained with users of the methods to identify problem
areas. A log of deficiencies will be maintained. These will be prioritized
in order of seriousness and appropriate research will be initiated to correct
the deficiencies. The methods will then be revised as appropriate.

Progress and Accomplishments

A continuing project to correct inadequacies of 304(h) methods for application
to specific matrices is maintained. Inadequacies are being reviewed and
appropriate action to modify methods is being taken. The Annual Report on
these deficiencies is being prepared. Specific areas being addressed are as
follow:

Pesticide Methods - The proposed regulation to add new methods to Part 136 and
move currently approved methods from Part 455 fell apart when the Agency
decided to remand the Part 455 regulation. All methods approved there will
now need to be reproposed in Part 136. A significant restructuring of the
package is now required.

Priority Pollutant Methods - The final rule of the October 26, 1984 interim
rule was redrafted and forwarded again to Office of General Counsel (OGC) and
the Work Group for comment, along with the final rule on the housekeeping
proposal of that date, and the notice of data availability on June 30, 1986.

Other Chemical Methods - The Virginia Edison Power Company (VEPCO) Settlement
Agreement and nationwide alternate test procedure (ATP) for inductively
coupled plasma (ICP) were approved by the Work Group at the annual meeting.
All chemical methods previously proposed for Part 136 by the Industrial
Technical Division (ITD) were withdrawn at the meeting.

The Sampling and Field Measurements Section continues to provide technical
assistance to the Underground Injection and Control (UIC) Program. A report
on "Flow Measurements for the UIC Program - A Review" has been drafted and is
undergoing technical and administrative review.

-------
Page _2_ of Project No. 06	Page 18 of 76

The project to develop a Kriging program for sampling sediments using IBM-PC
has been completed. A paper, "A Universal Kriging Program for the IBM-PC for
use in Monitoring Sediments in Lakes", has been submitted for publication in
the proceedings of the "Symposium on Chemical and Biological Characterization
of Municipal Sludges, Sediments, Dredge Spoils and Drilling Muds", which was
held in Cincinnati, Ohio, May, 1986.

In the area of technical and engineering support in the use of computers, a
draft report titled "Functional Requirements for the Single Laboratory Method
Validation System on the IBM-PC" was delivered early in FY 86. The program is
available in disk form and has been in great demand. More than 170 requests
have been filled to date.

Work on the organic accumulator project was halted during the 3rd quarter so
that the principal investigator could devote full time to the evaluation of a
wide-bore capillary column gas chromatography (GC) system employing the
photoionization detector (PID) and electrolytic conductivity detector (ECD) in
series for drinking water analyses.

A new method (Method 680), that resulted from work performed during FY 85, was
delivered to the program office early in FY 86. This method determines
polychlorinated biphenyls (PCBs) and pesticides by degree of chlorination.

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APPROACH
Industrial Waste - DU B116

Page 19 of 76
PE# BEflC

Verify and distribute quality control/performance
OUTPUT evaluation samples and repository standards.

A.

C. ORD Contact

Name Harold Clements
FTS No. 684-7325

Resources

B.	$(000) 71.8 PFT 0.5 OPFT 1.0 PFTE 	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 07

Inhouse Task: Develop Performance Evaluation (PE) Samples.

Purpose:	Provide a means for evaluating USEPA, USEPA contractor, state, and

local laboratories analyzing samples as required under the Clean
Water Act.

Approach:	As part of the Agency's quality assurance (QA) program, PE samples

are designed, developed, produced, and verified by repeated
analyses. Stable, homogeneous samples with known true values are
prepared as concentrates and used to evaluate 700-900 USEPA, state,
and local laboratories in formal semi-annual studies. Samples are
also distributed on request from USEPA project officers to USEPA
contractors.

Accomplishments: PE samples were prepared for total phenolics (3,000 ampuls), total

residual chlorine (6,000 ampuls), and mineral series (24,000 ampuls).
Initial analyses of the samples verified the theoretical concen-
trations. Final verification analyses were completed for all
samples before distribution in Water Pollution (WP) Studies 16 and
17. Samples were sent to 546 laboratories in WP Study 16 and 830
laboratories in WP Study 17. Most of these laboratories partici-
pated in both the organic and the inorganic portion of the studies.
In total 73 analytes were each tested at two separate concentrations.

Status:

Annual Report on Design, Development,
and Distribution of PE Samples

Completed
(12/85)

-------
Page 2 of Project No. 07



Paqe 20 of 76

APPROACH

PE# BEB1C

Industrial Waste - DU B116



Verify and distribute quality control/performance

C. 0RD Contact

OUTPUT evaluation samples and repository standards.

Name Paul Britton

A.

FTS No. 684-732$

Resources

B.	$(000) 59.1 PFT 0.2 OPFT 0.5 PFTE	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 07

Conduct Performance Evaluation (PE) Studies.

Provide a system for evaluating the skills of USEPA, USEPA
contractor, state, and local laboratories analyzing samples as
required under the Clean Water Act.

As part of the Agency's Mandatory Quality Assurance Program, PE
samples are designed, developed, produced, and verified by repeated
analyses. Stable, homogeneous sample concentrates with known true
values are prepared and used in formal PE studies to evaluate
700-900 USEPA, state, and local laboratories in semi-annual
studies. Samples are also distributed on request from USEPA project
officers to USEPA contractors.

Accomplishments: Two PE studies were conducted for USEPA, USEPA contractor, state,

and local laboratories as nominated by the Regions and states. The
73 analytes tested at two concentrations included 21 trace metals,
12 minerals, 5 nutrients, 3 demand, 2 polychlorinated biphenyls
(PCBs), 8 pesticides, 11 volatile organics, 6 aromatic purgeables,
total cyanide, non-filterable residue, oil and grease, total
phenolics, and total residual chlorine as analytes. Results were
compared with acceptance limits based on previous study data and
reports prepared for each laboratory. Performance in the studies
identified problems for investigation and resolution.

Samples were sent to 500-700 laboratories in each of the semi-annual
studies conducted during February and August 1986. New samples were
prepared for future studies in FY87 and beyond. In WP015, samples
were sent to 726 laboratories of which 555 responded with data.
Results were evaluated and reports sent on December 7, 1985. In
WP016, samples were sent to 552 laboratories of which 437 returned
data for evaluation. Results were evaluated and reports sent to
participants on June 6, 1985.

Inhouse Task:
Purpose:

Approach:

Status:

Individual Laboratory PE Reports Distributed to
Participants in Study WP015 and WP016

Completed
(7/86)

-------
Page 3 of Project No. 07



APPROACH
Industrial Waste - DU B116

Page 21 of 76
PE# BEB1C

OUTPUT QA Sample Repository
A.



C. ORD Contact
Name Harry Kolde
FTS No. 684-7325

Resources

B. R/D $19.25K $(000) 32.5 PFT 0.2 OPFT	 PFTE	 OPFTE

FY86 ANNUAL REPORT
Qua!ity Assurance Branch, EMSL-Cincinnati

Project No.: 07

Extramural Task: Referee Laboratory Services.

Purpose:	The large numbers and types of quality control (QC), performance

evaluation (PE) and spiking/calibration samples used in all USEPA
programs to assess the quality of monitoring data necessitates that
true or reference values associated with the samples are in fact,
valid. Otherwise poor decisions will result which could adversely
impact the environment. Therefore, referee laboratories are used to
establish the veracity of all samples.

Approach:	Referee laboratories are selected through the competitive

procurement process based on the PE and cost for the analytes of
interest. These include trace metals, nutrients, minerals, sodium
and corrosivity, demand, polychlorinated biphenyls (PCBs) in oil,
fish and sediment, and all synthetic organic contaminants specified
in the Clean Water Act and in the Consent Decree.

Accomplishments: Referee laboratories conducted a total of 3,299 analyses: (1) 126
neat organic analyses to establish purity of materials in USEPA's
Repository for Toxic and Hazardous Materials, (2) 2,669 analyses on
QC and PE samples produced inhouse and on contract, (3) 472 analyses
on spiking/calibration solutions from USEPA's Repository for Toxic
and Hazardous Materials, (4) no analyses on neat surrogates related
to USEPA Methods 624 and 625, and (5) analyses on 32 neat surrogate
solutions.

Status:

Report on Referee Analytical Services

Completed
(12/85)

-------
Page 4 of Project No. 07

APPROACH
Industrial Waste - DU B116

Page n of 76
PE# IEE1C

OUTPUT QA Sample Repository
A.

C. 0RD Contact
Name Harry Kolde
FTS No. 684-7325

Resources

B. R/D $4K $(000) 13.6 PFT 0.2 OPFT	 PFTE	 OPFTE

Extramural Task:

Purpose:

Approach:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 07

USEPA Repository for Toxic and Hazardous Materials, Produce, and
Distribute Calibration Standards and Surrogates.

The USEPA Repository for Toxic and Hazardous Materials provides
spiking/calibration solutions of organic compounds in support of
regulations under the Clean Water Act and Consent Decree for
Priority Pollutants.

Compounds of interest to the 304(h) and priority pollutant
regulations are purchased or synthesized, then purified, dissolved
in the appropriate solvent, and dispensed in 2 mL ampuls. The
verity of pure compounds and concentration of the solutions in
ampuls are verified by referee laboratories. Upon verification,
spiking/cali- bration solutions are distributed to USEPA, USEPA
contractor, state, and local laboratories engaged in monitoring the
environment.

Accomplishments: 1,

Spiking/calibration solutions for all 110 organic priority
pollutants under the Consent Decree are available for use by
USEPA, USEPA contractor, regional, state, and local labora-
tories. The remaining one is now being tested by referee
laboratories for verity.

2.	In FY86, 76,200 spiking/calibration solutions were distributed
to 1925 USEPA, regional, state, and local laboratories engaged
in environmental monitoring. Compounds available for distri-
bution listed in USEPA Quality Assurance Newsletter were
requested from the Quality Assurance Branch.

3.	Of the 16 gas chromatograph/mass spectrometer (GC/MS) Surrogates
specified in USEPA Methods 624 and 625, all are now available
for use as calibration standards.

4.	Native and l3C-labeled 2,3,7,8-tetrachlorodibenzo-p-dioxin
(TCDD) are available as calibration standards.

Status:

Annual Report on Repository

Completed
(12/85)

-------
Page 5 of Project No. 07



Page 23 of 7fi

APPROACH

PE# BEB1C

Industrial Waste - DU B116





C. ORD Contact

OUTPUT Continue NBS Traceability

Name John Winter

A.

FTS No. 684-7325

Resources



B. R/D $19.25 $(000) 32.5 PFT 0.2 OPFT

PFTE OPFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 07

Extramural Task: Establish Traceability of Quality Control (QC) and Performance
Evaluation (PE) Samples to National Bureau of Standards (NBS).

Purpose:	The QC and PE samples utilized throughout the United States and

internationally in water/wastewater related monitoring programs must
be of the highest quality since they are involved in many important
decisions by USEPA and the state agencies. As such, a stringent
quality assurance program is needed to assure the veracity of the QC
and PE samples; this program includes traceability to NBS.

Approach:	An interagency agreement (IAG) is maintained with the NBS to develop

a protocol for traceability of QC and PE samples, and then to
implement the protocol for those analytes and samples of interest to
the Agency for which NBS has expert analytical capabilities.

Accomplishments: NBS verified, thereby establishing traceability for trace pesticides

(lindane, endrine and methoxychlor for Water Supply (WS) Studies 19
and 20, two herbicides (2,4-D and Silvex), and 14 volatile organic
contaminants (VOCs) (trans and cis 1,2-dichloroethylene, dibromo-
chloropropane, o-dichlorobenzene, ethylbenzene, chlorobenzene,
sytrene, toluene, xylene, ethylene dibromide, chloroform, bromodi-
chloromethane, dibromochloromethane and bromoform). Seven sludges
which are to be used in an interlaboratory method validation study
are currently being analyzed.

Status:

Annual Report on Traceability to NBS

Completed
(12/85)

-------
Page 6 of Project No. 07





Paqe 24 of 76



APPROACH

PE# BEB1C



Industrial Waste - DU B116







C. ORD Contact

OUTPUT QA Sample Repository



Name Ed Berq

A.



FTS No. 684-7325

Resources





B. R/D $19.25 $(000) 32.5

PFT 0.2 OPFT

PFTE OPFTE



Extramural Task:

Purpose:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 07

Develop, Analyze, and Distribute Quality Control (QC) Samples £or
Water-related Analytes.

QC Samples are provided to USEPA, USEPA contractor, regional, state
and local laboratories as a check on the technique and analytical
methodology. Such checks are necessary to monitor the quality of
data being generated in carrying out mandates of the Clean Water Act
and Consent Decree for Priority Pollutants.

Bionetics, Inc., the technical service contractor, develops,
produces, and distributes QC samples. Development of new sample
types requires: obtaining chemicals of the highest purity, a
portion from the USEPA Repository for Toxic and Hazardous Materials,
selecting the methodology for the compounds of interest, conducting
retention time studies, combining groups of organic compounds to
minimize overlapping gas chromatography peaks, and conducting 0,
45-, and 90-day stability studies. Those compounds remaining stable
are produced at two concentration levels in lots of 3,000. Random
samples are withdrawn during production and sent to referee labora-
tories for verification analyses. Upon verification, the new
samples are advertised in the USEPA Quality Assurance (QA)

Newsletter and distributed to requesters.

