-&EPA
United States
Environmental Protection
Agency
GHsce of Radiation Programs
                     Eastern Environmental
                     Radiation Facility
                     P O Box 3009
                     Montgomery, AL 36193
EPA 520/1-83-007
June 1983
          Radiation
          Potential Health and
          Environmental Hazards of
          Uranium Mine Wastes

           Executive Summary
 Report To The Congress
         Of The United States
         Volume 1 of 3 Volumes

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                                  EPA 520/1-6-83-007
      POTENTIAL  HEALTH AND  ENVIRONMENTAL


        HAZARDS  OF URANIUM  MINE  WASTES




              Executive Summary
A Report to the Congress of the United States
      in Response to Public Law 95-604
                June 10,  1983
    l/.S. Environmental Protection Agency
        Office of Radiation Programs
           Washington,  D.C.   20460

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                              CONTENTS
SECTION                                                        Page

   I      INTRODUCTION                                            1
               Purpose  of  the  Report                              1
              - Contents of the Report                             1
               Scope of the Report                                3
               Brief Descriptfon  of Uranium Mining Operations     6

   II     ACTIVE  MINES                                            8
               Number of Mines                                   8
               Health Impact of Air Emissions                     8
               Health Impact of Water Emissions                  10
               Health Impact of Solid Wastes                     12

   III    INACTIVE MINES                                        14
               Number of Mines                                  14
               Health Impact of Air Emissions                    14
               Health Impact of Water Emissions                  16
               Health Impact of Solid Wastes                     16

   IV     CONCLUSIONS AND  RECOWODATIONS                        19
               Conclusions                                      19
               Recommendations                                  22

   V      OTHER FINDINGS                                        23

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                              SECTION  I

                            INTRODUCTION

PURPOSE OF THE REPORT

    Uranium  mining  operations release  some  radioactive  materials
into  both air  and  water and generate  large  quantities  of  solid
wastes containing low levels  of radioactive materials.   Solid wastes
produced  by  past mining  operations  remain  on  the  surface  at  many
inactive  mining   sites,   and  represent  a  potential   health   and
environmental hazard similar  in  concept to  uranium mill  tailings.
Contamination  of   surface   and   subsurface   water  supplies   also
represents  a  potential   problem.    To  evaluate   these  potential
problems,  the Congress,   in   Section 114fc)  of  the  Uranium  Mill
Tailings  Radiation  Control  Act  of  1978  (UMTRCA),  instructed  the
Administrator  of  the  Environmental  Protection  Agency  (EPA)   to
prepare  a  report  "which  identifies  the   location  and  potential
health,  safety,  and  environmental  hazards  of  uranium   mine  wastes
together with  recommendations, ff  any,  for a  program to  eliminate
these hazards."
    This  report   analyzes the  potential  health  and  environmental
impacts  of  both  active  and  inactive  uranium  mines,   lists   the
locations of  these mines, identifies additional  information  needs,
and recommends needed actions.

CONTENTS OF THE  REPORT

    This  Executive  Summary   contains a  brief  description  of   the
material  presented  in   the   main  text,  including  the  principal
findings,  conclusions,   and   recommendations.    The  full   report
consists  of  this  Executive  Summary,  a  main  text,  and  appendices.
The full  report  has  been reviewed by  the  uranium mining  industry,
States  and  the  Nuclear  Regulatory Commission.   Comments have  been
incorporated where possible.

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    Main text

    The main  text  consists  of seven chapters covering  the  following
subject matter;

           —a general description of uranium mining
           —an inventory of both active and inactive uranium mines
           --sources and amounts of pollutants released to  the
                 environment
           --amounts of solid waste generated
           —pathways of human exposure to pollutants
           --health risks and environmental  impacts
           --recommendations and conclusions

     Appendices

     The appendices cover the following subjects:

           —a detailed listing of the active and  inactive
                 uranium mines in the United States  and their
                 locations
           --observations of existing conditions at
                 selected inactive mines
           —a description of the methodology used in the health
                 risk and environmental  impact assessments

SCOPE OF THE REPORT

          This report  addresses potential  health impacts  caused by
air  and  water emissions  and  solid wastes  at active  and inactive
underground and  surface mines.   We  emphasize  radiological   impacts
because we  believe these to  represent the  most  significant health
hazards although  nonradiological  aspects  of  ground water  and  air
contamination  were   also   studied.    Impacts  from  other  mining
activities,   such   as  exploration,  site  preparation,   and   in   situ
leaching,    were   evaluated   In   proportion   to    their   potential
significance and  the amount  of available information about them.

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      Pathways  of  Exposure

      Underground   and   surface  mining   release   radioactivity  and
'chemicals  Into air and  water and  generate solid  wastes  that  may
ispread  through wind  and water  erosion  and release  radon-222 into
!air.  We  have  examined the  extent to which  people may be exposed to
-these released materials or residual solid  wastes and thereby incur
,an  Increased chance of cancer  or other health effects  from:

           --breathing  air containing radon daughters,
           --drinking water containing uranium and its  daughters,
           --eating  food contaminated by either air or  water, and
           —living  in  homes on land covered  by mine wastes.

Estimates  of  the  health  risks  from  each  of   these pathways  are
presented  in this report.

      Method of Analysi s

      Our    preliminary   evaluations    indicated    little    actual
environmental  data  is  available to evaluate the  impacts  of releases
from  uranium  mines.   Therefore,  we developed models of  active  and
inactive mines using  the available data  and evaluated these impacts
on  a broad   generic  basis.   To  the  extent  possible,  operating
parameters and pollutant  release  rates  characteristic of  the various
classes of mines  were used  in our models.  Finally  we extrapolated
the health risks  from  the mode] mines  to obtain an  estimate  of  the
total health effects  from all  active and  inactive mines  on regional
populations within  50  miles from each mine.  We  estimate  the risk to
the  total  U.S. population  is  no greater than  a  factor  of  3 or  4
higher than our estimates for  regional  populations.
      The   availability  of  information  to  assess  the  health  and
environmental   impact  from  uranium  mines  varied  greatly  depending

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upon the type of release and pathway  of exposure.   In  some  cases,  we
had to assume the most appropriate values  to use in the analyses.
For  some  release-pathway   combinations,  we  were  able  to  make   a
quantitative    risk    assessment.     For   other    release-pathway
combinations, the  information  was so  limited that we  could  identify
only the potential for impact.
     We have  expressed  the  health and environmental impacts  in  this
report in a number of different ways:
          —Estimates of the risk of cancer to individuals
               and to population groups
          --Estimates of the risk of genetic effects to
                 the descendants of exposed individuals and
                 population groups
          --Estimates of radioactiviy  and  chemical  concentrations in
                 the environment and a comparison of these
                 concentrations with air or water standards  or with
                 existing background levels
          --Estimates of land areas disturbed,  amounts  of
                 solid wastes generated, quantities of  water
                 discharged, and quantities of  contaminants
                 released to air and water
          --Qualitative observations of a  potential  health
                 impact
It must be  recognized  that  the primary effect of  radiation  exposure
is cancer although genetic effects are also evaluated,
   i

     Uncertainty of HealthRisk Estimate

     To assess the increased chance of cancer and  of genetic  effects
occurring after  exposure to  radiation,  Federal  agencies  base risk
estimates on  studies of persons exposed  at high  doses  and assume
that the effects at  lower doses will  be proportionately less.  Such
assessments are  based on a statistical'risk  to  all  persons  in  a
large population  exposed to  a  known  radiation  dose.  Because  of
uncertainties in the health risk  analyses presented in this  report,
these estimates should  be used  carefully.

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BRIEF DESCRIPTION OF URANIUN MINING OPERATIONS

     The  two major  mining methods  used  in  the  United States  are
underground and surface  (open pit) mining.  During  1978, underground
mines produced 5.5 minion metric  tons  of  ore containing 8300 metric
tons   of   uranium   oxide  ^Qg)  while   surface  mines   produced
7.5 million  metric   tons  of   ore   containing  8700   metric   tons
of UgOg.    In  situ   leaching,   heap   leaching,   and   mine   water
extraction methods  accounted  for the remaining  1300 metric  tons  of
ILQo production.

     Underground Hi ni ng

     Underground mining  uses  shafts  and  tunnels to  gain access  to
the  ore.   A mine  may  extend  underground for  a mile  or  more  at
several depths.   The  ore is moved  to  the  surface  and stored  for
transport  to a  yranium  mill.   Waste  rock   and  sub-ore*  generated
during mining  are  also stored  at  the surface as  a  waste pile.   At
most  underground  mines,  these  wastes  remain  on the  surface  when
mining ceases.
     Large  capacity  ventilation  systems  are  used  at  underground
mines  to  keep  the  radon-222  decay  product  concentrations  in  the
working areas  below  occupational  exposure limits.   Air is  usually
forced down through  the main  shaft along  the tunnels to  the  working
areas   and   then  exhausted  through   ventilation  shafts.    Large
underground mines  may have as  many  as a  dozen  ventilation  shafts.
However, while ventilation removes radon-222  decay products from the
working areas,  it discharges radon-222 to  the  atmosphere.
*Sub-ore contains  uranium at a  concentration  uneconomical  to  mill.
This  concentration  varies   with  the  "cutoff  level"  of  the mill
receiving  the  ore.  The  cutoff  level  is  usually  determined  by  the
cost of milling vs. the value of  the recovered  uranium.

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     Surface Mining

     Surface mining is done by excavating one or more  pits.   The  top
soil and  overburden  above the ore  are removed and  stockpiled.   The
uranium ore is then removed and  stockpiled for  shipment  to  a uranium
mill.  Sub-ore is  also  removed from the pit during  these  operations
and stockpiled for possible future use.
     The  present  practice at  most   surface  uranium  mines  is   to
backfill the mined out pits with  overburden as  part  of a reclamation
program.  However, even  though backfilling  is  performed, some  waste
remains on the surface after  mining is completed,  and the  final  pit
may  not   be   backfilled.    Most  older  inactive  mines   were   not
backfilled and little or no reclamation was  done.

     Mjje Dewatering

     Since  most  uranium  ore   deposits are   below  the  water  table,
groundwater  must  be  controlled to   prevent  mines  from  flooding.
Underground mines  and most surface  mines are dewatered  to  allow  for
excavation or  shaft  sinking and  ore  removal.   Both underground  and
surface  mines discharge   this  water  to  natural   surface   drainage
systems.  The discharged water,  if  necessary, is treated with barium
chloride and allowed to settle to reduce radium and  suspended solids
before it  is  released.   In addition to local effects,  the  long-term
impacts  on   regional  water   availability   and  quality   are  also
important considerations.

     Exploratory  and j)evelppment Dri 111_ng

     The  uranium   industry   has  drilled  approximately   1,300,000
exploratory and  development  drill  holes through  1977.   It  appears
from mine  site surveys  and  aerial  photography that  very   few  drill
sites  have  been  reclaimed.   Some States do require backfilling  of
drill holes.

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                                  8

     The  average drilling  depth  has  Increased with  time  and  will
probably continue to do  so  in  the future.   Deeper drilling will  tend
to  increase  the possibility  that aquifers  with  good  quality  water
may  be  degraded by  being  connected,  via  the   drill  holes,  with
aquifers of poorer quality water.

                             SECTION II

                            ACTIVE MIMES

NUMBER OF MINES

     In 1978 there were  about  340 active  uranium  mines in  the United
States.   A  11st of  these mines is  presented  in  Appendix  E  and
includes the type of  mine,  location, and  owner.   Table 1  summarizes
the locations,  numbers, and types of active mines:


                               Table  1
          Location of  Active Minesjin_United States |n  1978
                                                             Other
                                                                4
                                                                3
                                                                1
                                                                3
                                                                2
                                                                0
Total            60              256              11           13
HEALTH IMPACT OF AIR EMISSIONS-ACTIVE MINES

     Rad i olgg i cal Impac ts

     Exposure to radionuclide emissions  into air  from  active  uranium
mines increases the chance of cancer.  These risks  of  cancer  are the
State
Colorado
New Mexico
Texas
Utah
Wyomi ng
Other
Surface
5
4
16
13
19
3
Underground
106
35
0
108
6
1
In situ
0
0
8
0
3
0

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 ^'primary  public  health   impact  from  air  emissions  due  to  active
 'uranium mines.  Individuals  who might be  living  near uranium  mines
 I are, /exposed to higher radiation risks than those farther  away.   Our
 "V'H ,.ys*
 ''estimates  of  potential   impacts  are  based  on model  mines  in  the
 '"absence  of  adequate  field  data.    For  our  model  of   a   large
 ^underground mine we estimate  that individuals living for  a  lifetime
 tl^'mile from the  mine would  have  an  increased chance  of  fatal  lung
 ';;cancer  of  2   in   a   thousand  resulting   primarily  from  breathing
 ..radon-222 decay-products.  The  increased  risk caused by the mine  to
 ^•"an individual  living  25  miles away is  several hundred times  lower.
 | Risks from other types of uranium mines are somewhat lower.
 Vr    We estimated  the  health impact  from all active  uranium  mines
 t''
 y operating in 1978  by  multiplying  the  risks from  the model mines  by
 **, tfo number of  active mines  of  each  type.   This  procedure  provides
 -• ' ,% ;
 f"only  a very rough  estimate of  the total   population risks from  all
/.'"mines and is accurate only to the extent  the model mine  represents
••"an average for all  operations.  Based on this  rough  extrapolation  of
,-the total  risks  from all  mines,  we  estimate  that   the  radionuclide
 'emissions into air from  all  active uranium mines operating in  1978
  would cause less  than one  fatal  cancer in  the  regional  population
  living  around  these sites.
       The   risk  of  genetic  defects  in future generations due  to
  airborne   radiation  exposure  from  uranium  mines  is  very   small
 compared   to  the  natural  occurrence   of   hereditary  disease.    The
  largest potential  increase in genetic  defects would  occur  near  large
  surface mines.   Exposure  of the  population near a large surface  mine
  for one  year  is  estimated  to  result  in  a   very   small  chance  of
 additional  genetic effects to  their  descendants  (less  than 0.0001
  such  effects in the population).

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                                 10

     No n rad i o 1 og 1 c a 1 Imp ac t s

     We   estimated   the   air   concentrations   of   nonradioactive
pollutants produced by our model mines at an  assumed  location  of  the
nearest individual—1 mile from center of mine  site—and  determined
the  following  emissions  presented  minimal   potential  risk  to  the
population:

          —airborne stable trace metals
          —airborne combustion products  from  heavy equipment
               operation
          —nonradioactive gas emissions  at  in situ leach mines

However, the estimated concentrations of particulates in the form  of
dust in ambient air near  large  surface  mines exceeded the  national
ambient air  quality  standard.   Most dust near  active surface  mines
is caused by vehicle traffic.

HEALTH IMPACT OF HATER EMISSIONS-ACTIVE MINES

     Radiological Impacts

    " The health  risks due to  radionuclide  emissions  to  water from
active  uranium  mines are  lower  than  those  caused  by radionuclide
emissions to  air.   Although we  were able  to estimate cancer  risks
caused  by   radionuclides   in  discharged  water   from   our   model
underground and surface mines, we  could  not do so for in situ  leach
mines because of  insufficient  data,   However, radionuclide  releases
in water appear to be low from in  situ mines.  As  with our estimates
of air emission impacts, models utilizing some actual data were used
to develop this information.

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                                 11

     For our model of  an  average  underground mine,  we  estimated  that
individuals  living  for a  lifetime 1 mile  from an underground  mine
would  have  an  increased chance of cancer of about one in  a  hundred
thousand due to releases  to surface water.   We estimated  that  about
one additional  cancer  in  several  hundred years might  occur from  the
normal controlled releases from these mines.
     However, mine water  discharged to  nearby  streams can  recharge
shallow  aquifers,  many  of which  are  presently   used for drinking
water  or may be in the  future.  Ue do not have  enough  information  at
this  time  to evaluate  the potential health risks from using  these
aquifers, but  using  these aquifers  for  drinking  water could result
in increased radiation exposure.
     Where  such a problem may exist, the state radiological  program
should  investigate  existing  records to determine  the contaminant
levels   in   these  aquifers   due   to  mining,   and   evaluate   the
significance of the health risks  from using these  shallow  aquifers.
If a  state  determines  that sufficient data do  not exist to  perform
an evaluation,  additional  sampling and  analyses should be  performed
by the state to acquire the necessary data.

     Nonrad i o|og1ca1  Impacts

     We estimated the concentrations of  nonradioactive pollutants  in
the streams  used  by  the  general  population  of the  region from our
mine  models.   These  concentrations  were from  dewatering  the model
mines  and  were calculated after  the discharge was diluted  by the
receiving  stream.   Under  these  conditions,  none of  the  pollutant
concentrations  alone   or  in   combination  exceeded the  EPA  Water
Quality Criteria concentrations for  use  in  irrigation and  livestock
water.   However,  the   recharge  of shallow aquifers and the  use  of
these  aquifers  for   drinking water present   a   potential  problem
similar to  that discussed for radionuclide emissions.  Thus  States
may want to evaluate  pollution  concentrations to  ensure  drinking
water standards are met.

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                                 12

HEALTH, IMPACT OF SOLID. WASTES-ACTIVE  MINES

     Radiological Impacts

     Uranium  mining  operations generate  large quantities  of solid
wastes containing low  levels of radioactive  materials.   An  average
surface mine  generates about 6  million metric tons  of  solid waste
per  year,   while   an  underground  mine   generates  considerably
less—about 20 thousand metric tons  per year.   These wastes  consist
of  sub-ore,   waste   rock,  and  overburden.    At  surface  mines  the
sub-ore  comprises  only  a  few  percent  of  the  waste  while  at
underground mines, because much  less waste  is produced,  the  sub-ore
may comprise up to 90 percent of the  waste.
     Through  wind,  water erosion,  and  release of  radon-222, these
wastes can potentially contribute to air and water pollution.  These
wastes pose this hazard  because they contain elevated concentrations
of  radiu«n-226.   Sub-ore  (depending  upon  the  cutoff  grade  for
milling)  may  contain   up  to  50  picocuries  per  gram   (pC1/g)  of
radium-226,  and,  even  though the overburden and  waste  rock  contain
lower   concentrations   of   radium-226   than   the   sub-ore,  large
quantities of  these  wastes can contain  concentrations of radium-226
in excess of  5 pCi/g.*  EPA has proposed that uranium  mine wastes
containing radium-226  in quantities  greater  than 5  pCi/g  be listed
as "hazardous  wastes"  under  the Resource  Conservation  and  Recovery
Act  (RCRA)  and  has  also  proposed  regulations  for  the  treatment,
storage,  and  disposal  of these  wastes  (43 FR 58946,  December 18,
1978).  The EPA  is currently conducting an extensive study of solid
wastes  from  mines,   including  uranium mines at   the  request  of
Congress.    If warranted,  further  regulations  on  mining  would  be
proraugated.
*The radium-226 concentration of most soil  and rock  is  about  1  pCi/g.

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                                 13

     Usejof Wastes in Bunding Construction

     Using wastes  containing  elevated levels of  radium-226 as  land
fill  for  residential   construction   or   building  homes  on   land
contaminated by these wastes can greatly increase  the chance of  lung
cancer to  individuals  living  fn these structures.  Radon-222 formed
from  the  decay of radium-226  is  an   inert  gas  that  readily seeps
through foundations, floors, and walls and accumulates in the inside
air  of  a  house.    The  radon-222  then decays  to  daughter products
which, when  breathed,  will lodge  in   the  lungs and cause  radiation
exposure to the lung tissues.   For example,  the use of uranium  mill
tailings in  the  construction  of homes  in  Grand Junction,  Colorado,
resulted in radon-222  decay product concentrations inside  the homes
that  required  a  Federal-State  remedial  action  program  for   the
affected  structures   {Public   Law 92-314).    These  mill  wastes,
however,  contain much  higher  concentrations  of  radium-226  than  mine
wastes.   A survey  of homes in  Florida on  reclaimed land containing
wastes from phosphate  mining  showed about  20 percent of these homes
have  radon-222  decay  product  concentrations   in  excess  of   0,03
working level  (ML).*   Lifetime residency in  a  home with  this level
could  Increase the chance  of  lung   cancer  by  as  much  as  4  in
100—thus doubling the normal  risk  of  lung  cancer.
      The  mechanisms  by which  uranium mine  wastes may  cause health
risks are  similar  to  those which  have occurred  from  uranium  mill
tailings and phosphate wastes.  Although uranium mine wastes usually
have  a   lower  radionuclide content   and  are  less  suitable  as a
construction material than  the  sand-like tailings, these  wastes  are
still a  potential  health hazard  to individuals  if effective waste
disposal  methods   are  not  used.   EPA  has  provided  to  the  States
survey reports of  radiation anomalies  that  may be  due to use of  mine
wastes in  construction and will  continue to support State  use  of
this
*A working level  (WL)  1s any combination of short-lived radon decay
products  in  one  liter  of  air  that will  result  in  the  ultimate
emission  of  alpha rays  with a  total  energy  of  130,000 MeV.   The
working level expresses a concentration of radioactivity in the air,
not how  much radiation  a  person receives.   EPA  estimates  that the
average working level in U.S.  homes  is about 0.004 WL.

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                                 14

                             SECTION III


                           INACTIVE MINES


NUMBER OF MINES


     There  are  about 3400  inactive  uranium mines  in  the  United

States.   A  list  of  these  mines  developed  from  computer  listings

maintained  by  the  U.   S.   Department  of  Energy  is  presented  in
Appendix  F including  the  type  of  mine,  location,  and owner.   The

following  table  summarizes  the  numbers and  types  of Inactive  mines

by State:


                               Table 2

             Location of  Inactive Mines^ in United States


     State            Surface         Underground       Other

     Arizona            135                 189            2
     Colorado           263                 902           52
     New Mexico          34                 142           12
     South Dakota       111                  30            0
     Utah               378                 698           17
     Wyoming            223                  32           10
     Other              108                  43            8

     Total             1252                2036          101



HEALTH IMPACT OF AIR EMISSIONS- INACTIVE MINES


     Ra Prolog leal Impact


     Radionuclide  emissions  into  air at  inactive  mine  sites  are

small compared to  the emissions from active  mines according to  our

estimates  of  model  mines.    The   principal   radionuclide   emitted,

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                                 15

 radofi-222, emanates  from unsealed mine  vents,  portals  and  residual
 waste piles.   This causes only small  increases  in the  risk  of  lung
 cancer  to individuals living  near these  mine sites.  Utilizing  the
 same models  as for the  active mines, we  estimated risks of  cancer
 from radon-222 emissions to air from our model inactive mines.
     By multiplying the  risks  from our model mines  by the number of
 inactive  mines of  each  type,  we  extrapolated  the  total number  of
 potential cancers  from all  inactive  mines.  This  procedure  provides
 only a  very  rough  approximation of the total risk  from  all  inactive
 mines.
     By  these  estimates, radon-222  emissions  from, inactive  uranium
 mines would produce the following cancer risks:

          Individuals  living for a  lifetime 1 mile from  an  inactive
          mine  would   have  an  increased  chance  of lun§  cancer  of
          about 2-3 in 100,000,

          The  amount  of  radon-222   released  each year from   all
          inactive  uranium  mine  sites would cause about  0.1  lung
          cancers in the regional  population around these sites.

     Nonradiological Impacts

     We  did  not identify  any  significant  health impact associated
with nonridiological  air emissions at inactive  uranium mines.   Our
estimates of dust  emissions  from  wind erosion of waste  piles  showed
that  insignificant  concentrations   of   nonradiological  pollutants
would exist in air  at these  inactive  sites.

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                                 16

"HEALTH IMPACT OF WATER EMISSIONS-INACTIVE MINES

     The extent to which  Inactive  surface  and  underground mines harm
water  quality  is poorly  understood.   Ground  water  in  contact with
ore   bodies   and   consequently   in   mines   typically   contains
radionucTides  and  trace  elements,  and  the  flow  of  the  water away
from  the  site  carries  dissolved  and   suspended  radionuclides  and
trace elements.
     Site  specific  studies are  needed  to  determine  the  present  and
potential  impacts  of  inactive  uranium mines  on both   surface  and
groundwater quality.  As  with  active  mines,  the  potential  exists  for
contamination  of drinking  water  supplies.    States  may  desire  to
conduct sampling of drinking water  at a  few  sites  in  the vicinity of
inactive mining districts to provide  data  to evaluate  whether such a
potential is valid.

HEALTH IMPACT OF SOLID MASTES-INACTIVE MINES

     Surface Mines

     We  estimate that  over  1  billion  tons  of  solid  wastes  were
generated  at  surface  uranium   mines  through  1978.    These  wastes
consist of  sub-ore  and  overburden.   The sub-ore, which  may  comprise
about 3 percent of the total wastes,  contains  significantly  elevated
concentrations of radium-226 (up to 100  pCi/g).*   Although the  over-
burden contains  much  lower concentrations  of  radium-226  than  the
sub-ore,  large quantities  of  these wastes  can contain radium-226  in
concentrations in excess  of 5 pCi/g--the  level  EPA  has  proposed  be
used to judge whether wastes should be  considered  as a candidate  for
designation  as  hazardous  waste  under  RCRA.  Such  a  determination
would require that specified disposal methods  be developed for  these
mine wastes.
*The radium-226 concentration of normal soil and rock is about  1  pCi/g.

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                                 17
I--     In  many  surface nines opened  since 1970, the  general  practice
iis  to backfill  the  rained-out  pits  with wastes as  part of  a  recla-
ftiation  program.    However,  at  most  older  inactive  surface  mines,
•little or no reclamation was done.

      Underground Mines

      We  estimate   that  about  30  million   tons  of   solid   waste
consisting  mostly  of sub-ore  were  generated  at  underground uranium
mines through 1978.   As  in   surface  mining,  the  sub-ore  contains
significantly   elevated   concentrations   of   radiym-226   {up   to
IQQpCi/g).   There  his been  very  little  reclamation at  inactive
underground  mine  sites,   so  most  of  these  wastes  remain on  the
surface  at  these sites.

      Use of Hastes in Buijdirig Construction

      As  discussed  In  the  section  on  active mines,  uranium  mine
wastes  would  present  a significant hazard  to individuals  if  homes
are  built  on land contaminated  by  these  wastes  or if  these  wastes
are  used in construction materials  for homes.   Individuals living in
these homes  could  have  an  increased  chance of  lung cancer  from
breathing  radon-222  decay  products.    The extent  to   which  uranium
mine  wastes have previously been  used  for these purposes is not well
known.
      However, some information is available which shows that uranium
mine  wastes   may   have  been  widely  used  as   landfill   in  the
construction  of  various  types of  buildings.   In  1972 EPA and  the
former Atomic Energy  Commission (AEC)  tried to identify locations of
higher-than-normal levels of gamma  radiation in an  attempt to  locate
uranium  mill  tailings.   During this  study,  over  500 locations  were
identified  where  uranium  ore  was  believed  to   be  the  source  of
elevated gamma  radiation.    Since  it  is  unlikely  that  ore-grade

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                                 18

material  would  be  ysed  as landfill,  we suspect  that  uranium  mine
wastes  (perhaps  sub-ore)  may  be the  source  of  the  abnormal gamma
radiation at these sites.
     In  order to  better  define  the off-site  use of  uranium  mine
wastes, EPA  fs  studying  the extent to which  these wastes have  been
used  away  from the  mine  sites  for  landfill  or  in  construction
materials  for  use  in  homes.    If  mine  wastes  were  involved  fn
construction of homes, a  health  risk from radon-222 emissions would
exist.   A preliminary survey  has  already been completed  and   the
information  has   been  shared   with   the  Interested  agencies   in
appropriate States.

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                                 19

                             SECTION IV

                   CONCLUSIONS AND  RECOMMENDATIONS
     The evaluation  of  the potential impacts  of  uranium mining  was
performed   largely   by  means   of  analytical   studies  of   model
facilities.    We   believe  that   the   results   give  an   adequate
representation of the industry.   In  order to determine  the  extent of
possible problems,  oyr  studies  were specifically  designed to  give
conservative results.  It  should  be  recognized that actual mines  may
operate  under conditions  producing  substantially  smaller  impacts
than the results presented.
     Compared  to  uranium milling, health  and  environmental  effects
of uranium mining are  not  as well understood,  despite  the  existence
of over  3000 active and inactive mines.   We  have noted  throughout
this  report  instances  of  the  absence or  inadequacy  of  pertinent
information.

CONCLUSIONS

     Solid Wastes

     Solid uranium raining wastes are potentially hazardous to  health
when used as building materials or when buildings  are constructed  on
land  containing  such wastes.   The  hazard  arises  principally from
increased risk of lung cancer due to radon-222.  In a 1972  survey  of
communities  in uranium  milling  and mining  regions,  EPA  and  the
former Atomic Energy Commission found more  than 500 locations  where
such wastes had been used.

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                                 20

     Airborne Effluents

     a)   Individuals  living  very  near  active   underground   mine
exhaust vents would have  an  increased  risk of lung cancer caused  by
exposure  to  radon-222 emissions.   Surface  mines and  in situ  mines
are  less hazardous,  and  inactive  mines  do  not  have  significant
radon-222 emissions.  Other  airborne radioactive emissions from all
types of mines are judged to be smaller.
     b5   The  number  of   additional  cancers committed per  year  in
regional  populations  due to  radionuclide  air  emissions  from  the
approximately 340 active  mines and  3300  inactive mines  was estimated
to  be  about  0.6  cancers   in   1978.   This   number   of  estimated
additional  cancers  fs  small,  about   one-third  of   the  estimated
additional cancers  in regional  popylations  due  to radon emissions
from the  24  inactive  yranium mill tailings piles addressed by  Title
I of  the Uranium Mill Tailings  Radiation  Control  Act.  CThese  mill
tailings piles represent  about 13 percent  of all tailings currently
existing  due  to  U.S.  uranium  milling  and  mining).   These potential
effects  are   not  of   sufficient  magnitude  to  warrant corrective
measures,  especially   considering  the   large  number   of   sites
1nvolved.
     c)   The   following   emissions  were  judged  to   cause   an
insignificant health risk at all  types  of mines:
          1.   airborne nonradicactive trace metals
          2,   airborne combustion products  from heavy-duty equipment
              operations
          3.   nonradioactive emissions  from in  situ  leach sites
     d)  Airborne dust near  large  surface mines  (primarily caused  by
vehicular  traffic)  may   exceed   the  National   Ambient  Air   Quality
Standard for paniculate matter.

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                                  21
      Waterborne Eff1uents

      a)    We  estimate  that  an  insignificant  health  risk   accrues
 currently  to  populations  from waterborne   radioactivity   from  an
 average  existing mine.
      b)    Uranium mine dewatering  and water  discharges,  which are
 increasing as more and deeper  mines are created, may  in the future
 have  significant  effects  on   water  quality.    Current  treatment
 practices are controlling the  release  of  radioactivity into  surface
 waters.
      c)    Water  in inactive  surface and  underground  mines   usually
 contains  radionucTides   and   trace   elements    in   concentrations
 comparable  to  ground  water  in  contact  with  ore  bodies.   Some
 abandoned underground mines  in certain areas of Colorado and  Utah
 probably  discharge   such  waters   to  nearby   streams  and   shallow
 aquifers.   Available  data is not  sufficient  to   conclude  whether  or
 not  there is a problem.
      d)   We  could not determine,  using  models, that  there is  no
 health  hazard to  individuals who  drink water drawn  from  surface  or
 underground  sources.   Water  discharges from  active  mines  to nearby
 streams   and  stream  channels   may  extensively recharge  shallow
 aquifers,  many of which  are either  now  used or  could be used for
 drinking water.   Such  determinations  must  be made on  a site-specific
 basis, and take  account  of  the additive  effects of  multiple mines.
 These  studies  can  be made easily a  part  of  State  or  utility
 surveillance programs.

     Exploratoryand Development Drilling

     Harm  from   effluents  due  to   exploratory   and  developmental
drilling  is  probably  small compared  to effects  of operating  mines.
Under   current   regulations   and   practices,   however,   aquifers
penetrated at  different  levels  can mix, creating the potential  for
degrading good quality groundwater.

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                                 22
RECOMMENDATIONS TO CONGRESS

     1)   Based on  this  study,  we do  not  believe  at this  time  that
Congress  needs  to  enact a  remedial  action  program  like  that  for
uranium mill  tailings.   This  is  principally  because  uranium  mine
wastes  are  lower   in  radioactivity  and  not  as  desirable   for
construction purposes  as uranium  mill  tailings.   Nonetheless,  some
mining  waste  materials  appear  to have  been  moved  from the  mining
sites, but not. to the extent that mill tailings  were.
     2)    Some  potential  problems  were   found  that  might  require
regulatory  action,   but   none   of  these  appear  to   require   new
Congressional  action at this time.

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                                 23

                              SECTION V

                           OTHER FINDINGS

     1)   Regulations may  be  needed  to  control  wastes  at  active
uranium  mines to preclude  off-site use  and  to minimize  the  health
risks  from  these materials.  These  regulations  would  need  to address
the  use  of  the  materials  for  construction  purposes  as  well  as
ultimate disposal of the materials.
     EPA  proposed  such  regulations  in  1978  under  the  Resource
Conservation  and  Recovery  Act  (RCRA).   In  1980,  Congress  amended
RCRA  to  require  further  EPA   studies  before  promulgating  general
regulations for mining wastes.   An  EPA study by the  Office  of  Solid
Wastes on all  types of mines,  including  uranium mines,  is currently
being  conducted.   The  amendment does  not affect  EPA's  authority  to
regulate  use  of  uranium mine  wastes in construction  or reclamation
of lands containing such wastes.
     2)   Standards  are  needed  to  control   human   exposure   from
radioactive air emissions  from  uranium  mines.   This  is principally
because  of  potential  exposure  to  individuals  living  near  large
underground  uranium  mines  rather  than  concerns   regarding   the
exposure of regional  populations.    We  have proposed  such  standards
under Section 112 of the Clean  Air Act.
     3}  EPA has conducted two field studies in 1972  and  1978  which
define possible  sites  at which  mine  wastes  may  have  been  used  in
construction or placed  around  buildings.  The  information  developed
in  these  studies has  been sent  to State  health  departments.    The
States   should   conduct   follow-up   studies,   as   appropriate,   to
determine whether there are problems at these sites.
     4)  The  adequacy  with which NPDES  permits protect individuals
who may obtain drinking  water  near  the discharge points for  uranium
mine dewatering  should  be  evaluated  by  States.   Under the Public
Water Systems provision of the Safe  Drinking Water Act,  radionuclide
standards now exist for drinking water.

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                                    24

        5)   Some site  specific  studies should be  considered by States
   to  determine  the  extent to  which  inactive  uranium  mines  may be
   significant water pollution sources.
        6)   States with uranium mines  should  determine the  feasibility
   of  controlling   fugitive   dust   from   large   surface   mines   and
   incorporate the  recommendations  in  State  Implementation Plans.
        7)   States  should  require  borehole plugs in drilling operations
   that  will   prevent  interaquifer  mixing  (exchange) and  also   seal
   drilling holes at the surface.
AU SAFS

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                           EPA 520/1-6-83-007
POTENTIAL HEALTH AND  ENVIRONMENTAL
  HAZARDS OF URANIUM MINE WASTES
 A Report to the Congress of the United States
      in Response to Public Law 95-604
          Volume 2 of 3 Volumes
             June 10, 1983
    U.S. Environmental Protection Agency
        Office of Radiation Programs
         Washington, D.C. 20460

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                                                                      Page

     1.4.2   State Regulations     .......    1-42
           1.4.2.1   Colorado ........    1-45
           1,4.2.2   New Mexico    	    1-47
           1,4.2.3   Texas	    1-49
           1.4.2.4   Utah	1-49
           1,4.2.5   Washington    .......    1-50
           1.4.2.6   Wyoming  ........    1-51
     1.5   References    .,..,..;»    1-53
2.0   Inventory of Uranium Mines   .     ,  -   .     .    .     »    ,    2-1
     2.1  References	-   .     .    . .   2-16
3.0  Potential Sources of Contaminants to  the Environment and
     Man  **«••*•««**«    3—1
     3.1  Background Concentrations of Radionuclides and  Trace
          Metals    ......    .    .,.   . -   ,K    ••  ,  •-    «    •    3-1,
        3.1.1   Naturally Occurring Radionuclides ....   .3-1 .
        3.1.2. -  Stable Elements    .......    3-6
     3.2   Water-Related Aspects of Uranium  Mining     ,     .    ,    3-11
        3.2.1 - Previous.and Ongoing Hydrologic- and Water  Quality-
               Studies Related to Uranium  Mining  ....    3-11
        3.2,2  Mine Water Management         < .     .    .     .    .    3-13
        3.2.3  Water Quality Effects  of Mine Water Discharge     .    3-23
            3.2.3.1 Behavior of Contaminants in the Aqueous
                    Environment    .......    3-E3
                3.2.3.1.1  Dilution and Suspended Sediment
                           Transport     ......    3-25
                3.2.3.1,2  Sorption and Desorption     .     ,    .    3-25
                3.2.3.1.3  Precipitation     	    3-28
                3.2.3.1,4  Biological  Assimilation and
                           Degradation  ......    3-30
                3.2.3,1,5  Complexation ......    3-31
            3.2.3.2  Results of Field  Studies in Uranium
                     Mining Areas  ,..,.,.    3-32

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                                                                       Page

                 3.2.3.2.1  Colorado      ......     3-32
                 3.2.3.2.2  Wyoming	     .     3-34
                 3.2.3.2.3  Texas   	     3-38
                 3.2.3.2.4  New Mexico	3-39
          3.2.3.3  Summary    ...»,,,.     3-43
3.3  Surface Mining	     .     3-44
     3.3*1  Solid Wastes »         	3-44
         3.3.1.1   Overburden Piles      ......     3-45
         3.3.1.2   Ore Stockpiles  	     3-54
         3.3.1.3   Sub-Ore Piles   	     .     3-60
         3.3.1.4   Reclamation of Overburden  Piles      .     .     .     3-62
     3.3,2., Mine,Water Discharge   .......     3-63
         3*3.2,1,  Data Sources   ..   <  .     ,     .     ,     .     .     3-63
         1,3,2,2,, -Quantity'. and-C[ua.Vfty  0f, Discharge,,  .   ,'v  '  .     3-64'
     3,3.3 .Hydraulic and Water Quality  Effects.'of: Surface" •
            Mine Discharge    ,    .     ....     .     ,     .     3-68 .
         'j.,3.3,1  Runoff and Flooding  in the  Model Surface
                  Mine Area	3-68
             3.3.3.1,1   Study Approach  ......     3-68
             3.3,3.1,2   Description of  Area  .....     3-70
             3.3,3.1.3   Method of Study      .....     1-72
             3,3.3,1.4   Discussion of Results    ....     J-77
         3.3.3.2  Impacts of Seepage on  Groundwtter     .     .     .     3-89
     3.3.4   Gases and Dusts from Mining Activities     .     .     .     3-93
         3,3,4.1  Dusts and Fumes	     3-93
         3.3,4.2  Radon-222 from the Pit, Storage Piles, and
                  Ore Handling	,     3-99
3.4  Underground Mining  .»,..,,..     3-107
     3,4.1   Solid Wastes	3-107
         3.4.1.1  Waste Rock Piles	          3-109
         3.4.1.2  Ore Stockpiles   	     3-110
        -3.4.1.3  Sub-Ore Piles    .......     3-112
                                    iv

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                                                                      Page

     3.4.2  Mine Water Discharge   .,.*,.„    3-113
         3.4.2.1  Data Sources     .......    3-113
         3.4.2.2  Quality and Quantity of Discharge    .    .    .    3-114
     3.4.3  Hydraulic and Water Quality Effects of Underground
            Mine Discharge    ........    3-120
         3.4,3.1  Runoff and Flooding in the Model Underground
                  Mine Area   .,..,».,    3-120"
             3.4.3.1.1  Study Approach  ......    3-120
             3.4.3.1.2  Description of Area  ,    ,    .    .    .    3-122
             3.4".3.1.3  Estimate of Sub-basin Flood Flow    .    .    3-124
             3.4.3.1.4  Prediction of Sub-basin Water Quality    .    3-132
         •3.4*3.2  Impacts of Seepage on Qroundwater   .    ,    .    3-149
     3.4.4  Gases -and Ousts from Mining Activities     .    .    .    3-155
          3.4.4,1"  Radon-222 -in,Mine: Exhaust; Air:--,.,,>-  ..   .-   *  ,  3-155
          3.4.4.2  Aboveground Radon-22£ Sources  .    .         -    3-157
          3.4.4.3  Dusts and Fumes	 »    3-159
3.5  In Situ Leach Mining	3-168
     3.5.1  Solid Wastes .    ...    .    .    .    , -   .    .    3-169'
     3.5.2  Associated Wastewater  .         .    .    ...    .    3-172
     3.5.3  Airborner Emissions     .         .         .    .    .    3-174
     3,5.4  Excursion of Lixivfant .......    3-178
     3.5.5  Restoration and Reclamation ......    3-179
3.6 'Other Sources  ..........    3-185
     3.6.1   Mineral  Exploration   .......    3-185
         3,6.1.1  Environmental Considerations    »                   3-187
         3.6.1.2  Radon Losses from Drill Holes   ....    3-192
         3.6.1.3  Groundwater ........    3-193
         3.6.1.4  Fumes  .    .    . •   .    .    .    .    .    .    3-193
         3.6.1.5  Model Drilling   .......    3-194
     3.6.2  Precipitation Runoff from Uranium Mines    .    ,    .    3-194
3.7  Inactive Mines	3-204
     3.7.1  Inactive Surface Mines .......    3-204
         3.7.1.1  Waste Rock Piles' .    .,..-'.-..,   ...   „    3-213

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                                                                       Page

          3.7.1.2   Radon-222  from the  Mine Area    ....    3-216
          3.7.1.3   Land  Surface Gamma  Radiation    ....    3-222
     3,7.2   Inactive  Underground Mines   	    3-227
          3.7.2.1   Waste Rock Piles  .......    3-229
          3.7.2.2   Radon-222  from the  Mine Area    ....    3-232
          3.7.2.3   Land  Surface Gamma  Radiation    ....    3-237
     3,8  References  "	    3-24*2
4.0  Description  of Model Mines    	    4-1
     4.1  Surface Mine	    4-1
     4.2  Underground Mine     .,,...,.    4-4
     4,3  In Situ Leach Mine  .    .     .    .    .     ,     »    .    4-7
     4.4'* Inactive Surf ace-Mine*    .  •   .'	4-8
     4,5  Inactive Underground Mine  ' '	4-9
5.0  Poteatfal RaviJiwa-ysv .«,.<•. >. ,.,  ... . , •.,    ...,.,   ,  , ,  , ,., „ .•   5-1,
     5,1  General •'.,..   .»    ..  .-.    , .» .•  .~    .•,-.,.   .,    .    5-1
       h.l.L Vege,tatioa. „ ,,*.,,,,,    .,    ... .   ,.   ...    . ,   5-1 ,
       5.1.2  Wildlife	               5-1
       5.1.3- Land Use    ... '        ...    ,    .     .     .    .    5-2
       5.1,4  Population Near Mining  Areas   .....    5-2
       5.1.5  Population Statistics of Humans  and Beef Cattle    .    5-12
     5.2  Prominent Environmental Pathways and Parameters for
          Aqueous Releases     	    b-i2
       5.2.1  Individual  Committed  Dose  Equivalent Assessment    ,    5-13
       5.2.2  Collective (Population) Dose Equivalent Assessment .    5-15
     5,3  Prominent Environmental Pathways and Parameters for
          Atmospheric Releases      .,..,..    5-15
       5,3.1  Individual  Committed  Dose  Equivalent Assessment    .    5-16
       5.3.2  Collective (Population) Dose Equivalent Assessment ,    5-18
     5.4  Mine Wastes Used in  the Construction of Habitable
          Structures      .........    5-19
     5.5  References      ,......,.    5-20
6.0  Health and Environmental  Effects    .    	    6-1
     o.l  Healtn  Effects- and" Radiation Qosfmetry  ^  <  -i.   ~»    .,    5-U

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                                                                      Page

       6.1.1  Radioactive Airborne Emissions .....     6-1
       6.1.2  Nonradioactive Airborne Emissions   ....     6-26
          6.1.2.1  Combustion Products  ......     6-26
          6.1.2.2  Nonradioactive Gases 	     6-28
          6.1.2.3  Trace Metals and Participates in the Form
                   of Dust	6-28
       6.1.3   Radioactive Aquatic Emissions .....     6-35
       6.1.4   Nonradioactive Aquatic Emissions   ....     6-42
       6.1.5   Solid Wastes	6-44
          6.1.5".l  Radium-226 Content	6-44
          6.1.5.2  Estimates of Potential Risk    ....     6-45
          6.1.5.3  Using Radium Bearing Wastes in the Construction
                 of Habitable Structures     .....     6-46
             6.1.5..3..1". .Use of Uran.ium Mine.Wastes,,  ,   .,    .    ,.     6-48
     6.2  Environmental Effects    .     .    .    ...     .     .     6-48
        6.2.1.  General Considerations   ......     6-48
        6.2.2  Effects of Mine Oewatering    .    .   '  .     .     .     6-52
        6.2.3- Erosion of Mined.Lands.and .Associated Wastes .   ,  .     6-54
        6.2.4  Land Disturbance .from Exploratory and
               Development-Drilling     . .  . •   .     .    " .   .  .     6-56,
        6.2.5  Land Disturbance from Mining  .    .     .     .     .     6-59
          6.2.5.1  Underground Mines    ......     6-59
          6.2.5.2  Surface Mines   	     6-59
        6.2.6  Retirement Phase    	     6-59
     6.3  References	6-73
7.0  Summary and Recommendations   .......     7-1
     7.1  Overview  ..........     7-1
     7.2  Sources and Concentrations of Contaminants .  .     .     .     7-1
       7.2.1  Surface and Underground Mines  .....     7-1
       7.2.2  In Situ Leach Mines	7-7
       7.2.3  Uranium Exploration  .......     7-8
     7.3   Exposure Pathways  ........     7-8
     7.4  Potential Health .Effects ,.  .  .    . .   .    .     -     -     7-9
                                     VII

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                                                                      Page

       7.4.1  Radioactive Airborne Emissions  .....    7-9
       7.4.2  Nonradioactfve Airborne Emissions    ....    7-13
       7.4.3  Radioactive Aqueous Emissions   .....    7-13
       7.4.4  Nonradioactive Aqueous Emissions     ....    7-15
       7.4.5  Solid Wastes	7-16
     7.5  Environmental Impacts    .......    7-16
       7.5.1  Land and Water Contamination    .....    7-17
       7.5.2  Effects of Mine  Dewatering	7-22
       7.5.3  Erosion of Mined Lands and Associated Wastes   .     .    7-22
       7.5.4  Exploratory and  Development Drilling      . v        .    7-23
       7.5,5  Underground Mining        .    -.     .     .     .     .    7-23
       7.5,6  Surface Mining^  .  •  .    .     .     .     .     .     .    7-24
     7.6  Regulatory ^Perspective-   .......    7-25
     7,7" Conclusions,and- Recoawtindations.,'*',„,-  ,,,..,    -     7-25.
       7.7.1  Conclusions,.   .-  -    ,    .     .-  , '  .     -     .     .    7-26
        ,7.7,1,1.. Sal id Wastes	7-26
         7.7.1.2  Airborne Effluents ...'....    7-26
         7.7.1.31.  Waterboroe .Effluents.. •. -   .     .          .     .    7-27
         7.7.1.4  Exploratory  and Development Drilling  .     .     .    7-27
       7.7.2  Recommendations  to Congress- •. •  - .* •    ....    7-28
     7.8  Other Findings	7-28
     /.9  References	7-29

Appendixes (See Volume 3)

     A.   Summary of Federal Laws Potentially Affecting Uranium Mining
     B.   Federal Water Programs and Rights Activities
     C.   Congressionally Approved Compacts that Apportion Water
     0.   State Laws, Regulations, and Guides for Uranium Mining
     E.   Active Uranium Mines in the United  States
     F.   Inactive Uranium Mines in the United States
     G,   General Observations of Uranium Mine Sites in Colorado,
          New Mexico,'
                                   vi n

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H,   Influence of Mine Drainage on Seepage to Groundwater
     and Surface Water Outflow
I.   Computation of Mass Emission Factors for Wind Erosion
J.   Aquatic Oosimetry and Health Effects Models and Para-
     meter Values
K.   Airborne Pathway Modeling
L.   Health Risk Assessment Methodology

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                                   FIGURES

                                                                       Page
1.1  Uranium mining  regions  in  the western  United States    .     .     1-4
1,2  The percent  of  $50  U30Q reserves  located  in the principal
     mining states   ,..,...,,.     1-8
1.3  The percent  of  $50  ILOg reserves  located  in the various.  •
     mining regions  .               	1-9
1.4  Artist's conception of  open  pit mining  operation and
     support "facilities.	1-13
1.5  Generalized  underground mine showing modified  room and
     pillar method,of.mining      * .     .,     ,    »    .    ,     .     1-17
1.6  Diagrams of  some common injection-recovery  well  patterns
     used "in uranium; m< situ; leach" mining <'  .„,  , .,,   ,•*    „     ..    1-26
2.1.. location'of;active''and  tnact,ive--uranium-,minis,and- prinelpt/1  -  •
     uranium mining  districts in  Colorado  -   	     2-6
2.2 'Location of  active  and  inactive uranium mines  and'principal-
     uranium, mining  districts ,In  the Uravan,Mineral  Belt*of  ,
     western Colorado  ,,.,....,«     2-7
2.3  Location of,  active,and,  inactive u rani urn. mines,  in, the .Grants.,,
     Mineral Belt and other  areas of New Mexico    ....     2-8
•.'*•  Location of  active, inactive, and  proposed  surface and  in
     situ uranium mines  in Texas    ,....».     2-9
r.5  Location of  uranium mines  and mining districts in Utah  ,     .     2-10
2.6  Location of  uranium mines  and principal uranium mining
     districts in southeastern  Utah     ,»..,.     2-11
2.7  Location of  active  and  inactive uranium mines  and principal
     uranium mining  areas in  Wyoming     ......     2-12
2.8  Location of  active  and  inactive uranium mines  in the Gas Hills
     and Crooks Gap-Green Mountain  areas of  central  Wyoming  .     .     2-13
2.9  Location of  active  and  inactive uranium mines  in the Shirley
     Basin, South Powder River  Basin, and Pumpkin Buttes areas
     of Wyoming™    .-.    .    ....     ,„     ,_    .   .  .-         .  .   2-14

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                                                                      Page

3.1  The uranium decay series showing the half lives and mode of
     decay	    3-2
3.2  The thorium decay series showing the half lives and mode of
     decay      ...........    3-3
3.3  Disposition of drainage water from active surface and under-
     ground uranium mines	3-14
3.4  location of mines, ore and waste storage areas and monitoring"
     stations at the Morton Ranch mine. South Powder River Basin,
     Wyoming"    ...........    3-37-
3.5  Location of study areas, sampling stations and uranium mines,
     Poison Canyon area, McKinley County, New Mexico   ,    .    .    3-41
3.6- Sample locations for radionuclides and select trace metals
     in sediments, San Mateo mine, Ntw Mexico  '                       3-42
3.7* Potential  sources,of, env-ironnenttlvcontamination, from active , ,
     open pit uranium mines	    3-46
3.8  Storage, p-ile configurations, assumed at surface and underground
     mines      ...........    3-48
3.9  Sketch of  sub-bas.in,. basin,,and regional basin showing orien-s
     tation of  principal drainage courses, areas of drainage, and
     location of mines   .........    3-69
3.10 Average monthly flows for the Cheyenne River and Lance Creek
     near Spencer, Wyoming, for the period 1948-1970   «    .    .    3-71
3.11 Suspended sediment concentration to discharge, Salt Wells
     Creek and Tributaries, Wyoming     ......    3-75
3.12 Relation of discharge and specific conductance to time at
     Salt Wells Creek, Green River Basin, Wyoming ....    3-76
3.13 Periods of no flow in Lance Creek and the Cheyenne River
     near Riverton, Wyoming, for the period 1948-1978.  .    .    .    3-82
3,14 Configyration of open pit model  mines   .....    3-105
3.15 Potential  sources of environmental  contamination from active
     underground uranium mines     .......    3-108

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                                                                       Page

3.16 Sketch  of  sub-basin,  basin,  and  regional  basin showing
     orientation  of  principal  drainage  courses,  areas of drain-
     age, and location  of  mines  in  the  New Mexico model  area     .     3-121
3.17 Average monthly flows  for the  period  of  record for the Rio
     San Jose and  the Rio  Puerco  in New Mexico    ....     3-129
3.18 Periods of no flow in  the Rio  San  Jose and  Rio Puerco  .     .     3-131
3.19 Total flow volumes in  one-day  periods" far floods'of-various'-  •
     recurrence intervals  in  the  sub-basin and basins in New
     Mexico	          3-133
3.20 Total flow volumes in  seven-day  periods  for floods  of various.
     recurrence intervals  in  the  sub-basin and basins in New
     Mexico	     3-134
3.21 Principal streams  and-surface  water sampling stations in'the
     Churrhroelt.ainrt'GalJup.-a^eis/'i  ....   .   -.,.-.   .,.   ,    ...   ,     3-145
3.22. Average, deptJoLof^expflora-tory, drill;ing,'in  the U.S.. uraniwn-.".-••;
     indus.tcy from 1948 to, present  ....     ..,    .,    ..    .,         3-188
3.23 Annual waste  to  ore ratios for surface mining of uranium
     (1948,to 1979)  »   .    \,    ,.     .     „    ...    .          3-209
3.24 Cross section of model inactive  surface mine ,    .    .          3-214
3.25 Results of gamma exposure rate survey at  the 1601  pit and-
     environs, Morton Ranch uranium wine,  Converse County,
     Wyoming   ...........     3-226
3^26 Waste to ore  ratios for  inactive underground uranium mines
     from 1932 to  1977	3-228
3.27 Radon-222 concentrations  in  mine air  discharged  by  natural
     ventilation     ..........     3-236
3.28 Gamma radiation  survey around  an inactive underground uranium
     mine in New Mexico .        -  .     .     .     .    .    .     .     3-240
5.1   Potential airborne pathways  in the  vicinity  of uranium
     mines     ...........     5-17
                                  XI 1

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                                                                       Page

 6.1   Average  indoor radon-222  decay  product  measurements  (in
      working  levels)  as a  function of  average  radium-226  con-
      centration  in  soil	6-47
 6.2   Example  of  natural  reclamation  of drill sites      .    .     .     6-57
 6.3   Inactive underground  mine site      ......     6-60
 6.4   Example  of  active  and inactive  surface  mining activities     .     6-63
 6.5   Mine wastes eroded  by ephemeral-streams in  the Mesa'Mon-v'  •-
      tanosa area, New Mexico   .  •	6-64
 6.6   Basal erosion  of a  uranium mine waste, pile  by. an ephemeral
      stream in "the  Mesa  Montanosa area.  New  Mexico      .    .     .     6-65
 6.7   Scattered piles  of  mine waste at  the  Mesa Top mine,  Mesa
      Montanosa,  New Mexico    ........     6-66
 6.8   Close up view  of-easily eroded  sandy  and silty mine  waste
      from the. Mesa, Top  mine,. Mesa Montanosa,, New Mexico,    . .   .     6-66
 6.9   Gullying and sheet  erosion of piled and spread mine  wastes
      at the Dog  Incline  uranium mine,  Mesa Montanosa; New Mexico~.     6-67
 6.10  Recent erosion  of  unstabilized  overburden piles at the
      inactive Galen mine,  Karnes County,-Texas    . ,    .    .,„.,,    6-68
 6.11  Unstabilizied  overburden  p.iles  and  surface  water erosion at
      the Galen mine,  Karnes County,  Texas    ,.    .     .    .     .     6-68
 6.12  Aerial  view of the  Manka  mine,  Karnes County, Texas    .     .     6-70
 6.13  Overburden  pile  showing the weak  vegetative cover and
      gullying associated with  improper stabilization at the
      Manka mine, Karnes  County, Texas,       	     6-70
 6.14  Inactive Hackney mine, Karnes County, Texas  ....     6-72

Appendix G

G.I   Plan view of inactive underground uranium mine No. 1, related
     waste rock piles, and surface gamma exposure rates,  Uravan
     Mineral  Belt, Colorado    	     G-3
                                   xiii

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                                                                      Page
G.2  Sectional view of  inactive underground uranium mine No. 2,
     related waste rock piles, and surface gamma exposure rates,
     Uravan Mineral Beltt Colorado .......    G-4
G,3  Plan view of inactive underground uranium mine No. 3, re-
     lated waste rock piles, and surface gamma exposure rates,
     Uravan Mineral Belt, Colorado      .    	    G-6
G.4  Sectional view of  inactive underground uranium mine No. 4,
     related waste rock piles, and surface gamma exposure rates,
     Uravan Mineral Belt, Colorado .......    G-7
G.5  Plan view of inactive underground uranium mine No. 5, re-
     lated waste rock piles, and surface gamma exposure rates,
     Uravan Mineral Belt, Colorado      ......    6-8
G.6 ' Plan view of Inactive underground uranium mine No. 6, re-
     lated waste rock piles, and -surf, ace. gamma, exposure, rates,
     Uravanr Mineral-B&T*t,'*CoFOrad'6'  *.•'  .    «.    ,     ..,   .    *    G-91
G*7~ Plan view of inactive"underground*uranium mine NO.' 7, re-
     lated wa^ste'rock-piles*'an4\surface ganwi,exposure rates,-r ,- ,-- -•
     Central City District,  Colorado    ......    G-ll
G.8  Plarr view" of inactive urnderfround* uranium1 mine No. 8,-re-
     lated waste rock piles, and surface gamma exposure rates,
     Central City District,  Colorado    ...,,,   ,  .    .   , ,    G-12
G.9  Plan view of inactive underground fluorspar uranium mine No.
     9, related waste rock piles, and surface gamma exposure rates,
     near Jamestown, Colorado ........    G-13
6.10 Plan view of inactive underground uranium mine No. 10, related
     waste rock piles, and surface gamma exposure rates, Central
     City District, Colorado  ........    G-15
G.ll Typical mine waste pile associated with a small- to medium-
     sized inactive underground uranium mine, Uravan Mineral
     Belt, Colorado ..........    6-16
G.12 Side view of a typical  underground uranium mine located on
     the rim of a sandstone mesa, Uravan Mineral Belt, Colorado  .    G-16
                                   xiv

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                                                                      Page
G.13 Mine waste accumulations near the portal of a typical under-
     ground rim-type uranium mine, western Colorado    .     .    .    G-17
G.14 Mine waste dump associated with a typical rim-type under-
     ground uranium mine, western Colorado   .....    G-17
6.15 Movement of fluorspar-uranium mine wastes from a tailings
     pile into a stream, Jamestown area, Colorado ....    G-19
G.16 1972 aerial photograph of the Galen and Pawelek open pit  .
     mines, Karnes County, Texas  .     ......    G-27
G.17 1978 aerial photograph of the Galen and Pawelek open pit
     mines, Karnes County, Texas   .......    G-27
G.18 Results of gamma exposure rate survey at the 1601 pit and
     environs, Morton Ranch uranium mine, Converse County, Wyoming    G-31
G.19, lo.ca.tion of sampling stations at the Morton Ranch mine, South
     Powder River Basin, Wyoming   . ,        _    ....     .-    .    G-33
G.20 Sample locations for radionuclides and select trace metals in
     sediments-, San Mateo mine, New Mexico-  .    .    .     .    .    G-34

AppendixH

H.I  Wyoming model area sub-basin drainage system ....    H-3
H.2  Model area stream cross section    ......    H-3
H.3  New Mexico model area sub-basin drainage system   .     .    .    H-9

Appendix J

J.I  Surface stream flow pattern within drainage area  .     .    .    J-3
J.2  Conservation of mass relationship for resuspension model    .    J-13
                                    xv

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                                  TABLES

                                                                       Page
1.1       Domestic  uranium  production by  state  from 1948  to
          January 1,  1979	1-3
1.2       Projected annual  nuclear capacity  (GWe)  in  the  U.S.     .     1-6
1.3       Domestic  uranium  reserves by state as of January I,  1979     1-7
1.4       The quantities of U^Oo  produced  in 1978  by  the  various
          mining methods 	     1-10
1.5       The predicted methods of mining  ore reserves  .     .     .     1-10
1,6       Summary of  current  in situ leaching operations  as  of
          January 1,  1978      ........     1-21
1,7       Trace metal concentrations of recirculated  acid and
          alkaline  lixiviants  .;......     1-25
1.8'    "   Federal laws, regulations, and  guides for uranium  mining     1-32
1.9    '   Requirementsv-ta. obtain  righ*tS'."tO'"praspect,or.*"explore -.'
        •  by federal, state and. private"lands ,-'-.,   .  -   .     .  ,   1-37.
1.10      Requirements to obtain  rights.to mine ore by  federal,
          state and private lands  .    ."         .     .     .     .     1-39
1.11      Requirements.for,mining and environmental'plans'by
          federal,  state and  private lands   .....     1-41
1.12      State laws,1 regulations; and guides" for  uraniym mining  .     1-43
2.1       Type of U.S. uranium properties    .....     2-3
2,2       The location and  type of active  uranium  properties     .     t-4"
2,3       The location and  type of inactive  uranium properties    .     2-5
2.4       Cumulative  ore production through  January 1,  1979  ,     .     2-15
3,1       Gamma-ray energy  released by one gram of rock      .     .     3-4
3.2       Radionuclide content and dose equivalent rates  from
          common rocks and  soil    .......     3-4
3.3       Average dose equivalent rates due  to  terrestrial
          radiation in western m'nino steces .....     3-5
3.4       Radionuclide concentrations in  surface and  groundwater
          in the vicinity of a proposed uranium project      .     ,     3-7
3.5       Concentrations of selected elements in igneous  and
          sedimentary rocks   -. -   .    .    .     .,,    *     .    -.    -3-8
                                    xvi

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                                                                      Page

3.6       Concentrations of selected elements in surface water at
          five locations in the vicinity of a proposed uranium
          project	3-9
3.7       Concentrations of selected elements in groundwater at six
          locations  in the vicinity of a proposed uranium project.    3-10
3,8       Estimated  average concentrations of three metals in
          U.S. streams   .........    3-6"
3.9       Summary of feed water sources for active U.S. uranium
          mills      ..........    3-17'
3.10      Current and projected uranium mine discharges in the
          Grants Hineral Belt, New Mexico    .....    3-21
3.11      Estimated  surface areas associated with overburden piles    3-50
3.12      Particle size distributions of mil! tat! ings and mine
          overburden*    ..    _.        ..    ,,    .    .-        .,    3-52.
3.13      Natural radionuclide concentrations in various common
          rock types     .........    3-52
3.14      Annual  average airborne radionuclide concentrations
         ,in the vicinity.of an.open pit uranium mine  ,         .    3-53
3.15      Uranium and stable element concentrations measured in rock
          and soil samples from two uranium mines %    ...    3-55
3.16      Concentration of radionuclides and stable elements in
          overburden rock from the model surface mines .    .    .    3-56
3.17      Estimated average areas of ore pile surface and- pad    .    3-57
3.18      Distribution of ore reserves by the type of host  .    .    3-59
3.19      Average stable element concentrations in sandstone
          ores of Hew Mexico  ........    3-59
3.20      Estimated average surface areas of sub-ore piles during
          the 17-year active mining; period   .....    3-61
3.21      Summary of average discharge and water quality data for
          uranium mines in Wyoming and a comparison with NPDES
          limits      .    .     .     .    .    .    .    .    .    .    3-65
3,22      Water quality associated with surface and underground
          mines in various  stages of-construction and operation  .   -3-67
                                   xvi i

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                                                                      Page

3.23      Peak discharge and total volume for floods of 2, 5, 10,
          25, 50 and 100 year recurrence intervals     .     ,     ,    3-78
3.24      Summary of calculated total flow  in the Wyoming model
          area sub-basin using the USGS and SCS methods      .     .    3-79
3.25      Annual contaminant loading from one uranium mine and
          resulting concentrations in floods within the sub-basin
          for return periods of 2 to 100 years    ....    3-84^'
3.26      Concentrations in basin and regional basin streams as a
          result of surface mine discharge   .....    3-86
3.27      Comparison of potable and. irrigation water.standards and.  ,  .
          surface water quality affected by surface mine drainage     3-87
3.28      Northeastern-Wyoming groundwater  sources     .     .     .    3-91
3.29      Groundwater quality of wells sampled by the three major
          uraniunr..pradyee,rs.f in., the. Souths Powder,-River .Basin,,--
          Wyoming, : •	-       .    .-    ,     ,     .    3-92.
3.30      Estimated air pollutant emissions from heavy-duty
          equipment at surface mines    ......    3-94
3.31      Average annual dus.t1 emissions, from mining activities •   .    3-97
3.32      Average annual emissions of radionuclides (yCi) and stable
          elements (kg) from vehicular dust. at. the model-, surface
          mines     ..........    3-100,
3,33      Average annual emissions of radionuclides (pCi) and stable-1
          elements (kg) from mining activities at the model  surface
          .nines	3-101
3.34      Average annual emissions of radionuclides (vCi) and stable
          elements (kg) in wind suspended dust at the model  surface
          mines     ..........    3-102
3.35      Radon-222 releases during surface mining     .     .     .    3-107
3 36      Estimated average surface areas of waste rock piles at
          underground mines   ........    3-111
3.37      Estimated surface areas of ore stockpiles at underground
          mines     ..........    3-111
3.38 .     Estimated average „surface- areas, of sub.-ore* pi.les.at'- ,  ,
          underground mines,  .    ...    .    .           .     .    3-113
                                    xvi 11

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                                                                      Page

3.39       Summary  of  average discharge and water quality data for
           underground uranium mines  in the Colorado Plateau Region
           (Colorado,  New Mexico, Utah) and a comparison with NPDES
           limits	         3-116
3.40       Water quality associated with underground mines in
           various  stages of construction and operation .    .    ,    3-119
3.41       Total flow  volume for sub-basin floods of l-< and 7-day-
           durations and return periods of 2, 5f 10, and 25 years .    3-126
3.42       Summary  of  area, discharge, and irrigated acreage for
           the syb-basin, basin, and  regional basin hydrographie
           units in New Mexico	3-127
3.43       Dilution factors for the Rio San Jose, Rio Puerco, and
           Rio Grande  for 1-day flood flows with a 2-year recurrence
           interval  .	    3-135
3.44       Annual contamirrant loading from 14 uranium mines and
           resulting concentrations in sub-basin floods and in the
           average  annual flow of the"Rio San Jose, Rio Puerco, and
           Rio Grande	3-137
3.45.       Comparison  of-'potable-'amTfrrigatton water standards
           and surface water quality affected by underground
          mine drainage. .........    3-140
3.46       Radiochemical and stable element/compound water quality for
          selected acid and alkaline leach uranium mill  tailings
          ponds in the United States	»    3-142
3.47      Summary  of flood runoff water quality and uranium millpond
          quality   ..........    3-143
3,48      Flow and water quality in the Puerco River near Churchrock
          and Gallup,  New Mexico   «„..,.„    3-146
3.49      Groundwater quality in principal aquifers in the Grants
          Mineral  Belt, New Mexico „,.»,«,    3-151
3.50      Groundwater quality associated with the San Matea Creek
          and Rio Puerco (west)  drainages in the Grants  Mineral
          Belt,  New Mexico    ........    3-154
                                    xix

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                                                                      Page

3.51      Estimated annual radon-222 emissions from underground
          uranium mining sources    ,...,,,    3-158
3.52      Estimated air pollutant emissions from heavy-duty equipment
          at underground uranium mines  ......    3-161
3.53      Estimated average annual  dust emissions from underground
          mining activities   ........    3-163
3,54      Average annual-emissions  of radionuclides (pCi) and-
          stable elements (kg) from mining activities at the
          model underground mines.  .-         .     .     .     .      .    3-165
3.55      Average annual emissions-of radionuclides (uCi)-and
          stable elements (kg) in wind suspended dust at the model
          underground mines   .........    3-166
3.56     '"Average-annual emissions  of radionuclides (yCi) and stable
          elementst (kg)* from:.veWculajrdusfc.at, the/mGdel  -underground ,•?  , •
          mines     	.    .          ...      .    3,-167
3.57      Estimated, quantities of wastewater produced fay.an in situ
          leaching operation  ........    3-173
3.58      Estimated*'average concentrations, and1,annua.l • accumulation
          of some contaminants in waste water     ....    3-175
3.59      Estimated average-annual  airborne emissions from-the-
          hypothetical in situ leaching facility  ....    3-176
j 60      Estimated average concentrations and annual and total
          accumulations of some contaminants in restoration waste-
          water     	    3-181
3.61      A comparison of contaminant concentrations in pre-mining
          groundwater and pre-restoration mine water   .     .      .    3-182
3.62      Estimates of exploratory  and development drill  holes
          (1948-1979)    .     .   •	      .    3-189
3,63      Estimated source terms per bore hole for contemporary
          surface drilling for uranium  ......    3-195
3.64      Airborne dusts produced at an average mine site from
          exploratory and development drilling    ....    3-196
                                    xx

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                                                                      Page

3.65      Estimates of emissions from drill rig diesel power
          source    ..........    3-196
3,66      Sediment yields in overland flow from uranium mining
          areas     ..........    3-202
3.67      Consolidated list of inactive uranium producers by State
          and type of mining	3-206
3.68      Uranium mine waste and ore production   ....    3-207-
3.69      Cumulative uranium mine waste and ore production  .     .    3-211
3.70 ...   Average annual emissions af raxLionuclides, ( ^ C.i) and stable., .
          elements (kg) in wind suspended dust at the model inactive
          surface mine        .     .    .    .    .     .     .     .    3-217
3.71  ,    Average radon flux of inactive uranium mill tailings
        '  piles,     .	3-218
3.72      Average radon,flux .measured.*at'inactive, uranium mine.   ,
          sites	3-220
3.73      Background radon fTux estimates  •  .    .     .     .     .    3-221
3.74      Summary of estimated radon~222 releases from inactive
          surface mines. .........    3-223
3.75      Summary of land surface gamma radiation surveys in New
          Mexico, Texas, and Wyoming    ......    3-225
3.76      Average annual emissions of radionuclides (uCi) and
          stable elements (kg) in wind suspended dust at the model
          inactive underground mine     ......    3-231
3.77      Summary of radon-222 releases from inactive underground
          mines	3-238
3.78      Summary of land surface gamma radiation surveys in
          Colorado and New Mexico  .......    3-239
5,1       Number of uranium mines and population statistics for
          counties containing uranium mines. .....    5-3
5.2       Population statistics for humans and beef cattle  .     .    5-12
5.3       Aquatic environmental  transport pathways initially
          considered     .........    5-14
                                    xxi

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                                                                       Page

6.1       Annual  release  rates  (Ci)  used  in  the  dose  equivalent
          and  health  effects  computations  for  active  uranium
          mines      .....,,,,.     6-2
6.2       Annual  release  rates  (Ci)  used  in  the  dose  equivalent
          and  health  effects  computations  for  inactive  uranium
          mines      ..........     6-4
6,3       Annual  working  level  exposure from radon-222  emissions
          from model  uranium  mines  .......     6-6
6.4       -Annual  radiation dose equivalents  due  to  atmospheric  radio-
          active  particulate  and Rn-222 emissions'from  a  model  average
          surface uranium mine      .......     6-7
6,5       Annual  radiation dose equivalents  due  to  atmospheric  radio-
          active  particulata. and,.Rn-222 .emissions from  a  model  average
          large;surfacie uranium mine'4,-  -.;  . .    .     ..     .     .     6-8
6.6       Annual  radiation tloste' equivalents'due  to  atmospheric* radio-   ",
          jctive^partfcul'dtff and'-in~222"€mts&tans"froniw model.-ayerag-e .
          underground uranium mine  .......     6-9
6,7       Annual  radiation dose^equivalents  due  to  atmospheric  radio-
          active  particulate  and Rn-222 emissions from  a  model  average
          large underground uranium  mine,,   .    .,    .  ,        .     6-10
f,8.      Annual  radiation dose equivalents  due  to  atmospheric  radio-  /.
          active  particulate  and Rn-222 emissions from  a  model  inactive
          surface uranium mine      .......     6-11
6.9       Annual  radiation dose equivalents  due  to  atmospheric  radio-
          active  particulate  and Rn-222 emissions from  a  model  inactive
          underground uranium      .......     6-12
6.10      Annual  radiation dose equivalents  due  to  atmospheric  radio-
          active  particulate  and Rn-222 emissions from  a  hypothetical
          in situ uranium solution mine ......     6-13
6.11      Individual  lifetime fatal  cancer risk  for one year of
          exposure and estimated additional  fatal cancers  to the
          regional population due to annual  radioactive airborne
          amissions. froro'mode],,«uranium.mif)es>'^.  v .*,  .  **.-.  ...    ..     6-15
                                    xxi i

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                                                                      Page

6.12       Individual  lifetime  fatal cancer  risk due  to  lifetime
           exposure  to radioactive  airborne  emissions  from model
           uranium mines   .........    6-16
6.13       Genetic effect  risk  to descendants  for  one  year of  parental
           exposure  to atmospheric  radioactive airborne  emissions  from
           model uranium mines  ........    6-17
6.14       Genetic effect  risk  to descendants  for'a'30-year parental  -
           exposure  to atmospheric  radioactive airborne  emissions
           from model  uranium mines  .  . .  *~         -     ..   .     „   6-18
6.15       Percent of  the  fatal cancer risk  for the maximum individual
           due to the  sources of radioactive emissions at model ura-
          .niurn mines	6-20
6.16       Percent1of-the  fatal cancer risk  for the average individual
           in-the regional population,due,to.vthe.sources of radioactive
           emissions at model uranium mines    .     . "       .     .    6-21
6.17       Percent of  fatal cancer  risks due to radon-222 daughter con-
           centrations at  model uranium mine sites  ....    6-22
6.18       Percent of  the  fatal cancer risk  for principal nucl.ides and
           pathways'due to. radioactive, parttculate and Rn-222 emissions
          at model uranium mines.-   .......    6-23
6.19      Natural background concentrations and average urban concen-
          trations of selected airborne pollutants in the United
          States	6-27
6.20      Combustion  product concentrations at the site of the maximum
           individual  with comparisons   	    6-29
6.21      A comparison of the airborne concentrations of nonradioactive
          gases at the hypothetical in situ leach site with threshold
          limit values    .	6-30
6.22      Stable trace metal  airborne concentrations at the site of
          the maximum  individual	6-32
6.23      Comparison  of stable trace metal  airborne concentrations
          at the location of the maximum individual with natural
          background-concentrations and average urban, concentrations
          of these afrborne pollutants  .         .    ..    .    .,    6-33
                                   xxn i

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                                                                      Page

6.24      Comparison of trace metal airborne concentrations at the
          site of the maximum individual with threshold limit values
          (TLV's) in the workroom environment adjusted for continuous
          exposure to the general public     	    6-34
6,25      Annual radiation dose equivalent rates due to aquatic
          releases from the New Mexico model underground mine     ,    6-36
6,26      Annual radiation dose equivalent rates due to aquatic v
          releases from the Wyoming model surface mine .    .     ,    6-37
6.27      Individual lifetime fatal cancer risk and committed fatal
          cancers to the population residing within the assessment
          areas     ..........    6-38
6.28      Genetic risks to succeeding generations-of-an individual
          and committed genetic effects to descendants of the present
          oopulatitirvresldi'W wittMir-the, assessment-area';  ...    ..  . 6-4L
6,29    ,  Comparisojvaf•nofii^diologlcal,,waiertwrtte>emissions,'from-'.
          uranium mines with, recommended agricultural,water quality.
          limits    .    .    .    .    .    .     .     .    .     .    6-43
6.30   ."  Estimated lifetime, risk of fatal lung cancer-to individuals
          living in homes built on land contaminated by uranium mine
          wastes' •	6-45
6,31      Gamma radiation anomalies and causes    ....    6-49
7.1       Distribution of United States uranium mines by type of  '•
          mine and state .,,.,...,    7-2
7.2       Sources of contaminants at uranium mines     .    .     .    7-3
7,3       Concentration of contaminants in waste rock (overburden),
          ore, and sub-ore	         7-6
7.4       Summary of harm from radioactive airborne emissions of
          model uranium mines „•              	7-11
7.5       Percent additional lifetime fatal cancer risk for a lifetime
          exposure to the individual and the percent additional  cancer
          deaths in the regional population per year of exposure esti-
          mated to occur as a result of uranium mining .    .     .    7-12

                                   xxiv

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                                                                       Page

 7.6        Summary  of  the  fatal  cancer  risks  caused  by radioactive
           aqueous  emissions  from  model  uranium  mines    ,     .     ,     7-14
 7,7        Estimated lifetime risk of fatal  lung cancer to  the  average
           person living in a hope built on land contaminated by uranium
           mine  wastes     .    .....     .               7-16
 7,8        Summary  of  contaminant  loading  and stream water  quality from
           a model  surface uranium mine   ,     .     .     .     »     ,     7-20
 7.9        Summary  of  contaminant  loading  and stream water  quality
           from  a model "underground uranium mine   ....     7-Z1

 Appendix A
 A.I        Federal  laws,  regulations, and  guides for uranium  mining     A-l
0.1       State laws,  regulations,  and  guides  for. uranium  mining,.     D-t

Appendix E
E.I       Active uran;tuffl,»irwieSLim,the',Un,1 ted, .States--  -•'."»,    .     «     E-l -

Appendix F
f.l       Inactive uranium mines  in the United States                  F-l

Appendix G
G.I       Uravan and Jamestown areas    ......     6-14
G.2       Inactive uranium mine sites surveyed in  New Mexico      .     G-21
G.3       Status and location of  uranium mines in  Texas.     .     .     G-25
G.4       Trace elements and radionuclides  in water in  the south
          fork of Box  Creek drainage at UNC  Morton Ranch lease    ,     G-35
G.5       Radionuclides and trace metals  in  sediments in the south
          fork of Box  Creek at UNC  Morton Ranch  lease   ,     .     ,     G-36
G.6       Radionuclides and trace metals  in  soils  near  the 1601
          open pit mine, UNC Morton Ranch lease, Wyoming     .     .     G-37
                                    xxv

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                                                                       Page

G.7       Radionuclides  and trace metals in soil  profiles at the
          open  pit mines,  UNC  Morton Ranch lease, Wyoming   .    .    G-38
G.8       Radionuclides  and trace metals in sediments from the
          drainage of the  San  Mateo mine and from San Mateo
          Creek,  New Mexico   ........    G-40
G.9       Radium-226 and trace elements  in water  from San Mateo
          Creek near San Mateo mine discharge point    .     .    .    G-40"

Appendix H
H.I       Characteristics  of the sub-basin containing the model
          mines ...........    H-2
H.2       Seepage and outflow  calculations for the Wyoming model
          mine  drainage  system     .......    H-6
H.3"-       Characterrstf-cs1.  oft the-'sub^baam'.'hydf ogiraphic/ ant fi" it--the--.
          ,nodel~ underground'uranium-nrliifr-area* ,-,  t .    ..  .. ...    ..    H-8'.
H.4       Seepage, and, outfJon, calcu) a kiojis.^ai1?, the. New- Mexico ,. ...
          model mine area  drainage system	H-ll

Appendix J
J.I       Aquatic environmental  transport pathways examined .    .    J-6
ii.2       Characteristics  of the generic sites     ....    J-20
j.j       Stream  data for  Valencia County   j.     .    .     .    .    j-23
J.4       Estimation of  meat production  in Valencia County for
          1977  ...........    J-2o
J.5       Estimates  of meat production  in Converse County,
          Wyoming for 1976    ........    J-26
J.6       Annual  radionuclide  release rates to  streams for active
          uranium mines  .     .'         .    .     .    .     .    .    J-29
J.7       Freshwater fish  concentration  factors   ....    J-29
J.8       Normalized  human intake  rate factors  for radionuclide
          uptake  via  plant root  systems  ......    J-31
J.9       Irrigated  land usage	J-31

                                    xxvi

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                                                                       Page

 J.10      Soil  removal  rate constants and radioactive decay
           constants	J-33
 0.11      Milk  and beef concentration factors     ....     J-33
 J.12      Dose  equivalent conversion factors  .....     0-36
 J.13      Health effects conversion factors for internal  pathways.     J-37
 J.14      Health effects conversion factors for external  pathways.     J-37

 Appendix  K
 K.I  ,„    Characteristics, of the.generic sites    .          .    .     K-l
 K.2       Animal  and vegetable crop distribution for use  with
           AIRDOS-EPA     .........     K-3
 K.3       Sources of food for the maximum individual (percent)    .     K-4
 K.4       Seltcted input parameters to AIRDOS-EPA                     K-5
,K.5 .      Selected terrestrial- pathway parameters, by radJonucl.ide.     K-7
 K.6       Effective radioactive decay constants   ....     K-8

 Appendix__L
•L.I       Radionuclide  dose rate and health effect risk conversion. <
           factors used  1n uranium mine.assessments    ' .     .    .     L-4
 L.2       Additional Input data used by DARTAB in the health im-
           pact  assessment of airborne emissions   ....     1-21
 L.3       Example input data file for DARTAB  .....     1-22
 L.4'       Maximum individual  fatal  cancer risk for one year of  ex-
           posure to atmospheric radioactive emissions from model
           uranium mines  .........     L-23
 1,5       Fatal  cancer  risk to an average individual in the regional
           population for one year of exposure to atmospheric radio-
           active  emissions from mods!  uranium mines     .     .    ,     L-24
 L.6       Fatal  cancer  risk to the population for one year of ex-
           posure  to atmospheric radioactive emissions from model
           uranium mines  .........     L.-2S
                                     XXV11

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                                                                      Page

1.7       Genetic effect risk to descendants of maximum exposed
          Individual for one year of parental exposure to atmo-
          spheric radioactive particulate and Rn-222 emissions from
          model uranium mines ........    1-26
L.8       Genetic effect risk to descendants of average individual
          of the population for one year of parental exposure to
          atmospheric radioactive particulate «rnd Rn-222' emisstons
          from model uranium mines ..,,...    L-27
L.9       Genetic effect risk to descendants of the regional popu-
          lation for one year of parenta-l exposure to atmospheric- •
          radioactive particulates and.Rn-222 emissions from model
          uranium: mines 'V         .    .    »    .    .    .     .    L-28
                                   xxviii

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                                 FOREWORD
     The Uranium Mill Tailings Radiation Control Act of 1978 stipulates
that "...the Administrator, in consultation with the Commission, shall
provide to  the Congress a report which identifies the location and
potential health, safety, and environmental hazards of uranium mine
wastes together with recommendations, if any, for a program to eliminate
these hazards."  It is our understanding that the intent of Congress was
to determine if remedial actions similar to those for uranium mill
tailings are required for mine wastes.

