United Stoics
Environmental Pioieclion
Agency
METHANE EMISSIONS 1-TtOM TITH

NATURAL- GAS INDUSTRY

Volume 13:  Chemical Injection Tump?
GRI-94 / G?77 3t
EPA 600/R 9
June 1990

Energy Information Administration (U.S. DOE)
 National Risk Management
 Research Laboratory
 Research Triangle Park, NC 27711
                              fstflt*
                Na'.onal Te-Chnica! Inf

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                                     YECHNtCAi. HOH5HT DAiA
                                             **-***-"*'"*" !**•'«*•-!       IHSjiltilBHStr  tailt  *£t&3lR'i
                               'cinert'*iit fB'tiiicftims, itM»:-ii  \-}n,  v !»i   .i   .!-.{•  joji  7}.

    ; = irt-,in  a! lh«- » u "ior.iti *•-  r-.i-i-r   I ht  n «
    ^ici'i  VAC! ii" -t-   0. 5"r, -•! n-»tur.-,l f-   > . i <«.i
  !-• tit-o' t) oM»t i-' iy9°  Beoulln ftvi..  Wit-  pi •<» i -tit   '<  r Lird ti  < '1,1
  .- r.i ,is^i<.«p-  trom the fuel cjclc fo*  n^tnr?«l p, -  «nl.  n.t c .vi u^itii. lh«  ..In1 .1
  in,3 pott ifuil.s (tJVi Ps) rc«.enll\ pul liolad I ^ llu Inu i 4"i i rhm<>pta'  f-' » ci tu  LUJU--
  hr.nge (ll'f'C'). Ihu anftly^ij  sliowo>i  thai naiui ol K^L  <'ori''<-  U •-   i<, poi,  i   '
global  warming than to.il or oil, wlm-ii supports flit  tut i o> itciauf   >.i ntv.t'\ ^.uL't1'---  - >
by  tlielPC'C'  and other*. In addition,  shn'\ rcbulf.^- ate 1» HIC  u ,i >1 \>\  tli,  n^tm -1  n   -
inilu&try to ruduee  opt rating costa whilr j r>ducm,r riinsoioiiu .
                                  K.F Y WORDS AND OOCUMLN1
                   DESCRIPTORS
Pollution
Emission
Greenhouse Effect
Natural Gas
Gas Pipelines
Methane
 Release to Public
U.IDtNriFtcns/OPCN ! ftinpoTgRMj; |c. r.n.sAH ridd/iiiouy
 U'lcJar-sified
20 !»tl,t!K!I > CLAii, (1 /',.-., _•'
                             (HA
                             2ilJ
                             I5K
                             ovc
                                                                                 NO, or P
                                                                                    •12
EPA Porra 2720-1 (9-13)

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                                FOREWORD
    The U.S. Environmental Protection Agency is charged by Congress with pro-
    tecting the Nation's land, air, and water resources. Under a mandate of national
    environmental laws, the Agency strives to formulate and implement actions lead-
    ing to a compatible balance between human activities and the ability of natural
    systems to support and nurture life.   To meet this mandate, EPA's research
    program is providing data and technical support for solving environmental pro-
    blems today and building a science knowledge base necessary to manage our eco-
    logical resources wisely, understand how pollutants affect our health, and pre-
    vent or reduce environmental risks in the future.

    The National Risk Management Research Laboratory is the Agency's center for
    investigation of technological and management approaches for reducing  risks
    from threats to human health and the  environment. The focus of the Laboratory's
    research program is on methods for the prevention and control of pollution  to air,
    land, water, and subsurface resources; protection of water quality in public water
    systems; remediation of contaminated      and groundwater; and prevention and
    control of indoor air pollution.  The goal of thL; research effort is to catalyze
    development and implementation of innovative* cost-effective environmental
    technologies; develop scientific                 information needed by EPA to
    support regulatory and policy decisions; and provide technical support    infor-
    mation transfer to ensure effective implementation of environmental regulations
        strategies.

    This publication Jias been produced as part of the  Laboratory's strategic long-
    term research plan. It is published     made available by BPA's Office of Re-
    search and Development to assist the user community and to link researchers
    with their clients,


                               E. Timothy Oppelt,  Director
                               National Risk Management Research Laboratory
                               EPA

         This     has     peer and administratively reviewed by the U.S. Environmental
         Protection Agency, and approved for publication. Mention of            or
                  products does not         endorsement or recommendation for use,

         This document is        to the            the National Technical-Information
         Service, Springfield, Virginia 22161,
                          COPYRIGHT
ALL
NATIONAL TECHNICAL
U.S. DEPARTMENT OF COMMERCE

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                                     JEPA-600/R-96-080m
                                     June 1996
        METHANE EMISSIONS FROM
       THE NATURAL GAS INDUSTRY,
 VOLUME 13: CHEMICAL INJECTION PUMPS
              FINAL REPORT
                Prepared by:

              Theresa M. Shires

           Radian International LLC
            8501 N.  Mopac Blvd.
              P.O. Box 201088
           Austin, TX  78720-1088


            DCN: 95-263-081-08


                    For

      GRI Project Manager: Robert A. Lott
         GAS RESEARC:T INSTITUTE
          Contract No. 50.1-251-2171
          8600 West Bryn Mawr Ave.
             Chicago, IL 60631

                    and

  EPA T  oject Manager: David A. Kirchgessner
U.S. ENVIRONMENTAL PROTECTION AGENCY
           Contract No. 68-D1-0031
  National Risk Management Research Laboratory
       Research Triangle Park, NC 27711

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                                   DISCLAIMER

LEGAL NOTICE:  This report was prepared by Radian International  I i.(.' as mi are.ouni
oi work sponsored by tins Research Institute  (OR1) and the U.S. Environmental  Protection
Agency (EPA).  Neither EPA, Gill, members of Gill, nor any person iKfmu on behalf of
either:

a.            Makes any warranty or representation,  express or implied, with respect to the
              accuracy, completeness,  or usefulness of the information contained in this
              report, or that the use of any apparatus, method, or process disclosed in this
              report may not  infringe privately owned rights;  or

b.            Assumes any liability with respect  to the use of, or for damages resulting
              from the use of, any information, apparatus, method, or process disclosed in
              this report.