Approach:

Accomplishments: 1,

4.

Distribution of a total of 285,167 water pollution QC samples
containing such analytes as trace metals for atomic absorption
(AA) and inductively-coupled plasma (ICP) analyses, demands,
nutrients, suspended solids, minerals, 109 priority pollutants
for USEPA 600 series methodology, gas chromatograph/mass
spectrometer (GC/MS) base neutrals, acids and purgeables,
natural matrix samples such as polychlorinated biphenyls (PCBs)
in oil and sediment, metals and pesticides in fish, phenols,
cyanide, and crude oils. Sample types were advertised in the
USEPA QA Newsletter and distributed on request to USEPA, USEPA
contract, regional, state, and local laboratories.

A total of 181,000 ampuls were produced to replenish depleted
inventories and included such QC series as trace metals,
cyanide, PCBs in oil and acetone, pesticides, demand, nutrients,
and seven volatile organic series.

Of the list of 188 industrial waste analytes, 136 are available
as QC samples.

Twenty-three QC series were verified as to true values,
homogeneity, and stability by referee laboratories.

Status:

Report on QC Sample Program

Completed
(12/85)

-------


Page 25 of 76

APPROACH

PE# BEB1C

Industrial Waste - DU B116





C. ORD Contact

OUTPUT Externalization of QA Programs.

Name John Winter

A.

FTS No. 664-7326

Resources

B. R/D $ OK $(OOQ) 0 PFT 0 OPFT	 PFTE 	 OPFTE

Inhouse Task:
Purpose:

Approach:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 08

Externalization of Quality Assurance (QA) Programs.

Recover costs of production, distribution, and administration of
quality control (QC) and performance evaluation (PE) sample programs
associated with the drinking water, industrial waste, and water
quality program.

Prepare a white paper on externalization of QA, promulgate a cost
recovery rule for the preparation and distribution of QC and PE
samples, set up a mechanism for collecting such fees through the
USEPA Financial Management Office, and begin the externalization
process for these sample types.

Accomplishments: An externalization task force was formed of USEPA personnel from the
Comptroller's Office; Office of General Counsel; Office of Program
Management; Office of Acid Deposition, Environmental Monitoring and
Quality Assurance (OADEMQA); operating program offices; the regional
offices; and the three EMSL laboratories to study and recommend the
best option for externalization of QA support services. Concur-
rently, EMSL-Cincinnati prepared a white paper on costs, for
consideration by the Task Group. Discussions were also held between
the Contracts Management Division and EMSL-Cincinnati to explore the
best means to charge and collect user fees for these services and to
expedite return of funds to EMSL-Cincinnati for maintenance of the
QA program.

Based on these deliberations and discussions, OADEMQA prepared a
draft of a proposed rule: Proposed User Charges for Certain Quality
Control and Performance Evaluation Samples Under the Clean Water Act
and the Safe Drinking Water Act which was subsequently published in
the Federal Register on September 16, 1986. Comments are due by
October 31, 1986.

Status:

Report on the Externalization QA Program

Completed
(5/86)

-------
Page 2 of Project No. 08

APPROACH
Industrial Waste - DU B116

Page 26 of 76
PE# BB1C

Evaluate the performance of major NPDES discharger

C. ORD Contact

OUTPUT laboratories.

Name Paul Britton

A.

FTS No. 684-7325

Resources

B.	$(000) 338.1 PFT 1.1 OPFT 0.4 PFTE 	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 08

Extramural Task: Conduct Performance Evaluation (PE) Studies on Laboratories

Producing Data Required under Major National Pollutant Discharge

Elimination System (NPDES) Permits (Discharge Monitoring Report -
Quality Assurance (DMR-QA) Studies).

To provide an objective measure of how well laboratories can
perform, which produce DMR data for major dischargers.

With contract support, design and develop samples and conduct annual
PE studies for the most frequently-occurring analytes in NPDES
permits. Conduct a formal evaluation study on more than 7000 major
dischargers for up to 29 analytes each. Use computerized data
treatment to produce individual reports on each permittee and
summary reports. Use contract computer specialists to maintain,
improve, and expand the computer programs as necessary to support
the NPDES Laboratory PE Studies. Effort made to maintain files of
PE statistics and to use them to develop the best possible
relationships between the true concentrations and statistical
characteristics of analytical data. Statistical reports and
services provided as needed.

Accomplishments: Samples were made, verified, and shipped to 7383 major NPDES
dischargers for DMR-QA Study 6. Data were returned by 6496
permittees for an 88% response, and individual PE reports were
distributed by the end of August. The percentage of unacceptable
data was lower than in any previous DMR-QA Study, continuing a trend
of improvement with each successive study.

Samples for three new analytes were added for DMR-QA Study 6 at the
request of the Office of Water Enforcement and Permits: total
cyanide, total phenolics, and total residual chlorine.

Status:	Development and Distribution of Necessary Study

Materials to Regions, States, and Discharger
Laboratories

Final Report to each Participating Laboratory -
Annual DMR-QA Study

Purpose:
Approach:

Completed
(5/86)

Completed
(11/86)

-------
APPROACH

Page 27 of 76

7T1 OUTPUT: Evaluation and Recommendation of Actions on ORD Contact

NPDES Alternate Test Procedures	NAME: Terence M. Grady

FTS No. 684-7301

Resources:	"

B.	$(000) 165.1 PFT 1.0 OPFT 0.7 PFTE	OPFTE

ANNUAL REPORT	PROJECT NUMBER 09

Purpose and Approach

The Equivalency Program is intended to encourage analytical methods development
or improvement by the regulated community and by manufacturers of pollution
measuring instruments. These alternate test procedures (ATPs) may be approved
for case-by-case or nationwide use as mandated by 40 CFR Parts 136.4 and 136.5.
After receipt of unsolicited ATP applications, necessary external and/or internal
technical reviews are conducted and coordinated to provide a technically sound
recommendation on approval or denial of the proposed ATP. Items considered
during review include: availability of a well documented test procedure, docu-
mentation of the applicability of the proposed procedure, performance character-
istics such as accuracy, precision, and method detection limits, and equivalency
data to an approved test procedure.

Progress and Accomplishments

During FY86, a total of 51 requests for approval of ATPs were received. Ten of
the requests were for nationwide approval and the remaining 41 were for limited
use. Quarterly and annual ATP reports were distributed to the Regional and
Headquarters staff. The direct current plasma atomic emission spectroscopy
method for metals was recommended for nationwide compliance monitoring use.

The following table summarizes the applications received by this office and the
actions recommended:

National Pollutant Discharge Elimination System (NPDES): 51

a.	Nationwide:	10

b.	Limited Use:	41

c.	Action Taken:

1.	Recommended Approval:	19

2.	Recommended Disapproval:	6

3.	Non-Germane (Not ATP):	4

4.	Requested Further Data:	19

5.	Pending:	3

-------


Page 28 of 76

APPROACH

PE# BLC1A

Drinking Water - DU C104



Produce and distribute performance evaluation (PE)

C. ORD Contact

OUTPUT samples for water supply laboratory certification

Name Harold Clements

A. program.

FTS No. 684-7325

B.	$(000) 237.4 PFT 3.7 OPFT	 PFTE	 OPFTE

Approach:

Accomplishments:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 10

Performance Evaluation (PE) Studies for Certification.

Under the Safe Drinking Water Act (SDWA) and the National Interim
Primary Drinking Water Regulations (NIPDWR) and amendments,
acceptable performance in PE studies is an annual requirement for
certification of drinking water laboratories. In response to this
need, the Quality Assurance (QA) Branch develops and provides sample
series for each maximum contaminant level (MCL) analyte, and for
monitoring analytes, listed in the primary drinking water
regulations and amendments.

New series samples are designed, prepared and verified by analyses,
for each semi-annual study of approximately 1000 laboratories. Each
study covers 22 analytes at two separate concentrations each.

Over the past year the following ampuls were produced for future
studies: nitrate/fluoride (12,000 ampuls), sodium/corrosivity
(5,000 ampuls), volatile organics (6,000 ampuls), residual free
chlorine (3,000), and trace metals (12,000).

The ampuls were analyzed originally to verify the true concen-
tration and then by the QA Branch and the referee laboratories to
confirm homogeneity and stability over time.

In Water Supply (WS) Study 18, 1113 laboratories were sent samples
for testing 38 parameters/analytes, most at two concentrations. In
WS Study 19, 911 laboratories were sent samples for certification.
In the past year, 31 of the new volatile organic chemicals (VOCs),
and 1445 compounds have been included in the studies.

Status:

Design, Develop^and Prepare Performance Evaluation
Samples for Drinking Water Certification Program

Completed
(12/85)

-------
Page 2 of Project No. 10

APPROACH
Drinking Water - DU CI04

Page 29 of j£_
PE# BTC1A

OUTPUT Quality Control/Performance Evaluation
A.

C. ORD Contact
Name Harry Kolde
FTS No. 684-7325

Resources

B. R/D 80.4 $(000) 86.4 PFT 0.1 OPFT

PFTE OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 10

Extramural Task: Develop USEPA's Repository for Toxic and Hazardous Materials.

Purpose:

Approach:

The USEPA Repository for Toxic and Hazardous Materials provides
spiking/calibration solutions of organic compounds in support of
regulations under the Safe Drinking Water Act and those contaminants
specified in the Drinking Water Strategy Document.

Compounds of interest to the Drinking Water Program are purchased or
synthesized, purified, dissolved in an appropriate solvent, and
dispensed in 2 mL ampuls. The verity of pure compounds and
concentration of the compound in the ampul are verified by referee
laboratories. Upon verification, spiking/calibration solutions are
advertised in the Quality Assurance Newsletter and distributed to
USEPA, USEPA contractor, state, and local laboratories engaged in
monitoring the environment.

Accomplishments: 1,

Distributed 75,200 spiking/calibration solutions to 1930 USEPA,
state, and local environmental laboratories engaged in
monitoring. Compounds available for distribution listed in
USEPA Quality Assurance Newsletter are requested from the
Quality Assurance Branch, EMSL-Cincinnati.

All organic analytes specified in National Interim Primary
Drinking Water (NIPDW) regulations are available as certified
calibration standards.

Of the 126 organic analytes specified in the various Drinking
Water regulations and Strategy Documents, 90 are certified for
distribution as calibration standards.

All of the volatiles and herbicides listed in the November 1985
Drinking Water regulations are now stocked as neats.

Status:

Annual Report on Repository

Completed
(12/85)

-------
Page 3 of Project No. 10

Page 30 of 76
APPROACH	PE# "BCClA

			Drinking Water - DU CI04			

Produce and distribute quality control (QC) and	C. ORD Contact

OUTPUT performance evaluation (PE) samples for water supply	Name Ed Berg

A	.	laboratory certification program.	FTS No. 684-7325

Resources

B.	R/D $45 $(000) 51 PFT 0.1 OPFT	 PFTE	 OPFTE	

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 10

Extramural Task: Develop and Distribute Quality Control (QC) Samples.

Purpose:

Approach:

Status:

QC Samples are provided to USEPA, regional, state, and USEPA
contractors as a check on analyst technique and analytical
methodology. Such checks are necessary to insure that high quality
data are being generated in carrying out mandates of the Safe
Drinking Water Act.

Bionetics, Inc., the technical service contractor, develops,
produces, and distributes QC samples. Development of new sample
types requires: obtaining chemicals of the highest purity from best
purity sources such as the USEPA Repository for Toxic and Hazardous
Materials, selecting the methodology for the compounds of interest,
conducting retention time studies, combining groups of organic
compounds to minimize overlapping gas chromatography peaks, and
conducting 0, 45-, and 90-day stability studies. Those compounds
proven stable are produced at two concentration levels in lots of
3,000. Random samples are withdrawn during production and sent to
referee laboratories for verification analyses. Upon verification,
new samples are advertised in the USEPA Quality Assurance Newsletter
and distributed to requesters.

Accomplishments: 1.

Distributed 55,074 drinking water QC samples to USEPA, USEPA
contractor, state, and local laboratories. Analytes included
pesticides, herbicides, residual chlorine, turbidity, trihalo-
methanes, trace metals for atomic absorption (AA) and
inductively-coupled plasma (ICP) analytical procedures,
nitrate/fluoride, and corrosivity.

2.	Produced the following analyte groups to replenish depleted
inventories: sodium/corrosivity and residual free chlorine. A
total of 22,200 ampuls were produced.

3.	Conducted stability testing on 14 QC series (pesticides, metals,
and volatiles).

Annual Report on QC Samples

Completed
(12/85)

-------
Page 4 of Project No. 10



Paqe 31 of 76

APPROACH

PE# BLC1A

Drinking Water - DU CI04





C. URD Contact

OUTPUT Quality Control/Performance Evaluation

Name John Winter

A.

FTS No. 684-7325

Resources



B. R/D $30K $(000) 36 PFT 0.1 OPFT

PFTE OPFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 10

Extramural Task: Establish Traceability of Quality Control (QC) and Performance

Evaluation (PE) Samples to the National Bureau of Standards (NBS).

Purpose:	The QC and PE samples utilized throughout the United States and

internationally in water-related monitoring programs must be of the
highest quality since they are involved in many important
decisions. As part of a stringent quality assurance program to
assure the veracity of the QC and PE samples, traceability to NBS is
established.