     The report was prepared by.the Office of Radiation Programs and
addresses potential health effects caused by air emissions, water
effluents^  and so-lid wastes at active and inactive uranium.mines,*  Lt Is
probably the single most comprehensive report on the subject.  The
effects from other mining activities such as exploration, site
preparation, and in situ leaching were evaluated in proportion to their
potential significance and the amount of available information about
them.  Comments on this report from the uranium mining industry, States,
and the Nuclear Regulatory--Commission have also.been considered.

     The conclusions' and* recommendations- are--in they Executive Symnary and
Chapter 7 of the report.  The principal findings of this report are as
follows:

     1.  No problems were identified that require Congressional action.

     2.  Standards, *re probably- needed, to, control, human exposure from
radioactive emissions.from underground uranium mines.•  We have proposed a
standard for underground uranium mines under the Clean Air Act program to
develop radionuclide standards.

     3.  Regulations should be considered for maintaining the control of
solid wastes at active uranium mines to prevent off-site use and to
minimize the health risks from these materials.  This is part of the
overall agency consideration of mining wastes and is being carried out
under the auspices of the Solid Uaste Disposal  Act.

     4.  The report also identifies additional  studies that are needed to
completely elucidate the potential  for local  adverse effects as a result
of possible misuse of the mine waste materials in construction of
buildings.   Preliminary reports of field studies by EPA identifying
possible sites at which mine wastes may have been utilized in
construction or around buildings have been sent to the States for
follow-up studies.
                                             Glen L.  Sjoblom,  Director
                                             Office of Radiation Programs
                                KX1X

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                              ACKNOWLEDGEMENTS

      The  following persons of the Office  of Radiation  Programs  made
 substantial  contributions  to this report.

                   R. L. Blanchard, EERF,  Montgomery, AL*
 G.  G.  Eadie,  ORP-Las Vegas,  NY*        P.  J.  Magno,  CSD,  Washington,  DC
 T.  W.  Fowler,  EERF,  Montgomery, AL     J.  M.  Moore,  ORP-Las  Vegas, NV
 M.  M,  Gottlieb,  TAD,  Washington;  DC     D-  Nelson,  CSD, Washington, QC,<  •
 J.  M.  Hans,  Jr.,  ORP-Las Vegas, NV*     M.  F.  O'Connell, ORP-Las Vegas, NV
 T.  R.  Horton,  EERF,  Montgomery, AL     C.  M.  Petko,  EERF, Montgomery, AL
 T.  L.  Hurst,. ORP-Las  Vegas,  NV         J.  E.  Regnier, CSD, Washington, DC
 R.  F.  Kaufnann,  ORP-Las Vegas,  NV*     J.  S.  Silhanek, CSD,  Washington, DC
                                        J.  M.  Smith,  EERF, Montgomery, AL
*  Principa.1 Authors,-,1-.'  ,      .  •

     The following persons "provided data and  information used  in this report.

L. V. Beal, U.S. Geolog.ical Survey, .Albuquerque,, NM  ..       ,       .   ,
R. Beckman, U.S. Dept. of Labor, Denver, CO
J. D. Borland, U.S. Geological Survey,, Albuquerque,, NM
T. Buehl, Mew Mexico Environmental Protection Agency, Santa. Fe, NM. •
T. Bullock, Utah Industrial Commission, Salt Lake City, UT
A. 'J. Carroll, U.S. Dept. of  Interior, Denver, CO
T. Chung, U.S. Dept. of Energy, Grand Junction,  CO
L. M. Cook, Texas Dept. of Health, Austin, TX
J. T. Dale, USEPA, Region VIII, Denver, CO
J. G. Dudley, NM Environmental Improvement Div.,  Santa Fe,  NM
W. H. Engelmann, U.S.  Bureau  of Mines, Twin Cities, MI
J. R. Giedt, USEPA, Region VIII, Denver, CO
A. L. Hornbaker, Colorado Geological Survey, Denver, CO
S. J. Hubbard, IERL, USEPA, Cincinnati, OH
R. G. Kirby,~ USEPA, Effluent  Guidelines Division, Washington,  DC
                                    xxx

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J. L. Kunkler,  U.S. Geological  Survey, Santa Fe,  NM
H. W. Lov/hara, U.S. Geological Survey, Cheyenne, WY
H. D. May, USEPA, Region  VI, Dallas, TX
R. Meehan, U.S. Dept. of  Energy,  Grand Junction,  CO
A. T. Mullins,  TVA, Chattanooga,  TN
G. E. Niewiadomski, U.S.  Geological  Survey, Washington,  DC
B. L. Perkins,  Key Mexico Energy  and Minerals Department, Santa Fe, NM
C. R. Phillips, USEPA, EERF, Montgomery, AL
H. G. Plimpton, MSHA, Salt Lake City, UT
T. J. Price, Bendix Field Engineering Corp., Grand Junction, CO
J. G. Ra-nkl, U.S. Geological Sur-vey, Cheyenne,.. WY
R. F. Reed, U.S. Bureau of Mines, Washington, DC
G. C. Ritter, Bendix Field Engineering Corp., Grand Junction, CO
P. B. Smith, USEPA, Region VIII,  Denver, CO
J. P. Stone, U.S. Dept. of Interior, Washington,  DC ,
A.. B.. Tanner, U.S., Geological, Survey K.Reston, VA,.
S. Waligora, Eberline Inst. Co.,  Albuquerque, NM
R. E. Walline,  USEPA, Region VIII, Denver, CO
T. Willingham,  USEPA, Region VIII, Denver, CO
T. Wolff, New Mexico-.Environmental Protection. Agency, Santa .Fe, Ml
A. F. Wright, (formerly)  U.S. Geological Survey, Albuquerque,, NM
     The authors express their appreciation to Mrs. Winnifred Schupp,
ORP-Las Vegas, NY, and Mrs. Annette Fannin, EERF, Montgomery, AL, for
typing the-report and to Mrs. Edith Boyd, ORP-Las Vegas, NV, for pre-
liminary editing of the report.
                                    XXXT

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  SECTION* 1
INTRODUCTION

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                                                                      1-1
1.0   Introduction
1.10 Purpose
     This  report was  prepared  in  response  to Section  114(c)  of Public  Law
95-604  dated  November  8,  1978 (USC78).  This  Section of th'e Law stipulates
that, "Not later than January 1,  1980,  the Administrator,  in  consultation  with
the Comm4ssion-f-  shall-provide to- the  Congres-s  a  report which -identifies  the-
location  and  potential  health, safety,  and  environmental  hazards of  uranium
mine wastes together with recommendations, if any,  for a  program  to eliminate
these hazards."  The purpose of this  report  is to comply  fully with  this  re-
quest,  as accurately-and completely •as available  information  will   permit,

1.1.1  Contents
     This  volume has seven  major  sections.  The  content  of each section  is
described generally below:
     Section  1;  Brief reviews,, of  predicted fu.ture  uranium production  require-
     ments;   descriptions  of methods  of extracting--uranium from the  earth;
     and  presently  enforced  standards  and  regulations governing   uranium
     mining,
     Section  2:  A description  of the  active  and  inactive  uranium mine  in-
     ventory with a  discussion  of  its limitations.  The actual mine  listings
     are presented in Appendixes  E  and F.
   •  Section  3:  A  comprehensive  discussion  of  potential sources of  radio-
     active and  stable  contaminants to  the  environment  and  man from  uranium
     mining operations.  Annual  release  rates of contaminants from the  identi-
     fied sources computed on a generic  basis.
     Section  4:   A  description  of model  underground,  surface,  and  in situ
     leach mines with  operational  parameters  and  source terms.   Both  active
     and inactive model underground and  surface mines  are  described.
     Section  5:   A brief  and  general  discussion  of  the  environment that
     exists about  uranium  mines,  including vegetation,  wildlife,  domestic
     animals,  and  human populations.';. The,potential atmospheric and  aquatic
     pathways-' of/-contaminants .from^'the m,tnes-*ta:.'man.>are a:tso. defined/, ,  ,

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                                                                      1-2
     Section   6:   Computation  of  Individual  and population  dose  equivalents
     and  potential  health  effects from  mine  wastes  and  effluents based  on
     the  source  terms  developed  in  Section  3,  the  model  mines  defined  in
     Section  4,  and   the  pathways described  in  Section  5.   A  qualitative
     description  of  the  environmental  effects  based  on site visits is
     also presented.
     Section   7:   A  brief summary of  the report- followed  by .the* conclusions!
     and recommendations.

1.2  Uranium-Ore  Production  and Future  Uranium Needs
1-2.1      Past  Production
     Tabl.e/1.1'. listSi the ^quantities./.of  ore mined  and=uranium (U-jQo)  produced ,
in .the various-uranium mining  states-between,119.48 and. January .1, 1979,   Two'
states, New Mexico and Wyoming,  have, been the source  of  about 64 percent of
Che'uranruffl minech in-the' United"'Statesv''The-Colorado* Plateaui  which--Includes -
parts  of  New Mexico, Arizona,  Colorado,, and Utah  (see  Figure  1.1),  has  been
the  largest "source area of mined uranium,  accounting  for  about 70 percent of
the  UgOg  production  through  1976  (ST78).   During this same period,  the  Gas
Hills  and the  Shirley  and Powder  River  Basins  of Wyoming, produced  about 22,,
percent of the  total UjOg  (ST78).
     To produce 302,370 MT of  U.00 required the  mining of 145,811,000 MT of
                                J O
uranium ore  during the 31-year period  from 1948  to 1979(OOE79).   The average
grade  of  ore,  reported as  percent of  UJL,  was  0.208 percent  during  this
period.

1-2.2     Projected Needs  for Uranium
     The  expected  growth  in the  use  of  nuclear energy  for the pt uduction or ••
electric  power  in  the United States during  the  remainder of this  century  will
require an  expansion  of the uranium mining industry.   However, the magnitude
of this expansion  is difficult to  estimate, because the  forecasts that  pre-
dict the  growth, of  the nuclear  power  industry  differ considerably  (AEC74,
ERDA75,  EPA76,  - NRC75,  NUS76,*/Cu?7,* 'He7-7; 'NER77,', Ew78,"^Ni78;;
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       DM 2000, INC
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    San Antonio, Texas 78219
   (210)222-9124 FAX (210)222-9065
      THIS
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FROM DOCUMENTS
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                                                                 1-4
Figure 1 1  Uranium mining regions, m-the, western United States

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                                                                      1-5
      Table  1.2 gives examples  of  four typical forecasts.  The  Nuclear Regu-
 latory  Commission's  (NRC)  projected  annual  nuclear capacity  is  far  below
 former  predictions.  This lower projection,  which is 1n line with the admin-
 istration's  National  Energy  Plan  (NEP77),  is believed to be more realistic  in
 view of recent  drops in  demand  for  electricity,  labor problems,  equipment
 delays,  litigations  initiated  by  environmental  groups,  the, absence^- of-. a -
 publicly  accepted  waste  disposal  program,  and concern over  nuclear  prolif-
 eration.   The Department of  Energy  predicts that 293,120 MT  of U30& will  be
 required  to provide  nuclear generating  capacity through 1990  (DQE79).   This
 assumes no uranium  or plutonium recycling.

      Table  1.3,  which  gives domestic uranium reserves by state,  shows  that
 the  reserves are near the areas already mined.  Figure  1.2 shows the  distri-
 bution  of $50 ore  reserves  by  state,  and  F1g." 1.3" shows reserves by resource
 region  (see  Fig. l.l for  region  locations).   Future major, mining activities
 probably  will  be in  the-same general  areas'1 that have'already beerr mined.   To
 obtain  the  834»600 MT of  $50 U~0H reserves will  require mining about 1.14 x
  g                             JO
 10   MT of ore  with-an. average grade-of OV0731 percent?'UgQw.

 1.3   Oyerview  of Uraniurn Jlini ngOperations

 1.3.1     General
      The  two  major  uranium  mining methods  used  in the  United States are
 underground  mining  and  surface  (open  pit)  mining.  These  two  methods ac-
 counted for  more than 98 percent of  the  uranium mined in the  United  States  in
 1971  (AEC74).  This  has  decreased  only  slightly  to  about 93  percent  in  1978
 (DOE79).   However,  various  types  of  solution  mining  are  currently  being
 tested and probably will be  employed commercially more  frequently.

      Table 1.4 shows  the current  production capacities  of U30g  for the  var-
 ious  mining  methods.   Although underground  mines  are far more  numerous  than
 surface mines,  production by the  two methods  is  nearly equal.   This  is be-
 cause surface, mines  have  a   much  larger .capacity.   During 1978, 305 under-
 ground mines accounted, for about .46.percent  (8»350 MT) of the U^0g production
while 63  surface mines  produced about 47  percent"(8,710 HT)  of  the  l^Og.   In
situ  leach,in§r  heap Bleaching*  'mine- water*1 extraction-?  antf- otter alternative"1'
 methods accounted for the  renaitiinf •?  percent/(V;27
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                                                                 1-6
      Table 1.2  Projected annual nuclear capacity (GWe) in  the U.S.
Source
ERDMERQA75>
USEPA (EPA76)
Electric World (EW78)
NRC (NRC79)(a*
1980
71-92
80
, 92
61
1985
,160-245
188
160
127
1990
. 285-470
350
194
195
1995
445-790
578
237
280
2000
625-1250
820 •
380
^'Schedule, .assumed- for "this document;,,' -
Note.—The, actual nuclear -capacity, real ized irt 197T Wasv

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                                                                     1-7
                    Table 1.3 Domestic uranium reserves by state
                                as of January 1, 1979

State
New Mexico ,
Wyoming
Texas
Arizona,
Colorado,
& Utah.
Others(a)
Total

Ore
Ore, MT Grade, % U308
, 482,2 QQJQOOU,
431,300,000
83,400,000

>
• 107,300,000
35,700,000
1,139,900,000
0.09,.,
0.06
0.05


0.07
0.07
O.Q73>(b)

U3°8> MT'^
^34,000
258,800
41,700


75,100
25,000
834,600-

£ Total U0OX '
6 a
52 -
31
5


9,
3
100
     (a)
        Includes Alaska, California, Idaho, Montana, Nevada, North Dakota,
Oregon,"South Dakota and •Washington.
     '  ^Weighted average.
     Note.--The uranium reserves in this table include ore from which ILQ0 can
     	                                                              J o
be obtained at a forward cost of $50 per pound or less.  Costs do not include
profits or cost of money.
     Source:  DOE79.

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                                                                    1-8
                                        '  • Ariz-; Colo;; Uta*v49%)
Figure 1 2- The percent of S5Q U ap 8 reseryes,located,m the.
           principal m»nmg states.(DOE-79).,,

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                                                                                 1-9
                              Colorado Plateau (54%)
Northern Plams(1%)

         Other (9%)
                               Wyoming Basins (31%)
The perceo, „, $60 U3 o8
various mining regions (DOE 79)
                                                    ,o=a«M ,„

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                                                                  1-10
      Table 1.4      Quantities of lUOg produced  in  1978
                     by the various mining methods
Mining Method
Underground Mines (305) ^
Surface Mines (63)
Other (23): In situ leaching,
heap leaching, & mine water
Total
-'MT'of U30g
- 8350
8710

1270
18,330
Percent^.-.
46
47

7
100
        number' of .oai-nas- j or/ 3 i-tes,'.
   'Rounded  to. totaMOO"- percentv. •
Source:  ,OOE79^.  ...   •
     Table  1.5   Predicted methods of mining ore reserves  •
Mining Method
Underground Mining
Surface Mining
Other: In situ leaching.
heap leaching, & mine water
Total
MT of U308
547,000
260,400

27,200
834,600
Percent
66
31

3

Note.--These  are  reserves of the1 $50 per pound U.,CL or less cost  category.
*•--*	                                             *5 o
Source:  DOE79.

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                                                                      1-11
     Although  some mines  produced much  more  than others, one can  compute  a
 rough  estimate  of the  average  capacity of underground and  surface mines as
 follows.   The  average  grades  of  ore removed  from  underground and  surface
 mines  in  1978 were  reported  to  be  0.155 percent  and  0,120 percent  UqOg,
 respectively  (OOE79).   Dividing  the  annual  ILOg productions  (Table  1.4} of
 the  two  mining methods  by their,  respective  grades  indicates  that  the  305
 underground  mines  accounted for  5,387,100  MT  of ore while  7,258,300  MT were
 removed  from the 63  surface mines.  Hence, the  average ore  production capac-
                                                            4                c
 ities  of underground and  surface mines  are about 1.8  x  10   MT and  1.2  x 10'"'
 MT,  respectively.   From this assessment,  the  average ore capacity  of a sur-
 face mine  is about  seven times  that of an underground mine.

     The  trend.during the  past  few,years of an  increasing percentage  of U30g
 being  mirred  underground  will continue, because'shallow deposits of  high  grade
 ore  have  tended to-be, surface, mined first.   Table 1.5, which  displays  the
 distribution of-$50  reserves'-by  mining  method,- shows  the continued increase
 in the proportion of  LLOg  mined  by the underground method.  By the  Department
 of ' Energy  predictions',  future- production^ from'  underground";mines   will  more
 than double  that from surface mines.  The  NRC predicts u*30g production  by in
 situ leaching  to peak in  1990  at about  4000 MT/yr and total  76,000  MT by the
 year 2000 (NRC79).   If  this prediction  is realized, this resource will  un-
 doubtedly  draw from those  assigned  to  underground and surface mining in  Table
 1.5.   The production  of U,0« by  heap leaching  and mine  water extraction is
 predicted  to be  relatively small.

     It  is very difficult to predict how much  ILQg will  be produced  as  a
 by-product  from other mineral  mines, but  by-product  production should  in-
 crease total ILQg  production during  the next  20 years.   Approximately 180 MT
 of U000 are currently recovered each year from the phosphoric acid  production
    J Q
 at wet phosphate plants.   The  NRC predicts  that this will   increase  to 1800
 MT/yr by 1985-and possibly to 7000  MT/yr by the  year  2000 (NRC79),  If  planned
 leaching  facilities  are  actually built  at copper waste  dumps at Yerington,
 Nevada; Butte, Montana;  and Twin  Buttes,  Arizona,  to  supplement the  operating
 facility  at Bingham  Canyon,- Utah,  recovery  of,  UJDQ-from, .these operations,
could  reach 900 MT/yr  (NRC78).'  Hence,  by-product  UgOg   production  could
conceivably account  for  about^ eight: percent --of *-the- requvt-red* annual- ItjOg pro«,
duction.by the year 2QOQ.

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                                                                      1-12
      Although the depth  of  the ore deposit  is  the fundamental consideration
 in  selecting  the  mining method to  be  applied to  a  particular ore body, the
 size  and grade of  the  deposit are  also  important factors.  The shape of the
 deposit,  the overburden  rock  strength,  environmental   considerations,  and
 other factors may also  Influence  the selection.  Surface mining is generally
 used  for  relatively shallow  deposits;, rarely for those,-, be law, 400 feat.-{S±7#)v-u".
 However,  under some conditions,  it may be cheaper to mine a small, shallow,
 high-grade  ore deposit  by underground  methods;  whereas,  a  larger low-grade
 deposit at  a  greater depth may be  cheaper to mine by surface mining.  Because
 productivity  is greater  by   surface mining,   it  is generally  preferred  when
 conditions, are favorable.. .Other  factors, must  be  examined  when considering
 the use of  in situ .leaching, (see Section, 1^3.4)».

 1.3.2.  Surface Mining.    ..-
      The  use of  surface (open  pit)'1 mining methods 1s most' prevalentM'n the
 Gas• -Hills"  Region 'and' "the" ShrirTey  and' Pow'der RIVer" Baslrts" ftr%oming,  the '
 Laguna  District of  New, Mexico,^the, coastaL plains, in south Texas,, and  some
 areas  of  Colorado and Utah  (St78).  Fig.  1.4  illustrates  a  typical open pit
 mine.
      In surface mining,- an  open  pit  is  dug  to  expose the'uranium deposits;  •
 After the topsail  is  removed  and stockpiled nearby, the overburden is removed  • ••
 by the  method best suited to the nature  of  the rock.  If the  rock is easily
 crumbled, it  is  removed by  tractor-mounted ripper bars,  bulldozers, shovels,- ••
 or pushload  scrapers; if  it  is not, blasting  and drilling are required. The
 broken  rock  is then trucked  to a  nearby  waste dump.  Occasionally, dikes and
 ditches are constructed  around these waste piles to collect runoff and divert
 it to  sedimentation ponds.   Overall,  an  area of  a  hundred or  more acres may
 be covered by stored overburden wastes  (AEC74).
     As mining  progresses, the  overburden  is used as  it  is  removed to back-
 fill   mined  out areas of  the  pit.   When an area  is completely  backfilled, it
 is graded to  conform to  the  surrounding topography and to restore the natural
drainage, patterns,-  .The  area. H thert cohered .with t/jpsalL.and-seeded, to Wend  .,
with'the  na-ttiral   terra.in.v  .Most '-of the-: older; surface" rotnes1' 'were  not" back^v-
 filled  (see,"  Section, 3.7.1):,.;, and ne.it her a re''-many/of the- curretitlyv. active :
surface mines.

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Figure 1 4 Artist's conception of open pit mining operation and support faciJities (TVA78a)

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                                                                      1-14
      Contact  with  the  ore zone  is determined  by gamma  and x-ray detection
 instruments,  usually Geiger-Mul ler counters  that have been calibrated to in-
 dicate  the uranium content of the  rock.   Since uranium  is  usually in sand-
 stone formations,  the  ore is  easily removed.   Large  backhoes  and front-end
 loaders  are  often  used  to  remove ore  that  has been  loosened  with tractor-
 mounted  rippers.   Large  ore  trucks  carry the ore  from the pit-to stockpiles^
 at  the  mine  or "the mill.  Uranium ore  is  usually stockpiled by grade, e.g.,
 high-grade,   average-grade,  low-grade.   Sub-ore grade  rock  is  also  usually
 stored  separately  in  piles.   This  is  rock  that contains ILQg at a  concen-
 tration  below what the mill  will  now accept, but  which might later be-worth
 recovering.

      Drifts, (small  .tunnel s)«are sometimes drlvea into, the pit .wall to  recover
 small',  narrow ore"-'podsr,   Tne^jdrifCs' are" generalTy*short; sometimes'less than
 30  meters. ,  The "mining  techniques  in  these", drifts' a re*, like   those  used  in
 underground-rritvifnj  (see* $ectton\4^3i'3}.VJ.  •  ';.

      Surfdce'-ntinfng* requires a" network of roads from'and Taraund the pit area
 and  to  the mill.   Heavy   vehicles  operating  on  these  roads, and  the  digging
 itself, produce a certain amount  of rock and  ore-dust.   However, the, dust can*
 bo kept down  by routinely sprinkling  the roads with water or using other dust
 suppressants.   Treated water from the sedimentation ponds is  sometimes  used
 for this purpose.

      The ratio of overburden  to  the ore produced in an open pit mine can vary
 from  10:1  to as  high  as  80:1  (St78).   One source has  estimated  the  average
 ratio as  30:1 (Le77).  A recent  study of eight large  open pit uranium mines
 reported a  ratio  of 77 (± 36)  to 1  (N179).   Since the latter  study  did  no"".
 consider the  many smaller surface mines where the overburden to ore ratio is
 likely to  be  smaller than 77 to  1, this  report will  assume  an average ratio
of 50:1.   Considering  that  the average ore  capacity  of an open  pit  mine  is
approximately  1.2  x 105  MT/yr  (see  Section 1.3.1),  about 6 x 10  MT of over-
 burden; must- be removed-/  annualTy,--anrt -initially\stored^on.-, 'the. surface until'.-
reclamation procedures  can -be,' initiated'. --        •       '

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                                                                      1-15
      Since  most uranium deposits  lie  below the water table,  groundwater must
 be  prevented from  flooding the mining  area.   One method is to  surround  the
 pit  with several large  capacity wells to lower the water table near the pit.
 This  water  is discharged directly  into the natural  surface  drainage  system,
 in   accordance   with   the   National  Pollutant  Discharge  Elimination  System
 (NPDES)  discharge  permit   issued  to,  the mining  company.   I/slater: that  dpes.
 collect  in   the  pit (mine  sump water)  is  pumped  to a sedimentation pond  for
 solids removal  and, if necessary,  for  subsequent  treatment prior to discharge
 into  the natural  drainage  system.  Another mine  dewatering procedure  often
 used  consists of ditches dug  along  the interior perimeter of  the pit floor to
 channel  the water  to sumps  located  at  the lowest levels of  the  pit  floor.
 Water that  collects   in  the  sumps  is  pumped  to  one  or more  sedimentation
 basins for  solids  removal„„possible treatment, and final, discharge into  the
 existing  natural drainage  system  in accordance-with water-quality standards
 specified .in the NPDES  permit.  The rates,at which mines are dewatered  range
 from  0.28 m3/min"to1 288 m3/mirr (AEG74, TVA78a,-  NRC77a,-NRC77b-J.

      Barium ' cWffrfde'i  to1 coprecijri ta-te-" rad-Tunr, -and-,a.- flocculent- (an  agent
 causing  aggregate  formation)  to remove other contaminants are  usually  added
 to  pond  water  before it is discharged.   Water with a high  concentration  of
 dissolved uranium  is  often run through  ion exchange columns,  and  the  resin
 regenerant  solution  containing the  uranium  is  sent  to  the  mill for  pro-
 cessing.   The  precipitated  sludge that  collects  on the  pond bottom consists
 primarily  of  ferric  and   calcium  hydroxides,  calcium  sulfate,  and  barium
 sulfate  with  coprecipitated radium.   At  some sites, this precipitated  sludge
 is transferred  to  the mill tailings pond  at the end of  the mining operation.

      A small  amount of uncontrolled seepage may occur through  the bottom of
 sedimentation  ponds and, depending  upon  soil  permeability  and direction  of
 flow, may enter the water  table.   For example, the  seepage  rate  through  the
 bottoms of  two  settling  ponds  totaling 4.9  hectares at one site was less than
 0.57  m /min  (NRC77a).   In addition,  seepage  can  be reduced  by  lining  the
 ponds  (well-compacted  bentonite clay  is  sometimes  used  for this purpose),  and
by the sludge that .accumulates, on..the .pond  bottom., -           ..     ,.

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                                                                      1-16
      During  active  surface mining  operations,  a  total  of  several  thousand
hectares  of  land area will  be disturbed (St78, Th79).   When all  uranium has
been  mined  and the  operation  is completed, a pit  remains.   The walls of the
pit  may  be  contoured  and allowed to  fill  with  water, creating a  small  man-
made  lake,

1.3.3  Underground  Mining
      Underground  mining   is much  less  disruptive to the  surface  terrain  than
open  pit  mining.  The surface affected generally  involves  less than 41 hect-
ares,  but the mine  may  extend laterally underground for more than a mile and
at  several   depths.   Figure   1.5  illustrates  a  typical large,  contemporary
underground  mine.

      In underground, mining, access,"  to. the. ore body is.-gained, through one,or
more  vertical-shaftsi  generally, sunk to a slightly greater  depth than the ore
body,  or  through" fnerinesv declines-;  or'-adits; all ''cut" through"1 Waste rock.
The waste rock is  removed  to  a spoils area, that  may be, but usually is not,
surrounded'by  a ditch  to contain runoff,  as discussed above.

      The  sizes of the  accesses vary  considerably.   The,vertical haulage shaft
"say  vary  from  less than 8 feet  in  diameter, sufficient to accommodate, one>
small  ore skip (a  large bucket)» to a diameter  of EQ feet,  which  will accom-
"odate dual  ore skips  as well  as a man and  material  skip.  In some cases, the
near  horizontal  accesses are  sufficiently  large  to  allow  passage  of  large
diesel-powered vehicles.

      Underground  mines are  developed  in  a  way that minimizes  the  removal  of
waste  rock,   resulting  in  much  smaller  spoil  storage  piles  than  those  at
surface mines.  It  is estimated  that  the  ore to  waste  rock ratio generally
ranges  from  20:1  to 1:1 (ACE74,  Th79).   At seven  presently  active mines, the
ore  to waste rock  ratio ranges from  1.5:1  to  16:1  with an  average  ratio  of
9.1:1, (Ja80),., Us.ing.the average  ratio and,the.,average annual .ore..,capacity  of
an • underground' mine--" (see'- Section- 1.3.1JV- each vyear- the-"averagfrunderground
.nine will  -produce-about'2-.Q x ,10  MT. of waste  rock tlrat fs.  removed-andv stored
on the surface.'  Initially'all  waste rock is transported to  the surface, but,

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GENERALIZED UNDERGROUND URANIUM MINE
   MODIIITO DOOM AND PIUAH MIIMOD OF MINING
    Figure 1.5 Generalized underground mine showing modified room and pillar method of mining (TVA78b)

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                                                                       1-18
 as mining progresses,  it is sometimes  transported  to mined-out areas of  the
 mine and retained  beneath  the surface.  This  practice may diminish as  lower
 grade sub-ore becomes  more  economical  to mill.  Since waste rock may contain
 sub-ore, some waste rock will likely be kept available for milling.

      Ore deposits, outlined  by  development drilling, are foil owed- a.s- closely.  ~ •
 as possible.  When ore lies in narrow, long deposits, drifts are cut through
 the ore  body and raises or  stopes  are driven from  the  drift  to reach  small
 ore pods.   Crosscuts  are driven  from  the  haulage  drifts  when necessary to
 reach nearby deposits.   Large  area  deposits are commonly  mined by the  "room
 and pillar"  method.  This involves mining out blocks of ore while leaving  ad-
 jacent  pillars  of  ore  or  waste  as  support for  the roof.  The size of  the
 rooms depends- on. the,  niof  condition..-. The, roof , is  usually strengthened by
 bolts,  wire'.mestr,'  ti'mbersets,  and^ steel '"arches.  Whert an-'area-.ts completely"1
 min^d,  the, ore  pillars'are  removed  in a systematic sequence that-a!Tows safe '
 retreat.'

      Ore is  usually  broken 'by' drTlTin'g'-'anrf blasting. '  Tne  broken  ore is
 removed  and  transferred  to  mine rail cars.  The ore is then carried by rail
 cars  or wheeled  vehicles either directly to the  surface or to a skip at  the  ,
 bottom  of the haulage  shaft  and  lifted to the surface.  Haulage in large area  •->
 mines  is  often   accomplished  by  large  diesel-powered loaders,  haulers,  and
 trucks.   When the ore  is sufficiently soft,  it may be removed with continuous
 mining  machines  instead of  drilling  and blasting  techniques;  however,  most
 ore  bodies are too  small and irregular to mine economically this way.

      Ventilating systems are required  in  underground uranium mines to remove
 blasting  fumes  and  radon-222 (Rn-222)  that emanates  from the  ore  and  mine
water and to control  temperature.  Fresh  air is usually forced down the main
 haulage  shaft and  along the main haulage  drifts to  the working areas.   The
mine  air is  exhausted  through  ventilation  shafts to the surface.  The venti-
 lation air  is diverted  from  inactive areas  of the mine to  reduce air contam-
 ination.  • Inactive8,areas.,arwusually^sea'led, withv* airtight 'bulkheads" to^-pre*« . •
vent  radon." gas-, in  those area:s'"•from1  circulating.   The .ventilation'rate, should
be  sufficient to maintain -the  radon  daughter concentration of the  mine air
at, or- be>owv'leve}:r--ttart 'fleet-' faxsera^emtf'sta-ttf1 occiipatfrnTa^dxpoaKre1-start-- -' •

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                                                                      1-19
dards.   The rate  will  vary depending upon  mine  size (volume), grade of  ex-
posed  ore,  size of the  active  working areas,  rock  characteristics (diffusion
rate  of  Rn-222), effectiveness of  bulkhead  partitions,  atmospheric pressure-,
and other factors.  Ventilation rates  in  active mines vary from a  few hundred
 3                                  3
m /min to over  a hundred  thousand m /min.  For example,  the ventilation  rates
for seven  uranium  mines  in  the Grants, New  Mexico  area  ranged  from 4.4  x  10
            43                                33
to 1.1 x 10 m  /min, with an average of 7.4  x  10  m /min (Ja79).

      Because  ore bodies  often  lie in or beneath major  aquifers,  dewatering
operations  similar to those practiced in surface mining are required.   These
operations  commence during  the  initial shaft-sinking  process and may continue
throughout  the  working- life" of  the1  mine.   Water is  pumped from  wells that  are
driven into the water-bear ing strata- near< the  mining-operation  and discharged-
either directly into  the natural  surface drainage  system, in accordance with
an NPDES  permit, or  to  settling  ponds.   Water that  collects in the mine  is
diverted to sumps and pumped to a settling pond.  The impounded mine water is
treated  similarly   to.  that  described, above, at .surface- mines  (.see  Section
1.3.2). The discharge of water from  these- ponds' is-  in  accordance with  water
quality  standards  specified in the NPDES permit.   (Note.—About one-half  of
the active  New  Mexico mine  discharges have  NPDES permits  that  are presently
under  adjudication  and,  therefore, are   not  necessarily in accord  with dis-
charge limits [Pe79a].)

1.3.4  In Situ  Leaching
      In  situ  leaching has  less adverse  impact on  the environment  than con-
ventional uranium  mining and milling methods.  It  also  may permit  economical
recovery  of  currently  unrecoverable  low-grade   uranium  deposits  (NRC78).
Though in  situ   leach  mining currently  produces  only a small  amount of  the
annual U.S. output of  U^Og, variations  of  this technique are being widely
tested for  uranium extraction  and  have  potential  for  becoming commercially
significant  (La78,  NRC78,  TVA78b,  Ka78).  Table 1.6 lists in  situ  leaching
operations  for  uranium -as  of   January 1, 1978.   The operations are concen-
trated on   the  coastal   plain   of  southwest Texas  and  in  the  Wyoming  basin
regions.   -Most  commerc1a:l"l sized-  operations"''a re" -in •,southern  Texa's; Vwflere
recent expansion is. expected   to   increase, the  production .of  U^O  by this

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                                                                      1-20
 technique  to  about  900 MT  annually (TVA78b).  Two Texas  sites alone, Bruni
 and  Lamprecht,  are  expected  to  produce  annually 110 and  230 MT  of U,Q0,
                                                                          j o
 respectively (Wy77).  A number  of projects are currently  testing  the effec-
 tiveness  of  the in situ leaching technique. Though these studies usually last
 about  18 months  to  3  years,  some  feasibility tests  require  up  to  6 years
 before  expanding  to full  or  commercial  scale operations  (La78>5*
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                                                           1-21
Table  1.6   Summary of  current  In situ  leaching operations as  of
           January 1, 1978
Name
Sundance
Project
Red Desert
Site I
Red Desert
Site II
Charley
Site
Highland
Site
Double Eagle
Site
North Rolling
Pin Site
Collins Draw
Site II
Bear Creek
Site
Nine Mile
Lake Site
Red Desert
Site
Irigaray Site
Site No. I
S 1 te Nov. 2 ,
Crownpotnt* -
Project -
Location
Crook
County, WY
Sweetwater
County, WY
Sweetwater
County,. WY
Johnson
County, WY
Converse
County, WY
Carbon , .
County, WY
Campbel 1
County, WY
Campbel 1
County, WY
Converse
County, WY
Natrona
County, WY
Sweetwater
County, WY
Johnson
County, WY
McKinley
County, NM
Sandoval
County, NM
McKfrfley
County, NM
Pattern
5-SP
5-SP
5-SP
5-SP
7-SP
5-SP
5-SP
5-SP
5-SP
5-SP
5-SP
ND
4-SP
4-SP
4-SP' •'
Scale of(b) now Rate(c)
Operation (m /min)
RD-PS ND^
RD-I ND
RD-PS ND
RD' ND
RD-C ' 4.54
RD" - ND
RD-I ND
RD 0.38-0.57
RD-I ND
RD-PS 0.38
PS 0.38
C 6.06
PS- I ND
PS- 1 ND
AD* - ND" -

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                                                                 1-22
     Table  1.6       Summary of  current  in  situ  leaching  operations  as  of
                     January 1,  1978  (continued)
Name
Grover Site
Location
Weld County,
CO "
Palangana Dome Duval County,
Site , TX •
O'Hern Site
Bruni Site
Lamprecht v
Site
Zamzow Site
Boots/Brown
Site
Clay West
Site
Burns Ranch
Site
Moser Site
(a)Well
Figure 1.6.
research and
inactive..
fC)F1nw
Ouva.l County,
TX
Duval County,
TX
Bee County,
TX
Live Oak •
County,- TX
Live Oak
County, TX
Live Oak
County, TX
Live Oak
County, TX
Live Oak
County, TX
pattern: 5-SP
i are past or pr
development, _ 
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                                                                     1-23
charged  In  the +6 state)  uranium.  An  oxidant,  such as air, oxygen, hydrogen
peroxide, sodium  chlorate,  sodium  hypochlorite,  or  potassium permanganate, is
added  to oxidize  the  uranium  to  the hexavalent state.  For example:
Unfortunately,  there  is no  lixiviant specific  for  uranium.   Consequently,
other minerals commonly  associated with uranium deposits, such as iron,, sele-
nium, vanadium,  molybdenum, and arsenic, may  also  be dissolved.   This tends
to  contaminate  the  leach  solution  and deplete the  lixiviant.   Lixiviant
agents and their concentrations are selected to maximize uranium recovery and
minimize  undesirable  secondary  reactions.    Acidic  solutions  (pH   2)  are
avoided  because  they  are- less selective.   Neutral  or basic\. lixiviants ;(pH
6-10), such  as  ammonium or sodium carbonate or  bicarbonate,  are often used.

     Many  variables  affect the accumulation  of  trace elements  in leaching
solutions,  particularly the  chemical  and physical  nature  of the  host  for-
mation.  Table 1.7  illustrates  relative contaminant "levels' in  the  two lixi-
viant  types   in  a   laboratory  experiment.   Except  for  Ra-226»  significantly
greater  trace element concentrations  occur in the  acid lixiviant;  the total
dissolved solids is about eight times  higher  than  in the alkaline solution.
Hence,, it would be  necessary to bleed much larger volumes of acidic lixiviant
from the  system  prior to reinjection  in order to maintain acceptable levels
of these undesirable constituents.  Large volumes of liquid wastes containing
higher toxic  metal  concentrations are generally  produced  when  acidic lixi-
viants are employed.  Also, because calcium minerals are abundant in geologic
strata and carbonate  minerals are highly soluble in  acid  solutions,  partic-
ularly calcium carbonate, large amounts of calcium accumulate in recirculated
acid lixiviant,  and they must be removed by a purification process prior to
reinjection.  However, acid lixiviants  leach more rapidly than alkaline ones,
yield higher  uranium  recoveries — about 90 percent  with  sulfuric  acid com-
pared to  60  to 70  percent  with a bicarbonate solution --  and  generally  ex-
tract less radium (Wy77).

     The  number  of  wells,  their  spacing,  and their  pattern  depend upon  the

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                                                                      1-24
size  and  hydrologlc  characteristics  of  the  formation.   Figure  1.6  shows
diagrams  of  some common well  patterns.  Several  hundred injection  wells with
several  recovery wells may  be  employed.   Well  spacing  may vary from  10 to 60
m.   In  addition,  a  number  of monitoring  wells  are driven a  short  distance
from  the  well   field  to  detect  any  excursion of  lixiviant  from the  leach
field.   A commercial -size  operation  may  require  a  well  field  area-  of -20
hectares  or more (TVA78b).

     The  pregnant (containing uranium) leachate  from  the production, wells is
filtered  through a sand filter to  remove  suspended  particulates,  then  passed
through  a surge -tank- (storage  reservoir)  to  ion-exchange resin beds  that se-
lectively  remove the uranium  complex.  The  uranium is  washed  from the resin
     Some  processes, of solutioa miatng  produce  liquid  and solid wastes.   The
volume of  liquid wastes produced  is much  smaller,  per weight of IkOg produced,
than . that, from the. .dewatering .-activlties^-of,  'conventional mining ^methods.
There  is also  no  waste  rock.   Residues .obtained  from drilling are  a  solid
waste. Those" that  traverse 
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                                                                 1-25
     Table  1.7       Trace  metal  concentrations  of recirculated acid and
                     alkaline  lixiviants
Trace Metal
Arsenic
Chromium
Cobalt
Copper
Iron
Lead
Manganese
Molybdenum
Nickel
Selenium
Strontium
Vanadium
Zinc '
Zirconium
Radium-226^
TDS(e)
Acidic(a)
<0.05
0.15
0.2
1.0
25.4
0.7
1.2
NR
0.6
NR
3.7
1.0
4.3
3.3
390
7.8
Concentrations, mg/jr "
Alkaline^
<0.05
0.07
NR(c)
0.04
0.6
0.2
NR
0.9
0.06
1".6
1.5
NR
0.1
0.9
1750
1.0
(a)
(b)
(c)
(d)
(e).
Composition - 5 g/£ H-SQ. and 0.1 g/«.   NaCIO-,
Composition - 8 g/j, NH.HC03 and  1 g/£  ^2'
NR - Not Reported.
Units -~ pCi/£.
   Total dissolved solids in grams,
Source: Ka78.

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                                                                      1-27
      Atmospheric  emissions   from  in  situ  leaching  include  Rn-222 that  is
 vented  mainly from  the  pregnant lixiviant surge tanks and participate matter
 that may  escape  from  the  scrubbers  (exhaust filters)  of the  yellowcake
 (uranium  product) drying  and packaging units.  Radon-222  emanation  from the
 waste ponds  is  probably  negligible,  since the  sediment which  contains  the
 radium  remains submerged  and  little,Radon-222 will-diffuse through the water
 and  escape  to the atmosphere.

      When  the mining  operation is  completed, the water volume  of the leach
 zone will  be restored  to limits  set by  regulatory  agencies.   The  primary
 method  of  aquifer  restoration  is  flushing   the  zone  with groundwater  by
 pumping  from the  production  wells  and/or the  injection  wells.   This  process
 may  produce,  up  to  1.70 m /min  additional  liquid wastes that contain  a high
 concentration of  dissolved  solids  (NRC78).   This contaminated  water  passes
 through  an  ionrexchange uait and  then, discharges ,to  the waste ponds.  The
 barren  effluent  cart be-further  treated-by desalination and
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                                                                      1-28
 percolates  through the pile.  The percolated water is collected In the trough
 and recirculated until the concentration of uranium in solution is sufficient
 to  be  economically extracted.   The  leaching process  may require  up  to six
 months   to   recover approximately  80  percent  of  the uranium   in  the  ore
 (NRC77a).  The heap-leach pile at one mine contained an annual accumulation of
 approximately 360,000 MT  of low-grade  ore (NRC77a),  The  pile measured 3QQ m
 x 90 m  x 7.6 m with solution reservoirs of 22 m x 90 m x 1.5 in.

      After  leaching operations are  completed, the leached  pile is neutralized
 with lime to  a  pH of  about 7.   The  site is then contoured to blend with the
 surrounding  terrain, covered  with  layers of subsoil and  topsoil,  and  seeded
 to  control wind and water erosion.

      Because"  necessary  infamratiw is*  unavatiTable" and''the  contribution  of
 heap leaching to-the  total  uranium production is very minor and  not expected
 to  become significant (NRC79)»-an  assessment of the environmental  impact'.-of
 heap-leached piles  has  not been conducted.   However,  the NRC  has  recently
 concluded  that,'  although* the-- hazard  of-• tail ings: produced by heap  leaching
 will  be much  less  than  the hazard  of tailings at conventional uranium mills,
 the same  tailings  management and  disposal   criteria  should  possibly  apply
 (NRC79).

 1.3.5.2   Mine Water Reci reflation
     At  several  sites  mine  water is  recirculated to leach "worked-out areas"
 of  underground mines  (Pe79b).   In the  early uranium mining  years,  ore  with
 less  than about  0.15  percent U30g was  not mined.  This  grade is relatively
 high  compared to  present  day markets.    Consequently,  significant quantities
 of  uranium remain  in these abandoned*  areas.  Because the roofs of these areas
 collapsed  during  the  initial  mining retreat,  this  ore  is  difficult  to re-
 trieve  by  conventional methods.  To  recover a portion  of  this uranium,  holes
 are  drilled  to the  top  of the collapsed zone and  mine water is  sprayed  from
 these holes  onto the  shattered  ore.   Water for  leaching  may be  sprayed  from
 the  mine floor  if the^abandoned .area,  is, accessible, to the, workers..(Pe79a)..
 The  oxidized uranium  (uranyl  ion) is  leached  by the  slightly alkaline .mine
water,  which flows  to collection' sumps.   The'enriched water is  pumped1 to a
 resin  ion-exchange-"- unit, * to; -extract the'* uranium,'• and. then  .^•t'N-i'S'.-.

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                                                                      1-29
 After the  available  oxidized  uranium  has been leached,  the  process  is dis-
 continued for  a  few  weeks to  allow  more  uranium to oxidize.   Mine water is
 then circulated again through the ore.

      This process  increases  the  recovery of uranium  with  minor effort  and
 expense,  but it contributes  little  to  the total domestic uranium  production
 (NRC79).   In addition, the quality  of  the stored mine  water used will  be  en-
 hanced  after passing through  the  resin ion-exchange unit.  Hence, mine water
 recirculation has little  impact  on  the environment.   It  was  not assessed in
 this  study.

 1.3.5.3.   BoreJiole  Slurry Mining
      Hydraulic  borehole  slurry mining  is  a  reci^tly  proposed  technique  for
 extracting  uranium  ore (Ka78»  St78).   As  the narm  suggests,  this method uses
 pressurized  water to loosen  and  combine with ore-bearing material  to  form  a
 watery  mixture known  as   'slurry' that  is transported  from the  borehole  and
 then  conventionally milled.   This method  could  >>e applied  to  sandstone  de-
 posits  at depths of  30 m to about 100 m.  By present estimates, yellowcake
 from  ore  containing  0.06 percent LLOg and  mined  at  a  60 m  depth  by this
 method  would cost  $42 per  pound (Ka78).   This  method presently is  not as
 economical as the more  conventional methods of uranium  mining.

     The  process  consists of drilling  a 45-cm diameter hole to  approximately
 2 m  below the uranium-bearing  strata.   A  cutting  jet  assembly  is positioned
 in the  hole  at the end of a  rigid service column containing conduits for  the
 pressurized  water and  slurry transport.  The  slurry  pump  is  placed  at  the
 bottom of the hole. The  underground mining operation is started  with the  jet
 set at the lowest position.   The rotating  jet cuts material through an arc of
 somewhat  less  than 360  for a  distance of  up  to  25  m,  depending  upon  the
design of the  jet  system.   The  segment  of unmined  ore  acts  to support  the
overlying  strata.   After  the material  is  removed  as  a  slurry, the  jet  is
 raised to the  next  level  -of  ore and the process is repeated.  After milling,
the decanted water  from the  slurry is  recycled  for slurrying more ore.  The
tailings  from  the milling operation are used  to  backfill  the borehole cavi-
ties  and minimize subsidence.

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                                                                      1-30
      A 15 m  to  E5 m radius borehole can be mined in an 8- to 24- hour period
 (Ka78),   Large ore  bodies  might be mined by drilling, slurrying, processing,
 and backfilling  in  a  systematic pattern that leaves ore In between boreholes
 for support.   These areas could be mined in a second phase after the original
 boreholes are backfilled.

      Borehole mining for uranium  is currently only a proposed method with no
 pilot or  commercial  scale units  in operation.  Thus,  the possible  environ-
 mental  impact from this process was not assessed in this study.

 1.3.5.4.   ]Jram'umjisa  By-Product
      The  recovery  of  uranium  as  a by-product from other mineral mining  and
 milling operations was  discussed briefly in Section 1,3.1.  Since recovery i<»
 basically from  the milling operation,  any environmental problem that  might
 exist is  associated with milling  rather than mining.  Therefore, it  was  not
 assessed  in  this study.

 1.4   Current  Applicable  Standardsand Regulatlons

 1.4.1      Federal  Regulations
      Health,  safety, and  environmental  hazards associated with uranium mining
 are  regulated by  Federal  and  State laws.  This  review focuses on laws  and
 regulations  applicable  to  mine operations.   Nuclear  Regulatory Commission
 regulations  for  milling operations  apply  to in  situ  leach extraction  and  are
 therefore  included.  Some  laws and regulations on  exploration rights also
 cover the environmental  impact  of mining operations and wastes.

      Prior  to the  National  Environmental   Policy  Act (NEPA)   of 1969,  there
 were  few  regulations protecting the environment  of  lands  not controlled or
 owned by  the  Federal Government.   Even  with NEPA,  much Federal   authority on
 environmental  problems   was  unused  until  recently.   This Act  established a
 national  policy  concerning  the  environment.   Section  102(2)  (C) states that
 every agency  of  the Federal Government must "include in every recommendation
 or report on proposals for legislation and  other major Federal actions signi-
 ficantly  affecting the  quality of  the  human  environment,  a  detailed state-
ment" of  the  environmental  impact   of such  an  action.   Major Federal  actions

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                                                                      1-31
 "...  includes actions  with effects  that may  be  major and which  are  poten-
 tially  subject to Federal  control  and  responsibility ...  actions  include new
 and continuing activities,  including  projects  and  programs entirely or  partly
 financed,  assisted,  conducted,  regulated,  or  approved  by  Federal  agencies;
 new or  revised agency  rules,  regulations, plans, policies, or  procedures; and
 legislative  proposals  (Sections  1506.8,  1508.17) .... Approval  of specific
 projects,  such as construction  or  management  activities located  in a defined
 geographic area.   Projects  include  actions approved  by  permit  or other  regula-
 tory  decision as  well  as  federal  and  federally-assisted   activities"(40  CFR
 1500).

 ^.l.l   Federal JLaws, Regulations,  and Gutdejs for  Protection of  Health  and
          Environment
     Table 1.8 provides an overview  of  federal  law^ and  regulations for the
 protection of health or environment  and the administering agencies.  Federal
 agency responsibilities for water use, conservation  laws,  and exploration  and
 mining rights  are  indicated in columns 1-4.  Laws and regulations  for environ-
 mental  quality  and  health and  safety  are  indicated in  columns  5-10.   See
 Appendix A for an itemized list of the  laws and regulations shown  generally
 in  Table 1.8.

 1.4.1.1.1  Air Quality
     Regulations  on  air quality  have been promulgated  pursuant  to the Clean
 Air  Act  (42   U.S.C.  1857  et  seq),  which includes  the Clean Air  Act of  1963
 (Public  Law   88-206)  and  amendments  by  the  following:   Public  Law 89-272,
 Public Law 89-675, Public Law 90-148, Public  Law  91-604,  Public Law 92-157,
 Public Law  93-319,  Public  Law 95-95, and  Public  Law  95-190.   The Environ-
mental Protection  Agency  establishes  National  Ambient Air Quality Standards,
New  Source Performance Standards,  and National Emissions  Standards for Haz-
ardous Air Pollutants  under the  Clean Air Act  (CAA).   Primary standards are
set  to  protect  public health  and  secondary  standards are set  to protect
public welfare from known  or anticipated adverse effects.

     National Ambient Air Quality Standards  (NAAQS) have been established for
seven pollutants  in 40 CRF 50.   The Administrator of EPA is authorized to set
emission  standards for hazardous   air  pollutants  for  which no ambient  air
quality  standard  is  applicable.   Asbestos,  beryllium, mercury,   and  vinyl

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         Table 1.8  Federal laws, regulations, and guides for uranium mining
General
Conservation-
Water Preservation
Federal Agency Use Statutes
Mining
Permits Environmental Quality Health
Exploration Mining Water Land and
Rights Rights Air Surf KG Solids Reclam Safety

Dept. of Int. X X
BIA(a)
BLH(a) X
USGS(a)
Dept. of Energy X
Dept. of Agr. X X
USFS(a)
EPA X X
A!R-QAQPS(a)
Water
Surface OWPS(a)
Ground OSW(a)
Radiation-ORP^
U.S. Army
Corps of Engrs. X X
Dept. of Labor X
MSHA(a)
OSHA(a) ,.,
Nuclear Reg. Comm. X
XX X
XX X
XX 'X
X X
XX X
X
XX X
X XXX
X
X
X
XX XX
XXX XX X

X X
X
V '
X c.
rs
X X. XX X
(a)
   BIA-Bureau of Indian Affairs
   BLM-Bureau of Land Management
   USGS-United States Geological Survey
   USFS-Umted States Forest Service
                                                            OWPS-Office  of Water  Planning  and  Standards
                                                            OSW-Office of Solid Waste
                                                            ORP-Office of Radiation  Programs
                                                            MSHA-Mininq  Safety and Health  Administration
,.vOAQPS-Qffice of Air Quality,  Planning and Standards       OSHA-Occupational Safety and Health Administration
^ 'Nuclear Regulatory Commission (NRC)  regulations  and guides for milling do apply to in situ extraction or mining
   but not conventional surface  or underground mining where  NRC has no authority.

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                                                                      1-33
 chloride  emission standards  are  in subparts,  B,  C, E, and  F  of 40 CFR 61,
 respectively.   Section  122  of the CAA directed the Administrator  to determine
 whether emissions  of  radioactive pollutants, cadmium, arsenic, and polycyclic
 organic matter  (such  as  benzene) into ambient air will cause or contribute to
 air  pollution and  endanger  public health.  If they do, EPA must propose emis-
 sion  standards  for  them within 180 days  after that  decision.   The EPA has
 listed radionuclides  as  "hazardous pollutants" under Section 112  of the Clean
 Air  Act  in  December  1979  (44FR76738,  December  27,   1979).   To  date,  no
 standards for radionuclide  emissions in air have been promulgated.

     The  particulate  concentration  values  of the NAAUS apply to mining oper-
 ations.   Emissions (including dust) must be controlled to meet the standards.
 Du,t  from mining  operations was excluded from any air quality impact assess-
 ment  for  prevention  of significant air quality deterioration  (PSD)  (see 43
 F.R.  26395).   However,  as  a result of  the court  decision  in  Alabama Power
 Company v. Costle, 13 ERC 1225, EPA has proposed amendment of PSD regulations
 (44 F.R.  51924, September 5, 1979).

     The  emission  of radioactive  substances or gases from gaseous release is
 controlled by NRC regulations 10 CFR Parts 20 and 40 for uranium milling and
 in situ leaching.   The NRC does not have  this  authority over mining.  There
 are  no  Federal  regulations  for radioactive pollution of air from mining at
 this  time.  However,  MSHA enforces standards for radioactivity  in air inside
 mines (30 CFR  57.5-37 through 57.5-42).   Health and Safety standards of MSHA
 for Metal and  Nonmetallic  Mine Safety are given  in  30 CFR Parts 55, 57,  and
 58.

 1.4.1.1.2  Water Quality
     Standards  for water quality are  promulgated by  EPA under  the  Federal
Water  Pollution  Control Act   (FWPCA)   of  1948  (as  amended)  and  the  Safe
Drinking Water  Act (SDWA)  (as amended).   The FWPCA and SDWA regulate surface
water quality and groundwater quality,  respectively.

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                                                                      1-34
      The Federal  Water Pollution Control  Act Amendments  of  1972{Public Law
 92-500)  established  that  no one  has a  right,  without permit,  to discharge
 pollutants  into  navigable  waters of  the nation.   The  Act provides  for the
 establishment of  both  water  quality standards and  effluent limitations.   In
 addition to  requiring  effluent standards  for existing sources,  it  required
 EPA to  set  new  source  performance  standards for  uranium mining.  The  fol-
 lowing  standards and guidelines apply  to uranium mining and  milling:   Regu-
 lations  on   Policies  and  Procedures for  the National  Pollutant  Discharge
 Elimination  System (40 CFR  125),  Effluent  Guidelines  -  Mining and Processing
 (40 CFR  116), Effluent  Guidelines  and Standards for Mining  and Processing (40
 CFR 436),  and Protection of  the  Environment-Ore  Mining and Dressing  -  Point
 Source  Category  (40  CFR Part  440).   Table  1.12  lists other  pertinent  regu-
 lations  and  guides.

     The Safe Drinking  Water Act  primarily  protects municipal  water systems.
 Part C  of the Act  requires  that  states  establish underground  waste water in-
 jection  programs according  to  EPA regulations.   Most  mining  operations  dis-
 pose of waste  water through surface  discharges  subject to the NPDES permit
 program  and  to  the FWPCA.   However,  if a mine  or mill  seeks to  dispose of
 polluted water by injection and  such  injection may endanger  public drinking
 water  supplies,  then the Safe  Drinking  Water Act would apply.   Finally,  EPA
 will  be  developing  regulations pursuant to  Subtitle  C  of the Resource  Con-
 servation  and Recovery  Act  that  will  provide controls  on hazardous  uranium
 mining  wastes,  including protection  of  groundwater resources.  Section  4004
 criteria,  promulgated  on  September  13,  1979,  apply  to  the nonhazardous
 portion  of the wastes.

     The  NRC's water quality standards  for  radioactivity  in discharges  from
 uranium  milling  to  the environment  are  in  10 CFR Parts  20  and 40.   These
 would apply to in  situ  mining licensed by NRC  or an  agreement  state.

 1.4.1.1.3  Land  Quality
     Federal  regulations  on  solid  waste disposal  and land reclamation speci-
 fically  for uranium  mining  wastes are being  developed  pursuant to the Solid
Waste Disposal Act (as  amended).   The Surface Mining Control  and  Reclamation
Act  of  1977  only  applies  to coal  mining.  Uranium mining  occurs on Federal

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                                                                      1-35
 lands,  where the Departments of Interior and  Agriculture require reclamation,
 A large part of  the  western states  is  Federally owned land:   Arizona (43 per-
 ce/.i),  California (45  percent), Colorado  (36 percent),  Idaho  (64  percent),
 Montana (30 percent), Nevada  (87  percent), New Hexico (34 percent), Texas  (2
 percent),  Utah  (66  percent), Washington  (29  percent), and Wyoming  (48 per-
 cent).   State laws  and  local  zoning  ordinances may affect waste  disposal.
 Many states  authorize   counties  to regulate  land  use outside  incorporated
 areas.   Likewise, many  states  allow  cities,  towns,  and  villages  to  enact
 zoning  ordinances for land  use  within  their  boundaries.  Thus, mining  oper-
 ations   in  each  state   are subject to different  reclamation  requirements,
 depending upon land  ownership  and  location.

      Regulations  for hazardous  uranium mining  wastes  have been proposed  by
 the  EPA  pursuant to  Subtitle  C  of  the  Solid  Waste Disposal  Act as  sub-
 stantially  amended by the Resources Conservation  and Recovery  Act of  1976
 (Public  Law 94-580). These were published in  the  Federal Register (43  F.R.
 58946-59028)  on   December  18,  1978.  Waste rock and overburden from uranium
 mining  are  listed  as   hazardous  wastes,  because  they  contain radioactive
 substances that meet  the definition  of  hazardous wastes given  in Section  1004
 (5)  of  the  Act,   Special  waste standards (Part 250.46-4) were proposed for
 the  treatment, storage,  and  disposal of overburden and waste rock.

 1.4.1,2   Federal Mineral  Leasing and Location/Patent Laws
     Some Federal regulations govern mineral  exploration  and  mining rights.
 The  Mining  Law  of 1872  (30 USC §§ 21-50) permits   persons to  enter public
 lands to  discover, locate, and mine valuable  minerals.   The law has no pro-
 visions for facility siting, surface protection, or reclamation.  Free use of
 water and timber  for the mining operation and land for a mill site are ancil-
 lary  rights  granted   by  the law,   Most subsequent mineral  leasing  laws are
 similar,  designed to provide  an orderly system  for  locating, removing, and
 utilizing valuable mineral  deposits on federally owned and controlled lands.
 Pursuant to  Section  603  (C) of the Federal  Land Policy and Management Act of
 1976, DOI has  proposed  specific environmental  protection regulations (43 CFR
3800) for mining activities in potential or identified wilderness study areas
 (44 FR 2620),

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                                                                      1-36
 1.4.1.2.1  Prospecting  and Mining  Rights
      Consideration of environmental impacts may  be  required  before obtaining
 the right to prospect or explore.   Depending  upon  land  category,  prospectors
 may have  to  assess the  environmental  impact of  mineral  exploration  before
 being  permitted to explore.  Table  1.9 summarizes  these requirements.   Pros-
 pectors  on private lands  simply must have  permission  from  the owner of  record
 of  mineral  estate.  On  the other  hand,  Tribal  and  Indian  lands,  National
 Forest System-lands,  and  public  lands  (not public domain) all  have specific
 approval  systems that require exploration  plans or other  appropriate consid-
 erations.

      Obtaining  rights  to mine usually involves  the  same Government  agency
 involved  with  prospecting  rights.   Table  1.10 summarizes  applicable Federal
 laws  and regulations.

 1,4.1.2.2       Mining^ and Environmental  Plans
     Before  mining begins certain  operating or mining and reclamation  plans
 must  be  submitted  and approved.  Table 1.11  summarizes  these.  The  require-
 ments  parallel  those for  prospecting and mining rights.

 1,4.1.3    Laws  Having Potential Applicability
     Federal  laws  require regulation for quality of air, water, and  land. In
 addition,  though their direct  influence has not been evaluated in this re-
 port,  federal   laws protecting  wildlife and cultural  resources could affect
 uranium mining  activities.

     Water  use   is  also  of  potential   concern in  regard  to  uranium mining.
 However, except for in  situ mining, uranium  mining operations  have modest
 needs  for  water.   In  fact,  most  mines   typically  dispose   of significant
 quantities  from necessary  dewatering.   Appendix  B lists  federal  water pro-
 grams  and  rights activities  and  the lead  agencies administering  them; and
 Appendix  C  lists  Congressionally  approved compacts  that apportion  water.
 These compacts  apportion water to the affected states, and  each state in turn
allocates  its share of  the water among  intrastate  users on the basis of its
own system of water rights.

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          Table 1.9   Requirements to obtain rights to prospect  or  explore  by  federal,
                      state and private lands
     Land Category
                                   Requirements
Federal:
     Tribal
     Allotted Indian.,
     Public Domain,
     Acquired Public..,
Prospecting permit issued by BIA with consent of tribe. 25 CFR 171.27a.
Technical examination of environmental  effects of prospecting by BIA, 25
CFR 177.4.  Exploration plan submitted  to USGS.  Approval  of plan by USGS
required, 25 CFR 177.6.  Enforcement of plan by USGS, 25 CFR 177.10.

No specific provisions for prospecting.  Procedure for leasing to prospect
is same as for mining.  If allotted land has been patented, treat same as
private land.

No restriction on prospecting.  Entry under General Mining Law of 1872 (30
USC 22, 43 USC 1744, 43 CFR Part 3810), uranium included,  43 CFR 37461.

Prospecting permit from BLM, 43 CFR 3510.0-3 and 3511.2-1.  Acquired lands not
subject to prospecting permits are listed in 43 CFR 3501.2-1. If acquired
land is not under BLM jurisdiction, consent of governmental entity having
jurisdiction is required before permit issued by BLM (43 CFR 3501.2-6).
     Withdrawn Public... Public domain land withdrawn for power development is open to entry and lo-
                         cation under General Mining Law of 1872, 30 USC 621.   Agency having control
                         of withdrawn land reports any objections to mining activity based on land
                         use for which withdrawal was made.  If controlling agency recommends stipu-
                         lations in the permit, they are included (43 CFR 3501.3-1 (a}, (c).

     Reserved Public..,. Some Federal lands are disposed of with minerals reserved to the Govern-
                         ment; e.g., see 43 USC 299, 43 CFR 3814.1, 30 USC 50.  For these lands,
                         permit issued.by BLM requires conformance with law under which reservation
                         was made, 43 CFR 35013-2(2).  For lands reserved or segregated for partic-
                         ular purpose, special requirements may be made by BLM for protection and
                         use of land for purpose that it was reserved or segregated.  Leases
                         from Dept. of Energy may be possible under 42 USC 2097.

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Table  1.9  (Continued)
.and  Category
                               Requirements
National  Forest  System.
5tate...

3rivate,
,Public  domain  landsinside NationalForest  System boundaries  are  subject
 to General  Mining  Law of 1872,  with  the following conditions:  (a)   If Dept.
 of Agriculture requires operations plan,  it must be  submitted.  Dept.  of
 Agriculture approves plan, 36 CFR 252.1;  (b) Operations  must  minimize
 environmental  impact on surface resources in System  lands,  36 CFR 252,8;
 (c) Surface inspection and securing  compliance with  plan is responsibility
 of Dept.  of Agriculture, 36 CFR 252.7.  Acquired National Forest System
 land same as Acquired Public Land,

 Lease obtained from  appropriate State Agency according  to state law.

 Permission given by  owner of record  of mineral estate.
     Source:    San Juan Basin Regional  Uranium Study,  Working Paper No.  28,  Legal  Infrastructure Related to
Jranium Mining  in  the San Juan Basin,  United States Department of Interior.
                                                                                                                    CJ
                                                                                                                    OQ

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                      Table 1.10  Requirements to obtain  rights  to mine ore by
                                  federal,  state, and private  lands
    Land Category                     -                      Requirements


Federal:
     Tribal	  Secretary of Interior has general  authority for  leases,  25 USC  396a.   Tribe
                         must approve.  Leases given by bid.   Approval  of Secretary of  Interior re-
                         quired, 25 CFR 171,2.  Tribe may negotiate lease if Secretary  grants  per-
                         mission.  Secretary has discretion to reject lease negotiated  by Tribe,  25
                         CFR 171.2.  Secretary may issue charter of incorporation to Tribe which  may
                         include authority for Tribe to negotiate mining  leases without approval.

     Allotted Indian	Leases given by bid.  If Secretary of Interior approves, leases may be nego-
                         tiated by Indian owners, but negotiated lease subject to rejection by Secre-
                         tary, 25 CFR 172.4 and 172.6.  Approval of allottee required.  If patented,
                         treat same as private land.

     Public Domain	 No lease required.  Location of mineral deposit  (staking a claim) after min-
                         eral has been discovered, 43 CFR 3831,1 and 3841.3.  File locations with BLM
                         and in accordance with 43 USC 1744.  Also record in accordance with State law.
                         Obtain patent for land claimed, 30 USC 29, 43 CFR Part 3860.  Mill sites may
                         be claimed by location and patenting, 30 USC 42, 43 CFR Subpart 3844.  If claim
                         has been patented, treat same as private land.

     Acquired Public	 Mineral estate on acquired lands can be leased by BLMS 43 CFR 3501.3-1,  subject
                         to exceptions (43 CFR 3501.1-5 and 3501.2-1).   Permittee who prospected and
                         discovered is entitled to preference right lease, 43 CFR 3520.1-l(a)(3).   BLM
                         leases land which contains valuable minerals on competitive basis, 43 CFR
                         352Q.l-2(a),  If  land is not under BLM jurisdiction, consent of governmental
                         entity having jurisdiction is required before lease issues.                      7*
                                                                                                          to
                                                                                                          U3
     Withdrawn Public... For public domain land withdrawn for power development, laws are same as for
                         land in Public Domain, 30 USC 621.  If withdrawal does not preclude mining,
                         BLM can lease mineral estate.  Agency having jurisdiction of withdrawn land
                         reports any objections to mining activity, based on land use for which with-
                         drawal was made.  If controlling agency recommends stipulations in lease,
                         they are  included, 43 CFR 3501.3~l(a)(e),  Leases from Dept. of Energy
                         on lands withdrawn for DOE use under 42 USC 2097,

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Table 1.10 (Continued)
    Land Category
                                                      Requirements
6.
Reserved Public
7.    National Forest
      System
8.

9.
State

Private
Some Federal  lands are disposed of with minerals reserved to the government; see
e.g. 43 USC 299, 43 CFR 3814.1 and 30 USC 50.  For these lands, lease issued by
BLM requires conformance with law under which reservation was made, 43 CFR 3501.
3-2(2).  For lands reserved or segregated for particular purpose, special require-
ments may be made by BLM for protection and use of land for purpose that it was
reserved or segregated.

Public Domain land inside National Forest System boundaries are subject to Gen-
eral Mining Law of 1872, with the following exceptions:  36 CFR 252.1, (a)  If
Department of Agriculture requires operations plan, it must be submitted.
Department of Agriculture approves plan;  (b) Operations must minimize environ-
mental impact on surface resources on System Lands, 36 CFR 252.8; (c) Surface
reclamation required, 36 CFR 252.8(g);  (d) Inspection and compliance with plan
responsibility of Department of Agriculture, 36 CFR 252.7.  Acquired National
Forest System Land same as Acquired Public Land.

Leases obtained from appropriate State Agency according to state law.

Lease of mineral estate (or total estate) by private negotiation.
       Source: San Juan Basin Regional Uranium Study, Working Paper No. 28, Legal Infrastructure Related
to Uranium Mining in  the San Juan Basin, United States Department of Interior.

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                         Table 1.11   Requirements for mining  and  environmental  plans  by federal,
                                      state,  and private lands

     Land CategoryRequirements

Federal;
     Tribal	  Mining plan must be approved by  USSS.   If lease requires revegetation, the
                              revegetation work is included in mining plan.   Mining plan can be changed-
                              by mutual consent of USGS and operator, 25 CFR 177.6.  BIA evaluates environ-
                              mental effect of proposed operations and formulates environmental mitigation
            '                  requirements.  BIA consults with USGS, 25 CFR 177.4.

     Allotted Indian	Same as Tribal  Land, 25 CFR 177.1.,  unless allotted land has been patented.  If
                              patented, treat same as private  land.

     Public Domain .........  Plan same,as acquired public land.

     Acquired Public	  Geological survey approval of mining plan to mitigate adverse
                              environmental effects for federal leases, 30 CFR 231.10.

     Withdrawn Public	Stipulations can be put in the lease by the agency for whom the
                              land was withdrawn.  These could affect operations but no formal
                              submission of plans required, 30 CFR 231.10.

     Reserved Public	Lessee must conduct operations in conformance with such require-
                              ments as may be made by BLM.  Requirements will conform to pur-
                              poses for which land was reserved, 43 CFR 350.3-2{b).  Approval
                              of mining plan required, 30 CFR  231.10.

     National Forest System...Operations plan submitted to District Ranger, Department of Agri-
                              cultural, if he deems it necessary, 36 CFR 252.4.  Reclamation
                              of surface required under opertor's plan, 36 CFR 252.8(g).  Com-
                              pliance with Federal and State environmental laws, preserve
                              scenic values, wildlife, etc., 36 CFR 252.8.  District Ranger,
                              Department of Agriculture, inspects and assures compliance
                              with operations plan, 36 CFR 252.7.

State...	  Mine plan filed with and approved by State.

Private	  Same as State Land.
     Note.—Some states require submission of mining and reclamation plans for all land.
     Source:  San Juan Basin Regional Uranium Study, Working Paper No. 28, Legal Infrastructure
Related to Uranium Mining in the San Juan Basin, United States Department of Interior.

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                                                                      1-42
 1.4.2.  jtate Regulations
      Federal   statutes  and  regulations  control many  areas of  environmental
 quality.  Most state licensing or  regulatory  authority  is  often  the  result of
 a  Federal-State agreement.  However,  land  reclamation  for uranium mining on
 federal  and nonfederal lands  is  principally  under  state control.  Table  1.12
 shows  the regulatory scheme for  six  states with uranium mining, and Appendix
 D  lists  the  specific  laws, regulations,  and  guides  indicated  generally  in
 Table  1.12.

     Agreement states  have made formal  arrangements with  the  NRC to develop
 programs  to issue by-product,  source  material, and processing licenses.   The
 Atomic  Energy Act (Sec. 274), as  amended,  requires agreement  states to  pro-
 vide  by  1981  regulatory  programs  that  are  equivalent to  or  more stringent
 than the  federal  requirements  for mill operations.  Much of the environmental
 regulation  of mining operations outside  of federally controlled lands, espec-
 ially  for  reclamation  activities, currently  depends  upon  state  or  local
 requirements.  No  NRC  licenses   are   required  for  mining,  except  in  situ.

     The  Federal  Water Pollution  Control  Act amendments  of  1972  give   EPA
 National  Pollution Discharge Elimination System (NPDES) permitting authority.
 However,  Section 402 provides  for  approval of  a  state  or  interstate program
 to  permit.   The Administrator  has established  guidelines specifying   pro-
 cedural  and other elements  that  must be present to obtain approval  (40  CFR
 124).  Where states  have  not  been  approved,  applicants apply  for discharge
 permits from  EPA.   However, EPA asks  what state  requirements  should also be
 certified  so   that  state  standards are  met.   Column 2  of Table  1.12  lists
 states that are  approved to  issue NPDES permits.

     The  Clean  Air  Act  (CAAJ  amendments of  1970  and 1977  require,  under
 Section  110,   that State  Implementation  Plans  (SIP's)  must be  submitted  for
 approval  to EPA  for implementation of CAA on  a local level.  The approval  and
 implementation of  State plans  are given in 40  CFR  52.   In areas where NAAQS
are violated,  SIP's  must  produce  compliance  by  1982.   If a  state  fails to
enforce its plan,  EPA  may enforce it.  There  are  currently no  emission  stan-
dard regulations specific for uranium mining  by State governments.

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                   Table 1.12  State laws,  regulations,  and guides for uranium mining

                                                                                Mining
State
  NRC
Agreement
  State
General  ~
   NPBES
   Permit
   State
                                                              Permits
                                Environmental  Quality
                                            Health
Water Exploration Mining
Use     Rights    Rights
                                                                                             Water
                                  Land
Air
                                   and
Surf
UG
COLORADO      -                   Yes        Yes
Department of Health
  Water Quality Control Div.
  Air Quality Control Div.
Department of Natural Resources
 Div. of Water Reserves (State
 Board of Land Commissioners
 Mined Land Reel am Bd            -
 Division of Mines

NEW MEXICO                       Yes        No
 State Land Commission
 Dept. of Energy and Minerals
 Dept. of Natural Resources
  Env. Improvement Div.

TEXAS                            Yes        No
  Dept. of Water Resources
  R.R. Commission of Texas
  General Land Office
  Dept. of Health
  Air Control Board

UTAH                             No         No
  State Engineer
  Dept, of Social Services
   Division of Health
   Water Pollution Control Bd.
  Dept. of Natural Resources
                                                                                       x
                                                                                       x
                                                                                               x

                                                                                               x

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Table 1.12 (continued)
State
GENERAL
NRC
Agreement
State


NPDES
Permit
State


Water
Use



Permi
Exploration
Rights

ts
Mining
Rights Air

Mining



Environmental Quality
Wa te ! r
Surf
•


UG

Land
Solids Reel am


Heal th
and
Safety

 WASHINGTON                       Yes
   Dept. of Natural Resources
   Dept. of Ecology
    Office of Water Programs
   Dept of Social Services S Health  -
    Health Services Division
    Air Quality Division
           Yes
                                                                    (No)
 WYOMING
   State Inspector of Mines
   State Engineers Office
   Dept. of Env. Quality
    Air Quality Qiv.
    Water Quality Div.
    Land Quality Div,
    Solid Waste Management
No
Yes
                                                                              x
                                                                              x
     Note.—An "x" indicates the existence of one or more controTling laws,  regulations, or guides.
the specific laws, regulations, or guides.
                                                                   See Appendix D for a list of

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                                                                      1-45
      Applicable   laws,  regulations,  and  guidelines   that  apply  to  uranium
 mining  in  Colorado,  New  Mexico,  Texas,  Utah, Washington,  and Wyoming  are
 discussed  below.   Laws  and regulations  of  other previously mined or  potential
 uranium raining states,  such as  Arizona,  California, Idaho, Montana,  and  South
 Dakota, are not  reviewed.  However, the  basic environmental  considerations
 of uranium mining  should  not  be  significantly different  for other  states.

 1.4.2.1.   Colorado  ,
      Colorado  is  an NRC "Agreement  State"  and has been approved  by the EPA to
 issue NPDES discharge  permits.  Both radiation and  water quality regulatory
 activities  are  under  the  jurisdiction of  the  Colorado Department of Health.
 The   Health  Department's  Radiation and  Hazardous  Wastes  Control  Division
 administers  radiation control  activities and the control of hazardous wastes
 disposal.  However,  there  are  no operable  rules or  regulations for mining.
 Water quality  is  the  responsibility of  the  Water  Quality Control  Commission
 (affiliated  with  the  Health  Department),  which  promulgates  water quality
 standards  and  control regulations,  and  the  Health Department's  Water Quality
 Control Division, which administers and enforces the Commission's regulations
 and  issues NPDES  permits, as   well  as  being responsible  for numerous other
 water quality activities.

      Colorado's permitting of  discharges to "navigable"  waters  has  been ap-
 proved  by EPA.  Unlike most  states, Colorado has promulgated specific "Guide-
 lines for Control  of  Water Pollution from Mine Drainage" (November 10, 1970).
 These guidelines have the  status of regulation since the State does not issue
 the NPDES permit unless the  guidelines will be met.  Colorado also has "Rules
 for Subsurface Disposal  Systems" that,  in conjunction with  other  rules, may
 assure  protection of  groundwater.   These  "Rules"  cover  all  wastes  that are
 disposed  of  underground,   whether  by  direct  or  indirect means.   "Wastes"
 include  "any  substance,   solid,  liquid, or gaseous, including radioactive
 particles  thereof,  which  pollute or may  tend  to  pollute any  waters  of the
 State."   Solid  waste  and  other  land  disposals are   covered by  Section
 25-8-501,  CRS  1973,  as amended.  In cases  where  these regulations  do  not
control, the rules for subsurface disposal  systems  may apply.

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                                                                      1-46
      The Colorado Department  of Natural  Resources  administers water  use  In
 Colorado.   As with  most Western States,  water  is  not in great abundance  in
 Colorado,   Determination of  priority  of  water  rights  to  surface and  tributary
 groundwater is under the jurisdiction of a  system of Water  Courts,  while the
 Division of  Water Resources  (State  Engineer)  administers  and controls  the
 allocation  of actually  available waters  on an  annual  basis according to water
 rights  priorities.

      There  are  no State  air  quality  standards  or   regulations  that  apply
 specifically  to uranium  mining.  However,  the  National Ambient Air Quality
 Standards  and  various  State  emission  control  regulations  apply  to uranium
 minirg  activities  as they do  to all  other types of  emission  sources.   Colo-
 rado's  air  quality  activities  are  the  responsibility  of  the State  Health
 Department's  affiliated Air  Quality  Control  Commission  and its Air Quality
 Control  Division.  The Commission defines  State  air quality  policy  and  prom-
 ulgates  air quality ambient  standards and  emission control regulations,  while
 the  Division  administers and enforces the air quality regulations and  issues
 emission permits.

      The Board of Land Commissioners, affiliated with  the Colorado Department
 of Natural  Resources,  issues permits for  prospecting  and controls leases for
 mining  on  State lands.   The Board  has  policies and  regulations  concerning
 environmental  impacts on prospected or leased  lands.

      The  Colorado  Mined  Land  Reclamation Board was  created  in  1976.   It is
 adminstered by the Department of Natural Resources,  The Board  issues permits
 for  all  mining operations on all Federal  and  non-Federal lands in the State.
 The  stated  intent for  Colorado Mined Land Reclamation  Law  is "to allow for
 the  continued development of  the mining  industry  in this  State, while re-
 quiring  those  persons  involved  In mining  operations to reclaim land affected
 by such  operations  so  that  the  affected  land  may  be   put to a  use beneficial
 to the  people of this State.   It is the further intent...to conserve natural
 resources,  aid  in  the  protection  of wildlife  and  aquatic  resources, and
establish agricultural,  recreational, residential, and  industrial  sites and
to  protect   and  promote the   health,  safety,  and  general  welfare of the
people...."   The Board has established rules and regulations to implement the

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                                                                      1-47
 law.   Rule  5  (Prospecting  Notice  and Reclamation  Requirements)  considers
 prospecting  a  separate  activity,  but  still  covered  by certain  reclamation
 requirements.   The  reclamation performance standards  of Rule 6  have specific
 requirements  for grading,  hydrology and water  quality, wildlife safety  and
 protection,  topsoiling,  and  revegetation.   Rule 7  ("Surety")  assures rec-
 lamation.  Before the Board issues  any  permit and  before any Notice  of  Intent
 to  Prospect  is  valid,  the applicant  must  post  surety  with  the Board.   The
 amount  of surety,  established  by  the  Board,  is  to  be  sufficient  to fully
 reimburse  the State  for  all  expenses  it would  incur  in completing the rec-
 lamation plan in the event of default by the operator.

