United States
                   Environmental Protection
                   Agency
National Risk Management
Research Laboratory
Research Triangle Park NC 27711
                   Research and Development
EPA/600/SR-95/148  October 1995
4>EPA       Project  Summary

                   A Simple  Method of Composition
                   Shifting  with  a Distillation
                   Column  for a Heat  Pump
                   Employing a  Zeotropic
                   Refrigerant  Mixture
                   Peter I. Rothfleisch
                    The  report  presents a simplified
                   method of controlling heat pump ca-
                   pacity by shifting the composition of a
                   zeotropic refrigerant mixture with a dis-
                   tillation column. Simplicity is achieved
                   by incorporating the distillation column
                   into  the typical  suction  accumulator
                   used in residential heat pumps. An ex-
                   perimental system employing this con-
                   cept  has been  evaluated in the
                   laboratory for two hydrofluorocarbon
                   (HFC)  refrigerant mixtures—HFC-32/
                   HFC-134a (30%/70%) and HFC 32/HFC-
                   125/HFC-134a (23%/25%/52%). For the
                   binary  mixture, the circulating refriger-
                   ant composition  was shifted to  HFC-
                   32/HFC-134a (54%/46%). For the ternary
                   mixture, the circulating refrigerant com-
                   position was shifted to HFC-32/HFC-
                   125/HFC-134a (36%/36%/28%). Seasonal
                   calculations have shown that  these
                   composition shifts reduce the seasonal
                   resistance heat requirement by up to
                   5% compared  to a conventional heat
                   pump.  Additionally, the instantaneous
                   peak energy requirement of the  dwell-
                   ing has been reduced relative to a con-
                   ventional  heat  pump  by  6-9%
                   depending on the climate  region. The
                   distillation insert should be capable of
                   producing greater composition  shifts
                   after further optimization of the insert
                   and improved integration with the heat
                   pump system. For the ternary mixture,
                   it  is expected that the insert will  be
                   capable of producing a circulating  re-
                   frigerant composition composed en-
                   tirely of HFC-32/HFC-125.
                    This Project Summary was developed
                   by EPA's National Risk Management
                   Research Laboratory, Research Triangle
Park, NC, to announce key findings of
the research project that is fully docu-
mented in a separate report of the same
title (see Project Report ordering infor-
mation at back).

Overview
  The heating capacity of a single-speed,
air-to-air residential heat pump is directly
proportional to the outdoor temperature.
As the outdoor temperature falls, the sys-
tem heating capacity is reduced and the
compressor work input is increased, mak-
ing the system less efficient. The building
heat load requirement, on the other hand,
increases as outdoor temperature falls.
For most residential systems, as outdoor
temperatures get lower, a temperature is
reached (called the balance point) below
which the output of the heat pump must
be augmented with an auxiliary energy
source to meet  the heat requirement of
the heated space.
  The auxiliary energy is usually supplied
by electric resistance heating, which  has
an energy efficiency much lower than a
heat pump. Therefore, the heating sea-
sonal performance factor (HSPF) of a heat
pump can be increased by reducing the
dependence on auxiliary electrical heating
during cold weather and  modulating the
heat pump capacity to meet the building
energy load.  The increase in HSPF  can
be significant for colder climates, and the
reduction in peak load to the electric utility
can be beneficial.
  To reduce the amount of auxiliary heat
required, the heat pump capacity must be
increased to  match the building load as
the outdoor temperature  falls. The only
commercially available heat pumps  ca-

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pable of matching system capacity to build-
ing  load have been those which vary the
volumetric capacity of the compressor. The
most common ways of accomplishing this
are  by using two-speed  compressor mo-
tors and variable-speed  compressor mo-
tors with frequency inverters, both of which
require considerable additional cost. Re-
cent interest in the use of zeotropic refrig-
erant mixtures, prompted by the phaseout
of the use of chlorofluorocarbon-based  re-
frigerants, has provided an opportunity for
an  additional unique method of varying
heat pump heating capacity  by varying
the  composition of the zeotropic mixture.
Specifically, by controlling mixture compo-
sition the thermodynamic properties of the
refrigerant mixture  can be altered to  in-
crease system  capacity as the  outdoor
temperature drops. Using this technique,
the  heat pump would operate on the origi-
nal  refrigerant  mixture  until the  outdoor
temperature falls to the balance point and
then shift the mixture  composition to  in-
crease capacity.
  Methods  and systems for varying the
capacity of a heat pump by controlling the
composition  of a  zeotropic mixture may
be classified as either an  active  or pas-
sive  system. An  active system   uses a
distillation column, whereas a passive sys-
tem uses a more simple accumulator. Gen-
erally, the methods that use accumulators
are simple to  implement  but require a
large refrigerant charge. Additionally, the
magnitude of the  composition change is
limited  by thermal equilibrium properties
and  storage space in the accumulator.
Conversely,  the  column  methods  can
achieve much larger composition changes
at the cost of increased system complex-
ity. Many proposed active  systems have
been too complex and costly to  be ap-
plied in the  competitive  residential heat
pump market.
  This work  presents a simplified  method
of controlling heat pump capacity by shift-
ing the composition of a zeotropic refrig-
erant  mixture with a distillation  column.
Simplicity is achieved by incorporating the
distillation column into the  typical  suction
accumulator used in  residential heat
pumps. An experimental  system employ-
ing  this concept has been evaluated  in
the  laboratory for two hydrofluorocarbon
(HFC) refrigerant mixtures—HFC-32/HFC-
134a  (30%/70%)  and HFC-32/HFC-125/
HFC-134a  (23%/25%/52%).  For the  bi-
nary mixture,  the  circulating refrigerant
composition was shifted to HFC-32/HFC-
134a (54%/46%). For the ternary mixture,
the  circulating refrigerant composition was
shifted  to  HFC-32/HFC-125/HFC-134a
(36%/36%/28%).  Seasonal  calculations
have shown that these composition shifts
reduce the seasonal resistance heat  re-
quirement by  up  to 5% compared to a
conventional heat pump. Additionally, the
instantaneous  peak energy  requirement
of the dwelling has been reduced relative
to a conventional  heat  pump  by 6-9%
depending on the climate region. The dis-
tillation insert should be capable of pro-
ducing greater composition shifts after
further optimization of the  insert and im-
proved integration with the heat pump sys-
tem. For the ternary mixture, it is expected
that the insert will be capable of produc-
ing  a circulating  refrigerant  composition
composed entirely of HFC-32/HFC-125.
  Peter I. Rothfleisch is with the National Institute of Standards and Technology's
    Building and Fire Research Laboratory, Gaithersburg, MD 20899.
  Robert V. Hendriks is the EPA Project Officer (see below).
  The complete report,  entitled "A Simple Method of Composition Shifting with a
    Distillation Column for a Heat Pump Employing a Zeotropic Refrigerant Mixture,"
    (Order No. PB95-255821; Cost: $17.50, subject to change) will be available only
    from
          National Technical Information Service
          5285 Port Royal Road
          Springfield, VA 22161
          Telephone: 703-487-4650
  The EPA Project Officer can be contacted at
          National Risk Management Research Laboratory
          U.S. Environmental Protection Agency
          Research Triangle Park, NC 27711
United States
Environmental Protection Agency
National Risk Management
Research Laboratory (G-72)
Cincinnati, OH 45268
                                                           BULK RATE
                                                     POSTAGE & FEES PAID
                                                              EPA
                                                        PERMIT No. G-35
Official Business
Penalty for Private Use
$300
EPA/600/SR-95/148

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