Approach:	An interagency agreement (IA6) was signed with NBS to develop a

protocol for traceability of Drinking Water related QC and PE
samples, and then to implement the protocol for top priority samples
of interest to the Agency and those for which NBS has expert
analytical capabilities.

Accomplishments: NBS verified concentrations, thereby establishing traceability for
pesticides (lindane, endrine and methoxychlor) for Water Supply (WS)
Studies 19 and 20, two herbicides (2,4-D and Silvex), and 14
volatile organic contaminants (VOCs) (trans and cis 1,2-dichloro-
ethylene, dibromochloropropane, o-dichlorobenzene, ethylbenzene,
chlorobenzene, sytrene, toluene, xylene, ethylene dibromide,
chloroform, bromodichloromethane, dibromochloromethane and
bromoform).

Status:

Annual Report on Traceability to NBS

Completed
(12/85)

-------
Page 5 of Project No. 10

APPROACH
Drinking Water - DU CI04

Page 32 of 76
PE# BLClA

OUTPUT Quality Control/Performance Evaluation
A.

C. ORD Contact
Name Harry Kolde
FTS No. 684-7325

Resources

B. R/D $9.5 $(000) 15.5 PFT 0.1 0PFT

PFTE 0PFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 10

Extramural Task: Conduct Verification Analyses on all performance evaluation
(PE)/quality control (QC) Samples.

Purpose:	Usage of large numbers and types of QC, PE and spiking/calibration

samples in USEPA programs to assess the quality of monitoring data
necessitates that true or reference values associated with the
samples are in fact, valid. Otherwise poor decisions could result
which would adversely impact the environment. Referee laboratories
are used to establish the veracity of all samples.

Approach:	Referee laboratories are selected through the competitive procure-

ment process upon the basis of a PE study and competitive cost for
the analytes of interest. These include trace metals, nutrients,
minerals, sodium and corrosivity, demand, priority pollutants in
samples designed for gas chromatograph (GC) and GC/mass spectrometer
(MS), polychlorinated biphenyls (PCBs) in oil and fish, synthetic
organic contaminants specified in the Drinking Water Strategy
Document, and for other analytes regulated by the Agency.

Accomplishments: Referee laboratories conducted: (1) 90 neat SOC analyses to

establish purity of materials in USEPA's Repository for Toxic and
Hazardous Materials, (2) 3,199 analyses on QC and PE samples
produced inhouse and on contract, (3) 320 analyses on spiking/
calibration solutions from USEPA's Repository for Toxic and
Hazardous Materials, (4) No analyses on neat surrogates related to
USEPA Methods 624 and 625, and (5) analyses on 32 spiking/
calibration solutions for surrogate compounds related to USEPA
Methods 624 and 625.

Status:

Annual Report on Referee Analytical Services

Completed
(12/85)

-------
Page 6 of Project No. 10



Page 33 of 76

APPROACH

PE# BLC1A

Drinking Water - DU C104





C. ORD Contact

OUTPUT Externalization of QA Programs.

Name John Winter

A.

FTS No. 684-7325

Resources

B. R/D $ OK $(000) 0 PFT 0 OPFT	 PFTE	 OPFTE

Purpose:

Approach:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 10

Inhouse Task: Externalization of Quality Assurance (QA) Programs.

Recover costs of production, distribution, and administration of
quality control (QC) and performance evaluation (PE) sample programs
associated with the drinking water, industrial waste, and water
quality program.

Promulgate a cost recovery rule for the preparation and distribution
of QC and PE samples, set up a mechanism for collecting such fees
through the USEPA Financial Management Office, and begin the
externalization process for these sample types.

Accomplishments: An externalization task force was formed of USEPA personnel from the
Comptroller's Office; Office of General Counsel; Office of Program
Management; Office of Acid Deposition, Environmental Monitoring and
Quality Assurance (OADEMQA); operating program offices; the regional
offices; and the three EMSL laboratories to study and recommend the
best option for externalization of QA support services. Concur-
rently, EMSL-Cincinnati prepared a white paper on costs and other
considerations for the Task Group. Discussions were also held
between the Contracts Management Division and EMSL-Cincinnati to
explore the best means to charge and collect user fees for these
services and to expedite return of funds to EMSL-Cincinnati for
maintenance of the QA program.

Based on these deliberations and discussions, OADEMQA prepared a
draft of a proposed rule: Proposed User Charges for Certain Quality
Control and Performance Evaluation Samples Under the Clean Water Act
and the Safe Drinking Water Act which was subsequently published in
the Federal Register on September 16, 1986. Comments are due by
October 31, 1986.

Status:	Report on the Externalization QA Proqram	Completed

(5/86)

-------
Drinking Water Research Committee

Page 34 of 76
PE No. BnOT"

A. OUTPUT: Improved and Validated Organic Analytical

C. ORD Contact

Methods for Drinking Water

Name: J. E. Lonqbottom

FTS No. 684-7308

B. RESOURCES: % 84.OK FTE 2.0



FY 86 ANNUAL REPORT

Project No. 11

Purpose and Approach



The purpose of this project is to provide new, improved or, alternate
analytical methods for monitoring synthetic organic chemicals in drinking
water. Sample concentration techniques, capillary column gas chromatography
(GC), GC-mass spectrometry (MS), and high performance liquid chromatography
(HPLC) methods will be investigated.

Progress and Accomplishments

Methods for Volatile Organic Chemicals (VOCs) - Methods 502.1, 503.1, 504, and
524.1 were modified to reflect public comment on the proposed VOCs maximum
contaminant levels (MCLs) and monitoring requirement. The principal changes
to the methods at this time involved reduction of the scope of Method 524.1 to
reflect conventional packed column analytical practices and strengthening the
identification criteria in this method to reduce false positives. Two
compounds were deleted from the scope of all purge and trap methods due to
reactivity (pentachloroethane) or poor purging efficiency bis (2-chloro-
isopropyl ether). The quality control (QC) section of all methods was
tightened to focus on control near the method detection limit. The revised
manual was forwarded to the Office of Drinking Water (ODW) in September.

Future plans are to incorporate synthetic organic chemical (SOC) methods into
the manual.

Reference Methodology for SOCs - Method 524.2 - A capillary column method,
including both wide-bore and conventional fused silica capillary column (FSCC)
technique, suitable for determination of the volatile VOCs, "1445" compounds,
and volatile SOCs with a single analysis was forwarded to ODW in September.

Method 502.2 - A capillary column (wide-bore) method for volatiles using the
Hall and photoionization detector (PID) detector in series was drafted based
upon in-house work. As with the GC/MS method (524.2), the new method shows
excellent precision and sensitivity. It is scheduled for completion in
October.

Method 505 - A micro-extraction method for organochlorine pesticides,
polychlorinated biphenyls (PCBs), and the SOC, alachlor, was completed and
forwarded to ODW in September. The method offers substantial savings in
analytical costs, if it is sensitive enough to measure MCLs for these
contaminants.

-------
Page 2 of Project No. 11	Page 35 of 76

Method 515 - A FSCC update of the electron capture derivatization method for
phenoxyacid herbicides was forwarded to ODW in September. The method has been
optimized for the chlorophenoxy acids on the SOC list and for pentachloro-
phenol.

GC/MS Methods for Pesticides and PCBs - A capillary column method is being
developed for application to selected SOC pesticides. Work this quarter
centered around choosing selected ion monitoring (SIM) parameters for the
analysis of these SOCs. Method range studies for these compounds for both the
full scan mode and the SIM mode were completed but no methods write-up was
prepared pending further ODW guidance.

Method for Acrylamide - Decomposition of the synthesis product, dibromo-
propioamide, has slowed development of a method for this compound.

Instability and anomalies in GC have led to a redirection toward understanding
the reactions of acrylamide with chlorine in water. Work on this method is
expected to continue for, at least, another six months.

Analytical Methods for the National Groundwater Pesticides Survey - A total of
five broad spectrum methods, and a sixth method specifically for ethylene
thiourea (ETU) have been drafted. Revision of the methods to incorporate
final data and peer review comments continued through September and should be
completed in October. Two methods (507, Nitrogen/Phosphorus Pesticides and
508, Organochlorine Pesticides) were forwarded to ODW in September to support
the SOC proposal.

Analytical Methods for Disinfection By-Products—Work was conducted to test
the most promising analytical approach for chlorinated acetic acids. A
modification of Method 515 appears to be suitable for these compounds. Work
on this project will be accelerated in the next quarter.

-------
APPROACH

Page 36 of 76

J~. OUTPUT: Evaluation of Alternate Test Procedures to	uku contact

Meet Requirements of the Safe Drinking Water NAME: Terence M. Grady
Act	FTS No. 684-7301

Resources:

B.	$(000) 50.0 PFT 1.0 OPFT	PFTE	OPFTE

ANNUAL REPORT	PROJECT NUMBER 12

Purpose and Approach

The Equivalency Program is intended to encourage analytical methods development
or improvement by the regulated community and by manufacturers of pollution
measuring instruments. These alternate test procedures (ATPs) may be approved
for case-by-case or nationwide use as mandated by 40 CFR Part 141.27. After
receipt of unsolicited ATP applications, necessary external and/or internal
technical reviews are conducted and coordinated to provide a technically sound
recommendation on approval or denial of the proposed ATP. Items considered
during review include: availability of a well documented test procedure, docu-
mentation of the applicability of the proposed procedure, performance character-
istics such as accuracy, precision, and method detection limits, and equivalency
data to an approved test procedure.

Progress and Accomplishments

During FY86, a total of 23 requests for approval of ATPs were received. Five of
the requests were for nationwide approval. The remaining 18 were limited-use
requests. Quarterly and annual ATP reports were distributed to the regional
and Headquarters staff. As a result of the comparability data submitted by the
J. T. Baker Chemical Company, approval for the use of solid phase extraction
columns for pesticides was recommended.

The following table summarizes the applications received by this office and the
actions recommended:

National Interim Primary Drinking Water Regulations (NIPDWR): 23

a.	Nationwide:	5

b.	Limited Use:	18

c.	Action Recommended:

1.	Recommended Approval:	15

2.	Recommended Disapproval:	0

3.	Non-Germane (Not ATP):	2

4.	Requested Further Data:	5

5.	Pending:	1

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APPROACH

Page 37 of j£_
PE# BK1A

Drinkinq Water - DU C104





C. ORD Contact

OUTPUT Method Validation Study

Name Harold Clements

A.

FTS No. 684-7325

Pp^nnrrpc

B.	$(000) 0 PFT 0 OPFT	 PFTE 	 OPFTE

Inhouse Task:

Purpose:
Approach:

Accomplishments:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 13

Conduct Method Validation Study for Maximum Trihalomethane Potential
(MTP).

Verification of USEPA Method 510.1 with bias and precision data.

Produce performance evaluation samples and develop collaborative
study to produce data to support the use of the USEPA Method 510.1.

Samples were designed and produced to conduct a formal method
validation study for MTP (USEPA Method 510.1). Samples were
distributed in the second quarter of FY85 and data returned to the
Quality Assurance (QA) Branch in the third quarter. The necessary
statistical calculations were completed and the report written.

Status:

Final Report for MTP Method Validation Study

Completed
(9/86)

-------
Page 2 of Project No. 13

Page 38 of 76
APPROACH	PE# EOTlA

Drinking Water - DU CI04		 		

C. ORD Contact

OUTPUT Method Validation Study	Name Ray Wesselman

A	.	FTS No. 684-7325

Resources

B.	R/D $700K $(000) 741.7 PFT 1.0 OPFT	 PFTE	OPFTE 	

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 13

Extramural Task: Method Validation Studies for Volatile Organic Chemicals (VOCs),
Synthetic Organic Chemicals (SOCs), and Section 1445 Organic
Chemicals.

Purpose:	In support of the Safe Drinking Water Act (SDWA), interlaboratory

method validation studies (IMVS) are conducted for USEPA methods for
the purpose of establishing bias/recovery, precision, and other
statistics.

Approach:	MVSs are conducted by a prime contractor involving 10 contract

laboratories. The prime contractor provides three Youden pairs of
ampul concentrates containing the compounds specified. The
participating laboratories spike the concentrates of analytes into
water types and analyze the sample according to the USEPA method.
Analytical data are processed with USEPA's IMVS computer program
which provides regression equations for bias and precision and other
statistics.

Accomplishments: A request for proposal (RFP) was developed to obtain 10 participants
in an IMVS for 8 drinking water methods which included VOCs, SOCs,
and 1445 organics. Offerors' proposals were evaluated and those
judged technically acceptable were sent performance evaluation (PE)
samples to confirm laboratory capabilities. Contracts will be
awarded in October 1986 with the IMVS commencing shortly thereafter.

Status:

Status Report on the IMVS for VOCs, SOCs, and
Section 1445 Compounds

On Schedule
(9/«7)

-------
APPROACH
Drinking Water - DU C104

page 39 ot 2JL_
PE# TJLC1A

Produce and distribute microbiological performance
OUTPUT evaluation samples for water supply laboratory
A. certification program.

C. ORD Contact

Name Gary Collins
FTS No. ' 684-7325

R6S0urc6S

B.	$(000) 18.3 PFT 0.4 OPFT	 PFTE	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 14

Development and Preparation of Microbiological Performance
Evaluation (PE) Study Samples for Certification.

