EPA-600/4-7B-041
August 1976
1970 THROUGH 1974
FROM THE NATIONAL AIR
SURVEILLANCE NETWORKS
IWtorteg p* Soppert Laboratsry
of -'
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RESEARCH REPORTING SERIES
Research reports of the Office of Research and Development, U.S. Environmental
Protection Agency, have been grouped into five series. These five broad
categories were established to facilitate further development and application of
environmental technology. Elimination of traditional grouping was consciously
planned to foster technology transfer and a maximum interface in related fields.
The five series are:
1. Environmental Health Effects Research
2. Environmental Protection Technology
3, Ecological Research
4. Environmental Monitoring
5. Socioeconomic Environmental Studies
This report has been assigned to the ENVIRONMENTAL MONITORING series.
This series describes research conducted to develop new or improved methods
and instrumentation for the identification and quantification of environmental
pollutants at the lowest conceivably significant concentrations. It also includes
studies to determine the ambient concentrations of pollutants in the environment
and/or the variance of pollutants as a function of time or meteorological factors.
This document is available to the public through the National Technical Informa-
tion Service. Springfield, Virginia 22161.
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EPA-600/4-76-041
August 1976
AIR QUALITY DATA FOR METALS
1970 THROUGH 197*t
FROM THE NATIONAL AIR SURVEILLANCE NETWORKS
by
Gerald G. Akland
Statistical and Technical Analysis Branch
Environmental Monitoring and Support Laboratory
Research Triangle Park, North Carolina 27711
ENVIRONMENTAL MONITORING AND SUPPORT LABORATORY
OFFICE OF RESEARCH AND DEVELOPMENT
U.S. ENVIRONMENTAL PROTECTION AGENCY
RESEARCH TRIANGLE PARK, NORTH CAROLINA 27711
-------
DISCLAIMER
This report has been reviewed by the Environmental Monitoring and Support
Laboratory, U.S. Environmental Protection Agency, and approved for
publication. Mention of trade names or commercial products does not
constitute endorsement or recommendation for use.
i i
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PREFACE
The Environmental Monitoring and Support Laboratory of the Environmental
Research Center-Research Triangle Park (formerly the Quality Assurance and
Environmental Monitoring Laboratory), with the assistance and cooperation
of state and local agencies, conducts a variety of air sampling activities
to obtain information about the air quality in the United States. Metal
components of particulate matter are listed in this report.
Updated listings for this notebook will be provided as more current
data are available. Any subsequent changes in the introductory material
(site descriptions, data table presentations, laboratory methodology, etc.)
made by EPA will be forwarded on a routine basis.
i i
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ABSTRACT
Particulate pollutant data gathered during calendar years 1970
through 197^ by the cooperating stations of the National Air Surveillance
Networks provide the basis for listing the urban and nonurban concentrations
of 11 metallic components of suspended particulate matter.
The data are presented as a composite concentration value for each
site for each of the four quarters of the calendar year; a yearly average
is reported whenever valid data for all four quarters are obtained.
Two previous EPA publications, APTD-0978 and APTD-1467, list metal
components of suspended particulate matter collected during 1966 and 1967,
and 1968 and 1969, respectively.
iv
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CONTENTS
Preface .
Abstract
vi
List of Tables
vi i i
Acknowledgments
.... 1
Section I. Introduction
... 2
Sample Collection
^
Description of Data Tables . -
Section II. Quality Control
12
Section HI. Laboratory Methods
1 2
Suspended Particulate Matter
.... 13
Metals
Section IV. National Summary
. . 22
Section V. Data Tables
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LIST OF TABLES
Table
1-1
2-1
2-2
4-1
4-2
5-1
5-2
5-3
5-4
5-5
5-6
5-7
5-8
5-9
5-10
NASN Network Modification, 1970-1974 g
Blank Filter Concentrations and Yearly Analytical
Discrimination Values (yg/m ) , ]0
Analytical Precision, Bias and Confidence Limits ]]
Urban National Cumulative Frequency Distributions .... ]6
Nonurban National Cumulative Frequency Distributions ... 19
Beryllium, Urban Quarterly Composites and
Yearly Averages
Beryllium, Nonurban Quarterly Composites and
Yearly Averages
Cadmium, Urban Quarterly Composites and
Yearly Averages . _
Cadmium, Nonurban Quarterly Composites and
Yearly Averages
Chromium, Urban Quarterly Composites and
Yearly Averages ...
47
Chromium, Nonurban Quarterly Composites and
Yearly Averages
Cobalt, Urban Quarterly Composites and
Yearly Averages
Cobalt, Nonurban Quarterly Composites and
Yearly Averages
Copper, Urban Quarterly Composites and
Yearly Averages
Copper Nonurban Quarterly Composites and
Yearly Averaqes
81
VI
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Table Paqe
5-11
5-12
5-13
5-U
5-15
5-16
5-17
5-18
5-19
5-20
5-21
5-22
Iron, Urban Quarterly Composites and
Yearly Averages
Iron, Nonurban Quarterly Composites and
Yearly Averages
Lead, Urban Quarterly Composites and
Yearly Averages
Lead, Nonurban Quarterly Composites and
Yearly Averages ,,....
Manganese, Urban Quarterly Composites and
Yearly Averages .
Manganese, Nonurban Quarterly Composites and
Yearly Averages ........
Nickel, Urban Quarterly Composites and
Yearly Averages
Nickel, Nonurban Quarterly Composites and
Yearly Averages , . . .
Titanium, Urban Quarterly Composites and
Yearly Averages
Titanium, Nonurban Quarterly Composites and
Yearly Averages
Vanadium, Urban Quarterly Composites and
Yearly Averages :
Vanadium, Nonurban Quarterly Composites and
Yearly Averages
. . 83
- 93
. 95
105
, . 107
. . . 117
, . . 119
, . . 129
, . . 131
, , . 141
. . . 11*3
. . . 153
vii
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ACKNOWLEDGMENTS
The data reported in this publication could not have been gathered
without the generous cooperation of the many state and local air pollution
control agencies in the operation of the NASN stations. Also, gratitude
is due each of the 10 EPA Regions who since 1973 have participated in
this program by sending the high volume filters to the centralized
laboratory of the Environmental Monitoring and Support Laboratory for trace
metal analyses.
The personnel of the Analytical Chemistry Branch of the Environmental
Monitoring and Support Laboratory, EPA, North Carolina, are to be commended
for their diligent analytical efforts in producing the over 100,000 results
which have made this publication possible.
vi
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Section I
INTRODUCTION
The Environmental Protection Agency (EPA), with the assistance and
cooperation of state and local agencies, conducts a variety of air
sampling activities to obtain information about the air quality in the
United States. One such program, the National Air Surveillance Network
(NASN), has existed since 1953- The network has grown and undergone many
modifications since its beginning, especially during the 5 years covered
in this report. Table 1-1 catalogues these recent changes. The first
change, change in sampling schedule, was brought about to encourage
synoptic sampling with state/local ambient monitoring programs. The
second change, decentralization, was made to shift air monitoring expertise
from one centralized laboratory to 10 EPA regional laboratories. However,
one laboratory, the Environmental Monitoring and Support Laboratory (EMSL),
Research Triangle Park, North Carolina, retains a central function. Filters
are weighed at regional laboratories and forwarded to EMSL for analysis of
trace elements. As a result, the data on the concentrations of 11 metals
contained within this publication beryllium, cadmium, chromium, cobalt,
copper, iron, lead, manganese, nickel, titanium and vanadium -- have been
produced within one laboratory. Data on the concentrations of these 11
metals in suspended particulate matter collected at urban and nonurban
sampling sites during 1970, 1971, 1972, 1973, and 197^ are included in this
publication. Earlier publications of this type included concentration data
1
-------
for tin. However, recent recovery studies for these years indicate
that less than 20% of the spiked tin when applied to unexposed filters
is found upon analyses. Such information indicates that the tin data,
if reported, would be highly biased. This element, therefore, was
excluded from these listings.