     Colorado also  has regulations  that apply for  health  and safety  in mining
 operations.   For each  invidual  employee of any  mining  operation within  the
 state  a  lifetime history is maintained on exposure to radon daughter concen-
 trations  when  certain minimum  values are reached.  The State  Department of
 Natural Resources Division of Mines  administers these.

 1.4.2.2   New Mexico
     In New  Mexico, a mine plan must be filed with and  approved by  the State
 Mining Inspector  before  he will issue  a permit.   The  State Mining  Inspector
 does not  review  the  plan for  environmental impact.   Groundwater use rights
 are 'established  by the  State Engineer, and the  Land  Commission handles ex-
 ploration and mining  rights.  The engineer's office issues a permit  for bene-
 ficial  use of any water pumped  from uranium mines.  However, the Navajo tribe
 claims jurisdiction of the State's groundwater in  the northwest region of New
 Mexico.   It  is  likely that  the  Departments  of  Interior and  Justice will
 eventually become involved in this dispute as Trustees for the tribe.

     Approval status has been given, with some exceptions, by EPA to New Mex-
 ico's plan for  the  attainment and maintenance of  national  air  standards (40
 CFR 52.1622)."  However,  neither Federal nor State regulations Include speci-
 fic emission standards, for uranium mining.   But  "Ambient  Air  Quality Stan-
 dards"  (40  CFR  50.6) on  suspended  particulates  apply to all sources  of air
pollution.

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                                                                      1-48
      New Mexico is  an  NRC agreement state, but  It  is not an approved  NPDES
 state.   Part 2  of the  amended  Water Quality Control Commission  regulations
 applies  to  any  discharge that  is  not subject to a  permit  under the NPDES sys-
 tem.   The State requires  approved  discharge  plans for discharges that  could
 contaminate groundwater.  However, the applicable NPDES  regulations  (Subpart
 E-Uranium,  Radium and  Vanadium  Ores Subcategory,  40 CFR  440.50) have  been
 challenged  by  some  mine  operators.  They  claim  that   discharges  to  a dry
 arroyo  do  not  constitute  "the   discharge  of pollutants  into  the navigable
 water,  water of  the continguous  zone,  and the  oceans,"  Because more  than
 half  of active  New  Mexico mine  discharges have  NPDES  permits  that are now
 under adjudication,   there is no enforcement and  discharges may not  be  in
 accordance  with Standards.   If  the  NPDES  challenge is  sustained,  then New
 Mexicc's  Part 2 regulations could  be applied,  even  though they are  not  par-
 ticulirly  suitable for  uranium  mining  discharges.   PosMbly only the  regu-
 lations  on chemical   oxygen demand and settling  of  heavy metal  solids would
 apply to uranium mine wastes.  The  Part 3 "Regulations for  Discharges onto or
 below the Surface of  the Ground"  (3-100) that are  designed  to  "protect all
 groundwater"  would also  be important.  A discharge  plan  is required for ef-
 fluent discharges  that  move directly or  indirectly  Into  groundwater, if the
 effluent contains  any of the contaminants  listed  in Section  3-103 a, b, and
 c,  or toxic pollutants.  Since the  list of contaminants  includes  uranium and
 radium,  New  Mexico  can  approve  only discharge  plans meeting  the  drinking
water standards.

      There are no  state  regulations for solid wastes and  land reclamation for
mining operations.   The mining plan and bonding requirements associated with
mining permits determine the extent of mining reclamation.

      Radiation  safety  requirements {Sections 74-3-1 et seq NMSA 1978}  apply
to both mining and milling.  Air quality monitoring  in underground mines cur-
rently involves  potential   duplication of effort  by the  New  Mexico  Mine In-
spector  (69-5-7 et  seq  NMSA  1978)  and  the Federal  Mine  Safety  and Health
Administration (30 CFR 57.5-37).

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                                                                      1-49
 1.4,2.3   Texas
      Texas is an  NRC agreement state, but  not an EPA approved NPOES  permit
 state.  The Department  of Water Resources  controls water  use.   Even  though
 much  of the water  used  in Texas comes  from wells,  there are no regulations  on
 pumping groundwater.   However, some  counties  have regulations  that  limit
 groundwater withdrawal  to control  subsidence.

      Specific  regulations  for in  situ uranium  mining  are  enforced  by the
 Texas Department of  Health (TDH).  Since  Texas  is  an  agreement state, its
 regulations reflect all appropriate  NRC regulations.  The TDH also implements
 the  Safe  Drinking Water  Act  (SOWA) and monitors  groundwater to assure  that
 its provisions for radium and  selenium concentrations are met.

      The  General  Land  Office  (GLO)  issues  prospecting  permits  and mining
 leases  on  state-owned lands.   Mining and reclamation plans  for uranium mining
 on  state-owned  lands are reviewed for approval  by GLO.   The "Texas Uranium
 Surface Mining and Reclamation Act"  exempts state-owned lands from regulation
 by the  Railroad Commission.

      Surface  mining  is regulated  by the Railroad Commission,   All  require-
 ments of  state  and federal laws must be fulfilled  before a permit is issued.
 Mining  and reclamation plans  must  be  submitted  and  approved.  A  bond  is
 required to assure reclamation after mining.

      The Texas Air Control Board administers provisions of  the Clean Air Act.
 Except  for suspended  particulates, there are  no  applicable standards,  i.e.,
 there are  no state source  standards, for uranium mining.

     The Texas Guides and Regulations  for Control of Radiation (TRCR) do not
 apply to  surface uranium  mining.   They do apply to in situ  mining due to NRC
 agreement  state  licensing.   The  radioactive  content of water discharged from
 all mines  to the environment must not exceed TRCR limits.

 1.4.2.4   Utah
     Utah  is  neither an  NRC  agreement  state  nor an NPDES  permit  approved
state. The Utah  State Engineer's  Office is  responsible for approval  of water

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                                                                      1-50
 use  rights.   The Department  of Natural  Resources  oversees  exploration  and
 mining rights on State  lands.

      The Division of  Oil, Gas, and Mining  of the Department of  Natural  Re-
 sources issues permits for uranium  mining operations, except in  situ  mining
 licensed by the NRC.   A  mining and reclamation plan  must  be approved.  Rule
 M-10 standards include consideration  of  land  use, public  safety and  welfare,
 impoundment,  slopes, high walls,  toxic  materials,  roads and  pads, draining,
 structures  and  equipment,  shafts and  portals,  sediment control,  revegetation,
 dams, and  soils.   Bonding  requirements assure  reclamation.

      Discharges  to  surface  waters  are  regulated  under the  EPA  administered
 NPDES system  and  the Utah  Water Pollution Committee.   Utah  dees  have  separate
 regulations  administered  by  the Department  of Social  Services.   These  are
 applied to mining operations such  as  non-discharging  waste water  systems  and
 in  situ mining where no NPDES permit  is  required.

      No sources  of pollution will  be  allowed  to cause groundwaters to  exceed
 drinking water standards.  The applicable standards  for   classes  1A and IB
 domestic water sources  are given in Wastewater Disposal  Regulations,  Part  II.

      Utah  is  developing radiation safety  regulations.   We  do  not  expect that
 they will  apply  to  uranium  mining, since they are based  on the model state
 suggested regulations.

 1.4.2.5  Washington
      Washington is an NRC agreement state  and  an NPDES approved permit  state.
 The  Department  of Ecology regulates water use and water quality. Washington
 has  no  regulations  for groundwater.  These waters could  be protected under
 the  Safe Drinking Water Act.

      The  Department of Natural  Resources controls  exploration  and mining
 rights  for state-owned  lands only.  The mineral lease  law covers both surface
 and  underground  mining but  not in  situ  or  heap  leaching.   The  State Rec-
 lamation Act  applies to  state  and  private lands only.  A  mining and  recla-
mation  bond  is required  before a permit  is  issued.   Reclamation is assured

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                                                                      1-51
      Washington has a Clean  Air Act under which  regulations  have  been prom-
 ulgated consistent with the  Federal  Clean Air Act.  No source emission stan-
 dards  have  been  issued  for  uranium mining.   National  Ambient Air  Quality
 Standards could apply  to  suspended particylates.

      Washington has rules and  regulations  for radiation  protection»  but they
 do not apply to uranium raining.

 1.4.2.6   Wyoming
      Wyoming is an approved  NPDES permitting State but not an  NRC Agreement
 State.   The  State  Engineer's Office  controls water use rights.   Control  is
 primarily on the quantity of  water uced,  but there is       statutory  respon-
 sibility  regarding  sedimentation.   Discharges to surface waters  are regulated
 by the Water Quality Division of the Department of Environmental  Quality.  The
 construction of any water  or waste water facility  requires  a  construction
 permit.   Groundwater  regulations  have  been proposed.  These  include  ground-
 water quality  standards for  any activity.  Permitting requirements specific
 to in  situ   uranium  operations is  one "of a group of  special  process dis-
 charges.

      The  Land  Quality Division of  the Wyoming  Department of  Environmental
 Quality  is the  principle agency responsible  for enforcing  environmental pro-
 tection  standards  and reclamation standards  with respect to uranium mining
 operations.  The Division also enforces  mineral exploration regulations that
 afford  protection  to  groundwater  and  restoration  of significant  surface dis-
 turbances.

     Wyoming  law requires  that uranium mined  land must be restored to a use
 at  least  equal  to  its highest  previous use  (W.S, 35-il-4Q2(a)(i)  and (ii))
 and mining operations must be conducted to  prevent  pollution of waters of the
 State  (W.S.  35-ll-4G2(a)(vi)).   Before a mining operation  receives a permit
 it  must submit to  the Department a mining and reclamation plan that demon-
 strates compliance  with  the  law  and associated rules  and regulations.  The
plan  must contain  a plan  for  the disposal  of all acid-forming, toxic mat-
erials or  materials constituting a fire, health,  or  safety hazard  uncovered

-------
                                                                      1-52
 or created  by  the  mining  process:  radioactive material  is included  (W.S.
 35-ll-406(b)(1x)).

      An  operator must also,  in  accord  with  his  approved  mine and  reclamation
 plan,  cover,  bury,  impound, contain,  or  dispose of toxic,  acid-forming,  or
 radioactive  material  determined to be  hazardous  to  health  and safety  or  con-
 stitute   a   threat  of   pollution   to   surface  or   subsurface  waters   (W.S.
 35~ll-415{b)(iv}).  A  required surety bond assures that the operator will re-
 claim  the land according  to  his  approved plan.   If the bond is forfeited, the
 State  is responsible  for reclamation.

     Wyoming   has  legislated authority for  a position on  radiological   res-
 toration o-*  mined lands. It  is  described  in the Division's  Guideline No.  1,
 Section  III,   The  Division  is  presently  drafting  regulations for radiation
 protection on  uranium mined  lands and handling of uranium mine wastes.  These
 regulations  shall set standards.

     Wyoming  also has a  solid waste management  program  that  presently regu-
 lates  only  refuse  generated at mines.  Solid waste  disposal sites are  per-
 mitted  at  these facilities.  Solid  waste regulations could be  promulgated
 that affect mining.

     In  Wyoming, Ambient Air Quality   Standards  are  applied  to  mining oper-
 ations,  and fugitive emissions are controlled to the extent that these stand-
 ards  are met.  An Air Quality  Permit   is  required for the  construction  of a
 uranium  mining and/or processing facility, and the  applicant is  required to
 demonstrate that applicable  ambient and PSD {Prevention of  Significant Deter-
 ioration) provisions are  met.

     Wyoming  has radiation  protection  regulations  for  the  safety of mines
while  they are actually in  process.  These  regulations are under the juris-
diction  of  the State  Inspector of Mines.  According  to  Wyoming Law, the pro-
tection  of  miners  from  hazardous  exposure to radioactivity  must  conform to
the American  Standards  Association  revised  Publication  N 13.8,  "Radiation
Protection in  Uranium Mines  and Mills."  The uranium  regulations (94-R-ll)
are found in Chapter 3, Article 4 of Title 30 - Mines and Minerals.

-------
                                                                      1-53
 1.5   References

 AEC74  U.S.  Atomic Energy  Commission,  Directorate of  Licensing,  Fuels  and
      Materials,  1974,  "Environmental  Survey  of  the   Uranium  Fuel   Cycle",
      WASH-1248.

 Cu77   Culler,  F. L.,  1977,  "An Alternate  Perspective   on  Long  Range Energy
      Options",  Conference  on U.S.  Options  for  Long Term Energy Supply, Den-
      ver, Colorado,  Atomic Industrial Forum Report,  Vol. 3.

 DOE79  U.S.  Department of  Energy,   1979,  "Statistical  Data  of  the  Uranium
      Industry",  GJO-100(79).

 Du79   Durler,  D.L.,  0. S.  Steel  Corporation, Texas  Uranium Operations, Corpus
      ChHsti, TX, 12/4/79 personal communication,

 EPA76  U.S. Envirormental  Protection Agency, Office of Radiation Programs,
      1976,   "Final   Environmental  Statement for Environmental  Radiation Pro-
      tection Requirements  for Normal  Operations of  Activities in the Uranium
      Fuel Cycle", EPA 520/4-76-016.

 ERDA75   Energy  Research  and Development Adminstration, Office of the Assis-
      tant Administrator for Planning and Analysis,  1975, "Total Energy, Elec-
      tric Energy and Nuclear Power Projections, United States"»

 EW78   Electrical World, 1978, "Annual Electrical Industry Forecast",

He77   Hetland, D.  L. and Wilbur, D.  S., 1977, "Potential Resources",
      presented  at  the  Uranium  Industry  Seminar,   Grand Junction,  Colorado.

Ja7i  Jackson,  P,  0.,  Perkins,  R. W.,  Schwendiman, L, C.» Wogman,  N.  A,,
     Glissmeyer, J.  A.  and  Enderlin,  W.  I.,  1979, "Radon-222 Emissions  in
     Ventilation Air  Exhausted  From  Underground  Uranium  Mines",  Battelle
     Pacific  Northwest  Laboratory  Report,  PNL-2888  REV.,  NUREG/CR-0627.

-------
                                                                      1-54
 Ja80  Jackson, P. Q.»  Battelle  Pacific  Northwest Laboratory, Richland,  WA.»
      12/80,  Personal  Communication,

 Ka75  Kallus,  M.  P.,  1975,   "Environmental Aspects of Uranium Mining and  Mil-
      ling  in South Texas",  U.S.  Environmental Protection Agency Report,  EPA-
      906/9-75-004.

 Ka78  Kasper,  D.*, Martin, H.  and Munsey, U, 1978,  "Environmental Assessment
      of  In Situ Mining", Report  prepared by PRC Toups Corp. for the U.S. De-
      partment  cf  the  Interior, Bureau  of  Mines,  Contract  No.  J0265022,

 La78  Larson,  Vt.C., 1978,  "Uranium  In Situ Leach Mining in the United States",
      U.S.  Department  of  the  Interior, Bureau of Mines Information Circular 8777,

 Le77  Lee,  H.  and Peyton, T.O.,  1977,  "Potential Radioactive Pollutants Re-
      sulting  from expanded  Energy  Programs",   U.S.  Environmental  Protection
      Agency  Report, EPA  600/7-77-082.

 NEP77 National Energy Plan  (NEP), April 1977.

 Ni78  Nininger, R.  D.,   1978, Atomic Industrial  Forum Conference, "Fuel Cycle
      •78", New York,  NY.

 Ni79  Nielson, K. K., Perkins, R. W.» Schwendiman, L» C. and Enderlin, W. I.,
      1979,   "Prediction  of the Net Radon Emission from a Model Open Pit Uran-
      ium Mine",   Battelle Pacific Northwest Laboratory Report, PNL-2889 Rev.,
      NURE6/CR-0628.

 NRC76 U.S. Nuclear Regulatory Commission, Office of Nuclear Material, Safety
      and Safeguards,  1976,  "Final Generic Environmental Statement on the Use
      of Recycled  Plutonium in Mixed Oxide Fuel  in Light Water Cooled Reactors",
      NUREG-0002,  Vol. 3.

NRC77a  U.S. Nuclear Regulatory Commission, Office of Nuclear Material Safety
     and Safeguards,  1977,   "Draft Environmental  Statement Related to Operation
     of Sweetwater Uranium Project",  NURE6-0403, Docket No. 40-8584.

-------
                                                                      1-55
 NRC77b  U.S.  Nuclear Regulatory  Commission,  Office of Nuclear  Material  Safety
      and Safeguards, 1977,  "Final  Environmental  Statement Related  to  Operation
      of Bear  Creek  Project",   NURG-0129,  Docket  No.  40-8452.

 NRC78  U.S.  Nuclear Regulatory Commission,  Office of Nuclear  Material  Safety
      and Safeguards, 1978,   "Draft Environmental  Statement related to  Opera-
      tion  of  Highland  Uranium  Solution Mining  Project", NUREG-0404, Docket  No.
      40-8102.

 NRC79   U.S.  Nuclear Regulatory Commission,  Office of Nuclear  Material  Safety
      and Safeguards, 1979,   "Draft Generic  Environmental  Impact Statement  on
      Uranium  Milling",   NUREG-0511, Vol.  1.

 NLJS76  NUS Corporation, 1976, "Technical Assessment for  Specific  Aspects  of
      EPA Proposed Environmental Radiation Standard  for the Uranium Fuel Cycle
      (40CFR190)  and  its Associated Documentation",  A Report Prepared for the
      Atomic Industrial  Forum, AIF/NESP-011.

 Pe79a  Perkins,  B.L.,  Energy  and  Minerals  Department, State  of New Mexico,
      12/13/79, personal  communication.

 Pe79b  Perkins,  B. U,  1979,  "An Overview of the New Mexico Uranium Industry",
      Mew Mexico  Energy and Minerals Department Publication, Santa Fe»  New Mexico,

 St78  Stone and Webster  Engineering Corp., 1978,   "Uranium Mining,  and Milling -
      The Need, The Processes, The Impacts, The Choices",   A Contract Prepared
      for  the  Western Interstate Energy Board, U.S.  Environmental  Protection
      Agency Report, EPA-9Q8/1-78-OQ4.

Th79   Thomasson,  W.  N.,  1979,   "Environmental  Development Plan for  Uranium
     Mining,  Milling and Conversion",   U.S.  Department of Energy,  DOE/EDP-0058.

Th78  Thompson, W. E.,   1978,  "Ground-Water Elements of  In Situ Leach mining
     of Uranium",  A Contract  Prepared  by Geraghty and Miller, Inc.,  for the
     U.S. Nuclear Regulatory Commission,  NUREG/CR-0311.

-------
                                                                     1-56
TVA78a   Tennessee  Valley Authority, 1978,  "Final Environmental  Statement  -
     Morton Ranch Uranium Mining".

TVA78b  Tennessee Valley  Authority  and  the U.S. Department of  the  Interior,
     1978,  "Draft Environmental  Statement - Crownpolnt Uranium  Mining  Project",

USC78  U.S. Congress,  1978,   "Uranium Mill  Tailings  Radiation Control  Act of
     1978%  Public Law 95-604.

Wy77  Wyoming  Mineral  Corporation,  1977,   "Environmental  Report -  IHt,aray
     Project, Johnson County,  Wyoming",   Wyoming Mineral  Corporation, 3900 S.
     Wadsworth Blvd., Lakewood,  Colorado  80235.

-------
         SECTION 2





INVENTORY OF URANIUM MINES

-------
                                                                 2-1
2.0  Inventory ofUranium Mines
          To  inventory  the  numbers,  types,  and locations of uranium mines in
the United States, we used data from the Department of Energy, Grand Junction
Office  (DOE-GJO).   We produced the inventory  of  uranium mines  presented in
this section  and Appendixes £ and F  of this  report  from the DOE-GJO master
data  file (DOE79a)  and personal communications  with  DOE-GJO (Ch80» HE80a»
MESQb).  These two sources combined yielded our own  EPA master data file,
which we  divided  into two parts - active and inactive mines.

     Table 2.1  classifies active and  inactive  U.S. uranium properties  accor-
ding to the method  of uranium  production (mine type)  based on data  that  were
current as of 1978  (MeSOa).  The major  mining  methods are  surface and  under-
ground  mines  (DQE79b).  The  remaining mining methods  are only minor contrib-
utors to  the  total uranium ore production (DOE79b).

     Table 2,1 shows a total of 340 active mines.  This final total, which  is
52  less than  the original  total  of 392 active  mines  provided  by DOE-GJO
(MeSOa),  was  derived, in consultation with DOE-SJu (MeSOb), by eliminating 43
mines that were duplicated on the list and 9 that were small  producers (i.e.,
producing only  a few  tons of ore for  the entire year  of  1978).  Most (if not
all) of  the 52 eliminated mines were either  underground or  surface mines.

     The  original totals  of 305 active underground mines and 63 active sur-
face mines (DOE79b), whose combined total of 368 mines accounts for the later
eliminated 52 mines that were duplicate listings or small producers, were the
totals we used  in modeling the average  underground and surface mines in  this
study.   The differences between these totals and the smaller Table 2.1  totals
of 256 active  underground mines and 60 active surface mines are insignificant
compared  with other uncertainties  in predicting  health effects.  The smaller
totals  for underground and surface mines would  introduce differences of  less
than 17%  and  less than 5% for the active  average underground and  average
surface model  mines, respectively.

     Table 2.2 gives  locations  and types of active uranium mines by state.
With respect  to  the  number  of mines, Colorado  and Utah  dominate the inven-
tory,  especially  for underground  mines.   However, since  New Mexico  and

-------
                                                                 2-2

Wyoming  have  large  mines  (underground  in  New  Mexico,  and  surface  in Wyoming)
and  dominate  ore production.  New Mexico  is the site  of  our model active
underground mines and  Wyoming  is  the site of  our model  active  surface  mines.
Our  model  in  situ  leaching operation is also sited in Wyoming, which is one
of  two  states mining uranium with that method.  Appendix E gives a complete
inventory of active uranium mines.

     The  numbers  of inactive uranium  mines according to state and mining
method are given in Table 2.3.  Colorado and Utah have the greatest number of
inactive  mines,  but Arizona,  Wyoming, New Mexico, and  South  Dakota  also
contain significant numbers.  Since New Mexico and Wyoming have dominated ore
production over  the past  10 years  (DOE79b), New Mexico (because of its  large
underground mines)  is  our model  site  for inactive underground mining  and
Wyoming  (because of its large  surface  mines)  is the site  of  our model  inact-
ive  surface mine.   Appendix  F gives a  complete inventory  of  inactive uranium
mines.

     Figures  2.1  through  2.9 are  maps  showing  the locations,  status,  and
types of  uranium mines in Colorado, New  Mexico,  Texas, Utah,  and Wyoming
(Ch77, Co78a,  Co78b, Co78c, Ea73, 6175, H169, Pe79, Ut77).  Since it is not
always possible  to  show all  the mines  in  a given district, the maps indicate
only the  area and  number  of mines in  some major  mining districts, partic-
ularly for Colorado and Utah, The maps  do  not  show the location of many small
mines started  during  the  uranium boom of the 1950's  because  their  exact
locations are  unknown.  In Colorado alone there are  over a thousand  such
mines.

     Table 2,4 shows total  ore production through January 1, 1979  for active
and  inactive  surface and  underground mines.  The larger  mines {>910 MT ore
production) dominate the  list  of  active mines, and the smaller mines  (<910
MT ore production)  dominate the  inactive  list.  If remedial action becomes
necessary for  inactive mines,  the information in  Table 2.4 could help esti-
mate the magnitude  of  such an action,  at  least affording  a way to wake  rough
estimates of  waste  rock,  sub-ore, and  overburden  that are present at  the
inactive site.  A recent  DOE report (DOE79c) contains  additional  information
on mining waste tonnage and acreage of  specific properties.

-------
                                                                 2-3
                     Table 2.1  Type of U.S. uranium properties
     Uranium                       Number of                     Number of
Production Method^	Active Properties	Inactive Properties
Surface mine
Underground mine
Mine water production
Heap leach • dumps
Heap leach • ores
Dumps
Sub-ore
In-situ leijchlng
Miscellaneous
Tailings dump
Unknown
60
256
2
1
0
1
1
11
0
2
6
1252
2036
1
7
1
42
12
2
23
0
13
                 TOTAL                 340                         3389
     ^'Categories listed in this column  are modifications of the originals
(DOE79a).   Copper by-product and surface-underground combination categories
were eliminated because they contained no properties.  The miscellaneous-
phosphate  by-product category was reduced to miscellaneous because most phos-
phate by-product properties were not included in the DQE-GJO master data file
(DOE79a).  The low grade or protore category was changed to sub-ore to be con-
sistent with the rest of this report.

-------
Table 2.2  The location and type of active uranium properties
Surface
State Mine
^rtiona
Colorado
New Mexico
Texas
Utah
Washington
Wyoming
TOTAL
1
5
4
15
13
2
19
60
Mine
Underground yater Heap-Leach
Mine Production Dumps
1
106
35
0
108
0
6
25fi
0
0
2
0
0
0
0
2
0
0
0
0
0
0
1
1
Heap-Leach
Ores Dumps
0
0
0
0
0
0
0
0
0
0
I
0
0
0
0
1
Sub-ore
0
0
0
0
0
0
1
1
In-Situ
Leaching
0
0
0
8
0
0
3
11
Tailings
Miscellaneous Dump Unknown Total
0
0
0
0
0
0
0
0
0
1
0
1
0
0
0
2
0
3
0
0
3
0
0
6
2
115
42
25
124
2
30
340

-------
                               Table  2.3   The  location and type of  inactive uraiiitm  properties
Surface
Slate Mine
ftlaska
Arizona
California
Colorado
Florida
Idaho
Minnesota
Montana
Nevada
New Jersey
New Mexico
N, .Dakota
Oklahoma
Oregon
S. Dakota
Texas
Utah
Washington
Wyoming
Unknown
0
135
13
263
0
2
0
9
9
0
34
13
3
O
ft.
Ill
38
378
13
223
6
Underground
Mine
1
189
10
402
0
4
0
9
12
1
143
0
0
1
30
0
698
0
32
5
Mine
Water
Production
0
0
0
0
0
0
0
0
0
0
1
0
0
0
0
0
0
0
0
0
rfeap-leacti
_Jh£H£i_—
0
!
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
6
0
Heap-Leach
Ores Dumps
0
0 .
0
0
0
0
0
0
0
0
0
0
0
0
0
1
0
0
0
0
0
0
0
35
0
0
0
0
0
0
0
0
0
0
0
0
7
0
0
0
Sub-ore
0
0
0
1
0
0
a
0
0
0
8
0
0
0
0
0
1
0
2
0
In-Situ
leac*tinq Miscellaneous
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
2
0
0
0
0
0
0
0
10
1
0
1
0
0
0
1
0
0
0
0
0
6
0
2
2
Tail ings
Dump
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
(M known Total
0
1
0
6
0
0
0
0
0
0
2
0
0
0
0
1
3
0
0
0
1
326
23
1217
1
6
I
ia
21
J
183
13
3
3
141
42
1093
13
265
13
TOTAL
1252
2036
42
12
3389

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                                                               2 Acuve *nme&
                                                               7 lnaci&£ rfttjigs
GftAND^JUNC r/O/V
      «
                                                                     SPRfP/GS

                                                                        EL PASO

                                                                  nactwe mines
MONWOSE
                                                                             LEGEND
                                                                             • ACTIVE MINES, TYPE UNKNOWN
                                                                             a INACTIVE MINES, TYPE UNKNOWN
                 Figure 2 1 Location of active and inactive uranium mines and
                           principal uranium mining districts in Colorado
                                                                                                                          KJ
                                                                                                                          I

-------
                                                                              2-7
                                                      COLORADO
                                                 LEGEND
                                               A, • ACTIVE MINES. TYPE UNKNOWN
                                               I, D INACTIVE MINES, TYPt UNKNOWN
                                                           10
20
                                                                      I KilomBters
Figure 2.2 Location of active and inactive uranium mines
          and pnnapai uranium mining districts in the
          Uravan Mineral Belt of western Colorado

-------
                                                              8
                                                              0Q «.,,,.
     _ J
©
CBOWN POINT
MARIANO LAKE
                                      (nomsia take

                                        *©.•

                                      * •:•:-..
                                                         1   /

                                                         *   I
                                                                 	'-,0 C
                                              o_ ..._.   _
                                                W%*  |~ «>#Wrtll*!*.» >	*-
                                             _ j »,.,,i*«~^  
-------
                                                                                   2-9
                                    98
5 PLANNED IN-SITU OPERATIONS
AND 1 PLANNED OPEN PIT MINE
 4 ACTIVE IN-SITU OPERATIONS
                                        Karnes City

                                         *
                                            KARNES CO
                     Three Rivers
LEGEND
* ACTIVE SURFACE MINE
O PLANNED SURFACE MINE
  INACTIVE SURFACE MINE
(§) ACTIVE IN-SITU OPERATION
  PLANNED IN-SITU OPERATION
                   LIVE OAK CO.

                      m
                                                      0    15    30    45
                                                                              Kilometers
                                                                       2B'
                  Figure 2.4   Location of active, inactive, and proposed
                              surface and in situ uranium mines in Texas

-------
                                                                              2-10
     114"
                                         111
42
                                              MINES IN THIS AREA  ..
                                      WAV.NE '  : SHOWN IN FIGURE 2 6  "•'
   LEGEND
       DISTRICT CONTAINING SPECIFIED NUMBER OF MINES. TYPE AND STATUS UNKNOWN
       SINGLE MINE LOCATION. TYPE AND STATUS UNKNOWN
          Figure 2 5  Location of uranium mines and mining districts in Utah

-------
                                                                                 2-11
EMERY
                      VtK
              AM) SAN RAfAti
              MINING Disinters
                • COMBINCD,
                                                _._	„„	
                                                                    MINING DlSmiC'    37
./
                                    Scale
Note Number within mining district is total number
of mines, status arvd type unknown

                           100

                             Kilometers
           Figure 2 6 Location of uranium mines and principal
                      uranium mining districts in southeastern Utah

-------
11° 1
10°
109°
i
                                            108
                                                          SHERIDAN

                                                            if Sheridan
                                                      \          _^ „—»
                                                              JOHNSON    I
                                              WASHAKlE   i
                                                           Location of mines
                                                           m mes* areas snown

                                                         NA'-JB'ONA
                                 Location Ot mioes
                                 in inese areas show,
41
    111'
                   110
                                  109°
                                                               107
                                                                              106C
                                                                                             105"
                                           Kiijmtieis
                                                                          LEGEND
                                                                           A Aclit/e Surface Mine
                                                                           V Inactive Surface Mine
                                                                           • Active Underground Mine
                                                                           D Inactive Underground Mine
                       Figure 2 7  Location of active and inactive uranium mines
                                  and principal uranium mining areas m Wyoming
                                                                                                                                    INJ
                                                                                                                                    I

-------
                                                                           2-13
                                                                     -4--
                                                                            -43°
                                «l
                                        Gas Hills
                  if
                  Jeffery City
Split Rock
     Crooks Gap  Green Mountain
            5  10  15  20  25  30
   LEGEND
   A Active Surface Mine
   V Inactive Surface Mine
   3 Active Underground Mine
   O Inactive Underground Mine
                                KILOMETERS
Figure 28  Location of active and inactive uranium mines in the Gas
          Htlls and Crooks Gap-Green Mountain areas of central Wyoming

-------
                                                                                  2-14
                                                          Pumpkin Buiies
	1-
                     Tea Pot Dome
                                  *
                               *
                          Casper
                             Shirley Basin
                                                             Powder River Basin
                                                                                --43°
  N
                                                                            Douglas
                                                LEGEND
                                                A. Active Surface Mine
                                                V Inactive Surface Mine
                                                • Active Underground Mine
                                                D Inactive Underground Mine
                                                      10    20
40
                                                                       Kilometers
            Figure 2 9 Location of active and inactive uranium mines
                      m the Shirley Basin, South Powder River Basin,
                      and Pumpkin Buttes areas of Wyoming

-------
                        Table 2.4   Cumulative Ore Production
                               through January 1, 1979
                        Active
Inactive
Ore Production                                   Under-                                 Under-
      MT        No. Mines  (% of total)  Surface ground  No. Mines {% of total) Surface ground
< 91
91-910
910-91,000
> 91,000
Total
16
33
188
103
340
(4.7)
(9.7)
(55.3)
(30.3)
(100.0)
8
5
15
32
60
3
24
165
64
256
1553
753
986
97
3389
(45.8)
(22.2)
(29.1)
(2.9)
(100.0)
899
134
180
39
1252
628
588
766
54
2036
                                                                                                           r\>

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                                                                  2-16
2.1   References

Ch77   Chapman, Wood, and Griswold,  Inc., 1977, "Geologic Map of Grants Uran-
      ium  Region," New Mexico Bureau of Mines and Mineral Resources Geological
      Map  31  (rev.).

Ch80   Personal communication with William L. Chenoweth (DOE-GJQ), January 1980.

Co78a  Colorado Geological Survey, Department of Natural Resources, State of Col-
      orado,  1978, James L. Nelson-Moore, Donna Bishop Colli-is, and  A. L. Horn-
      baker,  "Radioactive Mineral Occurrences of Colorado and Bibliography", Bul-
      letin 40.

Co78b  Collier, J.D., Hornbaker, A.L., and Chenoweth, W.L., 1978, "Directory of
      Colorado Uranium and Vanadium Mining and Milling Activities", Colorado Geo-
      logical Survey Map Series 11.

Co78c  Cook, L.M., 1978, "The Uranium District of the Texas Gulf Coastal  Plain",
     Texas Department of Health, Austin, Texas.

DOE79a  Department of Energy, Grand Junction Office, 1979, magnetic computer tape
      of selected information on U.S. uranium mines.

DOE79b  Department of Energy, 1979, "Statistical  Data of the Uranium Industry", GJO-
      100(79), Grand Junction, Colorado.

DOE79c  Department of Energy, 1979, "Report on Residual  Radioactive Materials on
     Public or Acquired Lands of the United States", DOE/EV-0037, Washington, D.C.

Ea73  Eargle, D.H., Hunds, G.W., and Weeks, A.M.D., 1973, "Uranium Geology and
     Mines, South Texas",  Bureau of Economic Geology Guidebook 12, University
     of Texas at Austin.

G175  Glass, G.B., Wendell, W.G., Root, F.K, and  Breckenridge, R.M., 1975, "En-
     ergy Resources Map of Wyoming", Wyoming Geological  Survey.

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                                                                 2-17

H169  Hi!pert, US,, 1969, "Uranium Resources of Northwestern New Mexico", USGS
     Professional Paper 603.

MeBOa  Letter from Robert J. Meehan (DOE-GJO) to Thomas R.  Norton (EPA-EERF),
     dated January 16, 1980.

MeSOb  Personal  communication with Robert J. %ehan (DQE-GJO), January 1980.

Pe79  Perkins, B.L., 1979, "An Overview of the New Mexico Uranium Industry",  New
     Mexico  Energy  and  Minerals  Department,  Santa   Fe,  New  Mexico.

Ut77  State of Utah, Department of Natural  Resources,  Utah  Geological  and Mineral
     Survey, 1977, "Energy Resources  Map of Utah", Map 44,

-------
            SECTION 3

POTENTIAL SOURCES OF CONTAMINANTS
   TO THE ENVIRONMENT AND MAN

-------
                                                                        3-1

 3.0  Potential Sources of Contannnants to the^Environment and Man
 3.1  Backgrpund Concentratio ns of Rad 1 gnu c 11 des and Trace Me ta 1 _s_
 3.1.1 Najiujra 11 y Qc c u r r 1 ng Ra d \_o.n u_c_1_T_d_e_s

      Potassium-40 and  radionuclides In  the  decay chains  of  uranium-238 and
 thorium-232  are  the  principal  sources  In the  earth's  crust  of  background
 radiation.    Figures  3.1  and  3.2  show the uranium-238 and  thorium-232 decay
 chains.  Potassium-40  constitutes  0.0118  percent  of  naturally  occurring po-
                                       Q
 tassium.   Its  half-life  is  1.26  x 10   years  and, upon  decay, potassium-40
 emits a 1.46  MeV  gamma  ray in 11  percent  of  its disintegrations.   Table 3.1
 lists the  average  concentration of  and  garrma-ray energy released  by these
 radionuclides in one  gram  of rock.  Table 3,?  lists  the  radionucllde content
 and dose equivalent  rates  from  common rocks  and soils.   Potassium-40 and the
 thorium-232 decay chain each  contribute  aboui  40 percent of the dose rate at
 3  feet above the  ground while the  uranium~238 decay chain contributes approxi-
 mately 20  percent of the  total dose rate.
      Radon-222 occurs in the  uranium-238  decay chain and has  a half-life of
 3.8 days.    It is a  noble  gas and, upon  decay,  produces a series of  short-
 lived,  alpha-emitting daughters  {see Fig.3.1\   The average  atmospheric radon
 concentration in the  continental   U.S. is 0.26 pCi/liter (Qa72).  Under  most
 conditions,  the  radon daughters  contribute less than  10 percent (a  few  tenths
 of  a yrem/hr)  to the  terrestrial  external dose  equivalent rate.   However,
 inhaled  radon daughters contribute  a  large  fraction of the total  dose equiva-
 lent  rate to  the  respiratory  tract:  about 50 percent (90  mrem/yr)  to the lung
 and  nearly  all  of  the  dose   (450  mrem/yr)  to  the  segmental bronchioles
 (NCRP75).
      Eighty-five  percent of the  surface area of the United States,  and  nearly
 all of its  population, is underlain by rocks and  soils of  sedimentary origin.
 However,  the  correlation  between  the  bedrock  activity  and  the aboveground
 activity is not clear.
      In  most soils,  the amount  of water varies from 5 to 25 percent.    The
 soil  moisture attenuates gamma  radiation  from the soil.   The  potassium-40
dose  equivalent  rate can decrease  by  30  percent when the soil  water content
 increases from 0 to 30 percent (OA72).   Moisture can retard the  diffusion of
radon  into  the atmosphere  and reduce the  exposure to  airborne  radon  daugh-
ters.    Since  radon  daughters account for 95 percent of the gamma-ray  energy
from  the uranium-238  series,  their  accumulation in  the  ground  increases

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                                                                 3-2
              URANIUM — 238 DECAY SERIES
Figure 3 t The uranium decay series showing the half lives and mode of decay

-------
                                                                 3-3
              THORIUM - 232 DECAY SERIES
232
M11
14 x

a

228
88R
5.8 v










fi
10%



8
T,














/












228
S9Ac
61 hr.
/
P












/












228
90T
1,9 v
/
fry

224
88
3,6
i
220
86R
56 »

216
B4P
015



212
82*
10.6


h
r.

a, y

^3
da.
a, T
n
c
a, T
a
sec

a

3
hr.










212
S4Po
3 M 10"7iac.
/
212 X 64%
gjBi f p,v a.
I Ohr
/ , 	 i: 	 ,
Ay m% 208
r ' «,T 82»
Stable
/
208 /
a,Ti / ftv
3 1 min.
Figure 3 2 The thorium decay series showing the half lives and mode of decay

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                                                                  3-4
   Table  3.1   Gamma-ray  energy  released by one gram of rock

Isotope

Uranium-238 (in equi
decay products)
Uranium-235 (in equi
decay products)
Thorium-232 (in equi
decay products)
Potass iuirr4Q
Other Elements
Source: Oa72.
Table 3.2


Rock Type
f b)
Igneous basic
Silicic (granite)
Sedimentary
Shale
Sandstone
Limestone
Upper crustal
(c)
average
U.S. surficial -
(d)
average
Average
Concentration ,
Percent
1 ibrium with ,
2.98 x 10~*
1 ibrium with _.
0.02 x 10
1 ibrium with *
11.4 x 10
3.0
—
Radionuclide content and dose equival
common rocks and soil
Uranium Thorium
ppm mrem/yr ppm mrem/yr

0.9 5.2 2.7 7.3
4.7 26.9 20.0 53.8

3.7 21.2 12.0 32.3
0.45 2.6 1.7 4.6
2.2 12.6 1.7 4.6


2.8 16.0 10 26.9


1.8 10.3 9.0 24.2
Energy,
KeV/sec.


68.2

1.53

87.8
149
2.7
ent rates from

Potassiunr40
ppm mrem/yr

1.2 14.7
5.0 61.3

3.2 39.2
1.1 13.5
0.32 3.9


2.4 29.4


1.8 21.8













Total
mrem/yr

27.2
142.0

92.7
20.7
21.1


72.3


56.3
(a)
(b)
(c)
(d)
mrem/yr/ppm.  uranium, 5.73; thorium, 2.69; potassium-40, 12.3 (Be68).
Source:   C166.
Uranium and thorium averages (Ph64); potassium (He69).
Source:   Lo64.

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                                                                       3-5 .

 the  exposure   from   this  series.    Thus,   soil  moisture   decreases   the
 potassium-40 and  thorium-232  dose equivalent  rates and  increases  or  leaves
 unchanged  the uranium-238 series dose equivalent rate.
      Snow  cover  also  affects  the  terrestrial  dose equivalent  rate and  the
 radon emanation rate.   Gamma radiation attenuates exponentially as  a function
 of the density and thickness  of the  snow cover  (Oa72).   However, the overall
 influence  of snow on  population  exposure is  negligible since,  in  most popu-
 lated areas,   there  is  relatively  little  snowfall  that remains  for  long
 periods  of time.
      Table 3.3 shows  the average  dose equivalent  rate  due  to radiation  in
 some  Western  mining   states  (Oa72).    Terrestrial  radiation  in the Western
 uranium  mining states  is higher  than in the rest  of  the nation  due  to  the
 greater  concentration  of  the uranium-238  series.
          Table  3.3  Average dose equivalent  rates due  to  terrestrial
                    radiation  in western mining states
                                         Terrestrial Dose,
             State                          mrem/yr

           Arizona                           45.6
           Colorado                          65.8
           New Mexico                        51.7
           South Dakota                      45.6
           Texas                             29.0
           Utah                              45.6
           Wyoming                           45.6

     Concentrations  of  radionuclides  measured  in  surface and  groundwater
samples collected  on  a proposed uranium project site are listed in Table 3.4
(NRC79a).   The  large  variations among  concentrations at different collection

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                                                                       3-6

 sites are  typical  of surface  water concentrations.   (Concentrations  in sea
 water are  more uniform.)   Hence,  generalizations  about background  concen-
 trations  of radionuclides in fresh water systems are impractical.   Extensive,
 site-specific  studies  over an  extended  period  of time are necessary to obtain
 meaningful  background  concentrations for a  site.

 3.1.2  Stable  Elements
      Concentrations  of metals occurring  in  the  earth's crust  generally range
 from  several-   parts-per-billion   (ppb)   to  a  few  parts-per-million   (ppm).
 Measured  concentrations  vary widely  from site to site and often in different
 samples  taken   from  the  sama site.   Table  3.5 lists the results of measure-
 ments for selected elements.   It  should be  emphasized that  these are  general
 estimates  of element  competition  of rocks  in  the  United  States  and  do  not
 reflect large  variations  that  occur  within  the different rock  types.
      Concentrations  of  metals measured  in surface  and groundwater  samples
 collected  from different  locations  on  a proposed uranium  project site  are
 listed  in  Tables  3.6  and  3.7,  respectively.   There are  large differences  in
 the  composition of  surface and groundwaters.   Table  3.8 shows  the  average
 concentrations  of  three  trace metals that are sometimes  associated with mine
 discharge  water.   These values,  which  were  taken  from the results of  an
 extensive  study (Tu69),  approximate  average concentrations  in United  States
 Streams.   Background  concentrations  at any  specific   site  could  be much
 different.
        Table 3.8   Estimated average concentrations (ppb) of three
                    metals in U.S. streams

Element
Chromium
Molybdenum
Selenium
Turekian's
Resul ts
1.4
1.8
0.2
Other results from
Literature
1.0
1.0
0.2
Source: Tu69.

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                     Table 3.4  Radionuclide concentrations in surface and groundwater

                                in the vicinity of a proposed uranium project
i Concentrations, pCi/£
Radionuclide Location 1
i
U-238 9.8
Ra-226 0.4
Rn-222 145
Th-230 <0.1
Th-232 <0.1
U-238 2.0
Location 2
4.0
0.5
108
0.2
4.5
Location 3
Surface
Location 4 Location 5 Location 6
Water
2.5 1.8 1.6
<0.1 0.08 <0.1
42 <4 <4
0.3 <0.1 <0,1 —
Groundwater
2.3
3.2 3.8 1.2
Source: NRC79a.
                                                                                                              OJ
                                                                                                               I
                                                                                                              --a

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            Table  3.7   Concentrations of selected  elements in groundwater at six locations

                        in the  vicinity of a proposed uranium project
Concentrations, mg/£
Element
Aluminum
Antimony <
Arsenic
Barium
Beryllium
Cadmium
Cobalt
Chromium
Copper
Lead
Mercury
Molybdenum
Nickel
Selenium
Vanadium
Zinc
Location 1
<0.1
<0.01
<0.01
<0.1
0.001
<0.001
<0.01
<0.001
0.003
0.003
<0.0004
0.001
<0.01
0.06
0.01
4.4
Location 2
1
<0.01
<0.01
0.5
<0.001
<0.001
<0.01
0.003
0.00-3
<0.001
0.0012
0.002
<0.01
<0.01
0.01
0.07
Location 3 Location 4
0.8
<0.01
<0.01
0.5
<0.001
<0.001
<0.01
0.003
0.006
<0.001
0.0005
0.002
<0.01
<0.01
0.02
0.21
14.7
<0.01
<0.01
0.2
0.003
<0.001
0.01
0.004
0.027
0.003
<0.001
0.001
0.02
<0.01
0.01
0.07
Location 5
0.2
O.01
0.01
0.3
0.001
<0.001
<0.01
0.001
<0.001
<0.001
<0.0004
0.001
<0.01
0.13
0.02
0.01
Location 6
10
<0.01
0.04
0.7
<0.001
<0.001
<0.01
0.003
0.006
0.002
0.0017
0.003
<0.01
<0.01
0.08
0.02
Source: NRC79a.
                                                                                                               GJ
                                                                                                               I

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                                                                       3-11

 3.2  Mater-Related Aspects of UraniumMining

 3.2.1     Previous and Ongoing Hydrologle and Water Quality Studies Related
           to Uranium Mining
      In the late 1950's and early 1960's, the U.S. Public Health Service con-
 ducted field  studies  to  determine  the water quality impacts  of  the  uranium
 mining and  milling  industry.   The studies emphasized uranium  mining rather
 than mining.   The Federal Water  Pollution Control  Administration conducted
 extensive stream  surveys  to  assess  the effects of uranium milling  (but  not
 mining) on  the main  stem  and principal  tributaries  of the Colorado River.
 Subsequent  stream survey  work  in  Colorado by  the  Water Pollution  Control
 Commission and the U.S.  Geological  Survey (Mo74, We74) mentioned a portion of
 the Uravan  Mineral  Belt  and  uranium  mines  therein,  but the work  did  not
 emphasize uranium mines.   Significant amounts  of acidity  and  total  trace
 metal  concentrations  were  found in  streams from 18 different  mining areas.
 Dilution  and  chemical  precipitation  below  mine drainages decreased  concen-
 tration and  increased  the pH.  Given enough  time and distance,  the  streams
 recover naturally,  but  the accumulations  of  trace metals  in  the  sediments
 increase.    Field  observations  in  1971-72  of   streams  in  most  of Colorado
 indicated  that approximately  724 km  of streams  in 25 different mining  areas
 were adversely affected  by mine  drainage (We74).
      Discussions  of  the impacts of  uranium  mining on water quality or  quan-
 tity are incidental  in  numerous  impact statements and environmental  reports
 prepared  by  industry  and  (or)  the  U.S Nuclear  Regulatory Commission as  an
 integral  part of  licensing or relicensing uranium mills.   Coverage on mining
 is  usually minor  as the principal  focus is on  milling  impacts. The  same  is
 true for  the recently prepared  generic EIS  on  regulation of uranium  milling
 (NRC79b).'
     Radiochemical  assessment of  surface  and groundwater  in  uranium mining
 districts  of New Mexico is done by  self-monitoring programs  associated with
 NPDES  permits.   Also,  radiochemical  assessment  studies  have  been  funded
 recently by  the New Mexico  Environmental Improvement Division and  U.S  Environ-
mental   Protection  Agency-.   Self-monitoring,   particularly   in  the  pre-
operational  phase, characterizes  mining and milling operations  in  all of the
concerned  States.    These,  together  with  results  of  surveys  by  State per-
sonnel, have resulted in extensive files of water quality data, flow measure-

-------
                                                                       3-12
 ments,  field  observations  of  mine conditions,  and  exchanges  between  Industry,
 regulatory  agencies,  and   the  public.   Rarely  are  the data  assembled  and
 interpreted  for dissemination  outside a  given  agency.  States  experiencing
 rapid  growth  in uranium  mining  and  milling are  undoubtedly  placing  first
 priority  on  activities directly  related  to  licensing,  monitoring, and  other-
 wise  implementing  regulations.   Unfortunately,  there is no concerted  effort
 to  prepare broad assessments  of the  cumulative impacts  of mining  and milling.
 Texas,  New  Mexico,  and Wyoming  are  cases  in  point.   Critical review and  syn-
 thesis  of these  types of  data can produce  rather useful   information.   For
 example,  the  publication "Water Quality  Impacts  of  Uranium Mining and Milling
 Activities  in  the  Grants  Mineral  Belt,  New Mexico"  (EPA75)  addresses  the
 groundwater  and surface  water  changes  as  the  result  of  extensive uranium
 mining  and milling production in  a relatively confined  area,
     Some states have since  initiated review  of their data files, conducted
 field  studies,  and,   in  some  cases,  contracted study  teams  to investigate
 similar water quality changes.  For example, a  recent report by the Wyoming
 Department of  Environmental Quality  summarizes 16 years of aqueous radium  and
 uranium  data.   The  study  reports  that  significant  amounts  of  Ra-226  and
 uranium   were present  in  surface water  in the  Shirley  Basin as  a result of
 inadequate mine  water  treatment  (Ha78).
     In Texas, surface water and  groundwater  monitoring  conducted  by  indus-
 try, as well  as by State and Federal agencies,  reveal little or no change of
 chemical  quality attributable  to uranium mining  and milling  (Ge77,   Ka76).
 This conclusion is based  on  586  samples collected  from  198 stations  over a
 period  of 39  years  but primarily from  1961 to 1975.   The State monitoring
 program by several  agencies is continuing, but either summary reports are not
 issued  or are  two years  overdue, depending  on  the  agency.  Not all  of  the
 findings  exonerate the industry.   One survey (It75)  showed  that  none  of the
mine water  from the  10 lakes that were  sampled  was  suitable for human use.
 The lakes were  also  unsuitable for irrigation  due  to  mineralization  of the
 water  by  sulfate»  chloride,  and  TDS.  One of the  10 was suitable  for stock
watering,
     The  conditions  or limits  in the NPDES permits  consider the quality of
water being discharged, the quality of receiving water, and available, prac-
tical,  treatment technology.   Industry is required to monitor the discharges

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                                                                     \
                                                                       3-13

on  a  periodic  basis, usually  daily,  weekly,  or  monthly,  and  report  results to
EPA.   The  NPDES  permits  and related  monitoring  data  help  to estimate  the
quantity  and  quality of discharge allowed to enter  the  off-site environment.
      Intensive  studies of  the influence of uranium mining  on water  quality
and  availability  have  not been conducted.   Most investigations to date  have
been  site-specific,  of relatively short duration, and focused on the  influ-
ence  of  surface discharge or  subsurface seepage on  water quality.   Baseline
studies  from  specific  projects typically consist of quarterly  or semi-annual
sampling  and  are  oriented toward milling instead  of mining  activities.   The
effects  of  dewatering  on depleted water supplies  or on water  quality  shifts
in  the  aquifers of an area are  rarely considered, and, then oily on  a mine-
by-raine  basis.   Rarely  are   soil»  stream  sediment,  and  biologic  samples
collected in the preoperational period  for radiologic  analysis,,
3.2.2     Mine Water Management
     Figure 3.3  shows  a scheme for  considering  the  fate of water discharged
from underground  and  open pit mines,  including  principal  sources and sinks,
most of  which  affect  both water flow  and  quality.   Broken lines in Fig. 3.3
indicate  less  important  sequences  with respect  to  water quality.   For ex-
ample, those mines that handle all water by on-site evaporation are likely to
involve  small  volumes of  water,  and  impacts  on groundwater  as  a  result of
seepage are also likely to be small.
     Mine drainage  is  surface water or groundwater flowing from a mine or an
area affected  by  mining  activities.  Mine related point  and  nonpoint pollu-
tion sources  can contaminate  both  surface water and  groundwater throughout
all phases of  mining,  that is, during mineral  exploration, mine development,
mineral  extraction,  processing,  transport, and  storage,  and  waste  disposal.
While  mine-related  point  pollution  sources usually include only  milling and
processing plant discharges  and  mine dewatering discharges, nonpoint sources
can occur during any  or  all  phases of mining.  The  chemical and  physical
characteristics and the mode  of  transfer of these nonpoint sources  are vari-
able and  depend upon,  among  other things, the mineral  being  mined,  its  geo-

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Mine
Drainage
                          Evaporated
                          on Site
Ion Exchange
Plant U Removal


Uranium Mill
Process Water
mmJSm

Discharge to
Mill Tailings
Ponds
Settling
Ponds
Radium removed with
Barium Chloride


Discharge to
Streams and
Dry Washes
                         Discharge to
                         Streams and
                         Dry Washes
                         Agricultural
                         Use
Discharge to
Streams and
Washes
Discharge to
Streams and
Washes
                    Figure 3.3. Disposition of drainage water from active surface and underground uranium mines

-------
                                                                        3-15
 logic  environment,  the  interrelations  of all  associated  hydrologic systems

 (both  surface water  and  groundwater),  and  the  type of  processing, trans-

 portation,  storage,  and waste disposal  methods.   Some mine-related  nonpoint

 pollution sources are as follows (EPA77a):


      1.   suspended solids carried by immediate surface runoff
      2.   dissolved solids carried by immediate surface runoff
      3,   suspended and dissolved solids in proximate subsurface
           water seepage
      4,   dissolved-solids in groundwater recharge
      5.   dissolved solids in groundwater discharge
      6.   uncontrolled contributions from mine-related point sources:
           a.   high instantaneous concentrations of regulated pollutants
                1n excess of effluent discharge guidelines, but falling
                within the NPDES instantaneous and dally average discharge
                limitations
           b,   unregulated minor contaminants 1n point source discharges
                which are not specifically included under NPDES effluent
                limitations
           c.   untreated mine dewatering discharges during or following
                major storm events  (NPDES point source treatment systems
                may be bypassed during storm events of greater than a  10-
                year, 24-hour intensity)
      7.   reclaimed mine area and undisturbed area drainage diversion
           discharges
      8,   surface water and groundwiter contamination and degradation
           Induced by mine-related hydrologic disturbances and imbalances


 Typicallyi  waters  affected  by mine  drainage  are  chemically altered  by  an

 Increase  in  Iron,  sulfate,  acidity  {or  alkalinity),  hardness,  IDS,  and

'various metals, and are physically altered by an increase in suspended solids

 such as silt and sediment (Anon69,H168).

      Many but  not  all  uranium  mines  dewater  at  rates  of  1  to perhaps  20
  3
 m /rnin.  Typically, the water  from  the mine goes  to  settling  ponds and then

 either to the mill  or a  nearby  stream,  dry wash, river, etc.   Depending  on

 the amount  of  mine  water  recycled in the mill  and the amount of water pumped

 from the mines,  there may or may not  be any release to streams  or arroyos.

 In at  least one-instance in the  Grants  Mineral Belt, mine water is  totally

 recycled   through  the mine  to  enhance  solubilization  of  uranium  which  is

 removed with ion exchange columns.   Large evaporation ponds and some seepage
 losses  help maintain  a  water  balance and  minimize releases to  streams,

 arroyos,  etc.   Increasing competition   for  water In  the  western  states  1s
 likely  to induce maximum  mine  water reuse (in the mill),  reinjection, or use

-------
                                                                       3-16

 for potable  supplies  (H177)  or  power  plant  cooling.
      When  mill  tailings  ponds  are used  for final   disposal  of mine  water,
 there is significant addition  of  chemical  and radiochemical contaminants  to
 the water  in the  course of milling.   After treatment  to reduce  suspended
 solids,  mine water  may  be recycled  for  use  in the  milling  process or released
 to  nearby streams,  necessitating  radium removal  and reduction of  suspended
 solids.   Dissolved  uranium  in  mine water,  if present in  concentrations  ex-
 ceeding  about 3 mg/j,, is  recovered  by ion exchange columns.  Settling ponds  at
 the mines  remove suspended  solids.  The water is  then conveyed to  receiving
 streams  or  to the  mills for uranium recovery and (or)  to satisfy  mill  feed
 water requirements.   There  are rather  rigid  requirements for  release  to
 surface  water compared  to groundwater.
      A recent survey of  20  U.S. uranium mills (Ja79a) found large  variation
 in  the  degree of water  recycling.  Where mine water  is readily available,  it
 probably is  reused  less  than in water-short  areas.   More  efficient  water use
 by  uranium  mills   possibly  could   increase  the  amount of (relatively) high
 quality  mine water  being  discharged to  the environment; lessen adverse  impacts
 of  mill  tailings disposal  by reducing  the  amount of  liquid;  and  make mine
 water available as  a source  of potable water  {after treatment) in water-short
 areas such  as Churchrock and Gallup, New Mexico (H177). To  date, water qual-
 ity  deterioration   related to  seepage  and accidental  release  of tailings  to
 surface  streams  has received the most  study  and  has  been  the focus of regu-
 latory programs.  In the  future, it is likely that water quantity issues will
 become increasingly important, particularly in areas where water supplies are
 already  limited  and  where  extensive  dewatering  necessarily  accompanies
mining.
     Of  20  uranium  mills  surveyed, 6  reported part  or all  of  the  mill feed
water came  from mine drainage  (Ja79a),  In  New Mexico, 19  of  30  mines sur-
veyed by the State Environmental   Improvement  Division (J.  Dudley, written
communication)  had  off-site  discharge  to arroyos ranging  up  to  19 m  per
minute.   Those mines with no discharge utilized evaporation ponds or used the
water for dust control.   Most of the mines  discharged to arroyos.  In several
instances, however, water was  piped to a nearby mill  at flow rates of 5 to 8
m   per minute.   Relatively small  quantities of mine  water were used for sand
backfill  of mines,   in-situ leaching of old  workings,  and irrigation of grass-
                                                      3
lands.   In  summary, New  Mexico  mines  discharge  66  m  per minute  off-site.

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                                                                       3-17
              o
Of  this,  12 m  per minute  is  routed to mills, and  the  balance  is discharged
directly  off-site from  the mine.   Average  discharge  to streams and  arroyos
for  the  active underground mines  in the Grants Mineral  Belt  on  the whole was
1.8  m /min,  whereas  12  mines  in  the Ambrosia  Lake  District  averaged 1,7
 T
m /min.   In New  Mexico,  all mines  discharging to  an  arroyo practice  radium
removal  with approximately  90%  efficiency.  Uranium removal  from mine water
discharge  occurs  in  all  but two active mines.   Future  trends  are likely  to
reflect  increased  discharge  from the mine  to  the  environment.   Settling
ponds, radium  removal, or both will  be used  to meet discharge permit require-
ments.
     In  Wyoming,  discharge  from both  surface  and  underground  mines  may  be
used as  proces?  water  for uranium mills, discharged  to surface streams,  or
used for irrigation.  For  example, at the  North Morton  undergrourd  mining
operation, approximately 2 m  per minute of mine water discharge will  be used
to  irrigate  800 hectares of alfalfa.  At the South Morton surface mine oper-
ation, a like amount of discharge will  become mill feed water.
     A survey  of  all  active U.S.  uranium mills showed that  14 of 20 make  no
use  of mine  water (Ja79a).  This may reflect mines where water simply is not
encountered  or  the  fact  that mines  and mills  are not  co-located. Most mills
depend on  deep  wells,  except in New Mexico where  mine water  is the main mill
water  supply.   Table 3.9  summarizes water  sources  for U.S.  uranium  mills.
Proposed  NRC regulations on mill  tailings  disposal (44 Fed. Reg. 50012-59)
purport  to  make  long-term  tailings isolation  the primary  consideration  in
mill  siting.   In areas  subject  to  severe natural  erosive or  dispersive
forces,  this may mean that  mills  cannot  be  sited in  the  vicinity of  mines.
This may have effects on use of mine water for milling.
 Table 3.9  Summary of feed water sources for active U.S. uranium mills
       -    5OLjrce                            No. of Mills
           j  Reservoirs                           4
     Wells              .                          8
     Springs                                       1
     Unknown                                       1
     Mine Water                                   3
     Mine Water and Wells                         _3
                                                  20
     Source:   Ja79a.

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                                                                       3-18

      Although underground mining is now  dominant  in  the Grants  Mineral  Belt,
 the greatest  number  of mines ire  small  stripping operations that have  long
 been inactive.  This  type of mining  activity  has apparently had little  ad-
 verse impact on water  resources.   Few data are  available on  drainage  assess-
 ment of  large  open pit mines such as the Jackpile-Paguate.  The St.  Anthony
 pit discharges  about  0,076 m   per minute.  Usually,  the  ore  is  above  the
 water table.  Any water  present on the mine  floor presumably is  flood runoff
 or  discharge  from  a   nearby  underground mine.   Other strip  mines  in  the
 Mineral  Belt were not  studied;  hence,  no  conclusions were drawn  (J. L»  Kunk-
 ler, USGS,  in  preparation).
      Mine dewatering is done either by pumping the  mine pit/shaft directly or
 by drilling high  capacity wells peripheral  to  the  mine and pumping  a suf-
 ficient  volume of water  to at least partially dewater the sediments.  Because
 of the great volume of  water that must  be  removed  from an aquifer, the latter
 method  is  impractical  for deep  underground  uranium  mines.   This is  partic-
 ularly  true for  the  artesian aquifers of most of the  deeper  mines  in  the
 Grants Mineral Belt.  More commonly this method  is  reserved for shaft sinking
 and  open  pit mines  to depths of  several hundred  feet.  Most underground mines
 are dewatered  by pumping  the water  that collects in the mine  itself.  Borings
 ("longholes") made  into the ore  body for assay work and explosives facilitate
 drainage.   There is considerable difference in the  quality of water depending
 ort  the dewatering method  used.  Water removed from wells adjacent to the mine
 typically  is representative of  natural quality,  but water removed  from  the
 mine can  be high in radionuclides,  stable  elements, and suspended solids.  In
 large  part   this  is  due  to  the  disruptive nature  of mining.  However,  more
 subtle,  chemical  processes   of  oxidation  and  bacterial  action,  aided  by
 evaporation and  free flow of air in the mine, are also operative.
     The  extent to  which uranium  exploration  adversely  impacts water re-
 sources  is  not well  understood.   Land  surface disruption from  drilling  pads
 and  access  roads obviously affects  erosion rates and results  in mud pits and
 piles  of contaminated  cuttings  on or near  the  land  surface.   Subsurface
 effects are less obvious.  A potentially serious one is  interaquifer connec-
 tion via  exploratory  boreholes.   In Wyoming, 6 million  meters of exploratory
drilling took place in 1979,   Although State law requires  mining companies to
 plug  the holes  after  drilling,  it  is common  practice  to  install   only a
 surface  plug and  to  rely on  the   drilling mud  to effect a  seal at  depth.

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                                                                       3-19
 Similar situations are  likely In New  Mexico and Texas.  Shortages of  funds
 and  personnel  to  oversee  proper completion  and  abandonment exist at  the  State
 level.
      Hydraulic  effects of water  released from  mines,  whether from pumping  or
 gravity  flow,  include   increased   surface  discharge,  recharge  of  shallow
 aquifers  by infiltration,  and decline  of  static water levels  in formations
 intersected  by  the mine or  related  cone of depression.   Of  most concern are
 the  effects  relating  to  mine water discharge on downstream  users and any
 influences,  direct or  indirect, of pumping/dewatering  on water  quality in the
 ore  body  and contiguous strata.  In some locations, the Grants Mineral  Belt,
 for  example, the  ore  body  is  also  a major regional artesian aquifer; hence,
 dewatering affects present water  levels  and will  affect  water levels at  least
 to  the  year 2000, with complete  recovery taking  much  longer.   The extent and
 significance of uranium mine dewatering  are as  yet  poorly  documented.  Decent
 studies have been made in New Mexico where dewatering  is of concern because
 of  the  influence  on regional  groundwater availability for municipal use and
 in  relation  to  return   flows to  the   San  Juan River  (NRC79b;  Ly79).   In
 Wyoming,  static  water  levels  in wells  on  ranches  adjacent to uranium  mines
 owned by  Exxon,  Kerr-McGee, Rocky   Mountain  Energy Co., and other companies
 southwest  of Douglas  and between Pumpkin Buttes  and Douglas have reportedly
 dropped  7 to  10  meters  (Anon79).   Water  quality changes  associated  with
 dewatering generally are unknown  and not specifically  monitored  regardless  of
 the mining area location.
     Water  quality associated with  dewatering is  generally good,  although
 suspended  solids  may  be high, as expected.   Discharge from dewatering  wells
 will  be  low  in   suspended  solids   because of filtering  by soil   and  rock
 aquifers.   Overall water quality  from dewatering wells,  particularly for
 underground  mines,  is likely  to be  representative of ambient conditions  in
 the ore body and, to  a lesser extent,  the  adjacent formations that may also
 be dewatered.
     Recent  USGS  work on  groundwater in the  San  Juan  Basin Region has in-
 dicated that mining expansion will   have a  significant impact  on  the  water
yield of  the Morrison  Formation  (Ly79).   In   this  study,  although  no  water
quality data are  derived,  the recharge and  mine dewatering parameters  that
                                                                            o
 impact the expected drawdowns  in  the  aquifer imply  that  a  total of 7.03  x 10
 3
m  of water will  be produced by the  33 planned  or announced mines by the year

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                                                                       3-20
 2000.   If  the projected  development  of  72 mines  occurs,  dewatering  would
                  9   3
 exceed  1.48 x  10  m .  The  model  also estimates  that  flow in the San  Juan
                                          o
 River will  decline very slightly (0.05  m /min).   Similarly, flow in  the Rio
 Grande  Valley would  be  reduced by  0.85 m /min.   The  impacts will  continue
 after mining  and  dewatering cease.
     Table  3.10 summarizes New Mexico  uranium  mine discharge  in relation  to
 mine  type,   depth,  and  status (active  or   proposed).   Note  that  projected
 mining  is primarily  underground  and represents  an average  increase in  mine
 depth of  275 percent and  an  increase  in dewatering rate from 2.4 to 13.8 m
 per  minute.   One would expect numerous  water  quality  and quantity issues  to
 arise  if  these projections materialize.  For  example,  competition  for water
 supply  is likely to be widespread throughout 'he Upper Colorado River Basin,
 and  uranium  mines/mills  are already relatively large water users. Dewatering
 and  discharge  require no water rights  under  State  water laws  in New Mexico,
 but  the water  is essentially wasted.   Use  of water  in  mills constitutes a
 beneficial  use of  water,  and state water laws  therefore require filing for
 water rights.   Such  filings  may  be denied upon  protest  from  existing water
 users.
     Inactive  uranium  mines  and related wastes also influence water quality,
 particularly  as  a result of chemical and physical  transport by surface water
 runoff.   The main  reasons  why mine waste piles  erode more  quickly  than un-
 dis,turbed soils are lack of topsoil, steep angle of slopes, presence of toxic
 elements  and buildup  of salt  in  the near surface,  and  poor water retention
 characteristics.  Usually,  inactive surface and underground uranium mines are
 not  a source of direct discharge of water,  be  it contaminated or of ambient
 quality,  because  of the  low rainfall-high evaporation characteristics of the
 western uranium  regions, static  groundwater levels deep  below  the  land   sur-
 face  in mining areas, and,  in a  few instances,  recontouring  of  mined lands
 such  that drainage  is internal.   Whether  mines contaminate  groundwater by
 groundwater leaching or by recharge contacting exposed oxidized ore bodies is
 poorly  documented.  Preliminary  feasibility  studies  by  the U.S.  Geological
 Survey  (Hi77)  indicate generally  good  quality water from one inactive under-
 ground  mine  in the  Churchrock area of  New Mexico.   It is possible that this
water may be used as a municipal water supply for Gallup, New Mexico.

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                                                                       3-21
           Table  3.10   Current  and  projected  uranium mine  discharges
                       in  the Grants Mineral  Belt,  New Mexico
Mine Type
Active
Underground
Open pit
Proposed
Underground
Open pit
Number of
Mines

33
3

46
0
Average
Depth (m)

248
48

681
N/A
Average Discharge
(m /min)

2.42
0.045

13.8
N/A
 Source: Environmental  Improvement Division, State of New Mexico.
     For most uranium regions, the volume of discharge from inactive mines to
 surface water bodies, though poorly documented, is believed to be less signi-
 ficant  than that  from  active  mines.   The degree  to which  inactive mines
 contribute  contaminants,  directly or indirectly, to adjacent water resources
 can  only  be qualitatively  assessed.   The  significance of  inactive  mines is
 highly dependent on regional setting and mine type.
     Inactive surface mines in  Texas are,  with  rare  exception,  not  a source
 of direct  discharge  to  surface  water.  It  is unknown if there is any adverse
 impact  from standing water in the  mine  pits,  the most recent  of which have
 been  final-contoured  with  an  internal  drainage  plan.    Various  observers
 suspect  that water  quality  deteriorates  when  overland  flow  crosses  mine
 spoils associated  with  overburden piles  (It75 and He79).   Water in  the mine
 pits  is unsuitable  for  potable  and  stock use due  to high  stable  element
contents,  but it  is  generally acceptable in terms of radioactivity.  Water in
Texas  open pit  mines   is a  combination  of  runoff and  groundwater.  Before
release from  a  mine, water is  put  in retention ponds to  reduce total  sus-
pended  solids.  Holding  ponds are used for storing mine water, and discharge
is not allowed unless  such  discharge does not adversely affect the receiving

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                                                                       3-24

 Environmental  problems associated with  alkaline  and  saline  drainages  are  not
 well  documented  (Hi73).
      Water quality  impacts  from  uranium  mining  are  a  function  of  both  quality
 and  quantity of  discharge.  Underground  and  surface mines commonly  require
 dewatering prior to or during the  ore removal  phase, although there  is con-
 siderable  variation from one area or  mine to another.  In  New Mexico, large
 and   medium  sized  mines  are  essentially  dry,  whereas mines in  Texas   and
 Wyoming  require  extensive  dewatering.  Regardless of location,  underground
 mines rarely" are dry  and many require extensive  dewatering.   Considering  the
 variety  of water management measures,  regional  differences  in contaminants
 and  receiving waters,  and geochemical  characteristics  of ore bodies, detailed
 discussion of the  effects  of mine drainage or mining,  in  general, on water
 quality  must await  further site -  or area  -  specific study.   It is ques-
 tionable if  sufficient data  on mine drainage exist  to  assess effects on biota
 and  the fate of contaminants in  surface  or  sub-surface water bodies.
      Limited  data  from  Colorado,  Texas,  Wyoming,  and  New  Mexico   suggest
 adverse  impacts  on  water  quality from  discharge of  mine  water.   Effects of
 dewatering  on  deep  groundwater quality are very  poorly documented; hence, no
 conclusion as  to relative  significance is  drawn.   With respect  to   surface
 water resources,  discharge  of mine water  and overland movement  of water and
 suspended  or  dissolved   contaminants  may  be  significant.   Because   of  the
 dearth  of  data  on   overland flow,  emphasis  herein is on  contaminants  dis-
 charged  via mine drainage  water.  Substantial  studies  to  evaluate sediment
 yield  and  quality  from  lands mined for uranium, particularly from areas  of
 surface mining, have not been conducted, although recent work  in Texas (He79)
 is a  notable exception.
      Elements such  as  uranium,  radium, molybdenum, selenium, zinc, and vana-
 dium  may  be enriched  in  point  and  nonpoint discharges from  uranium mines.
 The dispersal, mobility, and uptake of such elements are directly relevant to
 the  subject  of  this report.  We  reviewed  selected  literature  and field  data
 to at least qualitatively  understand  what  processes  and  elements are  most
 significant  and   to  thereby  strengthen  some of  the  underlying  source  term
 assumptions in the transport and  health effects  modeling.  Despite the annual
 chemical  load introduced to ephemeral   streams by both dissolved and suspended
constituents in mine effluent and overland flow from mined  lands,  waste piles
etc.s a number of processes affect the concentrations in the ambient environ™

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                                                                       3-25

merit.   These  include dilution,  suspended sediment  transport,  sorption  and
desorption,   precipitation,   ion  exchange,  biological  assimilation  or  de-
gradation, and  complexation.
                                                                           /
3.2.3,1.1 Dilution  and Suspended  Sediment  Transport
      In many  uranium  mining  regions  there  is flooding  or  flash flooding*  Such
storms may  well be the  only  runoff  event  for a year or more at a  time.  It is
worthwhile  then to consider some of  the effects  of  such events on  mobili-
zation  of  contaminants  associated  with  uranium mining  wastes.   Typically
there  is  significant interdependence  between  the physical and chemical  pro-
cesses.
     A  principal  physical  process  is  dilution.   This  will  reduce  concen-
trations of  pollutants  released to  surface waters, but is considered  to  play
a relatively minor  role  over  the  short  term For water  percolating  through  the
soil to sources  of  groundwater  in arid  or  semiarid regions.
     Transport  of  suspended  sediments  in  floods  is another dominant process.
Suspended  load   is  largely  a result  of physical, hydraulic processes, hence
elements that are rapidly and thoroughly removed  from  solution as  a result of
solubility limits,  precipitation  with other ions, ion exchange, and sorption
may  well  be  transported in  the  suspended Toad.   In  metal mining  areas  of
central  Colorado,   total  and  dissolved metal  loads  in  streams  are  greater
during  high   flow  periods,  apparently  a  result  of  flushing  from mines  and
tailings piles  and scouring  of chemical  precipitates  from stream substrates
(Mo74).  Typically, total and dissolved  loads decrease downstream, regardless
of discharge.   Increase  in iron in the downstream direction reflects scouring
of  precipitate—an  amorphous,  hydrated  ferric  oxide.  Dispersal  occurs  for
quite a distance downstream.

3.2.3.1.2 Sorption and De_s_orpt_ion
     Sorption  can  play  an  extremely  important  role  in  purifying  waters,
particularly if- infiltration  or percolation is involved.   This is especially
true  when  contaminant  concentrations are  too  low to  undergo precipitation
reactions.   Virtually every  ionic species will  be sorbed  and removed to some
extent except   for  chloride and,  to a  lesser  extent, sulfate  and nitrate.
These seem  to  pass through  soils and  alluvium without  significant sorption
(Ru76).   Sorption processes can be highly specific, depending on  the  type  of

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                                                                       3-26
 contaminant and  the  physical and chemical properties  of  both  the  solution  and
 the  porous medium.
     There  have  been numerous  laboratory   studies  on  the sorption,  leach-
 ability,  and  mobility of stable elements in various  types  of soil.   A  recent
 review  of the literature on  radionuclide  interactions in  soils  specifically
 discusses  radium,  thorium,  and uranium, which are  especially  pertinent  to
 uranium mining (Am78).   Distribution coefficients, the ratio of concentration
 in  soil  to that  in  water,  ranged  between 16 and  270 for uranium in various
 soil-river water systems, between 200 and 470 fo*"  radium, and on  the  order  of
 10   for  thorium at  pH6.    These  observations appear  consistent  with  the
 generally accepted ideas that uranium is relatively mobile, thorium extremely
 immobile, and  radium somewhere in between  in neural water systems  (NRC79b;
 Ku79; Sa77a).
     Adsorption  is  believed to  be  important for  cadmium,  copper, lead,  and
 nickel, insofar  as  these are transported in the  suspended fraction, whereas
 manganese  and  zinc  are  primarily in the dissolved  fraction.  Adsorption  of
 metals  onto  precipitated manganese  oxides  or  hydroxides at elevated  pH  is
 probably insignificant in the case of most uranium mine discharges insofar  as
 these are  alkaline  and,  furthermore,  discharge to  or co-mingle  with  other
 streams that are alkaline.
     Radium sorption  and desorption  tests done on uranium  mill  waste solids
 and'river  sediments  collected  from several  locations in the Colorado Plateau
 (Sh64)  and  in Czechoslovakia  (Ha68)  showed that  leaching  is primarily con-
 trolled by the liquid-to-solid ratio, i.e.,  the volume of leaching liquid  per
 unit weight  of  suspended  solids.   Natural  leaching  from mining  and milling
 waste solids  freely  introduced  to  rivers  in  the  past  is  one of the  major
 factors in  radium contamination  of  rivers   (Ru58).   Although  settling  ponds
 are now used  to  remove or at  least  reduce  suspended solids from active mine
 discharges, the  dissolved  radium load  sorbed on sediments  presents  a source
 term that may  be somewhat analogous to river sediments  contaminated by dis-
 solved  and  suspended  milling  and mining  wastes.   The  manner in which  the
 radium  is  mobilized  .and the  significance   is  poorly  understood and  bears
 further investigation.  Apparently there is  a "leap frog" transport mechanism
 involving  combined chemical  and  physical  weathering processes.  There should
be a marked downstream attenuation  of both  dissolved and sorbed/precipitated
radium inventories  insofar  as sediment  burial  and  dilution  take place  and
Teachability  limits  are  reached,  i.e.,  no more radium can be removed regard-

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                                                                       3-27

 less of  the  duration,  frequency,  or Intensity  of agitation.   Should  the
 stream  eventually  discharge  into a  reservoir,  it  is  unlikely that  renewed
 leaching  will  take place.  Shearer and  Lee  (Sh64)  did not account for  some
 factors  that may be locally significant,  such  as  b1o-uptake  along  the  stream/
 river, use of water for  irrigation,  number of  uranium facilities discharging,
 and  other local  factors.
      Experiments were conducted in  Japan  (Ya?3)  to  determine uranium  adsorp-
 tion and  desorption using  carbonate  solutions  and  three soil types  (alluvial,
 sandy,  volcanic  ash).   Very high adsorption  ratios and very low  desorption
 ratios of uranium characterized  the  various soil  types  in contact with stream
 water and  help  explain  tne  decrease  in  soluble  uranium  with flow distance
 from mines  (Ma69).   When  wastewater flows into  streams at the maximum  per-
 missible  concentration (1.8  mg U/A)  recommended (ICRP64), Yamamoto  et al.
 (Ya73) conclude that the  uranium  behaves  as a uranyl carbonate complex anion
 and  that  essentially complete  sorption  readily  occurs in the  presence of
 (Japanese river) water  which contains  15 to  39.9 mg/i  bicarbonate.   Since
 this is  similar  to  concentrations  in surface waters  of  uranium regions in the
 western  states,  similar results  are  expected.
      Sorption or desorption  of heavy metals  such as  Co, Ni,  Cu,  and Zn in
 soils  and  fresh  water sediments  occurs  in response to the aqueous concen-
 tration  of metal, aqueous  concentration of other  metals,  pH,  and amount and
 strength, of  organic  chelates and inorganic complex ion formers  in solution
 (Je68).   Other controls  on the  heavy metal concentrations  in  soil and fresh
 water  include  organic matter,  clays,  carbonates,  and oxide  and hydroxide
 precipitates.
     To  what  degree solubility  acts  as  a limit  on stable element  concen-
 trations  in  natural  waters is unclear.  The crystal!ographic form or even the
 chemical   composition of a precipitate are often  unknown.   Elements  such as
 iron,  aluminum,  manganese,  and titanium  form insoluble hydroxides and  are
 likely to exceed equilibrium solubility limits (An73).   Hem (He60) partially
 disagrees,  saying "it is  not unreasonable to assume equilibirum for the iron
 species in water."   Whether mine discharges or overland  flow from mined areas
 are  in equilibrium  is unknown, but it is doubtful considering the underground
or flash-flood origin of such waters.  The non-equilibrium aspects of certain
peak runoff  events  has been documented for major streams of the world (Durum
and  Haffty,  1963),   Metals such as  iron,  aluminum,  manganese,  and titanium,

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                                                                       3-28

which  readily form rather  insoluble  hydroxides  as participates or  colloids,
may  be  dissolved  from  suspended  minerals  during  high  flow  conditions.
Organics present  in such  flood waters may assist through  formation of  soluble
complexes.   Resulting  metal concentrations may be higher than  solubility and
redox  relationships alone would  indicate.