Under the Safe Drinking Water Act (SDWA) and the National Interim
Primary Drinking Water Regulations (NIPDWR) and amendments,
acceptable performance in PE studies is an annual requirement for
certification of drinking water laboratories. In response to this
need, the Quality Assurance (QA) Branch develops and provides sample
series for each maximum contaminant level (MCL) analyte, and for
monitoring analytes, listed in the primary drinking water
regulations and amendments.

Approach:	Vials of lyophilized coliform organisms are designed, prepared and

verified by analyses. Each semi-annual study of approximately 100
laboratories is conducted using these cultures.

Accomplishments: Samples for studies WSM07 and WSM08 (concurrent with WS017 and

WS018) for total coliforms were completed and Study WSM09 initiated.

Task:
Purpose:

Status:

Develop and Prepare Coliform Samples for WSM07
and WSM08

Completed
(7/86)

-------
Page 2 of Project No. 14



Page 40 of 76

APPROACH

PE# BLC1A

Drinking Water - DU C104



Conduct semi-annual performance evaluation studies

C. ORD Contact

OUTPUT for chemical and microbiological analysis of

Name Paul Britton

A. drinking water.

FTS No. 684-7325

Resources

B.	$(000) 45.7 PFT 2.0 OPFT	 PFTE 	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 14

Conduct Water Supply (WS) Laboratory Performance Evaluation (PE)
Studies.

To provide an objective basis for evaluating drinking water
laboratory performance for certification, under National Interim
Primary Drinking Water Regulations (NIPDWR) of the Safe Drinking
Water Act (SDWA).

Laboratories that have applied for, or currently have, USEPA
Drinking Water Laboratory Certification, are required to participate
annually in PE studies for each analyte to be certified, and to
perform satisfactory. PE samples cover 8 trace metals, nitrate,
fluoride, 4 pesticides, 2 herbicides, 4 individual and total
trihalomethanes, turbidity, free residual chlorine, and total
coliforms at two concentration levels each, as well as one level for
sodium and corrosivity analytes. USEPA compares the analytical
results from each laboratory against acceptance limits generated
from the known true concentrations and results from the current and
past studies. Laboratories performing unacceptably or missing the
primary study can participate in a second (follow-up) study each
year. Laboratories performing acceptably in one study each year are
eligible for USEPA certification.

Accomplishments: WS-PE study reports were generated for studies WS017 and WS018, with
713 and 945 participating laboratories, respectively. Study WS019
was initiated and is to be completed next year. WSM07 and WSM08
microbiological samples were shipped to approximately 100 USEPA and
state laboratories at the same time as other WS study samples. The
laboratories reported the microbiological data separately, but final
study reports covered all data reported.

During the studies this year, special PE samples containing 20 new
volatile organics (VOCs) were provided at two levels each for
voluntary analyses to provide the Office of Drinking Water (ODW)
with background information on these compounds considered for
regulation but not for certification. VOC samples for other
volatile organics will be added for voluntary analysis in all future
studies.

Status:	Individual Laboratory PE Reports Distributed to	Completed

Participants in Study WS017, WS018, WSM07, and	(9/86)

WSM08.

Task:
Purpose:

Approach:

-------
Drinking Water Research Committee

Page 4} of 76
PE No. BNTTiA"

A. OUTPUT: Laboratory Certification Program for
Drinking Water Quality Assurance

C. ORD Contact
Name: J. J. Lichtenberq
FTS No. 684-7306

B. RESOURCES: % 455.7K FTE 6.0



FY 86 ANNUAL REPORT

Purpose and Approach

Project No. 15

The purpose is to evaluate regional laboratories and personnel for capability
to provide quality data in support of the National Interim Primary Drinking
Water Regulations (NIPDWR) monitoring program, to approve regional labora-
tories to do the required analyses, and to certify the regional staffs. This
will be accomplished by review of the regional certification program and
laboratory performance records and on-site evaluation of the regional labora-
tories.

Progress and Accomplishments

Laboratory Certification Courses - Annual laboratory certification courses
were prepared and conducted for chemistry and microbiology during the month of
June. These courses provided the regional/state chemists and microbiologists
the opportunity to become officially certified and be responsible for conduct-
ing on-site audits of state and local laboratories requesting certification
under the Safe Drinking Water Act 1974 (SDWA). All regional requests were met
and, with only a few exceptions, the states' requests and overall needs were
satisfied. These courses were presented by the Environmental Monitoring and
Support Laboratory - Cincinnati (EMSL-Cincinnati) staff with able assistance
from professional staff of the Technical Support Division, Office of Water.
Plans are to offer these two courses again in FY 87.

Annual Review of Regional Activities - Close liaison was maintained with the
regions through key contacts with the regional Quality Assurance Officers
(QAOs) and Drinking Water Representatives. Our laboratory QAO and Quality
Assurance Management Staff (QAMS) representative actively participated with
regional and program office representatives in developing and implementing QA
techniques at the regional/state level. On-site visits were made to Regions
4, 5, and 6. The United States Geological Survey (USGS) laboratory in Denver,
Colorado was evaluated for compliance with Drinking Water regulations on April
15-17. This was done at the request of Regions 2 and 8. The USGS laboratory
can be certified for inorganic and organic analysis of drinking water. Plans
are being made to begin the next round of regional visits during the second
half of FY 87. Eight regional on-site evaluation reports for state labora-
tories were reviewed in FY 86. These were discussed with appropriate regional
personnel and approved for distribution and subsequent certification actions.
Review of four additional reports are pending.

-------
Page _2_ of Project No. 15

Page 42 of 76

The Equivalency Program processed twenty-three (23) requests for approval of
alternate test procedures. Eighteen (18) of these were for limited use and
five (5) were for nationwide approval.

Conduct Performance Evaluation (PE) Studies - WS017 and WS018, PE studies
involving greater than 1000 laboratories each, were conducted in FY 86 for all
chemical maximum contaminant levels (MCLs) and control analytes. The chemical
sample concentrates were prepared, instructions written, PE samples
distributed as unknowns. Data were returned to the QA Branch for processing
and preparation of reports for each laboratory. Reports were sent to the
participants and copies to the respective regional QAOs for any follow-up
actions. WSM07 and WSM08, PE Studies for microbiological MCLs, for total
coliforms were also completed for certification of USEPA and state
laboratories in FY 86.

Analyze Trends in PE Sample Program and Provide Performance Criteria - Updated
statistics are provided on total analyses and method-by-method for Water
Supply (WS) Studies WS017 and WS018 to Maria Gomez-Taylor of the ODW. As a
special project, a computer program is being developed to summarize USEPA,
state, and "all" laboratory performances in WS PE studies over the past years
so as to identify those missing one or more analytes (exceeding acceptance
limits) in two and in three successive studies, on an analyte-by-analyte
basis. Generalized statistical estimates for each MCL contaminant (analyte)
are also provided. These stated the mean recoveries and standard deviations
of each analyte as a percentage of the MCL based on PE study data. Analytes
included the current MCLs and the nine proposed volatile organic chemicals
(VOCs).

Preparation and Distribution of Known Quality Control (QC) Samples, Calibra-
tion Standards and Unknown PE Samples for all Regulated Contaminants - All VOC
analytes specified in proposed revision of the primary drinking water regula-
tions are now available as certified calibration standards. Of the 126
analytes, VOCs and synthetic organic chemicals (SOCs) specified in the
Drinking Water Strategy, 90 are certified for distribution as calibration
standards. Over 75,000 calibration standards were distributed by
EMSL-Cincinnati to USEPA laboratories, contractors/grantees, state, and local
laboratories engaged in environmental monitoring.

EMSL-Cincinnati distributed over 55,000 drinking water QC samples to USEPA
regional, state, local, and USEPA contractor laboratories. Analytes included
pesticides, herbicides, residual chlorine, turbidity, trihalomethanes, trace
metals, nitrate, fluoride, corrosivity, Temik, and the new VOCs proposed for
regulation.

Provide Technical Assistance - Numerous telephone requests were handled
directly by technical staff on matters related to chemical and microbiological
methods usage, and to QA requirements/usage under the SDWA. In addition,
specialized laboratory analyses were provided to the regions and states for
uranium, gross alpha/beta, radium-226, and radium-228.

-------
Page 3 of Project No. 1^ Page 43 of 76

Revision of the Drinking Water Certification Manual was begun at the request
of the Office of Drinking Water (ODW). EMSL-Cincinnati has eight staff
members serving in various capacities on the Committee, including
Chairmanships of the Implementation and Analytical Methods and Quality Control
Committees, Analytical Chemistry Methods Work Group and as members of the
Steering Committee. Two steering committee meetings were attended at USEPA
headquarters. The Analytical Chemistry and Microbiology Work Groups have held
several meetings. Two of these included non-USEPA (state) members. The
second drafts of these revised chapters have been transmitted to ODW for
review.

-------
Drinking Water Research Committee

Page 44 of 76
PE No. BlCIF

A. OUTPUT: Standardized and Validated Radiochemical	C. ORD Contact

Methods for Analysis of Drinking Water Name: 6. D. McKee
			FTS No. 684-7372

B. RESOURCES: % 130.5K	FTE 3.0

FY 86 ANNUAL REPORT	Project No. 16

Purpose and Approach

The purpose of this project is to evaluate and modify as necessary procedures
for radiochemical analysis of drinking water and to provide analytical
technical assistance to the Office of Drinking Water (ODW). Methods for
radium, uranium, and radon will be investigated. Up to 1176 survey samples
will be analyzed.

Progress and Accomplishments

National Inorganics and Radionuclides Survey (NIRS) - Four-hundred and
seventy-five (475) samples for 37 elements totaling 22,191 analyses were
completed by inductively coupled plasma (ICP) this quarter. To verify the
sample analyses, an additional 8869 quality control (QC) analyses also were
completed. A total of 1176 samples were received for the NIRS project. No
additional samples are expected. The table below provides a summary of
samples received and analyses completed to date.



Samples

Samples

Samples

Completed

QC Samples

Analysis

Received

Started

Completed

This Quarter

This Quarter

Radon

1176

1176

1176

80



Uranium

1176

1176

1176

73

7

Gross A/B

1176

1176

1176

70

9

Ra-226

1176

1173

1128

86

12

Ra-228

1176

1144

1050

84

12

A summary report on this work was prepared and forwarded to the NIRS manager
in September.

The following technical assistance was provided in the area of radiochemistry
and other drinking water related problems:

o Four samples received by the Water Engineering Laboratory of Pima County
Health Department, Arizona were analyzed for uranium, gross alpha and beta.

o Five Ra-226 and 15 uranium analyses were performed for the Inorganics and
Particulates Control Branch, Drinking Water Research Division for the
pilot study for removal of radium at Lamont, Illinois. Ten analyses for
Ra-226, five Ra-228, and 10 gross alpha and beta were performed at the
request of the same division for the project to evaluate removal and waste
disposal at Redhill Forest Development in Colorado.

-------
FY 86 OUTPUT PLAN
MICROBIOLOGY SECTION, BMB, EMSL-CINCINNATI

DRINKING WATER - MONITORING SYSTEMS AND QUALITY ASSURANCE

Page 45 of 76	

PE* Zm

OUTPUT Coliform Analysis - Drinking Water - Quality Assurance

ORD Contact
Name

R. Bordner
FTS No. 684-7319

Resources:

$(000) 55.2K PFT 	1^0 OPFT 0.0 PFTE	UO OPFTE 0.0

Project 17

ANNUAL REPORT - FY 86

The final report on the comparison of the hydrophobic grid membrane filter
(HGMF) procedure and standard membrane filter (MF) methods for coliform
analysis was forwarded to the Office of Drinking Water and submitted to
the Journal of Applied and Environmental Microbiology for publication. No
significant differences were found between results from the standard MF
and the HGMF.

An interim report, "Development and Evaluation of an Alternative Total
Coliform Membrane Filter Medium," was prepared, peer reviewed, and
forwarded to the client program offices. The candidate and standard
media, ranked in order of verified coliform recovery, were m-TECM, m-LSB,
m-T7, m-Endo, and m-HAB. m-TECM and m-T7 were developed through
cooperative agreements with the University of Rhode Island and Montana
State University respectively, m-HAB was developed inhouse, m-LSB is a
British medium, and m-Endo is the standard test medium. In a
collaborative test of four media, m-TECM, m-T7, m-HAB, and m-Endo, by 23
laboratories from many different geographical areas analyzing local
samples, a statistical evaluation showed no significant difference among
the media. Plans were made for additional testing of lyophi1ized natural
samples to be shipped to and analyzed by all participating laboratories.

The statistical analyses of the data from the project to determine the
precision and accuracy of the MF and most probable number (MPN) total
coliform procedures were completed and an interim report entitled
"Precision and Relative Accuracy of the Membrane Filter and Most Probable
Number Total Coliform Methods Used for Drinking Water Analysis" was
prepared. There was a significant difference between the precision of the
two methods when natural samples were analyzed. Using the ASTM method for
determining relative accuracy, the MF test was more accurate than the MPN
method when the 23% positive bias of the latter was removed.

Microbiologists participated in on-site visits to the Environmental
Services Division, Region 3, Wheeling Office, and Regions 5 and 6, to
determine compliance with drinking water laboratory certification
requirements.

-------
Page 2 of Project No. 17

Page 46 of 76

A training course entitled, "Drinking Water Laboratory Certification for
Microbiology," was attended by 20 laboratory certification officers from
USEPA regions, states, and territories.