NOTE:  EPA's  Office of Research and Development quality assurance/".quality control
(QA/QC) requirements are applicable to sonic of the  count data generated by this project.
Emission data and additional count data are from industry or literature sources, and are not
subject to EPA/ORD's QA/QC policies. In all cases, data and results were  reviewed  by the
panel of experts listed in  Appendix D of Volume 2.

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Title
Contractor
Principal
Investigator

Report Period


Objective
Technical
Perspective
Results
Methane                {lie Natural Gas Industry,
Volume  13: Chemical Injection Pumps
Final Report

                    LLC

GRI Contract Number 5091-251-2171
EPA Contract Number 68-DI-OQ31

Theresa M.  Shires
March 1991 - June  1996
Final Report

This report          a       to quantify the annual methane
from       gas-driven          injection pumps,

The          use of        gas has been           as a        for
         the          for        warming.   During
gas          less              (CO2) per    of        produced than
either coal or oil. On the       of the amount of CO2 emitted, the
         for        warming could be reduced by                    gas
for coal or oil. However,  since natural     is primarily methane, a potent
                     of        gas       production, processing,
transmission,  and distribution could reduce  the                   of its
lower CO2 emissions.

To investigate this,  Gas  Research Institute  (GRI) and the U.S. Environ-
mental Protection Agency's Office of Research and Development (EPA/-
ORD) cofunded a major study to quantify methane emissions  from U.S.
natural gas operations for the 1992 base year. The results of this study
can be used to construct global methane budgets and  to determine the
relative impact on global warming of natural gas versus coal and oil,

The 1992 national                   for chemical injection pumps used
in the production          are 1.5 ± 203%  Bscf,

      on          the                                        natural
gas           are          to be 314 ± 105 Bsef for the 1992
year.   This is about 1.4 ± 0,5%  of gross natural gas production.  The
overall program             the           of                 for an
                                          in

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                              increase in        gas      would be significantly
                  than the

                  The program reached its accuracy goal and provides an accurate
                  of methane emissions that can be used to construct  U.S.
                  inventories     analyze fuel switching strategies.

 Technical         The gas industry has two primary types of chemical  injection pumps that
 Approach         discharge natural gas: piston pumps and diaphragm  pumps.  Gas-driven
                  pumps      for glycol circulation are presented in a separate study,

                  An emission rate for chemical injection pumps was determined by
                  developing an annual emission factor for typical practices and
                  extrapolating this value based on the total  number of chemical injection
                  pumps (activity factor) to develop a national estimate, where the national
                  emission rate is the product of the emission factor and activity factor.

                  Chemical injection pumps  are small positive displacement, reciprocating
                  units designed to inject  precise amounts of chemicals into
                           These pumps are      in the production segment to control
                             problems or protect equiprr^nt.   Typical  chemicals injected in
                  an oil or gas field are biocides, demulsifiers, elarifiers, corrosion
                  inhibitors,  scale Inhibitors, hydrate inhibitors,  dewaxers, surfactants,
                  scavengers.

                  The  emission-affecting characteristics of chemical injection pumps
                  include: frequency of operation, unit size, supply gas pressure, and inlet
                  methane composition.  The frequency of operation  was       on timed
                  stroke rates and operator information on the annual  use of the devices.
                  Manufacturer data provided the gas consumption rates per stroke.  An
                  equation relating these parameters wan developed and used to ca''.-ulate
                  annual methane emissions  from a typical chemical  injection  pump used
                  in natural as production.

                  The activity factor development (i.e., the number of chemical injection
                  pumps nationally) is presented in a separate report.  In general though,
                  the activity factor is based on the number of chemical injection pumps
                  per active gas well that markets gas. The national methane emission rate
                  for chemical injection pumps      then       on the product of the
                  emission factor and activity factor.

Project            For the  1992 base year, the                emissions         for the
                  U.S.        gas industry is 314     ± 105      (± 33%). This is
                  equivalent  to 1.4% ± 0.5% of gross        gas production,          from
                  this program           to  compare            gas           from the
                                           IV

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fuel cycle for natural gas, oil, and coal  using the global wanning
potentials (GWPs) recently published by the Intergovernmental Panel on
Climate Change (IPCC).  The analysis showed thai natural gas
contributes less to potential  global warming than coa! or oil, which
supports the fuel  switching strategy suggested by IPCC and others.

In addition, results from this study are being used by the natural gas
industry to reduce operating costs while reducing emissions.  Some
companies are also participating in the Natural Gas-Star program,  a
voluntary program sponsored by EPA's Office of Air and Radiation  in
cooperation with  the American Gas Association to implement cost-
effective emission reductions and to  report reductions to EPA.  Since this
program was begun after the 1992 baseline  year, any reductions in
methane emissions from this program are not reflected in this study's
total emissions.
Robert A. Lott
Senior Project Manager, Environment and Safety

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                           TABLE OF CONTENTS

                                                                        Page

 1.0   SUMMARY  	1

 2.0   INTRODUCTION  	2

 3.0   GAS-DRIVEN PUMP TYPES  	3

      3,1    Operation Overview	3
      3,2    Emission-Affecting Characteristics	 11

 4,0   EMISSION FACTOR DATA	 12

      4.1    Canadian Petroleum Association (CPA) Report	,	 12
      4.2    Methane Composition   	 12
      4.3    Site Data  	13
      4.4    Industry Boundaries	 16
      4.5    Manufacturers' Data	 18
            4.5.1  Diaphragm Pumps  	 18
            4.5.2 Piston Pumps	,	21

 5.0   EMISSION  RATE CALCULATIONS  	23

      5.1    Diaphragm Pumps	23
      5.2    Piston Pumps 	24
      5.3    National Emission Rate  	25

6.0   REFERENCES  .....	.26


      APPENDIX A - Production Source Sheet	 A-l

      APPENDIX B - Conversion Table	 B-l
                                     VI

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                                  OF

                                                                       Page

3-1   Piston Pump Schematic  	, .... 5

3-2   Piston Pump Cut-away Schematic	6

3-3   Texsteam Piston Pump Schematic  	,..,,,	?