3.2.3.1.3,     Precipitation
     Probably  one of  the most significant processes affecting  stable  element
solubility  in natural  water  systems is  adsorption  on  hydrous ferric  and
manganese  oxides.  Jenner  (Je68)  believes this is  the principal  control  on
the  fixation of  Co, Ni,  Cu,  and Zn (heavy metals)  in  soils and  fresh water
sediments.   For example,  ferric  hydroxide adsorbs one  to  two orders of magni-
tude more SeCU per unit weight than clays, and 90 to 99 percent adsorption is
possible at  a pH of seven to eight typical of most western streams (Ho72).  At
neutral or  slightly  alkaline pH, both iron and  manganese are  poorly  soluble
in oxidizing systems and, in general, exhibit very similar chemical  behavior,
although manganese  is  slightly more soluble.   Fixation of selenium in soils,
particularly by  iron  oxide  or as ferric  selenite,  renders it unavailable to
agricultural and forage crops, although specific selenium-accumulating plants
can  remove  the  element and, upon decomposition, release  it  in water  soluble
forms,  such  as selenate  and organic selenium compounds, available  to other
plants  (Ro64).   The  behavior and mechanism of selenium adsorption (as selen-
ium  oxyanion)  by  hydrous  ferric oxides  is  readily  extended  to the  inter-
pretation  of other similarly  bound minor elements  (Ho72).   Mobile  selenium
oxyanion in  slightly  alkaline waters  might be carried  to streams  by surface
runoff  or  in  groundwater.   Selenite selenium  sorbed  upon  ferric  hydroxide
should be transported in surface waters at neutral  or slightly acid  pH. Other
metals  forming highly  insoluble  hydroxides in the pH range of 6 to 9 include
copper  (above pH  6.5),  zinc (above  pH 7.5),  and nickel (above pH 9).  Molyb-
denum  is  thought to  hydro!yze to the bimolybdate ion  under acid  conditions
and  precipitate with  iron and aluminum.   Aerobic or oxidizing  conditions  in
the  vadose  zone  are  favorable for the  development  of many of these  oxides
(Cu,  Fe,  Mn, Hg, Ni,  Zn, Pb).  Reducing conditions deep in saturated zones
generally lead to increased mobility of these  metals.
     Reducing conditions  that  can exist  in the presence  of  organic  material
(bituminous  or  lower  ranking  coals,  anaerobic bacteria, fluidized  humates)

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                                                                       3-29
can  lead  to precipitation reactions  favorable  for  removing  contaminants  from
mine waters.  Reduction of uranium  to the quadrivalent  state and  its  fixation
on  clays  would  play  the major  role  in  protecting  groundwater supplies  from
uranium  if  the  appropriate  reducing agents  were  present  in  soils  (Ga77a;
Ku79).   Inorganic  reducing  agents could  include  ferrous  iron  and  hydrogen
sulfide  produced by  the  action of an aerobic  bacteria on  sulfates.  Natural
reducing  conditions  can  also,  theoretically,  cause  the  formation  of  such
native  elements  as  arsenic,  copper, mercury,  selenium,  silver,  and lead,
which  are  all  quite  insoluble in  their  elemental  form  (Ru76).    Hydrogen
sulfide  or other sulfides,  if  available,  will  serve  to reduce the  concen-
trations  of such metals  ar, arsenic,  cadmium,  copper,  iron,  lead, mercury,
molybdenum, nickel, silver, and  lead.
     The  metal-scavenging of hydrated iron  oxide precipitate  has been docu-
mented in a mined area of Colorado where relatively acid  schists and gneisses
give  rise to acid  runoff that  dissolves large quantities  of  aluminum, mag-
nesium, and zinc.  Runoff  from a  nearby  drainage basin underlain by basic
rocks  containing base  and  precious  metal  veins  carries  considerably  less
metal. However,  manganese oxide precipitated with  iron oxide  contains large
quantities  of  metals.    Ferric  hydroxide   precipitates  from  aerated water
solutions containing  more than 0.01 ppm iron at  pH values  of 4.5 and above,
aluminum  hydroxide  precipitates  in the pH  range of  5 to  7,  and  manganese
hydroxide  precipitates  above pH8 (He60; Ch54).   Considering the  alkaline pH
of most uranium mine discharges  and overland flow from non-point sources  such
as  mine  waste  piles,  precipitation  of  iron  and  possibly manganese seems
certain.  The scavenging effect of iron hydroxide at neutral  to  alkaline pH is
considerably less than that of manganese hydroxide precipitate.
     The extensive  studies  of  mine drainage in Colorado  by Morgan  and Wentz
(1974) revealed  the effects  of solubility  on  stable  element  transport.   In
the downstream direction, dilution and neutralization of  the acid mine drain-
age by bicarbonate  caused dissolved metal  to decrease due to dilution, chem-
ical  precipitation,  and  probably  adsorption  onto  ferric  hydroxide  preci-
pitate.   The  latter  creates  a coating  on  the stream  substrate  for  a  con-
siderable distance during low flow periods.   Subsequently, flood events scour
and transport the precipitates.   Manganese  and zinc remain  primarily in  the
dissolved  phase  for a considerable distance, whereas  cadmium,  copper, iron,
lead,  and nickel  concentrate  in  the suspended  fraction  and, when turbulence

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                                                                       3-30

 decreases,  precipitate.   The  mobility  sequence  for  the metals  studied  in
 Colorado  generally  follows  the order  Mn s Zn  > Cu > Cd >Fe>Ni>  Pb.  Ferric
 hydroxide precipitation and  scavenging  seems to be more important at neutral
 than at acidic pH's  (Je68).

 3.2.3.1.4 Biological  Assimilation and Degradation
      Biological  uptake and the  role  it has on  stable  element  concentrations
 in  water is  not  predictively  understood  (An73).   Plant  uptake  of  stable
 elements and resulting phytotoxicity  is  not merely a  function  of how much  is
 present in the  soils  or  water.   In the case of  arsenic, the chemical  form  of
 arsenic appears more  important  than  the  total  soil arsenic (Wo71).  For ex-
 a'pjile,  water-soluble  arsenic in  soil  created  more f.hytotoxic effects  than
 those  with  no  detectable water-soluble arsenic.   Soils  high  in  reactive
 aluminum  remained  less  phytotoxic,  despite  heavy applications  of  arsenic,
 than soils with low reactive  aluminum.   Selenium  in soils  can be  present  as
 elemental  selenium,  selenates,  pyritic selenium,  ferric selenites, and or-
 ganic  selenium  compounds  of  unknown  composition.   Selenates  and  organic
 compounds are  most available  to  plants,  although slow  hydrolysis  of the  other
 forms can occur  such  that they become  available  for plant uptake. The im-
 portance of  water soluble selenium versus  total selenium as  the  major factor
 affecting  plant  uptake has been  demonstrated  (La72; Gr67).   Where  sufficient
 selenium is  present  in plant-available  form,  all  species will  take  it  up  in
 sufficient amounts  to be  harmful  to  animals  (La72).  Naturally occurring
 soils containing such  available  forms  are  geographically confined to  semiarid
 regions  or areas of  impeded drainage.   Such  soils are not hazardous to humans
 and  only locally are they a threat  to  animals.
      Despite  numerous  examples  of  high selenium (up  to 2,7 ppm) in surface
 water,  particularly  that  associated with drainage  from seleniferous soils  in
 agricultural areas,  Rosenfeld and Beath  (Ro64)  reported only a few cases  of
 water-related  selenosis  in  man  or livestock.   Water  high  in  selenium   is
 typically  unpalatable  to  livestock and certainly to man.  Lakin  (La72)  con-
 cluded  that  environmental contamination  due  to selenium is increasing, but
 hazardous  concentrations are unlikely; mining and industrial wastes may cause
 local  problems;  and  the  effect  of added  selenium  in  waters in  combination
with other contaminants bears further study.
     Uranium uptake  by several  species of  native plants in the southeastern

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                                                                       3-31
 Utah portion of  the  Colorado Plateau varied, sometimes  strikingly,  with the
 species, time  of year, part of  plant,  availability of uranium in  the  soil,
 and chemical composition of the underlying rocks (Ca57).   The type of rooting
 system  and  the  soil  moisture  conditions  also were  influential.   In  some
 cases, there was  no  consistent relationship between the  amount of uranium in
 the soil versus  that  in the plant ash.   Plants are much less selective with
 respect to  cadmium uptake,  and  it has  been conclusively demonstrated  that
 plants  absorb  cadmium  from cadmium  containing solutions  and soils  (Pa73;
 Fu73). Phytotoxic-effects  vary considerably with plant species.   Cadmium and
 zinc  sulfides  tend  to  concentrate  in  the  organic matter  of soils.   Upon
 oxidation  to  sulfate,  plant  availability  increases  along with  solubility.
 Under alkaline conditions  (ph8),  cadmium is taken  up rapidly by biota  and by
>sediments.   However,  modelinc  of  cadmium transport  and  its  deposition  in
 aquatic systems  is very complex  and encompasses many variables,  most  impoY-
 tant of which are  pH,  carbonate content, chemical   form,  and  competing  ions.

 3.2.3.1.5  Complexation
      Published data on  Gibbs free energies,  enthalpies,  and entropies  of  42
 dissolved  uranium  species  and  30 uranium-bearing solid phases were  recently
 reviewed (La78).   Uranium  in  natural  waters is usually complexed with  car-
 bonate, hydroxide, phosphate,  fluoride,  sulfate, and perhaps  silicate.  Such
 complexes  greatly  increase the  solubility  of  uranium minerals and  increase
 uranium mobility  in  groundwater  and  surface water.  In waters with typical
 concentration  of  chloride,  fluoride,  phosphate,  and  sulfate, intermediate
 Eh's,  neutral  to alkaline  pH's,  and the presence of phosphate  or carbonate,
 uranyl  phosphate or carbonate  complexes  form and increase mineral solubility
 by several  orders of magnitude.   Sorption of the uranyl minerals carnotite,
 tyuyamunite, autunite, potassium  autunite,  and uranophane  onto  natural mater-
 ials is greatest in  the  pH range  of 5  to  8.5.   Uranium  content  of  small
 streams,  in  particular,  can  exhibit wide spatial and temporal  variations  due
 to pH  and  oxidation  state  of  the water,  concentrations of  complex-forming
 species such as carbonate  or sulfate,  and presence  of highly  sorptive mater-
 ials such  as organic matter, certain  metallic hydroxides, and clays (La78).
 Whereas sorption  is  probably a  dominant control on  stable  element concen-
 trations in  low temperature aqueous conditions, there  is  insufficient infor-
mation  concerning specific  sorbents  to  allow  accurate prediction.

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                                                                       3-32

 3.2.3.2   Results  of Field  Studies  injjram'um  Mining Areas

 3.2.3.2.1  Colorado
      Extensive  studies  of  the  effect  of  mine drainage on  stream water quality
 and biota  were done  in  centra]  Colorado (Mo74).  Although uranium  was  mined
 in 14  of  the  25  areas studied, other  metals  were  the   principal  products.
 Most  of the  ores  were  high in  iron  sulfides, and  associated drainage  was
 acidic.  Also  studied,  but  less  intensely, was  the Uravan  district of western
 Colorado where  the principal products are uranium and  vanadium from Mesozoic
 sandstone.   The Uravan Mineral Belt  is  different  in terms of  principal  pro-
 duct  dnd  geologic  features  from  other mining areas  studied in  Colorado.   For
 thesa  other  areas,   the  drainage  is  acidic  and  heavily enriched  in  heavy
 metals  and, therefore,  somewhat atypical of most Colorado  uranium mines  in  the
 Uravsn  area.
     After  a preliminary  field  survey  of  the temperature, specific  conduc-
 tivity, pH,  stream-bottom  conditions, and aquatic biota at 995 stream sites,
 192 were  chosen for detailed  sampling  and  analysis  during  1971-1972.   The
 data indicate the  contamination of  approximately 711  kilometers of streams  in
 25 different  areas,  mostly  in the  Colorado  Mineral  Belt.  The  water  quality
 effects  in these  areas  arise  from many varied  causes, including active and
 inactive mine  drainage, tailings pond seepage,  drainage tunnels, and milling
 operations.  The length of  the streams affected is not absolute as  it varies
 with the time of the  year and flow  conditions (Mo74).
     The general findings  indicate  that Mn, Se, and SO,  concentrations, and
 specific conductivity are poor indicators of mine drainage as natural sources
 can cause high  values for these parameters even  in undisturbed  areas. Uranium
 mines make  at  least some contribution to problems of contaminated streams  in
 central Colorado.  In central Colorado, the exact impact of uranium mining on
 stream water  quality  is unknown but believed to be less important or signif-
 icant  in most areas  as  compared  to impact from other  mining,  with  the  pos-
 sible  exception of  the  Boulder-Jamestown  area  (J.  Goettl and D.  Anderson,
 Colorado  Game,  Fish,   and  Parks   Division  and  Water  Pollution  Control
 Commission,  respectively,    personal  communication).   Cadmium, As,  and  Pb
 exceed  the U.S. Public Health Service  toxicity limits,  respectively,  12.5
 percent, 1.4  percent, and  2.1  percent  of  the  time.   Mercury  and  Ag limits
were never exceeded,  and Cr was never detected.   Iron and Mn  standards were

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                                                                       3-33

 frequently exceeded  by  large  percentages,  however,  these  limits  are  only
 based  on  aesthetics.    Concerning  the  negative  impacts  of  the  various
 constituents,  Cu  and Zn  {exceeding  the  limits  7.8 and  9.0  percent of  the
 time,  respectively)  pose  the  greatest  threat  to resident  aquatic  life.
 Mining  operations in the  Uravan  area are a relatively  minor  source of metals
 for the San Higuel River  (Mo74).   Potential  problem areas are  settling  ponds
 and  tailings  piles  associated  with  the mining  operation.   Although not  a
 source  of acid drainage,  these  sources  did cause increased concentrations  of
 copper,  iron,  manganese,   nickel,  vanadium,  and zinc  in the  river.   Only
 manganese exceeded  the standard  for drinking  water,  and no  metal  concen-
 trations  exceeded  the biological  criteria.  Seepage  (0.003 m /s,  pH 6.8,  3300
 mg/£ HCXL) from a mine  tailings  area  into Atkinson  Creek,  a tributary of the
 San  Miguel  River,  observed  in   December 1972  caused no  adverse  impacts.
      Because  of its  size, proximity  to population, and  effects  on  surface
 water quality, extensive  surface  water  quality  investigations  to  assess the
 impacts of mine  water  discharge  from the Schwarzwalder  mine  have  been made
 (EPA72).   Grab samples  of the mine  effluent taken  in 1972  revealed 15 mg/£
 uranium and 80 pCi/£ radium-226.   As  of 1972, overflow and seepage from the
 settling  ponds  used  to  treat the mine  effluent  significantly  degrade the
 radiochemical  quality of  nearby  Ralston  Creek.   This  was confirmed by both
 EPA and the State/Denver Water Boards monitoring  program. With 20-fold dilu-
 tion,,  Ralston  Creek  downstream  of  the  mine contained  3 pCi/st  and 82 pg/£
 dissolved  radium-226  and uranium,  respectively.    With  no  dilution,  as during
 July, concentrations  were  81  pCi/£ and  20,300 yg/£ . Influx  of contaminated
 stream  water  to  nearby Long  Lake raised  dissolved radium-226  to 0.8 pCi/£
 (4-fold  increase  over  background)  and uranium to 230 y g/s,   (20  times back-
 ground).   From these data,  conclusions  were  reached  that  the  mine water
 caused  a  5 percent  increase in  the  radiation dose  to consumers  in a local
 water system  (based  on  FRC and  NCRP standards  and  daily  consumption of 1.0
 liter water).   If  the 4.5 mg/£  uranium  limit proposed by  ICRP was  used, the
 estimated dose  increases to nearly 40 percent of the dose limit for a popu-
 lation  group.   Since  1972, the effluent  has  been treated  for radium-226 and
 uranium removal.   Trace  metals  analysis   of water  samples  collected from the
creek and the water treatment plants revealed concentrations comparable to or
greater  than  those  in   the effluent  as  of  July 20,  1978.   Concentrations

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 (pg/s, }  were as follows:
                                                                       3-34
 Mine Effluent
 Ralston Creek  (avg)
 Water treatment  plants (avg)

 *mg/«,
M
5
5
5
fi
1
1.3
0.55
Pb
15
32
97
Se
<2
<2
2
In
18
56
146
 3.2.3/4.2  Wyoming
      he  assessed  the effects  of mine  drainage  by  literature  review and  a
 limited  field study  in  the Spring of  1979.   Results of "Che latter  conclude
 this   section of  the  report.   The  effects  of  mine  dewatering,  in  situ
 leaching,  and mill  tailings seepage on  surface  water quality in the Shirley
 Basin were  previously studied  by the  Wyoming  Department of  Environmental
 Quality  (Ha78).  Sixteen years  of  data on aqueous  radium  and uranium indicated
 significant  amounts  of  radium-226 and uranium  reached  streams  because  of
 inadequate mine  dewater  treatment, mill tailings   pond  seepage, and  improper
 operation  of  a  precipitation  treatment  unit.   Uranium  concentrations  in
 stream water increased 60-fold because of mine  water discharge and  possible
 tailings pond  seepage.  The effects of past loadings  of  uranium  and radium  on
 fish  propagation or  migration  are  not clear,  although  biologic  uptake  of
 uranium  and   radium  has  occurred.   Phytoplankton,  algae, and  bottom fauna
 organisms  also do  not appear to  have been adversely  affected, but no  studies
 have  been conducted since 1962.   Long-term effects of increased  radioactivity
 levels are known and  merit further study:  "There exists real need for addi-
 tional  studies to determine  the mechanisms  involved in  the  dispersion  and
 ultimate  disposal  of  uranium  loaded  into  the   drainage  basin...Only after
 additional studies have  been  completed, may we understand the total and long
 range impact  that  the company's activities have  had  on  the aqueous environ-
ment" (Ha78).  This  latter finding related  specifically  to the current  (1978)
loading of uranium from treated mine discharge.
     Previous  studies by  the  State  of Wyoming  (Ha78)  found  that  solution

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                                                                       3-35

 mining by the  Pathfinder  Uranium Company noticeably affected ambient uranium
 concentrations  in   the  study  areas.  A  1968  survey  by  the Department  of
 Environmental  Quality  (Ha78)  indicated  relatively  high loadings  of soluble
 uranium and  radium  on  stream  sediments near  the  mine dewatering  outfall.
 Analysis of  fish skeletons indicated radium uptake corresponding  to dissolved
 radium-226 concentration  exceeding  1  pCi/£.   Resampling  in  1970 showed  a
 decrease in  radioactivity  values  in sediment but a tenfold  increase in fish
 uptake of uranium  relative to  other fish populations in  the  basin.   Radio-
 activity concentrations  in fish tissue  were highest near the mine  effluent
 outfalls but  did  not  constitute  a major  source  of  radioactive intake  by
 consumers.
      In June  1971,  the EPA Radiological  Activities Section  of  Region  VIII
 (Denver) made  a  field reconnaissance of uranium  mining  and  milling  activities
 in  the Shirley Basin area.  Radiological  analyses of water and sediment sam-
 ples  in the  Shirley  Basin  and  in the Bates  Hole  drainage  basin  to the  north
 unquestionably indicated  significant  increases  in  radioactivity  levels  in
 water,  sediment,  and fish  because  of effluent discharge from mines  and  mill
 tailings.  Concentrations  of dissolved  radium-226 and  uranium  in mine efflu-
 ent  were well  above  background.  The discharges were not considered  a source
 of  radiation  dose   to  the  populace (residents  and transients)  because  of
 remoteness and lack of water use,  but toxic effects on fish were  of concern
 (M.  Lammering,  written  communications,  1979).    Monitoring  in  1972  by the
 Wyoming Game and  Fish Department  showed  water quality effects as  far as  seven
 miles  downstream.   From  1970  to  1972, radium-226  concentrations  remained
 stable,  but  uranium  increased.   Fish  samples  collected in  1972 showed in-
 creased  amounts of  radium in  the flesh compared  to the 1970 results.   Soil
 samples  from a creek that  received  mine effluent  indicated relatively  large
 transport  and  enrichment  of  uranium and  radium.   Radium  in  particular was
 enriched in  the sediments  and  showed  temporal  variations  indicative  of  suc-
 cessive  scouring and removal,   presumably  in flood flows.  Precipitation  of
 uranium compounds was not apparent,  probably  because oxidized uranyl  species
 are quite soluble in  natural water.
     To  further  our understanding of the  role  aqueous  pathways play in  con-
 taminant dispersal,  we monitored stable and radioactive trace elements in the
Spring of 1979 in surface runoff from ore, sub-ore, and overburden  piles  From
the Morton Ranch area  of  active mining  in  Wyoming.   EPA  personnel selected

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                                                                       3-36

 the basic study areas  and  assisted  in sample collecting.   Most of the samp-
 ling,  analysis,  and interpretation  was  done under  contract with  Battelle,
 Pacific  Northwest Laboratories and  is  the  subject of a  draft report (Wo79).
 Appendix  G  contains a  more  complete  discussion  and  listing  of  the  data.
 Since  runoff  samples  were unavailable,  the sampling program emphasized  the
 collection  of  soil  samples  in  well-defined  runoff  gullies originating  at
 surface   stockpiles  of  minerals.   Where  the  drainage  systems  intersected
 flowing  water, upstream  and  downstream  samples  were collected. Most of  the
 samples  consisted of  the top five centimeters of  soil  in the bottom of  the
 drainage  channels and  three  core profiles.   Samples of the  source  material
 were also collected.
     Trace  element and radionuclide analyses of  runoff  from  the  Morton  Ranch
 area are  primarly based  on surface  sediments  and vertical sediment  profiles
 from the dry  stream beds, since few streams or other  forms of runoff were
 encountered.   Figure 3.4  shows  the waterways  surrounding the inactive 1601
 pit area  and the semi-active  1704 pit area.
     Three  vertical  soil  profile  samples were collected,  two  in  an  erosional
 drainage  area  from the  ore and waste pits south of  the 1601 pit  and  one  in  an
 erosional  drainage bed on the east  side  of the  waste pile  of the  1704 pit.
 The  radionuclide and chemical constituents  of these samples along with analy-
 ses  of other soil  samples are reported  in  Appendix G.   The  results  indicate
 aqueous  leaching  based  on the  radium/uranium ratios of about  12  in  rede-
 posited  material   in  the  alluvial fan  area of  the drainage, compared  to a
 corresponding  ratio  of  0.9 in the undisturbed  (sub-surface)  material in  the
 top  alluvium profile.
     Trace element data also  indicate limited transport of mine contamination
 with  respect  to  uranium, and  to a  lesser extent,  Se  and  V.   The profile
 samples containing 140  and 21 ppm U  resulted  from material   transported from
 the  adjacent  ore  piles.   The  aqueous samples  similarly showed  no unusual
 characteristics indicative of mine wastes.
     An  aqueous sample  and   the  soil  profiles collected near the  1704 pit
 similarly showed no  evidence  of mine-related pollution  or leaching  of uran-
 ium. This observation  is  based on the water and  particulate analyses and the
 radionuclide  analyses.    These  samples constitute  a  worst   case,  since the
 sediment  samples were collected in the redeposited material of the waste pile
drainage  and should  show  greater  levels of  pollutants  there than would fin-

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                                                                                3-37
            = -\ I Waste
        ^1704.  I  Area
          -Pit V
                                                 LEGEND
                                                  • W  Water
                                                  • S Soil
                                                    G Stream sediment
                                                    P - 76 cm soil profile
                                                 0 200
1000
Figure 3 4 Location of mines, ore and waste storage areas and monitoring stations at the
          Morton Ranch mine, South1; Powder River Basin, Wyoming

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                                                                       3-38
 ally  reach  the South  Fork  Creek bed.
      Pollutant  releases from the Morton  Ranch,  Wyoming uranium mining  oper-
 ations  were not  observable in water  drainages  of the surrounding area.   The
 only  significant movement  of  mine-related wastes  was the  transport  of  the
 stockpiled  ore in erosional drainage  areas on and immediately adjacent to  the
 waste pile  of   the  1601  pit.   Long-distance transport  of  these pollutants
 (primarily  uranium) into the South Fork of Box Creek was not observable.   The
 strongest  evidence that mine  wastes are  a  source  of local soil  and  water
 contamination  is  the radiochemical   data, and  uranium in  particular.  Pol-
 lutant  transport is  almost entirely confined  to the  immediate  area  of  the
 mines,  although  there  has been  some dispersal  via  water  in  the ephemeral
 streams.  There  is  considerable  disequilibrium  between  radium  and  uranium
 which  may  indicate leaching and  remobilization  of  uranium.   Tfie possibility
 of natural  disequilibrium  in the ore  body should not be overlooked.

 3.2.3.2.3 Texas
      A  very comprehensive  field  and  literature survey of elements associated
 with  uranium  deposits in south Texas (He79)  revealed  high  to very high con-
 centrations of molybdenum, arsenic,  and selenium in  areas  of shallow  miner-
 alization;  drainages  adjacent  to older,  abandoned mines;  and in some re-
 claimed  areas.   Areas  of  shallow  mineralization  have  concentrations  of
 several tens  of  ppm molybdenum and arsenic and  up  to 14 ppm selenium.  Near
 surface material exposed  by mining  may have several  hundred ppm molybdenum
 and arsenic.  Waterborne transport of suspended or dissolved solids away from
 open  pit mines resulted from mine water discharge and  (or) surface runoff and
 erosion of  abandoned  spoil  piles.   Molybdenum  from  the  mining  areas  could
 potentially aggravate natural  soil  problems  leading to molybdenosis (Kab79),
 Additional   careful  study is suggested,  particularly of areas  receiving  mine
 drainage as pumped water or overland flow.
     Lakes  or ponds associated  with  10  mine  locations in  Karnes and Live Oak
counties  contained water  unsuitable for drinking  without  prior  treatment
 (It75). Generally,  mineralization  was also excessive  and rendered  the water
unfit for irrigation.   Air and terrestrial sampling revealed no  health  haz-
ards   from mining wastes and mined lands,  but insects  and other bottom fauna
in the lakes concentrated radium-226 400 to 800 times the  water concentration
based on dry weight of the  organisms.

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                                                                       3-39

 3.2.3.2.4 New Mexico
      The principal  investigations  of the influence of uranium mining on water
 quality  includes EPA  and contracted  (Wo79)  work  by the U.S.  Environmental
 Protection Agency,  the Department  of  Interior (Ku79), and ongoing  studies by
 the State  of New Mexico  (J.  Dudley,  oral  communication, 1979).   Because of
 the co-location of  mining  and  milling  facilities,  it is difficult to identify
 impacts from one versus  the  other.
      Survey of  groundwater  and surface  water quality in close  proximity to
 the  Jackpile-Paguate,  Ambrosia Lake,  and  Churchrock mining  areas  (EPA75)
 revealed extensive  discharges of mine  water  to the  ambient  environment,  use
 of unlined ponds for settling  suspended  solids from mine dewatering,  use of
 contaminated mine water  as  a potable  supply  (one facility), and  failure of
 all  facilities  discharging  to  streams to have  a  valid  NPDES  permit.   The
 volume  of mine discharge,  particularly  in the  Churchrock  area and from  a mine
 near Mount  Taylor,  led  to  use  of  the  water  for  irrigation and  stock.   In
 other areas of Ambrosia Lake  and near  Churchrock,  infiltration  of  mine water
 mixed with  seepage  from mill tailings  ponds is  causing  local  contamination of
 shallow, potable aquifers,  but  the  problem  is not considered serious  and
 ongoing  studies are underway.  The  State of New Mexico has  installed a moni-
 toring  well network to determine temporal  and spatial trends in groundwater
 quality.  The  U.S.   Geological  Survey,  in  particular, is monitoring surface
 flows and water quality  in the Ambrosia Lake and Churchrock  areas.
      As  part of the San Juan Basin  Regional Uranium Study,  the  Department of
 Interior (DOI79)  assisted  by the  U.S. Geological  Survey  (Ku79) examined
 selected water quality  impacts  from mining and milling  and concluded that
 much  of the mine effluent is  suitable  for  irrigation, stock, and  industrial
 use.   Locally, it  supports  aquatic life and  wildlife.   Additional  data   on
 stream  sediments are  needed  to  evaluate  the  impact on  water  resources   of
 erosion  of  waste  rock  from mines   and  mill  tailings.   It  is  preliminarily
 suggested  (Ku79) that such erosion may be difficult  to  detect at distances  of
 more  than  a  few miles  from  the  source  because  of the  large  amount   of
 (natural)  regional  soil  erosion.   The results  of  the study are presently  in
 draft form  and  may therefore be revised.
     As  part of  the present study  on uranium  mining wastes, two New Mexico
areas containing  inactive  mines  were surveyed  in the Spring  of  1979.  Stable
and  radioactive trace  elements were monitored  in surface  runoff from sub-ore

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                                                                       3-40

 and  overburden piles in Ambrosia  Lake  and in the  nearby  Poison  Canyon  area.
 EPA  staff selected the basic  study  areas  and assisted in  sample collection.
 The  bulk of the  sampling,  analytical,  and interpretation phases was  done by
 Battelle,  Pacific  Northwest  Laboratories  (Wo79).   Appendix  G contains  the
 data and discussion.  As in  the case of the  Wyoming study  area,  the  sampling
 program  emphasized stream sediment sampling, cores, and shallow  (5 cm thick)
 grab samples at  the  land surface.   Samples  of  the source  material were  also
 collected.   Figures  3.5  and  3.6  show  the location  of the  study areas  and
 sampling  stations  in New Mexico.   Samples of  the  source material were  col-
 lected  at  one of  the  two  New Mexico drainage systems  investigated.    One
 system  in Poison  Canyon,  New Mexico,  was adjacent to several smsll   surface
 operations  as  well  as an underground mine site.   For  this system,,, no single
 source could bt defined for  the runoff  constituents.
      The  Poison  Canyon  mine drainage system  is  a  dry  creek bed.  The course
 of  this  creek passes an abandoned  underground  mine  site  from which it  can
 receive  runoff water.   It  then  passes  through  a dirt  roadway and follows a
 course adjacent   to  some  small open  pit mines.   After  a  distance of  several
 hundred  kilometers, it joins a second branch  drainage that originates  next to
 a  waste  pile  from  one  of the open pit mines.   Samples were  collected along
 this  waterway  starting  with a background sample upstream  of  the underground
 mine about  200 m from  the  road.  The  first  downstream sample was collected
 about 130 m downstream  from  the  roadway.   This was  upstream of the runoff
 source originating in  the  open  pit mine.   The remaining  samples were  col-
 lected along the  drainage  way {Fig. 3.5), below  contamination sources  from
 the  open pit operations.
      A second site, the San Mateo Mine  and environs, is located in the south-
 east  portion of the Ambrosia Lake mining district.   Large mine waste piles, a
 heap  leaching  operation,  and a mine drainage pond are prominent at the site,
 which drains northward to San Mateo Creek.
      Soil composites  were collected at the  waste  pile and heap  leach pile.
 These represent  the source  term  for possible contamination of the watershed.
 The drainage samples were collected following one channel  down the waste  pile
 face  to  the  intersection with  San  Mateo  Creek,   which  was  followed for a
distance  of 500 to 600 m from the site.   Additional  samples were collected in
the gullies  leading from the heap leach  area  and one of the off-site gullies.
The  latter  represents blank  soil  upstream of the  drainage water.  Sampling
 sites are noted  in Fig.  3.6.  No significant contamination  from the under-

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                                             MESA MONTANOSA
                               Background
                                        Inactive
                                     Surface  Mines
LEGEND
B  Active Underground Mine
  a  Inactive Underground Mine
 ^'--' Surface Mine
>»..>•» Ephemeral Stream Course
  ®  Well Water Sample
     Soil Sample
                                                                         N.M.  Highway 53
                                                      Kilometer
 Figure 3.5 Location of study areas, sampling stations and uranium mines, Poison Canyon area, McKmley County,
 New Mexico

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                                                                            3-42
                                                                 Highway
0  100
400
600
                           Meters
  Figure 3.6 Sample locations for radionuclides and select trace metals in sediments,
            San Mateo mine, New Mexico.

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                                                                       3-43

 ground  site was detected.   The  Ra-226  content of the  soil  was  about two times
 the  background level at the  furthest  downstream site.  This  sample  was col-
 lected  about 130 m  from  the apparent source.
      In  summary,  at the  New Mexico  inactive mine drainages the most prominent
 indicator of runoff from above-ground  mineral  storage  is  radium-226 in  stream
 bed  sediments.  Concentrations  in  the  source material  are almost  two  orders
 of  magnitude  higher than   those  measured  in  the  background   soils.  Elements
 such  as  uranium  and selenium  also have as  large a concentration  gradient,
 with  concentrations .decreasing  downstream.  At  Poison  Canyon, the  radium-226
 concentration  diminished to  two  times  background  in  a distance of  approxi-
 mately  100 m, while at  the San Mateo  site the  distance was about  400  to  500
 m.  This  may reflect either a more  rapid transport  by  faster flowing  water at
 the  San Mateo site  or,  more  likely, the larger  source  term there relative to
 background.   At  the  San Mateo  mine,  radiuni-226 concentrations in  water  and
 sediments are significantly elevated  downstream relative  to  upstream  of  the
 mine  drainage.

 3.2.3.3    Summary
      The  field studies conducted to date on  the impacts of uranium mining on
 water quality  are somewhat contradictory.  Although no cases  of gross,  wide-
 spread  contamination of  groundwater or  streams  can be documented for uranium
 mining,  there  are cases  of local contamination  of water and  sediments. From
 standpoints  of theory and  field  data,  there  is  need for cautious optimism in
 the  use  of local  soil  and  water resources  as sinks for  waste  discharge.
 Although  numerous studies  indicate that considerable  reliance can  be  placed
 on the various  physical  and chemical processes to protect  natural waters from
 contamination,  investigations  generally warn  against using such  studies  to
 predict what may  happen  in  other  situations (Ru76;  NRC79b; Ku79; Fu77;  Am78).
 Laboratory  results  are  highly  dependent on  the chemical   properties  of  the
 fluid matrix  and the physical and  chemical properties of  the  particular soil
 studied.   Results of field studies are site and time specific  and  have  often
 suffered  from  inconsistent and  undefined  sampling and  sample preservation
 techniques  and   questionable  analytical  measurements  (Ku79; Ha78;   Si77).
      Our  analyses reveal that  there  have been  local  water quality problems
from  mine  water and wastes.  Although widespread hazards  have  not  been  iden-
tified,  this may  be false security  insofar as the present status of knowledge
concerning  trace element   mobility in  aqueous  settings  representative   of

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                                                                       3-44
 uranium  mining areas  is  rather  unclear  from both theoretical and  real-data
 standpoints.   Most  often, effects of mining  are  interspersed  with and masked
 by  impacts  from uranium milling.  This complicates or  renders  impossible  any
 meaningful  interpretation of  the  mining-related data.   Despite  the attempt to
 sort  out some  of the  information  on trace  element  mobility,  there  is  in-
 sufficient  understanding at  this  time   to  dismiss  or  otherwise  reduce  the
 significance  of  trace  element  contributions  (from  mining  activities)   to
 surface  streams and, to a lesser  extent,  to groundwater.
     We  conclude that  there  is considerable  information  on  the  topics   of
 trace element  chemistry,   It is  also clear that  trace  element  concentrations
 in  natural  fresh water are highly variable on both macro and micro geographic
 scales.   There is great  difficulty  in correlating  concentrations  with such
 characteristics as streamflow or  lithologic environment.  Accurate prediction
 of  the  behavior  and  cycling of  trace  elements  through  water and  sediments
 first involves  characterization of  physical   states such as particle size  and
 form  (chelate,  colloid,  complex  ion,  precipitate,  etc.), speciation»   and
 availability to plants and animals (An73).  Andelinan concludes  "...that there
 can be  large  differences  in trace element concentrations [in water], on both
 a macro  and micro geographic scale, and  that such variations  often occur  in
 an unsystematic and nonpredictable fashion."
     We  recommend additional   studies of spatial  and  temporal  variations,
 sources  and sinks  of  trace elements, chemical interactions within the hydro-
 geologic  system,  interactions   between   surface  and  groundwater  systems,
 effects  on  aquatic  biota, and  effects on water use (human consumption, stock
 watering, irrigation).  Periodic  monitoring  in certain areas would  allow for
 the detection  of  the  long-term trends of potential changes that would accom-
 pany anticipated  increases in  future  mining  activity — during a  period  of
 increased competition for scarce water resources.

 3.3  Surface Mining

 3.3.1   Solid Pastes
     Surface mining consists of removing  materials, separating  them  into ore,
 sub-ore,  and  overburden,  and  storing  them  in separate piles  on  the  surface
near the mine  for  various  periods  of   time  (Section  1.3.2).  The  various
storage   piles  are managed differently,  vary in  size  and  level  of  contami-
nants,  and exist  for  varying  periods of   time.  All are potential  sources  of

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                                                                       3-45
 contamination  to the environment  via  dusts  suspended and transported  by  the
 wind,  precipitation  runoff,  and  Rn-222 emanation  (Fig.  3.7).
 3.3.1.1    Overburden Piles
     Surface mining  produces spoils  at a rate  of  millions  to  tens-of-millions
 of  tons per year.   Unless  this  material is used to backfill the pit,  large
 surface  areas  — 40 hectares to over  400 hectares  —  are covered to  depths
 varying  from a  few  meters  to over  100 meters (Ka75» NRC77a, NRC77b»  DQA78,
 Pe79).
     Most  of  the mines begun  since  the early  to  mid  1970's use  overburden  to
 backfill  mined-out   areas of the  pit  (Ka75).   Since older mines usually did
 not, erosion of  their storage  piles  by water and  wind may  present an environ-
 mental  problem  (Ka?5).   In  addition,  the  large  amounts  of  overburden that
 past and present mines have  used  for  road and dike  construction and backfill
 also may present an  environmental  problem,
     The annual  average ore production  of the 63 surface mines operating  in
 the  United States in 1978  was  1.2  x  105  MT  (Section  1.3.1).   Assuming  an
 overburden  to  ore   ratio of 50:1 (Section  1,3,2),  the average  annual pro-
duction of overburden was about 6,0  x  10  MT per mine.  A  recent study of the
eight  large mines that accounted for 68 percent  of the total  1977  United
States  ILQg production from surface  mines  recommends  the following  average
production parameters (N179):

     1.   ore production = 5.1 x 10  MT/yr
     2.   average ore grade = 0.11 percent ILO,,
     3,   overburden:ore ratio = 77
     4.   overburden   production = 4.0  x 10  MT/yr
     5,   mining days/yr = 330 d/yr

     Surface areas of hypothetical overburden  piles were  computed  using the
above 63-mine and 8-mine overburden production rates and the following  assump-
tions:        -  _

                                        3
     1.   an average  density of 2.0 MT/m  -  reported values vary between
          1.6 and 2.7 (Ro78, DOA78, NRC78a,  Ni79)
     2,   the dumps are on level  terrain
     3.   a rectangular waste dump with the  length twice the  width,  and
          sides that  slope at 45° angles (Fig.  3.8a)

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     £^i'Q$J^'^Vci'»""*o'
Wt^'j^^O.^*'-'^ '°%$y&$ff''SSrfv






jf«^^o'^^?q^?^^'£?fe>'^
            Figure 3 ?  Potential sources of environmental contamination from active open pit uranium mines.

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                                                                       3-47
      4.    a  waste  dump  in  the  shape  of a  truncated  right-circular cone with
           45°  angled sides {Fig.  3.8b)
      5.    a  bulking  factor of  25% or 1,25 {Burn's,  E.»  Navajo  Engineering
           and  Construction Authority,  Shiproek,  MM,  2/80  personal  communi-
           cation)
      Table  3.11 li-sts the surface areas of  the  hypothetical overburden  piles
 in  the  following  three cases;

      Case 1  -   one year  production with no backfilling

      Case 2  -   backfilling concurrent with mining - assumes 7 pits
                opened in a 17-year mine life with overburden from each
                successively mined pit ysed to backfill a previously com-
                pleted pit, resulting in an equivalent of one pit of over-
                burden {2.4-yr production) stored on the surface (Ni79)

      Case 3  -   no backfilling during the 17-year mine life

      The  quantities  of  dust and  Rn-222 that  become airborne  are directly
 proportional to the surface areas of waste piles.  Table 3.11 shows the  large
 variations  possible  between  surface areas  of  waste piles  at some  active
 minis.  Waste piles also  cover  various areas  of terrain.   However,  for the
 same  volumes, there are no significant differences in surface area or area of
 terrain covered for the two configurations of waste piles used in this study.
 Case  2  approximates  recently activated  mines, and Case  3  approximates older
mines.
     The type of  rock in overburden spoil piles  depends  on the locations of
 the ore zones,-. Common rock types of New Mexico, Wyoming, and Texas mines in-
clude sandstone,  claystone,  siltstone,  shale, and limestone,  and  unconsoli-
dated silt,  gravel, and  sand (Co78»  Pe79, Wy77»  R178).   In Texas, there are
a?so  lignite beds,   tuffaceous  silts,   and  some  nearly  pure volcanic  ash

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                                                                                    3-48

   a) A rectangular pile with length twice the width and 45 degree sloping sides
             b) A frustum of a regular cone with 45 degree sloping sides
Figure 3 8 Storage pile configurations assumed at surface and underground mines.

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                                                                       3-49

 (Ka75).   Coal  veins are often present in Wyoming and New Mexico (Wy77, R178).
 However,  the  most  abundant material  in  waste rock  dumps  will  probably  be
 clastic  sedimentary rocks: sandstone, siltstone, and shale.
      There  is  great  variation  in  the particle  size  of  material  in  waste
 piles,  and  this  variation  is  important.   Large particles  { >30vjjn)*,  because
 they  usually  settle within a few hundred  feet of their origin,  do  not con-
 tribute  to the airborne dust concentration (EPA77b).  The potential for human
 respiration of the wind  suspended  dusts  is  also strongly  influenced  by the
 mean particle  diameter (ICRP66).
      Overburden rock  is as  large  as available equipment can load  and haul  to
 the storage area.   Rocks  too  large to handle with  available  equipment are
 broken into manageable sizes by  small,  explosive charges.  Hence,  rock parti-
 cles will  vary from  less  than  a  ym to a  meter or more in  diameter.   Since
 weathering eventually breaks down the  larger stones,  the fraction of smaller
 particles increases over time.
      Particle  size distributions of  material  in waste rock  piles  at  uranium
 mines  have  not been  determined.    It  is  likely  that  this  material   has  a
 greater-  fraction  of larger  particles than that associated with crushed  uran-
 ium mill tailings.  Table  3.12  shows an example of the  particle size  distri-
 bution in the  latter  and  the mean particle size distribution from a  study  of
 shale  overburden   removed  from a  surface  mine  in  Pennsylvania (Ro78).  Al-
 though  the  distribution  fractions  differ,  a gross  comparison  can  be  made
 between  the particle  size  of mill  tailings  and overburden waste.  About  28
 percent  of the tailings were  less  than 50 urn  in  diameter,  and only  about  12
 percent  of  the particles  in the overburden pile  had  similarly   small  dia-
 meters.   Because  only  particles  smaller  than 30  ym  are  likely to  remain
 suspended  by the  wind for  any  significant distance  (EPA77b),  probably less
 than  10  percent   of  the overburden  is a  potential  source  of  environmental
 contamination  via  wind erosion.
     Table 3.13 shows the natural radionuclide concentrations in  common rock
 types  in  the  United States.  In sedimentary  rocks,  which  are common in the
 major  uranium  mining  regions, the U-238 concentrations  vary from  less  than  1
 pprn**  to  about 4  ppm.  Natural radioactivity usually is somewhat higher  in
 the  western states,  and the uranium content  in  overburden  prior to mining
*vm = micrometer =  10   meters.
**ppm = parts-per-raillion = 10~6 grams  per  gram  of  rock.

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                                                                 3-50
Table 3.11   Estimated surface areas associated with overburden piles
Management^3'
Pile
Height,
Overburden Surface Area
m Volume^ '» m of Pile, m
Terrain
Covered, Hectares
Rectangular Pile^c'

Case 1
Case 2
Case 2
Case 3

Case 1
Case 2
Case 2
Case 3
Truncated Con

Case 1
Case 2
Case 2
Case 3

Case 1
Case 2 --
Case 2
Case 3
.
65
65
30
65

65
65
30
65
,

65
65
30
65

65
65
30
65
Average Large Mine^ '
2.5 x 107
6.0 x 107
6.0 y W7
4.2 x 108
fe)
Average Minev '
3.8 x 106
9.0 x 106
9.0 x 106
6.4 x 107

Average Large Mine^ '
2.5 x 107
6.0 x 107
6.0 x, 107
4.2 x 108
Average Mine^
3.8 x 106
9.0 x 106
9.0 x 106
6.4 x 107

5.2 x 105
1.1 x 106
2.2 x 106
7.1 x 106

1.0 x 105
2.2 x 105
3.6 x 105
1.2 x 106


5.2 x 105
1.1 x 106
2.1 x 106
7.1 x 106

1.1 x 105
2.2 x 105
3.5 x 105
1.2 x 106

48
106
209
682

10
20
34
113


46
104
208
683

9
18
33
110

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                                                                       3-51

                            Table  3.11  (continued)
 ^Management:

           Case  1  -   one year  production  with  no  backfilling

           Case  2  -   backfilling concurrent  with  mining - assumes 7  pits
                     opened  In a 17-year  mine  life  and equivalent of one-
                     pit overburden  (2.4  year  production) remains on surface

           Case  3  -   no backfilling  during 17-year  mine life

 '  ^Volume  s  production (MT/yr) x  production years  x bulking factor  (1.25)
   * by density (2.0 MT/m3),
 ^length  of  pile is twice  the width and the  sides slope at a 45° angle
   (Fig. 3,8a).
 '  ^Overburden production *  4.0 x  10 MT/yr.
 f P\
 v  'Average 1978 overburden  production of all  63  surface mines, assuming an
   overburden:ore ratio of  50/1,  6.0 x 10 MT/yr  per mine.
 ^  'A frustum of a regular cone with 45°  sloping  sides (Frig. 3.8fa).
is about 4 ppm (N179).  However, during mining, some low-grade ore mixes with
the overburden and  may Increase the concentration  of  the pile to as high as
20  ppm U30g  (N179).   This is equivalent  to  12.6  disintegrations  per minute
(dpm)  per  gram of  overburden.   The progeny  of the uranium will  contribute
additional  radioactivity.   Although  there are local   disequillbria between
U-238  and  its principal  daughters,  Th-230 and Ra-226,  in  ore-bearing rock,
secular equilibrium will  be assumed  (Wo79).  Small quantities  of  Th-232 and
progeny will  provide  additional  radioactivity.  There  is  no apparent rela-
tionship between the Th-232 and U-238 decay chains,  Th-232 concentrations in
ores and host  rock  range from less than a pCi/g to a few pCi/g regardless of
the U-238 concentration (Wo79).

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                                                                       3-52
          Table 3.12   Particle size distributions  of mill  tailings
                       and mine overburden
Mill 1

Particle Size,
urn
250
125-250
53-125
44-53
20-44
7-20
1.4-7
< 1.4
railings{aj

Weight
Percent
60.3
7.5
4.2
3.8
7.8
7.2
9.1
0.0

ir\
Conc.(c)
Avg. Cone.
0.15
0.03
0.03
0.03
0,75
1.5
4.6

Overburden^ '

Particle Size, Weight
Mm Percent
>2000 75

50-2000 13

2-50 8

<2 4

     (a)
     (b)
     (c).
Source:  Sc79.
Source:  Ro78.
        The concentration of radionuclides in that fraction divided by the
average concentration.
          Table 3.13     Natural radfonuclide concentrations in various
                         common rock types
Rock Type
                        U-238
            ppm
pCi/g
     Source:  Qa72,
                                        Th-232
ppm
pCi/g
                                        K-40
ppm
pCi/g
Igneous
Basic
Granite- -
Sedimentary
Shale
Sandstone
Limestone

0.9
4.7

3.7
0.45
2.2

0.3
1.6

1.2
0.15
0.7

2.7
20

12
1.7
1.7

0.3
2.2

1.3
0.2
0.2

1.2
5.0

3.2
1.1
0.32

8.4
35

22
7.7
2.2

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                                                                      3-53
     Table 3.14  shows  the  results of an  extended  airborne particle sampling
program  near a  surface mine  in  New Mexico  (Ea79).   Although  the  on-site
source  of  the radioactivity measured on these  filters  is undetermined, ore
and  sub-ore  piles,  waste  rock  piles, and mining  activity all  probably con-
tribute.   The  higher   activities  reflect  a greater  contribution from ore
dusts.   From  these  air measurements, the above  assumed  average  uranium con-
centration in  overburden,  12.6  dpm/g (= 6 pCi/g),  appears reasonable.  These
data  also  indicate  that the  progeny  of U-238 through  Ra-226  are  in  near
secular  equilibrium.   The  Th-232 concentration  is about 1  pCi/g and,  as
indicated  above,  independent  of the  uranium  concentration.   Considering all
available  daca,  the  radioactive  source terms for overburden piles will  be as
follows: (1)  J-238  and progeny  = 6  pCi/g (0.0020  percent l^Ogj  (2) activity
ratio (dust:overburden)  = 2.5  (Section  3.3.1.2); and (3)  Th-232  and  progeny
=  1  pCi/g«  Figures 3.1 and 3.2 show the uranium and thorium decay  series.
          Table 3.14  Annual  average airborne radionuclide concentrations
                      in  the  vicinity of an open pit uranium mine,  pCi/g
Location
Jackpile Housing
Paguate
Bibo
Mesita
Old Laguna^
U-238
76
13
9
3
5
Th-230
80
12
7
2
2
Ra-226
70
13
5
3
3
Th-232
1.2
1.3
1.3
0.7
0.4
U-238/Th-232
63
10
7
4
13
     ^Background  location.

     Source:   Ea79.

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                                                                       3-54

      Little  information  is  available on  stable  element  concentrations  in
 overburden  rock.   Table 3.15 summarizes  the analyses  of a  few grab  samples of
 soil  and rock  from  a uranium mine  in New  Mexico and one in  Wyoming  (Wo79).
 Except  for  possibly  Se, V,  and As,  there  are no significant  concentrations of
 stable  elements  attributable  to  uranium  mining.  Considering the  typically
 high  natural  Se and  V contents of many minerals common  to  these areas  and  the
 limited number  of  analyses,  the  inference of  pollution  is indefinite.   A
 relationship  between uranium  and the  stable element concentrations does  not
 appear  to  exist.   Thus,  the stable element concentrations  in overburden from
 the model surface  mine  will  be the  average  concentrations  of  samples 6, 7,  and
 8 in  Table  3.15.   Table 3.16 lists  the average  concentration's.

 3.3.1.2  Ore Stockpiles
      Ore  is often stockpiled  at the mine as well  as the mill.  Although  ore
 stockpiles  are much smaller  than   the  overburden waste  piles,  the  concen-
 trations  of  most radioactive  contaminants are  much greater in  ore-bearing
 rock  than  in overburden.   In  addition,  ore is  stockpiled  at the  mine   for
 shorter periods of time  than  waste rock.   Ore  stockpile residence times vary
 from  mine   to  mine and  range  from   a  few days  to  a  few months.   The recent
 study of 8 large  surface  mines  cited 41  days as an  average ore stockpile
 residence time (Ni79).   We  will use this  value to estimate  the average area
 of ore  stockpiles.
      The average  of  the  63  operating  surface mines produced 1.2  x 10  MT  of
 ore during  1978.   Assuming  330 working days  per  year and a 41-day ore stock-
 pile  residence time, a 1.5  x  10  MT ore stockpile  would exist at the average
 mine.   In comparison, the recent Battelle  study  reported that the average  of
 eight large surface  mines produced   1550 MT of  ore  per day, which  would yield
 a  6.3 x 10  MT ore  storage pile,   assuming  the  same residence time  (N179),
 The ore piles  vary  1n height  at  different  mines  and  different  times.   One
 study reports a maximum  pile  height of  9.2 m  (30  ft) (N179), and at another
 site  the maximum  and equilibrium ore  pile  heights  are  estimated  to be 6.7 m
 and  3.1 m,  respectively  (NRC78a).  Using  these  parameters  and  a  bulking
 factor  of  1.25 (Burris,  E.,  Navajo  Engineering  and  Construction  Authority,
 Shiprock, NM,  2/80,  personal communciation), the pile  surface and  pad areas
were  computed for the  two  production  rates and  two pile  heights,  9.2 m  and

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Table 3.15  Uranium and stable element concentrations measured  in  rock and  soil  samples  from
            two uranium mines

Concentration, ug/g
Sample '•
Vlygming
1. Top Soil Piles
2. Sub-ore
3. Ore
New Mexico
4. Background Soil
5. Background Soil
6. Waste Pile
7. Waste Pile
8. Sub-ore + waste
9. Ore
As

3.2
<1.8
5.4
4.1
2.3
7.8
14
4.1
6.0
Ba

700
6800
800
450
440
540
280
45
64
Cu

13
9
9
12
9
11
21
22
27
Cr

46
<36
<27
<23
<20
<28
<43
<51
<48
Fe(a)

1.3
1.2
1.1
0.9
0.8
0.8
0.7
0.3
0.4
Hg

<4
10
<7
<4
<4
<5
<8
<6
<6
K(a)

2.2
2.3
2.3
1.8
1.6
1.4
0.5
0.1
0.2
Mn

190
140
180
200
190
260
750
446
673
Mo

2.9
<2.2
< 2.9
5.5
4.9
2.5
<2.8
<1.8
4.8
Pb Se

23 <1
22 2.1
16 28
12 <1
13 <1
10 <1
31 3.1
25 < 1.4
31 1.5
Sr

89
128
94
72
50
99
178
179
323
V

60
<100
200
<50
<50
<70
180
<55
<55
Zn

37
25
25
22
19
23
23
13
14
U

6
61
370
<5
<5
8
189
57
—
     Source: Wo79.
            s are percent.
                                                                                                             OJ
                                                                                                             I
                                                                                                             tn
                                                                                                             en

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                                                                       3-56
      Table  3.16   Concentration  of  radionuclides  (pCi/g)  and  stable  elements
                  (ijg/9)  in  overburden  rock  from  the model  surface mines
Element
Arsenic
Barium
Hopper
Jhromium
lron(a5
Hercury
Potassiunr '
Manganese
Molybdenum
Lead
Concentration
9
290
18
<51
0.6
<8
0.7
485
2.5
22
Element
Selenium
Strontium
Vanadium
Zinc
U-238
Th-230
Ra-226
Pb-210
Po-210
Th-232
Concentration
2
150
100
20
6
6
6
6
6
1
        Units are percent.
3.1 m, assuming the same geometric configurations as for the overburden piles
(Fig. 3.8).   Table  3.17 gives the results.  The computed surface areas of an
average  ore  stockpile  vary  with volume of  ore stored  and  pile height,  but
they are relatively independent of the pile shape.
     Uranium  deposits  exist  in  sedimentary,  metamorphic,  and  igneous  for-
mations.   Sedimentary formations, primarily  sandstone,  siltstone,  mudstone,
and  limestone generally  host stratiform  ore  deposits  often  accompanied  by
carbonaceous  material.  Vein-type  deposits  usually  occur  in  fractures  of
igneous  and  metamorphic formations.   In  the  Rocky Mountain  mining regions,
about 98  percent  of_ the recovered ILOg comes from  sandstone and related-type
rock  (St78).   Sedimentary  formations,  principally  sandstone,  have  been  the
predominant host for uranium in South Texas (Ka75).

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                                                                      3-57
     Table 3.17  Estimated average areas of ore pile surface and pad
Pile
Configuration^3'
Rectangular
Truncated Cone
Rectangular
Truncated Cone
Rectangular
Truncated Cone
Rectangular
Truncated Cone
Pile
Height, m
Average
9.2
9.2
3.1
3.1
Average
9.2
9.2
3.1
3.1
Surface Area
of Pile, m2
Large Mine^ '
6,300
6,200
14,000
13,700
Mine(c)
1,860
2,000
3,660
3,590
Ore Pad
Area , m
5,700
5,300
13,500
13,200
1,820
1,580
3,420
3,340
     U)
        See Figure 3.8.
     'b'Volume of ore = 6.3 x 10  MT (41 day production) x 1.25  (bulking  factor)
* 2.0 MT/m3 = 3.9 x 104 m3.
               of ore = 1.5 x 10  MT {41 day production) x 1.25  (bulking  factor)
•» 2.0 MT/m3 = 9.4 x 103m3.

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                                                                        3-58

       The DOE does  not expect the mineralogical  characteristics of uranium ore
  to  change appreciably in  the  future,  since the known  reserves  are  mainly in
  sandstone or a related  host (DOE79).   This fact  is apparent from the data in
  Table 3.18,  which  gives  the  distribution  of ore reserves in the  United States
  by  type  of  host  rock.   More than 97  percent  of  the uranium  reserves  are in
  sedimentary   formations,  primarily  sandstone.   Hence,  it  is  reasonable  to
  assume that  ore stockpiles in  the future  will  continue  to consist mainly  of a
  friable (easily crumbled)  sandstone  rock.
       No data are  presently available  on  the  particle  size distribution  of
  material  in  ore stockpiles.  Thus, the particle size distribution of ore  will
  be  assumed to be  similar to  that of  overburden  rock.
       The  average  grade of ore mined in  1978 was about  0.14 percent  U^Og,  but
  this  will decline  in  future  years  (DOE79).   The average  qrades of ore associ-
  ated  with tnr  "10  and $50 reserves  are 0.10  percent and 0.07 percent UgOg,
  respectively (DUE79).  Assuming  the average grade  of  ore mined in  the  next
  decade to be about 0.10  percent  U-jOg,  the average uranium concentration  in
  ore stockpiles  will be Z85  pCi/g  (632 dpm/g).  Although  secular  equilibrium
  in  the  uranium decay  chain  may not  totally exist in  some cases  due  to
  leaching  by  groundwater with  subsequent  redeposition,  it appears reasonable
  to  assume  that  radioactive  equilibrium   exists   in  a  general   assessment.
       As  discussed earlier, ambient Th-232 concentrations  in  the vicinity  of  a
  uranium  mine range between  1  to 2 pCi/g.   However, a  concentration of  0.01
  percent  thorium  is typical  for ore  from  some surface  mines (Mi76).   This
  concentration is equivalent  to 11 pCi Th-232/g  of ore.
       Uranium  occurs in  many ores as  a  secondary  deposition.   In a  reducing
  environment,  the  soluble uranyl  ion  converts  to  insoluble uranium oxide  and
'  deposits  preferentially on the smaller particles.   (The  total  surface area of
  a  given  mass  of smaller  particles  is  greater than for larger  particles.)
  Therefore, dusts  that consist primarily of  small   particles  have a greater
  specific  concentration  than ore  as  a  whole (Table  3.12).   The common pro-
  cedure for computing uranium concentration  in dust  is to multiply  the average
  concentration in the jjre by  2.5 (NRC77a, NRC78a).

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                                                                       3-59
      Table 3.18 Distribution of ore reserves by the type  of host

Host Type
Sedimentary^5'
Lignite Materials
Limestone
Igneous and Metamorphic
Totals
MT of
Ore (106)
1,143.2
2.2
1.3
32.7
1,179.4
MT Of
U3°8
810,000
3,000
1,200
20,400
834,600
Percent Total
Tons, ILQD
J O
97.1
0.4
0.1
2.4
100.0
      ^'Principally sandstone,  but  includes  conglomerates, shale, mudstone, etc.
      Note.—The reserves are $50 or less  per pound  ILQ0> effective January 1,
        "                                             O  O
 1979 (DOE79).
           Table 3.19  Average  stable  element  concentrations in sandstone
                       ores  of  New Mexico
Metal
Arsenic
Barium
Cadmium
Cobalt
Copper
Chromium
Iron
Mercury
Potassium
Magnesium
Concentration, pg/g^a'
86 (10-890)
920 (150-1500)
ND(b)
16 (3-150}
61 (15-300)
20 (7-70)
15,700 (3,000-70,000)
ND
25,000 (7,000-30,000)
^3, 500 (700-15,000)
Metal Concentration, yg/g^
Manganese
Molybdenum
Nickel
Lead
Ruthenium
Selenium
Strontium
Vanadium
Zinc

960 (70-3,000)
115 (3-700)
20 (7-70)
78 (3-300)
ND
110 (1-625)
130 (1.5-300)
1410 (70-7,000)
29 (10-70)

      *  'Range of concentrations given in parentheses.
      ^ND - not detected
     Note.--Ore samples are Dakota and Morrison sandstone from 25 uranium
mines (Hi69).

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                                                                       3-60

      In accord with the  above  discussion, we assume  the  following  estimated
 average radionuclide source tenns  for ore stockpiles:  (1)  U-238 and  progeny -
 285 pCi/g ore  (0.10 percent  U30g);  (2) Activity  ratio  (dustiore)  = 2.5; and
 (3) Th-232 and progeny =  10 pCi/g  ore.
      Stable elements  —  molybdenum, selenium, arsenic, manganese,  vanadium,
 copper,  zinc,  and  lead  —  often associated  with uranium  ore at  elevated
 concentrations may cause deleterious environmental  and  health  effects.   Mer-
 cury and  cadmium are  present  only  on rare occasions  (Th78).  However,  as
 discussed above,  there is  no apparent relationship between  concentration  of
 stable  elements  and  ore  grade  (Wo79).   Table  3.19  lists  measured  (Hi69)
 concentrations of stable  elements in  25  sandstone ores from  New Mexico  and
 average  concentrations  computed  from these  data.   We assume  the  average
 concentration  for the  ore from  the model  surface mine.

 3.3.1.3   Sub-ore Piles
      All  mines recover some  rock  containing  uranium ore that  at the  time  of
 mining  is uneconomic  to  mill.   The grade of  this "sub-ore"  varies with  the
 "cutoff"  level  assigned  by  the  mill.   Some  mines process  sub-ore  by heap
 leaching,  which changes the  chemical properties and constituents of the pile
 (Section  1.3.5.1).  However,  most mines  store  the sub-ore in  separate piles
 and  recover  it when  it  becomes  economically feasible.
   '   The  sizes of sub-ore dump piles vary with the  quantity  of ore mined and
 its  grade.   One study  suggests  that the  sub-ore accumulation rate equals the
 ore  production rate  (Ni79}» a  ratio  similar  to that reported  for the Sweet-
 water uranium  mining operation  (NRC77a).   Using this assumption with the ore
 production rates  given above  for the average large mine and average mine, 5.1
     5                    5
 x  10 MT/yr  and  1.2 x  10   MT/yr,  respectively, the average  sizes of sub-ore
 piles generated  at a constant  rate during the  17-year active  life of a mine
 were  based  on  an 8.5 year accumulation and a bulking factor of 1.25.  Figure
 3.8  shows  the  shapes of the  piles assumed,  and Table  3.20 gives the results
 for  piles"30 m high.  The surface areas of the two pile configurations differ
 very 1 ittle.
     The  mineralogical  characteristics  of ore  and  sub-ore  are  very  similar.
Thus, the distribution  in Table  3.18 will  apply  to sub-ore.  This  study
considers  the  particle size  distribution of  sub-ore  the  same  as  for over-
burden and ore.

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                                                                       3-61

      In the early mining  years,  the ore cutoff  grade  was  usually about 0.15
 percent U-,Ofl.   However, this has  continually decreased  until  today the cutoff
 ore grade is about 0.03 percent UgQg (Ni79» NRC77a).  Hence  the ore content of
 these piles will  be  less  than 0.03 percent U^Oo, and the average content has
 been estimated to be one-half the cutoff grade, or 0.015 percent U0Q0 (Ni79),
                                                                   J O
 which is equivalent  to  43 pCi U-238/g  (95  dpm/g).   Also,  the uranium in the
 sub-ore, as in ore,  Is assumed to be in secular equilibrium with its progeny.
 Because the occurrence  of uranium in sub-ore  is  the same  as in ore  and  the
 mineralogies are  similar, the uranium  in  sub-ore should be  concentrated  on
 small particles by the same factor as in ore,  2.5.
      The Th-232  concentration in  sub-ore  is  between  the  ambient  level  and
 that in the associated ore, 1  pCi/g to 11 pCi/g.   For lack  of measured Th-232
 concentrations, we  assume that less  than  2 pCi/g of Th-232  will  be  present
 (Table 3.14).   The radiological  significance  of  an error in   this  assumption
 will be small.
      From  the  above  discussion,  we assume the  following  estimated  average
 radionuclide source  terms  for sub-ore  piles:  U-238 and progeny = 40  pCi/9
 (0.015 percent  U~0g);  activity ratio  (dust:sub-ore) = 2.5;  and Th-232  and
 progeny = 2 pCi/g,   Figures 3.1 and 3,2  show the  uranium and  thorium progeny.
      Table  3.20  Estimated average surface  areas  of sub-ore piles during
                  the  17-year active mining  period

 Pile                          Surface Area                       Terrain
 Configuration^               of  Pile, m                   Covered, Hectares
Rectangular
Truncated Cone
Average Large Mine*1 '
1.2 x 105
1.2 x 105
11
11
                             Average Mine
                                      4
Rectangular                   3.5 x 10                            3.2
Truncated Cone  "              3.6 x IO4                           3.0

     (a)See Fig. 3.8.
               of sub-ore = 8.5 yr x 5.1 x iO5 MT/yr x 1.25 * 2.0 MT/m3 =2.7
x IO6 m3.
     '^Volume of sub-ore - 8.5 yr x 1.2 x IO5 MT/yr x 1.25 -t 2.0 MT/m3 = 6.4
x 105m3.

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                                                                       3-62

      Stable  elements  observed  in  ore will  also  be  present in  sub-ore.  Because
 stable  element  concentrations specific  to  sub-ore are  unavailable and  are
 unrelated  to ore grade, concentrations  in the  sub-ore from  the model  surface
 mine  will  be assumed  equal  to  those in  the ore  (Table  3.19).

 3.3.1.4    Reclamation of Overburden Piles
      Reclamation  is usually done  only  for overburden  piles.   Ore  stockpiles
 are continually being  disturbed  and their  residence   time  is short.   Also,
 sub-ore  piles generally are not  stabilized  in  anticipation of recovering  the
 uranium  at  a  later time.   Hence,  only overburden  and waste  rock  piles  are
 considered  for stabilization  and reclamation.   Section  1.3.Z gives a  brief
 description  of  these  practices.
      Backfilling  mined  out areas  of the pit  is  necessary  for an adequate
 reclamation   program.   Because  of  the  swelling  of earthern  nieterial  once
 mined,  sufficient  material  should be available  to completely  fill  the  pit
 when  mining  is  completed.   However, even  though  backfilling is  generally
 being performed  at most recently  active mine sites, sufficient overburden  is
 often not replaced  to  eliminate the  pit.
      Improperly  stabilized  spoil  piles  may  become sources of  contaminants  to
 the  environment.   The  wind can  suspend  and transport small-sized  particles
 containing  elevated  levels  of  contaminants.   Radon-222,  produced  by  the
 radioactive  decay of Ra-226 contained in the rocks,  can emanate  from the pile
 surfaces.   Precipitation  runoff from the  piles  can  carry particulate matter
 and  dissolved  contaminants  into 'the  natural   surface  drainage  system   if
 rainfall  exceeds  the  infiltration  and  holding capacity of  the  pile.   The
 general   procedure  for reducing wind and water  erosion  is to  grade the piles
 to  conform  to the  natural  terrain, cover the area  with  a  layer of topsoil,
 and seed it with a native grass.
     These  spoils  consist  of  unweathered  and  unconsolidated  rock,  coarse
 gravels, and  sands  and allied materials isolated  from  the  natural processes
 that  occur-on surface soils.  Consequently,  spoils  have  poor textural  prop-
 erties  and   low  water-holding  capacities.   Having  no established  flora   to
 aerate the  surface and  make nutrients  available, spoils are  barren of  nut-
 rients  required  for  plant  growth.   Hence,  to  sustain  vegetation  on  these
piles may be  difficult because of  poor  soil quality and the arid conditions

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                                                                       3-63

 in the principal mining  regions.   Therefore, all  plant growth depends on the
 topsoil  cover,  which is  generally  less than  30  cm  thick  (Re76).   This  is
 often inadequate  to store  sufficient  water and  nutrients  to  sustain  plant
 growth during extended  dry periods.   Soil  irrigation and fertilization may be
 required  for several years until  plants can sustain  themselves.
      Proper grading  of  the spoil  piles,  with  water  management and  conser-
 vation, can help reclamation.   The piles should have less than a 3:1  slope  to
 reduce surface water runoff and erosion (St78). Forming catchment  basins and
 terraces  to  hold  water  on  the   spoils  and reduce water  erosion will  also
 increase  the  amount of  runoff  available  to  the plants.   It  also has  been
 determined  that  vegetation on north-facing slopes requires  about half  the
 applied water of that on  south-facing  slopes  (Re76).  Water  requirements  of
 vegetation  on horizontal   surfaces and  east and west slopes are  about inter-
 mediate between  those of  the north and  south  slopes.   Hence, spoil  piles  with
 long,  north  slopes  will  conserve water and reduce the  irrigation required.
 Locating  piles on  leeward slopes and  away  from  natural drainage will  also
 reduce wind and  water erosion.
      The  reestablishment  of native grasses  and shrubs is essential for  con-
 trolling  wind  and  water  erosion and  providing  wildlife  habitat.   Wyoming
 requires  a  pre-mining vegetation  inventory  for use  in  evaluating post-mining
 reclamation  (Wy76).   Similar  statutes  governing  mine  reclamation  are  in
 effect in  other  states  (Section 1.4).   The  Soil  Conservation Service has
 recommended seed  mixtures that  are  best  suited  to climatic  and  soil  con-
 ditions in  different areas of  the West (St78).  Newly seeded areas are  usu-
 ally  protected from  grazing  by fencing for  at least  two growing seasons  to
 allow  the plants  to  become  established.
     Abandoned  pits fill  with water and  form small  lakes that  livestock and
 wildlife  can use  for drinking water,  if the water  is uncontaminated.  But,
 unless properly managed,  final  pits may be  hazards  to people and wildlife.
 Therefore,  steep walls should be graded  to give safe access into the pit, and
 after  grading, the  pit banks should be  seeded to minimize erosion and  prevent
 the sides from sloughing off.

3.3.2     Mine Mater  Discharge

3.3.2.1   Data Sources
     The principal  sources of  information used  to model  the mining region  in

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                                                                       3-64

 Wyoming  are the site-specific  EIS's  and ER's for active and proposed mining/
 milling  operations  and the NPDES permit data on  discharge volume and quality.
 Several  reports  by state  and federal  agencies  supplemented the  foregoing,
 particularly with  respect  to  estimating  ambient  water  quality  and  flood
 volumes  for various return  periods and annual or monthly  flows  in  principal
 streams  of  the  region.   Foremost among these is  work  by  the State (Ha78),  the
 U.S.  Geological  Survey  (Cr78,  Ho73),  and  the  Soil  Conservation  Service
 (DOA75).
      Self-monitoring data  collected by industry  and  reported to  EPA  were also
 checked  to  ascertain compliance with  NPDES  permit  conditions.  Unfortunately,
 the  permits do  not specify  limits  on  the volume of discharge; hence,  the
 total  mass  or  flux per unit  of time  may  or may not  agree with the  values
 orig.inally  estimated  by  the  discharges in  the  EIS, .ER,  or license  appli-
 cation.

 3.3.2.2   Quantity  and  Qua!ity  of Pischarge
     The purpose of this section  is to  identify water quality associated with
 surface  uranium mining in  the Wyoming  Basin.   This area  was  selected  for
 detailed  source term characterization  and  pathways  analysis because of past
 and  ongoing uranium production, primarily  by surface  mining.   A subsequent
 section  (3.4.2)  similarly  addresses  underground mining.   The  analysis  to
 follow is incomplete and preliminary,  owing  to the limited  existing  data,  the
 lack  of  opportunity for  significant  new investigations  in the  time of this
 study, and  the decision to  pursue the  objectives on a "model area/model mine"
 approach.   So  many variables  of ore  occurrence,  mining practices,  climate,
 geology, and hydrology  exist  that a  detailed investigation is unrealistic.
     Table  3.21  summarizes  water quality  data  for  seven  surface  and three
 underground  mines   in  Wyoming.   Uranium  averages  0.62  mg/i and  ranges from
 0.02  to  1.3  mg/£  .  Dissolved  radium-226  is typically  less  than  4  pCi/n t
 although  one  mine  reportedly discharged  10.66  pCi/£.     Suspended  solids
 average  24.9 mg/£  .   There  is considerable  variation  from one  facility  to
 another; the observed   range  is  2.7  to 87.2 mg/£  .   Zinc  is the only stable
 element  consistently  monitored,  probably because  the NPDES permit addresses
 it.  Concentrations average 0.04 mg/ £ and are  well below the 0.5 mg/£ limit in
the permits.  Barium and  arsenic are less  frequently monitored but appear to
be in the  range  of 0.05 mg/£  for barium to 0.005 mg&  for  arsenic.  Both of
these values are well  below the discharge limits.

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    Table 3.21  Summary of average discharge and water quality data for uranium mines

                in Wyoming and a comparison with NPDES limits
Radioactivity
Mine
Project Type
1 U
2 U
3 ' U
4 S
5 S
6 S
7 S
8 S
9 S
10 S
All Mine Types (1
Average:
Standard
Deviation:
Underground Mines
Average
Standard
Deviation:
Surface Mines (4
Discharge
m/min
0.85
6.57
0.70
1.89
3.60
5.68
3.52
1.21
0.10
4.55
through 10):
2.87
2.25
(1 through 3):
2.71
3.35
through 10):
Average 2.94
Standard
Deviation: 1.96
Summary of NPDES Permit Limits
Daily Average /Daily Maximum
Total U
mg/£
0.95
0.41
0.02
1.30
0.63
0.02
0.98
0.14
1.14
0.62
0.50
0.46
0.47
0.70
0.53
2/4
Ra-226
pCt/*
3.92
2.28
7.41
10.66
3.94
2.85
0.67
3.03
3.6
4.26
3.00
4.54
2.62
4.1
3.4
3/10^a'
10/30 Total

TSS S04
87.2
2.7 234
8.8
5.0
11.1
10
19.4 875
17.3
62.5
24.9 555
29.5 453
32.9 234
47.1
20.88 875
21.04
20/30
Radium
Major and trace constituents, mg/£
Zn Fe Ba Cd As
0.08 1.25
0.02 0.02 0.05
0.01
0.01
0.14
0.05
0.05 ' 0.004 0.005
0.02
0.16
0.06 0.64 0.05 0.004 0.005
0.06 0.87 -
0.04 0.64 0.05
0.04 0.87
0.071 0.004 0.005
0.063 - - co
0.5/10 -12 -11 0.05/0.1 0.5/1 S
     (a)
        Total  Ra-226 limit is not monitored.
     Source:   NPDES permits from Region VIII  (R.  Walline,  written  communciation),  site-specific
reports (EIS, ER),  and self-monitoring data.

-------
                                                                       3-66
      Mean  values from six surface  mining  projects in Wyoming were  the basis
 for  estimating  the  effects  of mine  discharge  on  water quality. Values  from
 mines in the South Powder River  Basin model  area compare  very  well with the
 Wyoming  mines,  thus supporting adoption of a model mine  in the  Basin.   There
 were no  strong  differences in  water  quality  between surface and underground
 mines.   Table 3.21 shows that  discharge is highly variable, ranging from 0.1
          3                               3
 to  6.57  m /min, with an average  of 2.87 m /min.   In  surface mining  projects,
                       q
 the  average  is" 2.94  m /min,  with  a   standard  deviation  of 1.96, indicating
 considerable  discharge  variation among  facilities.   This  study'assumes  an
                            3
 overall  average flow  of 3 m /min  from each  surface mine in the calculations
 of  chemical  loading  of local  and regional  streams  (see  Section  3.3.3  and
 Appendix H).
      Table  3.22 shows  water quality  and flow  rates  associated with open  pit
 mines in other  areas and in various stages of operation.  Ongoing development
 of an open  pit  mine in Colorado involves 28 m /min discharge and is  therefore
 well  above  the  average.  Radium, uranium, and suspended solids are relatively
 low.  Producing  open pit mines  in New Mexico are usually dry or nearly  so  and
                                  2
 are  dewatared at  rates  of 0.6 m /min or less.  The water  is  used  for dust
 control.  Radium concentrations can be very high (New Mexico Projects)  due  to
 long  residence  time  of groundwater  in the ore  body and  the concentrating
 effects  of  evaporation.   Similary, groundwater associated with ore bodies  in
 Texas and Wyoming may contain several   hundred picocuries per liter.
     Mine dewatering has the greatest potential for adverse environmental  and
 public health impacts.  Although  contaminant concentrations  in  the  effluent
 conform  to  NPDES requirements,  there   1s long-term contaminant loading  to  the
 ambient environment.  Contaminants concentrate on stream sediments because  of
 sorptlon and  evaporation and  become  available  for  transport  by  flood  water.
 Regional  or at  least  local  dewatering of ore bodies may deplete high quality
 groundwater.   Theoretically,  dewatering may  induce  horizontal   or  vertical
 influx of   poorer  quality  groundwater into productive  or  potentially pro-
 ductive  aquifers,  but  the  extent  of  this phenomenon is poorly documented. We
 strongly recommend  further study  because  the  work  done  to  date  is largely
oriented  toward determining  engineering feasibility  versus the  overall en-
vironmental  impact.

-------
Table 3.22  Water quality associated with surface and underground mines in various stages of
            construction and operation
Project

Discharge
m /min

Total U
mg/£

Dissolved
Ra-226
pCi/i
Milligrams per li
Pb-210 TSS S04 As
pCi/£

ter
Mo Se

Colorado
  Open pit mine:
  Development stage    28     1.044     4.10
New Mexico
  Producing open pit
  mine, seepage to
  pit                   0.13  2.5     180
  Open pit mine,
  ponded inflow water   0.58  2.6     220
Texas,
  Active open pit mine
  holding pond.                      50 to  100
17

26
                                                       16.2
                                                        168
                                                        23
2151   0.005
 842   0.005
                                                                   380  < 0.01
0.018  0.019
0.545  0.043
                   <0.01  <0.01
                                                                                                           OJ
                                                                                                           I
                                                                                                           Ch

-------
                                                                       3-68

      Overland  flow is  not dismissed  herein  as  a  significant pathway,  although
 its  impact is  of lesser  importance according to  data from April  1979  field
 studies  in New  Mexico and Wyoming  (see  Section 3.2.3.2 and Appendix G).   A
 recent U.S.  Geological Survey study for  the Bureau of  Indian Affairs  (Ku79)
 addresses  projected effects  of  runoff over long  time periods if wastes  and
 sub-ore  are not  stabilized or covered.  The  study  concludes, with essentially
 no real  data,  that stream flows  are too small  in  the sub-basin  to transport
 wastes.   In  the larger basins*  such as the  Rio  Puerco,  sediment  loads are  so
 great that addition of tailings and, presumably,  mine wastes would be insig-
 nificant.  It  is  our opinion that additional field study  is needed.   Overland
 flow in a long  time  period  could move radionucl ides  in  the wastes  into  the
 main stream  channels.  Since  this  source  will  be  available  for many years
 after mine closure, if wastes art not stabilized,  it  may become a major one.
      Seepage of contaminated water  from mine holding ponds, which  are op-
 erated  to  reduce suspended solids concentrations  in mine discharge water,  is
 believed  to  be insignificant.   Since the ponds  have relatively  small areas,
 their seepage  losses are  small compared to losses  by infiltration of  releases
 to the  watercourses.   In   some mining areas,  such  as the Powder River Basin,
 shallow  groundwater quality  is naturally poor.  Maximum attenuation  of con-
 taminants  is expected  in   the shallow, poorly permeable bedrock strata of the
 Wasatch and Fort Union Formations.

 3.3.3     Hydraulic and WaterQuality Effects of Surface Nine Discharge

 3.3.3.1   Runoff and Flooding In the Mode] Surface Mine Area_

 3.3.3.1.1 Study Approach
     Precipitation  and  runoff  estimation  for the model surface mine scenario
 in   Wyoming  considers  three  hydrographic   units:   sub-basin,   basin,   and
 regional basin.   Respective  surface  areas are 11,4, 5,400,  and 13,650 square
               2
 kilometers (km).   The  mine  is  located in the sub-basin.  The sub-basin, the
 basin,  and the  regional   basin  are  all   drained  by ephemeral streams.   The
 latter is drained by "a major regional river  that  has wide seasonal variations
 in flow  and  is dry or nearly so about  180 days each year.  The sub-basin has
similar flow variability.  Figure 3.9  depicts  the  mine in  relation to the
sub-basin, basin, and regional  basin.

-------
                                                                              3-69
           CAMPBELL COUNTY
      \
 Sub-basin area

 containing model

 mines
                                                           I
                                                           i   SOUTH
                                                               DAKOTA

                                                               NEBRASKA
               CONVERSE COUNTY
            20
           _i_
40
 i
 60
	i
                       (km)
      .......,.,Sub-basin boundary(approximate)

      	Basin  boundary

      —.—Regional  basin boundary
Figure 3 9 Sketch of sub-basin, basin, and regional basin showing orientation of principal drainage

         courses, areas of drainage, and location of mines

-------
                                                                       3-70

     The  first  general  approach  defined  quality  and volume  of mine  water
 discharge.   Hypothetical hydrographic  basins  were  then delineated and  flood
 flows  calculated for  return periods ranging  from  2  to 100 years. The  indi-
 vidual  and  collective effects of  discharge from  three  mines were  then  evalu-
 ated  in terms of perennial  flow,  flood  flow,  and chemical  transport.   Of  key
 importance  was an  estimation of  the extent of perennial  streams created  by
 mine  discharge  and the  influence of  contaminants on water quality  in  the
 river draining the  regional  basin.