A paper entitled "Reliable Data Begin with Well-Planned Sampling
Procedures," was presented March 23 at a workshop on "New Developments in
Drinking Water," sponsored by the Board of Education and Training of the
American Society for Microbiology.

The final report by Drexel University on the application of the Presence-
Absence (P-A) test in small water systems was sent out for peer review.
The P-A test gave equivalent or better recovery of total coliforms from
drinking water. The University presented a poster on "The Effects of
Water Quality Parameters on Coliform Detection by Clark's P-A Test," at
the Annual Meeting of the American Society for Microbiology, March 26,
1986, and a report on "Comparison of Clark's P-A Test and the Membrane
Filter Method for Coliform Detection in Potable Waters," was published by
the Journal of Applied and Environmental Microbiology.

The results from the research by McNeese State University (MSU) and
Florida International University (FIU) to determine sample holding effects
on bacterial populations confirmed in general the inhouse findings that
coliform counts decreased within 24 hours whereas heterotrophic plate
counts increased over time. MSU is modifying a third draft of the final
report and the FIU report is being peer reviewed.

The University of Rhode Island completed the field testing for the project
to develop an improved MF coliform medium.

-------


APPROACH
Solid Waste - DU D109

Page 47 ot jL.
PE# fsfflA

OUTPUT Quality Assurance
A.



C. ORD Contact
Name Harry Kolde
FTS No. 684-7325

Resources

B. R/D 184.2 $(000) 195.2 PFT 0.1 OPFT	 PFTE	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 18

Extramural Task: Develop and Maintain USEPA's Repository for Toxic and Hazardous
Materials.

Maintain the USEPA Repository for Toxic and Hazardous Materials to
provide spiking/calibration solutions of organic compounds in
support of monitoring under regulations of the Resource Conservation
and Recovery Act (RCRA).

Compounds of interest to RCRA are purchased or synthesized,
purified, dissolved in appropriate solvents, and dispensed in 2 mL
ampuls. The verity of pure compounds and concentration of the
compound in the ampul are verified by referee laboratories. Upon
verification, spiking/calibration solutions are advertised in the
Quality Assurance Newsletter and distributed to USEPA, Regional,
state, local, commercial, and RCRA contractor laboratories engaged
in monitoring the environment.

Accomplishments: 1. Of the 296 organic compounds listed in RCRA Appendix VIII, 272

compounds in neat form are in stock, of which 184 have been
certified for purity, 132 analytes have been certified for
distribution as calibration standards and 2 new standards are
being tested for verity by referee laboratories.

Purpose:

Approach:

2.	A total of 75,200 certified calibration standards were
distributed to 1930 USEPA, Regional, state, local, and USEPA
contract laboratories. This represents a 45% increase over FY85.

3.	2,3,7,8-tetrachlorodibenzo-p-dioxin (TCDD)-native and
calibration standards are certified for distribution.

4.	Of the 247 compounds listed in the RCRA Appendix IX ground water
list, 223 are stocked as neats in the Repository and 152 are
available as calibration standards.

Status:

Annual Report of Repository Activities

Completed
(12/85)

-------
Page 2 of Project No. 18



APPROACH
Solid Waste - DU D109

Page 48 of 76
PE# B5U1A

OUTPUT Quality Assurance
A.



C. 0RD Contact
Name Terry Grady
FTS No. B84-7325

Resources

B. R/D $127 $(000) 141.6

PFT 0.2 0PFT

PFTE 0PFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 18

Extramural Task: Conduct Verification Analyses on all performance evaluation (PE)/
quality control (QC) Samples.

Usage of large numbers and types of QC, PE, and spiking/calibration
samples in USEPA programs to assess the quality of monitoring data
necessitates that true or reference values associated with the
samples are in fact, valid. Otherwise poor decisions will result
which could adversely impact the environment. Therefore, referee
laboratories are used to establish the veracity of all samples.

Referee laboratories are selected through the competitive
procurement process upon the basis of performance evaluation and
cost for the analytes of interest. These analytes include trace
metals, nutrients, minerals, sodium and corrosivity, demand, trace
organics in samples designed for gas chromatograph (GC) and GC/mass
spectrometer (MS), polychlorinated biphenyls (PCBs) in oil, fish and
sediment, and synthetic organic contaminants specified in the
Organic Resources Conservation and Recovery Act (RCRA) Appendix VIII
compounds.

Accomplishments: Referee laboratories conducted: (1) 426 neat organic analyses to
establish purity of materials in USEPA's Repository for Toxic and
Hazardous Materials, (2) 3,668 analyses on QC and PE samples
produced inhouse and on contract, (3) 402 analyses on spiking/
calibration solutions from USEPA's Repository for Toxic and
Hazardous Materials, (4) No analyses on neat surrogates related to
USEPA Methods 624 and 625, and (5) analyses on 18 spiking/
calibration solutions for surrogate compounds related to USEPA
Methods 624 and 625.

Purpose:

Approach:

Status:

Annual Report of Referee Analytical Services

Completed
(12/85)

-------
Page 3 of Project No. 18



Paqe 49 of 76

APPROACH

PE# BSD1A

Solid Waste - DU D109



Performance evaluations and waste characterization

C. ORD Contact

OUTPUT for Agency and contract laboratories.

Name Harold Clements

A.

FTS No. 684-7325

B.	$(000) 80.7 PFT 1.1 OPFT	 PFTE 	 OPFTE

Inhouse Task;
Purpose:
Approach:
Accomplishments:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 18

Prepare Solid Waste Samples as Unknowns for Performance Evaluation

(PE) Studies

Evaluate the skills of Resource Conservation and Recovery Act (RCRA)
contract laboratories.

Develop a series of typical natural waste samples which are stable,
homogeneous, and capable of analyses as routine samples.

PE samples were prepared and distributed to RCRA contract
laboratories for:

1.	Interlaboratory Comparison Study V: Organic and inorganic type
solid waste samples were sent to 20 RCRA laboratories in January
1986. Results of the Quality Assurance (QA) Branch and referee
laboratories were returned to Office of Solid Waste (0SW).

2.	Interlaboratory Comparison Study VI: Organic and inorganic
samples were prepared and distributed to 50 USEPA, USEPA
contractor, and other RCRA laboratories. The QA Branch and its
referee laboratories analyzed the samples and provided
statistical estimates to the OSW. The OSW developed acceptance
limits for evaluating participating laboratories.

3.	Interlaboratory Comparison Study VII - Diatomaceous earth and
clay were used as a base to prepare a solid waste samples spiked
with selected Appendix VIII compounds. The PE samples were sent
in July 1986 to 50 laboratories for testing. The inorganic and
the organic samples were analyzed by the QA Branch and Its
referee laboratories and the results sent to OSW.

4.	Design of new samples for the next study is in the pilot stage.

Status:	Reports: PE Samples for RCRA Contract Laboratories	Completed

(12/85)

-------
Page 4 of Project No. 18



APPROACH
Solid Waste - DU D109

Page 50 of 76
PE# USUI A

OUTPUT Quality Assurance
A.



• C. ORD Contact
Name Ed Berq
FTS No. 684-7325

Resources

B. R/D $64.9 $(000) 70.9

PFT 0.1 OPFT

PFTE OPFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 18

Extramural Task: Maintain USEPA's Quality Control (QC) Sample Program for
Water-related Analytes.

Purpose:	QC samples are provided to USEPA, USEPA contractor, regional, state,

and local laboratories as a check on the analyst's technique and
analytical methodology. Such checks are necessary to monitor
quality of data being generated in carrying out mandates of the
Resource Recovery and Conservation Act (RCRA).

Approach:	Bionetics, Inc., the technical service contractor, provides personnel

to develop, produce, and distribute QC samples. Development of new
sample types requires: obtaining chemicals of the highest purity
from best sources including the USEPA Repository for Toxic and
Hazardous Materials, selecting the methodology for the compounds of
interest, conducting retention time studies, and finally combining
groups of organic compounds to minimize overlapping gas chromatog-
raphy peaks and conducting 0, 45, and 90 day stability studies.

Those compounds proven stable are produced at one concentration
level in lots of 5,000. Random samples are withdrawn during
production and sent to referee laboratories for verification. Upon
verification, the new samples are advertised in the USEPA Quality
Assurance Newsletter and distributed to requesters.

Accomplishments: 1. A total of 285,167 QC samples were distributed to USEPA, USEPA

contractor, state, and local laboratories.

2.	A total of 181,000 ampuls were produced to replenish depleted
inventories and included such QC series as trace metals,
cyanide, polychlorinated biphenyls (PCBs) in oil and acetone,
pesticides, and seven volatile organic series.

3.	Of the 369 analytes listed in Appendix VIII, 119 are available
for distribution.

Status:

Annual Report of QC Sample Program

Completed
(12/85)

-------
Page 5 of Project No. 18

Sol id

APPROACH
Waste - DU D109

Page 51 of 76
PE# TES1A

OUTPUT Continue NBS Traceability
A.



C. ORD Contact
Name John Winter
FTS No. 684-7325

Resources

B. R/D $20K $(000) 20 PFT 0.0

OPFT

PFTE OPFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 18

Extramural Task: Establish Traceability of Quality Control (QC) and Performance

Evaluation (PE) Samples to the National Bureau of Standards (NBS).

Purpose:	The QC and PE samples utilized throughout the United States and

internationally in water/wastewater related monitoring programs must
be of known quality since they are involved in many important
decisions. As such, there is a stringent quality assurance program
to assure the veracity of the QC and PE samples, the program for
traceability to the NBS is established.

Approach:	An interagency agreement (IAG) was signed with NBS to develop a

protocol for traceability of QC and PE samples, and then to
implement the protocol for those analytes of interest to the Agency
for which NBS has expert analytical capabilities.

Accomplishments: NBS verified concentrations thereby establishing traceability for
pesticides (lindane, endrine and methoxychlor), two herbicides
(2,4-D and Silvex), and 14 volatile organic contaminants (trans and
cis 1,2-dichloroethylene, dibromochloropropane, o-dichlorobenzene,
ethylbenzene, chlorobenzene, sytrene, toluene, xylene, ethylene
dibromide, chloroform, bromodichloromethane, dibromochloromethane
and bromoform). Seven sludges which are to be used in an
interlaboratory SW-846 method validation study are currently being
analyzed for trace metals.

Status:

Annual Report on NBS Traceability

Completed
(12/85)

-------
Page 6 of Project No. 18



Page 52 of /b

APPROACH

PE# BSD1A

Solid Waste - DU D109





C. ORD Contact

OUTPUT Externalization of QA Programs.

Name John Winter

A.

FTS No. 684-7325

Resources



B. R/D $ OK $(000) 0 PFT 0 OPFT

PFTE OPFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 18

Inhouse Task: Externalization of Quality Assurance (QA) Programs.

Purpose:	Recover costs of production, distribution, and administration of

quality control (QC) and performance evaluation (PE) sample programs
associated with the drinking water, industrial waste, and water
quality program.

Approach:	Promulgate a cost recovery rule for the preparation and distribution

of QC and PE samples, set up a mechanism for collecting such fees
through the USEPA Financial Management Office, and begin the
externalization process for these sample types.

Accomplishments: An externalization task force was formed of USEPA personnel from the
Comptroller's Office; Office of General Counsel; Office of Program
Management; Office of Acid Deposition, Environmental Monitoring and
Quality Assurance (OADEMQA); operating program offices; the regional
offices; and the three EMSL laboratories to study and recommend the
best option for externalization of QA support services. Concur-
rently, EMSL-Cincinnati prepared a white paper on costs, for
consideration by the Task Group. Discussions were also held between
the Contracts Management Division and EMSL-Cincinnati to explore the
best means to charge and collect user fees for these services and to
expedite return of funds to EMSL-Cincinnati for maintenance of the
QA program.

Based on these deliberations and discussions, OADEMQA prepared a
draft of a proposed rule: Proposed User Charges for Certain Quality
Control and Performance Evaluation Samples Under the Clean Water Act
and the Safe Drinking Water Act which was subsequently published in
the Federal Register on September 16, 1986. Comments are due by
October 31, 1986.

Status:

Report on the Externalization QA Program

Completed
(5/86)

-------
Page 7 of Project No. 18

APPROACH
Solid Waste - DU D109

OUTPUT Quality Assurance
A.

C. ORD Contact
Name Ed B
FTS No.

Rpcnnrrp^

B. R/D $ OK $(000) 0 PFT 0 OPFT

PFTE

OPFTE

Inhouse Task;

Purpose:

Approach:

Accomplishments:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 18

Performance Evaluation (PE) Samples for the Ground Water Monitoring
Program.

Evaluate the performance of laboratories providing analyses of
ground water samples collected at selected hazardous waste sites.

A set of organic and inorganic PE samples are prepared by Bionetics,
Inc., and sent to the field sample collection team at the hazardous
waste stie. The PE samples are integrated into the samples
collected at the site and then sent to laboratories under contract
to USEPA. The analytical results scored were based upon past PE
studies, interlaboratory method studies, analytical methods, and
other sources.

The PE samples for 15 sites were prepared and sent to two different
groups of contract laboratories. These results were then used to
help assess the quality of data being generated by the contract
laboratory for each site by a panel consisting of personnel from
EMSL-Las Vegas, EMSL-Cincinnati and the Office of Solid Waste
(Headquarters), ICAIR Life Systems, and the regional offices.