SAMPLE COLLECTION
Samples are collected at approximately 300 urban and 35 nonurban
NASN sites located across the country. The urban sites are generally
located within a city or town or adjacent suburbs. The nonurban sites
are generally located in rural or remote areas. Although, with the
passage of time, many of these rural areas, especially in the northeast,
have become more heavily populated and thus are subject to direct
influences of spreading urbanization. Voluntary operation of each
site is maintained through the generous assistance of local or state
agencies and individuals such as park rangers, firemen, or policemen.
A more detailed description of each site is available.
Prior to 1972, 24-hour samples (beginning at midnight) were
collected according to a biweekly (26 samples per year) modified
random sampling schedule. The schedule was modified to insure equal
representation for each of the seven days of the week. Since 1972,
however, samples have been collected every 12th day (30 or 31 samples
per year). The initial sampling date was January 10, 1972. Since
Directory of Air Quality Monitoring Sites, 1971. U.S. Environmental
Protection Agency, Office of Air Programs. Research Triangle Park,
North Carolina. Publication No. APTD-0979- April 1972.
-------
that date, samples have been collected every 12th day. This sampling
schedule eliminates the need for redesigning a new sampling schedule
each year. In addition, it encourages concurrent sampling with other
networks. Most importantly, it is easily implemented in the field.
Beg inning with the 197^ samples, the responsibility for managing
2
the NASN was given to each of the 10 EPA regions. Prior to that time
one centralized laboratory located at Research Triangle Park, North
Carolina, weighed the high volume filters. This centralized laboratory
has continued to provide all of the trace element analyses of the high
volume filters although the system has been changed since the decentra-
lization. The regions now send the weighed filters to North Carolina
for routine trace substance analyses and storage in the filter bank for
non-routine, special analyses as needed. The resulting data are published
by the Statistical and Technical Analysis Branch (STAB) of the EMSL and
are sent to the National Aerometric Data Bank (NADB) for archiving.
2
Region I - Boston, Massachusetts
Region II - New York, New York
Region III - Philadelphia, Pennsylvania
Region IV - Atlanta, Georgia
Region V - Chicago, Illinois
Region VI - Dallas, Texas
Region VII - Kansas City, Missouri
Region VIII - Denver, Colorado
Region IX - San Francisco, California
Region X - Seattle, Washington
3
'Metals, non-metal inorganic ions and BaP,
-------
DESCRIPTION OF DATA TABLES
Data are presented as quarterly composite and yearly average, values
expressed in micrograms (nanograms in the case of beryllium) per cubic
meter of air at'standard temperature (25 Centigrade) and standard pressure
(760 mm of mercury). All valid data appearing for a given site are shown
for each of the 5 years. Quarterly composites are judged to be
representative and are included in the tables if there are at least five
valid filters per quarter. tn order for data to be reported for a quarter
in which one of these months lacks any valid samples, the other two months
in that quarter must have at least two valid samples. If "zero"
concentrations values below the analytical discrimination valueare
reported (shown as L.D. in the data tables), the yearly mean is calculated
by replacing the "L.D." with a value equal to one-half the analytical
discrimination value shown in Table 2-1. If two or more quarters within
a site year are below the analytical discrimination value, the yearly
average Is not calculated. Prior to the analysis of 1970 samples, the
general procedure was to analyze for trace metal concentrations only when
the entire year was valid, i.e., all k quarters were represented. This
practice meant that the tables were complete without blanks. This procedure
has been liberalized during the period since 1970 to allow for analyses
of any valid quarters for a given station even though the entire year may
not be represented.
Table headings contain an expression representing analytical quality.
The expression states a 35% confidence interval within which the expected
k
-------
"true" value of the reported value lies, based solely on analytical error.
For example, if a reported beryllium value is shown as 0.2 ng/m , the
expected "true" value is within 0.11 to 0.36 ng/m3, 95% of the time.
Further details pertaining to quality of data are given in the next section,
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TABLE ]-). NASN NETWORK CODIFICATIONS, 1970..-
Month/Year
Change
tropact
January 1972
December 1972
April 1973
December 1973
January
Sample schedule changed from
random biweekly to 12-day
systematic samples; first
sample collected 1/10/72.
Decentralization, Reg ion 11.
Decentralization, Region I,
Decentralization, Regions V,
V(l, VI I I, IX, X.
Decentralization, Regions III,
IV, VI.
All sites
NJ, NY, PR
CT, ME, MA, NH, Rl,
VT
IL, IN, MS, MN, OH,
Wl, |A, KS, MO, NE,
CO, MT, ND, SD, UT,
WY, AZ, CA, HI, NV,
AK, ID, OR, WA
DE, DC, MD, PA, VA,
WV, AL, FL, GA, KY,
MS, NC, SC, TN, AR,
LA, NM, OK, TX
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SECTION I I
QUALITY CONTROL
INTRODUCTION
Beginning with this publication, estimates of analytical performance
are given with each data table. This section presents the quality
control information which forms the basis for determining these analytical
performance limits and analytical discrimination limits.
UNEXPOSED FILTERS AND ANALYTICAL DISCRIMINATION LIMIT
Table 2-1 lists the average concentration of blank filters. The
blank value was determined by pooling a large number of clean (unexposed)
filters and reanalyzing this single extract a number of times throughout
the analysis period. Thus, an estimate of homogeneity of the lot of
filter blanks is not possible. However, the value as shown provides a
representative estimate, averaged over the 5 years, of the blank concentration
levels.
The yearly analytical "limit of discrimination" (LD) values are
also shown in the table. A single value for each pollutant/year for
both nonurban and urban samples is a departure from previous analysis
periods when a separate value was determined for the nonurban sites and
the urban sites. The LD is defined as the concentration value for a
single element which produces a signal that can be distinguished from
analytical noise at zero concentration 95% of the time. The LD is
-------
determined by constructing a tolerance interval (95%~95%) centered at
zero concentration. The analytical variability of the blank filter
extract is used as the estimate of variability for calculating the
tolerance interval. Prior to 1972, a slightly different procedure was
used, but for consistency, the average LD for each element determined
for the three years, 1972-197^, is reported for 197Q and 1971-
PRECISION AND BIAS
Table 2-2 presents precision and bias information together with 95%
confidence limits. All the data are expressed as percentages, a necessity
because precision is concentration dependent.
Precision has been determined two ways--the standard deviation of
relative percent difference between analyses of the same sample extract,
and the standard deviation of relative percent difference between analyses
of different extracts of the same filter. Clearly, the added variation
caused by cutting and extracting can be seen between the two columns.
As a result the estimate for precision in constructing the 95% confidence
limits has been taken from the "Different Extract" column.
Bias, expressed as an average percent difference between true and
observed, has also been determined two ways--with prepared standard
solutions run through only the analytical process, and through spikes
(addition of known amounts of an element to one of a pair of sample
duplicates) run through both the extraction and analytical steps. To
compare the two measures of bias, the recovery averages should be subtracted
from 100%. The bias term preceeding the confidence limit expression has
been taken from the recovery information. It provides a measure of both
the. accuracy of the extraction process as well as the analytical process,
8
-------
although it does contain an indeterminate error associated with the
spiking process.