 3.3,3.1.2 Description  of Area
     We selected an  area  of active  mining and  milling  in the South fowder
 River Basin  of wyom-ng for  analysis.   The  area has four active or imminently
 active  uranium mills and a  number of  open  pit mines.  Available data on  the
 geology, hydrology,  and  water quality  of the  area  are  sparse, but becajse  of
 the mining and milling activity are relatively well known for a remote region
 like northeastern Wyoming.   The  study  team chose one mining and milling pro-
 ject  in the  area  For field  investigation   in  April  1979;  hence, additional
 data became available and are used herein as appropriate.
     Terrain  in  the area  has low rolling  hills  and  an average elevation  of
 1414 m  (MSL  datum).   Since the  climate is not  very  different  from  that  of
 nearby  Casper,  Wyoming,  meteorological  data  from  that station  are  fairly
 representative of  the region.   There are  no  relatively large  seasonal  and
 annual  variations  in precipitation intensity,  frequency, and  duration. Mean
 annual   precipitation  over  a 30-year  record  period  is  28.5  cm  and  occurs
 mainly  as  scattered  thunderstorms  in   late  spring and early  summer.  These
 thunderstorms  supply  25  to  50 percent of the  total annual  precipitation and
 are  usually  of  high  intensity,  short duration,  and can  be  quite  local.
 Potential  pan  evaporation  averages 110  cm  per year and greatly exceeds pre-
 cipitation.
     Streams  in  the  study  area  are ephemeral  and only exhibit measurable
 surface flow  during  snowmelt and heavy  thunderstorm activity.   Average total
monthly flow  for the period 1948  through 1970 for  Lance Creek  and the Chey-
enne River at Spencer,  Wyoming  reveal distinct high-  and low-flow periods  in
 the year  (Fig. 3.10).   We  believe that the streams  represent  the basin and
regional  basin  hydrographic  units  used herein.   Large watersheds  usually
exhibit measurable  surface  flow  for  about  180  days  per year.  Small  water-
sheds,   30  to  40 square  kilometers, may not flow at all  for several  consec-

-------
     —  100QOCC
      6    9.
o


o
Ik
>
«4
X

o
s
                                                                                    3-71


                                                                                 Cheyenne River
                                                                                 mean annual  flow
                                                                                 Lance Creek
                                                                                 mean annual
                                                                                        flow
                                                                                  3 mines  mean
                                                                                  monthly  flow
                                                                                  2 mines  mean
                                                                                  monthly  flow

                                                                                  1 mine mean
                                                                                  monthly  flow
                                        MONTH
Figure 310 Average monthly flows for the Cheyenne River and Lance Creek near Spencer, Wyoming, for the period
1948-1970  (DOI59, DOI64, DOI69, DOI73)

-------
                                                                       3-72

 utive  years.   Mean annual runoff  is  0,8 to 1.3 cm  or  0.0023  to  0.004 m /sec
       2
 per  km.
     Peak  flows  in  the  regional  basin and  basin  area are  a  result of  snowmelt
 in at  least 50 percent of the  cases.   This is  commonly  due to temporary but
 rapid  melting  from January to  March.   High flows  can  also result from wide-
 spread  summer  storms,  but these are  the exception.   For small basins  on the
 order  of forty square kilometers or less,  peak flows  occur  because of  thunder-
 storms  in  the  summer  months.   Thus  peak  flows  in   small  basins versus  the
 basin  or regional basin commonly occur  for different  reasons and  at different
 times  in  the year.  A  period of peak  runoff  from  the  sub-basin  might  coi.i-
 cide  with   a low flow or zero  discharge  condition  in  the  basin  or  regiotal
 basin.
     In the area of the Morton  Ranch project (DOA75)  there  are 14  sub-basir?,,
                                     2
 the  average of which is about 11.4 km.  Channel slopes are 11.4  to 31.4 m.'itm
 (average 21.2 m/km), and  basin  slopes are  about 88 m/km.  These are tributary
 to  larger  streams  with  channel slopes  of 2.17 to   17.0 m/km  (average  6.63
                                                          2
 m/km),  and  which drain  basins  with  an area  of 5,400  km  and a  mean  annual
               3
 flow of 0.80 m /sec.   These,  in turn, are  tributary  to a regional  basin  with
                     2                                3
 an area of  13,650 km  and mean annual flow of 1.47 m /sec.  All  three  hydro-
 graphic units  are  drained  by  ephemeral  streams.   The main stem of  the  re-
 gional system  is  dry  an average of 180 days per year.  The basin drains  into
 the  regional basin, assumed here to be the Cheyenne River Basin, which  drains
 an area of  13,650 km2 (Da75, Lo76, Ra77).
     Surface water  in  the model  area  is used mainly for stock  watering  and
 irrigation.  The amount  of  irrigated  area in  the  basin  is  1400 hectares,
 compared to 2800 in  the  regional  basin.  Because of extreme  variability in
 surface flow volume and  water  quality, almost all  municipal water comes  from
 wells completed in bedrock.  Stock water is from both wells  and impoundments,
 whereas single-family domestic  supplies are primarily from wells.

 3.3.3.1.3 Method of Study
     Because of  dilution considerations,  flow volume  rather  than peak  dis-
 charge rate is of  prime  concern.  For  the basin and  regional  basin areas,
only  peak   flow  rate  can be  readily  estimated on  a  probability  basis  for
annual  and longer time periods  of perhaps 2, 5, 10, etc. years.  Peak flow in
the  larger  hydrographic  areas  commonly does  not  coincide  with  that in  the

-------
                                                                       3-73

 smaller basins.  Also, there  Is  poor correlation between peak  flow rate (Q)
 and  total  flow  volume  (V) for  streams draining  large  basins.  Total  flow
 volume in the larger basins can be estimated from partial  duration flow data.
 That is,  we  can  estimate the  percentage  of the time, during the year,  flow
 will be of a  given  magnitude.
      Relationships  among runoff  volume,  rainfall,  and surface  area  in  small
 basins  {encompassing  less   than  30  square kilometers) in  the  Powder  River
 Basin have been developed  by  the U.S. Geological Survey  (Cr78) and the  Soil
 Conservation  Service  (DOA75).   Peak discharge  and  total  annual flow in  the
 basin and  regional  basin units  were  measured  by the U.S. Geological Survey
 for  Lance Creek at  Spencer, Wyoming and for the Cheyenne  River  near Spencer.
      We analyzed  the effects of perennial  or chronic  mine  discharge  on ehang-
 inq  existing  ephemeral streams  in the  sub-basin, basin, and regional  basin to
 perennial  streams  using  a  crude  seepage and  evaporation model.  The basic
 equations  and  approach, explained in Appendix H» are  similar  to  those used in
 the  Generic  Environmental   Impact  Statement  on Uranium  Milling  (NRC79b).
 Adjustments  were  made  for  mine  discharge rates and  infiltration  and evap-
 oration losses.  The main output  of the model  is an  estimate of which stream
 segments  might become  perennial  and what  the  net  discharge  would be from a
 number of mines operating  in the same sub-basin.  Water quality  impacts  can
 only be very  roughly assessed.   For  the  time  being,  we  assume that infil-
 tration and  evaporation  decrease flow but  do not effect the  chemical mass  in
 the  system.   That is, we assume  contaminants  in mine drainage  are  deposited
 on  or  in the  stream/wash  substrate  and  remain available for  transport by
 flood water.
     The  sub-basin  is as shown in  Fig.  H.I  (Appendix  H)  and contains three
                                                           3
 active  uraniym mines,  each of  which  discharges 4,320 m /day.  Quaternary
 alluvium  constituting the  channel  is  assumed to have  a porosity  of 40 per-
cent.   The sub-basin contains seven  streams or wash segments, three receiving
mine water directly.   Water from the mines dissipates by  infiltration, evap-
oration, and as-surface flow that may leave the  sub-basin entirely.  Appendix
H shows  the  basic equations and  assumptions  and gives a complete summary of
 "losses" due  to seepage  and evaporation as  well  as  any net outflow from the
sub-basin.

-------
                                                                       3-74

      Precipitation-runoff in the Wyoming  study area correlates rather closely
                                             2
 to basin  size.   Basins  of  about 105QQO  km  area  have  an annual  unit-area
                                                         2
 runoff of 0.43 cm/yr;  whereas  an area of perhaps  25  km  might have a runoff
 of only  5  cm/yr.  Decreased  runoff (on  a  unit area basis)  associates  with
 larger  basins   and  reflects   water  storage,   channel   losses,   and  evapo-
 transpiration  that occur mainly  in  the tributaries.   Impoundments are rarely
 on the  main  stem  of  streams,  where washouts  are a  problem,  but  rather  on
 tributaries.   The  average  impoundment   is  located  about every  130  square
 kilometers,  is "rather small, and is  used  for stock  water.   Very infrequently,
 small  flood-irrigation   projects  may use  impounded  water  for  grasslands.
 Seventy-five  percent of  the annual  runoff occurs  during the summer  thunder-
 storm  activity  in May, June, and July.   Snowmelt occurs  rather slowly and  is
 captured in  the  headwater areas,  whereas  rainfall  events are  rather  intense
 and  localized, causing  excess flows  that  reach the  main stem,  Lance  Creek and
 Cheyenne River.   Sediment loads  are  high  in both the  tributary and main stem
 streams.
     Contaminant  concentrations  in overland  and  channel flow during  peak run-
 off  events  in  the  sub-basin are  expected  to follow the pattern shown  in Fig.
 3.11,  the data  for which are  from the U.S.  Geological Survey  (H. Lowham,  in
 preparation) for  a  small  basin,  Salt Wells Creek, in the Green River Basin  of
 southwestern Wyoming.
     Note  in  the inset of  Fig.  3.11 that the washoff peak,  that portion  of
 the runoff enriched in dissolved  and suspended materials, precedes the  runoff
 peak.  Runoff  in small basins is typically associated with brief but  intense
 thunderstorms  that flush the  land  surface.   Total   suspended  solids (TSS)
 concentrations  are disproportionately high  in  the peak  flow  events.  Dis-
 charges  of  170 m /min  carry  100,000 mg/£ TSS; whereas flows  of  1 cfs might
 carry  only  500 mg/ji.   The  leading  edge  of the high  flow has  the greatest
 concentration of  suspended  solids and dissolved chemical  load.  Figure 3.12
 depicts  discharge and specific  conductance values   as  a  function  of time for
 the same  small  basin  in  Wyoming.  Specific  conductance  (SC)  is a rough mea-
 sure of  the total  dissolved  solids (OS)  content,  following  the approximate
 relationship:  DS  =  0.71 SC.   Note that the first rise in the flow hydrograph
 occurs about three  hours  after the peak  for specific conductance, indicating
 the presence of  a contaminated "front" laden with  salts  and  other suspended
and  soluble  materials.   The second  peak on  the   flow  hydrograph similarly
 precedes  and is  associated  with degraded  water  quality  due to this flushing

-------
200,000-
100,000_



 50,000-
 10,000-
  5,000.
  1,000-


    500-
    100.
CO
6
          o
          o
          o
          u
s
1/3
Q
P4
          IX
          to
       0.1
                                                            A
             General  sediment-transport
             characteristics of stream
             after flushing by leading
             edge  of  flood wave.
                                                                      Example hydrograph
                                                                      showing flushing
                                                                      action of floodwave,
                      TIME-
                                             LEGEND
                                              • Low-flew  conditions
                                              D Medium-flow conditions, Spring snowmelt
                                                runoff..
                                              « High-flow conditions, rainstorm runoff,
                                              A Samples obtained by automatic sampler of
                                                leading (rising) edge of floodwave.
             0,5
T
5
 i
10
                                   50
DISCHARGE, IN CUBIC FEET PER
                                                                              100
500   1,000
                                                                                                                       i
                                                                                                                      •u
                                                                                                                      U1
                  Figure 3 11 Suspended sediment concentration to discharge. Sail Wells Creek and tributaries, Wyoming (From U S
                  Geological Survey data, H Lowham, in preparation)

-------
   5.
o
u
tu
Pi  ,,
w  4-
CL,



fc
PJ
   3.
CO

B
UJ
C3


I

b
   2.
   1.
   0
                                         "FLUSHING" OF ACCUMULATED SALTS AND

                                        "MATERIAL
                                               Specific conductance
                                             Discharge
                        N.

                        i
                        t
                        i
                             i
                             i

                       *

             '   •**.	./
                                                                                         3,000
                                                                                         2,000
                                                                                              u
                                                                                              c
                                                                                              ift

                                                                                              CM


                                                                                              H
                                                                                               in
                                                                                               o
    H
.oooy

    §

    8

    u
    i— i
    uu
                                                                                              ex
                                                                                              t/)
 1800      2400                 1200

July  19                      July 20


                               Tim  (HOURS)
                                                        2400      0600       1200

                                                                       July  21
                                                                                     1800
  Figure 3,12 Relation of discharge and specific conductance to time at Salt Wells creek. Green River Basin, Wyoming

  (From U S Geologrcal Survey data, H Lowham, in preparation )
                                                                                                                         •-4

                                                                                                                         ON

-------
                                                                       3-77

 action. About 33  hours  after precipitation begins, runoff  water  quality and
 flow   very   nearly  approximate   antecedent   conditions.   This   indicates
 rather  thorough  flushing,  most  of  which occurred  in  an 18-hour  period.
      Assuming similarity  between  the  surface  mining  area  and  the situation
 described above, we believe intense flows of rather short duration flush most
 of  the contaminants  from the  land surface and  stream  channels.   Although
 sub-basin floods are expressed  in  terms of return period  for  Wyoming and in
 terms of partial duration  {l-day»  7-days)  and  varying  return  periods  for New
 Mexico, we believe-the  basic  approaches (total  flow vs.  partial duration) to
 be  rather  similar  because of  the  "flashy" nature of runoff  in   both  study
 areas.  In the  New  Mexico case, the mean discharge rate  and  the  flow volume
 for the 7-day event are  very  often  less than that  for  the  l~day  event  for the
 same  return  period.  This also confirms the  intense,  short-term nature  of
 runoff processes in the  Wyoming  and New Mexico  model areas.

 3.3.3.1.4 Discussion of  Results
      This section addresses  the interaction between  mine drainage and  flood
 waters.  Flood magnitude is addressed  first, followed by calculation of  water
 quality effects  due to mine water.   The U.S.  Geological  Survey technique
 (Cr78) for  estimating floods  in  small  basins in  northeastern Wyoming was  used
 to estimate peak discharge and  total  flow  volume  in the sub-basin.  Multiple
 regression  analysis reveals  that  the  variables  of area,  slope,  and relief
 provide roughly 90  percent  correlation  between  rainfall  and runoff  (Cr78).
 Considering  the  numerous assumptions made  throughout  the  analysis, only  the
 area variable is used herein.   It  accounts  for  70  percent of the  flow.  Table
 3.23 shows  the peak discharge rate  and total  flow volume from the sub-basin
 for floods  with  recurrence intervals  (r) of 2  to  100 years.  The basic  equa-
 tion  for calculating discharge rate  or  flow  volume  is--
      Qr or Vf -  a Abl                                        (3.1)
 where  a = regression constant
      b, ~ drainage  area  coefficient  for area: peak  discharge area;  volume
          relationships
       A = basin  area
        = 11.4 km2
Q  , V   = discharge  rate and flow volume for flooding events with return
          periods of 2,  5, 10, 25,  50,  100 years.

-------
                                                                      3-78
      The  flow volume  for the  two-year  flood is  32,921 m ,  and the instan-
                                  2
 taneous  peak flow  rate  is 387 m /min.   For  comparison,  we  assume that the
                              o                 <-   
-------
                                                                       3-79
      Maximum discharge from  the  basin and sub-basin is  expected  in  the late
 spring and early  summer  months  because of thunderstorms.  At this time, flow
 in the  river draining the  regional   basin  is also at or  near  maximum, thus
 there is high probability for considerable dilution of runoff contaminated by
 mine drainage.
      Total flow volumes  for  the  basin and regional basin were estimated from
 U.S.   Geological  Survey  records  for  the  period 1948  to 1970.    Figure 3.10
 shows average monthly flows  in  cubic  meters  for the Cheyenne River and  Lance
 Creek near Spencer,-Wyoming.   Immediately  apparent  is the close  similarity in
 overall  runoff pattern for the year.
      Table 3.24   Summary of, calculated  total  flow in  the  Wyoming  model  area
                   sub-basin  using  the  USGS and SCS methods
 Recurrence
 Interval,  r,
 in  years
     Sub-basin
Total  flow (m3)
     ^Source:  Cr78.
      ^Source:  DOA75.
      ^C'NC = Not calculated.
    Sub-basin
Total  flow (m
2
5
10
25
50
100
32,921
64,116
90,009
127,862
159,920
194,937
14,467
NC^
98,419
170,815
231,618
295,257
Minimum  flows occur  in  November, December, and  January,  and  peak runoff in
both  basins  occurs in May, June, and July.  Long-term average annual flow in
                       73               73
the basin  is 2.18 x  10  m  and  5.64 x 10   m   in the Cheyenne River.  These
                                                                            2
are almost exactly proportional  to the respective  basin  areas  of 5,360 km
              2
and 13,650 km , indicating similar climatic  and runoff conditions.

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                                                                       3-80

      Assuming there are  3  mines operating for a 17-year period and that each
 mine discharges  on  the  average 3.00 m /min continuously,  total  annual  flow
 volume from  the mines is 4.7  x 10  m .  Cumulative discharge  from  the  sub-
 basin  is  7.04  m /min or  3.7  x  10   m /yr,  which  causes  development  of a
 perennial  stream 12.8 km long within the basin.   Insofar as  the basin channel
 length is 141 km, the perennial stream ceases  to flow well  within the basin.
      Appendix H  explains  the methodology and intermediate  steps  involved  in
 deriving  these foregoing values.  Mine drainage  water is not expected to  flow
 the full  length- of  Lance Creek or reach the Cheyenne River.  However, on the
 basis of total  monthly flow, the volume  of mine drainage  from one  mine ex-
 ceeds the flow  in Lance Creek and the Cheyenne  River for three months of the
 year,  whereas flow  from three mines  exceeds  basin  flow for five months and
 regional  basin flow  for four months  each year (Fig.  3.10).
      The  aqueous pathway for mine  drainage is considered in  terms  of  chronic,
 perennial  transport  in  the  mine  water,  per se,  and  transport by flood waters
 that periodically scour  the channels  where most of the sorbed contaminants
 would  be  located.   Considering  the  random  nature  of  flooding and   the  re-
 sulting  uncertainty  as  to  when the next  2-, 5-,  or 10-year, etc. flood may
 occur,  it  is  assumed  that most contaminants  accumulate  on an annual basis and
 are  redissolved  by  floods  of  varying  return  periods (2  to  10  years)  and
 volumes.   Many  combinations  of buildup  and flooding  are possible,  such  as
 buildup  for  5 years  or 10 years with  perhaps several  2-year storms   and one
 5-year  storm.  Insofar as numerous assumptions are made in calculating volume
 and  quality  of mine  discharge,  basin  runoff, and fate  of the contaminants  in
 the  aqueous  system,  use of  annual accretion and  varying flood  volumes  in the
 sub-basin is  considered  adequate for estimating flood water  quality.
     Dilution of  contaminated  flows  originating in  the sub-basin  and  ex-
 tending  into  the  basin were conservatively calculated by assuming  that the
 total  flow  during the low period equaled the mean  annual flow.  Thus,  high
 flows  and associated  increased  dilution are ignored, tending to make  the
 analysis  conservative.   Contaminated  flows  from the  sub-basin are   diluted
 into these  adjusted  mean annual flows.   Definition  of  the  source  term on an
 annual  basis  is  most  compatible with the  radiation  dose  and health  effects
calculations  in  Section 6.   Use of the  low  flow segment of the total annual

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                                                                       3-81

 flow regime is decidedly conservative since total  flow during the five months
                                            3              3
 of low flow conditions amounts  to 111,610 m  and 218,336 m  for the basin and
 regional  basin, respectively.  Average  annual  flow for the  period  of record
 (22 years) is considerably  higher,  amounting to 2.184 x 10  m  for the basin
              7  3
 and 5.64 x 10  m  for the regional  basin.
      Runoff in  the  basin and  regional  basin is expected  to  markedly dilute
 contaminated flood -flows originating  in the basin,  Such  floods  would  scour
 contaminants  from  about 23  kilometers  of  channel  affected  by  contaminants
 from the  three  active mines.  Peak  runoff events in the  sub-basin  are  most
 likely in  the late  spring-early summer season  when runoff in the  basin  and
 regional  basin is  the maximum or  near maximum,  on  the average.  However,  peak
 runoff from the sub-basin could  also occur when the basin and r&qional  basin
 are at  low flow or zero discharge.   Such contrasts are  present  between  the
 basin  and  regional   basin  flow  regimes.   From  September through  December,
 Lance  Creek tan  be expected  to  have  no discharge from 45 to 65 percent of the
 time,  whereas the Cheyenne  River will  be dry, on  the  average,  from 65  to 85
 percent  of  the time  (Fig.   3.13).   Thus  there  is  a  distinct  chance  that
 contaminants  transported  in  Lance Creek  would not  be immediately  diluted  upon
 reaching  the Cheyenne River.
     Before discussing the  calculated  concentrations of  contaminants in  the
 basin  and  regional  basin streams,  several  other  conditions need to  be  men-
 tioned.   In water-short  regions  like Wyoming,  extensive  use is made of  im-
 poundments  to capture  aad  store  runoff.   On  Lance Creek, the model  for  the
 basin,  the  volume of  existing impoundments is  15.78 x  10  m  or 72  percent of
 the  annual  average runoff.   In  the regional  basin,  modeled "after  the Cheyenne
                          7   1
 River,  there are 4.2 x 10   m  of storage  volume,  which is 74 percent of  the
                          fi   O
 average  flow of 56.4 x 10   m .   Thus,  it  is  very  likely  that discharge  from
 the  sub-basin or basin will  not  exit the basin, particularly in  the periods
 of  low  flow.   Contaminant  concentrations,  particularly   those  affected  by
 sorption and  precipitation reactions,  are likely to be  reduced as  a  result of
 sedimentation  and  long residence  time in  the  impoundments, although  there is
 some  potential  for overtopping,  disturbance  by cattle, and so on.   Signif-
 icant  adverse impacts are not  likely considering  precipitation and  sorption
 reactions which  are  likely to  remove contaminants  from  the food  chain. Proof
of this  1s  lacking  and we recommend confirmatory studies  for  the  stable  ele-
ments.   Previous studies (Ha78;  Wh76)  emphasized   radiological contaminants.

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   100-
    90
o  80.
cc
M
o-
Ixl
70—-J






60-





50-






40.






30—1
                           Cheyenne  River

                           (Annual 0-Flow days  i=55.7l)
                                                                                 V
                                                   x'
^ Ort
o 20 —
LU
a.
10 —

•-— . ^••>y' Lance Creek

« (Annual 0-Flow days 55=42.9%)


JAN FEB MAR APR I MAY JUN JUL AUG SEP OCT


NOV DEC i
        [ Figure 3.13 Periods of no flow in Lance Creek and the Cheyenne River near R iverton, Wyoming for the period 1948-1978

        J (Summarized from flow records provided by H Lowham, U S. Geologies! Survey, Cheyenne, WY }

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                                                                       3-83
      Radlum-226  is  strongly  sorbed  onto  stream  sediments  and  (or)   it  is
 subject to  precipitation.   Partial  re-solution  in subsequent  floods  occurs
 but it  is  assumed  that  only 10  percent  of  the mass deposited on  an  annual
 basis   goes   back  into  solution   in  flood waters.   The  rationale  for  this
 assumption  is based on  laboratory studies (Sh64; Ha68),  field  data from New
 Mexico  (Ka75;  Ku79),  and  review  of the  literature.   Pertinent  field  and
 laboratory  data  specific  to  surface  water  quality  in  the Wyoming  uranium
 mining areas are scarce, although studies by the State  (summarized  by Harp,
 1978}  are noteworthy.   Sulfate is regarded  herein as rather mobile and,  as
 such,  most of it  infiltrates  the shallow aquifer.   Therefore,  only 20  percent
 of  the  mass  frcm a given  mine on an  annual  basis is assumed  available  for
 re-solution  in flood waters.  The fate  of zinc, arsenic, and  cadmium  is  in-
 sufficiently understood  to predict what fraction  in the mine discharge  will
 be  removed   from  solution versus  remain available for re-solution.  Studies
 along  these  lines  are  necessary.   Similarly,  not all  of  the contaminants
 potentially  present  in  mine  waters   from Wyoming are  necessarily  shown  in
 Tables 3.21  and 3.25,  which were developed based  on  available  data from NPDES
 permits, environmental reports, and  environmental  impact statements.  In  the
 case  of suspended  solids,  there  is  no  calculation of non-point source  con-
 tributions  from  mined lands.   Sediment  loads  from  such sources  could  be
 locally  significant, but  mined  land reclamation  and  natural  recovery seems  to
 effectively mitigate problems.  Only  suspended solids  from mine  drainage,  per
 se, are  considered.
     Table  3.25 shows the  flood  flow  volumes  (in the sub-basin) associated
 with events  having return periods  of 2, 5, 10, 25, 50,  and 100 years.  Also
 shown  are  the contaminant concentrations  calculated from the  annual contami-
 nant loading  diluted into the foregoing floods.  As expected, concentrations
 are high because  of the  low  dilution volumes associated with the small sub-
 basin.  Surface  water in  the  sub-basin might  be  impounded therein for  use  by
 stock  or, less possibly,  irrigation,  but it is more likely that  the  principal
 impoundments would  be  in the larger  hydrographic unit, the basin.   The flood
 flow  volumes  shown  represent  runoff from  the  entire  sub-basin.   When  the
second and  third  mines  begin to  discharge,  the  annual  loading and concen-
tration  values  shown would  have to be doubled or tripled.  The  reader  should
remember that background concentrations  already present in flood runoff would
be  additive  to the  values  in Table  3.25.  However,  these have been assumed

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                         Table  3  25   Annual  contaminant  loading  from one uranium mine and  resulting concentrations
                                     in  floods  within  the  sub-basin for return periods of  2 to 100 years
Contaminant and
concentration in
mine effluent
Total uranium 0.
Radlum-226 4
Total sus-
pended solids
Sulfate
Zinc
Cadmium
Arsenic
20.
875
0
0.
<0.
. 070 mg/ i
I pCi/i
.9 mg/ i
«g/ i
071 mg/ i
. 004 mg/ t
. 005 mg/ i
Chemical mass available
for transport on an annual
basis
110
0.00065
32,955
275,940
112.0
6.31
7 88
kg/yr
Ci/yr(a)
kg/yr
kg/yr(b)
icg/yr
kg/yr
kg/yr
Flood flow volumes (m ) and contaminant concentrations associated
with return periods of 2 to 100 years
V2 = 32921
C2
3.34
19.7
1001
83B1
3.40
0.192
0.239
V5 = 64116 V = 90009 \
C C
5 L10
1.72 1 22
10 1 7.2
514 366
4304 3066
1.75 1 24
0.098 0 070
0.123 0 088
?25 = 127862
0 86
S.I
258
2158
0.876
0.049
0.062
VM = 159920
C50
0.
4.
206
1723
0.
0.
0.
69
1


700
039
049
V10Q = 194937
C100
0
3
169
1416
56
3


0.575
0.
0
.032
040
        Ten percent of  the annual  loading  is  assumed available for solution.  The balance  is assumed sorbed onto sediments or present in
insoluble precipitates,
       'Twenty percent  of the annual  loading  is  assumed available  for  transport and  the  balance  is assumed to have infiltrated to the water
table or it is present  as an  insoluble precipitate.
        V  and C   refer to, respectively,  flood  volume, in cubic aeters, and concentration in milligrams per liter or picocuries per liter for an
r-year flood.   Concentrations are  in  milligrams  per  liter except radium-226, in pCi/t .
     Note.--Assumptions:   Mine discharges  continuously at a rate of 3.00 m /mm and  concentrations are the average of those shown in Table 3.21.
All suspended  and dissolved contaminants remain  in or on the stream sediments and are  mobilized  by flood flow.

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                                                                       3-85
 equal to zero In order to estimate incremental increases due to mining and to
 simplify the calculations.
      Table  3.26  shows  contaminant  concentrations  in  the  basin  and regional
 basin streams  from the  discharge  of one  mine.   For  cases  involving  two or
 more mines,  the  concentration  shown would be scaled up by a factor of two or
 more.  Basically,  the  table shows  the effects of  taking  contaminated flood
 waters from  the sub-basin  and  diluting them  in  the low flow volume  of the
 basin and regional.basin. As expected, concentrations decrease with floods of
 greater  volume  and  longer  return period.   Additional  dilution  occurs  when
                              * «
 discharge  from  the  basin enters  the regional basin.   Taking  the  two-year
 runoff event in  the  sab-basin,  for example, uranium is diluted from 3.34 mg/£
 (Table 3.25) to  0.76 mg/2. in the basin  and then to 0.44 mg/£  in  the regional
 basin.  There  is some question  as to  whether the  lesser  sub-basin  floods,
 particularly those with  return  periods  of 25 years or  less,  would  actually
 flow the length  of the  basin and enter  the  regional  basin.   Because  much of
 the  22.7  km reach of  stream  directly affected by mine discharge is located in
 the  basin, it is conservatively  assumed  that the  contaminants  will  reach the
 basin and  eventually  the regional  basin.   The foregoing analysis  is  struc-
 tured as  a worst-case, maximum-concentration scenario.
      Concentrations of contaminants  in flood waters  affected  by mine drainage
 are  compared  to  water standards for potable and irrigation  uses (Table  3.27).
 Radium-226 concentrations  in the  basin and" regional  basin  streams  (Table
 3.27)  range from 1.6 to  4.5  pCi/fe  and are  below  the drinking  water standard
 (for Ra-226 + Ra-228) of 5  pCi/£.   Uranium concentrations  range  from  0.26 to
 0.76 mg/£ , which is  roughly  equivalent  to  176  to  514 pCi/£.  On  the basis of
 chemical  toxicity alone,   such concentrations would  probably  present no prob-
 lem  for  short periods, but  radioactivity  is another matter. Reevaluation  of
 the  standard for uranium in potable  water is presently receiving attention
 within  the  Agency  (R.  Sullivan  and  J. Giedt,  USEPA,  oral   communication,
 1980).   Briefly, there   is  consensus  that  the radiotoxicity  of uranium  is
 similar to  that  of  radium-226 and 228.  For  continuous  ingestion  at a rate of
 2  liters  per day, it is  suggested that potable water contain no  more than 10
 pCi/i  (0.015  mg/ji)  natural uranium  to reduce the  incidence of fatal cancers
 to no  more than  0.7 to 3  per year per million  population (Office  of Drinking
Water  guidance to the State  of Colorado, July 7,  1979).  Realizing that  the

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          Table 3.26  Concentrations in basin and regional basin streams as a result of surface mine discharge
Parameter
Concentrations (ingA  ; pCi£  in the  case of  radium)
in basin discharge under low flow conditions due
to influx of sub-basin floods with  2, 25, and  100
year return periods*3''
                                     "25
                                      "100
                                                                           Concentrations  {mg/i ;  pCiA  in the case of radium) in regional
                                                                           basin discharge under  low-flow conditions due to influx of basin
                                                                           discharge,  also under  low-flow conditions, and sub-basin floods
                                                                           with 2,  25, and 100 year return periods^ '
"25
"100
Total Uranium
ftadium-226
Total Susp, Solids
Sulfate
Zinc
Cadmium
Arsenic
0.76
4.5
228
1909
0.774
0.044
0.054
0,46
2.7
138
1152
0.468
0.026
0.033
0.36
2.1
107
900
0.366
0.020
0.025
0.44
2.6
131
1098
0.445
0.025
0,031
0.32
1.9
95
797
0.324
0.018
0.023
0.26
1.6
79
668
0.271
0.015
0.019
     '^Calculated as follows:  Assuming a two year flood, uranium concentration in the outflow from the sub-basin equals 3.34 tng/i and flow
equals 32,921 m  (see Table 3.25).  Average total flow for 5 months of low flow conditions in the basin equals 111,610 m .  The concentration
in the basin outflow, after dilution of the contaminated inflow from the sub-basin for floods of varying recurrence intervals equals:
     C8asin = VSub-basin xCSub-basin = (32921 ro3) (3.34 mg/t )  = 0.76 mg/i
               (Sub-basin +  Basin)
                                 	It
                          32921 m3  + 111610 m3)
     * 'Calculations similar to "a" above, except average total flow volume for 5 months of low flow in the regional basin equals 218,336
 i                C                 V            C
m .  Hence,        Regional basin =  Sub-basinx  Sub-basin
                                     g
                                    ( Sub-basin +  Regional Basin)
                                                                                                                                                    CD
                                                                                                                                                    en

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               Table  3.27  Comparison of potable and irrigation water standards and  surface water quality affected by surface mine drainage
Parameter
            Range of  contaminant concen-
            j
            'trations  in flood flow
            affeeted  by mine  diseharge
               Basin          Regional  Basin
            Mm.      Max.      Hin.      Max.
     Potable water standards^
                                                                                                                   Irrigation
                                                                                                                             (c)
Maximum Pentiissable
    Concentration
Recommended Limiting
     Concentration
Recommendations for maximum concentration
  for continuous use on all soils (mgfa )

total U
Ra-226 + 228
TSS
Sulfate
Zinc
Cadmium
Arsenic

0.36
2.1
107
900
0.366
0.02
0.025

0.76
4.5
228
1909
0.774
0.044
0.054

0.
1.
79
668
0.
0.
0.

26
G


271
015
019

0.
2.
131
1098
0.
0.
0.

44
6


445
025
031

0.015/3.
Iff}
5/0.2Pa)



—
5 pCi/£
--
—
—
0.
0.
-
-
-
01
05
-
250
5
—
0
..

.0
-
.01

—
5 pCi/i
—
ZOO
2.0
0.010
0.10
     (a)
     W
Concentrations in milligrams per liter, except Ra-226 -228 which are in picocuries  per liter.
Sources:  U.S. Environmental Protection Agency (EPA76) and, in the case of uranium, suggested  guidance from the National  Academy of
Sciences (NAS79) to the USIPft and from USEPA (Office of Drinking Mater) to the State of Colorado (La79).
     ^Source:  NAS72.
     '   '0.015 nigA : Suggested maximum daily limit based on radiotoxlcity for potable water consumed at a  rate  of 2 liters per day on a
                  continuous basis.
     3.5  mgA : Suggested maximum 1-day limit based on chemical toxicity end intake of 2 liters 1n any one day.
     0.21  mgk "  Suggested maximum 7-day limit based on chemical toxicity and Intake of 2 liters per day for  7  days.

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                                                                      3-88
limit  of  10  pCi/£   (0.015  mg/£ } may  not be  cost effective, the  Agency  is
contracting  to  develop the  economic  and  technical  basis for a  uranium (in
water)  standard.  The  National  Academy  of  Science,  at  the request  of the
Agency, evaluated the chemical toxicity of uranium.  A maximum, 1-day concen-
tration  of 3.5  mg/£ (7  mg/day  based  on  daily intake of  2 liters)  is the
"Suggested  No Adverse  Response  Level"  (SNARL).  The  corresponding  concen-
tration for a. 7-day  period is 0.21 mg/£ .
     There  are  numerous  complicating  factors  surrounding  the foregoing sug-
gested radiotoxicity and chemical toxicity limits for uranium.  These include
economic justification, technical feasibility, gut to blood transfer factors,
and overall health of the receptor,  to name a few.  Of importance is the fact
that  a stricter  standard  for uranium in  water  
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                                                                       3-89

 3.3.3.2   Impacts of Seepage on Groyndwater
      The previous analysis  assumed  no Infiltration (to groundwater)  of dis-
 solved or  suspended contaminants*  thereby  creating a maximum  or worst-case
 situation with respect  to  transport via floodwaters.  In  fact,  contaminants
 will  also infiltrate through the stream deposits.   Anions  and selected stable
 elements like  uranium,  selenium, and  molybdenum  are most likely  to  migrate
 downward.  Insofar as the  alluvial,  valley fill aquifer may  be  used  locally,
 particularly in  the case of  larger  drainage  basins and the  regional  basin,
 some  analysis of  potential  impacts is offered  herein.
      Effects of  mine  drainage impoundments used  to settle  suspended  sol Ids
 are excluded  from  the  present analysis.   Such  impoundments are  relatively
 small, commonly  less  than  1 or  2 hectares, and  tend to become  self-sealing
 due to  settling  of  fines.   Potable  water  supplies  at  the mines  are  usually
 from  deep exploration  borings converted to water  wells  or from mine  water.
 Problems may exist with  such water being  contaminated, as has  been documented
 in  the Grants Mineral Belt  (EPA75),  but we do not  believe seepage from set-
 tling  ponds  to  be a  factor.
      Infiltration of  water discharged  to  ephemeral stream  courses  was  not
 calculated  separately.   It was  combined  into  a  lumped  term  incorporating
 infiltration and  evaporation.   Both  losses  are, in  part,  a function  of sur-
 face  area.   Infiltration takes  place  primarily  in the basin.   When  three
 mines  are operating, 22.7 km  of  perennial  stream is created and  extends  into
 a  portion of the  basin.  Infiltration  of the mine effluent adds  primarily to
 the amount  of water in  storage  in the  alluvium, versus acting as  a source of
 recharge  to  the deeper,  consolidated  strata.
     As  with many of the intermontane  basins  in  Wyoming,  water  in the  South
 Powder River  Basin is primarily groundwater  recharged by sporadic  runoff  from
 limited  precipitation (Ke77),   Some  stock  ponds that  collect surface  runoff
 are supplemented  by  groundwater from  wells or springs.  Mine water  discharged
 from  one underground mine  is used  to  irrigate approximately 65 hectares of
 native grass, alfalfa, oats, and  barley.  In general, groundwater  is not  used
 for  irrigation (Ho73).   Groundwater  use for  domestic  supplies  is  largely
confined  to the Dry  Fork of the Cheyenne  River (Ke77). The number of wells is
close  to  a  density of one per 400 ha (Ke77).  Typical wells are completed in
the alluvium and yield less than  1GCH /min.

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                                                                        3-90

       Geological  formations  in  the  southern portion of the Powder River Basin
  include in descending order and increasing age; the  1)  Alluvium,  2) Wasatch
  Formation, 3} Fort Union  Formation,  4} Lance Formation,  5)  Fox Hills Forma-
  tion, and 6)  older rocks  too deep  to be affected by uranium mining (NRC78c).
  Table 3.28 shows  the  well  depth for each formation, anticipated well yields,
  and the total dissolved  solids content in the  vicinity  of an active uranium
  mining and milling project in the South Powder River Basin.
       Water quality in  the Wasatch and Fort Union Formations ranges  widely and
  appears to  correlate with  the  permeability of  the  water-bearing  sand  and
  proximity  to  outcrops.   No relation  of water quality to  depth  is  apparent.
  Analyses of water from Cenozoic rocks show dissolved so'iids ranging  from less
  than 100 to more than  8000 mg/i (Ho73).   Of the  258 analyses performed by the
  US&S., 55 showed  dissolved  solids less than 500 mg/£ , 13J  less than  1000 mg/£ t
  and 125 more  than 1000 mg/i .   Sodium,  sulfate,  and bicarbonate are the dom-
  inant  ions,   and  water  is   usually  excessively  hard.   Iron  is  character-
  istically  a  problem   in  water  from  the  Wasatch  and  Fort Union  Formations
  (Ho73).    Element  distributions  show considerable  variability  due  to  clay
  lenses in  the sandy units  (NRC78c).   The clays act  as  barriers  to groundwater
  movement and preferentially concentrate  some  elements.   Table  3.29  shows  the
  ambient  groundwater quality  in the  immediate area  of three active mills  in
\ the South  Powder River Basin.
                                                                      3
     •  In  the  Wyoming model  mine  sub-basin,  total  inflow  equals 9 m /min  or
  4.73 x  10   m /yr,  and total  annual  infiltration  loss equals  4.65 x 10   m
  (calculated  in Appendix  H).  Restated,  98.2  percent of the discharge  infil-
  trates and  the remainder  evaporates.
       Infiltration  of  4.65 x 10   m /yr  is  not  likely to continue  for  the  full
  duration of mining unless the  bedrock  strata  have  the  same or  similar perme-
  ability  as the  alluvium  and (or) there  is  an extensive  zone of unsaturated
  alluvium to  provide  storage.   The   alluvium  in  the  Wyoming  study  area  is
  concentrated  along  the stream axes,  is  relatively  thin,  and is  underlain  by
  less  permeable  bedrock  strata.  It   is  probable  that  a  zone of saturated
  alluvium will  gradually  develop and  extend downstream as mine  discharge con-
  tinues.  Recharge  from the alluvium  to  the  underlying Wasatch or Fort Union
  Formations  will   occur but  at  a low  rate compared to  infiltration.  Water
  quality  in the alluvium is highly variable  (Table 3.29); it may or may not  be
  affected  by  mine  drainage.   Adverse  impacts,  if  any,  are likely  to  be a
  result of uranium, sulfate, and mobile elements.

-------
                    Table  3.28  Northeastern  Wyoming  groundwater sources
Geologic Period
Quaternary >
Tertiary

Cretaceous





Jyrassic
Triassic
Pennsylvanian
Mississippian
Qrdovician
Cambrian
Aquifer
Alluvium
Wasatch
Fort Union
Lance
Fox Hills
Mesaverde
Cody
Frontier
Dakota
Sundance
Spearfish
Minnelusa
Pahasapa
Bighorn
Flathead
Depth Range
of Wells, m
3-30
12-300
45-180
45-365
210-700
12-915
30-335
20-610
75-1830
120-210
6-275+
75-1980
150-2320
0-60
20-1800
Anticipated Well Yield, jtpm
Common
20-945
4-150
4-110
4-190
75-260
57-150
4-20
4-20
95-380
4-20
4-115
95-950
380-9460
3785
760
High
1140-2270
380-2370
380
1900
760-1900
225-265
380-7&0
380-1135
760-3410
95
380-760
1860-7470
26,500-35,600
3785

Total Dissolved
Solids, mgA
106-7340
160-6620
484-3250
450-3060
1240-3290
550-1360
6392-12,380
390-2360
218-1820
894-2310
2590
255-3620
290-3290
427-3219
124
Source;  NRC78b.

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                                                                      3-92
Table 3.29  Groundwater quality of wells sampled by the three major
            uranium producers in the South Powder River Basin, Wyoming
Parameter
     U)
reference Ke77.
     (b)
                            Range of Concentration Reported
            Kerr-McGee
                              (a)
TVA
                                        {b}
Exxon
PH
Spec. cond.
ymhos/cm
Ca
Mg
Na
HC03
SO,
Cl
Zn
Fe
Ba
Radium (pCi/jt)
Uranium (mg/i)
7.4-8.0

210-1100
28-343
8-81
5-71
30-380
28-980
<5-57
0.006-18.0


0.41 - 5.18
< 0.002- 2.3
7.4 - 8.5

250-1300
10-200
2-80
10-300
70-110
8-1000
11-25
0.03 -3
0.2 -20

0.2 -18
0.002-60
7.3-8.1

290-600
26-150
1-13
54-121
90-412
58-575
6-16
ND- 0.14^
0.01- 1.64
ND- 0.05
0.4 -12.0
0.0004 - 0.21
     (c)
     (d)
Shallow wells up to 61 meters depth, Tables 2.6-7 through  2.6-10 of
e Ke77.
From Figs. Cl and C3 of reference NRC78b.
Table 2.12 of reference NRC78d.
ND:  Not detectable.

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                                                                       3-93
      An actual  example  of this  saturated front developing  and  moving down-
 gradient is present at  the  Kerr-McGee Nuclear Corporation's  Bill  Smith Mine
 in South  Powder River Basin  (Ke77).   The mine discharges to  a  tributary of
                                      3
 Sage  Creek at a rate  of about 1.7  m /min.   From the period  January  1974 to
 late  1976, a  flow front  23 km long developed  as a result of infiltration into
 the sandy alluvium.  The  discharge  water maintains a high groundwater level
 in the  stream  bed.  Unfortunately,  no information is available on the geo-
 metry of the stream channel  to evaluate the volume  of  water that  has infil-
 trated   in  the  three-year period  or  on  any  water quality changes  that have
 occurred.
      In summary,  additional  field  data  are  needed  to  properly address  the
 water quality effects  of infiltrat.on.   Both  theory and at  least  one field
 example indicate extensive Infiltration  of effluent  containing at  least some
 mobile  stable and  radioactive contaminants.    Therefore,  we  recommend addi-
 tional  field  investigations to determine,  at the minimum, any hydraulic  and
 water quality  effects of mine  discharge on shallow  aquifers and the influence
 of dewatering  on regional water  levels and water quality,  regardless  of pre-
 existing or anticipated  local  water  use patterns.

 3.3.4   jases_and Dusts  from Mining  Activ11ies
      Dusts  and  toxic  gases  are   generated  from  routine mining operations.
 Combustion products are produced  by large diesel and  gasoline-powered  equip-
 ment  in the mine and by  trucks transporting  the  overburden,  ore, and  sub-ore
 from  the   pit   to  storage  pile   areas.   Dusts  are  produced by   blasting,
 breaking,  loading, and  unloading  rock and ore  and by haulage trucks  moving
 along dirt roads.  Finally, Rn-222  will  emanate from exposed  ore  in  the  pit
 and from the  ore as it  is  broken, loaded, and unloaded.  These sources will
 be  discussed individually.

 3.3.4.1  Dusts and  Fumes
     Most vehicular emissions  are  from the combustion  of  hydrocarbon fuels in
 heavy-duty,  diesel-powered  mining  equipment.    Surface  mines  produce con-
 siderably more emissions  than  underground mines,  since the overburden must be
 removed  before  the  ore  can  be mined.   The  principal emissions  are   parti-
culates, sulfur  oxides, carbon monoxide, nitrogen  oxides, and hydrocarbons.
The quantity of  these  combustion  products released to the atmosphere depends
on the number, size, and types of  equipment used.

-------
                                                                       3-94

     The EPA estimates the following emissions from mining  1350 MT of  ore per
day from a surface mine  (Re76).
                                        Emissions per Operating Day, kg/d
Pollutant                     Mining Operations             Overburden Removal
Participates                       17.0                            18.9
Sulfur oxides                      35.4                            39.3
Carbon monoxide       .            294.2                           327,4
Nitrogen oxides                   484.6                           538,4
Hydrocarbons                       48.4                            53.8
Assuming a 330 opt rat ing -day -year (Ni79), we adjusted these emission ,'ates to
ore production for the average surface mine (1.2 x 10  MT/yr) and tha average
large  surface mine  (5.1 x  10   MT/yr)  as described  in Sections  1.3.1  and
3.3.1.  Table  3.30  shows the  total  airborne  combustion  product  emissions.
These  estimated  emission  rates  are  somewhat  higher  than  rates  previously
suggested by the U.S. Atomic Energy Commission (AEC74).
               Table 3.30  Estimated air pollutant emissions from heavy-duty
                           equipment at surface mines

Pollutant
Participates
Sulfur oxides
Carbon monoxide
Nitrogen oxides
Hydrocarbons

Average Mine^ '
3
7
55
91
9
Emissions, MT/yr^a'
Average Large Mine
14
28
235
387
39
     ^a'Based  on  (Re76)  and 330 operating days per year (Ni79).
        Ore  production = 1.2 x 105 MT/yr.
                                 5
        Ore  production = 5.1 x 10  MT/yr.

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                                                                       3-95
      Oust  is  produced  from  blasting,  scraping,  loading, transporting,  and
 dumping ore, sub-ore, and  overburden.   Additional  dust is produced  when  the
 ore  is  reloaded  from the stockpile  for transportation  to  the mill.   Dust
 emissions  vary  widely,   depending  upon  moisture  content,  amount of  fines,
 number and  types  of  equipment  operating,  and climatic conditions.   Because
 ore is usually  wet,  the  relative  amounts of  dust produced from mining  and
 handling  it are usually small.  We  selected the following emission factors
 from those  suggested by  the EPA  for the  above listed mining activities  (Hu76,
 Ra78, Da79):
                Blasting  - 5 x  Iff4  kg  dust/MT
                Scraping  and bulldozing * 8.5  x  10   kg  dust/Iff
                Truck loading » 2.5  x ID"2 kg  dust/MT
                                     „?
                Truck dumping - 2 x  10    kg dust/MT

      We applied these emission  factors  to  the ore,  sub-ore, and overburden
 production  rates  of  the average mine  and average  large  mine and estimated
 average annual  dust emissions  for  these mining activities (see Table  3.31).
 These are  probably maximum  emission  rates  because  blasting  is  not  always
 required, and  some emission factors appear to  have been based upon data from
 crushed  rock operations,  which  would contain  more fines  than  rock removed
 from surface mines.  One-half the  emission factor values  were applied  to  ore
 and  sub-ore because they are usually wet, except when  reloading ore  from  the
 stockpile,  in  which case it is  assumed  to have dried during the 41-day resi-
 dence  period (Section  3.3,1.2),
      The  movement  of  heavy-duty haul  trucks  is  probably  the largest  single
 source  of dust emissions at surface mines.  An emission factor (EF)  for this
 source  can  be computed by the following  equation (EPA7?b),

      EF - 2.28 x Itf4  (s)   M   365_w (TF} (f)            (3>2)
                            \48J   365™
where,

     EF - Emission factor,  MT/vehicle kilometer traveled (MT/VKmt),
      S = Silt content of road surface,  percent,

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                                                                      3-96
      V  = Vehicle velocity,  kmph [Note: This tenn becomes  l
          for  velocities  less than 48 km/hr (EPA77b, DA79)]}
      W  = Mean annual number of days with 0.254 mm or more rainfall,
      TF  = Wheel correction factor, and
      f  = Average  fraction of emitted particles  in  the <30  vm diameter sus-
          pended  particle  size   range;  particles  having diameters  greater
          than 30 Mm will settle rapidly near the roadway.
Values  selected for  these  terms  in  the  solution  of Equation  3,2  are  —
      S = 10 percent (Da79),
      V  =  32 km/hr  for  heavy-duty  vehicles and 48 km/hr  for  light vehicles
                                                  o
          (therefore, the velocity term is (32/48)   and (48/48),  respectively),
      W = 90 days (EPA77b),
     TF = 2.5 (Da79) (heavy-duty vehicles only), and
      f  =  0.60, since the  weight percent  of particles of  less than  30  vm
          and greater  than  30 u m  in diameter  is generally  considered  to
          be 60 and 40 percent, respectively (EPA77b).

Substituting these  values into  Equation  3.2  yields 1.15 x 10   MT/VKmT and
          _3
1.03 x  10   HT/VKmt for  the  emission  factors of heavy-duty haul trucks and
light duty vehicles, respectively.
     Table 3.31  shows estimated dust emissions for  the  movement of heavy-duty
haul trucks  using the following information:

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Table 3.31  Average annual dust emissions from mining activities
Dust Emissions, MT/yr
Mining Activity
Blasting
Scraping/bul Idozing
i
Truck Loading
Total at Pit Site
Truck Dumping
Reloading stockpiled ore^6j
Total at Pile Sites
Vehicular dust^ '
Wind suspended dust
from storage piles
Average Mine^3'
Ore
0.03
1.5
1.53
1.2
1 3.0
4.2
14
10
Sub-ore^
0.03
NA
1.5
1.53
1.2
NA
1.2
14
3
Overburden
3.0
51
150
204
120
NA
120
304
30
Average Large
Ore(c}
0.13
NA
6.4
6.53
5.1
13
18.1
59
44
Sub-ore^
0.13
NA
6.4
6.53
5.1
NA
5.1
59
10
Mine(b)
Overburden
20
340
1000
1360
800
NA
800
2020
94
     ^a'Based on annual production rates of 1.2 x 10  MT of ore and sub-ore and 6.0 x 10  MT of overburden.
     ^ 'Based on annual production rates of 5.1 x 10  MT of ore and sub-ore and 4.0 x 10  MT of overburden.
     (0
     (d)
     (e)
     (f)
Assumed wet.
NA - not applicable.
Assumed dry.
Dust emissions from heavy-duty vehicular traffic along ore, sub-ore and overburden haul roads.
                                                                                                               u»
                                                                                                               UD

-------
                                                                       3-98
      EF - 1.15 x 10"3 MT/VKmt,
      Truck capacities - 31.8 MT for ore and sub-ore and
                         109.1 MT for overburden (Da79)f
      Round-trip haul  distance = 3.2 km to ore and sub-ore piles
                                 and 4.8 km to overburden dump,  and
      Annual  production1 rates -  given in Section 3.3.1 and in  the
                                 footnotes of Table 3.31.

      Additional  dust  emissions will  occur from  the  movement of  light-duty
 vehicles  along access  roads.  Using the emission factor derived above (1.03 x
   _o
 10"   MT/VKmT) and  assuming  that there are  24  km of access roads  traveled  4
 times a  day  for 330  operating days  per  year, about  33 MT of dust  will  be
 produced  from  this  source  annually.   Emissions  during  haulage  road  main-
 tenance is  relatively  small  and will  not  be  considered.
      Table  3.31  also  shows average  annual  dust  emissions from wind  erosion  of
 overburden,  sub-ore»   and  ore  piles  at the model  surface mines.  For  these
 computations,  we assumed the model  overburden  pile to  be that of  Case  2 and
 in  the shape of  a  65-m  high  truncated  cone  (Table  3.11).  The same was
 assumed for the average mine,  except the  pile  height  was 30 m.   The  sub-ore
 piles of  both mines  were  assumed  to  have a  truncated cone configuration
 (Table  3.20).  The same configuration  was  also  assumed  for the  ore  piles, but
 the  pile  heights were 9.2  m  for the  average  large mine and  3.1 m  for the
 average mine  (Table 3.17).
      Emission  factors, computed  in Appendix I,  are 0.850 MT/hectare-yr for
 overburden  and  sub-ore  piles  and  0.086  kg/MT  for the  ore  stockpiles. The
 first emission factor  was  multiplied  by  the  overburden and average  sub-ore
 pile  areas;  the  second  factor was multiplied  by  the  annual  ore production.
      In computing the  Table  3.31 dust  emissions, we assumed no  effective dust
control program  and  that  there was no vegetation  on  overburden  and  sub-ore
 piles.  Haul_ roads  are normally sprinkled  routinely during  dry periods, and
stabilizing  chemicals are  applied  primarily  to  ore  haul roadways  at some
mines.  Sprinkling  can reduce dust emissions along haul  roads by 50 percent,
and  up to 85  percent  by  applying  stabilizing  chemicals  (EPA77b,  Da79).

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                                                                       3-99

      The dust emissions from  vehicular  traffic (Table 3.31) (transportation)
 were summed  with  those produced  by light  vehicular  traffic  (33  MT/yr)  and
 considered  as one  source of  emissions.   Concentrations of contaminants in  the
 dust are unknown.   Some spillage  of ore and  sub-ore along haul  roads will
 undoubtedly raise uranium  levels  in  roadbed  dust.  As  an  estimate,  uranium
 and  daughter concentrations  in the  dust  were considered  to  be twice  back-
 ground,  8  ppm  (2.7  pCi/g)»  while concentrations  of  all other  contaminants
 were considered to be  similar  to  those  in overburden  rock  (Section  3.3.1.1,
 Table 3.16).   Table  3.32  shows  the annual  emissions  computed  with  these
 assumptions.
      Table  3.33  lists   annual  contaminant emissions  from mining  activities
 (scraping,  loading,  dumping, etc.) according  to  source location, at  the  pit
 and  at  the  piles.   Contaminant  emissions  were computed  by multiplying  the
 total  annual  dust  emissions  at  each  pile  (Table 3.31)  by the  respective
 contaminant  concentrations   in  each source  —  overburden (Section 3.3.1.1.;
 Table 3.16),  sub-ore  (Section 3.3.1.3; Table  3.19) and ore  (Section  3.3.1.2;
 Table 3.19).   Contaminant emissions at the  site  of the  pit  were computed  by
 multiplying  the total  annual dust  emissions of ore,  sub-ore, and  overburden
 (Table 3.31)  by their  respective  contaminant  concentrations.   The  three pro-
 ducts  of the multiplication  were  then  summed   to give  the  values in  the 4th
 and  8th  data  columns of  Table  3.33.   The health impact  of the sources  at each
 location will be assessed separately  in Section 6.1.
      Table 3.34 lists annual contaminant emissions  due  to wind  suspension and
 transport of dust.  These values were computed  by multiplying the annual mass
 emissions  (Table  3.31)  by   the   contaminant   concentrations  in  overburden,
 sub-ore,  and  ore listed in  Sections 3.3.1.1,  3.3.1.3, and 3.3,1.2,  respec-
 tively.  The  uranium  and uranium daughter concentrations  were also multiplied
 by an  activity  ratio  (dust/source) of 2.5  (Section 3.3.1.2).  Although some
 metals may  also be  present  as secondary deposits,  it was believed  that there
 were  insufficient data to justify multiplying their concentrations by  the 2.5
 ratio.

 3.3.4,2   Radon-222 from the Pit, Storage Piles, and Ore  Handling
     Rn-222 will be released from the following sources during  surface mining
operations:

-------
                                                                 3-100
          Table 3.32   Average annual emissions of radionucl ides (yd)
                       and stable elements (Kg) from vehicular dust at
                       the model surface mines
Contaminant
Arsenic
Barium
Copper
Chromium
Iron
Mercury
Potassium
Manganese
Molybdenum
Lead
Selenium
Strontium
Vanadium
Zinc
Uranium-238 and
each daughter
Thorium-232 and
each daughter
Average Large
Surface Mine^3'
20
630
39
<111
13,030
<17
15,200
1,050
5.4
48
4.3
330
220
43

5,860

2,170
Average
Surface Mine^
3.3
106
6.6
<19
2,190
<2.9
2,560
177
0.9
8.0
0.7
55
37
7.3

990

370
(a)
(b)
Mass emissions = 2,170 MT/yr.
Mass emissions = 365 MT/yr.

-------
Table 3.33     Average annual  emissions of radionuclides (yd")  and stable elements
               (kg) from mining activities at the model  surface mines
Average Surface Mine^
Overburden
Contaminant Pile Site
Arsenic
Barium
Cobalt
Copper
Chromium
Iron (
Lead
Magnesium
Manganese
Mercury
Molybdenum
Nickel
Potassium
Selenium
Strontium
Vanadium
Zinc
Uranium-238 &
each daughter
Thorium-232 &
each daughter
1.1
35
NR(b)
2.2
<6
720
2.6
NR
58
<1
0.3
NR
840
0.2
18
12
2.4

1,800

120
a)
Sub-ore Ore Pit Site
Pile Site Pile Site
0.10
1.1
0.02
0.07
0.02
19
0.09
4.2
1.2
ND^
0.14
0.02
30
0.13
0.16
1.7
0.04

120

2.4
0.36
3.9
0.07
0.26
0.08
66
0.33
15
4.0
ND
0.48
0.08
105
0.46
0.55
5.9
0.12

2,990

42
2.1
62
0.05
3.9
<10
1,270
4.7
11
102
<1.6
0.86
0.06
1,500
0.74
31
25
4.2

4,300

220
Average Largje Surface Mine^
Overburden
Pile Site
7.2
232
NR
14
<41
4,800
18
NR
388
<6.4
2.0
NR
5,600
1.6
120
80
16

12,000

800
Sub-Ore Ore Pit Site
Pile Site Pile Site
6.44
4.7
0.08
0.31
0.10
80
0.40
18
4.9
ND
0.59
0.10
128
0.56
0.66
7.2
0.15

510

10
1.6
17
0.29
1.1
0.36
284
1.4
63
17
ND
2.1
0.36
453
2.0
2.4
26
0.52

12,900

180
13
406
0.21
25
<70
8,360
31
46
672
<11
4.9
0.26
9,850
4.2
206
154
28

25,700

1,440
      (b)
      (c)
'Mass  emissions from Table 3.31.

 NR -  Not reported.

 ND -  Not detected.
                                                                                                                U)
                                                                                                                 I
o

-------
Table 3.34
    Average  annual  emissions  of radionuclides (yCi)  and stable elements


         in  wind  suspended' dust at the model  surface mines
Average Large Surface Mine
Contaminant
Arsenic
Barium
Cobal t
Copper
Chromium
Iron
Mercury
Potassium
Magnesium
Manganese
Molybdenum
Nickel
Lead
Selenium
Strontium
Vanadium
Zinc
Uranium-238 &
each daughter
Thorium-232 &
each daughter
Overburden Sub-Ore
Pile Pile
0.85
27
NR(a)
1.7
<4.8
564
<0.75
660'
NR
46
0.24
NR
2.1
0.19
14 ,
9.4
1.9

1,410

94
0.86
9.2
0.16
0.61
0.20
157
ND(b)
250
35
9.6
1.2
0.20
0.78
1.1
1.3
14
0.29

1,000

20
Ore
Stockpile
3.8
40
0.70
2.7
0.88
690
ND
1,100
154
42
5.0
0.88
3.4
4.8
5.7
62
1.3

31,300

440
Averaqe Surface Mine
Overburden
Pile
0.27
8.7
NR
0.54
<1.5
180
<0.24
210
NR
15
0.08
NR
0.66
0.06
4.5
3.0
0.60

450

30
Sub-Ore
Pile
0.-26
2.8
0.05
0.18
0.06
47
ND
75
11
2.9
0.35
0.06
0.23
0.33
0.39
4.2
0.09

300

6.0
Ore
Stockpile
0.86
9.2
0.16
0.61
0.20
157
ND
250
35
9.6
1.2
0.20
0.78
1.1
1.3
14
0.29

7,100

100
- Not reported.


- Not detected.
                                                                                              o
                                                                                              ro

-------
                                                                       3-103

      I.   Ore,  sub-ore,  and  overburden  during  rock  breakage  and  loading
           in  the  pit and  unloading  on the  respective piles.   (Since  rock
           breakage,  loading,  transporting, and  unloading  usually occur  in
           a short  time period,  they are considered  one release.)
      2,   Ore during  reloading  from the  stockpile after a 41-day  residence
           time (Section  3.3.1.2).
      3.   Exposed  surfaces  of  overburden,  ore, and  sub-ore  in  the active
           pit area.
      4,   Overburden,  ore,  and  sub-ore  pile  surfaces.

 The annual  quantities  of  Rn-222 released from  sources  1  and  2 above were com-
 puted using the  following factors  and assumptions:
      1.   Rn-222 is  in secular equilibrium with U-258.
                                                                 3
      2.   The density  of  ore, sub-ore,  and overburden  is 2,0 MT/m ,
      3.   Annual  production rates  of ore,  sub-ore, and overburden  are those
           given  previously  in  this Section and in footnotes  "a"  and "b" of
           Table  3.31.
      4.   All  Rn-222  present,  Q.OQi65  Ci/m   per  percent  U30g,  Is available
           with an  emanation coefficient of  0.27,   [Although an emanation co-
           efficient  of 0.2  1s commonly  used (N179), recent emanation-coeffi-
           cient  measurements for   950  samples of  domestic uranium  ores  by
           the  Bureau  of  Mines  indicate a  value  between 0.25 and  0.3 to be
           more appropriate  (Au78,  Tanner, A.B., Department of Interior, Geo-
           logical Survey, Reston,  VA, 11/79, personal communication).
           Therefore, an emanation  coefficient  of 0.27 was selected.]
      5.    The  quantities  of lUOg  present in ore, sub-ore, and overburden are
           0.10,  0.015, and 0.0020  percent, respectively.
Substituting  these values into  the following  equation  yields  the  Rn-222 re-
leases  given  in  Table 3.35  for the average  mine  and the average large mine.
                                  0.00565   C1
Rn-222 (Ci/yr)  =  (Percent U^g) I  ^3 x  percer,J   (0.27)    fu "'/     (3.3)

                  X (Production Rate,  MT )
                                       yr
     The quantities of  Rn-222 that emanate from exposed overburden, ore, and
sub-ore surfaces  in the pit were estimated by the following method.  Exposed

-------
                                                                       3-104

 surface  areas of ore and  sub-ore are assumed  equal  since  equal  quantities of
 each  are mined.  The computation  assumes  an ore  plus  sub-ore  zone  12 m thick
 (h^  in  the  shape  of  a  truncated cone  with  45 degree  sloping sides  (Fig.
 3.14),   The radii of  the zone,  r,,  and r^,  can  be  computed  using  the following
 equation from  the  relationship  r~  = r.  + 12 and  the volumes  of ore  plus
                                                  fi  *%              Si *3
 sub-ore  mined  in a  2,4 year period  —  1.22  x 10 nr  and  2.8  x 10V at  the
 average  large mine  and average mine, respectively (the bulking  factor is  not
 considered in  computing the pit volume),

                                               ?        9
          V (ore + sub-ore zone)  = 1/3 •„ hj (ri "f"rir2"l"r? )       (3.4)

     The computed radii, r, and r2, were 174 m and 186 m at the  average  large
 mine  and 80  m  and   92 m  at the average mine.  The  surface areas (S.)  of
 exposed  ore  and  sub-ore  fn  the  pit are then  one-half  that  given  by  the
 equation,

          SA -  1/2TT   (dj + d2)(slant  height) +* r^,       (3.5)

where  d, and  d,  are the  diameters   related to  r,  and  r,,.   Exposed  surface
 areas  of ore  and  sub-ore were  computed  to  be  equal   and 57,170  m  at  the
                               o
 average  large mine and 14,650 m  at the average mine.
     The  shape  of the overburden   zone was  assumed to  be the same as the ore
and  sub-ore  zone (Fig. 3.14).   The  thickness,  fu,  and radius,  r~» of this
zone can be computed using the following equation with  the relationship, r, =
                                               7 "J                fi  *?
 r~  +  h2» and knowing  the  volume—4.8  x  10 m  and 7.2  x   10 m --at the
average  large mine and average mine,  respectively.

          V (overburden) = 1/3 ir h2 (fg2 + r2r3 * r%2^        (3-6J

Since r« was computed above to be   186 m at the average  large mine and 92 m at
the average mine, Equation 3,6 becomes
          4.8 x 107_= 1.087 x 105h2 + 584h2Z + 1.047h23       (3.7)

for the average large mine, and

-------
             Ore plus sub-ore Zone
Figure 3,14  Configuration of open pit model mines.
                                                                                               O
                                                                                               Ul

-------
                                                                       3-106
           7.2 x  106  =  2.659  x  104h2  +  289  h^   +  1.047h23          (3.8)
 for  the average mine,

 Solving these equations yields  the  following  parameters:
                                                                        r2
average  large mine                  188 m              374 nt            186 m
average  mine  -                     105 ra              197 m             92 m

     The surface area  (S.)  of the exposed overburden  is  then given  by the
following equation.
          SA =  1/2w (d2 + d3)  (slant height),                   (3.9)
where  d. and  d0 are  the diameters  related  to r9 and r_.  Areas computed were
          52               52                ifa
4.68  x  10 m  and 1.34  x  10  m  for the average  large ralne  and average mine,
respectively.
     Multiplying the  exposed ore, sub-ore,  and overburden areas by their U,0fl
                                                                          u 0
contents (0.10%,  0.0152 and 0.0021, respectively) and by a Rn-222 exhalation
                   2
rate  of  0.092  ti/m  per year  per  percent U^Og*  and summing gives the  annual
Rn-222 releases shown in Table 3,35.
     The emanation  of Rn-222 from  overburden, sub-ore, and ore storage piles
                                            o
is, based on an exhalation rate of 0.092 Ci/nr per yr per percent UgOg (Ni79),
and  ore  grades of  0.002 percent,  0.015  percent, and  0.10 percent, respec-
tively.  The  surface areas used were those  computed previously for the  case 2
model  mines  and  listed  in Tables  3.11,  3.17 and  3.20.   The  areas  for the
                                                    f\ *?               R ?
average  large  mine  and average mine  are  1.1 x 10 m  and  2.2 x  10 m  for
                           52              42
overburden piles,  1.2 x 10 m  and  3.6  x  10 m  for sub-ore piles,  and 6.2 x
  32              32
10 m  and 3.6  x 10 m  for the ore  piles, respectively.   Applying these para-
meters,  the  annual   Rn-222  emissions  from  the  overburden,  sub-ore,  and  ore
piles at the average mine and average  large  mine were  computed.  Table 3.35
presents the results.
     The total  annual Rn-222 released during surface mining operations  is the
sum  of  the releases  from the sources  considered:   331 C1 from the average
mine and 1261 Ci from the average large mine.  Considering ore production and
*The  average value  of measured  exhalation  rates  at surface  uranium mines
 (N179).

-------
                                                                       3-107
           Table  3.35   Radon-222  releases  during  surface  mining,  Ci/yr
Source
Ore loading and unloading
Reloading ore from stockpile
Sub-ore loading and unloading
Overburden loading and unloading
Exposed surface of overburden,
ore, and sub-ore in the pit
Ore stockpile exhalation
Sub-o^e pile exhalation
Overburden pile exhalation
Total
Average Mine
9
9
1
9

180
33
50
40
331
Average Large Mine
39
39
6
61

691
57
166
202
1261
grade  differences,  these values agree  reasonably well with those computed by
other  procedures  (Tr79).

3,4  jJnderground Mining

3.4.1     Solid Wastes
     During  underground mining, like  surface  mining,  materials are removed,
separated according to  ore  content,  and  stored  on the  surface for various
periods  of  time  (Section 1.3.3).  These separate piles consist of waste rock
produced  from  shaft sinking operations and  from  cutting  inclines, declines,
and  haulage  drifts  through barren rock, sub-ore, and ore.  The waste rock is
similar  to  overburden  removed  at surface mines,  except much  smaller  quan-
tities  are  involved and none  are returned to  the  mine.   However,  as mining
progresses,  waste rock  is sometimes used  to backfill  mined  out areas of the
mine  and retained  beneath  the  surface.   The  ore  and  sub-ore will  also  be
similar in nature to those described previously for surface mines, as is their
potential to be  sources  of  contamination  to the environment  (Fig.  3.15).

-------
Figure 3 15  Potential sources of environmental contamination from active underground uranium mines
                                                                                                             o
                                                                                                             00

-------
                                                                       3-109
 3.4.1.1   Waste Rock Piles
      Much smaller  quantities of  waste  rock accumulate  at underground mines
 than overburden  at surface  mines.   The weight  ratio of  waste rock  to  ore
 depends mainly upon the size, depth, and age of the mine.  During the initial
 mining  stages, all  material  removed  is waste  rock.   As  entry  into  the  ore
 body occurs  and  ore mining  begins, the quantity  of waste  rock  removed  per
 metric  ton of ore  decreases  sizably.   Once in the  ore  body, as little waste
 rock as  possible .is  mined.  The ratio of  ore to waste  rock  removed  from
 underground  mines varies  considerably.   At  seven  presently  active underground
 mines,  the ore to waste rock ratio varies from  1.5:1 to  16:1, with an average
 ratio  of  9.1:1   (Jackson,   P.O.,  Battelle  Pacific   Northwest  Laboratory,
 Richlandj WA, 12/79, personal communication).   As  future mines become larger
 and   deeper,  the   overall  ore to waste  rock  ratio will  probably  decrease.
      Since the annual  average ore capacity  of underground mines was 1.8 x  10
 MT in  1978  (Section 1.3.1),  the  average of the 305 underground mines  would
 have produced  2.0  x  10  MT of  waste  rock during that year, assuming  the
 average  9.1:1  ore to waste  rock ratio.   This will  be  considered the  pro-
 duction  rate  of  the "average underground  mine."  Like  surface  mines,  rela-
 tively  few  of the  305 active  underground mines account  for a  significant
 portion of  the  total  ore produced  by  the  underground method.   Also,  future
 underground  mines are  expected  to  have larger  capacities  than many of  the
 current mines  (Th79).   Therefore,  a  second  underground  mine  will  be con-
 sidered,  which is defined as  the "average  large mine."  Its  annual  ore pro-
 duction rate is assumed to  be 2 x 10   MT,  the average  ore capacity of five
 large  underground  operations (Ja79b,  TVA79,  TVA76,  TVA78a,  TVA78b).   The
 quantity  of waste  rock  removed  annually will  be 2.2  x  10   MT,  assuming  the
 ore  to  waste  rock  ratio to be the  same as for the average mine.   Assuming  the
                                              3
 density of waste  rock  to be about 2.0 MT/m  and  a  bulking factor of 1.25
 (Burris,  E.,  Navajo  Engineering  Construction Authority, Shiprock, N.M.,  2/80,
 personal  communication),  the  average mine and average  large mine  will  produce
                                         33             43
 waste rock  at an  annual rate  of 1.3 x 10   m  and 1.4  x 10  m  ,  respectively.
 Since waste  rock  is  not presently  used to backfill mined-out  areas, this rate
 of accumulation will continue for the  life of  the mine, which  is  assumed to
 be the  same as that  for an open  pit mine, 17 years.
     Table 3.36 lists estimated  average  surface areas  of  the  waste  rock  piles
during  the  lifetimes of  the  two  mines  defined  above.   The following para-

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                                                                       3-110
 Parameter _         Average HI ne _ Average Large Mine
Waste rock production rate, MT/yr
Rock density, MT/m
Bulking factor
Waste rock volume, m /yr
Active mine life, yr
Pile height, m
2.0 x 103
2.0
1.25
1.3 x 103
17
6
2.2 x 104
2.0
1.25
1.4 x 104
17
12
     These  estimated areas  assume  no backfilling  and  that the piles are  on
 level  terrain.   Because waste  rock  is  sometimes  used  to backfill and  is  often
 dumped   into  a   gorge  or   ravine,  these  surface  areas  represent  maximum
 conditions,
     The  mineralogy,  physical  characteristics, and composition of waste rock
 from underground mines  are assumed to be  identical to the  overburden removed
 from  open  pit   mines  (Section 3.3.1.1).   Also,  reclamation  procedures for
 waste  rock  piles at underground mines  should be  similar to  those described  in
 Section 3.3.1.4  for overburden dumps.

 3.4.1.2   Ore Stockpiles
     Because ore is  often stockpiled at the mine and/or at the mill, it be-
 comes  a  potential source  of contamination to  the mine environment during the
 storage  period.   These  piles will be  smaller  than  the waste rock piles, but
 the concentration of  most contaminants in the ore-bearing  rock will  be much
 greater.
     Ore  stockpile residence  times  can  vary  considerably  with  time  and ore
management.  Residence  times  commonly  range from a few days to a few months.
The same  residence time will be assumed for underground mines as was selected
above  for surface mines,  41 days.   Assuming  a  330 operating-day-year  and a
 1.25 bulking factor, the ore stockpiles of the average mine and average large
                          q             3
mine will contain 1,400 m  and 15,500 m   of  ore, respectively.  The surface
areas  of  the ore stockpiles were computed using these  volumes  and assuming
3.1  m   high rectangular  piles  (NRC78a).   Table 3.37  lists  the  estimated
surface areas.

-------
                                                                       3-111
                Table  3.36   Estimated  average  surface  areas  of  waste
                            rock  piles at  underground  mines

Mine Size
• (b)
Average minev '
Average large mine
Average
Accumulation,^3' m
1.1 x 104
(c) 1.2 x ID5
Surface Area
2
of Pile, m
2,700
14,100
Surface
of Pad, m
2,460
12,800
Area
2


      *  ^Assumes average  volume of waste rock accumulated during 17-yr. mine
 life  with no backfilling  (1/2 total volume accumulation).
      ^Annual waste rock production = 2.0 x 10  MT.
      f c\                                       4
      k  'Annual waste rock production = 2.2 x 10  MT.
      Note.—Waste rock piles are rectangular with length twice the width
 and sides sloping at 45°  (Fig. 3.8 a).
          Table 3.37  Estimated surface areas of ore stockpiles
                      at underground mines
Mine Size
Average
Average
(a7
(b)
(c)
Steady
Accumulation
State
.(•> m3
mine(b) 1,400
(c)
large minev ' 15,500
Assume
Annual
Annual
41-day residence
ore production =
ore production =
time
1.8
2 x
*
x 104 MT.
105 MT.
Surface Area
of Pile, m2
680
5,800

Surface
of Pad,
620
5,480

Area
™2


     Note.—Ore stockpiles are rectangular with length twice the width and
sides sloping at 45° (Fig. 3.8 a).  Pile height is assumed to be 3.1 m
(NRC78a).

-------
                                                                       3-112
     The  mineralogy, physical  characteristics,  and  composition  of ore  from
underground mines are assumed to  be  identical  to the  ore  removed  from  surface
mines  (Section 3.3.1.2).  The UgOg  grade  of ore may average  somewhat higher
from  underground mines  than from  surface  mines.   However, a grade  of  0.1
percent  U,0g probably approximates  reasonably well  the ore reserves  minable
by  the underground  method  (DOE79).   Uranium  and  its decay products  in air-
borne  dust  from these  ore piles will  be  concentrated  by a  factor  of  2.5
(Section 3.3.1.2).

3.4.1.3   Sub-Ore Plies
     The  quantity  of sub-ore rained  at an undetground  mine,  as at a  surface
mine,  is considered to be about equal to the quantity of ore mined, 1.8 x  10
                                   5
MT  at  the  average  mine and 2 x  10  MT at the dverage  large mine.  Assuming
                                      •j
sub-ore to  have  a  density of 2.0 MT/m  and after removal a bulking factor of
1.25,  the  average volume  of  sub-ore  to  be  on the  surface during the 17-yr
operational life of the average mine and average large mine will be 9.6 x 10
 O              £  -5
m   and 1.1  x 10  m , respectively {i.e., one-half the  total of 17-yr accumu-
lation).
     Although  sub-ore  is often  placed  on top of  piles  of previously mined
waste  rock  (Perkins,  B.L.,  New  Mexico Energy  and  Minerals  Department, Santa
Fe, NM, 12/79, personal  communication), we assumed  separate rectangular piles
in  computing  the surface areas  of the piles  at  the model mines.   Table 3.38
lists  the estimated surface and pad areas of the sub-ore piles.  These compu-
tations were based on pile heights of 6 m at the average mine and 12 m at the
average large mine.
     At underground mines,  the  cutoff grade ranges from 0.02 to 0.05 percent
ILQg,  yielding an  average  sub-ore  grade  of  0,035  percent U,0g  (99  pd"/g)
(Perkins, B.L.,  New Mexico Energy  and Minerals Department,  Santa  Fe, N.M.,
12/79,   personal  communication).   The mineralogy,  physical  characteristics,
and other constituents of  sub-ore from underground mines are  assumed  ident-
ical to the sub-ore removed  from surface  mines (Section 3,3,1.3).

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                                                                       3-113
           Table  3.38     Estimated  average  surface areas  of sub-ore
                          piles  at underground  mines

                          Average             Surface Area        Surface Area
 Mine Size      	Accumulation,^8* m	of  Pile, m	of Pad, m
Average mine* '
Average large mine^0'
9.6 x
1.1 X
104
106
18,800
104,900
17,700
99,400
      ^One-half  that which will accumulate  during  the  17-yr mine life.
      *  'Annual  sub-ore  prodyction =  1.8 x  10 MT.
      tr\                                     c
      ^  'Annual  sub-ore  production -  2.0 x  10 MT.
      Note.—Sub-ore  piles are rectangular  with  length twice the width and
 sides sloping at  45° (Fig. 3,8a).

 3.4.2  Mine Water Discharge

 3.4.2.1   Data  Sources
      Information  concerning  the amount and  quality of  water discharged from
 underground uranium  mines in  New Mexico  is  from  field surveys conducted 'in
 1975  (EPA75,   P.   Frenzel,  USGS,  written  communication,  1979)  and
 (Wo79j»  from  site-specific environmental  impact statements and reports, from
 NPDES permits,  and from a State study (Pe79).
      Many mining companies maintain  that permits are not required because the
 formerly  ephemeral   streams  into which  discharge  occurs  are, in  effect,  a
 result  of the discharges  and  do not meet  the definition of navigable bodies
 of  water.   Nevertheless,  the  companies have  applied  for  permits,  together
with  a request  to the courts  for a ruling concerning their necessity.
      The New  Mexico  district  office of the  U.S.  Geological  Survey  (L. Beal,
USGS, written  communication,  1979) provided discharge rate and volume for the
regional drainage systems,  namely  the  Rio San Jose, Rio  Puerco  (east), and
the  Rio Grande.   We followed  procedures  developed by  the USGS  (Bo70)  to
calculate runoff from ungaged  basins.