Status:

Status Report on PE Samples for the Ground
Water Monitoring Laboratories

On Schedule
(12/86)

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APPROACH
Solid Waste - DU D109

Page 54 of 76
PE# ES1J1A

OUTPUT Interlaboratory Method Study
A.

C. ORD Contact

Name Ray Wesselman
FTS No. 684-7325

Resources

B. R/D $325K $(000) 325 PFT 0 OPFT	 PFTE 	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 19

Extramural Task: Conduct interlaboratory method validation studies (IMVSs) to obtain
precision and bias statements for USEPA Solid Waste (SW) 846
methodology.

Purpose:	In support of the Resource Conservation and Recovery Act (RCRA),

IMVSs are conducted for USEPA analytical methdology to establish
precision, bias, and other statistical estimates of performance.

Such statistics are used to develop enforcement limits, establish
quality control (QC) charts during routine analyses of pollutants,
and provide confidence limits for QC samples.

Approach:	MVSs are conducted by a prime contractor involving 10 laboratories

selected by USEPA. The selection is based upon laboratory
experience with similar analyses, and performance on similar
analytes. The prime contractor prepares three Youden pairs of
samples as concentrates, each containing compounds specified in the
method. The participating laboratories spike the concentrates into
reagent water and solid waste matrices and analyze them according to
the USEPA SW-846 methods. Analytical data are processed with the
IMVS computer program which provides regression equations for
recovery and precision and other statistics. Final reports are
prepared for each USEPA method. The regression equations are used
to develop performance criteria which are then incorporated into the
method write-up.

Accomplishments: A request for proposal (RFP) was developed and sent to perspective
participants in the IMVS for SW-846 Method 8270, Base/Neutrals.
Technically-acceptable laboratories received PE samples and 10
laboratories selected based on good performance. The IMVS should
commence early in FY87.

Status:

Status Report: IMVS on SW-846 Method 8270

On Schedule
(9/87)

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Page 2 of Project No. 19

APPROACH
Solid Waste - DU D109

Page 55 of 76
PE# ESUIA

OUTPUT Interlaboratory Method Study
A.

C. ORD Contact

Name Ray Wesselman
FTS No. 684-7325

B. R/D $325K $(000) 325 PFT 0 OPFT	 PFTE 	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 19

Extramural Task: Conduct interlaboratory method validation studies (IMVSs) to obtain
precision and bias statements for USEPA Solid Waste (SW) 846
methodology for Acrolein and Acrylonitrile.

Purpose:	In support of the Resource Conservation and Recovery Act (RCRA),

IMVSs are conducted for USEPA analytical methdology for the purpose
of established accuracy, precision, and other statistics. Such
statistics are used to develop enforcement limits, establish quality
control (QC) charts during routine analyses of pollutants, and
provide confidence limits for QC samples.

Approach:	MVSs are conducted by a prime contractor using 10 laboratories

selected by USEPA based upon their performance with similar analyses
and performance on similar analytes. The study includes analyses of
three Youden pairs of ampul concentrates containing the compounds
specified in the analytical method. The participating laboratories
spike the concentrates into reagent water and solid waste matrices
and analyze them according to the USEPA SW-846 methods. Analytical
data are processed with the USEPA IMVS computer program which
provides regression equations for bias and precision and other
statistics. Final reports are prepared for each USEPA method.

Accomplishments:

The IMVS for acrolein and acrylonitrile was temporarily delayed
until research and development work can be completed on the
analytical procedure.

Status:

Status Report: IMVS on SW-846 Method 8230
Acrolein and Acrylonitrile

On Schedule
(9/87)

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Page 3 of Project No. 19

APPROACH
Solid Waste - DU D109

Page 56 of 76
PE# BSD1A

OUTPUT Interlaboratory Method Study
A.

C. ORD Contact
Name Ed Berq
FTS No. 684-7325

Resources

B. R/D $0K $(000) 0 PFT 0 OPFT	 PFTE	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 19

Extramural Task; Conduct interlaboratory method validation study (IMVS) to obtain
precision and accuracy statements for USEPA Solid Waste (SW) 846
methodology for Trace Metals by Atomic Absorption (AA).

Purpose:	In support of the Resource Conservation and Recovery Act (RCRA),

IMVSs are conducted for USEPA analytical methdology for the purpose
of established accuracy, precision, and other statistics. Such
statistics are used to develop enforcement limits, establish quality
control (QC) charts during routine analyses of pollutants, and
provide confidence limits for QC samples.

Approach:	MVSs are conducted by a prime contractor using 10 laboratories

selected by USEPA based upon their performance with similar analyses
and performance on similar analytes. The study includes analyses of
three Youden pairs of ampul concentrates containing the compounds
specified in the analytical method. The participating laboratories
spike the concentrates into reagent water and solid waste matrices
and analyze them according to the USEPA SW-846 methods. Analytical
data are processed with the USEPA IMVS computer program which
provides regression equations for bias and precision and other
statistics. Final reports are prepared for each USEPA method.

Accomplishments: A request for proposal (RFP) was developed and sent to prospective
participants in the IMVS for SW-846 methods 3005, 3010, and 3050 -
Trace Metals by atomic absorption (AA)-Flame. Technically
acceptable laboratories received PE samples and 10 laboratories were
selected from the good performers. The IMVS should commence early
in FY87.

Status:

Status Report: IMVS on SW-846 Methods 3005,
3010, and 3050 - Trace Metals by AA-Flame

On Schedule
(9/87)

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Solid Waste Research Corranittee

Page 57 of 76
PE No. BSWT

A. OUTPUT: Evaluated Analytical Monitoring Methods	C. ORD Contact

for Waste Characterization	Name: J.J. Lichtenberq

FTS No. 684-7306	

B. RESOURCES: £1206.3 K FTE 7.0

FY 86 ANNUAL REPORT	Project No. 20

Purpose and Approach

The purpose of this project is to develop, evaluate, and validate extraction
and analysis procedures for the identification and measurement of hazardous
waste components including those not amenable to gas chromatographic tech-
niques. Appropriate analytes listed in 40 CFR, Appendix VIII, Appendix IX,
and the Michigan list will be studied to determine the applicability of gas
chromatography (GC), GC-mass spectrometry (MS) and liquid chromatography
(LC)-MS techniques to analysis of these compounds. Analytical methods
published in SW-846 "Test Methods for Evaluating Solid Wastes - Physical/
Chemical Methods" will be evaluated.

Progress and Accomplishments

A "Report on Evaluation of Metals Dissolution for Chromium", deliverable Item
No. 1696[A] was delivered to the Office of Solid Waste (OSW) on September 26,
thus concluding this phase of the project to improve hexavalent chromium
methodology.

Evaluation of SW-846 Methods 8320 and 8330 - The project was initiated this
quarter by Technology Applications, Incorporated (TAI), our in-house
contractor. Retention times and chromatographic conditions have been
established for revelant Appendix VIII analytes. Preliminary solubility and
extraction efficiency studies have been performed. Several solvent solubility
problems were identified.

Testing and Evaluation of OSW Methods 8010/8015/8020 and Single Laboratory
Validation of each Method - The draft final report has been received,
reviewed, and returned to Battelle for extensive revision. Most analytes
tested were considered to be within the scope of the method tested. However,
the study identified a few analytes for each method that produced poor
chromatography or purged very inefficiently. These are noted in the report.

Testing and Evaluation of SW-846 Method 8240 - The reorientation of this
effort toward capillary column chromatography has been underway. Testing both
in-house and at Battelle has confirmed the scope of the method for water and
solids. As a result, several additional analytes formerly assigned to solvent
extraction methods are now being tested for inclusion in the broadened scope
purge-trap-desorb (PTD) method. A status report in the form of comments on
the Appendix IX proposal were submitted to OSW in September.

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Page _2_ of Project No. 20	Page 58 of 76

Development of a Method for Formaldehyde to Replace SW-846 Methods 8410 and
8411 (Polarographic Procedures) for underground water and solid wastes - A
draft final report on cartridge extractors and single laboratory validation of
an high performance liquid chromatography (HPLC) method was submitted by
Battelle in September. It has been reviewed and returned for revision. The
cartridge extraction method showed promise but was subject to significant
variations between suppliers of the extractors. Work on this project is
continuing in an effort to resolve interference problems and reaction of
formaldehyde precursors which tend to form formaldehyde during the analysis.

Testing and Evaluation of SW-846 Method 8270 - The scope of 8270/3510 was
established by determining which of the 127 compounds found to be within the
scope of 8270 were extractable by the 3510 base-neutral/acid extraction
protocol. These results reported to 0SW for its use within the Appendix IX
comment period.

Evaluation of Clean-up Procedures for Organics Included in the SW-846 Methods
Manual - The contract intended to address this project was awarded to S-Cubed
in the last week of September. A mid-October meeting was held at the contrac-
tor site to finalize the workplan.

Development of a Heated PTD Method for Intractable Volatile SW-846 Analytes -
The Appendix VIII meeting participants (December 9-13, 1985) identified 13
intractable volatile analytes. Currently no method, other than direct aqueous
injection, exists for their analyses. A work assignment has been issued to
Battelle-Columbus Laboratories for them to investigate the possibility of
developing a heated PTD method for these analytes. The chromatographic work
has progressed well. The wide-bore polar columns (Carbowax-1ike) have
demonstrated excellent separations and peaks. A problem exists with the
instrument transfer lines. The polar materials such as acetone partition into
condensed vapors, requiring all lines to be heated above 100"C.

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Page 59 of 76

Solid Waste Research Committee

PE No. BSD1A

A. OUTPUT: Development of New Methods for Analysis

C. ORD Contact

of Solid Wastes

Name: W. L. Budde



FTS No. 684-7309

B. RESOURCES: $ 70.0 K FTE 0.0



FY 86 ANNUAL REPORT

Project No. 21

Purpose and Approach



The purpose of this project is to develop and evaluate liquid chromatography/
mass spectrometry (LC/MS) methods for nonvolatile non-gas chromatographable
compounds on Appendix VIII of the Resource Conservation and Recovery Act
(RCRA) regulations. Evaluation of a state-of-the-art thermospray interface
for LC/MS will be done under a cooperative agreement with Cornell University.

Progress and Accomplishments

Work continued at Cornell University during the year. A LC/MS system was
utilized to investigate methods for nonvolatile hazardous substances.

Emphasis continued to be placed on methods for carbamate, amide, urea, and
triazine pesticides that are not amenable to gas chromatography (GC) and for
which no generic methods exist. These compounds appear on the Appendix VIII
list of the RCRA regulations. A deliverable, Item 1678[A], "Report on
Evaluation of Thermo- spray for MS/MS" is scheduled for delivery in December
1986.

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APPROACH
Solid Waste - DU D109

Page 60 of 76
PE# T55&1A

OUTPUT Dioxin Method/QA
A.



C. ORD Contact
Name Harry Kolde
FTS No. "684-7325

Resources

B.	$(000) 100 PFT 0.0 OPFT	 PFTE	 OPFTE

Extramural Task:

Purpose:
Approach:

Accomplishments:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 22

Reference materials for chlorinated and brominated dibenzo-p-dioxins
and dibenzo-furans at ppt level.

Provide quality assurance support to dioxin monitoring committee.

As an extramural effort, prepare or purchase, and purify, as
necessary, dioxin and benzo-furan compounds. Prepare solutions of
known concentrations. Verify qualitatively and quantitatively and
distribute to DMP laboratories. Begin effort with the most toxic
compounds, i.e., the isomers of 2,3,7,8 dioxin and benzofuran. If
resources are available the brominated dioxin series and benzofurans
will be purchased.

The following chemicals were obtained in FY86: 50 mg each of tetra-
bromodibenzo-p-dioxin (BDD), penta-BDD, hexa-BDD and octa-BDD, 50 mg
of tetrachlorodibenzofuran (TCDF) and 5 mg of it as ^o^-labelled
TCDF. Delivery of hepta-BDD is awaited. All funds allocated for this
project through FY86 have been expended..

Status:

Report - Purchase of Reference Materials for the
Dioxin Monitoring Program

Completed
(12/85)

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Solid Waste
Research Committee

Page 61 of 76
PE No. BSTHTT

A. OUTPUT: Analytical Methods and Quality Assurance	C. ORD Contact

Guidance for Dioxin Monitoring	Name: W. L. Budde

FTS No. 684-7309

B. RESOURCES: $130.0 K	FTE 0.0

FY 86 ANNUAL REPORT	Project No. 23

Purpose and Approach

The purpose of this extramural project is to develop and evaluate analytical
procedures to identify and measure tetra-, penta-, hexa-, hepta-, and
chlorinated octachlorodibenzo dioxins (CDDs) and chlorinated dibenzofurans
(CDFs) in environmental samples. The project will be carried out under a
contract with Battelle-Columbus laboratories.

Progress and Accomplishments

An internal report, titled "Automated Procedures for Mass Spectrometric
Determination of Polychlorinated Dibenzo-p-dioxins and Polychlorinated
Dibenzofurans by Isomer Class", was delivered to the program office in
February, 1986. Under an interagency agreement with the Lawrence Livermore
Laboratory of the Department of Energy, excellent progress was made in the
effort to develop an immunochemical method for dioxins and furans. An enzyme
linked immunosorbent assay (ELISA) was developed using the antibodies
described in the last report. The assay proved to be highly reproducible and
sensitive. A presentation on this work was made at a seminar in Cincinnati on
August 7, 1986 and at the 6th International Symposium on Chlorinated Dioxins
and Related Compounds, September 16, 1986 in Fukuoka, Japan.