3-4   Texsteam Piston Pump Cut-away Schematic ........................... 8

3-5   Diaphragm Pump Schematic	9

3-6   Diaphragm Pump Cut-away          ..............................  10




                             LIST  OF TABLES

                                                                       Page

4-1   CPA            of Fuel-Gas Venting Rates for Gas-Operated
      Chemical Injection Pumps  .	.,,,.,	13

4-2   Summary of Site Data	  15

4-3   Site	16

4-4   Data Set Comparison  for Chemical  Injection Pumps	» , . , .  17

4-5   Pump Manufacturers'  Data for Diaphragm  Pumps . ,	  19

4-6   Pump Manufacturers'  Data for Piston Pumps	  20
                                    VH

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1.0          SUMMARY

             This report is one of several volumes that provide background information
supporting the Gas          Institute and U.S. Environmental  Protection Agency Office of
Research     Development (ORJ-EPA/ORD) methane emissions project.  The objective of
this comprehensive program is to quantify methane emissions from the gas industry for the
1992 base year to within ± 0,5% of natural gas production starting at the wellhead  and
ending immediately            of the

             This report describes a study to quantify the annual emissions from chemical
injection pumps.  Piston       and                  are the most common types  of
       gas-powered          injection pumps      in the production           An
emission factor for these types of pumps was developed based on site data, manufacturer's
data, and results from a Canadian study.  The resulting annual  methane emissions from
chemical injection pumps are 1.5 Bscf ± 203%.

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2.0           INTRODUCTION

              di'-niiofil  injection pumps art," small  positive displacement,  reciprocating  units
designed In inject precise amounts  of chemicals inlo process streams,  'these  pump;; arc
used in 'ho iijitun-il gas production segment  to control processing problems or protect
equipment.  Gas-driven chemical injection pumps,  which use gas pressure to drive other
fluids, arc  commonly used iu production fields when- eluciiie.ity is nut readily m';-ulnblo

              The characteristics thai alTeel emissions from chemical injection pumps
include; the si/.e  of the unit, frequency  of operation, supply ;.ias pressure,  and mlei mothcine
i'oitipysiiton   tmissiofi factors for  diaphragm and piston pumps were determined by
converting a manufacturer's  reported gas consumption per volume  oi' dj«ni«il pumped u>
gas emitted per stroke, based on the plunger diameter and stroke length of typical pumps.
The frequency of operation was based on timed stroke rates from  site visit; and operator
information on the animal  use of the devices.  An eijtrdthm refmtCL- ihovr  puamdt-ix \va>.
developed for each tvpe  of chemical  injection pump (piston pumps and diaphragm pumps}.
The number of gas-operated  pumps  in the U.S. production segment was determined by
establishing a ratio of pumps to wells that market natural gas.  Annual methane emissions
from chemical injection pumps were calculated baswl on tin- piwHet of the emission taetor
for a typical pump and the activity  factor (count of chemical injection  pumps; nationally).

              This report presents an estimate oi loial  I! S. emissions from f icse pumps.
'Hie following sections quantify the  amount of methane thai is  released  from chemical
injection pumps nationwide.  A description  of ehcmk..il injection pumps typieatly used  in
the natural gas industry is provided  in Section 3.  Section 4 describes the sources of
information used to determine methane emission  factors  for these pumpK   National inmuai
emissions are  calculated  in Section  5.

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 3.0           CAS-DRIVEN

              This section describes chemical injection pumps found in the natural gas
 industry,  as well as differences in installations in various segments of the industry,

 3.1           Opera tion Overylew

              All industrial pumps      two                    a driver     and a motive
 side.  The driver provides the energy for the pumping operation; the motive     delivers
 the energy to the fluid being moved. For  a typical industrial centrifugal  pump, the driver
 might be  an electric motor; the motive       is an         and

              In the natural gas industry, gas-driven pumps  are small pumps used in the
 production field where electricity is not readily available.  These pumps use gas pressure to
 drive other fluids.  The supply gas can be             air (as in gas            plants), but
 most  often it is natural gas       directly from the           stream.  The      majority of
 gas-driven pumps in the field have one of two purposes: glycol  circulation  (see Volume 15
 on gas-assisted glycol pumps') or chemical injection,

              Chemical injection is needed in the field to add small amounts of chemicals
 that control processing problems and protect the equipment.   Typical chemicals injected in
 an oil or gas field are biocidcs,                                                 inhibitors,
 hydrate inhibitors, paraffin                                         and
 (H2S) scavengers.  These chemicals are normally injected at the wellhead and into gathering
 lines  or at production separation facilities.   Since the injection      are typically small, the
pumps are also small. They are              to                  the          being
 injected.

              Chemical injection pumps are                      reciprocating units
designed to inject precise amounts  of             a                 Positive

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 pumps work by allowing a fluid to flow into an enclosed  cavity from a low-pressure
 source, trapping the fluid, and then forcing it out into a high-pressure receiver by
 decreasing the volume of the  cavity.  A complete reciprocating -stroke          two
 movements, referred to as an  upward motion or suction stroke, and a downward motion or
 power stroke.  During the suction  stroke, the chemical is lifted through the suction check
 valve into the fluid cylinder.  The suction check valve is forced open by the suction lift
 produced by the plunger and the head of the liquid  being  pumped.  Simultaneously, the
 discharge check valve remains 'closed, thus allowing the chemical to        in the fluid
 chamber. During  the power stroke, the plunger assembly  is Forced downwards,
 immediately  shutting  off the suction check valve. Simultaneously, the chemical is
 displaced, forcing  open the discharge check valve and allowing the fluid to be discharged.
 This complete movement represents  one full stroke.

              The two types of gas-driven pumps commonly used in the natural gas
 industry  are the piston pump and the diaphragm pump.  These pumps operate in the same
mariner,  but with different reciprocating mechanisms.  The barrel-type       pump,
illustrated in Figures 3-1 and 3-2, consists of a cylindrical piston-plunger assembly.2
Movement  of the larger-diameter piston provides the force       to move the  plunger,
Another  type of piston pump observed at. sites in California (Figures 3-3  and 3-4) uses a
horizontal plunger to operate a gear mechanism that drives the plunger,3  The diaphragm
pump, illustrated in Figures 3-5 and  3-6, uses a flexible diaphragm to move the plunger.4'5

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3-1. Kston Pump Schematic

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GAS
OUT

                                      FLUID
                                    SUCTION
               Figure 3-2.  Piston Pump Cut-away Schematic

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              IAS
              CAR SIDE)
               GAS
             EXHAUST
  FLUID
DISCHARGE
                                         3-6,           Pump Cut-away

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3-2           Emission-Affecting. Characteristics

                                                               the gas-driven        in
chemical  injection  service include;

              »      Frequency  of operation (pumping rate);
              »           of the     (volume              of the motive chamber);
              •      Supply gas pressure  (which affects density); and
              *      Inlet methane composition.