-------
                                                                       3-114
 3.4.2.2   Quality and quantity  of Discharge
      To estimate average or  typical  conditions  for mine water  discharge,  11
 projects in Colorado, New  Mexico,  and Utah were selected.   Table  3,39 shows
 the summarized flow and water  quality data.  The center of  current domestic
 underground mining  is  1n   the  Colorado Plateau  and  the San Juan  Basin.   In
 this  area,  there  is  an   increasing  trend toward  underground mining.   In
 Wyoming, both  underground and  surface mining activity  are significant.  In
 Texas,  surface  mining and,  to  a  lesser  extent,  in situ  leaching are the
 principal  methods used.  Climatic  and geologic  characteristics and  land and
 water use patterns in the  Colorado-Utah-New Mexico uranium area are  broadly
 similar; and  the  Grants  Mineral Belt  in general  and the Ambrosia Lake Dis-
 trict in particular  are  representative of  this  area.   There are many comp-
 licating variables such as the  geologic  and geonhemical characteristics  of
 the ore body  and host rock.   Water-yield  and  qua"ity associated with mines
 also vary within  the region,  as do  the  size  ana relative  location of the
 populace.   The  Grants Mineral  Belt scenario  is  conservative.   The mines
 discharge  relatively  large amounts  of water to streams that  are used for
 irrigation  and stock  watering  and that flow by  or through local centers  of
 population.
      Table  3.39 shows  discharge from  selected  underground uranium mines  in
 the Colorado  Plateau areas of  Colorado, New Mexico,  and Utah.  On the aver-
                        3                                         3
 age,  discharge  is  2.78 m /rain,  with a standard deviation of 4.34 m/nrin.  The
 selected underground  mines  discharge an amount of water similar to that from
 the Wyoming surface  mines.  In  the  Grants Mineral  Belt  area, average flow
                                   3
 from 28 underground  mines   is 2.4 m/min (J. Dudley,  New Mexico Environmental
 Improvement  Division, written  communication).  Of  the 27 active underground
 mines  being  dewatered,  17  discharge  to the  environment at an average rate of
 3.2  «r/m1n.   The remainder are  In a  closed  circuit.  That is, their discharge
                                                                       T
 1s  used as mill  feed water.   The  range for  17 mines is  0.2  to 19 m/min.
 Average  discharges  from   New  Mexico  underground mines  are  significantly
 greater  than  those   from  mines  in   Colorado  and  Utah,  which  average  0,68
 3         " *"
 m /rain.  Most  of  the ore production  in New  Mexico has been from mines 200 to
 300 meters deep.  In recent years, mines have become  progressively deeper and
 involve  more  dewatering.  For example, the Gulf  Mount Taylor mine, which  is
not yet  producing ore, discharges 15 m /min and will  produce ore from a depth

-------
                                                                       3-115

 of 1,200  meters.   Most of  the water  is  now diverted to a  nearby  ranch for
 irrigation and stock watering.  When  the mill goes  on  line,  most of the mine
 water will be used there.
      Of the  16  active mines  in  the  Ambrosia Lake  district, 13  discharge to
                                                          3
 offsite areas at  an average  rate of approximately  1.6 m /min.   For modeling
 and to  be conservative,  we assumed  that  14 active mines are present  in the
                                                                        3
 model  mine area and that  the average discharge rate  per mine  is 2,0 m /min.
 This  is somewhat  less  than  the average condition  for the Grants  Mineral  Belt
       3
 (3.2  m /min) as a whole  in  tens of discharge  rate,  but the high density of
 mines assumed present  in the  model  area  partly compensates for  the  differ-
 ence.
      For the New  Mexico project  shown  in  Table 3.39, numbers 4,  5,  6,  and  7
 have  discharge that comes directly  from  the mine  portal  to settling  ponds
 before  discharge.  Neither  ion  exchange   for  uranium  recovery  nor  barium
 chloride treatment for radium  removal  is  used.   Facilities 8 through  11 use
 ion exchange columns for  uranium  removal  before discharge.  Settling may or
 may not be used,  depending on  the suspended solids  content of the particular
 discharge.   Project number   10  removes radium  prior  to discharge.   Radium
 concentrations  in  the  combined effluent from two  active  mines in  the Church-
 rock  area (projects 8  and 4),  both of which  use  settling  ponds  as  the  only
 treatment, have ranged  from 1,9 to 8.9  pCI/n since  1975.  In  the  first  survey
 (EPA75),  effluent  from these same mines contained  30,8  and  7.9  pCi/ i , The
 combined  discharge from both mines was sampled  by  the U.S. Geological Survey
 in  1975,  1977, and  1978   (P. Frenzel,  written commanciation) and by the EPA
 (EPA75)  in   1975.   Concentrations   were  30,   14,  2.6,  and  2.6  pCi/x   ,
 respectively.
     It  is  apparent  that  there   are  marked  temporal  trends In  nine water
 quality  and  quantity.    Major factors  responsible  include  changes  in  the
 dewatering  rate accompanying  shaft  sinking  versus actual  ore  production.
 Simultaneously, there are  changes  1n  the mineral quality and leaching rate of
 strata  as  the ore  body is approached and then penetrated..  Mining practices,
 oxidation  of the  ore  body and possibly bacterial   action may also assist in
 the solubilization of   toxic  stable and radioactive trace  elements.  Sample
 handling  and analytical  procedures can also markedly affect  results.   For
example,  if  suspended   solids  are  high  and  a sample  is  acidified  prior to
filterings soluble radium, uranium,  and  other  trace  constituents typically

-------
Table 3.39     Summary of average discharge and water quality data for underground
               uranium mines in the Colorado Plateau Region (Colorado, New Mexico,
               Utah) and a comparison with MPDES limits



Dissolved




•


Radioactivity
D1
Project
Utah/,
llaj
Colorado
2
3
New Mexico
4
5
6
7
8, ,
9 ;1
I0(a
11 a
Average
Standard
Deviation
scharge
31
m /min

0.67

1.31
0.06

14.67
3.79
1.89
0.95
0.18
0.82
6.06
0.216
2.78

4.34
Total U,
mg/£

1.35

2.20
0.25

1.0
0.67
0.02
0.18
4.2
1.9
1.1
2.6
1.41

1.25
Ra-226,
PC1A

1.25

0.53
10.00
fb)
89}:{
23 \l\
14* '
0.1
1.9
4.7
2.3
4.3
13.7

25.9
Pb-210.
pCl/£






15
33
15
0
9.7
16
14
14
14.6

9.1

TSS

7.5

14.3
144.9

25.4
2.6
51.5


1
1.08
2.2
27.8

46.9
Ma^or and
S04 Zn



872 0.02
0.065

60.6
213.7
744
1045
67.2
675
705
837
580

368
trace
Ba



0.19


2.13



0.88
0.17

0.56
0.81

0.80
constituents, mg/£
Cd As



< 0.01 < 0.01
0.003 0.055

<0.005 <
0.011
0.005
<0.005
<0.005 <
0.011
< 0.005
0.012
0.012

0.015

Mo



0.4
0.054

0.01
0.24

0.05
-0.01
0.45
0.62
0.79
0.29

0.29

Se






0.03
0.008
0.004
0.002
0.094
0,407
0.027
0.035
0.076

0.137

-------
                           Table  3.39  (continued)
Summary of NPDES permit
State
New Mexico
Utah
Colorado

Dissolved
Radium-226
3/10
10/30 Total
Radium
3/10
and
3/10
and
Dissolved
Uranium
2/4
2/4
and
-12
3/5
and
2/4
limits for daily average/daily maximum, mg/i except Ra-226, pd"/£
Total
Suspended
Solids
5Q/150(dayrd
20/30(month)
20/30^
20/30
Total
Dissolved
Solids Zinc Barium Cadmium Arsenic
:) 0.5/1.0
NA/650 0.5/1.0
3500
4899G/m 0.5/1.0 1/2 0.05/0.1 1/2
122476^ and and
kg/day -/I 0.5/1
Vanadium
5/10
     ^'Average discharge rate per mine is shown.   Two or more  mines  constitute  the  project.
     (b),
     (c)
     (d)
     (e)
     (f)
'BaCl?  treatment for radium  removal  faulty;  repaired  in late 1979.
 Values shown  are for untreated  water.   BaCl?  treatment now used.
 Applies to discharge associated with shaft  construction.
 Maximum of 10 mg/£ for  30-day  period and  20 mgA  for 7-day period effective July  1, 1980.
 Receiving water standard.
     Source:  Chemical analyses from in-house studies (EPA75)  and State of New Mexico (J.  Dudley,  Environmental
Improvement Division, written communication).  NPDES permit data from Regions VI,  VIII  (H. May,  R.  Walline,
written communication).  Other references include site-specific reports (EIS.ER) and  company monitoring  data.

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                                                                       3-118
 will  increase, as  compared to  samples  that are  filtered prior to acidifi-
 cation  (Ka77).  Therefore, development  of  "average" or "typical" trace  ele-
 ment  concentration  data  is  questionable  and may  be  erroneous without detailed
 knowledge  of  the many  variables  affecting the final  results.
      Despite  the foregoing  difficulties, available  chemical data assembled  in
 Table 3.39  provide  much  of  the source term input data used  in subsequent  cal-
 culations.   The reader  should  bear in  mind  that  uranium concentrations are
 likely  to  be  less   than  3 mg/jt simply because it is  economically practical  to
 use  ion exchange  recovery  for concentrations greater than  this level.  Daily
 average radium-226 concentrations  on  the  order of  3  pCi/n are specified  in
 valid NPDES permits,  and reliable  data  from USGS, EPA, and state sources re-
 veal  stream concentrations  near  the point of discharge to  be on the order  of
 3  to  14 pCi/fc  in  recent years.  Therefore, the "average"  radium-226 concen-
 tration of 13.7  pCi/2.  used  in  the subsequent  modeling  calculations  is  at
 least slightly conservative.  Actual concentrations of  stable  elements  (Zn,
 Ba, Cd» etc.) appear to be well  below  the  NPDES limits, which were also de-
 veloped from  analysis of  uranium mine effluent.  Thus,  it is  presumed  that
 the average values  in Table 3.39 for these  elements are reasonably correct.
 The  variables of  mine size, age,  host rock, and  water  treatment  (ion  ex-
 change,  barium chloride, settling  ponds)  are reflected  in the data.   Water
 quality for mines examined  in Utah and Colorado generally agrees with the New
 Mexico  cases, with the  exception of Project  Number 3 mine, which  is  being
 dewatered  and may, therefore, temporarily  have excessive  suspended  solids.
 We recommend that the NPDES data  for uranium mine discharges be evaluated and
 that  additional compliance  monitoring  be conducted  to confirm .the quality of
 mine  discharge.  Such  studies  should focus  on situations where  mine water is
 being used  for irrigation and stock watering.
     Table  3.40 shows  discharge  and water  quality characteristics  for under-
 ground  mines under  construction and not yet  producing ore.  The  first  example
 involves water  pumped from a  deep mine shaft  under construction.   Consid-
 erable  water  is encountered above  the  ore  body;  water quality is good  and
 representative  of   natural  conditions;  and  suspended  solids are  high as  a
 result  of  construction.  The second  case is  similar except that flow  is  re-
duced,  but  radium   and suspended  solids concentrations are greatly  elevated
due to construction and possible  ore body oxidation.  The third  case involves

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               Table 3.40  Mater,quality  associated with  underground mines in various
                           stages  of  construction  and  operation
Dissolved
Discharge Total U Ra-226 Pb-210
Project m /min mg/£ pCi/£ pCi/ji TSS
New Mexico
1. Underground mine 5.76 0.03 0.07 10 23.8
shaft construction;
dewatering
2. Underground mine 1.73 <0.01 29 0 554
shaft construction;
dewatering
3. Underground mine; 1.43 0.08 0.2 0 1
dewatering wells
4. Underground mine 0 0.32 29 17 1.1
recirculating leach
solution from s topes
(after ion exchange)
Concentration, mg/£
S04 As Mo Se
134 <0.005 0.01 0.003
527 0.012 0.007 0.005
144 <0.005 0.01 0.003
1060 <0.005 3.2 0.268
Source: J. Dudley, State of New Mexico, written communication,  1979.
                                                                                                                to
                                                                                                                 I

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                                                                       3-120

 dewatering  wells used  to dewater  the  ore body  before mining.  There  is  no
 oxidation  and  suspended sol Ids  are very  low as  is radium-226.   Dissolved
 radium-226  in  the ore body  is  on  the  order  of  10  pCiA  or less  in the  natural
 state,  but  concentrations rise to 100 pCi/£ or more  after mining  takes place,
 possibly  due  to oxidation  and  bacterial  action  in  the  workings (EPA75).
 Project Number 4,  in  the Ambrosia  Lake  district, is an  inactive underground
 mine  now used  as  a  type  of  in  situ leach facility.   Mine water  is recir-
 culated through  the workings.   Leached uranium is selectively recovered  using
 ion  exchange.   The  process is a closed one,  hence  no effluent is  involved.
 Water quality  after uranium  removal reflects the  buildup  in  radium,  lead-210,
 sulfate, molybdenum,  and selenium.
3.4.3.    Hydraulic and Hater QualityEffects of Underground Mine Discharge

3,4.3,1   Runoff andFlooding in the Model Underground MineArea

3.4,3.1.1 Study Approach

     We  chose  to  study  an area of  rather concentrated  underground  mining,
similar to the Ambrosia Lake district of New Mexico,  All of the mines in the
district  dewater  to  different  degrees  because the  principal  ore  body is in
the Westwater  Canyon  Member of the Morrison Formation, which is also a major
aquifer.   In  the  analysis,  flows  from  some  14  active mines  discharge to
formerly  dry washes  and  dissipate  downstream by evaporation and, more impor-
tantly,  infiltration.  Suspended and dissolved constituents  persist  at the
land surface and  become  available  for resuspension  and  transport  in  surface
floods with  recurrence intervals of 2 to  25  years.  Contaminated runoff from
the sub-basin is then  diluted in average annual flows of progressively larger
streams and rivers of  the region.
     Similar to the analysis presented for surface mines in Wyoming, there is
a  three-basin  hierarchy:  sub-basin,  basin,  and regional  basin  (Fig.  3.16).
These correspond to  Arroyo  del  Puerto-San Mateo Creek,  Rio  San  Jose and Rio
Puerco, and  the Rio  Srande,   Of these,  the  Ri,o  Puerco  is  distinctly ephe-
meral.  The Rio  Puerco drains  into the Rio Grande, which is perennial, due in
large part  to  the heavily  regulated flows and storage  reservoirs.  Because

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                                                                              3-121
                   MCKINLEY  COUNTY
Sub-basin area  containing
model  mines
0    iO   20   30   40   50
     .1     I     r     i     §
      	 Sub-basin boundary
      	Boundary of a portion of the Rio San Jose basin
            upstream from the sub-basin
      —	  Rio Puerco basin boundary
          A USGS gauging station
      Note: Boundary of the FUo  Grande  regional basin above Bernardo is not
            shown
 Figure 3 16   Sketch of sub-basin, basin, and regional basin showing orienta-
             tion of principal drainage courses, areas of drainage, and loca-
             tion of mines in the New Mexico model area

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                                                                       3-122

 the Rfo Grande is  the  major regional  river and  the  basis of extensive irri-
 gation  projects, it  is included  in  the. analysis.   The mining area  is  well
 away from the Rio  Grande  Valley,  and  it is unlikely that noticeable  changes
 in  flow or water  quality  because of raining  would  occur.
      Flow volumes for the  sub-basin and  open file USGS data  (I,  Beal,  written
 communication,  1979} for  flows  in the  basin  and regional basin are  used  to
 transport and dilute contaminants originating in the mine effluent.  It  is
 initially assumed that  all contaminants  are available for transport  by  sur-
 face flow  so -as to deliberately create  a  worst-case  situation.   Section
 3.4.3.2 reviews  infiltration of  water  and  solute  for  possible  effects  on
 groundwater.
      We do  not  address the  effects  of  seepage  from settling  ponds  because
 such ponds  are relatively small,  tend  to be  self-sealing, and  are well  away
 from inhabited   areas.    Supposedly,   settled  solids from  thete  ponds  are
 removed and incorporated with uranium  mill  tailings.  Limited  field  studies
 to  determine  whether  such  ponds cause groundwater contamination  is warranted.
 In  some instances,  the  ponds have synthetic liners,  and  leakage is expected
 to  be  minimal.   The influence  of mine  dewatering   (by  wells, shafts,  and
 pumping of mine  workings)  on  groundwater  quality  or  availability  is  not
 addressed  primarily  because  of the  lack  of  data.   We  strongly  recommend
 further study of  the  hydraulic and groundwater quality effects of dewatering.
 Th,is aspect  of  mining  is   coming  under  increased  scrutiny  by  regulatory
 agencies  at  the  State  and Federal level  because  of the influence on water
 quality and availability.
      In  summary,  our approach  defines the quality and  volume of  mine water
 discharge;   outlines hydrographic basins; and   calculates  flood  flows  for
 various  return  periods  ranging  from 2 to 25 years  in the sub-basin.   These
 flows are then diluted  into the average annual  flow in the basin and regional
 basin.  The principal objective is to develop a rough estimate of contaminant
 loads resulting from mine discharge.

 3.4.3,1.2 Description of Area
     The Grants Mineral Belt of northwestern New Mexico is in the Navajo and
DatH sections  of the Colorado Plateau  physiographic province (Fe31). Char-
acteristic landforms  in the  study  area include rugged mountains, broad, flat

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                                                                       3-123

 valleys,  mesas,  cuestas,  rock  terraces,  steep  escarpments,  canyons,  lava
 flows,  volcanic  cones,  buttes,  and arroyos  (Ki67;  Co68).   Elevations  in the
 area  range from  1,980  m at  Grants  to an  average of  2,160  m near Ambrosia
 Lake,   Just north of Grants is Mount Taylor, the highest point in the region.
 It rises from Mesa Chivato to an elevation of 3,471 m (Co68).
      The study area has a mild, semiarid, continental climate.  Precipitation
 averages 25.4 cm/year, and there is abundant sunshine, low relative humidity,
 and  a  comparatively  large annual  and  diurnal  temperature  range.   Average
 annual  precipitation  at Gallup,  Bluewater,  and Laguna  is  27.12,  24.55, and
 22.31  cm,  respectively.  In  the  higher elevations, the average is  51  cm  or
 more because of thunderstorms in July, August, and September and snow accumu-
 lations  in the  winter  months  (Co68,  6o61,  Jo63).  Only  thunderstorms are
 significant in the lowlands.   Heavy summer thunderstorms (40 to 70 in number)
 of high intensity and  local  extent can  result  in 5 cm of rain with  local,
 damaging flash floods.
                                                                            o
      The watersheds of  the Rio  San Jose and Rio Puerco encompass 19,037 km .
 Most of the  larger  communities  in the basin are located in the floodplain  of
 the Rio Grande  and  principal  tributaries.  Extensive irrigation with surface
 water  occurs  in  the  watersheds  of  the  Rio  San Jose,  Rio Puerco, and Rio
 Grande.  In  the sub-basin, there  was  no  perennial  flow  before mining  and,
 thus  no irrigation, but  increasing use is being made  of the  mine  discharge,
 which  is  regarded as an  asset in a  water-short  area.   Subsequent  sections
 summarize  the   surface  water  quantity  at  some   of  the  principal   gauging
.stations in the  Middle  Rio Grande Basin and  the  irrigated areas below these
 stations.   Groundwater is used  for essentially  all public water supplies  as
 the temperature, quality, and year-round  availability  are assured.   Numerous
 wells scattered  across the  landscape,  particularly in  the stream valleys, are
 used  for stock  water  and,  to a lesser  extent,  for potable use on the  scat-
 tered ranches  and Indian settlements.
      Under  completely  natural  conditions,  streams  in   the  study area  were
 distinctly  ephemeral, and  many of the  smaller  ones did not  experience  flow
 for periods of  several years.   The Rio Grande experiences  peak  flows  in the
 April-June  period  when  snowmelt  and  precipitation cause  gradual  rises  to
 moderate discharge levels involving large  volumes  of flow and  long  durations.
 Peak  discharge  rates   (volume  per time)  occur  in  the  summer flash  floods.

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                                                                       3-124
 Construction of dams and  conveyance channels to eliminate  flooding  problems
 has  been extensive.  In  the tributaries such as  the  Rfo San Jose and  upper
 reaches  of  the  Rio Puerco,  there  is considerable  streamflow regulation  to
 minimize flood damage  and maximize  use  of  available  water for  irrigation.
      Conditions  in the  Ambrosia Lake district  with respect  to  the  type  of
 mining  operations  and discharge of  effluent  to  ephemeral streams are dupli-
 cated  elsewhere in the Grants  Mineral Belt.   In the Churchrock district, two
                                                          3
 mines  discharge  to the Rio  Puerco at rates of 4.7 to 15  m /min.  Most of the
      •3
 4.7  m /min  discharge  from one  mine  is now used  in a nearby  mill.  At Mariano
 Lake,  located between  Ambrosia Lake and Churchrock, and at the Marquez and
 Rio  Puerco  mines east of  Ambrosia Lake,  mines are expected to discharge 0.8
         3
 to  4.5 m /min  to  various ephemeral  streams.  Another large  mine will  soon
                      3
 discharge up to 5.3 m /min  northward into  the San Juan  River Basin.  In the
 mid  1980's,  construction  is  expected  to  begin  on  five  large  underground
 mining  projects that will  have a  combined   discharge on  the  order  of  71
 m /min.  Most  discharge will  be  into the San  Juan Basin,  reflecting the trend
 of mines becoming  deeper and requiring more  dewatering as  the mining center
 moves  from  the south  flank of the San Juan Basin into more interior portions.

 3.4.3.1.3    Estimateof Sub-basin Flood Flow
     Since  we use a  dilution-model, emphasis is on flow volume  rather  than
 peak  discharge  rate  in  the  sub-basin, basin, and regional basin hydrographic
 units.   Gaging records  from the U.S. Geological  Survey  WATSTORE  system (L.
 Beal, written communication, 1979) provide average discharge rates for runoff
 events with various  return  periods  and durations.   The  latter specify  the
 time,  in days, and the associated flow rate that will be equaled or exceeded.
 Flows for arbitrary periods of time ranging from 1 to 183 days are specified.
 Probability  can  be  stated  in  terms   of N-year  recurrence  interval.  By
combining discharge rate  (volume per time} and time (partial duration),  flow
volume can  be calculated.
     In  the_ungaged  sub-basin, runoff volumes associated with  events  having
return  periods of 2,  5,  10,  and  25 years were calculated from  regression
equations developed  by  the  USGS (Bo70).  The equations  were  generated  from
multiple regression  of  discharge records  from  gaged basins against  various
basin  characteristics.   These are   area  (A), precipitation  (P.),  longitude
                                                                u

-------
                                                                       3-125

 at the center  of  the sub-basin (Lo), soils infiltration index (Si), and mean
 basin elevation (£„]•   Through  use  of appropriate constants and coefficients
 (Bo70), flow volumes can be calculated for 1-day and 7-day events with return
 periods of 2, 5, 10, and 25 years.   For the sub-basin, the basic equation has
 the following form:

           FV = a Abi Pb9  Lo1^  S5 E                      (3.10)
where     A = 95 mi
         P  = 2.9 i
          3
         Lo = 7.85 (longitude in decimal  degrees minus 100)
         S. - 8.5
         E  = 7.0 thousand feet
          P  = 2.9 inches
           3
 Table 3.41 contains the  regression  coefficients and total flow volume  data.
 Short-term,  1-day and  7-day,  events  were  of  main interest because  these  would
 be  expected  to  provide greater  flushing of contaminants  stored  at  or  near the
 water-substrate interface in  the  streams  receiving  mine  discharge.
      The  extent to which  mine discharge transforms  existing ephemeral  streams
 into  perennial  ones is evaluated with a  crude  seepage  and evaporation  model
 (see  Appendix  H).   The basic  equations  and approach  are patterned  after  a
 similar  analysis  in the  Generic  Environmental  Impact  Statement  on  Uranium
 Milling  (NRC79b).
      Figure  3.16  shows  the relationship of the  sub-basin,  basin, and  regional
 basin  boundaries  and the  principal drainage  courses  and  gaging  stations.   The
 confluence  of  the  Rio Puerco and Rio San Jose is  shown approximately  55 km
 closer to the Rio Grande  than  is actually the  case  in order to simplify flow
 routing and  to  reduce  the  number of dilution calculations.   Table 3.42 sum-
 marizes the  key characteristics of  these basins in terms of catchment  area,
 discharge,  and   irrigated  farmlands  downstream from points where  mine  dis-
 charge might be  tributary  to  the  streams.   Mine  discharge  occurs  in  the
 sub-basin  which in turn discharges  to the  Rio  San  Jose  and  then  to  the  Rio
 Puerco.  No mine discharge and no significant runoff are associated with  that
 portion of  the basin  tributary  to San Mateo Creek  between the Rio San  Jose
and the  sub-basin.  For  modeling,  flooding  within  and  runoff  from the  sub-

-------
               Table 3.41   Total  flow volume for sub-basin floods of 1- and 7-day durations
                            and return periods of 2,  5,  10, and 25 years
Flood
Volume
FV 1
FV 1
FV 1
FV 1
FV 7
FV 7
FV 7
FV 7
|2(a)
,5
,10
,25
,2
,5
,10
,25
Regression Coefficients

1.
1.
5.
2.
8.
2.
8.
3.
a
08 x
27 x
07 x
39 x
60 x
99 x
97 x
06 x

lO"4
Hf3
lO"3
ID'2
10~7
1Q-4
lO'4
ID'3
bl
0.931
0.941
0.953
0.972
0.965
0.904
0.910
0.922
b9
1.83
1.40
1.17
0.929
2.36
2.55
2.37
2.17
b!4
-1.43
-1.89
-2.18
-2.51
-1.61
-2.09
-2.39
-2.76
b!5
4.09
4.07
4.02
3'. 95
4.22
3.53
3.61
3.68
Volume
b4
2.
6.
1.
_ "1
1.50 5.
8.
1.
«*. o
(Bl3)
16 x
23 x
02 x
76 x
95 x
79 x
43 x
26 x

104
104
105
105
103
103
104
104
(a)
   FV 1,2 indicates a flood of 1-day duration and a return period of 2 years.
                                                                                                        CO
                                                                                                        CFt

-------
able 3.42     Summary of area, discharge, and Irrigated acreage for the sub-basin, basin, and
              regional basin hydrographic units in New Mexico
                                                                         2             3
                      USGS                                   Number of km     Average m /min    Average Annual
                      Station                   Period of    Under Irrigation Discharge (for    Discharge (m )
                                           2
                      Number       Area (km )   Record Yrs.  Below Station   Period of Record) for Period of Record
iub-basjn
iasins
 Rio San Jose
 near Grants
 Rio Puerco
 near Bernardo
tegjcma]Basin
 Rio Grande at
 Bernardo
              246

3435        5957          42
     (2927 non-contributing)
3530       19037          38
     (2927+ non-contributing)

3320       49810          41
     (7610 non-contributing)
2.43+
 N/C
    (a)
 11.09
               81.05
1649.35
5.83 X
                      4.26 x
86.69 x 10'
     (a)
        N/C  *  Not  Calculated.
                                                                                                             rsj

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                                                                       3-128
 basin Is,  in  effect,  routed  without  change  in flow and quality and allowed to
 enter the  Rio San  Jose.   Flow from the  San  Jose is further diluted In the Rio
 Puerco,  then  diluted  again  in the  Rio  Grande.  In actuality, flow  from the
 Ambrosia Lake district rarely,  if ever,  enters  the Rio San Jose because flood
 volumes  are  small  and infiltration  losses are  large.   This departure  from
 true  conditions  is justified  within  the  context of  the modeling  approach
 used.  Basically,  the model  draws from  a specific area  but  does  not attempt
 to  closely duplicate  its conditions. If a  specific area  were  exactly repre-
 sented,  the  model  would  still be  incorrect  to  varying  degrees for  other
 areas, and  the  generic value  of the  assessment  would depreciate.
      Of  special interest  is the effect of contaminated flows on  irrigation
 projects present  on the Rio  San Jose and Rio Grande.  An extensive system of
 dams  and  conveyance  channels regulates flow in  the  Rio Grande, and  partia!
 duration flow data are unavailable.   Instead,  the  average  annual  flow volume
 is  used  to provide the final  dilution  estimate.   For the  sub-basin  in  which
 the mines are  located, flood volumes are calculated using the USGS regression
 equations  (Bo70).   The maximum return period for which  flows are calculated
 is  50 years.   The remainder  of  this   section  first  considers the  flow or
 hydraulic  aspects  of  the surface water pathway.  Finally,  several   factors
 concerning  the  quality of runoff water  are mentioned to  balance conservatism
 and realism in the pathway analysis and, subsequently,  in  the health  effects
 modeling to follow.   The  emphasis here is  on  surface water  impacts, and we
 assume  maximum transport  for  this  pathway.   The  influence  of infiltrating
 mine water  is discussed in Section 3.4.3.2,
     All of the streams, except the Rio Grande and certain  reaches of  the Rio
 San Jose  are  distinctly  ephemeral  under  natural  conditions.   In  the sub-
 basin, there  is perennial  flow because  of  mine discharge.  In Fig. 3.17 are
 the average monthly and annual discharges  for  the Rio San Jose and  the Rio
 Puerco  in   comparison  to  cumulative  annual  flow  from  14 mines,  each dis-
                3
 charging at 2  m /min.  The monthly data reveal pronounced seasonal  variations
approaching 1  to  2 orders  of  magnitude.   The  streams do  not  show the same
 seasonal  variations,  further attesting  to  varied  patterns of  runoff, irri-
gation diversion,  and  control  features  such  as  impoundments  and conveyance/
irrigation  channels.   Figure  3.18  shows  the percentage  of each month during

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10-
         LEGEND
                                                                                  3-129
         L
        Rio  San Jose near Grants,  N.M.
        Rio  Puerco at Rio Puerco,  N.M.
        Rio  Puerco near Bernardo,  N.M.

Jan
Feb
                        Mar
Apr   May
Jun
                                      Jul
Aug   Sep
                                                   Oct   Nov
                                                                                 Dec
       Figure 3 17 Average monthly fI ows for the period of record for the Rio San Jose
       and the Rio Puerco in New Mexir-n^i'^^anzed from flow records provided by
       L Beat, U S Geological Surve        erque)

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                                                                       3-130

 which  there  Is no  flow in  the  Rio San  Jose  and  Rio  Puereo.  The  average
 period of  annual or  monthly no flow is  as  follows:

                Rio San Jose near  Grants:        0  Percent
                Rio Puerco at Rio  Puerco:      45  Percent
                Rio Puerco at Bernardo   :      71  Percent

     It  is ilso assumed that  flow  from the sub-basin  reaches the first major
 stream,  the  Rio   San  Jose, -with no change in  flow or  quality.   Runoff  is
 minimal  in the lower  reaches  of  San Mateo Creek  because  of internal drainage
 and  considerable  infiltration.   Historical   evidence  indicates   that  onl.y
 rarely,  if ever,  would •Hood  runoff  from Ambrosia  Lake enter the  Rio Se.,,
 Jose,   In  the interests of  conservatism,  total  flow laden with contaminants
 is  transported to the Rio  San Jose.  Dilution first  occurs  within the sub-
 basin  and  then,   successively,  in  the  Rio San  Jose,  Rio  Puerco,  and Rio
 Grande.  The  latter  is  the  regional  basin.
     There  is an  infinite  number of combinations  of flood volumes  and dilu-
 tion volumes  for  the  sub-basin,  basin, and regional  basin  streams.   Use of
 average  annual discharge  volumes in the  receiving streams  simplifies  what
 would otherwise  be a burdensome, confusing series of calculations.   Flushing
 action  from the sub-basin  is handled on  a probabilistic basis 1n terms of
 flow duration and  return period.  Concentration values are based on  14 mines,
 a loading period of  two years, and flow and water quality data shown in Table
 3.39.   When,   for  example,   5-year  or  10-year  events  are considered,  it  is
 conservatively assumed  that events  with shorter return periods  do  not occur.
 The accretion  period remains constant  (2 years), and  only the  return period
 and duration  are varied, resulting  in  varying  flow  volumes.  It  is conceiv-
 able that  contaminants  could  concentrate  for  3,  4, or 5 years and  then  be
 flushed by a 2-year event,  but this  was  not evaluated.
     Minimum  and maximum return  periods  for  floods from  the sub-basin  were
 set at 2 and  25 years, respectively, for several  reasons.  The  2-year event,
 i.e., runoff  volume  over a  duration of 1  day or  7 days and  occurring on the
average of  every  2  years,  is expected  to occur rather  frequently over  the
life of  the  mines  (17  years).  The intermediate-sized storms with  return
periods  of  5  or  10 years would result  1n considerable contaminant transport,

-------
   100
e   so
    8°
s
•6
T5
    70
    60
I  50


'3  40

 o

 g  30
 o
 f-
Cu
    20


    10


     0
                         Puerco near Bernardo
                         ...... '
                                          -



               \

               Rio Puerto at Rio Puerco
                                                     \
                                                      V
                                                          ^
             The  Rio San Jose near Grants exhibits no periods  of zero flow.


1
Jan I Feb

Mar

Apr

May

Jun

Jul
| 1
Aug |Sep |0ct

Nov

Dec
    Figure 3.18 Periods of no flow in the Rio San Jose and Rio Puerco (Summarized from flow records provided by L. Seal,
    U.S. Geological Survey, Albuquerque)

-------
                                                                       3-132

 but concentrations  would be low owing  to  dilution and to annual  or semiannual
 scouring  provided by smaller  floods.   The 25-year event is a  practical  maxi-
 mum expected  to occur during  the  lifetime of  the  mining district.   Still
 larger floods, with return  periods  of 50 or 100 years,  can be calculated  but
 are less  important because  of  their infrequent  occurrence. Figures  3.19  and
 3.20  show  calculated   flow  volumes  from  the  sub-basin  for  1-day and  7-day
 durations  and  return  periods  of 2 years  to 50  years.  The extreme  range  in
 flow volume  is from 2.16 x 104  m3  to 2.55 x 105  m3.
     Figures  3.19  and  3.20 show flow  values   in  the Rio San  Jose  and  Rio
 Puerco for  1-day and  7-day durations and  return  periods of 1 to  100 years.
 For the Rio San Jose,  1-day volumes range  from  1.24  x  10  m   to  1.68  x  10
  3                                                                3
 m .  The mean annual  discharge  rate in  the Rio San Jose is 11.09 m /min.  Flow
 from the  Rio  San Jose  enters  the  Rio  Puerco where corresponding  flows (1-day
                             6              73
 duration)  range from 0.6 x 10   to  2.15 x  10 m   at the point of  inflow to  the
 Rio Grande.  Average daily discharge in the Rio  Grande seasonally ranges from
         53             53
 8.87 x 10    m   to 59.5  x 10  m  .  Average  annual  flows rather  than  peak  1-day
 or  7-day flows were used in  the subsequent calculations.
     The maximum probability for peak runoff from  the  sub-basin and resulting
 contaminant  transport  is  in the summer months,  at which  time the  Rio Puerco
 has  no flow  about 22 to 75 percent of the  time.   Flow  in  the Rio  San  Jose and
 Rio  Puerco from June through September ranges  from 3.96 x 10  to  1.97 x 10
  2
 m  per month for the period  of  record (Fig.  3.17).

 3.4.3.1.4  Prediction of Sub-basin Hater Quality
     Table 3.43 outlines dilutions based  on the  foregoing  discussion of flow
 patterns and discharges and considering  only the  1-day sub-basin flood event
 with a 2-year  recurrence interval.   The  dilution constant is  the ratio  of
 concentration  in the receiving  water to that in  the contaminated  (relatively)
 inflow.  It  is more commonly expressed as  the  dilution  factor,  which is the
 reciprocal.  Thus,  in  the case  of the sub-basin  flood flow entering the mean
 annual   flow  of  the  Rio  San Jose,  there  is  a   271:1  dilution  (Table 3.43).
     With  development  of the foregoing (mine water)  source term and  surface
water  pathway,  the - remaining  discussion  emphasizes  contaminant  concen-
trations in  surface water.  This,   in turn, serves as  input  data  to health
effects modeling for the water pathway.   Chemical  concentrations in  the Rio

-------
                                                                                  3-133
   10 i
3
UH
                                                             LEGEND
                                                             O Sub-basin (Arroyo  del
                                                                Puerto @ San Mateo Creek)

                                                             "A Basin (Rio San Jose near
                                                                Grants,  #3435)

                                                             O Basin (Rio Puerco  near
                                                                Bernardo, #3530}

                                                             NOTE:  Total flood flow for
                                                             one day  duration not  calcu-
                                                             lated  for regional basin
                                                             (Ilio Grande).
                                                   I
                                                   10
I
25
I
50
                                 RECURRENCE INTERVAL (YEARS)
                 Figure 3 19 Total flow volumes in one-day periods for Hoods of various
                 recurrence intervals in the sub-basin and basins in New Mexico {Summarized
                 from (low records provided by L Beal, U S Geological Survey, Albuquerque)
 I
100

-------
   5.

   4—J

   3.
10'
   9
   8—|
   7.
10
10'
   1=
   8_
   7.
   6_
                                                                                 3-134
                                                           LEGLND

                                                            O Sub-basin  (Arroyo  del Puerto @
                                                              San Mateo  Creek)

                                                            & Basin  (Rio San Jose near
                                                              Grants, #3435)

                                                            O Basin  (Rio Puerco
                                                              near Bernardo,  #3530)
NOTE: Total flood for  seven days
duration not calculated  for regionaJ
basin (Rio Grande).
                                                 i
                                                 10
                                  RECURRENCE INTERVAL
      25
(YEARS!
             50
100
          Figure 3 20 Total flow volumes in seven-day periods for floods of various

-------
               Table 3.43  Dilution factors  for the Rio  San Jose, Rio Puerco, and Rio Grande
                           for 1-day flood flows with  a  2-year recurrence  interval
Hydrographic Basins
Rio San Jose near Grants^9'
Rio Puerco' ^
Rio Grande near Bernardo^
Flow Ratio
(m3/m3)
2.16 x 104
5.83 x 106 + 2.16 x 104
2.16 x 104
4.26 x 107 + 2.16 x 104
2.16 x 104
Oi iution
Constant
0.0037
0.00051
0.000025
Dilution
Factor
271
1973
40135
                                86.69 x 107 + 2.16 x 104
     ^'Calculated using mean annual  flow in the Rio San Jose (near Grants,  NM)  station:
Dilution =  	Sub-basin flood flow	,
            Rio San Jose flow + Sub-basin flood flow
     '  ^Assumes Rio San Jose enters the Rio Puerco at Bernardo:
Dilution =              Sub-basin flood flow
            Rio Puerco flow (includes Rio San Jose flow) + Sub-basin flood  flow
     ^Dilution =  	Sub-basin flood flow	
                    Rio Puerco flow + Rio Grande flow (at Bernardo)  + Sub-basin flood flow
CO
tn

-------
                                                                       3-136

 San Jose,  Rio  Puerco  (at  Bernardo), and  in  the Rio Grande  (near Bernardo)  are
 shown  in Table 3.44 along with  1-day and 7-day flood flow  volumes from  the
 sub-basin  for  return  periods of 2» 5, 10, and 25 years.  These flood volumes
 are diluted  into  the  mean annual flow of the Rio San Jose  (near Grants), Rio
 Puerco (at Bernardo),  and Rio Grande (near  Bernardo),  The principal reason
 for using  mean annual  flow  is that the radiation dose and  health effects
 model  (Section 6.0) stresses estimating average annual dose to the population
 over the duration of  mining activity.
     For example, the  1-day duration flood  flow (with a 2-year return period)
 contains 1920  mg/£  uranium, which decreases to 7.09 mg/£  in the Rio San Jose
 and 0.973  mg/£ in the  Rio Puerco.  Because  of the short duration of most
 floods  in  the  sub-basin,  there is Irctle difference in flow volume and, thus,
 dilution between  the  1-day and 7-day events.  With progressive dilution down-
 stream, the  difference in size between sub-basin floods of varying durations
 and return periods becomes insignificant relative to the mean annual  flow
 volumes of the basin and regional  basin streams.  As a result, concentrations
 tend to reach  a minimum and remain unchanged at this degree of accuracy.
     As in the case of the Wyoming surface-mine scenario, we assume
 that most  contaminants in the mine water collect on or near the land
 surface and  are available for transport.  This assumption is open to ques-
 tion, but  field data are scarce to support contentions as to the fraction of
 cpntaminant  load that  becomes unavailable.  For example, extensive field
 studies along  the Animas, San Miguel, and Dolores Rivers in Colorado con-
 cluded that  "...once radium becomes a part of a stream's environment,  it
 constitutes  a  relatively long-term and continuous source of water and  aquatic
 biota contamination"  (Si66).  However,  cessation of uranium mill  discharges
 to the Colorado River tributaries  effectively negated this source, which is
now believed to be buried behind the Lake Powell  and Lake Mead impoundments.
 Similarly,  dissolved radium reverts to background levels of several  pico-
curies per  liter in natural  streams receiving mine  water in Colorado and New
Mexico. -Although it is likely that flood waters  resuspend precipitates and
sediments  with sorbed radium, laboratory experiments (Sh64; Ha68)  indicate
that only  minor re-solution takes  place.  This phenomenon is supported  by
recent surface water data collected in  the Grants Mineral  Belt of New  Mexico
(Ku79). Therefore, concentrations  of dissolved radium in flood water  are

-------
Table 3,44  Annual  contaminant loading  from 14 uranium  mines and resulting concentrattons in sub-tasin floods and in the
            average annual  flow of  the  Rio San Jose,  Rio  Puereo, and Rio Grande
Contaminant
concentration
in mine
effluent {mg/l
except as noted)
Total Uranium
1.41


Radium-226
13.7 pCi/j,


lead-210
14.6 pG1/l


Cadmium
0.007


Arsenic
0.012


Selenium
0.076


3
Mass available 1- and 7-day flood flow volumes (m } and contaminant concentrations associated with
for transport 1-Day
(fci/yr extent .
as noted) 
-------
Table 3.44 (continued)
Contaminant
concentration
in nine
effluent (mg/t
except as noted)
Molybdenum
0.29


Barium
0.81


Zinc
0.043



Sulfate
580


Total Suspended
Solids
27.8

Mass available 1- and 7-day flood flow volumes (m ) and contaminant concentrations associated with
for transport 1-Day
(kg/yr except, , .
as noted}u' V =2.16x10*
2 C2
300 390
1.4
0.20
0.0093
850 1100
4.1
0.56
0.026
45 58
0.21
0.029
0.0014
R n
1.22 X 10* 1.58 x ICr
584
80
3.8
29000 38000
140
19
0.90
V, =6.23xl04
5 C5
130
1.4
0.19
0.0089
380
4.0
0.55
0.026
20
0.21
0.029
0.0014 •
A
5.43 x 10*
580
80
3.8
13000
140
19
0.89
" *C10
82
1.4
0.20
0.0092
230
4.0
0.55
0.026
12
0.21
0.029
0.0014
A
3.35 X 10*
574
80
3.7
8000
140
19
0.90
'25"£"°5
48
1.4
0.20
0.0091
140
4.1
0.58
0.027
7.2
0.21
0.030
0.0014
*
1.94 x I(T
568
80
3.8
4600
130
19
0.89
*2-5947
1400
1.4
0.20
0.0092
4000
4.1
0.56
0.026
210
0.21
0.029
0.0014
r
?j.?4 x 10
586
80
3.8
140000
140
20
0.92
V5=3794 V
965
1.4
0.20
0.0093
2700
4.1
0.56
0.026
140
0.21
0.029
0.0014
L
3.8S X 103
584
80
3.8
92000
140
19
0.89
return periods of 2 to 25 years' '
7-Day
I0=1.43xl04
590
1.4
0,20
0.0091
1700
4.2
0.57
0.027
88
0.22
0.030
0.0014
E
2.38 x 105
582
80
3.7
57000
140
19
0.90
*25-2.26x!0
370
1,4
0.20
0.0092
1100
4.2
0.58
0.027
56
0.22
0.030
0.0014
c
1.51 x 10s
584
80
3.8
36000
140
19
0.89
     (a)
        Mass values shown are on an annual, per-mine basis.
     ' 'v  and C_ refer respectively to flood volume, in cubic meters, and concentration in runoff for an r-year flood.  Concentrations are in
ntg/1, except for radium-226 and lead-210, which are 1n pCi/*.  Concentrations shown are from accretion or loading 1n the sub-basin for 2, 5, 10,
25 years, yielding the first value shown in each set.  The next three values below this initial value represent, in downward order, concentrations
in the flood flow as diluted by the mean annual flow in 1) the Rio San Jose near Grants (5.83 x 10  m 5, 2) the Rio Puerco at Bernardo (4.26 x 10
n3), and 3) the Rio Grande near Bernardo (86.69 x 10  m3).
     Note.—Assumptions:  Mines discharge continuously at a rate of 2.0 m3/min.  Concentrations are the average of those shown in Table 3.39.  Except
for radium and sulfate, all suspended and dissolved contaminants remain 1n or on the stream sediments and are mobilized by flood flow.  Twenty per-
cent of the sulfate and 10 percent of the radium are available for resolution.
f
*-*
iff
as

-------
                                                                       3-139

 arbitrarily set at 0.00144 C1/yr or 10 percent of the annual  loading from the
 model  mine.
      Sulfate is also considered  an  important exception in the  total  "trans-
 port"  concept.   Because sulfate  can  be a highly mobile anion,  it is  assumed
 that 80 percent of  the  load  enters  the shallow groundwater reservoirs and 20
 percent is  available for  solubilization and  chemical  transport in  surface
 flows.  No distinct pattern of  groundwater contamination from mine water, per
 se»  was  documented  in  an earlier  Grants Mineral Belt  survey  (EPA75),  but
 recent data from  the State indicate groundwater deterioration as a  result of
 mine drainage  (J.  Dudley,  New Mexico Environmental  Improvement Division,  oral
 communication,  1979).  It is likely  that considerable fractionation t»F other
 stable and radioactive trace elements  occurs,  but  field data specific to the
 uranium mining  regions are quite  scarce, with  the  exception  of Texas  (He79),
 where  only stable elements were  studied.  Because  of our  imperfect, non-pre-
 dictive understanding  of  trace  element  transport  in  aqueous  systems,  our
 analysis  assumes total  transport  for  most constituents in lieu  of  numerous,
 equally unfounded assumptions  for resuspension factors, fractionation,  etc.
 Floods of  1-day  and 7-day duration  and return periods of 2, 5, 10,   and  25
 years  are  arbitrarily selected  as  providing  the  necessary  flushing  action
 associated  with intense, short-term runoff events.   It is  likely that storms
 of  shorter  (less  than  1-day)  duration and possibly  greater discharge  rate
 also transport  contaminants.  The  flow  volume and thus  the  dilution  cannot  be
 estimated  for these  events.
     Calculated water quality in  basin  and  regional basin streams  is shown  in
 Table  3.45  along with established and  suggested standards  for selected  con-
 taminants.   For  uranium,  concentrations  in  the basin exceed the  suggested
 limits  based on chemical toxicity and  radiotoxicity.   Radium-226/228  exceeds
 the  standard in  the basin but  is well  below  the  standard for the regional
 basin.  The same is  true for sulfate, cadmium,  arsenic, barium, and selenium.
 Zinc  is the only  contaminant consistently below  the potable and irrigation
water  standards.   As  in the  case of the  surface mine scenario for Wyoming,
 uranium is apparently well above  suggested limits and warrants further  study,
as do  the stable  toxic  elements  in  the  basin  area(s)  closest to the  mining
centers.
     With  the   exception  of  radium-226  and  sulfate,  the  concentrations of
radionuclides and  other  parameters shown in Tables 3.44 and  3.45 reflect no

-------
                    Table 3,45     Comparison of potable and irrigation  water standards  and
                                   surface water quality affected  by  underground mine drainage
Parameter
Range of contaminant concen-
  trations in flood flow  , .
affected by mine discharge^ '
  Basin         Regional Basin
Hln.    Kax.    Win.      Max.
     Potable water standards (mg/t  )*  '
Maximum Penmssable   Recommended  Limiting
 Concentration           Concentration
             .Irrigation
Recommendations for maximum concentration
 for contmyous yse on all  soils {mg/t  }
Total U
Ra-226 +
TSS
Sulfate
Zn
Cd
As
Ba
Se
6.9
228 6.7
130
574
0.21
0.03
0.061
4,0
0.37
7.1
6.9
140
584
0.22
0.03
0,063
4.2
0.38
0.045
0.044
0.89
3.7
0.0014
0.0002
0.00039
0.026
0.0026
0.046 0.015/3. 5/0.2^
0.044
0.92
3.8
0.0014
0.0002
0.00041
0.027
0.0026
...
...
0.01
0.05
1
0.01
5 -fi*
250
5.0
...
0.01
...
...
5 pCi/t
200
2.0
0,010
0.10
—
0.02
     ^'Concentrations fn milligrams per liter,  except Ra-226 -228 which are !n plcoeurfes  per liter.   Data shown apply  to  the Basin  (Rio San
Jase near Grants) and Regional Basin (Rio Grande near Bernardo) streams (Table 3.44).

     '  'Sources:  U.S. Environmental Protection  Agency (EPA76) and, In the case of uraniam, suggested guidance  from the  National  Academy of
Sciences (NAS79) to the USEPA and from USEPA, (Office of Drinking Water) to the State  of Colorado  (U79).

     ^Source:  (NAS7Z).

     ^ '0.015 mg/i :Suggested maximum daily limit based on radfotoxicity for potable water consumed at a rate of 2 liters per  day  on a continuous basis
3.5 ing/m  Suggested maximum dally limit based on chemical toxicity and intake of 2 liters  in any  one day
0.21 mg/e:  Suggested maximum daily limit based  on chemical toxicity and intake of 2 liters per day for 7  days

-------
                                                                       3-141

 reductions  for  Ion  exchange, precipitation,  or sorption.  Rather,  a  simple
 dilution  model  is used  in  which  the  mass  loading  from  mine discharge  is
 calculated  as the product  of concentration and discharge  (volume).   There are
 problems  with this approach.   In  some cases,  the calculated  concentrations  in
 flood  waters  probably exceed  the  solubility limits,  as in  the  case  of sulfate
 in  the  presence  of  barium.   In other  instances,  precipitation  of  barium
 sulfate  or iron  and  manganese hydroxides might greatly  reduce the  concen-
 tration  of  radium and uranium, both  of which would coprecipitate.   Thus  the
 stream concentrations shown  in Table 3.44 are probably high  (conservative).
 To  improve  the  analysis, additional comparisons  or parallels were drawn  using
 mill tailings solutions and  stream water quality  as  affected by mine  drainage
 and a  mill  tailings spill.
     Contaminant  concentrations   in uranium mill  tailings  liquids provide  an
 upper  limit estimate  of runoff concentrations  insofar as  the solvent action
 of  tailings solutions  maximize dissolution of  minerals  present  in the ore (J.
 Kunkler,  USGS,  written communication, 1979).  Table 3.46 is a compilation  of
 mill  tailings  water  quality  data  from numerous previous  reports  and  sum-
 marized  by  EPA and USGS  staff (Ka79; Ku79).   It  is apparent  that there are
 wide variations  as a function of mining region and  whether an acid or  alka-
 line leach  mill  circuit is used.  The Nuclear Regulatory Commission  (NRC79b)
 assumption  for  the composition of a  "typical" acid  leach mill is shown  along
 with other  average or representative  analyses.   A conservative (worst  qual-
 ity) analysis for  uranium  mill   pond  water quality is  estimated as follows
 (Table 3.47)  and  compared  to the average  concentrations  calculated from the
 mixing of mine effluent and flood volumes  (Table 3.44).
     The  data in  Table  3.47 suggest  that calculated concentrations  in the
 sub-basin  almost  without  exception  exceed those  in  uranium  mill  tailings
 solutions.  Thus,  the calculated  values  are probably erroneously high. Calcu-
 lated  concentrations  in  flood waters  of the basin and regional basin streams
 are considerably  less and are  in rough agreement with field  data,  at least
 for the  stable constituents.   Radium-226  and  lead-210,  however,  still  seem
 excessively  high  considering the  various  natural   processes of  sorption,
 precipitation, and  so on^   To understand  the degree to which natural  streams
 transport contaminants,  we  reviewed  water quality data  from  selected New
Mexico streams receiving mine drainage.

-------
Table 3 46  Radiochetnical & stable element/compound water quality  for  selected acid & alkaline  leach  uranium  mill  tailings  ponds in the Unittd States

i.

2.


_
4.

5,

6.

7.

8.

9.

10.






Tailings Pi la U Th-230 Ra-226 Pb-210
Location (mg/t) (pC1/z)
Split Rock, MY 10.5 41600 4800
(acid)
Canon City, CO — — — > —
(acid)
:
M h IIT V n £ft inn
United Nuclear, 14 --- 38
NH (acid)(a)
Anaconda !nj, 130 — §3 —
Well Feed, NH
Kerr-McGee, NH 32 — 58
(acidKa)
y»-HP, Grants, 150 — 52
NH (alkaline)
Huneca, WY 68.4 110 240
(acid)
USNRC-Uranium 8 0 150000 400 400
Hilling ElS(acid)
Representative
acid mllpond, *
in New Mexico1 ' — —
"Average" (Exclusive
of 9 and 10) 58 13920 760
Maximum value:
"Average" versus
HRC GE1S 58 150000 760 400
Po-210 As Hn Cu Se Mo V SO
fitjtt)
940 1.1 15.5 0.2 1 0.05

10.1 25.0 18 0.6 190 7.1 34000



50 3 0.005 3 30

340 — 0.03 — 6.3 4900

30 5 0.18 7 10

	 0.92 70 6,8 4300




400 0.2 500 50 20 100 0.1 33000





6 160 S,5 0.32 54 10 10000

-
400 i 500 50 20 100 10 30000
Na Fe IDS NH Ca NO Cl

280 11810 374 560 43.5 65

19000 280 77400 — 380 140 6500


icififtrtil „«» »..„ 	 — ^flfl
300 1000 	 700 	

1200 — — §9 — 7.4

500 1000 	 300 —

4300 — — 4.4 — 4.4 2

11700 0 5 — 460 — - li 16000

500 1000 35000 500 500 — 300





6200 510 227 485 40 1700


6200 1000 80000 500 500 40 1700
     (a)
     (b)
Source:   Ku79.
Ammonium ion.

-------
                    Table  3.47     Summary  of  flood  runoff  water quality  and
                                  uranium  mill pond  quality

Parameters
Uranium (mg/8,)
Radium-226 (pCi/i)
Lead-210 (pCi/i)
Polonium- 2 10 (pCi/O
Arsenic (mg/£ )
Manganese (mg/£ )
Copper (mg/x.)
Selenium (mgA )
Molybdenum (mg/i)
Vanadium (mg/£, )
Sulfate (mg/ji)
Concentration
in Concentration in
uranium mill flood waters of the
tailings solution sub-basin
58
760
400
400
6
500
50
20
100
10
30,000
235 -
229 -
2430 -
NC
2.1 -
NC
NC
11 -
48 -
NC
9.7 x 104 -
6970
6780
72000
(b)
61


220
2400
2.87 x 106
Concentration in
flood waters of the
Rio San Jose^ '
7
6.9
73
NC
0.062
NC
NC
0.34
1.4
NC
2901
(a)
(b)
Refer to Table 3.44.
Not calculated.

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                                                                       3-144
      The  USGS,  by water sampling  in  the  Churchrock area of New Mexico  (J.L.
 Kunkler,  USGS,  written communication, 1979),  determined water quality  in  an
 ephemeral  stream  receiving  rather  large and continuous mine discharges.  Data
 are  also  available  from the  Schwarzwalder Mine near Golden, Colorado (EPA72).
 Until  1972,  this  mine discharged  effluent high  in uranium, radium, and  trace
 elements  to  Ralston Creek and subsequently to two  lakes/reservoirs used for
 irrigation and potable supply (Section 3.2.3.2.1).
      The  way in  which surface runoff water quality is created or affected  by
 nnne discharge  is  complex.   In the  Churchrock  area,  numerous water quality
 changes occur as  the mine discharges flow toward Gallup  (Fig.  3.21 and Table
 3.48).  As  in other uranium mining areas in New Mexico, stream volume con-
 stantly decreases with  flow distance, but water quality  changes are erratic.
 infiltration, discussed in more detail in the following section of the report
 and  in Appendix  H,  amounts to  about 90  percent or more of the water loss.
 The  balance  is  by evaporation.   On a percentage basis,  similar losses occur
 in  the principal  drainage  courses in Ambrosia  Lake.   Dissolved  Ra-226 de-
 creases from 30 to  0.88 pCi/£ in a reach of 9.2  km and, on a later date, from
 14  to 0.95  pCi/£ in a distance of  26.7  km.   Based on  the  limited flow and
 water  quality data,  it appears that radium is strongly sorbed onto the stream
 sediments.   In October  1975, soluble uranium decreased  from 1150  to 740 yg/
 in the reach immediately below the mine discharges, yet  in July 1977 and May
 1978  uranium increased  in  the downstream direction from  580 to 860 ug/£  and
 from  970  to  2800  yg/£.   These changes bear no consistent relation to fluctu-
 ations  in dissolved or  suspended  solids along  the flow path.  Both  of the
 latter  parameters appear to increase in  the  direction of flow and  may  be  a
 result  of flash   floods  in   lower  reaches  of  the basin.   Uranium  appears  to
 undergo little change and  may actually increase  in the downstream direction.
 Of the  stable trace elements,  vanadium,  selenium, iron,  molybdenum, and zinc
 show no consistent change with distance.
     A third approach used  to assess surface  runoff quality involved a brief
 review of  some of the data collected to monitor a July 1979 tailings accident
 in New Mexico.    The  mill  tailings dam  at  the  Churchrock mill  breached and
                 3
dumped 223,000 m   of liquid and  1,000  metric  tons of  solids into  the Rio
 Puerco drainage  system.   The catastrophe immediately  spurred  numerous  water
quality studies  by State and Federal  agencies.   Numerous  inter-

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                                                  O  Twin  Lakes
                                                                     Mine Effluent, KM S UNC mines and Puerco River tributary
                                                                     below mines                                     '
                                                                     Pipeline Canyon at Trestle near Churchrock. N M
                                                                     Effluent from Pipeline Canyon, N M
                                                                     Puerco River near Sprmgst«ad, N M
                                                                     Puerco River at the Hogback near Gallup N M
                                                                     Puerco River a! Gallup N M
                                                                     Puerco River at Manuelito, N M
                                                                     Pyerco River near state line of  N M ana Am
Figure 3.21  Principal streams and surface water sampling stations in the Churchrock and Gallup areas

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               Table 3.48    Flow and water quality  in the Puerco  River  near Churchrock and Gallup, New Mexico
Location and
(Station Number)
Oct. 16, 1975
!
Puerco River tributary
below mines - (!)
Puerco River near
Springstead, NH -(4)
Puerco River at
Gallup, m - (6)
Puerco River at
Nanuelito - (7)
July 6, 1977
Puerco River tributary
below mines - (1)
Puerco River at the
, U nat.
m /mm pg/t as 11,0,,
14.5 1150
12.4 740
5.11
6.8(est) 540
11.55 580
6.47 860
Ra-226
pCIA
30
0.88
0.52
0.25
14
0.95
Total
Dissolved
430
480
640
800
410-
520
Solids, ma/.
Suspended
410
1600
2300
2800
260
15000
Suspended solids,
metric tons
per day Ba Cd
9.5
8.67
5.14
—
800 1
100 1
Concentrations vg/i
Cr Pb Mo V Zn Se As Fe
21-27 - 20
13-25 - 30
5.7 - 26 • - 40
--- - - . - -
06 - 0 25 1(3) 10
0 11 - - 50 20 1(19) 80
Hogback, near Gallup,
NM  - (5)

Puerco River near       15.5
State line (NM/AZ)  - (8)
83
0.27    600
44000
1700  4      02
30   5   6(7)  90

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               Table 3.48 <  (Continued)
Location and
(Station Number)
m /mm
                U nat.    Ra-226
                     Suspended  sol ids,
Total Solids, mq/a.    metric  tons    	
                                    Ba   Cd
as U,Qg  pCi/i     Dissolved    Suspended   per day
Cr   Pb   Ho
                                                                  Concentrations
                                                                                Zn    Se    As   Fe
Hay 25, 1978
Effluent from Kerr  ,    10.9
McGee and United Nuclear
Mines, Churchrock, KM-
(1)

Effluent from Pipeline   9
Canyon, NM - (3)

Puerco River near        10.88
Springstead, KM - (4)
(sampled 5/18/78)

July 11-12. 1978

Pipeline Canyon at       14.45
trestle near Churchrock,
m - (2)

Effluent from Pipeline   14.3
Canyon, NH - (3)

Puerco River near        —
Springstead, KM - (4)
            807
Z.6
2800
1100
940
1120
1130
1.5
0.8
8.6
1.3
2.2
                                                         12    19
820
12
230
260
240
28 - 110
16 - 0
11 -
6-11
9-13
— -
- 15
- 540
- 70
- 40
Source: New Mexico District office of ffie U.S. Geological Survey  (Peter Frenzel, written communication, 1979 and Kunkler, 1979).

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                                                                       3-148
 pretations  of   the  data  have  led  to  some  confusion,  compounded   in  some
 instances  by  inconsistent  sample collection  and  preservation.   However,
 several  general  findings  seem true.   Dissolution  of stable and  radioactive
 trace contaminants in flood  waters does  not seem significant  providing  that
 pH of  the flood  is  in  the  range  of 4 to  7.   After several days,  the  mill
 tailings  liquid  was  diluted and neutralized  and contaminant  concentrations
 decreased -- sometimes to  levels lower than before  the  accident  (J.  Kunkler,
 USGS, written  communication,  1979).  At  a  downstream sampling station  near
 Gallup,  some 30  kilometers  from  the spill,  dissolved uranium  and  radium-226
 about 36  hours  after the spill were  3.1  mg/£  and Q.9F pCi/jt, respectively.
 Suspended sediments  contained 19 pprn  uranium and 0.72 pCi/g  radium-226.   For
 the  latter,  this is  less than background.
      The  surface water quality  data pertaining  to discharge of  mine effluents
 and  to the  July  1979 spill  seem  to  indicate  rapid  and thorough removal  of
 radium-226 as a  result of  sorption,  precipitation, pH adjustment, etc.   How-
 ever,  stream sediment analyses  in   the Grants  Mineral  Belt  are  scarce,  and
 there are no analyses of  suspended  solids in flood waters.   Stream-bed sedi-
 ment  analyses by the USGS  indicate  less  sorbed  radium-226  and uranium  than
 expected   (Ku79).   During  this spill  incident, uranium  and  selenium  were
 relatively mobile in  surface  streams.
      From  the foregoing  review of  the literature  and field  data  and  prelim-
 inary  calculations of  runoff  quality  (Table  3.44), the following general  con-
 clusions  are  offered:
      1.    Radium-226  is  removed from  surface water  in  the  New Mexico study
 area  at  rates  of 0.5 to  3 pCi/£   per kilometer  of stream.   Final  concen-
 trations  are on  the  order of 0.25  pCi/£-   Resolution  in  successive  surface
 flows  occurs, but it is not significant.
     2.    Uranium and  certain stable trace  elements, such as selenium, van-
 adium, molybdenum, and iron, show no consistent reduction with flow distance
 and may show  an  increase, at  times.
     3.  ~Considerable more  data  collection  is  needed to understand the fate
 of dissolved and  suspended contaminants from mine drainage.  The present data
 base  is  rather  limited  in terms of sampling frequency,  variety  of  contam-
 inants measured,  and  types  of measurements,  for example,  suspended solids
analyses for flood waters.

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                                                                       3-149

      4.   With  the exception  of  radium-226, the  preliminary  calculations of
 runoff quality  in Table  3,44 are  believed  to be  a  first approximation of
 field conditions.  Additional  studies  specific to the  principal  mining  dis-
 tricts are  needed.
      5.   Dissolved  radium-226 concentrations  in  runoff  are  believed to be
 several  picocuries per liter or less under natural conditions.
      6.   Uranium  is  fairly mobile  and probably  the most  significant  radio-
 nuclide  in  uranium mine effluent.

 3.4.3.2    Impacts of  Seepage onGroundwater
      The  principal use of  grouncfwater  in  the immediate area  of  the  mines is
 for stock water.  Wells  in the highland areas are  typically  one to  two  hun-
 dred  meters  deep  and completed  in  underlying bedrock  strata (Co68j  Ka75).
 Contamination of  such  wells  by  mine discharge is  considered extremely  un-
 likely.   Shallow  wells  are few  in  number and  located along  major drainages
 that  are typically  ephemeral.  Such  shallow wells are  susceptible  to  con-
 tamination   if   located   downgrade   from  mine  discharges.  Municipal  water
 supplies  are usually  developed from  wells  because  groundwater  is  consistently
 available and has acceptable  suspended  and dissolved  mineral  contents.   The
 aquifers  tapped  by municipal wells are  mostly either quaternary lava  flows or
 deeper mesozoic  sandstone and carbonate sequences.  Considering  the  distance
 from  the  mining  centers  to  the communities  and the hydrogeologic  conditions,
 it  is 'unlikely  that mining  will  cause  measurable  deterioration of municipal
 water quality. The greatest likelihood  for contaminated  groundwater is  in  the
 shallow,  alluvial  aquifer beneath  streams  receiving  mine  drainage.   It  is
 extremely unlikely that  water quality  in  deeper, artesian aquifers  will  be
 adversely affected by  mine  discharge or  overland flow  affected by  solid
 wastes.   Shallow wells in these locations  have been constructed  in the past,
 but there are only a few  and  they  are used  for stock watering.   It  is poss-
 ible  that recharge of  substantial   quantities  of  mine  water  to the shallow
 aquifer will  encourage additional use of it,  in which case water quality will
 be of  concern,
     Table  3.49  shows  average and   extreme  concentrations  of  various common
and trace constituents  in  groundwater and  other  measures  of  water quality.
The data  are composited  from a previous  study (EPA75)  and from unpublished

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                                                                       3-150

 analyses  by  the  New Mexico  Environmental  Improvement Division (J.  Lazarus,
 NMEID,  oral  communication, 1979).  We  have categorized  the  data according to
 principal  aquifers, which are  in  areas where  the  groundwater  is not  believed
 to  be  contaminated  by mining.  Because it is common  for  a  well  to  tap  more
 than  one  aquifer,  the differences  in  water quality  in  Table  3.49 are  approxi-
 mate  at best.  The  data  reveal  no  sharp differences in water  quality amongst
 the three  major   aquifers.   The San Andres  Limestone,  a major  aquifer  for
 municipal  and  industrial  uses  in  the  Grants  and  Milan  areas,  has  equal  or
 greater concentrations  of most  constituents  as  compared  to the Westwater
 Canyon  Member and Gallup  Sandstone units, which  are closely associated  with
 uranium mineralization.
     Theoretical  analysis of  radionuclide  transport  in  groundwater  beneath
 and adjacent to a uranium mill  tailings pond  reveals  very  limited migration
 of  radionucl ides   in  groundwater (Se75).  Using  a seepage  rate of 4 x  10~
 cm/sec  and  a  10  percent  loss  of  soluble radionuclides,  numerical solutions
 for steady state  flow and  transport into unconsolidated sand for periods  of 5
 years and  20 years reveal up to several meters movement of  radium-226, thor-
 ium-230/ 234,  uranium, and lead-210 after 20 years  of  leaching.  For  example,
 radium  in  groundwater to  a  depth  of 3 meters is  10  percent  of that in the
 tailings pond.  Because the other isotopes tend to have even greater sorption,
 migration  distances  are  further reduced.  Although  field  studies  at three
 uranium  mill  tailings  piles  in the Grants  Mineral   Belt substantiate only
 local   migration  of  radionuclides  {EPA75}," extensive  lateral migration of
 stable  chemical  species  has  been  observed at  uranium  mills in  Colorado,
 Wyoming, and Washington   (Ka79,  Ka78a,   He79).   For example, with  respect to
 the old Cotter uranium mine at Canon City, Colorado, the Colorado  Department
 of  Health  has  stated  in  its  Final  Executive  Licensing  Summary,  August 17,
 1979,  that "contamination attributed to tailings  liquid was  observed in an
 off-site water well  ten  years  after the  mill began  depositing tailings, a
 [migration]  rate  of  over  five  hundred  feet  per year."  With  respect to the
 same  site,  one researcher has  stated  that  "the  soluble uranium  content of
 Lincoln Park ground  waters is highly elevated  with respect to  Arkansas River
water and  exceeds  suggested thresholds below which  ecological   and health
effects are  not expected. Molybdenum concentrations  in  these ground waters
greatly  exceed  irrigation standards  as  well as  the ALG based on  health and
ecological  effects...."  (Dr79).   Near neutral  pH and  relatively low concen-

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                                                                       3-151
           Table 3.49  Groundwater quality  in  principal  aquifers  in  the
                       Grants  Mineral  Belt,  New Mexico
Parameter
PH
Spec. cond.
ymhos/cm
IDS
Cl
mg/s.
Se
mg/£
V
mgA
Radium-226
pCi/£,
Uranium,
mgA,
Th-230,
pCi/£
Th-232,
PC1/A
Po-210,
pCi/ji

San Andres
Limestone
- 7.2^
(6.9 - 7.5)
1900
(720 - 3500}
1680
(490 - 4500)
98
(<0.2 - 270)
0.31
(0.01 - 1.52)
0.88
(0.4 - 1.3)
0.47
(0.11 - 1.92)
1.31
(0.04 - 2.6)
0.12
(0.017 - 0.52)
0.11
(0.0053-0.54)
0.75
(0.070 - 2.3)
Aquifer
Westwater Canyon
Member, Morrison Fm.
and
Gallup Sandstone
7.9
(6.7 - 9.15)
1800
(550 - 4250)
1160
(340 - 2300)
15
(0 - 98)
0.02
(0.01 - 0.13)
0.3
(0.3 - 0.3)
0.71
(0.07 - 3.7)
0.35
(0.02 - 1.0)
0.030
(0.015 - 0.053)
0.015
(<0. 01-0. 036)
0.42
(0.19 - 0.79)

Quaternary
Alluvium, Tertiary
Volcanics, and
Chinle Formation
7.6
(6.25 - 8.8)
1715
(700 - 4000)
1240
(490 - 3800)
57
(6.2 - 260)
0.59
(0.02 - 1.06)
0.55
(0.3 - 1.3)
0.22
(0.05 - 0.72)
4.72
(0.07 - 14)
0.212
(0.018 - 0.65)
0.123
(0.0094-0.99)
0.193
(0.010 - 0.55)
     (a)
        Mean and range of values shown.
     Note.—Selenium, vanadium, and uranium values for the limestone and alluvium/
chinle aquifers are based on 4 to 5 analyses and must be regarded as tentative.

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                                                                       3-152
 trations  in mine effluents,  together with  low hydraulic  heads,  indicate short
 migration distances  in  groundwater for radionuelides  and most  stable trace
 elements  in mine effluents.
      Discharge of water pumped  from  mines  to arroyos has both  hydraulic and
 water quality  impacts  on  shallow  groundwater in the alluvial aquifer.   The
 seepage  model  {Appendix  H)  and  scattered  field measurements  in the  Grants
 Mineral Belt substantiate  that  significant  groundwater recharge  is associated
 with mine discharge.  Water quality  effects  on groundwater are  poorly docu-
 mented,  however.  We  do not address  the   influence  of  impoundments used  to
 remove suspended solids from mine  effluents  before discharge.  Seepage water
 losses fr.im  such impoundments  are  believed to  be  small,  especially  when
 compared  to infiltration losses  in  the arroyos  and open  fields receiving  most
 of the wastes  not piped  to  mills  for  process water.   The Impoundments  are
 rather small and tend to  become self-sealing due to  settlement of fines.   In
 at least  one  instance in Ambrosia Lake,  the mine -pond is  lined to prevent
 seepage.
      Unpublished  flow and  water quality data from the U.S. Geological  Survey
 (P.  Frenzel,  written communications  1979)  document  conditions in  the  Rio
 Puerco drainage  near  Churchrock and Gallup,  New Mexico.   Figure 3.21 shows
 the  sampling  station locations, and  the   chemical  data are  in  Table 3.47.
 From October  1975 gaging  data, seepage  and  evaporation  reduce flow  9.39
  1                                                 3
 m /min in   a  reach  of  30.2  kma a  loss  of  0.31 m /min/km.   Conservatively
                                                                3
 assuming  20 percent  of this is  by  evaporation, seepage  is 7,5 m /min or  3.94
 x 10  m  /yr.   Gaging  data  for July 1977 and May  1978  similarly  indicate
 average bed losses  of 0,24 m /rain/km.  In the Ambrosia Lake district (data
 not  shown),  discharges (to San  Mateo Creek and Arroyo del Puerto) from about
 a dozen  mines total  about 10.8  x  10   m /year,  and   the  total length of
 perennial  stream  is about  15 kilometers.  Assuming an average stream width of
 one  meter and  the  above  evaporation rate, evaporation  and  infiltration are
       3                 3
 0.06  m /min  and  75§4 m  /min,  respectively.   In  this case,  infiltration
 amounts to  99  percent  of total loss.  Dissolved solids range from 520 to 1231
 mg/£ {mean 743 mg/£ )» and Ra-226 ranges from 0.2 to 23 pC1/£  (mean 6.6 pCi/n  ),
 Selenium and molybdenum average  0.010 and 0,22 mg/t, respectively.
     Considering  these two  areas,  evaporation averages about 4  percent of
mine  discharge versus  the value of  one percent calculated  in  Appendix H.
Obviously,  increased evaporation Is  accompanied  by  decreased infiltration.

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                                                                       3-15
 Infiltration ranges  from  at least 90  percent  to perhaps 99  percent  of mine
                                 3
 discharge,  or from 1.8 to  1.98  m /min per mine-   The foregoing field data and
 the more theoretical  approach used in Appendix  H show reasonable agreement on
 the relative amounts  of infiltration and evaporation.   We  conclude then that
 most of  the mine effluent  infiltrates within  relatively short  distances  of
 the mine(s) and recharges the  shallow water table.   The dissolved, generally
 nonreactive contaminants such as  chloride  and  sulfate are expected to  reach
 the water tables but  reactive  contaminants  such  as  radium-226 and  most  trace
 metals  would sorb  or precipitate  in the soil  (substrate)  in the  course  of
 infiltration.
      The influence of mine discharge on  groundwater quality  beneath formerly
 ephemeral  streams  now receiving  the discharge  is  currently under investi-
 gation   by  the  New  Mexico  Environmental Improvement  Division.   Monitoring
 wells have  been  installed at several  locetions along the Rio  Puerco (west)  in
 the Churchrock area and  San Mateo Creek in  the Ambrosia  Lake  district.   Table
 3,50 summarizes  partial  results  of samples taken  in  the  last-12  to  18 months.
 In  the  Ambrosia Lake  district,  marked  deterioration in  water quality between
 the Lee Ranch and Sandoval Ranch  stations  on San Mateo  Creek is a  result  of
 either  natural  causes and (or)  mine  drainage from a nearby  deep underground
 uranium mine. Between  Sandoval  Ranch  and  Qtero Ranch  even  more  pronounced
 changes occur.  In  this short reach  of 2.5 km, contaminated flows  from uranium
 mines,  ion-exchange plants, and  seepage from  an acid  leach uranium mill  enter
 Arroyo  del   Puerto,  a  tributary  of  San Mateo  Creek.   Additional  study  of
 surface water quality in the  Arroyo  del  Puerto is  recommended  to further
 characterize  the  obviously  interconnected  surface  water   and  groundwater
 systems.
      In  the  Churchrock areas drained  by  the  Rio Puerco, groundwater quality
 changes  in  the  downstream  direction are not readily apparent (Table 3.50).
 Although  there  is an  acid  leach mill also adjacent  to  the  Rio Puerco  trib-
 utary receiving  the  mine discharges, the mill is relatively new  (1978 start-
 up)  and may  not yet influence stream  quality.  Most  of the discharge from one
 of  the  two  mines is used as mill  feed water, thereby causing decreased dis-
 charge  from  the mines  to the stream.  Nevertheless,  the  reach  of the perennial
 stream  is increasing,  indicating infiltration of remaining mine effluent and
addition  of  water to  storage  in  the  shallow aquifer.   Storage changes have
been confirmed by  static groundwater level measurements  in  the area east of

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                                                                       3-154
           Table  3.50   Groundwater  quality  associated  with  the  San Mateo  Creek
                       and  Rio  Puerco  (west) drainages  in the Grants  Mineral
                       Belt,  New Mexico
Station
                          Sulfate
                          (rag/ £ )
                                        Molybdenum
                      Selenium    Uranium
 San MategCreek

 Lee Ranch

 Sandoval Ranch

 Otero Ranch
                         125.7

                       225-274

                       463-989
103-235

350-516
 < 5         <10

4-14.7       293-400

 33-59        680-860
Rio Puerco  (west)

Hwy. 566 Bridge on
N. Fork Rio Puerco

Rio Puerco at
Fourth St. Bridge,
Gallup
                       101-223


                       163-244
<10-284


<10-215
 20-22


   9-26
530-760


 550-625
Source:  'Based on unpublished 1978 data developed by the New Mexico
         Environmental Improvement Division (J. Lazarus, oral
         communication, 1979).'
Gallup. A massive spill of mill tailings into the Rio Puerco occurred in July

1979 and will complicate water quality investigation, insofar as the mine and

mill influences-are  now superimposed in terms of both solid and liquid waste

loadings in  the  watershed.   The tailings "flood," estimated to contain about
         O                 —
360,000 m  of fluid and 1000 MT of solids, was traced into Arizona.

     In summary  and  considering  the high volume of  dilute mine discharges,

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                                                                       3-155

 which are  enriched  in certain  stable and  radioactive  toxic  trace  elements
 (EPA75;  Hi77), we recommend  that  water quality effects of  mine discharge be
 very carefully evaluated  in at least a few selected  areas.   Available stream-
 flow data  indicate that  infiltration  is  the principal  means of disposal,  yet
 the water  quality data base,  in particular, is rather weak  to assess whether
 adverse  impacts  are  likely.  It  is expected  that  future   discharges  in  the
 Churchrock area  alone will amount  to  about 40 m /min and  will  contain  less
 than 400  mg/«.   dissolved  solids,  most of which  is  sodium  and  bicarbonate.
 Dissolved  concentrations  of uranium, radium, iron, selenium, and vanadium  are
 elevated   relative  to  drinking water limits  and  infiltration  of  uranium,
 selenium,  and  possibly other stable  elements warrants  study.  Use of  settling
 ponds and  barium chloride  treatment  greatly  reduces  the   suspended  solids,
 uranium,   and  radium  concentrations.  The  final   composition and  ultimate
 disposal  of pond  sediments and added chemicals  is  essentially  undocumented
 and bears  additional  investigation.  Lastly, mine dewatering  creates  marked
 regional cones of depression  and reduces  the flow  of water to  existing  supply
 wells and  the  baseflow component in major  drainage  systems such as the  San
 Juan River (Ly79).

 3.4.4     Gases  and Dusts  from Mining  Activities

 3.4.4.1    Radon-222 in Mine Exhaust  Air
      Unlike surface mines,  large capacity  ventilating  systems  are  required  in
 underground uranium  mines,  primarily  to   dilute  and remove  Rn-222  that  em-
 anates  from the ore  (Section  1.3.3).   Ventilation  rates  vary  from  a  few
 hundred  to a few  hundred  thousand cubic  meters of  air  per  minute,  and mea-
 sured  Rn-222  concentrations  in  mine  vent  air range  from 7 pCi/i to  22,000
 pCi/s. (Ja79b).   The concentration  of Rn-222  in mine  exhaust air varies  de-
 pending upon ventilation  rate, mine size  (volume) and age,  grade of exposed
 ore,  size  of active working areas, rock characteristics (moisture  content  and
 porosity),  effectiveness   of  bulkhead  partitions, barometric  pressure,   ore
 production  rates,  and  mining practices. The emanation of Rn-222 dissolved  in
water that  seeps into most mines may also contribute to Rn-222  in  the exhaust
air.

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                                                                       3-156

      Because  of the numerous  variables  that affect Rn-222 concentrations  in
mine  air» it  is difficult  to confidently model  radon releases from  under-
ground  mines.  A useful model  would  be  one that would  relate  radon  emissions
to  the  production  of  U30g.   Measurements  relating radon  emissions  to ore
production  have been  made  at  seven  underground  uranium mines in New  Mexico
(Ja79b).   The  results  of these measurements  varied at  the  different mines
from  1,380 to  23,500  Ci Rn-222  per APR*, with  an  average  rate of 4,300  Ci
Rn-222  per  AFR.   The higher emission rates  were  noted to occur at  the older
mines.   This was  believed  due  to  larger surface  areas of exposed ore and
sub-ore  in  the  older mines.   That is, inactive mined-out areas increase with
mine  age, and  the  ceiling, floors,  and walls of  these areas stiTi contain
certain amounts  (if ore and  sub-ore.   Radon emanating from these suffice areas
tend  to  increast the  Rn-222 content of exhausted mine air  unless   !hese in-
active  areas  of the  mine (rooms,  stapes,  drifts,  etc.)  are  e~-"actively
sealed.   Because the  radon  emission  factor is so variable in  terms  of Ci per
AFR,  an emission rate  based on cumulative U30_ mined  has  been proposed for
modeling  purposes  (Ja79b).   It is  believed that  this  relationship  would
reduce the apparent dependence  of the emission rate on  the mine age. However,
data  are  not presently available to make this  latter correlation.
      Although the average measured  Rn-222 exhaust factor  of 4,300  Ci/AFR is
tentative and may  be  improved  by studies in progress (Ja79b),  it is the only
value currently  available for modeling  purposes and will, therefore, be used
in the  present  assessment.   Assuming that 1 AFR is equivalent  to 245 MT** of
U308  (Ja79b),  0.017 Ci  of  Rn-222 will  be released from  the  mine  vents  per
metric  ton  of  0.1  percent  grade ore  mined.   This emission rate will include
all  underground  sources,  i.e.,  emanation  from  exposed  ore  and  blasting,
slushing,  loading,  and transporting  ore bearing rock.   Radon-222  emissions
were  estimated   for  the  two  model   underground  mines  by multiplying  their
 *AFR = Annual Fuel Requirement for a 1000 MWe LWR.
**The AFR value on which the exhaust factor was based.