PERFORMANCE QUALITY ASSESSMENT
Precision and bias estimates discussed above have been combined to
form what is termed "Analytical Quality." A quarterly composite value
appearing In the,data tables based on the estimates of bias (recovery)
and precision (duplicate or different extracts) is expected to be
analytically correct within the 35% confidence interval. To apply the
confidence interval to a given datum point, one should multiply the
value by 100 percent plus the bias percent and to this value, add and subtract
the value times the percent associated with the precision term. For
example, the first beryllium value above LD in Table 5-1, is 0.2 ng/m ,
with a stated analytical quality of 16%^62.4%. The confidence interval
is constructed as follows:
Upper Limit = (1.16 + .624) (0.2) = 0.36 ng/m , and
Lower Limit = (.1.16 - .624) (0.2) = 0.11 ng/m .
These estimates only include sample preparation and analytical variability
for an average of duplicate analyses. Furthermore, if additional
information were known concerning variation due to factors such as
sampling, then these confidence intervals would be wider. As a result,
all confidence limits are underestimates for the total variability of
the sampling and analytical processes.
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TABLE 2-1. BLANK FILTER CONCENTRATIONS AND YEARLY ANALYTICAL
DISCRIMINATION VALUES (yg/mj)
E lement
Beryl] i urn
Cadmi um
Chromi um
Cobalt
Copper
1 ron
Lead
Manganese
Nickel
Ti tani um
Vanadi um
Blank Fi Iter
Concentration
.0006
LD**
.004
LD
.007
.18
.02
.007
.005
.068
LD
Analyt icai
1970
.00005
.00023
.00071
.00069
.0011
.0082
.022
.00040
.0014
.0039
.0021
1971
.00005
.00023
".00071
.00069
.0011
.0082
.022
.00040
.0014
.0039
.0021
1 Discr iminat icn Values
1972
.00004 -
.00019
.00062
.00052
.0012
.0059
.015
.00024
.0012
.0032
.0017
1973
.00007
-00027
.00080
.00076
.0010
.010
.029
.00055
.0017
.0045
.0025
1974
.00008
.00036
.00084
.00063
.0012
.010
.014
.00064
.0019
.0061
.0028
>)jg/m are obtained by multiplying Mg/mL by a factor to convert to
total ug/fliter and dividing by an assumed air volume of 2500 m .
;LD is below the Analytical Discrimination Limit.
10
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TABLE 2-2. ANALYTICAL PRECISION, BIAS AND CONFIDENCE LIMITS
Element
Be
Cd
Co
Cr
Cu
Fe
Mn
Ni
Pb
Ti
V
Precision, % Bias
Same
Extract
Std.
No. Dev.
NA
228 10.73
NA
1536 ^2.29
2035 3-60
2138 9-07
2008 11.14
698 19.69
2032 5.59
1791 19.2
536 11.65
Different
Extract
Std.
No. Dev.
20 31.23
41 22.72
20 29-15
56 21.43
58 19.27
54 19-04
40 20.51
26 20.67
48 22.55
56 14.93
16 20.23
Standards
Std.
Mean Dev.
0.0 4.5
8.7 7-1
13.7 14.7
0.7 3-4
- 2.7 2.5
- 6.3 3-0
- 2.3 1.0
0.3 2.5
0.7 5.4
0.3 3.4
8.3 6.6
Recovery
s
x Std.
Mean Dev.
84 6.0
91 13.5
86 9.9
79 17-9
72 24.9
75 6.7
71 10.4
79 15.2
86 12.9
58 18.8
79 14.5
95% Confidence
Limits, %
16 +_ 62.4
9+45.44
14 + 58.30
21 +_ 42.86
28 +_ 38.54
25 ± 38.08
29 + 41.02
21 + 41.34
14 + 45.10
42 + 29.86
21 + 40.46
NA = Not available, most sample pairs are below the LD.
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SECTION III
LABORATORY METHODS
SUSPENDED PARTICIPATE MATTER
The mass of particulate matter per volume of air is determined by
drawing air through a preweighed glass-fiber filter with a high volume
(hi-vol) air sampler and then weighing the soiled filter. In order to
obtain the flow rate, a calibrated rotameter is read at the start and
finish of the sampling period, and the averaged value is used with a
calibration table for that rotameter. The known sampling period (2k hours)
and the measured flow rate allow for calculation of the volume of air
samp]ed.
The hi-vol samplers, operating at approximately 1.7 cubic meters
per minute, collect particulate matter from about 2500 cubic meters of
air during the 24-hour sampling period. The filters used are 20.3 by
25-4 centimeter flash-fired glass-fiber filters, selected for low and
uniform background concentrations of those substances to be measured.
As a precaution against pinholes or other flaws that could affect
air flow, the filters are screened for imperfections on a light table.
Prior to weighing, the filters are equilibrated for a minimum of
24 hours at a temperature of 24° Centigrade and a relative humidity of
50 percent or less. Because any crease in a filter can seriously affect
the air flow, filters are weighed with a balance that permits weighing
without bending.
12
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The filters are then distributed unfolded to the cooperating local
agencies for the urban sites or to the designated participant responsible
for operating the nonurban site. After sampling, the filters are folded
in half with the collected participate matter inside. They are then
returned to a laboratory. The filter with the collected particulates is
again equilibrated for at least 24 hours at a temperature of 24 Centigrade
and a relative humidity of 50 percent or less, after which they are
weighed to determine the amount of particulate matter that was collected.
METALS
In the analysis for metals, a 2.5 by 18.0 centimeter strip is cut
from each filter. The length of each strip is determined by the number of
filters included in the quarterly composite. (The total area is fixed
at 113 square centimeters.) For example, if there were 5 valid samples
in a quarter, a strip approximately 9 cm long would be cut from each filter.
The 5~8 strips for the quarter are composited and ashed in an oxygen plasma
to oxidize organic material. The metals are then extracted by refluxing
for 3 hours with a mixture of nitric and hydrochloric acids.
Quantitative analysis is accomplished by measuring the intensity of
the emission line for each metal as the sample is excited in an optical
emission spectrometer, and by then comparing these measurements with a
calibration curve obtained with standard concentrations. Beginning in 1970,
each reported result is the average of two determinations made from the
same composite extract at different times. If a particular element were
found in both determinations, results were averaged. When the element was
found in only one of the determinations, it was regarded as noise, and no
detectable quantity was reported. The present emission spectrometer provides
13
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a general overview of the metals' concentrations. However, the present
instrument Is not considered to be as sensitive or precise a method as a
specific determi nation ..method for a single element, such as in the case of
determination of lead by atomic absorption. The emission spectrometer
method does indicate the relative order and the general level of metals'
concentrations occurring in various urban and nonurban areas of the
United States.
Data for samples collected prior to 1966 may not be directly comparable
to the results presented in this report because samples taken from 1957
through 1965 were ashed in a muffle furnace at 500 Centigrade, causing
the loss of varying amounts of the elements. This deficiency has been
corrected by ashing in an oxygen plasma.
-------
Section IV
NATIONAL SUMMARY OF AIR QUALITY MEASUREMENTS
The data in Tables 4-1 and 4-2 are cumulative frequency distributions
by element of all quarterly results by year for urban locations and
nonurban locations respectively. Consider for example the line for urban
1974 lead. The first number, 594, gives the.number of site quarters of
lead data for the year. The next entry, minimum, is the lowest urban
site quarter result of 0.08 yg/m . Other entries, such as 1.61 under
the 90th percent Me column, are to be interpreted such that 90 percent
of the 594 site quarters (535) were equal to or less than 1.61 yg/m .
The usual descriptive statistics, means and standard deviations
(arithmetic and geometric) are shown in the last 4 columns. Comparisons
among years within a pollutant provide a relative indication of trends.
For example, lead values across the country appear to be decreasing--not
only on the average but also for all percent! les of the frequency
distribution shown in Table 4-1.
15
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TABLE 4-1. URBAN NATIONAL CUMULATIVE FREQUENCY DISTRIBUTIONS
Ari thmet ic
Element
Beryl 1 ium*
Cadmi um
Chromi um
Cobalt
Year
1970
1971
1972
1973
197^
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
No.