              For this study, the frequency of                          by        the
stroke intervals and collecting  information about pump operating schedules.  Determination
of the unit size was based on manufacturers' data for the types of pumps observed during
site visits. Supply  gas pressure,  which affects the density of the gas,      noted during site
                  of an                gas                                 on literature
data.  These                are          in            in        to their      on the
emission  calculations in the following section.
                                           n

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4.0                      FACTOR DATA

             Four        of information          to                           from
chemical injection pumps:  results of a study performed by the Canadian Petroleum
Association, literature data for methane composition, data collected from site visits, and
pump manufacturers* data.

4,1          Canadian PetroleumAssociation CCPA) Report

             The Canadian Petroleum Association (CPA) conducted a study to quantify
                      oil and gas                     in Alberta,6            from
diaphragm chemical injection pumps were determined from bagging tests of five pumps.  The
measurements were very consistent, ranging from 254 to 499 scfd/pump (see Table 4-1).
The average natural gas emission factor from the Canadian study was 334 ± 30%
sefd/pump,

4.2          Methane Composition

             Emission factors for methane are calculated from the rate of natural gas
                  by the        composition. The          of         in
natural gas                to be 78.8% ±5%.              this value are available in
Volume 6 on       and           sources.7
                                         12

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                                                           5- OF -FUEL-GAS                    FOR"''
^,; ' =  ">:-lr.X-,:  r';-~ r -~\   -CAS^PERATED" CHEMICAL-INJECTION PUMPS' V-';-' / " -'

r~-~.-  i~;,'-'_ •-"--.:"*  "-:_• St%\ ,,-,'^ "   "-;••*.'     Quantity'   -   '----_.' -  '   ---O, \/   _,  •-" -^ .-'"-„
--, v ; '-"-'"-„ /,>,", \Type'of -r^Tjipfc of.  .-" .Type,.of--."_ Measured  -  Min.Flow:^    Max, Flow  ," -'-_ ^Avg^.Flow; .
 •r^~ J"s'7*;?",: "-v  , '-^n'st -^-J¥aclI%rf:"Ea»ipnient  --' if Qnce\  [._  Rate/Puni|t  -  v,^Kaife/Piimp *",/ ,'Rate/iPiiinp,
                          Oi!,Battery' Line.Heater    "'  -l.,~      - -  0\- -"       °0  -, ,        498.9 scfd -_-

  _i;   '•S"icJ;7:'- CIP ":V 'oil Battery;      Line-  '"'   1  /    ' 165.8 scfd '   "'-; .=349:6 scfd",, .-."- .-.--254.4'scfd

  ;> ''  \ "—-•-'';  JCIP/   -OiLBsttery  Sales~L*ine      ;' -1  /     -  ^ "0 --    -- '  ->1917 scfd -    _   3'73.7 scfd "

   -  •--''; ~~_-~'„"" ,GD>'  " l^Mitttfr Oil   Wellhead"   -   -  1  r.'    "  '  b -  '   '    --" b-   _  '-,: _--254.3 scffl ---
  *  '.'  ""•"""-   „ "  -.' . "-FttW-- .-"-"-_/"'/"•'--      "  "  --   ''     --'-""    ''."'"
         ^".      CIP -   Minor Oil  "-Wellhead'   -    , II-         "   b    -'   . -   _  , b-         290.3 scfd /
  :./  ,{r"--_-,*       ^  'Retf   ;/;  -:'"_  -.•.'-."-.    .   '  -;'.-'"       ----..%-'     '   '     ..:-••

  ",-",--:-:-"  '-.;.'   ;--.  ". \   -  ",-:   '  •',  AVERAGE"-  '-'   -     ,*    ':'   -~'       334scfa±3o%
               ,  * CIP *= Chemical Injectio
              " \ b Minimum and ntaximun) flow rates were jiot measured in these cases, only the average rate.   _"."


               ;4.3-:-'-^,   SitePata  "    '   "-'-••    .  '   ' r  "      '•.-.:     '   -  '~  '
            V ' -" ,    _ ,     Chara.K ,-" »ics that allow populations and average pump cmissioa factors to be
             I ^estimated were gathered from 19 sites by telephone contacts or,site visits.  .The.information  -
                - collectedJncluded:  ,^
                                     .Total number of chemical injection pumps fora particular site; -  .  -  .

                                     Number, of chemicaljnjection pumps used in natural gas production ' -1
                                     (see Volume 5 on activity factors*-for more infoimation on the industry
                                     boundary definition); -  -   -    .-, ~  ,  •    . i

                                     Energy source (gas,-air," or electric);

                                     Frequency of=operation (pumping rate in strokes/tnin);          *    .

                                     Number of puinps active or idle;      =     _-,";•_

                                     -Pump operation schedule;    -_'_.'      -.        -       ,

                                     Size of the unit (volume displacement of the motive chamber);
                                                            13
^-~' P  r  ,,,~-_'"^ f'-

 *~ ?V*.C "-"•'

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              •     Maimfaeuirer and mode! immher of the unit; and
              •     Supply gas pressure,

Table 4-2 lists the site  mform?.uo» and Table 4-3 summarizes the sir;: data by pump rype.
This information was used to produce an estimate of equipment populations
characteristics for  the U.S. population of gas-driven ehcmk'al injection pumps.

             The frequency of operation, or pinupUig rate (Mruke/min). WHS based oil limed
stroke intervals measured during site  visits  The number of rate samples is shown in Table
4-2 for siies where this parameter was measured. For silc.s with no rale sample
measurements,  calculation of zm average value lor the pump type (either pjston or dia-
phragm)           on measurements from other sites,

             The fraction of eaeli pump type, piston versus diaphragm, was calculated
      on the total T>umber of each type of p'_7iip observed.  Table 4-2 shows that piston an<1
           pumps are equally distributed for the     visited (49 8/1 piston pomps compared
with 50.2% diaphragm pumps).

             Some of the pumps are only opemred on a seasonal ha.^is.  Therefore, opera.o1'
information and  observations from site visits were used to determine the fraction of lime  the
pump operated annually.  Table 4-3 shows that piston pumps operate approximately 45 A  of
the year, while diaphragm pumps are in use 40% of the year.