Another internal report on the "Development of Analytical Methods for Dioxins
and Furans" is scheduled for delivery in December, 1986.

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Page 2 of Project No. 23



Page 62 of 76

Solid Waste Research Committee

PE No. BSD1A

A. OUTPUT: Analytical Methods and Quality Assurance

C. ORD Contact

Guidance for Dioxin Monitoring

Name: W. L. Budde

FTS No. 684-7309

B. RESOURCES: $130.0 K PFTE 0.0



FY 86 ANNUAL REPORT

Project No. 23

Purpose and Approach



The purpose is to provide standard approaches for sampling and analysis of
2,3,7,8-Tetrachlorodibenzo-p-dioxin (TCDD) and other chlorinated
dibenzo-p-dioxins and chlorinated dibenzofurans (CDFs) in environmental
samples and to provide quality assurance procedures which document the
precision and accuracy. Emphasis will be placed on procedures to identify and
measure tetra-, penta-, hexa-, hepta-, and octachlorodibenzo dioxins (CDDs)
and CDFs. Existing procedures will be reviewed and evaluated and standard
methods for sampling and measurement will be prepared.

Accomplishments and Results to Date

Full scan mass spectra were acquired for 20 CDD and CDF congeners. A computer
data library was built and verified for correctness. Initial testing of an
automated identification procedure was begun. Efforts are being made to
acquire additional standards through an exchange with another agency that has
an intensive systhesis program underway.

Identification and Measurement of tetra-, penta-, hepta, and octachlorodi-
benzodioxins and dibenzofurans in environmental samples - The work assignment
was completed on schedule and a draft journal article titled "Automated
Procedures for Mass Spectrometry Determination of Polychlorinated
Dibenzo-p-dioxins and Polychlorinated Dibenzofurans by Isomer Class" was
delivered. This document will be reviewed and modified for a scheduled FY 87
deliverable. Software to support this method through automated raw data
interpretation and computations was also delivered. During FY 87 both the
method and the software will be extensively tested, debugged, and documented.

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Page 63 of 76

Superfund - Hazardous Emergency Response	PE No. F6Y1A

Committee

A. OUTPUT: Monitoring Methods and QA Support for	C. ORD Contact

Situation Assessment	Name: J.J. Lichtenberg

FTS No. 664-7306	

B. RESOURCES: % 0.0 K	FTE 2.5

FY 86 ANNUAL REPORT	Project No. 24

Purpose and Approach

The purpose of this work is to provide guidance on sampling and analysis
procedures, instrumentation and quality assurance that will allow decision
makers to establish priorities between sites and provide scientific basis for
decisions. The latest techniques and instrumentation will be applied to
provide accurate information. An electronic data transfer system will be
developed to collect and manage analytical data generated by the Superfund
program.

Progress and Accomplishments

A report titled "The Need for Automated Data Handling in Environmental
Monitoring" was delivered to the program office early in FY 86.

In-house work was devoted to the support of the contract laboratory program
(CLP) multilaboratory test of Method 680 for "Determination of Pesticides and
PCBs in Water and Soil/Sediment by Gas Chromatography/Mass Spectrometry" which
was revised after receiving comments from program offices, laboratory
directors, and regional division directors. The method is supported by
specialized software which automates the interpretation of the raw data and
completes the calculations required for the polychlorinated biphenyl (PCB)
level of chlorination approach. A document titled "Users' Guide for Software
for Automated Identification and Measurement of Pesticides and Polychlorinated
Biphenyls" and copies of the software prepared for this purpose, have been
sent to many laboratories interested in field testing the method.

Data from a six-laboratory collaborative study of the method were extensively
analyzed and an oral report on the study was made at the CLP program meeting
in August. Further information on the method and study was presented at the
CLP October 1986 meeting.

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APPROACH
Superfund - DU Y105

Page 64 of 76
PE# IHT71A

OUTPUT Monitoring and QA Support for Situation Assessment.
A.

C. ORD Contact
Name Ed Berq
FTS No. 684-7325

Resources

B.	R/D $(000) 56 PFT 0.2 OPFT	 PFTE	 OPFTE

FY84 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 25

Extramural Task: Performance Evaluation (PE) of Superfund Contractors.

Purpose:	Quality assurance (QA) support is needed for USEPA and USEPA

contractor laboratories for Superfund. Some measure of performance
is needed to monitor the quality of data generated by Comprehensive
Environmental Response Compensation and Liability Act (CERCLA)
laboratories.

Approach:	Natural wastewater samples are prepared, verified as to concen-

tration, and distributed in quarterly evaluations of Superfund
contract laboratories, in cooperation with EMSL-Las Vegas.

Accomplishments: Full-volume natural wastewater samples spiked with approximately 20
compounds were prepared and shipped to approximately 60 Superfund
contract laboratories, and to USEPA Regional laboratories once each
quarter. Concentration levels were designed for gas chromatograph/
mass spectrometer (GC/MS) capillary analyses and included volatiles
and semi-volatiles. Verification analyses were conducted on the
full-volume samples and data submitted to EMSL-Las Vegas. In the
first, second, and third quarters, samples were sent to Regions 1, 6
and 7 for distribution to Contract Laboratory Program (CLP)
laboratories. During the fourth quarter, the samples were sent
directly to prospective CLP laboratories as preaward PE samples.

Status:

Annual Report on PE of Superfund
Contractors

Completed
(12/85)

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Page 2 of Project No. 25

APPROACH
Superfund - DU Y105

Page
PE#

65 of 76
ESV1A

OUTPUT Monitoring and QA Support for Situation Assessment.
A.

C. ORD Contact
Name Ed Berg
FTS No. 684-

-7325

Resources

B. $(000) 126 PFT 0.1 OPFT

PFTE OPFTE





FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 25

Extramural Task: Maintain USEPA's Quality Control (QC) Sample Program for
Water-related Analytes.

QC samples are provided to USEPA, regional, state, and USEPA
contractors as a check on the analyst technique and analytical
methodology. Such checks are necessary to monitor the quality of
data being generated in carrying out mandates of the Resource
Conservation and Recovery Act (RCRA).

Bionetics, Inc., the technical service contractor, provides
personnel to develop, produce, and distribute QC samples.

Development of new sample types requires obtaining chemicals of the
highest purity such as those from the USEPA Repository for Toxic and
Hazardous Materials, selecting the methodology for the compounds of
interest, conducting retention time studies, and finally combining
groups of organic compounds to minimize overlapping gas
chromatography peaks and conducting 0, 45-, and 90-day stability
studies. Those compounds proven stable are produced at one
concentration level in lots of 5,000. Random samples are withdrawn
during production and sent to USEPA referee laboratories for
verification analyses. Upon verification, the new sample is
advertised in the USEPA Quality Assurance (QA) Newsletter and
distributed to requesters.

Accomplishments: 1. A total of 285,167 QC samples were distributed to USEPA,

regional, state, local, and USEPA contractor laboratories.

2. A total of 181,000 ampuls were produced to replenish depleted
inventories and included such QC series as trace metals,
cyanide, polychlorinated biphenyls (PCBs) in oil, PCBs in
acetone, pesticides, and seven volatile organic series.

5. Of the 618 analytes listed in Appendix A, 135 are available for
distribution.

Purpose:

Approach:

Status:

Annual Report of QC Sample Program

Completed
(12/85)

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Page 3 of Project No. 25

APPROACH
Superfund - DU Y105

Page 66 of 76
PE# ESYlA

OUTPUT Monitoring and QA Support for Situation Assessment.
A.

C. ORD Contact
Name Harry Kolde
FTS No. 684-7325

Resources

B. R/O $(000) 106 PFT 0.1 OPFT

PFTE OPFTE



FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 25

Extramural Task: Develop and maintain USEPA's Repository for Toxic and Hazardous
Materials.

Purpose:	Maintain the USEPA Repository for Toxic and Hazardous Materials to

provide spiking/calibration solutions of organic compounds in
support of monitoring under Comprehensive Environmental Response
Compensation and Liability Act (CERCLA) regulations.

Approach:	Compounds of interest to Superfund (SF) are purchased or

synthesized, purified, dissolved in the appropriate solvent, and
dispensed in 2 mL ampuls. The purity of pure compounds and
concentrations in the ampuls are verified by referee laboratories.
Upon verification, spiking/calibration solutions are announced in
the Quality Assurance Newsletter and distributed to USEPA, SF
contractor, state, and local laboratories engaged in SF monitoring
the environment.

Accomplishments: Approximately 608 compounds are specified in the Appendix A List.

The Repository contains 480 of these as neat materials in stock; 228
of the neat materials have been certified for purity and 156
certified analytes available for distribution; and nine new
chemicals are currently being tested by referee laboratories.

Status:

Annual Report of Repository Activities

Completed
(12/85)

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Page 4 of Project No. 25

APPROACH
Superfund - DU Y105

Page 67 of 76
PE# EG71A



C. ORD Contact

OUTPUT Monitoring and QA Support for Situation Assessment

Name John Winter

A.

FTS No. 684-7325

B. R/D $ OK $(000) 0 PFT 0 OPFT	 PFTE 	 OPFTE

Inhouse Task:
Purpose:

Approach:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 25

Externalization of Quality Assurance (QA) Programs.

Recover costs of production, distribution, and administration of
quality control (QC) and performance evaluation (PE) sample programs
associated with the drinking water, industrial waste, and water
quality program.

Promulgate a cost recovery rule for the preparation and distribution
of QC and PE samples, set up a mechanism for collecting such fees
through the USEPA Financial Management Office, and begin the
externalization process for these sample types.

Accomplishments: An externalization task force was formed of USEPA personnel from the
Comptroller's Office; Office of General Counsel; Office of Program
Management; Office of Acid Deposition, Environmental Monitoring and
Quality Assurance (OADEMQA); operating program offices; the regional
offices; and the three EMSL laboratories to study and recommend the
best option for externalization of QA support services. Concur-
rently, EMSL-Cincinnati prepared a white paper on costs, for
consideration by the Task Group. Discussions were also held between
the Contracts Management Division and EMSL-Cincinnati to explore the
best means to charge and collect user fees for these services and to
expedite return of funds to EMSL-Cincinnati for maintenance of the
QA program.

Based on these deliberations and discussions, OADEMQA prepared a
draft of a proposed rule: Proposed User Charges for Certain Quality
Control and Performance Evaluation Samples Under the Clean Water Act
and the Safe Drinking Water Act which was subsequently published in
the Federal Register on September 16, 1986. Comments are due by
October 31, 1986.

Status:	Report on the Externalization OA Proqram	Completed

(5/86)

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Page 5 of Project No. 25

APPROACH
Superfund - DU Y105

Page 68
PE# rGY

of 76
1A

OUTPUT Quality Assurance
A.

C. ORD Contact
Name Ed Bi
FTS No.

Resources

B. R/D $ OK $(000)

PFT

OPFT

PFTE

OPFTE

Inhouse Task:

Purpose:

Approach:

Accomplishments:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 25

Performance Evaluation (PE) Samples for the Ground Water Monitoring
Program.

Evaluate the performance of laboratories providing analyses of
ground water samples collected at selected hazardous waste sites.

A set of organic and inorganic PE samples are prepared by Bionetics,
Inc. and sent to the field sample collection team at the hazardous
waste site. The PE samples are integrated into the samples
collected at the site and then sent to laboratories under contract
to USEPA. The analytical results scored based upon past PE studies,
interlaboratory method studies, and other sources.

Separate PE samples were prepared for 15 sites and sent to two
groups of contract laboratories. The results were then used to help
assess the quality of data being generated by the contract
laboratory for each site. A panel of personnel from EMSL-Las Vegas,
EMSL-Cincinnati and the Office of Solid Waste (Headquarters), ICAIR
Life Systems, and the regional offices reviewed the results of the
quality assurance work and agreed in a concensus evaluation for each
site, through telephone conference calls.

Status:

Status Report on PE Samples for the Ground
Water Monitoring Laboratories

On Schedule
(12/86)

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Paqe 69 of 76

APPROACH

PE# E6Y1A

Superfund - DU Y105





C. ORD Contact

OUTPUT Provide Technical Support to Enforcement Program

Name Harold Clements

A.

FTS No. 684-7325

PpcnurrPQ

B.	$(000) 7 PFT 0.1 OPFT	 PFTE	 OPFTE

Inhouse Task:
Purpose:

Approach:

Accomplishments:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 26

Conduct Performance Evaluation Studies for Remedial Programs

Evaluate performance of Hyde Park litigant laboratories in the
Comprehensive Environmental Response Compensation and Liability Act
(CERCLA) Program.

Develop a series of samples which are stable and homogeneous and
capable for use as unknown samples to conduct studies and evaluate
results.

The Quality Assurance (QA) Branch prepared and distributed samples
to Hooker Chemical Company, Niagara Falls, New York in support of
the Hyde Park agreement. Twenty-one target compounds were spiked
into an organic solvent for gas chromatograph/mass spectrometer
(GC/MS) analyses. Series VII and Series VIII were sent December
1985 and July 1986, respectively, to Hooker Chemical Company for
analyses. The data were evaluated on return to the QA Branch and
reported to the USEPA Hyde Park Litigation Program Coordinator in
Region 2. Laboratory performance in these two studies was
acceptable. The next study sample will be sent in December 1986.