787
742
708
559
594
797
717
708
559
594
797
717
708
559
594
797
717
708
559
594
Min.
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
10
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
30
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
.001
LD
.003
LD
LD
LD
LD
LD
50
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
.006
.007
.004
.004
.005
LD
LD
LD
LD
LD
70
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
.009
.010
.006
.007
.007
LD
LD
LD
LD
LD
90
0.2
0.2
LD
LD
LD
.008
.010
.007
LD
.006
.017
.019
.011
.015
.012
LD
LD
LD
LD
LD
95
0-3
0-3
LD
LD
LD
.012
.017
.011
.007
.009
.024
.026
.017
.023
.015
LD
LD
LD
LD
LD
99
0.6
0.5
LD
LD
LD
.027
.059
.034
.012
.022
.046
.057
.040
.074
.035
LD
LD
LD
LD
LD
Max.
2.9
0.7
LD
LD
0.2
.099
.295
.112
.032
.077
.130
.171
.143
.228
.073
.014
.085
.042
.027
.029
Mean
LD
0-1
--
LD
LD
.003
.004
.002
.001
.002
.008
.009
.006
.007
.006
LD
.001
LD
.001
LD
Std.
Dev.
0.2
0.1
.007
.016
.007
.003
.005
.011
.014
.010
.015
.006
.001
.003
.002
.002
.001
Geometr i c
Mean
0.01
0.03
--
LD
LD
LD
LD
LD
LD
LD
.006
.008
.004
.004
.005
LD
LD
LD
LD
LD
Std.
Dev.
4.91
3.22
--
4.40
5-21
4.97
4.89
4.90
2.80
2.97
3-17
3.62
2.37
3-11
7-05
5.97
4.45
4.85
'-Expressed in ng/m"
(Conti nued)
-------
TABLE 4-1 (Continued)
Arithmetic
El ement
Copper
1 ron
Lead
Manganese
Nickel
Year
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
No.
790
715
706
555
590
796
717
708
558
594
797
717
708
559
594
795
716
708
559
594
797
717
708
559
594
Min.
LD
LD
LD
LD
LD
LD
LD
LD
LD
.1
LD
LD
LD
LD
.08
LD
LD
LD
LD
LD
,001
.001
.001
.001
.001
10
.04
.04
.03
.03
-04
.6
.8
-5
.4
.4
.47
.42
.46
35
.36
.02
.02
.01
.01
.01
.001
.001
.001
.001
.001
30
.06
07
.06
.06
.08
1.1
1-3
.8
-7
7
.75
71
-72
-58
-57
.03
.04
.02
,02
.02
.001
.001
.001
.001
.001
50
.10
.10
.09
-09
.11
1.4
1.7
1.0
9
.9
1.05
1.01
-97
-77
.75
.04
.05
-03
.02
.02
.001
.001
.001
.001
,001
70 90
.16 .32
-18 .37
15 -35
.14 .34
.17 .36
1-9 3-2
2-3 3-6
1.4 2.2
1.2 1.9
1.2 1.9
1 .37 2.01
1.42 2.21
1-25 1-93
1 .05 1 -62
1 .00 1.61
.06 .15
.07 .16
.04 .09
.04 .07
.04 .07
.019 -045
.018 .045
.013 .031
.013 .036
.012 .026
95
.50 .
-59 1-
.49 1.
.45 .
51
4.2 6.
4.9 8.
2.8 4.
2.6 3-
2.4 3.
2.59 4.
2.86 4.
2-57 3-
2.08 3.
1-97 3-
-23 -
.24 ,
.12 .
.11 .
.11 .
.066 .
.064 .
.045
.066 .
.034 .
99
99
28
00
79
78
4
1
1
8
9
14
38
69
03
16
49
46
22
29
21
127
126
100
133
057
Max.
1.51
1-56
1.57
1.44
1.33
14.2
16.0
6.4
6.9
6.2
5.83
6.31
6.88
5-83
4.09
2.10
1.95
.86
-56
^35
-277
.347
.268
.439
.639
Mean
.15
.18
.16
.15
.17
1-7
2.1
1.2
1.1
1.1
1-19
1.23
1-13
92
.89
.07
.08
.04
.04
.04
.015
.015
.011
.014
.009
Std.
Dev.
.18
.22
19
17
.16
1-3
1.6
.8
.8
.7
.80
.87
.78
.64
.57
.12
.11
.06
-05
.04
.028
.028
.023
.037
.029
Geometr i c
Mean
.10
.11
.10
.10
.12
1.38
1.65
1.04
-89
.89
-99
1.00
.93
-76
.75
.04
.05
.03
.02
.02
.01
.01
.01
.01
.001
Std.
Dev.
2.57
2.62
2.60
2.49
2.26
98
98
.83
-89
.87
1.84
1.89
1.87
1.87
1.80
3.13
2.81
2.76
2.72
2.39
3-41
3-34
3-55
4.19
4.60
(Continued)
-------
TABLE 4-1 (Continued)
Ari thmet ic
Element
Ti tan ium
Vanad i urn
Year
1970
1971
1972
1973
197^
1970
1971
1972
1973
1974
No.
797
716
707
559
593
795
718
708
559
594
Min.
LD
LD
LD
LD
LD
.001
.001
,001
.001
.001
10
.02
LD
LD
LD
LD
.001
.001
.001
.001
.001
30
.03
LD
.02
.02
.02
.001
.001
.001
.001
.001
50
.04
.03
03
.04
-03
.001
.001
.001
.001
.001
70
.06
.05
.05
-05
05
.029
.026
.001
.001
.001
90
09
.09
.08
.08
.07
.162
-117
-075
.057
.058
95
.12
.12
.10
.10
-09
.244
.204
.100
-077
.083
99
.18
.20
.14
.14
.14
.544
.496
.195
.151
.185
Max.
.26
.51
.48
.23
.22
1 .222
1-325
.858
-393
.248
Mean
.05
.04
.04
.04
-04
.052
.041
.022
.016
.019
Std.
Dev.
.03
-05
.03
-03
.03
.116
.108
.056
.034
-037
Geometric
Mean
.04
.02
.03
-03
.03
.020
.014
.006
.005
.006
Std.
Dev.
1.85
2.66
2.21
2.01
2.06
3-82
4.20
4.06
3.68
3-51
00
-------
TABLE 4-2. NONURBAN NATIONAL CUMULATIVE FREQUENCY DISTRIBUTIONS
Arithmetic
El ement
Bery 11 ium*
Cadmium
Chromium
Cobalt
Year
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
No.
124
97
137
100
79
124
97
137
100
79
124
97
137
100
79
124
97
137
100
79
Min.
LD
LD
LD
LD
LD
.0001
.0001
.0001
.0001
.0002
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
10
LD
LD
LD
LD
LD
.0001
.0001
.0001
.0001
.0002
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
30
LD
LD
LD
LD
LD
.0001
.0001
.0001
.0001
.0002
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
50
LD
LD
LD
LD
LD
.0001
.0001
.0001
.0001
.0002
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
70
LD
LD
LD
LD
LD
.0001
.0001
.0001
.0001
.0002
LD
.005
.002
.001
.002
LD
LD
LD
LD
LD
90
LD
LD
LD
LD
LD
,0001
.0001
.0001
.0001
.0002
.007
.007
.005
.007
.005
LD
LD
LD
LD
LD
95 99
LD .24
LD .16
LD LD
LD LD
LD LD
.0001.0001
.0001 .0001
.0001.0001
.0001.0001
.0002.0002
.017 .042
.011 .034
.006 .009
.017 -039
.008 .009
LD LD
LD LD
LD LD
LD LD
LD LD
Max.