             At four of the sites visited,  both piston and diaphragm pumps were observed.
However, no estimate of the relative  number of each type of pump was made; only {he total
number of chemical injection pumps was provided.  For these sites, the fraction of piston
versus diaphragm pumps observed from the other sites were applied so that the pump
operating data collected at the four sites could he used.
                                          14

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TABLE 4-2. SUMMARY OF SITE DATA


Site
i
~i
t+
3

4

5
6
7

8


9

10
II
12

13

14
IS
16
I?
IS
19


Pump Type
Piston
Piston
Piston
Piston

Diaphragm
Diaphragm
Diaphragm
Diaphragm
Piston

Diaphragm
Piston

Diaphragm
Diaphragm
Diaphragm
Diaphragm
Piston

Diaphragm
Piston
Piston
Piston
Piston
Piston
Piston

Power
Media
Nat, Gas
Nat. Gas
Nat. Gas
Nat. Gas

Nat. Gas
Nat. Gas
Nat, Gas
Nat. Gas
Nat. Gas

Nat. Gas
Nat. Gas

Nat. Gas
Nat. Gas
Nat. Gas
Nat. Gas
Nat. Gas

Mat. Gas
Electric
Eiectric
Nat. Gas
Air
Air
Nat Gas
Total
Number of
CIPs at the Site
108
5
203

666

5
28
273

60


36

4
12
8

25

115
24
1
4
5
I
CIPs Within Gas
Industry Boundaries
at (he Site
to
5
0

0

5
28
273

0


36

0
12
8

25

§
0
0
0
0
]
Number
of Rate
Camples
14
0
8
0

0
1
I
1
0

0
1

2
3
0
0
0

0
-
-
1
4
3
1

Strokes/ ' %
win Gperiiling
6.64 63.6
93
16.8 61,9
27.3

27.3
2 90
12 25
30 50
3.8

3.8
0.5 100

15 100
9,2 81.3
100
50
100

100
--
-
0.33
55
65
40

Number
Operating
68.7
4.6
125.7
9ft. *,

91.1
4.5
6.9
136.4
1.2

1.2
17.9

18.1
3.3
12.0
4.0
12.5

12.5
-
--
--
--
--
--
              15

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                          TABLE 4-3.        DATA
Pislon Pumps
Total Number of Gas Operated CIPs
Observed from Site Visits
% by Type
% Operating
Average Strokes/min

49
44
26
327
,8 ± 38%
.6 ± 62%
.3 ± 29%
Diaphragm Pumps

50.2
40.0
13,6
329
± 38%
i- 52%
+ 49%
4.4           Industry Boundaries

              The "gas industry" boundaries include ail gas well           but excludes
equipment           with oil production. This boundary definition is significant for
chemical injection             a             of            are      specifically for
chemical addition to oil wells.

              During site visits, data were collected for all pneumatic chemical injection
pumps regardless of the associated equipment.  As shown in Tables 4-2 and 4-3, data
collected for the purpose of this characterization report consist of actuation measurements
    pump make/model types for pneumatic chemical injection pumps, including pumps
r;-~-_;-,Tted liy            air and              to the oil industry.  The decision          to
include all     for the          factor            but to account for the industry boundary
definition in the activity factor.  (That is, the activity factor only includes natural gas
powered chemical injection pumps associated with the natural gas industry.)

              To examine the effect of this decision, emission estimates were determined
      two     sets:  one containing all of the available data,     the other using only data
for gas-operated chemical injection        within the natural gas industry. The res-'ts of this
            are           in Table 4-4,
                                           16

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   TABLE 4-4.  DATA SET COMPARISON FOR CHEMICAL INJECTION PUMPS
Using AH Data

Percent of Total Pumps, %
Pump Actuation Rate, strokes/mill
Number of measurements
Number of sites

Piston
49.8 i 38%
26.32 ± 29%
32
7

Diaphragm
50.2 ± 38%
13. M ± 49%
8
5

Using Only Natural Gas
Industry Data
Piston
4.5 ± 6?S%
3.57 i: 42%
15
2

Dixpliragm
95.5 ± 32%
14.75 ±
61%
5
4
  Operating Fraction, %
   Number of sites
  Methane Emissions Factor,'
  scfd/pump
44,6 ± 62%     40,0 ± 52%
    ?             10
       248 ± 83%
77.5 ± 148%    58.0 ± 39%
     4             6
       668 ± 88%
"Details on the emission factor calculation arc presented in Section 5.

              Limiting the     to strictly gas-operated        within the natural gas industry
significantly reduces the database from which the emission factors are calculated and results
in a much larger emission factor.  A follow-up conversation with a manufacturer of both
      of                that          the       are            on the         of
required and the injection pressure, the type of production        gas or crude) is not a
leading factor for selecting the pump type.  Both pump types can accommodate  conditions
associated with either natural gas production or crude production. This was confirmed by
industry contacts as well.  Therefore,  because a definitive reason for choosing one pump type
for       gas production       not be             the           set—using all of the
data—was used to determine the emission factor per pump. The actual number  of pumps
operating on gas within the natural gas industry boundaries is accounted for in the activity
factor.
                                           17

-------
 4.5           Manufacturers'.Data

              Stroke frequency (strokes per minute) was determined from site daia; however
 chemical injection                          gas      to the volume of chemical
 (scf/gal).  To convert scf/gal to scf/strokc,  the volume of chemical displaced per stroke was
 calculated based on manufacturers' data for stroke length and plunger diameter (for
 diaphragm pumps) or piston diameter (for piston pumps) as «;}i0wn.2'M*19'RU1
        Gas Usage, scf _  Strokg_Length (in.)    » Diameter (in.)-  _   gal.     „   ,,  t  ( set \   /|\
           stroke            stroke               4         231 iu,J
Tables 4-5 and 4-6           the information provided by the diaphragm and piston pump
               respectively.  The           gas       per       is also        for
pump size,

4,5.1         Diaphragm Pumps

              The diaphragm pump              provided gas       in       of standard
cubic feet of gas (at 1 aim and 60°F) required to pump one gallon of liquid, where gas usage
for each pump varies slightly with discharge pressure.  Despite the wide range of pump sizes
available, the                              to          an                 rate per
      (with a 90% vonfidenee interval  of ± 10%) for the pumps shown in Table 4-5,  The
pump manufacturer     were examined over the          pressure       of 0 psig to 1000
psig {discharge pressure ranged from 20 to  1060 psig for  sites visited), for which the gas
usage varied  by only 20%.   For example, the gas  usage for the 3/8-inch Western Chemical
          105 to 118        over the                        of 0     to 1000 psig.*
Calculation of the                   per                 on the                 and
stroke        as shown by Equation 1.  Combining the calculated liquid displacement for
each plunger size over the range of gas usage values, results in a matrix of calculated
sef/stroke values.  Table 4-5 shows      values which vary from 0.0451 to 0,1660