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                                                                       3-157

 respective  annual  ore capacities  by  the  above  emission  rate.  Table  3.51
 lists  the results.
     The estimated  annual radon release  computed  for the average underground
 mine  is compared below with  releases  reported elsewhere.  Agreement  is  rea-
 sonably good.

     	Source	                    Annual  Release  of Rn-222,  Ci
     This Study                                         306
     Tr79                                          289 - 467^
     TVA78a                                           1577
     TVA78b                                            180
     TVA79                                             215
     Th79                                               87
      a'  Adjusted for 0.1 percent ore grade.

     By  properly capping  the  exhaust vents  and sealing  the  shaft and mine
entrance,  radon  emission  rates  from inactive  mines  will  be  a  negligible
fraction of the  radon release rate that occurs during active mining.

3.4.4.2   Aboveground Radon-222 Sources
     Radon-222  will   be   released  from  the  following  aboveground  sources.
     1.   Dumping ore, sub-ore, and waste rock from the ore skip into haul
          trucks and unloading them on their respective piles.
     2.   Reloading ore from the stockpile after a 41-day residence time.
     3.   Emanation from waste rock, sub-ore, and ore storage pile surfaces.
     The annual  quantities  of  Rn-222 released by  sources  1  and 2 were esti-
mated using the following factors and assumptions.
          Radon-222 is in secular equilibrium with U-238.
          The density of ore, sub-ore, and waste rock is 2.0 HT/m .
          Annual production rates of ore and sub-ore are equal and
                                4                                  5
          assumed to  be 1.8 x 10  MT at the average mine and 2 x 10
          MT at the average large mine (Sections 3.4.1.1 to 3.4.1.3).
          The production  rate ratio of ore to waste rock is 9.1:1 (Sec-
          tion 3.4.1.1).
                                                                   3
          All  Rn-222  present is available for release, 0.00565 Ci/m  per

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                                                                 3-158
Table 3,51     Estimated annual  radon-222 emissions from
               underground uranium mining sources

Average
Source Miners Ci/yr
Underground
Mine vent air
A bo ve|| round
Ore loading and
dumping
:,:ub-ore loading
ind dumping
Waste rock loading
and dumping
Reloading ore from
stockpile
Ore stockpile exhalation
Sub-ore pile exhalation
Waste rock pile exhalation
Total
^Annual production of ore
2.0 x 103 MT.
^ 'Annual production of ore
x 104 MT.

306

1.4
0.5
0.003
1.4
6.3
61
0.5
377
and sub-ore =
and sub-ore =
Average Large
Mine^, Ci/yr

3,400

15.3
5.3
0.03
15.3
53
338
2.6
3830
1.8 x 10 MT, waste rock =
2 x 105 MT, waste rock - 2.2

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                                                                       3-1S9

           percent U,0g (N179), with an emanation coefficient of 0,27
           (Au78, Tanner, A.B,, Department of Interior, Geological
           Survey, Reston, VA.» 11/79, personal  communication).
           The quantities of LUQg present in ore, sub-ore, and waste
           rock are 0.10 percent, 0.035 percent  and 0.0020 percent,
           respectively (Sections 3.4.1.1 to 3.4,1.3).
      Substituting  the  above  values  into the  following  equation yields  the
 Rn-222  releases  given in  Table 3.51  for  the  average mine  and  the  average
 large mine.
      Rn-222 (C1/yr)  = (percent LLQD) f 0.00565 Ci  1(0.27)   /   m3
                                 •J G  I  O
                                        ij
1   1(0.27)  /  m3
ent/        b.O WT
                                       m  ,  percent/        12.0 MT
                     x (Production Rate, MT)                        '    (3.11}
                                         yr
 These releases  are  maximum values  since very little time will have  elapsed
 between   the  underground  (blasting,  slushing,  loading,  etc.)  and  surface
 operations.   A significant amount  of  the radon that is  available for  release
 will   emanate  during  the  underground  operations  and  invalidate  the  first
 assumption above  concerning  radioactive  equilibrium.   Nevertheless,  these
 estimated maximum  releases  are  very small in  comparison  to the  radon released
 from  the mine exhaust vents.
      The emanation of Rn-222 from waste rock,  sub-ore, and ore  piles is  based
                                    o
 on  an exhalation rate of  0,092  Ci/m *yr*percent ILQg (N179) and ore  grades of
 0.002 percent,  0.035 percent,  and  0,10 percent,  respectively.   Surface  areas
 of  the  ore piles  (Table 3.37),  sub-ore piles  (Table 3.38), and waste rock
 piles (Table  3.36)  were  ysed  in these calculations.   Applying these  para-
 meters,  the annual  Rn-222  emissions  from  the waste  rock,  sub-ore, and ore
 piles at the  average mine  and  average large  mine were  computed.  Table 3.51
 gives the results.  Total  annual  Rn-222 emissions during underground mining
 operations  is  the sum of  the  releases from  all  sources considered:  377 Ci
 from  the average mine  and 3830  Ci  from the average  large mine.  More than 801
 of  the Rn-222 emissions results from the mine  vent  air.

 3.4.4,3    Dusts andFumes ~
      Vehicular  emissions  resulting  from the  combustion  of hydrocarbon fuels
 in  gasoline ind diesel-powered  equipment are considerably less  at underground
mines  than  at  surface mines (Section  3.3,4.1),   The principal  emissions are

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                                                                       3-160

 participates,  sulfur  oxides,  carbon  monoxide, nitrogen  oxides,  and  hydro-
 carbons.  The quantity  of  these combustion  products  released  to  the atmosphere
 depends  on the  number,  size,  and types of  equipment  used,  all of which  are
 directly  related  to ore  production.
      EPA  has estimated the  following emissions  from mining 1350 MT of  ore  per
 day  from  an underground mine (Re76).

           Pol lutant                     Emissions per Operating^ Day, Kg/d
           Participates                                 2.4
           Sulfur  Oxides                                5.0
           Carbon  Monoxide                             41.9
           Nitrogen Oxides                             68.1
           Hydrocarbons                                 6.9

     Assuming  a  330  operating-day year (Ni79), these emissions were adjusted
 according  to the  annual ore production of the average mine (1.8 x 10  MT) and
 the  average  large mine  (2 x  10  MT).  Table  3.52 lists  the total  airborne
 combustion product emissions.  These emissions are  small  compared to those at
 surface mines  (Table  3.30).  For example, these estimates  indicate  that the
 emissions  of  combustion  products  at the average surface mine  are  more than
 100  times  greater than those at the average underground mine.
     At underground mines,  dust  is produced by both  underground  and surface
 operations.  No  measurements have  been made of dust  concentrations  in mine
 exhaust air.   Because  underground mines are wet, which  greatly reduces dust
 production, and   since a  large  portion of  the dust  produced would  probably
 deposit underground, dust emissions  from underground  operations are probably
 relatively small.  Hence, dust emissions from underground operations  will not
 be assessed.
     Aboveground  sources of dust include dumping ore,  sub-ore, and waste rock
 from the skip into haul trucks; dumping these materials onto their respective
 piles; reloading  ore  from the  stockpile; using dirt  haul  roads by vehicular
 traffic; and dust suspended by the wind from the waste rock,  sub-ore, and ore
 piles.  These  sources "will  be  assessed as  was done  previously  for surface
mines (Section  3.3.4.1).

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                                                                       3-161
           Table  3.52      Estimated  air pollutant emissions  from heavy-duty
                          equipment  at underground uranium mines

Pollutant
Participates
Sulfur oxides
Carbon monoxide
Nitrogen oxides
Hydrocarbons

Average Mine^ '
32
67
560
910
92
Emissions, Kg/yr^a'
Average Large Mine^
350
740
6,210
10,100
1,020

C)





        'Based  on Re76 and  330  operating  days  per year.
                                         4
        Annual ore  production  =  1.8  x  10  MT.
      fc)                               5
      v  'Annual ore  production  =  2 x  10  MT,
     Dust  emissions  will  vary  over a  wide  range  depending  upon moisture
content, amount  of fines, number and types  of equipment operating, and cli-
matic  conditions.  Because ore is generally wet, the relative amounts of dust
produced  from its mining  and handling  are  usually  small.   The  following
emission  factors were  selected  from those suggested  by the EPA for loading
and dumping operations  (Hu76,  Ra78»  Da79):
          truck  loading = 2.5  x 10~2 kg/MT; and
                                  _9
          truck  dumping = 2.0  x 10   kg/MT.
     Average  annual  dust  emissions  were estimated for the aboveground mining
activities by applying  these emission factors to the ore, sub-ore, and waste
rock production  rates of the average mine and average large mine.  Table 3.53
lists  the results.  One-half the emission factor  values were applied to ore
and  sub-ore  because  they  are generally wet,  except when reloading ore from
the stockpile.   In that case, it is assumed  to  have dried during the 41-day
residence period  (Section  3.4.1.2).  Also,  the  emission  factor  for  truck
loading was  assumed valid for  loading the haul trucks from the mine skip. The
dust emission  for  truck dumping may be high since it was based on dumping of
aggregate,  which would  have  a smaller  particle  size distribution  than the
ore, sub-ore, or waste rock (Hu76).

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                                                                       3-162

      The movement  of heavy-duty  trucks  is a  Urge source  of dust  at  most
 uranium  mines.   The  magnitude  of  this  source  depends  upon a  number  of
 factors, including  the particle size distribution  and moisture content of the
 road bed material, vehicular  speed  and distance traveled,  and meteorological
 conditions.   Emission factors  for heavy-duty  haul trucks  (1.15 kg/VKmT)  and
 light duty vehicles  (1.03  kg/VKmt)  are the same  as  those  computed  for these
 vehicles at  surface mines (Section 3.3.4.1).   Dust emissions  for the movement
 of  heavy-duty  haul  trucks  were  estimated  using  the  appropriate  emission
 factor and assuming —
          31.8  MT truck  capacities;
          round-trip  haul  distances  of 1.61 km to  the ore and sub-ore
          piles and 3.22 km to the waste  rock  pile;  and
          the annual  production  rates given  in  Sections  3.4.1.1,  3.4.1.2
          and 3.4.1.3.
 Table 3.53 lists  the  results.
      Additional  dust  emissions  will  occur from light-duty vehicular  traffic
 along access roads.   Using the emission  factor  derived  in  Section  3.3.4.1
 (1.03 kg/VKmt)  and  assuming that  there are 16 km of access  roads traveled 4
 times a day  during  the  330 operating  days  per year,  about  22 MT of dust will
 be  produced  from  this source  annually.   Emissions that  occur during  haulage
 road  maintenance  is relatively  small and will not  be  considered.
      Heavy-duty,  haul truck traffic  at underground  uranium mines  produces
 considerably  less dust than  at  surface  mines.  This  is to be  expected  because
 of  the  vast  quantities  of  overburden that must  be transported as  well  as
 larger  ore and sub-ore capacities  at surface-type  mines.
      The  dust emissions  computed above  for  transportation assume no effective
 dust  control  program.   But,   haul  roads  are  normally sprinkled  routinely
 during  dry  periods,   and  stabilizing  chemicals  are  applied  to  roadways,
 usually  to  the  ore  haul   roads.   Dust emissions  along haul  roads  can  be
 reduced by 50 percent from  sprinkling and up to 85 percent by the application
 of stabilizing chemicals (EPA77b,  Da79).
      Table 3.53  also  lists  average  annual  dust  emissions  caused  by wind
 erosion of waste rock,~sub-ore, and ore piles at the model  underground mines.
 Emission  factors,  computed  in  Appendix I, are  2.12 MT/hectare-yr  for waste
 rock  and  sub-ore  piles  and 0.040 kg/HT  for the  ore stockpiles.   The first
emission  factor  was multiplied  by the waste  rock  and  sub-ore pile  surface

-------
Table 3.53   Estimated average annual dust emissions  from underground mining activities
;
Source^
Loading truck from
skip at mine shaft
Truck dumping at
piles
Reloading stock-
(el
piled ore1 '
Wind suspended dust
from piles
Transportation^'

Average Mine*1
Ore^ Sub-ore^
0,23 0.23
0.18 0.18
0.45 NA^f'
0.72 4.0
1.0 1.0
Dust
Emissions
, MT/yr

3' Average Large Mine^ '
Waste Rock
0.05
0.04
NA
0.57
0.23
Ore^
2.5
2.0
5.0
8.0
11.6
Sub-ore' c'
2.5
2.0
NA
22
11.6
Waste Rock
0.6
0.4
NA
3.0
2.6
                                               4                                    3
         on annual production rates of 1.8 x 10  MT of ore and sub-ore, and 2.0 x 10  MT of waste rock.
'  'Based on annual production rates of 2 x 10  MT of ore and sub-ore, and 2.2 x 10  MT of waste rock,
^Assumed wet.
*  •'Aboveground activities.
ie\
v  'Assumed dry,
      - Not applicable.
        emissions from heavy-duty, vehicular traffic along ore, sub-ore, and waste rock haul roads.
                                                                                                               00
                                                                                                               1
                                                                                                               CTs

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                                                                       3-164

 areas   given   in   Tables   3,36  and   3.38,   respectively,   while   the  second
 factor  was  multiplied  by  the  annual  ore  production.
     Table  3.54 shows  annual contaminant  emissions  caused by mining  activ-
 ities  (loading and dumping)  according to  source location, at the mine shaft
 and  at the  piles.  Contaminant  emissions  were computed  by multiplying  the
 total  annual  dust emissions  at  each  pile  {Table  3.53)  by  the respective
 contaminant   concentrations   in   each  source—waste  rock   (Section   3.4.1.1;
 Table 3.16),  sub-ore  (Section 3,4,1.3; Table  3,19), and ore (Section  3.4.1.2;
 Table  3.19).   -Contaminant emissions at  the site of  the mine shaft were  com-
 puted  by  multiplying  the annual  dust emissions of ore,  sub-ore, and over-
 burden  (loading truck  from skip  - Table  3.53) by their respective contaminant
 concentrations.  The  three products  of the  multiplication  were then summed  to
 give  the  values listed in the 4th and 8th data columns of Table 3,54.  The
 health  impact of  the sources  at  each location will be assessed separately  in
 Section 6.1,
     Annual  contaminant  emissions  due  to  wind  suspension  and  transport  of
 dust are listed in Table  3.55.   These values were computed  by multiplying the
 annual mass emissions  (Table  3.53) by the contaminant concentrations  in waste
 rock,  sub-ore, and  ore  listed   in  Sections  3,4.1.1,  3.4.1.3,  and   3.4.1.2,
 respectively.   The uranium and uranium daughter concentrations in dusts from
 all  sources were  also  multiplied by an activity  ratio  (dust/source) of 2.5
 (Section 3,3,1.2).  Although  some  metals  may also  be present  as  secondary
 deposits, it was believed  that there were insufficient data to justify multi-
 plying their  concentrations by the 2.5 ratio,
     The dust  emissions from vehicular traffic listed in  Table  3.53  (trans-
 portation)  were summed with  that  produced  by  light  vehicular  traffic  (22
 MT/yr)  and  considered  one source of  emissions.  Concentrations  of  contam-
 inants  in  haul road  dust have  not  been measured and  are  not  known.   Some
 spillage of ore and  sub-ore  along haul  roads will  undoubtedly raise  uranium
 levels in roadbed  dust.  As  an estimate, uranium and daughter concentrations
 in the dust  were  considered  to  be twice background, 8ppm   (2,7 pCi/g),  while
 concentrations  of  all  other  contaminants  were  considered  to  be  similar to
 those  in  the  waste"rock (Section  3.4.1.1).   Table  3.56 shows  the annual
emissions  computed with these assumptions.

-------
Table 3.54  Average annual emissions of radionuclides (yCi) and stable elements (kg) from
            mining activities at the model underground mines
Average Underground Mine^
Contaminant
Arsenic
Barium
Cobalt
Copper
Chromium ,
Iron
Mercury
Potassium
Magnesium
Manganese
Molybdenum
Nickel
Lead
Selenium
Strontium
Vanadium
Zinc
Uranium-238 and
each daughter
Thorium-232 and
each daughter
Waste Rock
Pile Site
0.0004
0.012
NR(b)
0.0007
< 0.002
0.24
< 0.0003
0.28
NR
0.02
0.0001
NR
0.0009
0.0001
0,006
0.004
0.0008
0.6
0.04
Sub-ore
Pile Site
0.02
0.17
0.003
0.01
0.004
2.8
ND(cJ
4.5
0.63
0.17
0.02
0.004
0.01
0.02
0.02
0.25
0.005
45"
0.4
Ore
Pile Site
0.05
0.58
0.01
0.04
0.01
9.9
ND
16
2.2
0.60
0.07
0.01
0.05
0.07
0.08
0.89
0.02
450
6.3
Mine
Site
0.04
0.44
0.007
0.03
<0.01
7.5
<0.001
12
1.6
0.47
0.05
0,009
0.04
0.05
0.07
0.65
0.01
222
2.8
Average
Waste Rock
Pile Site
0.004
0.12
NR
0.007
<0.02
2.4
< 0.003
2.8
NR
0.19
0.001
NR
0.009
0.001
0.06
0.04
0.008
6
0.4
Large Underground Mine^ '
Sub -ore
Pile Site
0.17
1.8
' 0.03
0.12
0.04
3.1
ND
50
7.0
1.9
0.23
0.04
0.16
0.22
0.26
2.8
0.06
495
4
Ore
Pile Site
0.60
6.4
0.11
0.43
0.14
110
ND
175
25
6.7
0.81
0.14
0.55
0.77
0.91
9.9
0.20
4,990
70
Mine
Site
0.44
4.8
0.08
0.32
< 0.13
82
0.005
129
18
5.1
0.58
0.10
0.40
0.55
0.74
7.1
0.16
2,410
31
emissions from Table 3.53.

Not reported.

Not detected.
                                                                                                                    Co
                                                                                                                    I
                                                                                                                    en
                                                                                                                    en

-------
Table 3.55 Average
           (kg) in
annual emissions of radionuclides (yCi) and stable elements
wind suspended dust at the model underground mines
Average Large Underground Mine
Waste
ntaminant Pi
r
Arsenic '
Barium
Cobal t
Copper
Chromium
Iron
Mercury
Potassium
Magnesium
Manganese
Molybdenum
Nickel
Lead
Selenium
Strontium
Vanadium
Zinc
Uranium-238 and
each daughter
Thonuin-232 and
each daughter
Rock
le
0.03
0.87
NR{a)
0.05
<0.15
18
<0.02
21
NR
1.5
0.008
NR
0.07
0.006
0.45
0.30
0.06
45
3
Sub-Ore
Pile
1.9
20
0.35
1.3
0.44
345
ND(b)
550
77
21
2.5
0.44
1.7
2.4
2.9
31
0.64
5,450
44
Ore
Stockpile
0.69
7.4
0.13
0.49
0.16
126
ND
200
28
7.7
0.92
0.16
0.62
0,88
1.0
11
0.23
5,700
80
Average
Waste Rock
Pile
0.005
0.17
NR
0.01
< 0.03
3.4
< 0.005
4.0
NR
0.28
0.001
NR
0.01
0.001
0.09
0.06
0.01
9
0.6
Underground Mine
Sub-Ore
Pile
0.34
3.7 .
0.06
0.24
0.08
63
ND
100
14
3.8
0.46
0.08
0.31
0.44
0.52
5.6
0.12
990
8
Ore
Stockpile
0.06
0.66
0.01
0.04
0.01
11
ND
18 -
2.5
0.69
0.08
0.01
0.06
0.08
0.09
1.0
0.02
513
7.2
                                                                                                         CO
                                                                                                         I
                                                                                                         Ol
                                                                                                         Ch
    -  Not  reported.

    -  Not  detected.

-------
                                                                 3-167
     Table 3.56  Average annual emissions of radionuclides (pCi) and
                 stable elements (kg) from vehicular dust at the model
                 underground mines
Contaminant
Arsenic
Barium
Copper
Chromium
Iron
Mercury
Potassium
Manganese
Molybdenum
Lead
Selenium
Strontium
Vanadium
Zinc
Uranium- 2 38 and
each daughter
Thorium-232 and
each daughter
Average Large
Underground Mine^
0.43
14
0.86
<2.4
287
<0.38
335
23
0.12
1.1
0.10
7.2
4.8
0.96

129

48
Average
Underground Mine^
0.22
7.0
0.44
<1.2
145
<0.19
170
12
0.06
0.53
0.05
3.6
2.4
0.48

65

24
(a)
(b)
Mass emissions = 47.8 MT/yr,
Mass emissions = 24.2 MT/yr.

-------
                                                                       3-168
3.5   In Situ Leach Mining
      Because  in  situ  leaching of uranium  (see general description  in  Section
1.3.4)  is  in  its  infancy,  a  data base  for performing  a  detailed  generic
environmental  assessment  does not presently  exist.   The  fact that the  para-
meters  for  assessing  this process are so  site specific and depend  upon  oper-
ational  procedures  further  impedes  a generic  assessment.  Current research
projects  may help to  resolve many of the present uncertainties and  provide
the data  needed  to better quantify the potential source terms (La78).
      In view  of  the  expected future expansion  of  this uranium mining method
(Section  1.3.4), a qualitative  assessment that can  be modified  later when
additional  data  become available was deemed  necessary.   This assessment was
possible  because of  recent laboratory experiments  and field  measurements  at
pilot-scale plants (Wy77, Ka78b, NRC78b, Tw79).
      Similar to  other  uranium mining methods, in situ leaching also produces
liquid, solid, and airborne  wastes.   However, the quantities of these wastes
and their characteristics  differ considerably from those produced at  surface
or underground mines.   Also,  because the  recovery, drying, and  packaging  of
the U30g  produced is  often  performed at the mine  site, wastes  from  these
processes should probably be included in the mine assessment.
      This  assessment  uses the  parameters of a hypothetical  "typical"  com-
mercial-sized  in situ  solution  mine.   Unlike surface or  underground  mines,
relatively  few in  situ  facilities exist, and they are all somewhat different
because of  site  specificity and  the  rapid  development  of  new  or modified
techniques.  The following parameters for the hypothetical  mine were based
upon  those  of the Highland,  Crownpoint,  and Irigaray uranium  projects and
those reported by Kasper et al.  (1978) (Wy77, NRC78b,  TVA78b).
                   The Hypothetical In^ Situ Solution Mine

     (1)  Size of deposit = 52.6 hectares
     (2)  Average thickness of ore body -8m (Ka78b, NRC78b)
     (3)  Average ore grade = 0.06 percent UgQg (Ka78fa, Tw79)
     (4)  Mineralogy - Sandstone

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                                                                       3-169
      (5)  Ore  density  *  2  MT/m3
      (6)  Ore  body  depth * 153 m
      (7)  Mine life =  10 years (2-yr  leach  period  in each of
          5  sectors)
      (8)  Well  pattern = 5 spot (NRC78b,  TVA78b» Ka78b)
                         Injection wells  =  260
                         Production wells = 200
                         Monitoring wells - 80
      (9)  Annual UgOg  production * 227 MT (Wy77, NRC78b,  Ka78b)
     (10)  Uranium leaching  efficiency = 80  percent  (Ka78b)
     (11)  Lixlviant *  Alkaline
     (12)  Lixiviant flow capacity » 2,0002./min (Ka78b, Wy77» NRC78b)
     (13)  Lixiviant bleed  = 50*/fnin (2.5 percent) (Wy77,  NRC78b, TVA78b)
     (14)  Uranium In Lixiviant = 183 mg/i   (TVA78b,  Ka78b, NRC78b)
     (15)  Calcite (CaC03)  removal required = 2 kg calcite per kg ILQg
          (Wy77)

     The  solid, liquid,  and  airborne wastes generated  by  this facility are
described below.  Wastes and  quantities generated, as well as operations and
procedures selected, will  naturally  differ  to varying degrees  from those at
some operating sites.

3.5,1    . Sol id Hastes
     The  quantity  of   solid wastes  generated depends upon  the  leachate, the
ore  body,  and  operational procedures  that effect  the  mobilization  of ore
constituents.   Little  information  is available  on  the  quantities  of solids
generated because  of  this  site dependence, the  newness  of  the  process, and
the  apparent  relatively small  quantities  that  are produced.   Examples  of
solid wastes  that  might be expected  to  be generated by the  alkaline leach
process are listed  below:
     (1)  Materials filtered from  the  lixiviant  line
     (2)  Sediments  from  the surge  tanks
     (3)  Calcium carbonate from  the calcium control  unit

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                                                                       3-170
      (4)  Barium sulfate  from  the  contaminant  control  in  the
          elution/precipitation circuit  of  the recovery process
      (5)  Materials deposited  in the evaporation  ponds
      (6)  Drill hole residues
      (7)  Solids from aquifer  restoration

Sources1 and 2
      No  information concerning quantities  of  solids  from these two  sources
could  be  found, in  the literature, but they are described  as being relatively
small  compared  to  other  sources   (NRC78b).  These  wastes are transferred  to
evaporation ponds and retained beneath a liquid seal,
Source 3
     One  of  the  larger sources of solids is the calcium control unit  (Wy77).
Calcite,  CaCOg, which  is  removed  prior  to  injection of the refortifled lixi-
viant, coprecipitates  radium and  any residual uranium.   It has been reported
that  the  amount of  calcite produced  is less  than  2.8 kg per  1  kg of UoOg
recovered (Wy77).  Assuming  this ratio to be 2.0, and if Ra-226 is in  secular
equilibrium  with  U-238 in  the ore,  and 2,5  percent  is   solubilized  by  the
lixiviant  (Wy77,  NRC78b),  454  MT  of  calcite  will   be  produced  annually and
contain a total  of  1.6  Ci  of Ra-226.  Also,  calcite  has been  observed  to
contain between 1 to 2 percent U,,00 by weight  (Wy77).  Assuming an average  of
                                a a
1,5 percent  lUQg,  about  1.9 Ci (6.8 MT U,Qg)  of U-238 may also be present  in
the calcite waste.
     Radium-226 and its daughter, Rn-222, are  probably the most radiologically
significant radionuclides associated  with  uranium mine wastes, and the small
amount  of Ra-226  retrieved by  in  situ leaching  is  a  distinct  advantage.
Conventionally mining  the  quantity  of ore assumed  for the  hypothetical   in
situ mine would contribute  64 Ci  of Ra-226 per year to the surface.  Because
of the insolubility  of RaSQ.»  acid lixiviants containing  HgSCL mobilize even
less radium  than alkaline lixiviants.   It  is  reported  that  the latter mobi-
lizes up .to 4,5 times the  radium as acid leach solutions (Wy77).
     If practical,  the calcite waste  is transferred to  the mill  to recover
the coprecipitated uranium.  Otherwise,  the waste is transferred to an evap-
oration pond and retained beneath  a liquid seal to minimize atmospheric dis-
persion and radon  emanation.

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                                                                       3-171
 Source 4
      If necessary,  the  sulfate concentration  in the  eluant circuit of  the
 uranium recovery unit may  be  controlled by the precipitation of BaSO,.  There
 are no data on  the  contaminant levels expected  in  the BaSO, waste,  although
 less  than  730  MT per year are  anticipated (Wy77).  These wastes  are impounded
 beneath a  liquid seal  of an evaporation pond,
 Source 5
      An assortment of precipitation compounds will  be  produced by evaporative
 concentration  of impounded waste  solutions.  The principal  products  expected
 are alkali chlorides, carbonates,  and  sulfates.   The  quantity of solids pro-
 duced by this  mechanism  and their  rate  of accumulation on the pond bottom  has
 not been reported.
 Source6
      Residues  produced from drilling the numerous wells required for in situ
 leaching constitute  another solid  waste.  The  hypothetical   1n  situ  leaching
 facility defined  above  requires  a total of 540  wells drilled to a  depth  of
 153 m: 200 production,  260 injection,  and  80 monitoring wells.  A diameter  of
 10.2  cm will  be assumed  for all wells,  although  5.1 cm, 12.7 cm, and 15.2  cm
 diameter wells  have  been  used (Wy77).   To accommodate a concrete and  steel
 casing,  a  drill  hole of approximately 20  cm will  be  required.    The  residue
 from  drilling  the monitoring wells  will  consist  mostly of barren  rock; how-
 ever,  an equivalent  of  an  8-m section  of  each  injection and  recovery well
 will  contain 0.06  percent  grade ore.  Hence, drill hole  residues  will  consist
 of  4,960 MT of barren  waste rock and 230  MT of  ore containing 138 kg  of  UgOg.
 These  wastes are in  relatively  small quantities and  should be-manageable. The
 waste  rock and ore,  if mixed and stored  in  a 2-m-high  rectangular pile,  would
 only  cover an area  of about 0.15  hectares and average 0.0027 percent  U,,00,
                                                                         o  o
 Source 7
          During  the  active mining period,  all  solid  wastes are generally
 retained beneath a liquid  seal in  lined  evaporation ponds to minimize  atmo-
 spheric  dispersion and  radon  emanation.   A  plan for  the  final disposal  of
 solid  wastes has-not been  determined.  Suggested procedures  are  to transport
 the wastes to a conventional  uranium mill for further treatment to  recover
any  UjOg  present,  treat  the   effluent  as  mill  wastes, construct long-term
tailings ponds on  the site, or ship the  wastes to a licensed  off-site burial
ground.  Solid   wastes  probably comprise the  least  significant type waste
relative to health and the environment.  Solid wastes generated from recla-
mation  procedures will be discussed in Section 3.5.5,

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                                                                       3-172
 3.5.2   Associated Wastewater
     Water  flushed  through the leached  area when  restoring  the well  field  is
 the  largest source  of wastewater  (see Section 3.5,5),  The  principal  sources
 of  wastewater generated by the hypothetical facility during  the  leaching and
 recovery operations are as follows:

          (1)  Lixiviant bleed —  barren lixiviant removed from the
               leach circuit to produce  a net inflow into the well-field
               area and to control contaminant concentrations
          (2)  Resin wash -- water to wash resin of excess NH.C1  used  to
               regenerate the resin.  Lixiviant bleed is sometimes used for
               this operation, and it reduces the total quantity  of waste-
               water produced (Ka78b)
          (3)  Eluant bleed -- barren eluant removed to control salt accum-
               ulation, principally NaCl and NagCOg, and maintain proper
               volume
          (4)  Well cleaning — water used to flush injection wells to pre-
               vent clogging

     The sources of wastewater and the quantities produced vary at different
sites,  depending upon the lixiviant and recovery circuit chemistry as well  as
the  production rates.   However,   estimates  were  made  of the quantities  of
was'tewater  generated  by the  four principal  sources for  the hypothetical  in
situ facility, and  they are listed in Table 3.57,   It  is assumed that waste
from backwashing the sand filters is lixiviant bleed waste water and does not
contribute  to the total  wastewater generated.   The total volume of wastewater
                                         4   3
estimated to be  generated is 8.43  x 10  m /yr.   Assuming  the  evaporation
ponds are  3,05 m deep  with a 0.604  m  freeboard (Wy77) and  a natural evap-
oration rate of 142  cm/yr  (TVA78b),  a  pond  capacity  of 34,770  m  /yr which
would encompass  a  surface area  of about 1.4 hectares/yr would  be  required.
Using evaporation  data  assumed for  the Irigaray  Uranium Project,  about  75
percent of  the annual  wastewater inventory would evaporate,  which  would leave
           4   3
2.11  x  10   m /yr  and  require  a  surface  area  of   0.85  hectares/yr.  If
necessary,  the  pond  size  can  be reduced by  using mechanical  evaporators.

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                                                                      3-173
          Table 3.57  Estimated quantities of wastewater produced by an
                      in situ leaching operation

Source
Lixiviant bleed (2.5%)
Resin wasfr3^
Eluant bleed
Well cleaning^
Total
Flow Rate,
( j!/min)
50
26
17
__

Annual Accumulation,
(m3/yr)
2.63 x 104
1.37 x 104
8.9 x 103
3.54 x 104
8.43 x 104
             may be included in the lixiviant bleed.
     ^Assumes 260 injection wells flushed twice each  month with  5680  liters
of water.
     Source:  Data from Wy77 and Ka78b proportioned  to  an  annual ILOn production
of 227 MT and a lixiviant flow of 2000x/min;  aquifer  restoration is excluded
(Section 3.5.5).

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                                                                       3-174
      The  liquid wastes are  generally  brines.   They, contain large  amounts of
 sodium  chloride  consisting  of  1,500  to  5,000 mg/s,  total  dissolved  solids
 (TDS),  trace  metals  ranging  from  0 to  10 mg/fc,  and  small  quantities of radio-
 activity.   The quantities of contaminants  generated each year  were estimated
 for  the hypothetical solution mine  by using the annual  mass emissions  esti-
 mated for the Highland Uranium  Project and adjusting  the flow  rates  to pre-
 dict  the concentrations  (NRC78b).   Table  3.58 lists these estimated  concen-
 trations  and  annual  emissions.   Because the contaminants from  the  lixiviant
 bleed were not  included  in  the  source document,  the  trace metals that  are
 mobilized  by  the  leachate  do   not  appear  in  the  tabulation,  and Ra-226
 presence  is  grossly underestimated  (Table  1.7, Section  1.3.4).  Considering
 possible  trace metal concentrations and their toxicities, their presence  in
 the lixiviant  bleed  wastewater may be  significant.  Assuming that 2.5  percent
 of  the  Ra-226  in  the ore  is extracted, the  pregnant  leachate will  contain
 about 1,520  pCi/fc , yielding  1.6  Ci/yr.  However,  it is  assumed that  most  of
 this  radium will be  removed  by the calcium control unit.
      There  are no planned releases  of liquid wastes to the environment  at  in
 situ  solution mines.  The  contaminants dissolved  in ,the liquid wastes will
 accumulate  on the pond bottoms as the liquid evaporates.  Barring  dike  fail-
 ure and  seepage through  the  lined pond bottoms,  no impact should  be  imposed
 upon  the environment by this  source  during operation.
      Another  method, other  than  evaporation, to remove wastewater  from  an  in
 situ -site  is  deep well injection.   This is  the dominant  method  of  wastewater
 removal  at  operations  in  South Texas  (Durler,  D.L.,  U.S. Steel Corporation,
 Texas Uranium Operations, Corpus  Cristi,  TX,  9/79,  written communication).

 3.5.3  Airborn e Emissions
     Airborne emissions from  an in situ solution mining operation will origi-
 nate  from three principal  sources:   the uranium recovery  and processing  unit,
 the waste storage evaporation ponds, and the radon released from the pregnant
 leach surge tanks.   The  primary  radioactive species emitted  is Rn-222.   The
nonradioactive^ species emitted   are  a  function  of  the lixiviant  and the
uranium recovery process.es employed.   Fugitive dust emissions, primarily from
vehicular traffic, will also  occur on  the site.  However, because very little
heavy equipment is used,  the potential for adverse environmental impact from
this source will not be significant and is not considered in this assessment.

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                                                                       3-175
           Table 3.58  Estimated average concentrations  and  annual
                       accumulation  of some  contaminants in  wastewater
Contaminant
Calcium
Chlorine
Carbonate
Bicarbonate
Magnesium
Sodium
Uranium- 238
Radium-226
Thorium-230
Concentration, tng/£
64
2,070
31
36
24
1,320
1
21(a)
6(a)
Annual Accumulation, kg
5,380
173,880
2,600
3,020
2,020
110,880
84
1.
0.







8(b)
5(b)
             s  are  pC1/i
      ^  ^Units  are  mCi.
      Note.—Mass   emissions   estimated  for  the  Highland  Uranium  Project
 (NRC78b),  adjusted for  flow rates and  U.,0n production  of  the hypothetical
 solution mine.
      Estimated  average  annual  airborne emissions were computed for the hypo-
thetical  facility using  data  supplied by  the  Irigaray  and Highland Uranium
Projects  and  from the report of  Kasper,  et al.  (1978) (Wy77, NRC78b). Table
3.59  gives the  results,  proportioned to  a production  rate  of 227  MT/  yr.
      The  major  sources  of  emissions  from  the uranium  recovery  plant  are
by-products  of combustion  from  the dryers,  volatilized  solution residuals,
and U^Og  fines generated during product drying.  Carbon dioxide is the major
combustion  product emitted, although sulfur dioxide may  also be significant
if oil is usedj.o  fuel the  dryers.  Ammonium salts, used in the precipitation
of  uranium  and  resin  regeneration,  will  volatilize as  both ammonia  and
ammonium  chloride  during  yellow  cake drying.   Airborne  particulates  that
include uranium  and  some  decay products are generated during the drying and
packaging processes.  The emission rates  of U_0a  and  daughter products were
computed on the  basis of an average release  rate  of 363 kg of U,,0ft per year

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                                                                       3-176
           Table  3,59   Estimated  average  annual  airborne  emissions  from the
                       hypothetical  in  situ  leaching  facility
 Source
Annual Release Rate
 Recovery  PI ant^a
     Uranium-238
     Uranium-234
     Uranium-235-
     Thorium-230
     Radium-226
     Lead-210
     Polonium-210
     Ammonia
     Ammonium chloride
     Carbon dioxide
     1.0 x 10"1 C1
     1.0 x 10"1 C1
     4.8 x 10"3 Ci
     1.7 x 10~3 CI
     1.0 x 10"4 Ci
     1.0 x 1C"4 Ci
     1.0 x 10"4 Ci
     3.2 x 10° MT
     1.2 x 101 MT
     6.8 x 102 MT
Surge Tank
Radon-222^
Storage Ponds^c'
. Ammonia
, Ammonium chloride
Carbon dioxide
6.5 x ID2 Ci
i.o x io2 MF
3.0 x IO2 MT
7.5 x IO1 KT
     ^'Includes the calcium control unit.
     ^ 'Assumes all radon formed dissolves in the lixiviant and 100 percent
is released on contact with the atmosphere.
     ^Based on a release rate of 14.6 MT/yr of NH3» 10.6 MT/yr of C02 and
42.0 MT/yr of NH.C1 per hectare of pond surface (Wy77), and an average pond
surface area of 7.1 hectares (1.42 ha/yr x 5 yrs).

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                                                                       3-177
 from a 227 MT/yr facility  (Wy77,  Ka78b).   High  efficiency filters and scrub-
 bers are  used,  which  significantly  reduce  the  releases from  the  uranium
 recovery  plant.
      Emission rates from the wastewater  storage  ponds are determined by  the
 composition of the  waste  solutions,  evaporation  rate,  feed rate to the ponds,
 and  the water temperature.  The principal  emissions  from storage ponds ser-
 vicing an alkaline leach process, as  defined  for the hypothetical  facility,
 are  ammonia,  ammonium  chloride,  and  carbon  dioxide.   Different atmospheric
 releases  would result from waste  ponds servicing  an acid  leach facility.  The
 release of Rn-222"from  the  pond surfaces  has not been  measured.  The emission
 rate of  Rn-222  resulting  from the decay of  Ra-226  contained  in  the pond
 sediments will be  inhibited  by the liquid seal  maintained  over the entire
 surface area  of  the  pond.   Because of its low  solubility in the unagitated
 pond skater, it is  reasonable to conclude that  the rate of release  for radon
 from the  water surface will be small compared to that  from the pregnant leach
 surge tanks.   The  liquid seal  maintained over  the pond  area minimizes air-
 borne particulate emissions from the storage ponds.
      The  principal  source of airborne  radioactive  emissions is the release of
 Rn-222  from the pregnant  leach surge tanks.  Rn-222 is mobilized from  the ore
 zone during  solution  mining and  will be  largely soluble in  the  lixiviant
 under the  very high  pressure (-15  atm)  that  exists  at  the ore zone depth
 (-500 ft).   Upon  reaching the atmosphere  at the  surge tank,  nearly complete
 release of  the  absorbed  radon  will  take place.   Since nearly  all  Ra-226
 remains underground  in  the  leach  zone—only  2.5 percent is assumed to  be
 extracted—Rn-222 will  continue  to be generated in areas  leached of uranium.
      Consider  a 2-year  leach  period in each of  5 sectors that is 80 percent
 efficient and yields an  average  of 227  MT of UgOg per year.   If  U-238 and
 Ra-226  are initially in  secular  equilibrium and  97.5 percent  of the Ra-226
 remains underground,  156  Ci  of  Ra-226  will  be  continually available  for
 Rn-222  production.   This quantity  of  Ra-226 will yield  a lixiviant concen-
 tration in the  252,800  m3 aquifer (Section  3.5.5)  of 6.18 x 105  pd*/£  ,
 assuming  a maximum emanating power  of 100  percent.   The  latter assumption
 will  result  in  a  maximum  Rn-222  concentration  in  the   Hxiviant.   A  high
 emanating  power  is  probable  considering the conditions  that exist  in  the
 aquifer:   high pressure,  high permeability due to leaching,  the  presence  of
water in  the  rock pores,  radium present on grain surfaces, and the flow rate
of water  through  the ore zone  (Ta78,  Tanner, A.B., Department  of Interior,

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                                                                       3-178
Geological  Survey, Reston,  Va,  11/79,  personal  communication).   Therefore,
applying  these  maximizing  conditions with a pumping rate of  2,000  jt/min,  650
Ci/yr  of  Rn-222  will  be  released at  the pregnant  leachate  surge  tanks.
     Apparently  very  few measurements  of Rn-222  concentrations in  pregnant
leachates  have  been made at  operating  facilities.   One investigator  reports
that  measured  concentrations  range from 10,000  pCi/£  to  over  500,000  pCi/jt
and  may  vary  with  time  at  the  same  well  by factors  greater  than  ten
(Waligora,  S.,  Eberline Instrument  Corp.,  Albuquerque,  N.M., 1979,  personal
communication).  The concentration  computed  above for the model  facility lies
above the observed range.

3.5.4  Excursion of lixiviant
     A production  zone  excursion refers to the event when the leach  solution
flows from the leach field contaminating the surrounding aquifer.  Production
zone  excursions  are usually  prevented  by bleeding a small  fraction  (2 to 7
percent)  of  the  lixiviant  before reinjection.   This imposes  an  imbalance  in
the injection-recovery  volumes and  causes groundwater to flow into the  leach
field from the surrounding stratum.
     Production  zone  excursions are detected  by  wells placed 60 m  to 300 m
from  the well  field.  These  wells are  routinely monitored, generally bi-
weekly,  to  detect  concentration  increases of one or more constituents of the
lixiviant.  Lixiviant  constituents  monitored   may be chloride,  ammonia, bi-
carbonate,  sulfate,  calcium,  or  uranium.   In  addition, conductivity and  pH
measurements are usually included.  When one  or more  of  the indicators ex-
ceeds a  maximum  limit specified  in the operator's pemn't,  the observation  is
verified by resampling.   If positive, sampling  frequency is increased, appro-
priate  government  agencies  are  notified and  corrective actions are begun.
     An  excursion  from  the  production  zone may  be terminated by one of the
following suggested methods (Wy77):

          (1)  Overpumping  - increasing the flow rate of the recovery
               wells to increase the inward  flow of native  groundwater
          (2)  Reordering - applying different  pumping  rates of the recovery
               wells to different areas of the  well  field,  providing a
               greater inflow of native groundwater at specific points

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                                                                       3-179
                (a variation of overpumping)
           (3)   Reducing Injection - another  method of increasing the ratio
                of recovery flow to injection flow providing the same effect
                as overpumping
           (4)   Ceasing  to Pump - stopping both recovery and injection flows
                (migration is then due entirely to natural  groundwater flow,
                which  is many orders of magnitude less than with wells pumping)
           (5)   Begin  Restoration - initiated when all  other efforts  have
                failed to stop the migration  of lixiviant from the  leach
                field  (Section 3,5.5)
      Excursions  are likely  to  occur  during  the operation  of an in situ  leach
 mine.   Adverse  consequences  of an excursion  will  be  determined  by  its extent,
 the rate of  outward  flow,  contamination levels, aquifer  hydrology,  and  the
 effectiveness of  corrective  measures  applied.

 3.5.5   Restoration  and  Reclamation
     Restoration  is the process  by which the in situ  leach  site  is  returned
 to  an  environmentally  acceptable  state  after mining  is  complete.    Surface
 restoration  consists  of  removing all  structures,  pipelines,  and so on  and
 sealing  the  evaporation  ponds.   Subsurface  restoration, the primary area  of
 concern,  is  done by  discontinuing  lixiviant injection  and  continuing  pumping
 to  sweep  fresh  groundwater  from  the  surrounding  area  through the  leached  ore
 zone.  , It is anticipated  that this process will  flush  out  the remaining lixi-
 viant  and  chemical  compounds or  elements  that have adsorbed or reacted with
 the mineral  content of the  aquifer.   The water recovered  can  be  purified  by
 chemical  precipitation,  ion  exchange,  reverse  osmosis,  or other processes,
 and then recycled.  This  reduces  considerably  the quantity  of water that must
 be  managed.   Between  75 and  80  percent of the water can be reinjected while
 the remainder containing  the contaminants  is  transferred  to an  evaporation
 pond (Wy77, NRC78b).  During  the  initial  restoration  process, it is generally
 cost effective to recover  the uranium from the  process  wastewater.
     Aquifer  restoration  continues  until   the  groundwater  quality  in   the
mining zone  meets a criterion established on  a basis of the premining water
 quality. In many cases, the  premining groundwater quality criterion is diffi-
cult to  establish  because water quality can  vary  considerably over the ore
zone region and  may contain high  natural levels  of contaminants.  Samples  of
water  front wells  monitored prior  to mining  in Texas contained  concentrations

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                                                                       3-180
 of Rn-222  approaching  20,000  pCi/£  (Tanner, A.B.,  Department of  Interior,
 Geological  Survey,  Reston,  Va,  11/79,  personal  communication),  and it  is
 probably unrealistic to  attempt to  restore  an aquifer  to  a  better  quality
 than  existed  naturally  before  mining.  Wells and  flow rates  used  in  this
 process must  be  carefully  selected  and  controlled  to  provide  efficient
 groundwater sweeps and  to insure that all affected  areas  of the leach  zone
 are restored.
      The affected  aquifer volume that  is  to  be  restored may be estimated  by
 the following  equation:
      affected  volume =  area of well field x aquifer thickness        (3.12}
                        x  (porosity)
                                    •
                          100 percent
 Assuming a  porosity for sandstone of  30 percent (NRC78b), the affected volume
 of the  hypothetical in situ  solution mine defined in  Section  3.5 would be:
      affected  volume =  52.6 hectares  x  8 m x
                        30 percent/100 percent ~ 1.26 x  10  m .
 Because of  mixing  leach  solution with  the incoming sweep water and  the grad-
 ual  desorption of  some  contaminants  from clays present in the ore body, more
 water is required  to adequately flush  the contaminants than one pore  volume.
 It has  been  estimated  that  five to  seven  pore  volumes  of water  would be
 required  for  adequate   restoration   (Wy77,  NRC78b).    Using  the  seven  pore
 volume  value  and  assuming  that  80 percent of the sweep  water  is reinjected
 after purification,  a  total of  1.76  x  10  m  of  wastewater  having  high IDS
 would be transferred  to the evaporation  ponds during  the restoration phase.
 If the  aquifer is  swept at a flow rate of 2,000 £/min, restoration would take
 8  years (1.6  yr per sector), and wastewater  will  accumulate at about 2.22 x
   C O
 10 m  /yr during  this  period.   With careful control,  restoration  can be con-
 current  with leaching in  different areas of the well  field.
      Table  3.60 lists estimated average concentrations of contaminants in the
 restoration  wastewater  (NRC78b)  and  annual  accumulation  rates of  the  con-
 taminants based  on a  flow rate of 2,000 £/min.  In the last column are esti-
mates  of" the  total  mass  of  substances  produced  by  restoration  that would
 become  sediments in .the evaporation  ponds.  Data were  not  provided  for cal-
 cium, magnesium, chloride,  and  ammonium ions, even though the latter two are
major constituents expected  from  an alkaline  leach  process (Wy77).   These
concentrations reflect  average  values,  but concentrations  in  the wastewater
during the initial  phase of the restoration process will be  much higher.  For

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                                                                       3-181
Table 3.60  Estimated average concentrations  and  annual  and  total  accumula-
            tions of some contaminants in restoration wastewater
Contaminant
     (a)
     (b)
     (c),
            Concentration
                mg/t
                                        Annual
                         Total
Accumulation, Kg  '  Accumulation, MT  '
Arsenic
Calcium
Chloride
Carbonate
Bicarbonate
Magnesium
Sodium
Ammonium
Selenium
Sulfate
Uranium-238
Thorium-230
Radium- 2 26
Radon-222
0.2
NA(c^
• NA
450
550
NA
550
NA
0.10
150
< 1^
100(e)
75(e>
618, 000^
210
NA
NA
473,000
578,000
NA
578,000
NA
100
157,000
<900
Q.10^
0.08^
650^
1.7
NA
NA
3,780
4,620
NA
4,620
NA
0.8
1,250
<7.2
0.8
0.6
5,200^
   Produced only during the estimated 8-yr restoration period.
   Total  accumulation during the estimated 8-yr restoration period.
        NA - Data not available.
     ^ ^Concentration after uranium extraction.
^  '
            s are pCi/i-
       'Units are Ci/yr or total  curies.
     Source:  Concentrations based on those estimated for the Highland  Urani-
um Project {NRC78b},  adjusted for a flow  rate of 2,000 £/min.

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                                                                 3-182
Table 3.61  A comparison of contaminant concentrations in pre-mining
            groundwater and pre-restoration mine water (Wy77)
Contaminant
Arsenic
Barium
Boron
Cadmium
Chromium
Copper
Manganese
Mercury
Nickel
Selenium
Silver
Zinc
Lead
Chloride
Ammonia
Bicarbonate
Uranium (U3Qg)
Radium-226
Total dissolved solids
Pre-mining
Water, mg/j,
<0.0025
0.12
0.16
< 0.005
0.0135
0.019
0.12
0.0028
0.018
0.013
<0.005
0.003
0.0035
10.75
<1.0
139
0.098
27(a)
793
Pre-restoration
Water, mgA
0.021
0.069
0.283
0.014
0.002
0.220
0.97
<0.0002
0.218
1.75
0.015
0.22
0.110
524
235
805
24.4
371U)
1324
         are pC1/£.

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                                                                       3-183
 example,  Table 3.61 compares concentrations  of  substances  in  the  groundwater
 before mining  with  those  after mining  but  before restoration.  These  data  are
 from  tests conducted for the Irigaray Project (Wy77) and indicate those sub-
 stances whose  groundwater concentrations may  be  elevated by  in situ leaching.
      Radon emission during  the  restoration  process  has not been  considered
 (Wy77,  NRC78b, Ka78b).   Because  essentially all  Ra-226 remains  in  the  ore
 zone  (about  97.5 percent),  it appears  reasonable to expect Rn-222 emissions
 to  continue  during restoration.   A  leached-out  sector of the model mine will
 contain 156  Ci of  Ra-226 in  an  aquifer volume  of 2.53  x  10  m   (1.26 x  106
 m   *  5).   Although no measurements  have  been made,  it would appear  that  the
 restoration  wastewater will  contain about the  same Rn-222 concentration as
 the  pregnant  leachate  during  leaching,   6.18 x 10  pCi/fc  (Section  3.5.3).
 Assuming  a pumping  rate of 2,000  £/min, a  maximum of 650 Ci of Rn-222 will be
 released  during each year  of restoration, resulting in a  maximum tot-il   re-
 lease of  5,200 Ci during  the  estimated 8-yr restoration.
      Restoration   Is  presently  in  the   experimental  stages.    No  com-
 mercial-sized  facility has reached that phase of operation.  Although restor-
 ation  by  flushing  appears  feasible,  there have been  problems when  alkaline
 Hxiviants were  used,  particularly those  containing ammonium ions.   Ammonium
 is the preferred cation because sodium causes the clays to swell and  plug  the
 formation, and calcium forms an insoluble  sulfate  that also  decreases   the
 permeability of  the formation.   However,  ammonium ions  adsorb  tightly  on  to
 clays  by   replacing the  calcium  and  magnesium   atoms  in  the  clays.  Mont-
 morillonite, prevalent in the Texas mining areas, has extensive surface areas
 that  result  in  very  large  ion-exchange  capacities.   Once  adsorbed,   the
 ammonium  ions  desorb at  a very slow rate and prolong the restoration. It  has
 been  reported  that  after  sweeping a  leached ore  zone with 10 ore zone volumes
 of water,  the  ammonium concentration of the water was reduced to 15 to 25 mg4
 (Ka78b).   This concentration of  ammonium  may not be  significant, although,
 under aerobic  conditions, ammonium  ions  can be oxidized  to  the  more  toxic
 nitrate.   In a deep aquifer, this oxidation  process  is  not likely to occur,
 and,  because  of the very low Teachability of ammonium  ions from  clays,  any
 ammonium  retained  after  restoration  will  move  to surrounding aquifers  at a
 very slow  rate.
     Several  ongoing research studies  are  trying to solve  the ammonium prob-
lem (Ka78b).    Potassium is  being  tested as a cation  replacement for ammonium

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                                                                       3-184
in  hopes  that its adsorption  and  swelling characteristics will be  favorable.
Sweep  solutions  enriched in calcium and magnesium are  being  tested  to  deter-
mine if they will facilitate the flushing of the ammonium ion by replacing  it
on  the clays by  ion-exchange.
     Restoration of  the aquifer after mining stops is  in the research  stage.
The adequacy  of the  restoration  process and  the procedures  required will
depend on  a number of  factors: the lixiviant used, concentration of specific
ions in  the lixiviant, the physical character of the stratigraphic unit, and
the geochemical  nature  of  the ore deposit.  Undoubtedly,  research will im-
prove  the  process in the next few years.  If the criteria of the restoration
process are met, it is unlikely that there will be any adverse environmental
impact from a  properly  restored aquifer.
     Generally,  the goal of reclaiming the site surface is to return the area
to  a state  similar to that which existed naturally before mining.  This often
means one suitable for  livestock grazing and wildlife habitat.  The following
site reclamation actions have  been proposed (Wy77):
     (1)  Remove all structures and exposed pipes and plug all wells with
concrete.
     (2)  After  all impounded  liquids have completely evaporated, cover
the remains with overburden to a depth [2 m has  been suggested at the
Irigaray site  (Wy77)j that will support plant growth and suppress
Rn-222 emissions or transport and deposit the remains in a mill  tailings
impoundment.
     (3)  Before backfilling, dispose of the solids containing sufficient
radioactivity  to warrant removal by one of the methods suggested in
Section 3.5.1.
     (4)  Grade  surfaces of the backfilled ponds and all other barren areas
to  create a suitable topography and then revegetate them.
     (5)  Irrigate and  fertilize sites to develop adequate plant cover.
     (6)  Maintain fences to prevent grazing  by  livestock until  stable vege-
tative cover becomes established.
     (7)  Monitor reclaimed sites for radiation, verification of vegetative
cover,  and the absence of adverse erosion.
     (8)  Sample monitoring wells one year after restoration to  verify aquifer
restoration.

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                                                                       3-185
 3.6  OtherSources

 3.6.1  Minera1  Exploration
      During early exploration,  uranium  was identified by  its  mineral  color,
 i.e., pitchblende from the Central  City  District in Colorado and carnotite in
 the Uravan Mineral Belt  in Utah and Colorado.   It  was  usually mined in con-
 junction  with  other  metals  and minerals.  Later,  when  portable  radiation
 survey meters became available,  a substantial  portion of the uranium findings
 (generally outcrops) were  made  by  non-geologic prospectors (UGS54).   Current
 uranium exploration "uses extensive geological  studies  to  locate  formations
 with a strong  potential  for  uranium ore content.  These  formations  are then
 explored  and  field  surveyed  to verify the  presence of  ore.   Much of  the
 current exploratory  activity is  directed  at  expanding  known deposits  and
 mining areas.
      As the surface and  near-surface  uranium  deposits are found, mined,  arid
 depleted,  exploration for  reserves  must  be conducted at greater depths.  The
 deeper uranium deposits,  however,  offer  few radiometric  clues  on the surface
 regarding  their  location.   In  these  cases, geologic studies and field work
 postulate  the  existence  of promising  geological  formations.  Actual  explor-
 ation must be done by  drilling.  Drilling  is also  used  to  extend and  explore
 known uranium  producing  areas.
      There  are two  categories  of  drilling:   exploratory  and developmental.
 Exploratory drilling  is used to  sample  a promising  formation to determine  if
 uranium ore is present.   The drilling is  generally  done'on  a  grid with  the
 drill  holes spaced  60 m to 1.6 km  or more apart.   Development drilling,  to
 define the  size  and  uranium content of the   ore  body, occurs when ore  is
 struck in  an exploratory  hole.  The development  hole  spacing ranges  from 8 m
 to   100  m,  depending  on  the  characteristics  and  depth  of  the  ore  body.
 Usually,  the same  drilling equipment  is used  for  both  the exploratory and
 development  drilling.
      Ordinarily,  there are  three  vehicles   in  a  drilling unit.  One vehicle
 carries and operates  the  drill  rig, the second  carries  the  drill  rods, and
 the  third  carries water.  Although  the  drill  rig is a well-engineered, com-
 pact  design, its  physical  size  is  increasing   to meet the  demands  of deeper
drilling  (Personal  communication with G.  C. Ritter,  1979, Bendix  Field En-
gineering Corp., Grand Junction, CO).

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                                                                       3-186
      Early   drilling   (1948-1956)  was   predominantly   done   with   percussion
drills.  These drills could drill  to depths of about  76  m using 2.8  cm  dia-
meter drill  steel.  The drill  bit was  cooled and cuttings were removed  from
the   drill  hole  by  forcing  air  down  the center  of  the drill  stem.   The
cuttings  (chips,  sands, and  dusts)  were carried  up and out of  the  drill  hole
by the air stream with  velocities  of 914-1520 m per minute (Ni76).   The chips
and  coarse   sands  collected  near the bore  hole while  the fine sands  drifted
and  deposited around the drill  site.  Dusts, however,  were free to  drift  with
the  winds.
      Rotary  drilling,   used   for  boring deep  holes,   generally has replaced
percussion drilling.   Drill  stems of 7.3'  cm  diameter  are used to  bore holes
to depths of about 1300 m.   Stems with diameters of  11.4 cm and   larger  are
used  for drilling holes  in  excess of 1300 m.  The  rotary drill  bits   are
cooled generally  in  the same manner as percussion  drills.  When groundwater
is encountered, water is used as a drilling medium and for removing  cuttings.
The  cuttings are removed  from  the  drill   hole  in  the form  of a  slurry or
drilling mud.  They are usually stored  in basins, either fabricated  or  dug in
the  ground.   If unavailable,  water is hauled to the drill   site by truck.   The
drilling muds and water are  stored  in  portable tanks or an earth impoundment
for  recirculation.  After  the drilling  is completed, very often the cuttings
are  scattered and the  drilling mud  left at the site.  This practice has  been
discouraged  over  the past 10 years in the Uravan area  (Personal  communication
with  S.C. Ritter, 1979, Bendix Field Engineering Corp., Grand Junction,  CO).
In some  cases,  the cuttings  are disposed  of  in  a trench  and covered up with
earth.    Drilling muds  are  also  sometimes  covered.   In  either   case,
containment  of  the drilling  wastes   does  not  appear  to   be  a  prevalent
practice.
     Development  drilling  is conducted  if ore is  struck in an  exploratory
hole.   The   offset distance  (i.e,  the distance between development  drill
holes) is dependent  on  the  previous history  of  the  ore body sizes  in  the
area.  Offsetting may  occur as soon as  ore is struck, or it may  be delayed
until the exploratory drilling is completed.

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                                                                       3-187
      The  ore body may  be  evaluated  by bore hole  logging  or by examining and
 analyzing  cores.  Core  drilling,  if used,  usually  begins at the top  of the
 ore  horizon.  Ore {cores  and  cuttings)  removed from  the  bore  hole  are some-
 times  removed from  the drill  site.   In cases  where  the ore is  not  removed
 from  the drill  site, it  remains  with  the  dry cuttings  or in  the drilling
 muds. The drill  hole  collar  is sometimes  plugged with  0.9  -  1.5  m of concrete
 after the  bore hole  has been  evaluated.   In some  states,  the drill hole must
 be   plugged  to   seal   off   aquifers   in   order  to  minimize   groundwater
 contamination.
3.6.1.1   Environmental  Considerations
     By  1977, the uranium industry  had completed  101  x  10  meters  of  surface
drilling,  with an  all-time  yearly  high  of 12  x 10  meters  (DOE79).   From
1958-1977,  about  821,900 surface holes were drilled,  resulting  in  87,8 x  10
meters  of bore holes.   No statistics  are available  on the  number of holes
drilled  from  1948-1958,  but the annual and cumulative  meters drilled for  that
period is known (DQE79).   In order to estimate the number of drill  rig place-
ments for that period,  the total annual meters of drilling was divided by  the
annual  average  bore  hole  depth.   The average depth  per bore  hole was esti-
mated  by plotting  the  average  annual  bore  hole depths for  1958-1977   then
using  that  data  to  estimate the  annual  bore hole  depths for  1948-1957 by
linear regression analysis {Fig. 3.22).
     The data points  in Fig.  3.22 appear to fall into two groups:  1958-1966
and  1966-1977.   The  average  drilling depth of  the  1956-1977  group  of data
points  probably  reflects  the  deep drilling  in  the Srantst  New Mexico area
that  became  significant  in  1969.   Using this  information,   the  1948-1958
average  drilling  depths  were estimated  from  regression analysis  using   the
1958-1966 data points only.  Table 3,62 is a summary of the DOE drilling data
and the number of estimated bore holes by type and year.

-------
  175 f
  150 	
  125 -
E-i
CM
pa
p

a
3
M
a

w
I
  100
   25
     1948
1952
1956
1960
1964         1968

       YEAR
                                                                                    1972
                                                                                1976  '
                                                                                 1980
 1

M
00
              Figure 3,22 Average depth of exploratory drilling in the U.S uranium industry from 1948 to present.

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                                                                      3-189
Table 3.62 Estimates of exploratory and development drill holes (1948-1979)
Surface Drilling (10 Meters)
Year
1948
1949
1950
1951
1952
1953
1954
1955
1956
1957
1958
1959
1960
1961
1962
1963
1964
1965
1966
1967
1968
1969
1970
1971
1972
1973
1974
1975
1976
1977
1978
1979
TOTAL
Exploration
0.052
0.110
0.174
0.329
0.415
1.11
1.24
1.61
2.22
2.24
1.15
0.722
0.427
0.402
0.451
0.268
0.294
0.354
0.549
1.67
4.97
6.25
5.49
3.47
. 3.60
3.29
4.88
5.03
5.94
7.89
10.8
9.94
286
Development
0.012
0.016
0.063
0.106
0.091
0.112
0.169
0.232
0.457
0.564
1.06
1.00
1.28
0.972
0.741
0.604
0.381
0.289
0.731
1.62
2.30
2.86
1.69
1.23
1.10
1.70
1.83
2.74
4.48
4.45
5.24
5.18
149
Average Hole
Depth(Meters)
3J.1&
39.6^
4l!l£a?
4l.i;a<
42.?Sa<
42.7U;
44.2^1
45.7iaJ
45.7
45.7
48.2
53.9
50.0
61.9
39.6
42.4
47.5
67.7
110
125
120
122
121
128
146
168
139
154
155(a)
158(a)

Number of Holes
Exploration
2',88o£?J
4»380h
8,OOOi°C
1Q,100JP(
26,100,Px
29,000
36,300^
48,600)^
49,000
25,300
16,300
7,340
8,260
6,440
8,470
5,970
6,230
5,750
12,800
38,500
47,900
44,000
28,400
26,900
22,600
27,400
34,300
40,400
6Z,600(b)
69,200;°<
62,700*- ;
823,000
Development
320^)
424^
1'600(b)

2'220ffi
2,620
(b)
5'260(b)

12,300
22,900
19,600
24,400
19,300
12,900
13,500
9,910
7,330
13,200
16,900
19,500
28,000
14,900
10,400
9,710
11,700
12,300
21,600
27,200
30,90Q,bv
32]700(b)
454,000
        Indicates estimated average depth from Fig.  3.22.

        Indicates number of drill holes estimated by dividing the annual
exploration and surface drijling depths by the average hole depth.

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                                                                       3-190
     Cuttings  produced  by  drilling  can degrade the  drill  site area  and  the
 local  air  quality.   For convenience of evaluation,  the cuttings are  divided
 into  two general  categories—dusts and wastes.  The  dusts are drilling  fines
 that  become airborne,  and  wastes are  drilling  chips  and  sands  deposited
 around  the borehole.   The maximum dust production occurs when compressed  air
 is  used solely for cleaning the  boreholes.   Generally the drilling industry
 uses  foaming  agents  injected  into the compressed air stream to help remove
 drill  cuttings.   The  foam traps and contains  the  fine partieulates and sub-
 stantially  reduces the  airborne dust.   In  practice,  the  drillers minimize
 airborne dust,'because  it causes excessive wear on  engines  and compressors.
 Dust  production  also  indicates improper drilling  energy  being  used to grind
 up  cuttings  in the  borehole rather than bore.  Occasionally some  water may
 also be  injected into the air stream to remove cuttings and to keep the drill
 H)le from collapsing when loose materials are encountered.
     There are some estimates of airborne dust production and general  assump-
 tions concerning drilling practices (Private communication with Mr.  T. Price,
 Bendix  Corp.,  Grand Junction,  CO and E, Borgerding,  Borgerding  Drilling Co,
 Inc., Montrose, CO),  They are as follows:
     (1)  The  ratio by  weight of  the  chips, sands,  and dusts  produced  by
 drilling is approximately 60:37:3,  respectively  (i.e., 3  Kg  of  every 100 Kg
 of cuttings removed from a borehole is available  as airborne dust).
     (2)  Fifty percent of  all  drill  holes are wet (mud)  drilled and 50 per-
 cent  are air drilled;  ninety-five  percent of  the latter are  drilled using
mist or foara (i.e., 2.5 percent are dry-drilled).
     (3)  The first 6,6 m of all drill holes  are  drilled dry (i.e.,  no mist
or foam is used).
     We  estimated  dust  production from  contemporary drilling  by  averaging
drilling data  from  Table  3.62  for the years  1975  through 1979,   The  average
depth of the holes  for this period is  148 m.   The annual average numbers  of
exploration and development  holes  are  53,800 and 29,200,  respectively.  Air-
borne dust production from those holes  that are drilled with  mud (wet), foam,
or mists  (97,5 percent of  both the exploratory  and  development  holes)  will
originate only from the  first  6.6 m depth.   The  weight of dust generated per
hole will be as follows:

                                                3                   3
     Airborne  dust (kg) = Volume of borehole  (m ) x  density   (kg/m )  x air-
     borne  dust fraction (.03)  per drill tiole

-------
                                                                       3-191
     =  ( 7tr2h) (2000kg)(0.03)        where  h  -  6.6  m
                     m                       r - 0.0865 rn  (assumed average  rad-
                                                ius  of 2  bit sizes  r = 7.3 cm
                                                and  10 era)  (Pe79)
     = <3.14)(7.48 x 10*3) m2 x 6.6 m x 2000 kg x 0.03
                                               3
                                             m
     = 9.3  kg
     The  average  weight of airborne dust  (kg) produced  from all contemporary
 annual drilling (first  6.6 m) is
          83,000  drill  holes x    9.3 kg    =  7.7 x 105  kg.
                               drill hole
     The  annual  total  weight (kg) of airborne dust produced from  2.5 percent
 of the annual number of drill holes bored  (dry) where no mud, mists, or foams
 are used
     = 83,000 drill  holes x    148 m    x  0.025 x 47 kg  cuttings x
                            drill hole               m
     0,03 kg dust/kg cuttings = 4.3 x 10   kg/yr.                        (3.13)
 The total weight of airborne dust  produced   annually from  each  dry-drilled
 borehole  is 209 kg.
     Assuming that  each development hole  penetrates the 3.6  m ore body,  the
 total  amount of  airborne  ore  and  sub-ore dust   produced from  development
 drilling  annually is
     '29,200   dril1 holes   x  3.6 m (ore ajid sub-ore)   x m47kg^  cuttings  x
                   yr               drill  hole               m
     0.03 kg dust/kg cutting x 0.025 = 3.7 x 103 kg,                   (3.14)
The total weight of  airborne ore and sub-ore dust produced from each develop-
ment drill hole (no  mudj mists, or foams used)  is 5,1 kg.
     The  estimated  annual  quantity of ore and sub-ore brought to the surface
by contemporary drilling equals:

       29.200 drill  holes  x  3.6 m     x        47  kg cuttings          (3.15)
                  yr        drill hole              m
     = 4.9 x 106 kg  or 4.9 x 103 MT

     Most of the ore will remain at the drill  site  with  drilling muds or with
the drilling wastes  around  the  drill holes.   Since the  ore most usually will
be the last material removed from the boreholes, it will be deposited on  the

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                                                                       3-192
 surface of the cuttings  and  drilling muds.  This will  expose  the ore to the
 elements and  subject  it to erosion.

 3.6.1.2  Radon ...Lossesjrom Or i 11HoiQS
      When the development drill  penetrates  an  ore body, some of  the  ore and
 sub-ore bearing  formations will  be  exposed  to  air in  the drill  hole.  Some of
 the radon gas produced  in  the  ore can enter into the air  in the drill  hole
 and escape to the atmosphere.  The  mechanisms  affecting the release  rate of
 radon from boreholes  are poorly understood.  Tanner observed  a wide  variation
 in  radon  concentrations  as  a function of depth  in an open borehole as  com-
 pared to a closed  borehole  (Ta58).   Tanner also noted  that  strong  winds could
 significantly reduce  the total  radon content of  an uncovered borehole. Since
 so  little is  known about  radon discharges  from development boreholes, radon
 losses;  in this report  are assessed  on a "worst  case"  bisis using the  fol-
 lowing  assumptions:
           1.   The drill  hole is  not  plugged.
           2.   About  3.6 m of ore and sub-ore were drilled.
           3.   All radon  released into  the borehole escapes to the
               atmosphere.
           4.   The average grade of the ore and sub-ore  is 0,17 percent.
           5.   No water accumulates 1n  the borehole.
      The  surface area of the borehole passing through  the ore and sub-ore  body
 is  •
      2  wh  = 2 x 3.14 x 0.0865 ra x 3.6 m = 2.0 m2.                    (3.16)
 The radon release rate is estimated for ore and sub-ore  in the borehole using
                                ?
 an exhalation rate of 0,092 Ci/m  per year per percent of ILQg (N179).   The
 quantity  of radon (Q) per development hole escaping per unit time is
 0.092  Ci   x 0.171 x 2.0 ra2 x	x 1012 B& = 990 pCi/sec  (3,17)
m2 yr *                        3.15 xlO7 sec/yr       Cl
The  total  quantity of  radon  per annum escaping   from  all  development holes
drilled through  1979
                    11 holes x
                               sec-drill hole
• 4.5 x 105 drill holes x    990  pCi     x 3.15 x 107 sec/yr
                    1
                 10l2pC1
                     Ci
     - 14,000 Ci/yr                                              (3.18)

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                                                                       3-193
      The  "worst case" estimate  can  be modified by assuming 50 percent of the
 holes are  wet  and  30  percent  of the  remaining holes  are plugged  or  have
 collapsed.   In this case,  the  total  source term  would  be  about 4,900 Ci/yr.
 Since about 31  percent of the  development  drill  holes are at  surface  mines
 and  are consumed  by the pits,  the  annual  Rn-222 release  from  the  remaining
 holes will  be  3,400  Ci/yr.

 3.6,1.3  Ground waiter
      Progressively  deeper holes are being drilled as  the ore  bodies  near the
 surface  become  depleted.   As  the  drilling  depths  increase,  one  or  more
 aquifers may be intercepted by  a  drill  hole, and an  aquifer  with poor water
 quality may be connected with an  aquifer with  good  water quality.  Depending
 on  the direction of flow,  the  quality of water may be downgraded in a  good
 aquifer.   Most states  require  some  plugging of  the drill  holes to seal  the
 aquifer  in  order to maintain water  quality.   Adequate plugging of the drill
 holes  requires a  conscientious  effort  on  the  part of the driller  and  the
 regulatory  agency.   Since the movement of groundwater  is  relatively slow,  the
 change  in  the  quality of water  -in an  aquifer will  not be  apparent for  some
 time.   Thus, it may take  a long  time to correct the  quality of  water  in  a
 downgraded  aquifer.

 3.6.1.4  Fumes
      It  is  estimated  (Pe79)  that 11,2  liters  of diesel fuel  are needed to
 drill  1.0 m.   In 1979, the average  borehole  depth was estimated to be 158 m
 and  would   require  about 1770   liters  of diesel  fuel.   This fuel  would be
 burned  at   a  rate of  approximately  173 liters  per  hour.   Some  individual
 holes, however,  are  drilled in  excess of 914  m and require 10,200 liters of
 diesel fuel.   It is estimated  that  about 170 million  liters  of diesel  fuel
were consumed for all 1979 drilling.
     The principal   emissions  from the  drilling  power  sources are  partic-
 ulates: sulfur  oxides, carbon  monoxide,  nitrogen oxides,  and hydrocarbons.
 Because of  the  transient nature of the  drilling,  these releases are not ex-
 pected to substantially lower air quality over time.

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                                                                       3-194
 3.6,1.5  Model  Drilling
      About 1,3  x 10  holes have been drilled and bored for all uranium mining
 from 1948  through  1979  for  approximately 3000 mines.  This  would  amount to
 about 430 holes per  mine.   Thirty-six percent of the holes were for develop-
 ment drilling,  and 64  percent were for exploratory  drilling.   Assuming that
 50  percent  of   the exploratory and  development holes  are air drilled  (see
 Section 3.S.I.I),  the  airborne dust  production for  an average mine  may be
 estimated as  follows;
 Airborne otust from  all  drill  holes (first  6.6 m of depth air drilled dry)
      =  430 drill  holes  x      9.3 kg        * 4000 kg.                  (3.19)
                           drill hole
 Airborne dust from  all  dry air drilling, less the first 6.6 m»         (3.20)
      =  (430 drill holes x  209 kg dust  x 0.5 x 0.05) - 100 kg = 2100 kg.
                            drill  hole
 Airborne ore  and  sub-ore  dust produced by  dry air drilling
      «  430 drill  holes  x  0.36 x 0.5 x  0.05 x 5.1 kg dust  = 20 kg.     (3.21)
                                               drill hole
 Total airborne  dust produced  from  all  drilling at an  average mine site
      -  4000 kg  -i- 2100 kg  =  6100 Kg - 6.1 MT.                     (3.22)
      Twenty  kilograms  of  the  total  dust  produced will be  ore and  sub-ore
 dusts.  The  Rn-222 emissions from the bore  holes  at  an  average mine site would
 be
  4'30 drill holes (0.5)(0.36)    (990   pCi	)  =  7.7 x  ID4  pCi.   (3.23)
                                 sec-drill  hole                 sec
 or 2.4  Cl/yr.
 Development  drill  holes  at  a  surface  mine  would be  consumed by  the  pit.
      Tables  3.63--3.6B show  airborne particulate source  terms for uranium
 drilling  for  Individual drill  holes and for an average uranium mine.  Table
 3.63  lists  the  airborne dust produced for each  type exploratory and develop-
 ment  borehole;  Table  3.64 summarizes  the  quantity  of airborne dust produced
 by all  types  of drilling at  an average  mine  sitej and  Table 3.65  lists  the
 pollutants emitted  from a drill rig power source,

 3.6.2  PrgcfpJtation Runoff from Uranium Mine's
     Unquestionably,  overland  flow  or  surface  runoff from  precipitation
transports  dissolved  and  suspended contaminants  from  mining  areas  to  the
offsite  environment.   Unfortunately, the significance of  this pathway re!a-

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     Table  3.63   Estimated  source terms per borehole  for  contemporary  surface  drilling  for uranium
,
'
Type of Drilling
i
Exploratory
Air (dry)
Air (mist or foam)
Wet (mud)
Development
Air (dry)
Air (mist or foam)
Wet (mud)
Thickness of Ore
and Sub-ore Bodies
(•)


NA(b)
NA
NA

3.6
3.6
3.6

Ai rborne
Total (kg)


209
9.3
9.3

209
9.3
9.3

Dust Production
Rate(kg/min)^


0.27
0.27
0.27

0.27
0.27
0.27
Airborne
Dust
Total (kg)


NA
NA
NA

5.1
NA
NA
Ore and Sub-Ore
Production
Rate(kg/min)(a)


NA
NA
NA

0.27
NA
HA
(a)
(b)
Based on an air drilling rate of 11.5 m/nr.
NA - not applicable.
                                                                                                           vo
                                                                                                           en

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                                                                       3-196
          Table 3.64   Airborne dusts produced at an average mine site
                       from exploratory and development drilling

  Type of Drilling                         quantity of Airborne Dust (kg)

All types (first 6.6 m depth)                        4,000
Air drilling (dry)                                   2,100
                                      Total          6,100 kg^

     ^'Twenty kg of the total will be ore and sub-ore dusts.
          Table 3.65   Estimates of emissions from drill rig
                       diesel power source
Pollutant
Carbon monoxide
Hydrocarbons
Nitrogen oxides
Al dehydes
Sulfur oxides
Participates
Production Rate
(kg/103 liters fuel)
12.2
4.49
56.2
0.84
3.74
4.01
Quantity^3'
(kg/drill hole)
20.2
7.4
93
1.39
6.2
6.6
Rate(a)
(kg/hr)
1.5
0.55
6.9
0.10
0.46
0.49
              on  a  drilling  rate of llm/hr.
     Source:   EPA77b.

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                                                                       3-197
 tive to uranium mines is highly site specific and poorly understood. Very few
 field studies  of runoff  from  uranium mining areas have  been  conducted, and
 what field  data  do  exist  frequently  relate  to  the combined and  probably
 greater  influences  of  mine  water  discharge  and milling.   Most  of  the NRC
 regulations  apply to mill  operations,  since mining is generally  exempt from
 the  agency's  charter.   The  EPA  regulations  (Environmental  Radiation  Pro-
 tection Standards for Nuclear  Power Operations;  40 CFR Part 190)  applicable
 to the  uranium  fuel  cycle establish  dose limits for  individuals  to  provide
 protection for populations living  in  the  vicinity  of  uranium mills.   Uranium
 mines are excluded, and  30 are liquid effluent guidelines for  ore mining and
 dressing  (40  CFR 440,  Subpart  E).  Regulations being  developed under  the
 Resource Conservation and  Recovery Act  (RCRA)  of 1976 apply  to  radioactive
 wastes  not covered by the  Atomic  Energy Act of  1954,  as  amended.   Solid and
 liquid  waste  categories  will   be  defined  in forthcoming  EPA regulations  de-
 veloped  under RCRA,  but it is  not  anticipated  that runoff from mined  lands
 will  meet  the  waste characteristics  in  the  regulations.   Similarly,  the
 Federal  Water  Pollution  Control  Act  Amendment of  1972,  the Clean Water Act of
 1977,  the Safe  Drinking Water Act, and State  regulations in general  do  not
 address   surface  runoff  effects  of mining.   Without the  regulatory  base,
 studies  and  field data are, not surprisingly, rather  scarce.   In  New  Mexico,
 the State's  208 Water quality  Management  Plan calls for,  among other  things,
 improved  data  collection  on  runoff from  active  and inactive tailings  piles
 and from  drilling,  exploration,  and  development activities such  as  access
 road  and  drill site construction  (So79).
      We  have not  estimated chemical  transport by  overland  flow  because of  the
 limited  time for  the  study.  But,  it is reasonable to expect  that  such trans-
 port  may be  quite significant  in  an arid  and semiarid climate where much of
 the precipitation that does infiltrate is  discharged back  into the atmosphere
 as  water vapor.   This has been  well demonstrated in the case of uranium mill
 tailings  (K178).   Water  moving  back  out  of  the soil  transports dissolved
 salts that are deposited on the  soil  surface  when the carrier (water) evap-
 orates.   Subsequent  precipitation  further  transports  these  salts downward
 into  the soil  and  laterally  to  offsite areas.   So-called  "blooms"  of salt
crystals,  composed mainly  of  sulfate  and  chloride compounds, characterize
uranium  ore  bodies,  mill  tailings  piles,  and  mine  wastes  in a  number of
Western  States,  and  we  must  presume  that such  salts  solubilize  in runoff.