Status:

Report of Technical Support to Region 2,
Evaluation of Performance in Enforcement Action

Completed
(12/85)

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1

1 APPROACH
I Manage Agency Mandatory Quality Assurance Program -

DU

Page 70 or 76 1
PE# 1
H109 1

I Technical Information and Management Support to
1 A. OUTPUT: Quality Assurance Management Staff (QAMS).
I Communication between QAMS and EMSL-Cincinnati as
1 well as between QAMS and the Regional, Headquarters
1 and National Laboratory Quality Assurance Officers.

C.

UKD Contact 1
NAME: Daniel F. Bender I
FTS No. 684-7301 I

1
1

1 RESOURCES:

1 B. $(000) 49.8 PFT 0.9 OPFT PFTE

1

OPFTE t

1



1

ANNUAL REPORT - FY86	PROJECT NUMBER 27

Purpose and Approach

This project is an on-going function involving the supplying of technical and policy
information and technical services such as document review, committee and work group
membership, document and report preparation, and the coordination of the input into
these activities of regional, headquarters, and national laboratory Quality Assurance
Officers (QAOs).

Accomplishments and Results to Date

1.	Routinely-Used Measurement Method (RUMM) Work Group (WG): The RUMM compendium
document was prepared for review by U.S. Environmental Protection Agency (USEPA)
and state users. EMSL-Cincinnati's review was obtained. The contractor, Re-
search Triangle Institute, the WG Chairman, and myself, reviewed the final changes
with each individual EMSL-Cincinnati reviewer. EMSL-Cincinnati concurrence as to
technical accuracy was obtained. After a teleconference with the Environmental
Services Division (ESD) Directors, the compendium was reviewed by USEPA users and
some state laboratories; a summary of comments was prepared. Several teleconfer-
ences concerning the next phase of the RUMM project were held. USEPA Project
Summaries for all of the EMSL-Cincinnati Method Validation Studies were gathered
and transmitted to the WG Chairman for use in the next phase.

2.	Audits: Prepared the "Follow-up Audit" section for the Office of Research and
Development (ORD) Management Systems Audit (MSA) Protocol.

3.	QAO Meetings: The annual FY 86 Fall QAO meeting was attended. The annual ORD
QAO meeting was hosted by EMSL-Cincinnati. A newly organized series of bimonthly
Regional QAO conference call meetings was initiated. The quarterly Andrew W.
Breidenbach Environmental Research Center QAO meetings were held and the minutes
were reported to Quality Assurance Management Staff (QAMS). The planning for the
FY 87 Fall QAO meeting was initiated.

4.	QA Document Preparation and Review: Assisted in the preparation of the EMSL-
Cinclnnati Quality Assurance Program Plan (QAPP) (Parts 1 and 3) through several
revisions. Reviewed the Office of Acid Deposition, Environmental Monitoring, and
Quality Assurance (OADEMQA) QAPP through several revisions. Reviewed the Quality
Assurance/Quality Control (QA/QC) Estuary Methods Manual for the Office of Marine
and Estuary Protection. Prepared the 304(h) statement for residual chlorine.
Reviewed the Quality Assurance Project Plan (QAPjP) for Underground Injection
Control in Region 9.

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Page 2 of Project No. 27

Page 71 of

5. Other Assignments: Participated in a National Association of Science Program
Review of EMSL-Cincinnati QA activities. Reviewed an International Union of Pure
and Applied Chemistry (IUPAC) document on sampling nomenclature. Worked on
Standard Methods, 17th Edition Joint Task Groups (JTGs) on Residual Chlorine,

Chlorine Dioxide, and Ozone. Participated, as a lecturer, in a laboratory short
course at the University of Florida Training Research and Education for Environmental
Occupations (TREEO) Center sponsored by the Florida Society of Environmental Analysts.
Successfully completed the Chemical Laboratory Drinking Water Certification Course
and the Contract Officer 40-Hour Certification course.

Status:

1.	RUMM WG: Method 624 is being prepared by the contractor for inclusion in RUMM.
The Sampling Subgroup is preparing a strawman project summary outline based on
a number of Standard Operating Procedures and sampling manuals obtained from
Superfund, EMSL-Cincinnati, Region 4, and the Office of Solid Waste.

2.	Audit: Several audits are being finalized; more active participation in future
audits by the EMSL-Cincinnati Liaison is planned.

3.	QAO Meeting: Participation in the Fall FY 87 national QAO meeting is planned.

Input to the planned ORD QAO meeting and the Regional QAO meeting will be
forthcoming.

4.	QA Document Preparation and Review: EMSL-Cincinnati Liaison participation in a
variety of QA and method development activities is expected.

5.	Other Assignments: Participation in the Standard Methods JTGs will continue.
Participation in two other JTGs was recommended by the EMSL-Cincinnati Director
at the last Joint Editorial Board Meeting: Reagent Water and Safety. Partici-
pation in the laboratory short course at the TREEO Center is anticipated.

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Acid Deposition Research Program Office

Page 72 of 76
PE No. CVNTTT

A. OUTPUT: Wet Deposition Monitoring Methods	C. ORD Contact

Name: J.J. Lichtenberq
FTS No. 684-7306

B. RESOURCES: $100.0 K	FTE 0.0

FY 86 ANNUAL REPORT	Project No. 28

Purpose and Approach

The purpose is to provide improved methods for collection and analysis of Wet
Precipitation Samples. The approach will be to develop and evaluate analyti-
cal methods for inorganic ions and other parameters in atmospheric deposition
samples under a cooperative agreement with the State of Illinois.

Progress and Accomplishments

A methods manual which includes methods for pH, Ca, Mg, K, Na, NH3, CI,
NO3, PO4, SO4, F, and specific conductance has been published and a
report on "Standard Methods for Collection and Analysis of Precipitation" was
delivered to the program office in April 1986.

A new cooperative agreement was awarded to the Illinois State Water Survey to
evaluate methods for reactive aluminum. The project is scheduled to begin
early in FY 87.

Development and Evaluation of Methods for the Analysis of Ions in Atmospheric
Deposition—A draft method, "Dissolved Aluminum, Cadmium, Copper, Iron, Lead,
Manganese and Zinc in Wet Deposition by Graphite Furnace Atomic Absorption
Spectrophotometry", has been received from the contractor. This draft method
was reviewed and returned to the authors for revision.

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APPROACH
Chemical Assessment - DU L104

^ge 73 of 2£L
PE# CRL1A

OUTPUT Quality Assurance for Toxic Substances
A.

C. ORD Contact
Name John Winter
FTS No. 684-7325

Resources

B. R/D $20K $(000) 20 PFT 0 OPFT	 PFTE 	 OPFTE

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 29

Extramural Task: Establish Traceability of Quality Control (QC) and Performance

Evaluation (PE) Samples to the National Bureau of Standards (NBS).

Purpose:	The QC and PE samples utilized throughout the United States and

internationally in water related monitoring programs must be of the
high quality since they are involved in important decisions. As
part of a stringent quality assurance program to assure the veracity
of representative QC and PE samples, traceability to the NBS is
established.

Approach:	An interagency agreement (IAG) was signed with NBS to develop a

protocol for traceability of QC and PE analytes, and then to
implement the protocol for top priority samples of interest to the
Agency and those for which NBS has expert analytical capabilities.

Accomplishments: NBS verified, thereby establishing traceability for the pesticides

lindane, endrin and methoxychlor, two herbicides (2,4-D and Silvex),
and 14 volatile organic contaminants (trans and cis 1,2-dichloro-
ethylene, dibromochloropropane, o-dichlorobenzene, ethylbenzene,
chlorobenzene, sytrene, toluene, xylene, ethylene dibromide,
chloroform, bromodi- chloromethane, dibromochloromethane and
bromoform). Seven sludges which are to be used in an interlabora-
tory method validation study are currently being analyzed.

Status:

Annual Report on Traceability to NBS

Completed
(12/85)

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Page 2 of Project No. 29

" Page 74 of 76
APPROACH	PE# "CRU1A

	Chemical Assessment - DU L104	 	

C. ORD Contact

OUTPUT Quality Assurance for Toxic Substances	Name Harry Kolde

A.	FTS No. 684-7325

Resources

B. R/D $60.4 $(000) 60.4 PFT 0 OPFT 	 PFTE 	 OPFTE

Extramural Task:

Purpose:

Approach:

Accomplishments:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 29

Conduct Verification Analyses on performance evaluation/quality
control (PE/QC) Samples.

Usage of QC, PE, and spiking/calibration samples in the Toxics
program to assess the quality of monitoring data necessitates that
true or reference values associated with the samples are in fact,
valid. Otherwise poor decisions could result which would adversely
impact the environment. Therefore, referee laboratories are used to
establish the veracity of samples.

Referee laboratories are selected through the competitive
procurement process upon the basis of performance evaluation and
cost for the analytes of interest. These analytes include trace
metals, polychlorinated biphenyls (PCBs) in oil, synthetic organic
contaminants specified in Toxics regulations, and for other analytes
regulated by the Agency.

Referee laboratories conducted 74 analyses to confirm the veracity
of PCB calibration standards.

Status:

Annual Report on Referee Analytical Services

Completed
(12/85)

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Page 3 of Project No. 29

Page 75 of 76
APPROACH	PE# URTlA

	Chemical Assessment - DU L104			

C. ORD Contact

OUTPUT Quality Assurance for Toxic Substances	Name Ray Wesselman

A	.	FTS No. 684-7325

Resources

B.	R/D $35 $(000) 35 PFT 0 OPFT	 PFTE 	 OPFTE 	

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 29

Extramural Task: Prepare, Analyze, and Distribute Quality Control (QC) Samples.

Purpose:	QC Samples are provided to USEPA, USEPA contractor, state, and local

laboratories as a check on the analyst's technique and analytical
methodology. Such checks monitor the quality of data being
generated by laboratories conducting analyses under the Toxic
Substances Control Act (TSCA).

Approach:	Bionetics, Inc., the technical service contractor, develops,

produces, and distributes QC samples. Development of new sample
types requires obtaining chemicals of the highest purity from the
best sources including the USEPA Repository for Toxic and Hazardous
Materials, selecting the methodology for the compounds of interest
to TSCA, conducting retention time studies, and combining groups of
organic compounds to minimize overlapping gas chromatography peaks
and conducting 0, 45-, and 90-day stability studies. Those
compounds proved stable are produced at one concentration level in
lots of 5,000. Random samples are withdrawn during production and
sent to USEPA referee laboratories for verification analyses. Upon
verification, the new sample is advertised in the USEPA Quality
Assurance Newsletter and distributed to requesters.

Accomplishments: • A total of 285,167 QC samples for all analytes were distributed

to USEPA, state, local, and commercial laboratories engaged in
water/wastewater monitoring.

Produced the following sample series to replace depleted
stocks: polychlorinated biphenyls (PCBs) 1254, 1248, 1260,
1016, and 1242 in acetone and in oils.

A total of 181,000 ampuls were produced to replenish depleted
inventories and included such QC series as trace metals,
cyanide, PCBs in oil and acetone, pesticides, and seven volatile
organic series.

Participated in interlaboratory method study for PCBs
monstration program for PCB distruction. The set consisted of
PCB congeners (mono, di, tri, and tetra biphenyls) and Aroclors
1242, 1254, and 1260. Fifty sets of each were supplied to the
Office of Toxic Substances (OTS).

Status:

Annual Report on QC Sample Program

Completed
(12/85)

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Page 4 of Project No. 29

Page 76 of 76
APPROACH	PE# flRTlA

Chemical Assessment - DU L104

C. ORD Contact

OUTPUT Quality Assurance for Toxic Substances	Name Harry Kolde

A.	FTS No. 664-7325

Resources

B. R/D $31.2 $(000) 31.2 PFT 0 OPFT	 PFTE 	 OPFTE

Extramural Task:

Purpose:

Approach:

FY86 ANNUAL REPORT
Quality Assurance Branch, EMSL-Cincinnati

Project No.: 29

Develop and maintain USEPA's Repository for Toxic and Hazardous
Materials.

The USEPA Repository for Toxic and Hazardous Materials provides
spiking/calibration solutions of organic compounds in support of
regulations under the Toxic Substances Control Act (TSCA).

Compounds of interest to the Office of Toxic Substances (OTS) are
purchased or synthesized, purified, dissolved in the appropriate
solvent, and finally dispensed in 1.5 mL ampuls. The verity of pure
compounds and concentration of the compound in the ampul are verified
by referee laboratories. Upon verification, spiking/calibration
solutions are advertised in the Quality Assurance Newsletter and
distributed to USEPA, USEPA contractor, state, and local
laboratories engaged in monitoring the environment.

Accomplishments: 1.

2.

3.

A total of 75,200 certified calibration standards were
distributed to 1930 USEPA, USEPA contractor, state, and local
laboratories. This represents a 45% increase over FY85.

Twenty different individual polychlorinated biphenyl (PCB)
standards in methanol or isooctane solutions are now available.

Sixty-five of the special PCB calibration standards containing
the mono-, tetra-, octa-, and deca-chlorobiphenyl isomers were
distributed to OTS contractors.

Status:

Annual Report on Repository

Completed
(12/85)

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