                                          18

-------
    TABLE 4-5.  PUMP MANUFACTURERS' DATA FOR DIAPHRAGM PUMPS


Manufacturer/
Model
Western Chemical
Pumps, Inc. ''

Texsteam Series
5000 4





Texsteam Series
5100s



CPA

Diaphragm Pumps
Plunger
Diameter, Stroke
in. Length, in.
3/8 7/8
5/8 7/8

1/4 i/2 1 1/4
3/8
1/2
3/4
t
f 1/4

1/8 1/3 - 1
1/4
3/8
1/2

ft
Diaphragm Pump Average

Natural
Gas Usage,
scf/gal"
105-118
42-5?

280 - 756
140 - 3(,g
80.6 - 212
36 - 117
20.6 - 62
13.6 - 44

457 - 1407
244 - 810
120 •• 492
53 - 186




Calculated
Natural Gas Usage
scf'/stroke8
0 047-U.O:> 1
0.054 0.073
Average — 0.0563
0.0744 - 0.0813
0 0837 - Q.WI4
0.0853 - 0.0978
0.0851 0.1329
0.0860 0.1360
0.0866-0.1660
Avcn,ge =-= 0 ()%?
0.0546- 0.0561
0.0519-0.0574
0.0574 - 0.0784
0.0451 - 0.0527
Average - 0.0567
Average - 0.01701'
0.0719 ± 10%
 To convert from sef of natural gas to scf of methane, multiply by inol % methane in
 natural gas.
* The Canadian emissions, reported in Table 44 as scfd/punip. where converted to sef/strokc
 based on (lie diaphragm pump actuation rale  determined from site daU* and shown in
 Table 4-3.

-------
       TABLE 4-6. PUMP MANUFACTURERS' DATA FOR PISTON PUMPS

                                    Piston Pumps
Manufacturer/
Model
Line Mfg.2
Piston
Diameter, in.
2 1/2
Stroke
Length* in.
1/4
I
Calculated
Natural Gas Usage
scf/stroke8
0,0022
0.0086
 Arrow Specialty Co.

Williams Chemical
Instruments "
Texsteam 3703 J
Piston Pump
J 1/4
1 1/4
2 1/4
2 1/4
„
Average
1/8
W
1/8
i
„

0.0003
O.OOli
0.0009
0.0070
0.0013b
± 65%
 Conversion of act" to scf is based on a typical supply gas pressure of 30 psig determined
 from reference material12 as well as pressures observed  at eight sites.
1 The piston size and stroke  length were not specified for this type of device.  Instead, the
 manufacturer provided the  gas usage per gallon of chemical pumped, which ranged from
 160 to 500 scf/gallon for discharge pressures of 0 to 1000 psig.  Based on the average
 stroke frequency observed  at Sites 17 and 18. the corresponding gas usage per stroke
       from 0.00063 to 0.00195, with an average value of 0.0013 scf/stroke.
                                         20

-------
 scf/stroke.  Calculating the average of the range of manufacturer data and the Canadian
 measurements results in the average gas emission of 0,0719 scf/slrokc ± 10% for the
 diaphragm pumps.

 4.5.2         Piston Pumps

              Manufacturer      for the Texsieam piston pump were similar to that provided
 for the           pumps;  standard cubic feet of gas required to pump one gallon of liquid.
 In addition, the  manufacturer provided ranges for the volume of chemical pumped (gal/day),
 corresponding to different actuation rates (stroke/min).  Actuation measurements  from the
 two sites where  the Texsteam  pumps were observed were used to convert the gas discharge
 rate per volume of chemical to the discharge rate per stroke as shown in the following
 equation:
                            Gas Usage, scf _  scf    gal.     day                          r
                            —~_—.	~,— _ 	  x  ~ -   x	—                        V
                               Stroke      gal.    day   strokes

              For the barrel  type piston pumps, the gas usage was calculated based oil the
manufacturer specifications for the piston diameter and stroke length:
               Gas Usage, acf  _ Stroke Length (in.)  _  H Diameter (in..)2  .  	tf              n\
                   stroke           stroke               4          1728 in,3
Piston pumps are not as diverse as diaphragm pumps and have a limited number of piston
sizes.  Based on the use of these pumps in the natural gas industry, the 114-inch to 2'/2-inch
piston diameters would be typical.

             The stroke length is adjustable for the piston-type pumps.  Since specifics
concerning the typical              for pumps at each site were not known, die range of
manufacturers* values (1/8 to 1-inch) were used.  In addition, the supply gas pressure can
affect the gas usage for these pumps due to the effect of pressure on gas density.   Based on

-------
manufacturers' data, piston pumps are designed for supply gas pressures ranging from 15 to
85 psig,  A supply gas pressure of 30 psig was used for the emission calculations based on
an        of         and reference material,'2  Combining the data from the four
manufacturers, the average gas usage for the piston pumps was determined to be 0.0037
scf/stroke ±65% (Table 4-6)-

-------
 5,0                      SATE CALCULATIONS

              Sile information was used to determine the average actuation rate
 (strokes/min}, the fraction of each type  of pump (piston versus diaphragm), and the
 percentage of operating time for each type of purnp.  The manufacturers' data were used to
 determine the volume of gas         per      stroke (scf of gas/stroke).  Radian combined
 the site information and manufacturers'  data, as          in this section, to calculate
         emissions for each type of pump in standard ethic     per day per pump. An
 average pump emission factor was calculated by combining the emission factors (EF) for
 diaphragm and piston pumps:
          pump   •""     piaeB pumps * *1*'pkifln pumps ~*~ "ac"*'%iajjl!tsfm pumps ^ *-*" diaphragm pninp

                        x 50 scfd methane/pump)^ +
                (50,2% x 446 scfd methane/pump)djaphragni
                248 scfd methane/pump
where, the fraction of each       type is from Table 4-3,  Details           the data values,
               calculations, and the         national              are          in this
section -

5.1           Diaphragm .Pumps

              Calculation of the emission factor for the diapliragm pumps was based on the
fol lowing equation:
                         &s Usage (scf/slrokc) x  Frequency (strokes/day)  x Operating
                         tLne x % Methane                                         (5)
                                          23

-------
 where;
       Gas usage         =   calculated gas      from Equation 1 (0.0719 ± 10%
                             scf/stroke).
       Frequency         =          per day of the        pump (19,642 + 49%
                             stroke/day).
       Operating time     =   portion of the year that the pump is operating (0.40 ± 52%).
       % Methane        =   78.8 mol % ± 5% for the production segment.
The total methane emission factor for diaphragm pumps is 446 scfd/pump ±77%.