.24
.24
LD
LD
LD
.0001
.0001
.0001
.0001
.0002
.075
.061
.039
.066
.009
LD
LD
LD
LD
LD
Mean
LD
.01
LD
LD
LD
.0001
,0001
.0001
.0001
.0002
.003
.004
.002
.003
.002
LD
LD
LD
LD
LD
Std.
Dev.
-03
.03
. 0000
.0000
.0000
.0000
.0000
.009
.007
.004
.009
.002
--
"
--
--
Geometr i c
Mean
LD
LD
LD
LD
LD
.0001
.0001
.0001
.0001
.0002
LD
LD
LD
LD
LD
LD
LD
LD
LD
LD
Std.
Dev.
7-62
6.10
--
1-00
1.00
1 .00
1.00
1.00
1.00
4.60
3.48
3.58
4.16
2.67
--
--
--
--
--
(Continued)
*Expressed in rig/m .
-------
TABLE 4-2 (Continued)
Arithmetic
Element
Copper
I ron
Lead
Manganese
Nickel
Year
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
No.
124
96
137
99
78
124
97
137
99
79
124
85
137
100
79
124
97
137
100
79
124
97
137
100
79
Min.
.001
.014
.001
.011
.023
LD
.07
LD
.01
LD
.003
.003
.007
.015
.007
LD
LD
LD
LD
LD
.001
.001
.001
.001
.001
10
.029
-029
.025
.035
.039
.13
.18
.05
.02
.04
.003
.003
.007
.015
.007
.003
.003
LD
LD
LD
.001
.001
.001
.001
.001
30
.056
.086
.058
.075
.081
.22
-27
.12
.11
.12
.003
.003
.007
.015
.053
.006
.009
LD
LD
.001
.001
.001
.001
.001
.001
50
.081
.141
.116
.119
.124
-32
.43
.19
.16
-19
.003
.003
.107
.058
,087
.012
.013
.003
.002
.004
.001
.001
.001
.001
.001
70
.164
.208
.193
.219
.238
.45
.63
31
.21
.28
.003
.003
,166
.132
.141
.018
.022
.007
.004
.007
.001
,001
.001
.001
.001
90
.342
495
377
.440
.461
.68
.90 1
.56
.34
-47
.267
.127
.294
.233
.221
.035
.032
.016
.009
.017
.019
.001
.009
.014
.001
95
.526
.648
.660
571
.643
.85
.04
.68
-47
.55
-383
.204
392
.392
317
.041
.041
.029
.011
.023
.024
.001
.015
.059
.006
99
1.053
.785
.804
.849
.860
1.58
1,52
1.06
.88
-65
.628
.783
.950
.698
.496
.066
.064
.039
.022
.027
.076
.046
.076
.188
.020
Max.
1-195
.880
.812
.983
1.147
1.62
2.80
1.15
1-19
.69
1.471
1.134
1.048
.939
.534
.068
.102
.046
.030
.033
.097
.083
.082
.280
.026
Mean
.158
.205
.178
.196
.208
-38
.51
-25
.19
.24
.088
.047
-139
.110
.111
.015
.018
.007
.004
.006
.005
.003
.004
.011
.002
Std.
Dev.
.188
.196
.183
.196
.210
.27
.38
.22
.18
-17
. 190
.155
.169
.149
.111
.013
.015
.009
.005
.007
.014
.011
.012
.037
.004
Geometric
Mean
.081
.150
.116
.138
.147
-31
.41
-19
.14
-19
.040
.008
.090
.068
.083
.012
.013
.003
.002
.004
.001
.001
.001
.001
.001
Std.
Dev.
2.56
2.24
2-33
2.30
2.31
1.90
1.95
2.11
2.19
1-92
3-72
4.80
2.59
2.77
2.30
2.11
2.09
2.81
2.79
2.52
4.58
5-28
4.64
4.93
3.62
(Continued)
-------
TABLE 4-2 (Continued)
Ari thmet ic
Element
Tt tan ium
Vanad i urn
Year
1970
1971
1972
1973
1974
1970
1971
1972
1973
1974
No.
124
97
137
100
78
124
97
137
100
79
Min.
.002
.002
.002
.002
.003
.001
.001
.001
.001
.001
10
.002
.002
.002
.002
.003
.001
.001
.001
.001
.001
30
.007
.002
.011
.012
.003
.001
.001
.001
.001
.001
50
.011
.002
.024
.027
.016
.001
.001
.001
.001
.001
70
.015
.028
.038
.040
.026
.001
.001
.001
.001
.001
90
.023
.042
.054
.054
.043
.021
.001
.001
.001
.001
95
.028
.059
.069
.068
.049
.035
.036
.025
.001
.001
99
.047
.065
.081
.076
.053
.112
.004
.047
.028
.021
Max.
.093
.069
.092
.084
.066
.112
.209
.205
.035
.023
Mean
.013
.017
.027
.028
.020
.008
.007
.004
.002
.002
Std.
Dev.
.011
.020
.022
.021
.017
.019
.024
.019
.005
-004
Geometric
Mean
-Oil
.010
.024
.024
.014
.001
.001
.001
.001
.001
Std.
Dev.
2.15
2.54
2.04
1.93
2.09
4.04
5.04
5-77
3-88
3-36
-------
Sect ion V
DATA TABLES
22
-------
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"OLLUTANT : I'laS - RFRYLLTUM
METHOD : HI-VOL "^MISSION SPFCTRA ILOH TrHP ASH)
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fOLLUTANT : 17105 - RFRYLLlUI
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28
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POLLUTANT ; 17105 - KF»YLLTUM
METHOD : HI-VPL rHissio*! SPCCTRA
UNITS t NO/ru HFTFR 17"; ri
OATA'TYPF : OUAP.TFRLY'COMPOSITE
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29
-------
POLLUTANT : 12105 - SFRYLLTUM
METHOD : HI-VOL FHTSSTDN SPFCTRA 67.1»1
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"OLL1JTANT : 17105 - nFPVLLTUM
METHOD ! HI-VOL rMTSSTON IprrTR* ILOM Trxp A'H)
UNIT"; : N0/r;u MFTrP. ( 2" r)
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"OLLUTANT : 17105 - BFRYLLTUH
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POLLUTANT ; l?uo - r
METHOD : HT-VOL rMTSSTON SPrrTRA (LOW TEMP «SH>
UNITS IJO/CUI MFTFR [71; (-1
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PPLLUTftNT ; j:»iiu - r-ApMTUM
M£TH"n : HT-VOL FHT^^TON SPFI:TPJ
UNITS : DC/nil MFTFR (7f rl
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41
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POLLUTANT : 17110 - r»PMTUM
METHOD ; HI-vnL rKTSSTOM SPTTRA IL1W TFMP ASHI
UNIT"; : un/rii MFTF" I?B <>
OATA TYPT : HUA^TC-RLV POMPOSTTF
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42
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"OLLUT«NT : 17110 - CADMIUM
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UNIT-; : us/cu MFTFP 12* M
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-------
POLLUTANT : 1711? - CHROMIUM
KETHOn J HT-VOL FMTSSTON SPECTRA (LOU TFHP ASHI
UNITS ; uis/ru METFR 17* n
OAT« TYPF : QUARTERLY COMPOSTtf
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POLLUT.ANT : i?n? - CHROMIUM
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UNITS r UR/ru MFTF" (»« ri
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POLLUTANT
METHOD T HI-VOL tMISSTON SPFCTRA (LOW TFMP
UNITS : us/cu MF.TF.R 175 c)
n»T« TYPF : QUARTFRLY TOHPOSTTE
PROJ. CLASSIFTCATTON : URBAN
LOWER DISCRIMINATION LFVFL (Ln)
ANALYTICAL
t
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1
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t
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LOCATION
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SPBINnFTELO
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49
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"OLLIJTANT r 1?H7 - CHPOMTIIM
"FTHon : HT-VOL FMISSTON <-prcTR« (tow TFHP
UNITS t Dti/rll MFTFP t71 f)
DATA TYPF r 'HURTFUL/ POMPOSTTE
ppnJ. rLflSSIrlr«TTON - IIRBIN
ANALYTICAL QUALITY : 71H-IH7.SG1
OISCRTHT.HATION LFVFL ft fl
7o - .nnn7
71 - .nnnT
72 - -nnos
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1
1
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METHOD : Hl-VOL tt-^SlON SPFrTRA ILOM TrMP ASHl
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"OLLUT»NT
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61
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POLLUTANT : i7ii-» - COBALT
MEiHtm : HT-VOL ^MISSION SP«TTR« ILOK TFMP ASHI
UNIT1; : UG/CII MFTFR frx r.1
DATA TYPF ; miARTFRLY rO
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70 - .0007
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POLLUTANT : 17113 - COBALT
METHOD : HI-VOL rMTSSTON SprrTRA (LOW TFMP ASH)
UNITS : UG/CU HFTFR tzs c>
DATA TYPE : OUARTFRLY COKPOSTTF
PROJ. cLASSIrlcATTON URn«N
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POLLUTANT : 1711T - rOBALT
METHnn : HI-VOL FMTSSTON sprrTRA ILOH TFMP «SH)
UNITS : uG/ru MFTFP < 2* r)
DATS TYP*- ; QUARTERLY COMPOSITE
PROJ. rLASSlFTK«TTON : URBAN
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POLLUTANT : 17113 - rrORALT
METHOD : HT-VOL FHTSSTON SPFCTRA ILOH TEMP «SHI
UNITS : UB/CU MFTFR izs ri
DATA TYPF : OUARTFRLY COMPOST'TF
PROJ. CI.ASSlfTCATTON : URBAN
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POLLUTANT : t'ln - COBALT . . :.