5,2          Piston. Pumps


             Caiciiiation of the         factor for                      on the following
equation:
                       —  Gas usage (acf/ stroke) x Density (scf/acf) x Frequency
                          (strokes/day) x Operating time x % methane               (6)
where;
       Gas Usage       = Calculated gas      from Equation 3 (in actual ft'/stroke).
       Density          — scf/aef at supply gas pressure (average 30 psig)
                          (combined average value of volume and density is  0.0037 ±
                          65% scf/stroke).
       Frequency       =        per day of the average pump (37,901 ±29%
                          strokes/day).
       Operating        =        of the year that the pump is         (0.446 ± 62%).
       %               = 78.8 mol %  ±5% for the production segment.

The resulting methane emission factor for piston pumps is 48.9  scfd/pump + 106%.


       Using Equation 4, the diaphragm pump and piston pump emission factors are
expressed in a ratio based on the  fraction of each type of pump  observed from site visits
(0.498 ±38% piston pumps and  0,502 ±38% diaphragm pumps from Table 4-3) to
produce an emission factor for a typical chemical injection pump of 248  ±83% scfd/pump,
                                         24

-------
5,3          National Emission Kate

             The                     is calculated using the emission factor per average
pump (248 scfd/pump from Equation 4) multiplied by the number of pumps used in
production fields nationwide.  The number of gas-operated pumps in the gas industry
production segment was determined by establishing the ratio of the number of pumps to
active       that market gas. Details on this calculation are provided  in Volume 5 on activity
factors,* The resulting        activity factor is a     of 16,971 ±  143%       in the
production sector,

             Multiplying the chemical injection pump emission factor by the activity factor
yields the total annual emissions for gas-operated chemical injection pumps:
             ER^p = 248        -     y 365       x  16^71 ±m%  pumps
                                pump        year
The resulting         emissions for the production segment are 1.5 Bscf + 203%,
                                         25

-------
6.0          REFERENCES
1.           Myers, D.B., and M.R. Harrison.  Methane Emissions from 
-------
    APPENDIX A




Production Source Sheet
        A-l

-------
                                   PRODUCTION SOURCE SHEET

SOURCES:                                    Wells, Gathering Facilitii*
COMPONENTS:                               Chemical In)ection Pumps
OPERATING JVIOtM'l:                          Normal Operation
EMISSION TYPE:                             Unsteady, Vcnlcd
ANNUAL EMISSIONS:                        1.5 Bscf + 203%

BACKGROUND:

Cias-driven cliemical injection pumps use gas pressure acting on a piston Ui pump a dicmioi! im the apposite
side of the piston.  The gas is then vented directly to The atmosphere. The pumps are used lit add f.hermetf»,
such as corrosion inhibitors, scale inhibitors, triocidc,  deiiiulsiiier. dariffer, and hydrate inhibitors to operating
et)uip!iieoi.  Two types of       were observed: I) piston pumps, and 2)  diaphragm pinups.  Some of flu:
pumps observed  wen-  inactive al (lit: time or had seasonal operation.
EMISSION FACTOR:   24fi scftl/average pump  ± 83 %

           (This was adjusted tor the production methane content in natural gas al 78.8 UM>|%.)

This average emission factor is based npon the following equation:

        EF^ „,,,, = Fr,m x EF;,«,,  •}•  F,,,,,,^,, x EFltaph,,K1,,

        where:
        Fpjs^..      —     fraction of the pump population that is the piston iype- = 4V.8'* + 38%
        EFp,,,,,    =     emk's'oti factor of an average piston pump — 48,9 sci'd/pump i- 106%
        Piimiirjwis   =     fraclioTi of the pump population thai is the diaphragm type — 50,2% ± 38%
        £?<»»*.!.,,•»  =     emission factor of an average diaphragm pump = '146 scW/piimp  ± 77%

The average device emission factor was determined by an aggregation of device emissions calculated for
multiple U.S. sites.  For piswn pumps, the emission factor was determined by  ihc following equation.

        EFpBM1          =      Gas usage (aef/slroke) X Density (sef/acf)  X Frequency (strokes/day)  >;
                               Operating lime x % methane.

where:
        Gas usajje       =      calculated gas usage based on piston dinmeiet anil stroke IfHi'.lh (in  u^tuul
                               ft3}:
        Densiiy         =      scf/aef at supply  gas pressure (average 30 psig) (combined average  v.iiw. oi
                               volume and density is 0.0037 J,  65% scf/stioke),
        Frequency       =      strokes per diiy of the average, pump (37,901 j_ 2fJ% sirokcs/day),
        Operating time   =      poninn of time thai the pump is operating (0 -'Wd  -\ 67%); ami
        %  methane       =      78.8nioi?>- + 5?v for the productiuti scgnieut.

Based on siie and  manufacturer data, the resulting national pLtOn pump emission factor IK 4S *J scltj/pmnp -i
106%.

-------
 For diaphragm chemical injection pumps, the emission factor was determined by the following equation:
 win. e:
            ophntnt        ~    Gas usage (scf/gal) x Volume (gal/stroke) x Frequency (strokes/day) x
                             Operating time x % methane

        Gas usage       =    volume of gas (in standard ft3) required to pump one gallon of liquid chemical
                             (provided by the manufacturer);
        Volume         =    liquid displaced per stroke based on the plunger diameter and stroke length
                             {combined average value of gas consumption and  volume is 0.0719 ±  109,
                             scf/stroke);
        Frequency       =    strokes per day of (he average pump (19,642 ±49% strokes/day);
        Operating lime   =    portion of lime that the pump is operating (0,40 ± 52%); and
        %              =    78.8 ntol% ±5% for the production segment,

Using the site, manufacturer, and measured data to calculate the emission factor equation terms, the total
diaphragm pump emission factor was determined to be 446 scfd/pump ±77%.