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METHOP : HI-VOL FMTSSTON
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POLLUTANT ; T>13? - MANGANFSr
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LOCATION
NFU HFXTCn
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SITE IIGI
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-------
POLLUTANT ! 1713? - MANPANFSF
METHPn : HT-VOL FMTSSTON SPrrTRA HOW TFHR «SH>
UNIT-; : un/cu KFTFR 175 n
DATA TYPF : OIIARTFRLY COMPOSTTF
PROJ: nLASSTFTrATTON ; uRi«N
ANALYTICAL. OU«LTTY : ?9l»->4l.07J
LOWER OTSCRIMINATTON LFVL (L P>
70 - .nnn
71 - -non
72 - .nnn
73 - .nnl
71 - .nni
! LOCATION
PNORTH CAROLINA
.'NORTH
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F STTE 001
FOHIO
T AKRON
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nni
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LOCATION
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-------
POLLUTANT : 1717.7 - "ANGANt-SF
METHOD : HI-vnL rMTSSTON SPrrTRA II.IH TFMP ASHI
UNIT"; : uo/ru MFTFR {?*. r\
DATS TYPF : QUAPTFRLY COMPOSITE
PRPJ. cLasslFTciTTON : URPAN
AHALYTIPAL OUALTTY ! 7q( +-) 1] .07?
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LOCATION
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POLLUTANT : 12136 -
METHon : HI-VIL
UNITS : ur./r.u MFTFR i?s >'
DATA TYPF : QUARTERLY COMPOSITE
PPOJ. russlFirATTON : URPAN
ANALYTICAL QUALITY ! 7.1 ( -f- 111 .311
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POLLUTANT :
MFTHnn ; HT-vnL rMTSSTON SprrTRA (LOW TFMP
UNTTs LiP/ru HFTD I ?; ri
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POLLUTANT : 1213S - NTCKFL
METHOD : HI-VOL FHTSST.ON SPrrTRA ILOH TEMP ASH)
UNITS : uc/ru MFTFR (75 >-i
naTA TYPF - OUARTFRLY rOMPOSTTF
PROJ. CLASSTFTCATTON UPniti
ANALYTICAL DUALITY : 7", It-mi.311
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POLLUTANT : T>136 - NTI-KrL
METHOD : HI-VOL rMTSSTON SPrcTRj
UNITS : IIP/PI) MFTF9 I 75 <'
p«T4 TYPF i OUARTFRLY I-OMPOSTTF
°POJ. CLASSI^TCATTON : IJOntN
AN5LYTTPAL QUALITY '. 2U+-I11.31J
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LDUER OTSPRIMINATTON LFVFL (L"1
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"OLLIITHHT : 17136 - NrrKrL
HETHOD : HT-VOL FMTSSTON SPTTRA mow TrHp ASH)
UNITS r uR/rll MFTFR (?; r)
DATA TYPE : OUAPTF°LY TOMPOSITF
POOJ. |-L«SSIrT<;ATTON URBAN
ANALYTICAL OUALTTY : 7if+-ni.ii>
LOWER OTSrRTMIMATTON LFVL (L "I
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LOCATION
IRPINlA
RICHMOND
STTE 002
ROAMOKF
SITE oil
ASHINGTON
SFATTLF
STTF 001
SPOKANE
STTE 001
T AC DMA
STTE noi
EST VIRGINIA
CHARLESTON
STTF DPI
HUNTING TON
STTF pni
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SITF 005
SOUTH CHARLESTON
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STTF U01 ' 7n i .03 .00 ' -07 F .03 F
71 i .OS ! .PZ F .P6 F .00 t
! 77 ' .07 ! .02 ' ' .02 F F
i 77 i i .03 ' LD F ,.n** f
70 .01 F .03 F LP LO »
* i i * i
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ALTFO"NTA IF F i ! 1
ANAHFTM IF1' F
STTF 001 ' 7P F .Oq F .11 ' .12 F .10 F
F 71 .13 F .10 F .oq .07 r
77 F .04 F .08 F .06 .11 '
F 73 i .0 8 F .07 F .Oq ! ?
F 74 .05 F .03 F .06 .10
ii i i F f
1F8KFLEY F F F '. r
STTF Oil F 70 F .07 i .T3. F .PS F
i 71 F LO LO
i 77 ' .05 F .01 F .02 .00
i 73 F .D« F .11 i .0" .06
71 F .OS F .02 F .04 F .P3 I
ii i i i *
ii i
R1IRRANK F 1 ! F !
STTF 002 F 70 i .07 ! .11 i .1= .07
' 71 F .11 F .17 .IB F .11
! 77 .06 ! .06 F LO LD
73 i .06 F .Oq F .73 ! .11 f
i 70 ' .07 F .07 F .04 ! .C9 F
ii i i i
11 i i
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STTF U02 F 70 .07 F .P7 F .15 ,H9 >
F 71 ' .03 .10 F
I 77 F in F .06 .02 F .OR '
i 7' F .10 F .11 .12 ! .11
i 71 .06 ! .05 F .17 ! .11 '
11 I i F
PLFUnALE F ' F F . '
STTF Ml F 7n F .06 ! . OK F ' .Oq ! .06
71 F .07 F .04 F .07 F .10 f
I 77 ' .05 F .08 F .01 '. .P6
F 73 F .07 ' LP ! .06 F ~ LD r
i 71 ' .04 F .02! F
ii i ' *
LONG WTACH ! F »
>;TTF oni 70 .08 F ,PB .aq F .07
i 71 F .01 F .05 ' .06 F .01
77 ' .01 ! -ri F .05 .01
i It F .01 ! .07 " '
! 70 F .11 F .07 F .10 ! .10
LOS ANGELES ! F F F !
STTF nni " 70 .09 F .08 F .11 F ,P6
i 71 .04 F .T1 F .03 ' .09
77 i .13 ! .07 F .12 ' .M
71 F .07 F .02 F .12
'. 70 F .01 ! -Pfi '- -OB F .10
it i ' i
ii T
OAKLAND F ' F '
STTE ooi 70 ' .07 i .03 F ,ns -PS
! 71 F .01 F LP F LB F LD
77 F .01 F .02 .02 F .01
F 73 F .01 F .PI .02 F
F 71 F .07 ! ."7 .CF ! .OB
II 1 r i
ONTAHTO F F ' F F
STTF am ' 70 F .09 ! .12 J .21 ! .17
i 71 F .13 ! .11 F1 .70 I .13
! 77 .10 F .06 .06 ' .10
i 73 .06 F .OB '
74 F .OS .21 F
.027
-P3P
.104
.100
.072
.059
.021
.071
.035
.101
.138
.120
.058
.094
.039
.118
.103
.P67
.157
.058
.P73
.048
.042
.10?
.087
.051
.099
.072
.033
.01
.04
.13
.14
.08
131
-------
POLLUTANT : 171R1 - TTTANTUM
METHOD : HT-VOL FMTSSTON SPrrTRA (LIU TrMP ASH)
UNITS : un/cu KFTFR i?s "i
DATA TYPF : QUARTERLY POMPOSTTF
PROJ. CLASSIFICATION : I|P°«N
ANALYTICAL QUALITY ; «?(4) ?q.RG)
LFVL H p>
r
i
! LOCATION
i '
f
^CALIFORNIA
! PASflOfTNft
! STTE nni
f OASADF.NH
f S^TE: on?
»
f
?
i
! RIVEPSlnF
j "?ITE n^i
i
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;
! SAC^flMENTQ
f ^irr nni
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!
!
t
! SAN RFflK'ARDTMO
.' ^TTE nni
!
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;
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! srrr pni
»
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!
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! SAN FRAMfKr^
f STTE nni
!
!
!
*
9
t SAN josr
F STTE OH2
f
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f SANTA *p)A
f ^TTE nni
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f
j
!
f T03RAMCE
1 ^TTE noi
!
T
;
>
fCQLORADO
! DENVER
r SITF nnj
F
!
r
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!
f
""f I-
! i
! YP.!
! !
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! 71 !
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' 71
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r 71 r
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! 71 f
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70 - .001
71 - .001
72 - .nn3
73 - -.005
71 - .one
LOCATION
HARTFORD
STF 001
NF.H HAVEN
STTF ool
WATEOBURY
STTF GUI
OFLAWARE
N FW APK
STTF ciol
WILMINGTON
STTF 003
nTSTPTCT OF POI.'IMni
W AS HT NO TO N
STTF UOl
FLO°TnA
JACKS ONVTLLF
STTF un2
MIAMI
STTF U02
c- T PrTfR^PUQQ
STTF UQ2
TAMPA
STTF nn2
n r« P'lTA
ATLANTA
STTF UOl
r
' 1
YP.F
r
73 F
71
r
t
70 '
71 '
72
73 F
71 '
i
r
7n
71
73 '
71 F
t
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70
71 '
77 '
7T f
7"
i
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70 '
71 '
77 >
7* '
71 '
t
i
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71 F
77 F
73
71
I
F
1
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71 '
77 I
71 '
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70 '
71
77
73
71 '
i
i
70 F
71
77 F
73 F
71 '
r
r
70
71
77
73 F
71
i
r
7n F
71
77 F
73 '
71 '
F
1
i
70 '
71 '
77 1
T*
71 '
r
t
ST. F
OTR. F
I
.06 F
.01
t
f
.01 F
.OG
.10 F
.10
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i
f
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-OB F
.07 F
i
i
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.09 '
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Ln '
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f
.01 '
.01 !
.01 '
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.01
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.11 '
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-D7
in
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*
.03 F
.01 F
.07 F
LO
i
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in F
1.0
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1.0 F
.03 F
in i
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Ln F
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.rs F
r
F
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10 F
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F
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f
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.05 '
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F
1
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1
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1
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1
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LH !
.05 '
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f
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1
1
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i
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r
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.02
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f
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1.0 F
f
1
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.03 F
t
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i
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F
1TH. '
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r
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r
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»
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.08
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i
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t
r
r
f
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.01 '
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LD F
»
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.03 '
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r
r
r
r
.02 '
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LD
.03 '
LD F
1
r
LO F
LO '
.P7
t
LD F
t
r
.01 '
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LO '
r
LO
r
1
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F
.07 '
. P"7 '
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»
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.01
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LD
YR.
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.015
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.P67
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.018
.015
.011
.012
.030
.011
.016
.071
.017
.PIT
.055
132
-------
LOWER DISCRIMINATION LFVFL ILT>I
POLLUTANT : 17161 - TTTANTUM 7Q
METHOD : HI-VOL fMTSSTON <"PrrTRA 79 .« 6' ._ ______
i
! LOCATION
t
GEORGIA
! OOLUMBUS
SITE 001
t
i
i
i
i STTE nni
i
i
;
FHAWAIT
! HONOLULU
! SITE oni
!
t
IDAHO
i
i
JILLIMOIS
i CHICAGO
STTE nni
i
i
i
EA*T ST LOUIS
r STTE noi
1
i
EAST <5T LOUIS
! t-TTE onu
SITP oni
i
i
i
i
! HOLINE
SITE DPI
I
i
! NORTH CHITA'S
STTE nnz
\
i
i
i
! PEOPlA
! <-TTF nni
1
,
ROCKFPRO
STTE Onl
!
i
i
"7-- "" -."«-- -- , ,
! ! 1ST. 7Nn. ! 3RO. 1 1TH. ! YR . !
YO.! CSTP.F 1TR.I OTR.I OTP.I AUG.
;;,,.!
, i i F
70 ! .01 ! -01 ' -01 -07 ' .037 !
71 i .ns .01 LD i Ln |
73 ' In' In3 ' .02 .01 .026 '
7« ! .03 ' Ln F .01 ! !
ii i ii '
'itl 1 ^ f * ' *
-i __ , p Q i QY » « n ^ * «n7^
71 ! Ln LD LI ' LO !
. 77 ! ! .07 ' .1)3 ' '
77 i ,ns F .17 ' -05 ' '
, 1 I I !'
! ! ' ' ' '
II 1 1 1 F
i 7n ! .on .ns ! .05 ' .os ' -uss
' 71 1 .09 ! .07 ' .07 ' .08 .077
i 7- ! i .01 .a* ' .01 '
T> ! .OP ! .05 i .05 F .02 ! ."13 !
71 ! .03 .01 -02 ' .03 .U30 1
ii i i
i ' i i i ' ' '
i ! ' ' ' !
i 70 ' ,n? ! O1' ' -07 ' .OS -061 !
i 71 ! .01 ! .05 .11 ' -05 ' .OT2
! 77 ' .ns F .07 ! .07 LH C .019 '
73 ! .0' ! -Ill ' .11 ' "PI '' -UB* '
71 ! .05 .05 "!
1 i i ' ! F
i i i i
! ! F
70 ! Ln P Ln ' LD ! Ln
i 71 i >fvj i .07 i .U3 ' .07 i .016 !
77 ! .ni ! .07 .03 ' -03 ! .013 F
i 71 i i .01 ' ' '
i 70 , | . LO
;;;.-!!
' 7tl ' 'n7 ' ! n? '
' 77 LO I '.07 -02 .02 ! .015
73 I .05 ! .OS !
i 70 ' ! i .06 '
ii ii i "
itl
ii i i ' '
i 7n ' ! .03 ' ' !