Stroke volume was calculated from pump manufacturers' data and site observations of manufacturer and model
number.  Density was calculated based upon observed site supply gas pressure, and frequency was based upon
timed stroke intervals observed while on site. Operating time was estimated by site personnel (if seasonal), or
was            the percent of        at the site that were          during the visit. The emission factors
shown above (in scfd/pump^ have been corrected for the natural gas composition in the production segment of
78.8 mo! %  methane.
EF DATA
        3,

        4.


        5.

        6.
                       The report entitled Methane Emissions from the Natural Gas Industry, Volume 13:
                       Chemical Injection Pumps (1) establishes the important emission-affecting
                       characteristics.
                       Site visit data and reference material established the density from supply gas pressure
                       at 30 psig.
                       For the piston pumps, the stroke volume was estifliated from manufacturers* data of
                       pumps found at each site.
                       Manufacturers*      for the diaphragm       provided scf of gas required lo pump
                       one gallon of chemical.  This information was      with the calculated liquid
                       displaced  for a range of pumps to give an average     volume.
                       The frequency of          per day was determined from 40 timing
                       taken at 12 sites.  The operating time was determined from data at 13 sites.
                       Measurements of 5 diaphragm chemical injection pumps were provided from an
                       emissions estimate program by She Canadian Petroleum Association,
EF ACCURACY:
        Basis:
        1.

        2.

        3.
                       Operating lime confidence bounds (at 90% confidence) were calculated by analysis of
                       the spread of ? sites for piston pumps and 10 sites for diaphragm pumps.
                       Actuation confidence bounds (at 90% confidence) were based on measurements from
                       7 sites for the piston pomps and 5 sites for the diaphragm pumps,
                       It was        that the manufacturers' data are completely accurate.  Data for the
                       piston pumps were       on information from 4 manufacturers,  Diaphragm pomp
                       data were provided by 2 manufacturers.
                                                 A-3

-------
        4.
                90% confidi«,€e bou,"ds for each value were carried through error propagation to
                result in (lie t.nal  90% confidence bound,
 ACTIVITY FACTOR:  I6,«>71 pumps in (he production segment + 143 %

 The number of gas actuated pumps used in the production segment was determined by establishing the ratio of
 the number of       to active wells (oil or gas) that market      Si»e data wen: organized inio regions and
 regional values were determined.  The regional ratios were then multiplied by the regional count of active wells
 that market gas in that region to         the     count of         injection       in the region. Finally,
 regions were added  together to determine the national number. The activity factor is then:
(1)
National AF =
n
E
                           (Regional AF)
where n = lota! number of regions
(2)
Regional AF =  (R,'s) x  (W)
                                               where Rj = ratio of tola! pumps to total wells in Region j
                                               where W = number of wells in the region
AF DATA
        2.
        3.
               The active oil and gas weils are from A.G.A. Gas Facts (2).  The active oi! wells that
               market gas are determined by multiplying the total national active oil wells times the
               fraction that market gas. The fraction is determined from a Texas Railroad
               Commission iease study that shows the percent of oil leases that market the associated
               gas in Texas (3).
               The pump counts were obtained during the site visits.  Inactive, electrically driveri, j)r
               air driven pumps were not counted.
               Regional extrapolation by gas well count was used.
AP ACCURACY:
        Basis:
        1.
        2.
               The accuracy for the active gas weils is assigned by engineering judgement, based
               upon the fact that the number of active wells is tracked nationally and known
                         by A.G.A./DOE, etc.
               The accuracy for the national AF is           error propagation from the production
               sites visited.
ANNUAL EMISSIONS:  1.5 Bscf ± 203 %

The national annual emissions were determined by multiplying an emission factor for a typical pump by the
popt lation of chemical injection pumps in the production segment.

REH5HENCES

1.      Shires, T,M,  Methane Emissions from the Natural Gas Industry. Volume 13: Chemical Injection
        Pump,       Report, GRI-94/0257.30aiid EPA-600/R-96-080m, Gas         Institute and U.S.
        Environmental Protection Agency, June 1996.
                                                A-4

-------
2.      American Gas Association. Gas Facts: 1993 Data, Arlington, VA, 1994.




3,      Texas Railroad Commission, P-l, P-2 Tapes, Radian flies, Austin, TX, 1989,
                                                A-5

-------
             1
Conversion Table
      B-l

-------
                               Unit Conversion Table
                            English to Metric Conversions
    I scf methane
    3 Bscf methane
    1 Bscf methane
    1 Bscf
    1 short ton (ton)
    1 Ib
    1 ft3
    1 ft3
    1 gallon
    ] barrel (bbl)
    1 inch
    ! ft
    1
    1 hp
    1 hp-hr
    1 Btu
    1
    1
    T(T)
    1 psi
     19,23 g
     0.01923 Tg methane
     19,230 metric tonnes methane
     28.32 million         cubic
          kg
           kg
            m3
     28,32 liters
     3.785 liters
     158.97 liters
          cm
           m
          km
     0,7457 kW
     0,7457 kW-hr
     1055 joules
     293
     430 g/GJ
     1.8 T f C)  + 32
     51,71 mm Hg
                            Global Wanning Conversions
Calculating carbon equivalents of any gas:
=        of gas) x
                                            MWi
                                           \  MW, gas
                                                          x (GWP)
                                        B-2

-------
 Calculating CO2 equivalents  for methane:
                                                         cev,
                   of CO2 equiv.  =        CH4)  x  j	 | x
                                                        , CH,,
where MW (molecular weight) of CO2 = 44, MW carbon = 12,  and MW CH4= 16.
Notts


scf



Bscf


MMscf


Mscf



Tg


Giga (G)



Metric tonnes


psig


psla


GWP




MMT


MMTCE


      of CO2 eq.
Standard cubic feet.  Standard conditions are at 14,73 psia and 60°F.


Billion          cubic feef (10* scf).


Million         cubic feet.


Thousand standard cubic feet.


Teragram {1012 g).


      as       (10*).


1000 kg.


Gauge pressure.


Absolute pressure (note     =      + atmospheric pressure).


Global Wanning Potential of a particular            gas for a given

time period.


Million metric        of a gas,


Million metric tonnes, carbon equivalent.


Million metric tonnes, carbon dioxide equivalent.
                                          B-3

-------
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