It il 1 !
i i 1 1 '
70 ! .03 ! -U5 ' .03 ' ' '
! 71 ! .no ' .07 LP ! ! '
77 ! Ln ! Ln i L" .0? ! '
77 ! .01 ! .OF .02 ' ' |
ii i i i
ii ' ' ' '
| 77 ! .03 i .03 ' .07 '
i 77 ! ,nr T ,nu i .02 ' '
i 7« I LO ! .01 ! .0.3 Ln !
i i i i ' '
i -
70 ! .P* ! .11 "i ' -O* ' -05'' '
71 ! Ln .02 « LO ' LO !
77 ! ."f .00 ' .07 ' .03 ' .033
i 73 ! ,n7 LR ' .02 ' '
! 7 1 ! . 09 ! ' . ' ' '
i i i i ! j
70 ! .09 .10 ' -13 .12 ' .109 '
i 71 ! Ln LD ! .01 ' ."5 '
' 77 ! .09 .OS ' .01 .07 i .019 !
77 .01 LD -07 ' '
»''
, i i ' '
70 ! .07 .07 111'
71 ' Ln - LP ' '
77 ! ."1 ! .01 L" ' !
73 ! ! .01 ' ' '
71 ! ' ' ' Ln
!!'''
CATION
STTE U01
PPINGFTELO
STTF 001
nTANA
r AS T CH 1C AO 0
STTF UOl
fVANSVTLLF
STTF 001
FOPT UAYNF
SITE D01
FnRT WAYNE
SITF UOZ
"ABY
SITF 001
HAMMOND
STTF U01
HAMMOND
STTF UOZ
TNDTANAPOI.TS
STTF UOl
MUNCTF
STTF UOl
NFU ALBANY
STTE 002
SOUTH BENO
STTF 002
TFPRF H«UTE
STTF UOl
- .001
- .nni
- .003
- .nns
- .006
I i 1ST. 2NP. ' 350. 1TH. ' YR.
YR.! OTR. ! OTP.J-. QTfl.l QTR . ! «VG..
"i~n"» Io7~!~Ipir'""o3'"'"".OF .031
71. ! .07 ! LP. ! ' -P2 ' -OS t .P23
77 LO ! .03 ! .02 ! '
i 77 i ir .PE !
i 7H ' .07. ! ' .01 ! -PI '
i i i ! ff
'. '. *
i 70 ' .03 .OS .03 ! .03 .036
71 .01 ! .OS ! LD ! LO r
77 .01 .03 .0? ! 10 .072
i T3 .05 .07 F .0? ! t
i 7, i m Ln .03 .03
i i ! ! * '
iii! t f
70 .08 .12 ! 0'< -17 " -102
71 ' Ln .P3 ! .PS ! .PF ' .035
i 71 in .03 ! LD .PG '
ii'! '
i 70 .01 .PI ' -fl" ' -P" ' 'Wl>
i 71 in ! .01 ! LO LD
77 .CI1 f -P5 ! LD » .01 .031
77 .07 .IT! ' -P.* '
i 71, ! ! .01 ? ' .01 ! .P3
11 ! ! *
!.;
70 .03 .03 ! .02 -01 | .P27
71 in L« ! -07 < .03
, 77 10 ! ,<^ 1 ' .01 ' .05 .030
i 77 .05 .05 .05 ! ?
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70 ' .08 ! .06 .11 ' -OK ' "«
71 .08 ! .06 t ' .1?. 1
! 7? ' .t)B ! -PI t -OS ! .06 .018
i 77 i .07 ! .C6 ! -t)S f f
i 71 .01 ! .03 .13 .03 .P37
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, , i r i
i 70 .09 .01 ! .16 .06 .nsi
! 71 LO .p7 ! .01 .01 .0311
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i 77 .05 .11 ' .12 ! -OS .08
1 73 .05 .05 ! .13 !
i 71 .03 .02 ! .13 ! .01 .03
1 ! ' ' '
i i i i * '
70 i .03 .01 .05 I' .07 .01
i 71 i in i Ln r LD ! .r1! !
. Ti .10 .02 .n* ! '.
i 70 i i Ln .06 ! '
.'
i t ' '
i 70 .03 .03 '
f 7j r ! 1.0 ' ^^ *
i 77 i .01 ! ? ' '
!
70 .07 .01 .OZ '. .113 ' -PI
I 71 ' .07 ! F ' '
77 i .03 ! .05 LD !
I 77 I [D .01 LO '
, 7, . .P3 ! '
''!',;
70 .03 .01 .01 .Clt .02
71 .08 LP ! -O"1 ! '
i 77 1 ! .PS l.n LD F
i 77 in ! .03 LD ! '
i 71 ! .03 LP ! -01 I LO '
ii i r ! '
i ! » '
70 .06 .PS -01 ! -07 ! .0
i 71 .06 ' -05 '
i 77 .07 Lr ! LD t .PI *
77 .01 .PI ' '
i 7n i ' .07 .03 ! .^9
' ROCK
133
-------
POLLUTANT : 17.161 - TTTANTUM
METHOD : HT-VOL ^MTS^T-ON ^PFCTRA IL"« TFMP «SHI
OMITS : UG/ru MFTFB I?*,,*1!
n«TA Typir ; IJUARTFRLY. ^OMPOSTTIT
PROJ* CL ASSlFT(?ATTON t'tfRoflN
ANALYTICAL QUALITY i»?t+-)71.!lB»
L"UER nTSTRIMIMATTON LFVI (f)
70 - -ono
7i - .001
72 - .003
73 - .nns
71 - .nas
r
r
! LOCATION
r
r
ft QUA
' CEOjR RAPIDS
' STTE oni
f
t
t
t
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-------
TECHNICAL REPORT DATA
(Please read Instructions on the reverse before completing)
1. REPORT NO.
EPA-600/4-76-041
3. RECIPIENT'S ACCESSION-NO.
4. TITLE AND SUBTITLE
AIR QUALITY DATA FOR METALS 1970 THROUGH
From the National Air Surveillance Networks
5, REPORT DATE
August 1976
6. PERFORMING ORGANIZATION CODE
7. AUTHOR(S)
Gerald G. Akland
8, PERFORMING ORGANIZATION REPORT NO.
9. PERFORMING ORGANIZATION NAME AND ADDRESS
Environmental Monitoring and Support Laboratory
Environmental Protection Agency
Research Triangle Park, North Carolina 27711
10. PROGRAM ELEMENT NO.
1AD606
11. CONTRACT/GRANT NO.
12. SPONSORING AGENCY NAME AND ADDRESS
Environmental Monitoring and Support Laboratory
Office of Research and Development
U.S. Environmental Protection Agency
Research Triangle Park, North Carolina 27711
13. TYPE OF REPORT AND PERIOD COVERED
Final
14. SPONSORING AGENCY CODE
EPA/ORD
15. SUPPLEMENTARY NOTES
16. ABSTRACT
This report lists the urban and nonurban concentrations of 11 metallic components
of suspended particulate matter from samples gathered during calendar years 1970
through 197V by the cooperating stations of the National Air Surveillance
Network (NASN). The data are presented as a quarterly composite concentration
value for each site for each of the four quarters of the calendar year.
17.
KEY WORDS AND DOCUMENT ANALYSIS
DESCRIPTORS
b.IDENTIFIERS/OPEN ENDED TERMS
COSATI Field/Group
Metals containing organic compounds
Air polIution
Moni tors
Quali ty control
NASN
13B
18. DISTRIBUTION STATEMENT
RELEASE TO PUBLIC
19. SECURITY CLASS (ThisReport)
UNCLASSIFIED
21. NO. OF PAGES
20. SECURITY CLASS (Thispage)
' UNCLASSIFIED
22. PRICE
EPA Form 2220-1 (9-73)
155
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Technical Information Staff
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AN EQUAL OPPORTUNITY EMPLOYER
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Book
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