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                                                                       3-198
 This also  indicates  that there  may be large concentrations  of  contaminants
 available for plant uptake.  Molybdenum,  in  particular, is one  of  the toxic
 elements on  such  blooms,  and  uranium is  also  highly suspect.   Selenium,
 arsenic, and  vanadium may  also be  present,  since  their  anions are  mobile
 under oxidizing  conditions  characteristic of  the near-surface,  unsaturated
 zone (Fu78).
      Overburden  has been  used extensively  to  backfill  surface  mines  operating
 since the early  to  mid 1970ls»  but  this is  not true at many  if not most older
 and  now  inactive mines.   Erosion of these  piles  by water and wind may  present
 the  greatest problem  (Ka75).   Using  overburden  to construct acc?:;s  roads  and
 dikes distributes contaminants  in the local environment  and  may ijgravate  air
 and  water  pollution.,   Considering  that 75 percent  of  the  overburden  has  a
 grain size  exceeding 2000 \im  (see Table 3.12), it  is  unlikely  tha': widespread
 physical  transport  v/ill  result  from  overburden  piles.  However,   using  over-
 burden  for  roads decreases  the  grain  size.  The  association  of  uranium  and
 progeny  with the smaller sediment-size fractions,  by a  factor  of 2.5,  in-
 creases  the potential  for transport by overland  flow.
      Tables 3.15, 3.16, and 3.19 show stable and  radioactive  trace elements
 in  ores, sub-ore,  and  overburden from uranium  mines.  Understandably,  uran-
 ium,  thorium, and  radium are  high.   Arsenic,  selenium, vanadium, and  moly-
 bdenum  are  almost  always  closely   associated  with  uranium.   Barium,  zinc,
 manganese,  copper,   iron, and  potassium may also be associated in certain
 mineral  provinces and districts.   Mercury  and  cadmium are  occasionally pre-
 sent (Th78).  There is no consistent  relationship  between ore  grade and  trace
 metal content in  selected New Mexico  and Wyoming study areas (Wo79).
      Particularly  in  the case  of  active  or  recently active  mines, surface
 runoff  is  collected  with  dikes and  ditches that  route water  to  settling
 ponds.   Water spray or  chemical additives can  control  road dust.  They are
 commonly  used in the  active  mining stage, but  almost never used during ex-
 ploratory drilling.  Grading piles  to a slope  of 3:1 or  less also  helps  to
 reduce  runoff (St78),  and  this practice  is becoming  common in Texas and
 Wyoming.    Proper planting  techniques  further   reduce runoff   by increasing
 infiltration and decreasing sediment  transport.
     The  significance  of surface  runoff   from  mining areas  as  a dispersal
mechanism was  investigated  as  part of  this  study (Wo79)  (see also Section
 3.2.3.2).    We  examined  stable and   radioactive  trace  elements  in   soils

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                                                                       3-199
 affected by  runoff from  ore,  sub-ore, and mine  waste/overburden  piles from
 one active  surface mining area in Wyoming and two inactive areas (surface and
 underground mines)  in New Mexico,   Although there  was evidence  of  offsite
 movement of  uranium and  radium  at all  sites,  transport is  limited  and de-
 creases with distance from the site.  In Wyoming, pollutant releases from the
 mine studied do not reach nearby water courses  although  onsite transport of
 stockpiled  ore as  a result of precipitation runoff does occur.
      A U.S. Bureau  of  Mines  (BOM,  no  date) study of strip and surface mining
 operations  and  their effects  in  the  United States  involved  questionnaires,
 literature  survey, and onsite examinations  of 693 selected sites, among which
 were uranium mines in New Mexico  and Wyoming.   At 60 percent of the sites,  on
 a  national  basis,  there  were no   serious  problems  because  vegetation  was
 reestablished and  the slope  of  the land  was  gentle  both  before  and  after
 mining.  Thirty percent of the sites  had eroded to  depths  of 0.3  m or less,
 and the remainder were  gullied to  greater  depths.   There  were sediments from
 mined lands in 56  percent of the ponds and 52  percent of the streams  on  or
 adjacent to the sample  sites.  Spoil  bank  materials  ranged  in pH from 3 to 5
 at 47 percent of  the  sites  and are thus not amenable to  plant growth.  Field
 observations  substantiate that rained  land  areas,  be they former  forests  or
 grasslands,  did  not return to  the  pre-mining condition.   Idle land increased
 almost fourfold because  of  mining.   The  study  concluded  that natural  pro-
 cesses need  to  be  strongly  supplemented  if mined  sites are  to  revert  to
 former uses.  Since only 6.3  percent of  lands  mined for  uranium were  re-
 claimed from 1930  through 1971 (Pa74),  it  seems reasonable to  conclude  that
 there are increased sediment loads, gullying,  and  poor revegetation at  most
 older inactive mines  that  were  poorly  stabilized,  if  at all.
      The  Bureau  of Mines  study concluded that  peak sediment  loads  in  runoff
 are characteristic  of areas  with   high  intensity storms and steep  slopes,
 particularly  during  and shortly after mining.   Such  problems  are less  severe
 in  arid regions,  but large quantities of  sediment are discharged  from mine
 workings, spoil "heaps, and access roads.   In some  instances,  effects  of wind
 and  water erosion  on steep spoil  banks  in  arid lands are evident many years
 after  abandonment.   In  areas  outside Appalachia,  86 percent  of  the areas
 investigated had sufficient runoff control,  and those  areas where there was a
problem  almost exclusively  involved  coal, phosphate, manganese,  clay, and
gold.

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                                                                       3-200
      Incidences  of  radioactive  contamination  of  local  surface  water  have  been
 documented  for  the Shirley Basin  uranium  mine (Utah  International,  Inc.)  in
 Wyoming  (Ha78).   The  most pronounced  changes in water  and stream  sediment
 quality  coincided with initial  strip  mining  and mill processing  operations.
 Early acid-leach  solution  mining  also   had  a  decided  impact.    Pollutant
 loadings  from  overland flow, per  se,  were not determined but  are  presumed  to
 be minor  compared  to aqueous discharges from mines and mills.  These  findings
 contradict  those  of  an  earlier  study  (WH76)  of  the same mine.   Soil  and
 vegetation  collected from 1971  through 1975 at 28 stations  in  the  vicinity  of
 the  mine  were analyzed  for gross  alpha   and  gross  beta (1971  to 1974) and
 total  uranium,  Ra-226  and Pb-210  (1975).  The study  (Wh76) concluded  that--
      1.   concentrations  of the foregoing  parameters were extremely variable
          but reasonably  consistent with previously  reported information;
      2.   there  is no evidence  that radionuclide concentration in  soil  or
          vegetation collected  from routine monitoring stations are changing
          with time;
      3.   concentrations  of radioactivity  in soil and  vegetation correlate
          with distance from the mill  area to  a distance of  1.2 miles;  and
      4.   measurable ecological  effects from radiation in the environs  of
          the Shirley Basin mine cannot be demonstrated.
 The  absence of  statistically  significant  soil  and  vegetation contamination
 from  the  mine  versus the mill  is  noteworthy.   Overall,   vegetation  tends
 toward  higher  alpha  and  beta  concentrations  than  soil,  except  at  the
 close-in, upwind  sampling areas.  This selective concentration in vegetation
 suggests aerial deposition of contaminated dust particles on vegetation, with
 some  additional possibility for  root uptake.
      Estimates of surface drilling for uranium  reveal that relatively large
 land  areas  are  involved.   The  volume  of cuttings removed from borings  in the
 period  1948 through  1979  is  calculated  using  286 x 10   m  of  exploratory
 drilling,_and 104  x 10   m  of development drilling  (from   Table  3.62).   We
 assumed that 30  percent  of the mines  are  surface mines, which eliminates the
 borings and  related debris.  Thus  the value of  149  x 10  (in Table 3.6H) is
 reduced by  30  percent.  Average diameter  for  8.5  x  10  m  of  borings in  the
 period 1948  through 1956  is 2.8 cm versus 7.3 cm for  the period 1957 through
 1979  (see Section 306.1)  when  426 x  10  m of drilling  took place.  A  sample
calculation  for  the volume removed from borings made  in the period 1975-1979
fn 11 nw; •

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                                                                       3-201
      V  = Trr  h /       \                                    (3.24)
         =  (3.14)17.43 cm]2 (146m)
                  V    2  /
         -  0.632 m3
 Assuming a bulk density  of 2000 Kg  per m s  each  boring  results in 1265 Kg  of
 cuttings at land  surface.   There were  415,300 borings, resulting  in  263,000
 m  of  cuttings-   Assuming  that the average  thickness  of cuttings is  0.5  m,
          2            2
 526,000 m  or 0.53 Km  is  affected.  The inclusive  area  affected  by drilling
 from 1948 through  1979 is 3.6  Km2.
      Table 3.66 summarizes the surface  areas affected by  mine wastes, ore
 piles, and exploration and  development  activities.   Maximum use was made  of
 data developed  elsewhere  in this report  on  the  number of mines, waste  pile
 dimensions and surface areas,  *wd the summary of  exploration and development.
 The estimate  is,  at   best,  a  first  approximation and needs considerable re-
 finement.
      For  example,  grain size,  degree  of consolidation,  slope,   vegetative
 cover,  and other  characteristics may vary considerably between ambient  soil
 and rock materials versus mine wastes.   The  latter very often occur in  steep,
 unvegetated  piles  and  are composed   of easily-eroded,  friable   sandstone,
 boulders,  and fines.   It is likely, therefore,  that the sediment yield  on a
 mass  per time per area  basis  exceeds that of  the surrounding areasj thus the
 estimate developed  below may well be on  the  low side.
      Sediment  yields   from  areas affected  by various mining "operations are
 roughly estimated from  consideration  of  land  areas affected  and  unit  soil
 loss  values  for the surrounding regions.  Actual values for individual tail-
 ings  or waste  piles  may be considerably different,  but  refining  the values
 given  will require additional  analysis beyond the scope of the  present study.
      Potential  coal mining  lands in the  Northeastern Wyoming range lose  soil
                          3   2
 at  rates of 4.8 to 167  m /Km  /yr (Ke76).  Upland erosion and  stream channel
 erosion  in the Gillette study area are not generally serious problems, since
 land  dissection Ms  presently minimal  and  vegetative  cover is well  estab-
 lished.  The  potential   for. increased sediment yield  Is  large,  if vegetative
 cover  were  to  be  reduced   or eliminated  and slopes  steepened  because of
mining.  Certainly,  during  active mining, these conditions will  be at least
                                                 3   2
locally  present.  Erosion rates of 600 to 1,100 m /Km /yr from mined lands in
the South  Powder River Basin are expected,  and  they are reasonably close to

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               Table 3.66   Sediment  yields  in  overland  flow  from  uranium mining areas
Source Term
Active Mines
Underground
Ore piles
Sub-ore piles
Waste rock piles
Surface
Ore piles
Sub-ore piles
Overburden piles
Factor
603 m2/mint
26,700 m /mine
26,700 m2/mine
4.15 x 103 m2/mine
67 x 103 m2/tnine
380 x 103 m2/mine
No. Installations
251 mines
251 mines
251 mines
36 mines
36 mines
36 mines
Cumulative
2
Source, Km
0.15
6.7
6.7
0.15
2.4
13.7
Annual Sediment
Loading, m
143
6385
6385
143
2287
13056
Inactive Mines
 Underground
  Waste piles and
     sub-ore
4.07 x 103 m2/raine
2108 mines
 0.86
  820
 Surface
  Overburden and
    sub-ore
6.73 x 104 m2/mine
 944 mines
64
61000
                                                                                                               o
                                                                                                               ro

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Table 3.66 (Continued)
Source Term
Factor
                    Cumulative
                              *
No. Installations   Source, Km*
     Annual  Sediment
     Loading, m 'a'
Exploration and Development
Drilling
1948-1979 435 x 106 m 1.28 x 106 borings 3.6
1975-1979 1265 kg/boring 415,300 0.53
3431
506
  Access roads and
    pads            1.25 acres or
                    0.5 ha/boring
               1.28 x 10l
                 6500
6.2 x 10"
     ^'Assumes average sediment yield of 953 m /Km .
     Note.—Data in this table are based on average mine vs. average large mine as defined in Section 3 of
report.
                                                                                                              to
                                                                                                              I
                                                                                                              1X3
                                                                                                              O
                                                                                                              to

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                                                                       3-204
 natural, pre-mining  conditions  (R. Loeper,  Soil  Conservation  Service, 1979,
 personal communication).   At the Bear  Creek mine,  the  reclamation design
                                                            3   2
 calls for maximum  losses  from overburden piles of  1,100  m /Km /yr initially
          3   2
 and 600 m /Km /yr after the first 3 years.  In general,  erosion and soil loss
 from uranium  mining  in this  part of  Wyoming is not a  significant problem,
 mainly  because  of reclamation  by industry.  Sediment yields  in  the Grants
                                     3    2
 Mineral  Belt  range  from 95 to  240 m /Km /yr  in  the area of the  large Jack-
                                                3   2
 pile-Paguate  surface  mine  to  500  to  1,400  m /Km  /yr  near the  underground
 mining   centers 'around  Smith  Lake,  Ambrosia Lake,  and Churchrock  (P. Boden,
 Soil Conservation  Service,  1979, personal  communication).   Considering  both
 the  Wyoming  and  New Mexico  model  mine  areas,  this study used  an  overall
                                          3    2
 average  annual  soil  loss  rate  of 953 m /Km.   This average  sediment yield
 rate is based on  studies  by the Soil  Conservation  Service  of  large areas  in
 New Mexico,  Wyoming,  and other Western  States.
      In  summary, the total  land area  directly affected  by  uranium mining  is
               2                                                         1    ?
 about 6600  Km .   Assuming an overall  average sediment  yield of 953  m /Km,
                                                                         ft   "3
 annual  sediment  transported by  overland  flow is  approximately 6.3  x  10  m .
 Obviously  exploration  and development  activities  affect  the  greatest area
          2
 (6500  Km ),  but  they   do   not  necessarily  have  the   greatest  impact.
 Exploration  and  development,  for example,  affect large areas, but most of the
 area affected   is  a result  of   constructing  access  roads  and  drill  pads.
 Whereas  sediment  yields  from ore, sub-ore,  overburden,  and  waste rock  is
                      3
 estimated  at 90,000 m   per year.   Surface mining, although it  supplies only
 about 30 percent  of U.S.  production,  affects the  second  greatest area (80
   2
 Km ).   We have not attempted  to characterize  the quality of  sediment  runoff.
 The  fate of  these  sediments  is  very poorly understood and  has not been the
 subject  of  intensive investigation.  Further  study  in the  area of  intensive
 surface  mining such as  in  Texas  and Wyoming  is needed to determine  changes  in
 erosion  rates resulting from mining and  to  quantify the contaminant flux and
 fate.
3.7   Inactive Mines

3.7.1  Inactive Surface Mines
     For  generic  purposes,  a model  inactive open pit or surface uranium mine
must be  defined  in  order to estimate the environmental impact from this type

-------
                                                                       3-205
 of mining.  We  have  assumed  that an  inactive  surface mine has a single hole
 or pit in the  ground,  with all of  the  materials (wastes) stacked into piles
 adjacent to the pit  area.  The size  or volume of the pit  would  be approxi-
 mately equal  to  the  volume of the ore and wastes removed from it. Since only
 6.3 percent of all  of  the land  used for uranium mining  has  been  reclaimed
 from  1930  through 1971  (Pa74),  no credit  for  reclamation  is given  to  the
 model  mine.
      Ideally,  the model mine  size could be established  by  averaging  the ore
 and waste production for  each  inactive surface mine.   Unfortunately, these
 statistics  are  either  not thoroughly  documented  or  they  are   retained  as
 company  confidential  information.   In  lieu of  specific information,  the model
 surface  mine  size was  established from annual  ore and waste production sta-
 tistics  for  all  surface  mines,   divided  by  the number  of  inactive  surface
 mines.
     Table  3.67 is a summary  of  inactive mines,  obtained from the Department
 of Energy mine  listing.   The  mines are  listed  by type, surface and  under-
 ground.   Most  of  the inactive surface  mines  are in Colorado, Utah,  Arizona
 and New  Mexico.   For model derivation  purposes, we  assumed  that  there  are
 presently  1250  inactive  surface uranium  mines.
     Table 3.68 lists mine waste  and  ore production  information  from  1932  to
 1977.  Uranium  mine waste  and  ore  production  statistics,  on  an annual  basis,
 were available  from  both  surface  and  underground uranium producers  from 1959
 to 1976  (DOI59-76).    Annual   uranium  ore  production   statistics  for  each
 uranium  mining  type  (surface and  underground)  are available for  1948  to 1959
 (DOE79) and for  combined uranium production from  1932  to  1942 (DOI32-42).   In
 order  to estimate  waste production for  the years  prior  to  1956, the  annual
 mine  type ore   production  records  were multiplied  by waste-to-ore  ratios.
 These  ratios were  estimated from published 1959 to 1976 ore  and waste  produc-
 tion statistics  (DOI59-76).  Very little  uranium ore  was mined from  1942  to
 1948,  since  most  of  the  uranium  was  obtained by  reprocessing vanadium and
 radium tail ings, (personal   communication with  S.  Ritter, Bendix   Field  Engi-
 neering  Corp.,  Grand Junction,  CO, 1979).  The  annual  waste  production for
 surface  mining  from   1948 to  1959  was  estimated  by  extrapolating   known
waste-to-ore ratios (1959  to 1976) through the  1948 to  1959  time period  using
a  "best  fit"  regression analysis  (Fig.  3.23).  This method  cannot be used  to
estimate  waste-to-ore ratios  because the waste production is finite and will
always  occu'% and  also  surface mining for uranium essentially  began in 1950.

-------
                                                                    3-206
        Table  3.67    Consolidated  list  of  inactive  uranium  producers  by
                     State and  type  of  mining
State
AL
AZ
CA
CO
ID
MT
NV
NJ
NM
ND
OK
OR
SD
TX
UT
WA
WY
Surface
0
135
13
263
2
9
9
0
34
13
3
2
111
38
378
13
223
Underground
1
189
10
902
4
9
12
1
142
0
0
1
30
0
698
0
32
Percent of Total
Surface Mines
0.0
11
1.0
21
0.16
0.72
0.72
0.0
2.7
1.0
0.24
0.16
8.9
3.0
30
1.0
18
Percent of Total
Underground Mines
'0.1
9.3
0.49
44
0.20
0.44
0.59
<0.1
7.0
0.0
0.0
<0.1
1.5
0.0
34
0.0
1.6
Total
1246
2031

-------
      Table 3,68  Uranium mine waste and ore  production  (MT x 1000)
Surface ..Mini rig
UndergroundMlnlng   Surface Mining
Underground
   Mining
  Total Ore
 Produced By
Surface and/or
Year
1977
1976
1975
1974
1973
1972
1971
1970
1969
1968
1967
1966
1965
1964
1963
1962
1961
1960
1959
1958
1957
1956
1955
1954
Crude Ore
5059
4238
3809
: 3510
3800
3447
2656
2490
1653
1989
1393
905
1630
2344
3578
2895
3051
2691
2494
2139
1462
1131
339
241
Waste
237800
190700
139700
129700
182300
155100
120200
76870
81000
31360
32510
24400
17710
26680
33120
44640
42500
73570
46790
19240
11700
9048
2650
1930
Crude Ore
4305
3569
2485
2222
1614
2439
2836
3304
3171
3382
2897
2777
3055
3227
3575
4892
5017
5104
3796
2558
1888
1595
1043
762
Wasti
3487
2605
2195
1424
934
593
858
962
1184
1163
10Z4
863
809
941
946
1087
1117
1868
941
690
510
414
271
198
Waste/Ore
47
45
37
37
48
45
45
31
49
16
23
27
11
11
9.0
15
14
27
19 ,.
9.0(a)
8.0
8.0
8.0
8,0
Waste/Ore Underground Mines
0.81 •
0.73
0.88
0.64
0.58
0.24
0.30
0.29
0.37
0.34
0.35
0.31
0.26
0.29
0.26
0.22
0.22
0.37
0.25,..
0.27(b)
0.27
0.26
0.26
0.26
9364
7807
6295
5732
5414
5886
5492
5794
4824
5371
4290
1768
4685
5571
7153
7787
8068
7795
6290
4697
3350
2726
1382
1003
                                                                                                        i
                                                                                                        r>o
                                                                                                        O
                                                                                                       -sa

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Table 3.68 (continued)
  Total  Ore
 Produced By
Surface and/or
         Surface Mining
Underground Mining   Surface Mining
Underground
   Mining
Year Crude Ore Waste
1953 162 1300
1952 59 472
1951 25 203
1950 21 167
1949
1948
1947
1946
1945
1944
1943
1942
1941
1940
1939
1938
1937
1936
1935
1934
1933
1932
Crude Ore Waste Waste/Ore
503
341
289
207
156
34
0
0
0
0
0
0
0.824
0.7221
5.68
3.89
1.55
1.31
1.03
0.230
0.047
0.0553
126 8.0
85 8.0
73 8.0
50 8.0
37
8.3






0.181
0.151
1.19
0.817
0.310
0.261
0.207
0.0461
0.00896
0.0105
Waste/Ore
0.25
0.25
0.25
0.24
0.24
0.24
0.24
0.23
0.23
0.23
0.22
0.22
0.22
0.21
0.21
0.21
0.20
0.20
0.20
0.20
0.19
0.19
Underground Mines
665
400
314
228
156
34






0.824
0.722
5.68
3.89
1.55
1.31
1.03
0.230
0.047
0.0553
      Ijjjwaste to ore ratios  from 1950 - 1958 estimated from 1959 - 1972 ratios.
      *  'Waste to ore ratios  from 1932 - 1958 estimated from 1959 - 1972 ratios.
                                                                                                               PO
                                                                                                               o

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60
50
40
                                                                                         *  *
20
                                                        •  *
                                                                                                                            UJ
                                                                                                                             I
0

1948
              1952          1956         1960         1964         1968          1972

                                                       YEAR

                 Figure 3.23 Annual waste to ore ratios for surface mining of uranium (1948 to 1979).
1976
1980

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                                                                       3-210
      Since  early surface  mines recovered ore  bodies  very close to  the  sur-
 face,  the ore-to-waste  ratio  would  be  expected to  be relatively small.   A
 range of waste to  ore  ratios of  8:1  to 35:1 for surface  mining  has  been
 estimated  (C174),    The  lower  ratio  was  selected to  be typical for surface
 mining  from 1948 to 1957 and  was used to estimate  the waste production  for
 that  period.   The   increase *in waste-to-ore  ratios  from 1959  to  1976  was
 probably  due to several  reasons.  The  gradual  depletion of near surface  ore
 deposits  required  mining deposits at increasing  depths, and the development
 of  surface mining equipment now permits economical recovery of ore  at greater
 depths  below grade.   The waste-to-ore ratios for 1976  to  1977 were projected
 with  the  previous regression analysis line fit.
      The  estimated  annyil cumulative waste  production  from  uranium  surface
                                                   9
 mining  for  1950 to  1978  (Table 3.69) is  1.73 x 10  MT.  A crude estimate of
 the  waste  production  for the model  inactive  surface  mine  can be  made by
 dividing  the total   waste produced  to 1978 by  the  number of inactive mines.
 But,  this  overestimates  waste production because  some  of  the  contemporary
 wastes  are  being produced by  active  mines, and the waste production  per mine
 has  increased  with  increasing contemporary  waste-to-ore  ratios.   To adjust
 the  contemporary waste  production  for the active  mines and  the  increasing
 waste-to-ore ratios,  we  assumed a cutoff date  of 1970,  based on the  descrip-
 tion  of a contemporary  active surface mine  (N179).   The model  mine age is
 about  1 year as of  June  1978, and  has an expected  life of  approximately 17
 years.  Those mines  that were active in  1970 are all  assumed to have become
 inactive  between 1970  and 1978.   Their  percentage of the  annual waste  of
 about 12,5 percent was assumed  to decrease linearly with time from  1970-1978.
 For example, all  of  the  wastes produced by surface mines in 1970 (i.e., 7.69
 x 10  MT) were  produced  by surface mines that would be  inactive by 1978. The
                                                                      8
 waste production for the following  years (1971-1977) was:   1.05 x 10  MT in
 1971; 1.16 x 108 MT  in  1972;  1.14  x  108 MT in  1973;  6.49 x 107 MT  in 1974;
 5.24 x 107 MT in 1975; 4.77 x  1C7 MT  in 1976; 2.97 x 107 MT In 1977.  The ore
 production was calculated in the same manner as for the wastes and was 3,27 x
 10  MT  in 1970.   The ore production  for the following years was:  2.32 x 10
MT in 1971;  2.58 x  106 MT in  1972;  2.38  x 106 MT  in  1973;  1.76 x 106 MT in
 1974; 1.43  x 106 MT in  1975; 1,06 x 106 MT in  1976,  and 6.32  x  105 MT in
1977.  The adjusted  cumulative wastes from surface mining from 1950-1978 was
         9                                                              7
1.11 x  10  MT,  and  the adjusted cumulative ore production was 4,49 x 10  MT.

-------
Table 3.69   Cumulative uranium mine  waste  and  ore  production
Year
1977
1976
1975
1974
1973
1972
1971
1970
1969
1968
1967
1966
1965
1964
1963
1962
1961
1960
1959
1958
1957
1956
1955

Surface
1733000
1496000
1305000
1165000
1036000
853200
698100
577800
501000
420000
388600
356200
331800
314000
287300
254200
209600
167100
93510
46720
27470
15770
6720
Waste (103MT)
Underground
29250
24950
21380
19180
17760
16820
16240
15370
14410
13220
12060
11040
10180
9369
8425
7479
6391
5273
3406
2466
1776
1266
852

Surface
59220
54160
49920
46110
42600
38800
35350
3E700
30200
28550
26560
25170
24260
22640
20290
16720
13810
10770
8075
5580
3442
1979
848
Ore (103MT)
Underground
73100
68840
65210
62760
60500
58960
56510
53600
50330
47160
43810
40910
38090
35000
31750
28210
23310
18320
13150
9433
6839
4943
3356
                                                                                                   u>
                                                                                                   1
                                                                                                   PO

-------
,   Table 3.69 (Continued)
Year
1954
1953
1952
1951
1950
1949
1948
1947
1946
1945
1944
1943
1942
1941
1940
1939
1938
1937
1936
1935
1934
1933
1932
Waste (lp3MT)
Surface Underground
r
4071 580
370 171
842 257
370 171
167 98.9
48.6
11.4
3.18
3.18
3.18
3.18
3.18
3.18
3.18
3.00
2.85
1.67
0.844
0.533
0.272
0.0656
0.0195
0,0105
Ore [103MTJ
Surface Underground
509 ' 2313
46.3 702
105 1043
46,3 702
20.9 413
206
49.8
15.3
15.3
15.3
15.3
15.3
15.3
15.3
14.5
13.8
8.12
4.24
2.68
1.37
0.333
0.102
0.0553
                                                                                                                      OJ
                                                                                                                      I
                                                                                                                      IV

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                                                                       3-213
 Using  these adjusted waste and ore values, the model inactive uranium surface
 mine produced 8.88 x 105 MT of waste and 3.59 x 104 MT of ore.
      The volume  of the remaining pit of the model  surface mine would be equal
 to  the total  of  the volume of wastes and ore that were removed from the mine.
                                 3
 Assuming a density  of  2,00 MT/m , the volume  of  wastes and qre removed from
                                 c               43
 the mine pit would  be  4.44 x 10  and  1.80 x 10  m ,  respectively.   The pit
 was assumed to have the shape of an  inverted truncated cone with a wall  angle
 of  45°  (Fig.  3.24).   The ore body was  assumed to be a  solid  right  cylinder
 with a radius of  43.7  m and height of  3.0 m.   The pit depth (ground surface
 to  bottom  of ore  bed)  was 36.7  m,  and  the  ground surface area  of  the pit
 opening  was calculated  to be 2.03 x  10  m .

 3.7.1.1   Waste Rock Piles
     Overburden  and  sub-ore wastes  from  surface  mines  have been  handled  in
 several  ways  in  the  past.   In one  case, the sub-ore  (generally the  last
 material  removed  from  the pit)  was  piled  on  top  of the overburden.  In  an-
 other  case  the sub-ore  was piled separately and blended with higher grade ore
 for shipment  to  the ore buying  stations  or mills.   If  the quantity of sub-ore
 was in excess of  that required  for blending,  it was  also dumped on top of the
 overburden  (personal communication  with  G, Ritter, Bendix  Field  Engineering
 Corp.,  Grand  Junction,  CO,  1979).    The  earlier  surface mining  practices,
 therefore,  generally produced waste  piles with their cores  containing  over-
 burden  and  their  outer  surface containing   a  mixture  of  overburden and
 sub-ore.
     The  actual method  of removing and  stacking overburden  and  sub-ore varies
 from mine to mine.   In many cases the wastes  were  dumped in depressions  or
 washes or stacked  in more than one pile.   For calculation purposes, we assume
 that  wastes are  stacked  on  a  single pile  in the  shape of a solid truncated
 cone  10  m  high  with  a  45  degree  slope.   It is further  assumed that the
 sub-ore  removed  from the pit is  placed evenly on  top of the stacked  over-
 burden.  The area and depth  of  the sub-ore placed on  the waste pile  is  esti-
mated by  determining the areas  of the base and  top  of  the  pile by  iteration,
 computing the exposed  surface area of  the pile, computing  the volume of the
 sub-ore, and  calculating  the depth of the  sub-ore.
     The  areas of  the  base  and  top  of the  waste  pile (truncated cone) were
determined from the following equation:

-------
                                                                              80.4
                                                           43.7
Figure 3,24 Cross section of rnodei inactive surface mine (meters).
 i
KJ

-------
                                                                       3-215
 V = Jl (Ag + AT +X/lgM   where V = volume of wastes (overburden     (3.25)
     3                               and sub-ore) (m )
                                                        o
                                   = area of the base (m )
                                                       2
                                   = area of the top (m )
                                 h = perpendicular distance between
                                     the base and top (10 m)
 Different values of AD were  substituted Into the equation until  the value of
                      D
 V was equal to  the  combined  volumes of the overburden and sub-ore (I.e;  5.55
 x 10  m ) using a"  bulking  factor of 251.   The area of the cone  top was  com-
 puted (assuming a 45 degree  slope)  from the diameter  of the  top (0^), which
 is equal  to the diameter of  the base  (DD)»  minus  20 meters or D, * Dn - 20-.
                                         D                        I     D
 The  calculated  diameters,  DT  and  DB» are  256 m  and 276 m» respectively.
      The  exposed  surface area  of  the  waste pile  was calculated using  the
 following  equation:

 S = S, -f  ST                 where S,  =  lateral  surface area (mz)    (3.26)
                                   \ HE (CB  +  CT>
                                                          7
                              and S, =  area of  the  top  (m )
                                    I        2
S = JL '(Cp + CT) "•" ir*V       where Cg = circumference of the base (m)
    2                              c, = circumference of the top (m)
                                   L = slant height (m)
                                  r, = radius of the top (m)
                         2
S = 14.1 (w DT + wDR) + irr  where  DT = diameter of the top (m)
      2                           Dl = diameter of the base (m)
S a 14.1 (3.14) {256 + 276) + 3.14 (16384)
      2
S = 6.33 x 10  m  (exposed surface area of waste pile)
The volume  of- sub-ore  removed  from the  pit is  assumed  to be  equal  to the
volume of ore removed from the pit. The thickness (T) of the sub-ore plate on
the overburden 1s —
T • 1° s 2.25 x 104fn3  - 0.36m.
    S    6.33 x 104m2                                                  (3.27)

-------
                                                                       3-216
      In  summary,  the waste pile  produced  at an inactive uranium surface mine
 is  to be  in  the shape of  a  truncated  cone  having  a  surface  area  of 6.33 x 10
  p
 m .   The  pile  is assumed  to have  an  inner-core  of overburden  plated  with 0.36
 m of  sub-ore  on  its exposed  surface.    In  practice,  the plate  would  be  a
 mixture  of overburden and  sub-ore with  the  sub-ore concentrations  increasing
 towards the  pile surface.
      Table 3.70 lists  average  annual emissions  of contaminants due  to wind
 erosion  of the overburden  pile.  To  compute these  values,  an  emission factor
 of  0.850  MT/hectare-yr»  computed in Appendix  I, was multiplied by  the pile
 surface  area,  6.33 hectares,  and the stable element concentrations  listed  in
 Table  3.19.   Uranium and thorium concentrations  were assumed  to be  110 pCi/g
 and  2  pCi/g» respectively.

 3.7.1.2   Radon-222 from the Mine  Area
     After the termination  of active mining, Rn-222 will  continue  to  exhale
 from  the  wall  and  floor  of the  pit.   Since all  of the  ore has been removed,
 the  Rn-222 will originate from the overburden and sub-ore surfaces.   The sur-
 face  area of the sub-ore region  of  the pit  is estimated  from the  volume of
 ore  and  sub-ore {3.£
 following  equations:
ore and sub-ore  {3.6  x  10  m ) and  the  shape and size, of  the  pit using the
          V - 1/3 h (AT -f- AB +\/A^" }where: AT =  * r?              (3.28)

          S - 1/2 L {CB + Cb) + AB          AB   =  7rr|               (3.29)

The  terms in  the  equations are  defined in  the  previous Section.   By sub-
stituting  the terms  rg +  h  for r,  in  Equation  3.28,  h  can be  solved  by
iteration.
V = 3.6 x 104 m3 - 1/3 h [it (rn + h}2 +  IT rf +
 \A (rn + h}2 { Trr2) jwhen h = 5.3 m
        '-•'
The exposed surface-area of the pit that contains the sub-ore is
          Ss = 1/2 (7.50) Tr(87.4 + 98.0} + 6000 = 8.18 x 103 m2,

and the surface area of the overburden section  of the pit is
          SQ - 1/2 (44.4) (TT) (98.0 + 161.0) = 1.81 x 104 m2.

-------
                                                                      3-21?
     Table  3.71  shows the  results  of radon flux measurements made  at 20 of
the tailings  piles  at inactive uranium mil! sites.   Also shown  is the esti-
mated average  Ra-226  content of the  tailings and  the average Ra-226 content
Table 3.70  Average annual emissions of radionuclides (pti) and stable
            elements (kg) in wind suspended dust at the model  inactive
            surface mine
Contaminant
Arsenic
Barium
Cadmium
Cobalt
Copper
Chromium
Iron
Mercury
Potassium
.
Magnesium

Manganese
Overburden
Pile(a)
0.46
4.9
ND^
0.09
0.33
0.11
84
ND
135

19

5.2
Contaminant
Molybdenum
Nickel
Lead
Ruthenium
Selenium
Strontium
Vanadium
Zinc
Uranium-238 and
each daughter
Thorium-232 and
each daughter

Overburden
0.62
0.11
0.42
ND
0.59
0.70
7.6
0.16

1480

11

     (b)
     Emissions = 5.38 x 10  g/yr.
ND - Not detected.

-------
                                                             3-218
Table 3.71  Average radon flux of inactive uranium mill tailings piles
Location
ARIZONA
Monument Valley
Tuba City
COLORADO
Durango
Grand Junction
Gunnlson
Maybe! 1
Naturita
New Rifle
Old Rifle
Slick Rock
IDAHO
Lowman
NEW MEXICO
Ambrosia Lake
Shiprock
OREGON
Lakeview
SOUTH DAKOTA
Edgemont
TEXAS
Falls City
Ray Point
UTAH
Green River
Mexican Hat
Salt Lake City
WYOMING
Spook Site
Average All Sites
Average
Radon Flux'3^
(pCi/m2-sec)
20
193
197
359
470
86
1446
458
553
70
125
173
340
660
143
65
430
77
290
1200
1770
466
Estimated
Ra-226(b)
Tailings Content
(pCi/g)
50
924
840
784
420
252
756
504
980
171
760
700
420
448
518
140
784
896
356
563
Average
Ra-226
Background
Soils(a)(pCT/g)
0.95
0.95
1.48
1.52
1.48
1.52
1.48
1.52
1.52
1.48
1.12
1.02
1.7
0.81
1.33
0.93
0.93
1.43
0.83
1.4
0.99
1.26
Reference^8'
FBD-GJT-4 (1977)
FBD-GJT-5 (1977)
FBD-GJT-9 1977}
FBD-GJT-9 1977)
FBD-GJT-12 1977)
FBD-GJT-11 (1977)
FBD-GJT-8 1977 r
FBD-GJT-10 (1977)
FBD-GJT-10 (1977}
FBD-GJT-7 (1977^
FBD-GJT-17 (1977)
FBD-GJT-13 (1977)
Bernhardt et al.
(1975)
FBD-GJT-18 (1977)
FBD-211 (1978)
FBD-GJT-16 (1977)
FBD-6JT-20 (1977)
FBD-GJT-14 (1977)
FBD-GJT-3 (1977)
Bernhardt et al.
(1975)
FBD-GJT-15 (1977)
JPJFBD77.
(DJ Sw76.

-------
                                                                       3-219
measured  in  representative background  soils for each site.  The average radon

exhalation  rate  per  average Ra-226 content of tailings  material  from these
                         2
data  is 0.83 pCi  of Rn/m -sec per pCi  of Ra/g.

      Data  analysis by  Schiager  (Sc74)  indicates  a radon exhalation  rate  of
                2
1.6  pCi  of  Rn/m -sec per pCi of Ra/g.   This value has often been used in the

environmental  impact  statements to assess the radon flux from tailings mater-

ials.

      Table   3.72  summarizes  data  obtained  during  radiological  surveys  of

inactive  uranium mine  sites in  New Mexico and Wyoming during the spring  of

1979  (Wo79).  Radon  exhalation  rates  were measured with  charcoal  cannisters

and  the;  radium-226  concentrations were  determined   for composite  surface

samples  taken from  overburden,  sub-ore,  and waste rock  piles.  The  average

radon-222  exhalation rate  per  average  radium-226  content of the overburden,
                                                                    2
sub-ore,  and waste rock  piles  was 0.27, 0.11,  and  0.12  pCi  of Rn/m -sec per

pCi of Ra-226/g,  respectively.

     Measurements  of  the background flux  and Ra-226 content  of typical  back-

ground  soils  were  reported  for  the  Edgemont, South Dakota  site (FB078).
                                                 2
These data  indicate a value  of 1.05 pCi  of Rn/m -sec  per pCi of  Ra/g.   Table

3.73  summarizes  background  radon flux  estimates  for several regions  of the

United States.   Considering the  average  U.S. background flux to be 0.82 pCi
       o
of Rn/m -sec  (Tr79) and  the average U.S.  background  soil  Ra-226 content  to  be

1.26 pCi of  Ra/g  (Oa72),  the  average U.S.  background radon exhalation  rate  is
                                   2
estimated  to be  0,65 pCi  of  Rn/m -sec per  pCi of Ra/g.  The average  back-

ground radon exhalation  rate  for New Mexico and Wyoming  (Table  3.72) was  0.33
            2
pCi of  Rn/m -sec  per pCi of Ra/g.  Therefore,  the grand average U.S.  back-
                                                                         2
ground radon exhalation  rate has  been  estimated to be 0.68  pCi of Rn/m -sec

per pCi  of  Ra/g,  and the 'grand  average  U.S. background soil Ra-226 content

has been estimated to be  1,6  pCi/g.

     We estimated  the total radon released  from the model abandoned surface

mine area  from the following  parameters:

     1.    Radon,.exhalation  from  the sub-ore  surface  area of the pit—
                                                              3  2
          .  the exposed  sub-ore  surface area (S )  = 8.18  x 10  m ;

          .  the average  radium-226 content  of the sub-ore -  110 pCi/g;  and
                                                             2
             the radon flux rate  for sub-ore = 12 pCi of Rn/m -sec.

-------
"able 3.72  Average radon flux measured at inactive uranium  mine  sites
.ocation
r
Inderg round Mints
i
San Mateo Mine,
New Mexico

Barbara J # 1 Mine,
New Mexico
lurface Mines
Poison Canyon 1,
New Mexico

Poison Canyon 2,
New Mexico
Poison Canyon 3,
New Mexico
Morton Ranch
(Pit 1601),
Wyoming
irand Averages



Area


Waste pile
Heap leach pond
Background
Waste pile
Background

Sub-ore
Overburden piles
Background
Sub-ore
Overburden pile
Sub-ore

Sub-ore
Overburden
Background
Sub-ore
Overburden
Waste Rock
Background
Average Radon
Flux (pCi/mZ-sec)


18
38
0.29
7,9
0.41

7.0
6.7
0.33
5,3
9.8
11

24
9.7
2.3
12
8.7
13
0.83
Number of
Flux Measurements


11
3
1
6
1

1
5
1
3
6
2

12
4
2




Average Radium-226
Content of Surface
Sample (pCi/g)


117
81
0.77
110
3

43
62
2.1
—
—
___

170
23
3
110
32
110
2.2






















                                                                                                                  I
                                                                                                                  r\3
                                                                                                                  ro
                                                                                                                  o
     Source: Wo?9.

-------
                                                                       3-221
          Table  3.73    Background  radon  flux  estimates
                                              Radon  Flux
                                                  2
Location	;	pCi/m  -sec
Background Soils of  the U.S.
Champaign County,  Illinois                    1.4
Argonne, Illinois  "                           0.56
Lincoln, Massachusetts                        1.3
Socorro, New Mexico                           0.90
Socorro» New Mexico                           1.0
Socorro, 1'ew Mexico                           0.64
Yucca Flat, Nevada                            0.47
Texas                                         0.27

                                               2
Average U.S. Background Radon Flux = 0.82 pCi/m -sec.

Source: Tr79.
Therefore,  the radon  released  from the  sub-ore surface area  of the pit  is
8.18  x  103 m2  x 12 pCi  of  Rn/rn2-sec  x 86400 sec/day  =  8.48 mCi of Rn/day.

     2.   Radon exhalation from the overburden surface area of the pit—
          .  the exposed overburden surface area (S } =
                      4.  9                         °
             1.81 x 10* m*;
             the average radium-226 content of the overburden = 32 pCi/g; and
                                                                  2
          .  the radon flux rate for overburden  is 8.7 pCi of Rn/m -sec.

Therefore,  the  radon  released  from the overburden surface area of the pit  is
1.81 x  104  m2  x 8.7 pCi  of  Rn/m2-sec  x 86400 sec/day  =  13.6 mCi of Rn/day.

-------
                                                                       3-222
      3.    Radon exhalation from the overburden pile remaining at the pit—
           .   the exposed surface area of the waste pile (S,,) =
                        4  ?
               6.33 x 10  m ;
           .   the Ra-226 content of the surface of the overburden pile is
              the same as the  sub-ore content = 32 pCi/g; and
           .   the radon flux rate for the overburden pile is 8.7 pCi
                      2
               of Rn/m -sec.
                                                                             4
 Therefore,  the radon  exhalation  rate from the overburden  pile  is  6.33 x 10
 m2  x  8.7  pCi  of Rn/m2-sec x 86400 sec/day -  47.6 mCi  of Rn/day.
      The  total radon  release rate  at the abandoned  surface  mine  site is the
 sum of  the   above  three  source terms,  69.7 mCi/day.   The estimated  radon
 release  rate for background soils  for an undisturbed area  equivalent to the
 surface mine  area  uses the following parameters:
      .   the  ground surface area equivalent to the area  of the pit  opening
         (2.03 x 10  m2)  and the overburden pad area (5.98 x 10   m2)  = 8.01
             4  2
        x 10   m ,  and
      .  the  radon  flyx rate for background soils  in uranium mining
          areas =  0.83 pCi  of Rn/m  -sec  (Table 3.72).

 Therefore, the radon exhalation  rate  from an undisturbed area  equivalent  to
 the model surface mine is
                       4   ?                   2
              8.01  x  10  m  x 0.83 pCi  of  Rn/m -sec  x  86400 sec/day =
              5.7 mCi  of  Rn/day.

     Table  3,74  summarizes  the  annual   radon-222 release  from  the  model
 inactive  uranium surface  mine and all  inactive uranium  surface mines.
3.7.1.3  Land Surface Gamma Rad_1at1o_n_
     The  surface mine  uranium  overlying strata must  be  removed in order  to
gain access^.tg  the uranium-bear ing host materials and the ore body.  The ore
body consists  of ore and sub-ore, and the sub-ore is  simply  that fraction  of
the  ore  body that  contains  ore uneconomical to recover.   The  end result  of
the  mining  is  that   the  residues  (sub-ore)   enhance   natural  radioactive
materials.  That is, they are exposed or brought to the earth's  surface.  The
enhancement  will  cause,  in  most  cases,   increased  aboveground  radiation

-------
                                                                       3-223
 Table  3.74     Summary of estimated radon-222 releases from
              inactive surface mines
 Source
 Estimation Method
Annual Release, Ci
Mine  Pit

   Sub-ore  are**


   Overburden  «
-------
                                                                       3-224
 exposure rates around the mining area.  Ore and sub-ore lost through handling
 are subject to wind  and  water erosion.  This  effectively  increases the mine
 site area  in  a  radiological  sense.   The gamma radiation  exposure  levels on
 and around a  mine  site  can  be high enough  to  restrict use of the area after
 mining.
      Gamma radiation surveys were  conducted  at some inactive uranium surface
 mining  areas.   Table 3.75 lists  the ranges  of exposure  rates found.   Appendix
 G contains more  specific information  concerning  the  surveys.  The residual
 exposure rate  levels  would  probably  preclude  unrestricted use of  the pits,
 waste piles,  and  overburden.
      Figure 3.25  depicts gamma  radiation  measurements made  on radials  ex-
 tending outward  from  an  inactive  surface  mine pit.   The  measurements  were
 made with a pressurized  ion chamber  (PIC)  at approximately 61  m intervals on
 each radial. As expected,  the  exposure  rate  decreases with  distance  away  from
 the pit, indicating surface contamination  from wind and water  erosion  of the
 spoils  and ore  piles.   Some  of  the contamination  may also have originated
 from ore and  sub-ore dust losses  during mining.
      Since  the pit resides over  a  former ore body and  connecting or adjacent
 ore bodies may  be  located  near the mine,  some  caution  is necessary  when
 interpreting the  gamma exposure rates as  indicative  of  surface  contamination.
 Development  drilling,  indicating the presence  of   ore  bodies, is  prevalent
 throughout  the north, west,  and  south  areas  around  the pit.   The northeast,
 east, and southeast areas around the  pit  have  exploratory  drill holes only.
 They  indicate  the probable absence  of ore bodies.  Although  the  north,  north-
 west, west, and  southwest  radials  cross  below grade  ore  bodies,  it  is  not
 reflected  by   the gamma measurements.   Unless the  ore  body is  very close to
 the  surface,  its  gamma radiation will  not  be measured  (i.e.,  the 1/10 value
 layer  for earth  shielding is  about 0.3 m).  The south radial, however,  did
 cross an  ore outcropping.
     If  the exposure rate measurements made at the  end points  of the radials
 (south  radial  excepted)  are  assumed to be  near background, their  mean value
 is 14.4yR/hr  with a 2 sigma error of 1.6y R/hr.
     Assuming  all measurements  in excess  of  14.4 +  1.6 u R/hr or 16.0 yR/hr
are  a  result   of  eroded ore  and  sub-ore from the mining  activities, an  iso-
exposure  rate  line  enclosing  the eroded materials can  be  constructed around
the  mine  site.  The  line is  constructed  on Fig. 3.25 and is qualitatively

-------
                                                                       3-225
           Table  3.75  Summary of land  surface gamma radiation surveys
                       in New Mexico, Texas and Wyoming
 Location
    Area
                                                  Gamma Radiation
                                                  Exposure Rate  (y R/hr)
Poison Canyon,
New Mexico
Pits
Waste piles
Overburden
40 to 190
65 to 250
25 to 65
Texas
Morton Ranch, Wyoming
(1601 Pit)
Pits
                                                        5 to 400
                                                       16 to  63
                                                       59 to 138
Source: Wo79 for New Mexico and Wyoming and Co77 for Texas.
Pit
Ore piles
Overburden
adjusted on the south radial to compensate for the ore outcropping.  The line
bulges  into the  southeast  quadrant  indicating  erosion by  the predominant
                                                 2
northwest winds and contamination of about 0.3 km.
     In summary, it appears that the residual gamma radiation exposure levels
at surface  mining  pits  and overburden piles  would  preclude these areas from
unrestricted use.   It also appears that wind and water erosions of the spoils,
ore, and  sub-ore  are  occurring  and causing  land contamination  far removed
from the  mining  area.    Several  surface mines  were  gamma surveyed  in  New
Mexico.  The mines could not be individually gamma radiation surveyed because
of their  close proximity,  cross  contamination from eroded ore  and  sub-ore,
and possible ore outcrops.

-------
                                                                   13$
                                                                141
                                                              fSJ
                                                            149
                                                         1SI
     GROSS GAMMA EXPOSURE BATE
                                              231 58S   \210   224,^220  f|E  1«3  173 1701S1162 ISO 15S  132

                                                X        '                                   \
                                                              344
                                                                 Z31
                                                                   S42
                                                                           170
                                                                               1S4
Figure 3,25  Results of gamma exposure rate survey at the 1601 pit and environs, Morton Ranch uranium mine,

            Converse County, Wyoming {/* R/hr)
 I
t\>
f-J

-------
                                                                       3-227
 3.7.2  Inactive  Underground Mines
      The model  Inactive underground mine is basically defined by dividing the
 total reported  volumes  of ore and waste removed by inactive underground
 mining by the number of inactive  underground mines.   The number of Inactive
 underground  mines  has been obtained from the U.S.  Department of Energy mine
 listing in Table 3.67.   Table 3.67 lists the mines by state and type of mine.
 Forty-four percent of the inactive underground  mines  are located in Colorado,
 34 percent in Utah,  9.3 percent in Arizona, and 7.0 percent in  New Mexico.
      For model ing'purposes,  we assume that  there are  presently  2030 inactive
 underground  uranium  mines.  Table 3.69 lists the estimated  underground mine
 waste and ore production for 1932 to 1977.   Uranium mine waste  and ore1 pro-
 duction statistics,  on  an annual  basis,  were available for  underground pro-
 ducers from  1959 r,o  1977 (DOI59-76).   Annual  uranium  ore production statis-
 tics  for underground mining  are available from  1948 to 1959 (DOE79) and from
 1932  to 1942 (DOI32-42).  We  estimated the mine  waste  production for the period
 of 1932 to 1960  from underground  mining  waste-to-ore  ratios and established
 waste-to-ore ratios  using the published  ore and wastes production  statistics
 from  1959 to 1976  (DOI59-76). These ratios were fitted with a  line by re-
 gression  analysis  in order to estimate the  waste-to-ore ratios  from 1932 to
 1959  (Fig. 3.26).  Two lines  were  fitted  to  the  known  waste-to-ore  ratios
 because of the abrupt change  in the ratios  from 1972  to 1976.   We  assumed
 that  the  steeper slope  was caused  by increased  waste  production from the
 larger and deeper  underground mines operated  during this time.   The estimated
 annual  waste-to-ore  ratios were multiplied  by the  published annual  ore pro-
 duction values to  estimate the annual  waste production from 1932 to 1959.   We
 assumed  that no  ore  was  produced  from 1942  to 1948 because  most of the uran-
 ium was obtained by  reprocessing  vanadium and radium  tailings during  that
 period  (Private  communication with  G,  C,  Ritter, 1979, Bendix Field Engi-
 neering Corporation,  Grand Junction,  Colorado).  Table 3.69 lists  the  cumu-
 lative  annual waste  production from underground mining from 1932 through
 1977.   The total waste  produced for this  period was 2.92 x  10   MT,  and the
 total ore  produced was  7.31 x  10  MT.
     A  simplistic  way to  identify a model inactive underground  mine would be
 to divide the cumulative  tonnage of ore and wastes by  the number of inactive
mines.  We estimated  the  number of  inactive mines  from the  U.S.  Department of
 Energy mine  listing  (Section  2.0 and  Table  3.67).  The model  inactive  under-

-------
     1,2-
     1,0-
    0,8_
g  0.4-
                                                                                      *  *
    0,2 —
        1932
1937         1942         1947        1952          1957         1962         1967

                                          YEAR

    Figure 3 26 Waste to ore ratios for inactive underground uranium mines from 1932 to 1977.
1972
1977
                                                                                                                                  u>
                                                                                                                                   I
                                                                                                                                  to

                                                                                                                                  03

-------
                                                                       3-229
                               4                         4
 ground  mine  produced  3.60 x  10  MT  of ore and  1.44  x  10  MT of waste.   Unfor-
 tunately,  some  of the contemporary  waste  and ore  production has  been  produced
 by ^th active  and inactive  mines.   In  order to adjust  the contemporary ore
 and waste  production  for  that  portion of  the ore  and  wastes generated  by
 active  mining,  we assumed a  model active  mine  having  a  mining life  of  15
 years  (St79). The mid-life of  the mine  was assumed  to have occurred in 1978,
 with production beginning in 1971.
     We also assumed  that some of the mines became  inactive during  the
 1971-1978  period and  that their  numbers decreased linearly.  For example,
 2.44 x  10  MT of ore  was  produced in  1972 and  85.7  percent of that  ore pro-
 duced was  from  mines  that were inactive by 1978.  Therefore, adjusted  ore
 production was  2.09 x 10   MT for 1971.  The ore production for 1973 was  I.IS
 x  106 MT and 1.27 x 106 MT in  1974;  1.06  x 106 MT in  1975; 1.02 x 106  MT in
 1976; and  6.16  x 10   MT in 1977.  The adjusted waste  production was:   5.08  x
 105 MT  in  1972;  6.67  x 105 MT  in 1973;  8.13 x  105 MT  in 1974; 9.43  x 105 MT
 in 1975; 7.43 x  105 MT in 1976;  and 4.99  x 105 MT in  1977.
     Through 1978, the cumulative adjusted ore production from inactive
 underground mines was 6,37 x 10  MT,  and  the cumulative adjusted waste pro-
 duction  was 2.04 x 10 MT.   The model  inactive underground mine was assumed
                           4                         4
 to have  produced  3.14 x 10  MT of ore and 1.00 x  10   MT of waste.  Assuming a
                       3                                                    4
 density  of 2.0 MT per m ,  the  volume  of ore and waste removed were  1.6 x 10
 and 5.Q  x  10  m  ,  respectively.
     Fifty percent of the waste  volume mined we assumed to be sub-ore.   The
 volume  of  waste  rock  (i.e.,  containing no sub-ore)  removed during the  mining
           3  3
 is 2.5 x 10  m  .  Assuming an  entry dimension  of  1.83 m x 2.13 m, about  615 m
 of shafts  and haulways are in  the model mine.  The ore  body we assumed to
 have an  average  thickness  of 1.8 m with a length  and  width of 91.2 m each.
                                                   3  2
 The  surface area  of the passages would be 4.83 x  10   m  .  The surface  area  of
                                          4  2
 the mined-out ore body would be  1.71  x 10  tn .

 3.7.2.1  Haste. Rock Piles
     Wastes produced  from  underground uranium mining were generally cast or
 dumped near the mine  entries.  Those wastes that  were dumped on relatively
 flat terrain formed dome-shaped piles.  Wastes cast from rim mines generally
 formed long,  thin sheets down  the canyon  slopes.  Since most of the inactive
underground mines are in  the Uravan Mineral Belt, the waste pile shape  (dome)

-------
                                                                       3-230
 is  assumed  to be predominant  (see Appendix S.I,2) and  Is used  for the
 calculations of the waste  pile dimensions.
     The waste produced  at a  typical underground mine  consists of waste  rock
 and sub-ore,  The waste  rock  is assumed to be on the bottom of the waste  pile
 since  it was generally removed first.  Sub-ore, which  was removed later,  is
 assumed to  cover or plate  the waste pile.  The waste piles are assumed to  be
 dome shaped, covering a  circular area of 0,40 hectares.  The dome 1s assumed
 to  be  a spherical segment  with a height (b) and base (c) of 71,8 m.  The
                                             3  3
 volume (V)  of the spherical segment, 6,3 n 10  m  when corrected for bulking,
 is  equal to the volume of  wastes and is expressed as
     V =1   trb (3c2 + 4b2).                                           (3.30)
         24
 The surface area of the  spherical segment is given by  the expression
     S • 1   w(4b2 + c2} where  S = Surface area (m2).                   (3.31)
         4
 The term b  is solved by  substitution and iteration in  the former equation and
 is  substituted  in the  latter equation  to determine the surface area  of the
 wastes:
     V - 6.3 x 103 m3 = 1  TT b (15465 + 4b2) where;  b « 3.1 m.          (3.32)
                       24
 The  surface area of the waste pile is
     S = I  7t(4b2 + c2)                                               (3.33)
         4
       - i  (3.14) (38 + 5155)
         4
       • 4.08 x 103 m2.
The thickness (T) of sub-ore on the surface of the waste pile 1s
                                       3  3
          volume of sub-ore  _ 3,2x 10  m
          area of waste pile   4.08 x 103m2
volu-me of sub-ore  _  3.2_x_103J?   =0j8ni,                 (3.34)
     In summary,  the waste  pile  at an inactive underground uranium  mine is
assumed .to have  the  shape of a spherical  segment  with a surface area 4.08 x
  3  2
10  m .  The  pile  is assumed to have  an  inner core of waste rock covered or
plated with  0.78 irTof  sub-ore  on  its  exposed surface.   It  is  expected that
the plate  of  sub-ore  on the waste  pile  would  be  more  pronounced  than the
sub-ore plates  on  overburden piles  at surface  mines because  of  diminished

-------
                                                                      3-231
blending,  mining  practices,  and  the  lower  waste-to-ore ratio.   The  grand
average  of the  radium-226  concentrations in  the  waste  rock' and overburden
piles (Table 3.72) appear to confirm this expectation.
     Table  3.76 lists average  annual  emissions of contaminants  due to wind
erosion  of  the waste rock pile.   These  values  were  estimated by multiplying
an emission factor of 2.12 MT/hectare-yr, derived in Appendix I, by the  waste
pile  surface  area,  0.408  hectares,  and  the  stable  element concentrations
given in Table 3.19.  We assumed uranium and thorium concentrations to be 110
pCi/g and 2 pCi/g, respectively.
Table 3.76  Average annual emissions of radionuclides (uCi)  and stable elements
           (kg) in wind suspended dust at the model  inactive underground mine
Contaminant
Arsenic
r*,
Barium -
Cadmium
Cobalt
Copper
Chromium
Iron
Mercury
Potassium
Magnesium
Manganese ~ -

Waste Rock
Pile(a)
0.07
0.80
ND
0.01
0.05
0.02
14
ND
22
3.0
0.83
--
Contaminant
Molybdenum
Nickel
Lead
Ruthenium
Selenium
Strontium
Vanadium
Zinc
Uranium-238 and
daughter
Thorium-232 and
daughter
Waste Rock
Pile(a)
0.10
0.02
0.07
ND
0.10
0.11
1.2
0.03
each
238
each
1.7
     (b)
     emissions = 8.65 x 10  g/yr.
ND - Not detected.

-------
                                                                       3-232
 3.7.2.2   Radon-222 from the Hlne Area
      We estimated  the total  radon  released from  the model  inactive  under-
 ground  mine from the following parameters:
      1.   Radon exhalation from the  waste rock  pile—
                                                                   3   2
           .  the exposed surface area of  the waste pile = 4.1 x 10  m ,
           .  the average Ra-226 content of  the  waste pile is HO pCi/g;  and
                                                                      2
           .  the radon flux rate for the  waste  pile is 13 pCi  of Rn/m -sec.

 Therefore, the  radon released from the waste pile  is

    4.1  x  103  m2 x 13 pCi  of Rn/m2-sec x 86400 sec/day - 4.6  mCi  of Rn/day.

      2.   Typical  background release rate--
           .   the ground  surface area equivalent to  the area  covered  by
                                      3   2
              the waste pile = 4.1  x  10  m ,  and
           .   the radon flux rate for background soils  in  uranium mining
                                     2
              areas = 0.83  pCi of Rn/m -sec  (Table  3.72),

 Therefore,  the  radon exhalation rate from  an undisturbed area  equivalent  to
 the waste  pile  of  a  model  underground mine  is

   4.1  x  103  m2  x  0.83 pCi  of Rn/m -sec x 86400 sec/day = 0.29 mCi of Rn/day.

 The net radon release rate  due to the waste  pile at the  inactive  underground
 mine  is 4.6  minus 0.29  or about  4.3 mCi  of  Rn/day above normal  background.
      Natural  ventilation will occur  in  most  mines  and usually  is considered
 by  mine ventilation engineers  when  planning  the forced  ventilation systems.
 The natural   force  that can  maintain a  natural air flow due to  temperature
 differences  is   thermal  energy.   The  thermal  energy  added  to a  system  is
 converted  into  a pressure difference.   If  the  pressure difference is suffi-
 cient to overcome  head losses,  a flow of afr will occur.
      Natural  ventilation  depends upon  the difference  between the  temperature
 inside  and  outside .of a mine and  the difference between  the elevation of the
mine  workings and the surface.  Air flow by natural ventilation is generally
                    •j
small  (140 - 566  m /min)   in  shallow mines  (Pe52).   In  deep mines, natural
                                                   •3
ventilation flows  may range from  1,420  to  4,250 m/min  (Pe52).  The flow  1n
either  the  shallow or deep mines depends  upon the depth,  size, and number  of

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                                                                      3-233
openings.   The  intensity of thermal  energy-induced  natural pressure usually
ranges  from a few  hundredths  to  a  few tenths cm of  water in shallow  (less
than 460 m  deep)  mines (Pe52).  The maximum pressure drop  per 305 m of  depth
in deep mines  is  about 2.54 cm  of water in winter and  about  0.84 cm during
the summer  (Pe52).
     In general,  natural  ventilation is subject to considerable fluctuation.
It usually  increases  to a maximum in winter and a minimum  in summer for deep
mines.   The  typical   inactive  underground  uranium  mine  would  be  shallow;
therefore,  the natural  ventilation would be expected to reach its maximum 1n
the winter  and summer"and its minimum in the spring and fall (air temperature
in the mine closfely approaches the outside temperature during the spring and
fall).
     A first approximation  of  the annual release of  Rn-222 from an inactive
underground mine  simply would  ba that all  Rn-222  released  Into the mine air
will   be  exhausted  by natural  vsntilation  before a  significant  radioactive
decay occurs.  That is, the quantity of radon released into the mine is equal
to the  quantity  of  radon released  from the mine.   The quantity  of  Rn-222
released from  the sub-ore  surfaces  remaining  in  the mined-out  ore  body is

                          = A x  *so'                                 (3,35)

                              where A is the surface  area of the mined out
                                              2
                                   ore body (m )
                 sec
                                         = exhalation  rate of  the Rn-222 from
                                      sub-ore per unit  area per unit time,  12
                                      pCi  (Section 3.7.1.2}
                                      2
                                     m -sec
          Q = (1.71 x 104 m2) (12 pCi) = 2.1 x 105 pCi/sec.
                              m -sec
     It  should  be  noted  that <{>   is the  average  radon flux physically mea-
sured  from  sub-ore  bodies  in  inactive  surface  mines  (Section 3.7.1.2). Be-
cause of safety considerations, no measurements were made from sub-ore bodies
in inactive underground mines during the April 1979 field surveys. The annual
Rn-222 source  term  from  the mined-out  ore body  in  an inactive underground
uranium mine, using the preceding assumptions, is

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                                                                       3-234
      Q  (C1)  «  2.1 x  105  pCf x  3.6  x  ID3  sec  x  24 _hr_ x  365 4 x
        yr              sec              hr       d       yr
      1     =  6.6  C1
  1012£Ci      yr  "                                                   (3.36)
       Ci

 The  annual  Rn-222 source  term  (Q) from  the passageways,  assuming an exhalation
 rate  of 8.7 j)Ci_ for overburden,  is  (Section  3.7.1.2)
          m -sec

        (4.8 x 103 m2)  (2.7 x  10"4   CIj  )  = 1.3  Ci.                     (3.37)
                                   yr-m           yr
                                               3
 The  air flow rate from  the mine, assuming 140 m /min for an average shallow
 mine,  will  exchange the mine air every three hours.  The average annual
 radon-222 concentration will be

      7,9 Ci/yr x  	1	  x      1      =  107 pCi/*.
                   7.4 x  107 m3/yr       1000 £/m3

 The  radon daughter concentration will be about 87 percent of equilibrium with
 the  radon,  assuming  a mean residence time of the radon  in the mine to be 1.5
 hours.
      Several inactive mines in the Grants, New Mexico  area were monitored for
 radon  discharges  by  natural   ventilation.   One  of the mines  monitored  was
 relatively  small  and  had  a vertical shaft access.  Five cased 30 cm diameter
 vents  were  found  and  were assumed to be connected  with the mine.  The shaft
 was  covered with  steel  plate, but access holes were cut in the plate and one
 corner had  been pried  up.   Four vents  were capped with  buckets.   Just one
 cover  was  gas tight.   One vent  was partially covered with a  piece  of wood.
 Only  very  small  flow rates due  to  natural   ventilation  were measured  at the
 shaft  and vents.  The maximum radon emission from  the mine per day was esti-
mated  to  be 2.8 x 10  wCi.  This low radon  discharge  rate is probably due to
 partial blockage of  the vents and water in  the mine.  The mine was partially
flooded,  and  flowing  water could  be seen  at  the  bottom  of the  shaft.   The

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                                                                       3-235
 effect of  the  water would be to  partially  or completely close off  the mine
 workings  and substantially reduce  natural  ventilation.   The water would also
 dissolve  and substantially suppress the radon exhaling from the surface areas
 of the mine.   Thus, we believe that  the radon discharges  from wet  inactive
 mines via natural  ventilation will  be  minimal.
      Investigation at another inactive mine  revealed that it was connected to
 three other  inactive mines  that  were subsequently  connected  to  two  active
 mines.  Ventilation  fans  at the  connecting active  mines  were usually  shut
 down after the end  of  the day shift and  on  weekends.  Mine air was exhausted
 by natural ventilation through the  shaft (highest opening) and vents  of the
 mine investigated.  A flow rate up to 88 m  /min was observed coming  from the
 shaft, and radon-222 concentrations reached 11,000 pCi/£.  The average  flow
 rate observed over a weekend  was 75 m  /min,  with an average radon-222 concen-
 tration of 9,800  pCi/2.  The  average radon emission was  1.1 Ci/day.
      Figure 3.27  is  a plot of the  changes in the  Rn-222  concentration  in the
 air from   the shaft  of the  inactive mine  investigated.   The average  of the
                                                                  3
 measurements  of the  air  flow rate from  the  shaft was about 76 m /min.   The
 Rn-222 concentration increased almost  linearly with  time for about  20  hours
 after the fans  were  shut  down at  the  end of the day shift on April 27,  1979.
 The Rn-222 concentrations  also leveled  off at about'10,000 pCi/n .   A  dip,
 presumed  to have  been caused by high  winds,  occurred in the Rn-222 concen-
 tration curve from  about 1000 to 1600  hours  on April  28,  1979.
      Since the  curve is relatively  flat  at  10,000 pCi/a.  it is assumed  that
 the rate  of production of the  Rn-222  is  equal to  the rate  of removal  of the
 Rn-222 from the six  mines.   The  average residence  time  of the radon  in  the
 mine  air   is  assumed to be  approximately 10  hours,  and  the radon daughters
 would  be  in near-equilibrium  (assumed  to  be =  90 percent).   Assuming  that all
 six interconnecting mines contributed  equally to  the source term measured,
 the release rate of  Rn-222 for a single mine  will  be
      10,000 pCi/£ x  76,000 £/min x  1440 min/day x  10"12Ci/pCi * 6
     = 0.18 Ci/day.

     Based  on the  preceding  estimation of Rn-222 and  progeny released  from a
 typical mine  on the  Colorado plateau  and physical  measurements at six  con-
 nected mines, the  annual  radon release rate may  range from 7.9 to 66 Ci/yr.
These source term estimates,  of course, are  based on a single mine. Many  mine
workings  are, in  fact, interconnected.   If  these  interconnected workings  are
assumed to constitute  a   single  mine,  then  the  upper  limit  of  Rn-222  and

-------
                   Ventilation

                 Fans Operating
                                                     Ventilation

                                                 Fans Nol Operating
o
a.
c
v
u
c
o
o

(N
!M
r-l

c
O
•
    14000
    12000
    10000
     8000
6000
     4000
     2000
          ftpr.127 197£
                                         28.1979
                           April 23,1979
                                 April 30.1979
         o
         o
                    o
                    o
                    o
                          o
                          o
o
o
o
o
w   T,me
o
o
N
O
o
o
ts!
O
o
O
o
CD
O
O
o
          Figure 3 27 Radon-222 concentrations in mine air discharged by natural ventilation.
                                                                                                                            I
                                                                                                                           K3

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                                                                       3-237
 progeny discharge  known at  this  time  will  be about  10,000 pCi/£  with  an
 annual  Rn-222 source term of about 400 Ci/yr.  For example, 67 percent  of all
 inactive  underground uranium mines are in or near the Uravan mineral  belt and
 are probably dry.   Their aggregate Rn-222 discharge by natural  ventilation is
 estimated  to be
       1360 mines x 66 Ci Rn-222 =  9.0 x 104 Ci/yr.
                          yr-mine

      In summary,  there  is little  information available on  the discharge  of
 Rn-222  and its  progeny  from  the vents and entries  of  inactive  uranium mines
 by natural  ventilation.   Some  physical  measurements indicate  that  the  dis-
 charges may  be  substantial.   It  is  known,  through  surveys  conducted  to
 support this study,  that a  large  majority of  the  inactive  uranium mines are
 not isolated from the atmosphere  and are capable  of discharging their  Rn-222
 and progeny  into  the local  environment.  It  is  also known that some  self-
 sealing will  probably occur  at  some  of the mines,  due  to flooding, cave-ins,
 and  subsidence.  Table  3.77  summarizes estimates  of  the  annual  radon-222
 releases  from inactive  underground uranium mines.   This potential  source  of
 exposure  could  be  practically eliminated  by proper sealing of the  inactive
 mines.

 3.7.2.3 Land Surface Gamma  Radiation
      Gamma  radiation  surveys  were conducted  around underground mining  areas
 in  Colorado and New  Mexico.   Table  3.78 lists the  ranges  of gamma radiation
 exposure  rates  measured  at some  of  the mines.   The elevated  gamma  ray ex-
 posure  rates on  the  waste piles  are due  primarily  to plating  those piles  with
 sub-ore removed  during the mining  process.
      Some radioactive materials  originating from ore and sub-ore handling can
 be  lost into the local  environment around a  mine site.  Erosion of  the  mine
 wastes  can  also  disperse contaminants  into  the  local  environment. Figure  3.28
 illustrates  gross  gamma  radiation exposure  rate  measurements  around an in-
 active  underground uranium mine  in New Mexico.  Background gamma-ray exposure
 rate  measurements made  around  the   mine area ranged  from 12  to  15 yR/hr.
 According to  the measurements made,  exposure rate levels exceeded background
 from 50 to more  than  100 meters  from  the  waste  piles.  The area  that has  been
contaminated  far exceeds  the  area   physically disturbed  at the mine  site.
Gross gamma exposure rates  measured on  the  waste  piles  averaged about 95

-------
                                                                       3-238
 Table 3.77   Summary of radon-222 releases from inactive underground mines
 Sou rce
   Estimation Methods
Annual Release, Ci
 Model  Mine

   Waste Rock Piles


   Underground workings


     Sub-o<"? Surfaces

     Passageways
Background
Model Mine
Actual Mine
  Underground workings
    (dry)
  Underground workings
   (wet)

Waste rock piles
 Calculated  volume  &  surface
   area;  limited  field measure-
   ments  of  radon flux
 Radon  release  based  on  natural
   ventilation  rate for  shallow
   mines
 Calculated  surface area; limited
   radon  flux measurements of sub-ore
 Calculated  passageway surface
   area;  limited  measurements of
   radon  flux from  overburden

 Field measurements of radon flux;
   and projected  area of waste
   rock pile

 Total ridon .source minus back-
   ground
Field measurements

Field measurements

Calculated volume & surface area;
Limited field measurements of
  radon flux
      1.7
      6.6
                                                                  1.3
      0.11
                                                                 9.5
    66

     1.1
                                                                 1.7

-------
                                                                      3-239
Table 3.78
Summary of land surface       radiation surveys In
Colorado and New Mexico
Location
          Area
   Gamma Radiation
Exposure Rate (v R/hr)
Boulder, Colorado
Uravan, Colorado

San Mateo, New Mexico
Mesa Top Mines,
New Mexico
     Waste piles
     Waste piles

     Waste pile
     Ore
     Overburden
     Background

     Waste piles
   40 to 100
   50 to 220

   35 to 275
  100 to 350
   20 to 120
   10 to 13

   25 to 290
Barbara J II Mine,
New Mexico
     Waste piles
     Background
   21  to  170
   12  to  15
Source:  Wo79,

-------
                               Vent
                        .Vent
                               21
                    17
     0    25    SO    75   100

            METERS

GROSS GAMMA RAY EXPOSURE RATE
                                        18
                                              I23
                                         14    *20
                                                                 12
     Vent \k
• 16     *^
     Figure 3.28 Gamma radiation survey around an inactive underground uranium mine in New Mexico,
                                                                               I
                                                                               N
                                         I
                                         to
                                                                                        O

-------
                                                                       3-241
yR/hr, which would make them unsuitable for unrestricted use.
     In  summary,  wastes   from  underground  uranium mining   technologically
enhance  natural  radioactivity  and may -be considered  low-level  radioactive
wastes.  Improperly  controlled  wastes  will be dispersed into  the surrounding
environment by the mining activities and erosion.

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                                                                      3-242

 3.8   References
 AEC73    U.S. Atomic  Energy Commission, 1973, "Final Environmental Statement
   Related to Operation of  the Highland Uranium Mill by the Exxon Company,
   U.S.A.", Docket No.  40-8102.

 AEC74    U.S. Atomic  Energy Commission, Directorate of Licensing, Fuels and
   Materials, 1974, "Environmental Survey of the Uranium Fuel Cycle,"
   WASH-1248.

 Am78      Ames,  L.L. and Rai, D., 1978, "Radionuclide Interactions with Soil
   and Rock Media,"  U.S. Environmental Protection Agency, EPA 520/6-78-007.

 An73      Andelman, J. B., 1973, "Incidence, Variability and Controlling
   Factors for Trace Elements in Natural, Fresh Waters," i_n Trace Metals and
   Metal-Organic  Interactions in Natural Waters (Philip C.  Singer, Ed), Ann
   Arbor Science  Publishers Inc., Ann Arbor, Michigan.

 Anon69    Anonymous, 1969, "Acid Mine Drainage in Appalachia,"  Howe Document No.
   91-180, 91st Congress, 1st Session, Committee on Public Works, Washington, D.C.

 Anon79    Anonymous, 1979, "Uranium Exploration Damages Groundwater," Water
   Well Journal, July,  p. 15.

 Au78      Austin, S.R. and Droullard, R.F., 1978, "Radon Emanation from Do-
   mestic Uranium Ores  Determined by Modifications of the Closed-Can,  Gamma-
   only Assay Method,"  Department of Interior,  Bureau of Mines Report of
   Investigations 8264.

Be68      Beck, H.  and de Planque, G., 1968,  "The Radiation Field in Air
  Due to Distributed Gamma-Ray Sources in the  Ground,"  U.S.  Atomic Energy
  Commission Report,  HASL-195.

Be75      Bernhardt,  D.E.j Johns, F.B.  and Kaufmann, R.F.,  1975, "Radon Ex-
  halation from Uranium Mill Tailings Piles,"  U.S.  Environmental Protection
  Agency,  Technical  Note ORP/LV-75-7(A).

-------
                                                                      3-243

 Bo70      Borland, J.P., September 1970, "A Proposed Streamflow - Data Pro-
   gram for New Mexico," U.S.  Geological Survey, Water Resources, Open file
   report, Albuquerque, Mew Mexico.

 Ca57      Cannon, H.L., 1957, "Description of Indicator Plants and Methods of
   Geobotanical Prospecting for Uranium Deposits on the Colorado Plateau,"  U.S.
   Geological Survey Bulletin  1Q3Q-M,  pp.  399-516.

 Ca64      Cannon, H.L,, 1964, "Geochemistry of Rocks and Related Soils  and
   Vegetation in the Yellow Cat Area,  Grand County, Utah,"  U.S.  Geological
   Survey Bulletin 1176.

 Ch54      Chariot, G., 1954,  "Qualitative Inorganic Analyses,"  Translated  by
   R.C.  Murray, Wiley Publishers,  New  York,  p.  354.

 C166      Clark,  S.  P.,  Peterman,  Z.E.  and Heier,  K.S.,  1966,  "Abundance of
   Uranium," Thorium and Potassium,"  Handbook of Physical  Constants  (Revised
   Edition),  Geological Society of  America,  Inc., New York,  NY,  pp.  821-541.

 C174      Clark,  D,  A,,  1974,  "State-of-the-Art, Uranium Hining,  Milling,  and
   Refining Industry,"  U.S.  Environmental  Protection Agency,  National  Environ-
   mental  Research Center,  Corvallis,  Oregon.

 Co77      Cook,  L.  M., Caskey,  B.W. and Wukasch, M.C., 1977, "The Effects  of
   Uranium Mining  on Environmental Gamma Ray  Exposures" in Proceedings IRPA
   IV International  Congress,  Paris, April  24 -  30,  pp. 1029-1032.

 Co78      Cook,  L.M.,  1978, "The Uranium  District  of  the Texas Gulf Coastal
   Plain,11  Texas Department  of  Health  Resources, Austin,  Texas.

 Co68      Cooper,  J.B.  and  John, E.C.,  1968, "Geology and Groundwater
   Occurrence  in Southeastern HcKinley County, New Mexico,"   New Mexico
   State Engineer,  Technical Report 35,  prepared in  cooperation with the
   U.S. Geological  Survey.

Cr78      Craig, G.S.  and Rankl, J.G.,  1978, "Analysis of Runoff  from Small
  Drainage Basins  in Wyoming,"  USGS Water Supply  Paper  2056.

-------
                                                                      3-244
Da79      Dale, J.T., 1979, Air Program Branch, U.S. Environmental Protection
  Agency, Region VIII, Denver, CO., Memo concerning Uranium Resources Develop-
  ment Company's Mining Operation in San Juan County, Utah - PDS Permit
  Requirements.

Da75      Dames and Moore, 1975, "Environmental Report, Bear Creek Project,
  Converse County, Wyoming," for the Rocky Mountain Energy Company.

DQA75     U.S. Department of Agriculture, Soil Conservation Service, 1975,
  "Surface Water Hydrology for the Tennessee Valley Authority on the
  Morton Ranch Lease," U.S. SCS, Casper, Wyoming.

DOA78     U.S. Department of Agriculture, Forest Service, Rocky Mountain
  Region, 1978, "Dr<*ft Environmental Statement for Homestake Mining CoiKiany's
  Pitch Project".

DOE79     U.S. Department of Energy, 1979, "Statistical Data of the Uranium
  Industry," GJQ-1QO(79).

00132-42  Department of Interior, U.S.  Bureau of Mines, 1932-1942,  "Minerals
  Yearbooks".

D0159     U.S. Department of Interior,  U.S.  Geological  Survey,  1959,
  "Compilation of Records of Surface Waters of the United States through
  September 1950, Part 6-A, Missouri River Basin above  Sioux City,  Iowa,"
  USGS Water Supply Paper 1309.

DOI59-76  Department of Interior, U.S.  Bureau of Mines, 1959-1976,  "Minerals
  Yearbooks",

DOI64     U.S. Department of Interior,  U.S.  Geological  Survey,  1964,  "Compi-
  lation of Records of Surface Waters of the United States,  October 1950 to
  September 1960,  Part 6-A, Missouri River Basin Above  Sioux City,  Iowa,"
  USGS Water Supply Paper 1729.

-------
                                                                       3-24-5
 DOI67      U.S. Department of  Interior,  Bureau  of Mines,  1967,  "Surface
   Mining  and  Our  Environment,"  Prepared by  the Strip  and Surface Mining
   Study Commission, Bureau of Mines.

 00169      U.S. Department of  Interior,  U.S. Geological Survey, 1969, "Surface
   Water Supply of the United  States  1961-1965,  Part 6, Missouri River  Basin,
   Volume  2, Missouri River Basin  from Willisten, North Dakota  to Sioux City,
   Iowa,"   USGS Water Supply Paper 1917.

 DOI73      U.S. Department of  Interior,  U.S. Geological Survey, 1973, "Surface
   Water Supply of the United  States  1966-1970,  Part 6, Missouri River  Basin,
   Volume  2, Missouri River Basin  from Williston, North Dakota  to Sioux City,
   Iowa,"   USGS Water Supply Paper 2117.

 DOI79      U.S. Department of  the  Interior,  1979, "Uranium Development  in the
   San Juan Basin  Region - Draft,"  San  Juan Basin Regional Uranium Study,
   Albuquerque, New Mexico.

 Dr79       Oreesen, O.K., 1979, "Final Report,  Investigation of Environmental
   Contamination,  Canon City,  Colorado,"   Los Alamos Scientific Labs.

 Du63       Durum, W.  H., and Haffty, J., 1963, "Implications of the Minor Element
   Content  of some Major Streams of the World,"  Geochim.   Cosmochim.  Acta 27:1,

 Ea79       Eadie, G.  G,, Fort, C. W. and Beard, M.  L.,  1979S "Ambient Airborne
   Radioactivity Measurements  in the Vicinity of the Jackpile Open Pit Uranium
  Mine, New Mexico,"  U.S. Environmental Protection Agency Report,  ORP/LV-79-2.

EPA72     U.S. Environmental  Protection Agency, 1972,  "Impact of the Schwartz-
  walder Mine on the Water Quality of Ralston Creek,  Ralston Reservoir, and
  Upper Long Lake,"  Technical  Investigations Branch,  Surveillance and Analysis
  Division, U.S.  EPA,  Region VIII.

EPA75     U.S. Environmental  Protection Agency, 1975,  "Water Quality Impacts of
  Uranium  Mining and Milling Activities in the Grants  Mineral  Belt, New
  Mexico," U.S.  EPA  906/9-75-002,  Region VI, Dallas, Texas.

-------
                                                                      3-246
EPA76     U.S. Environmental  Protection Agency, Office of Water Supply, 1976,
  "National Interim Primary Drinking Water Regulations," U.S. Environmental
  Protection Agency Report, EPA-570/9-76-003.

EPA77a    U.S. Environmental  Protection Agency, 1977,  "Water Quality Manage-
  ment Guidance for Mine-Related Pollution Sources (New, Current, and Aban-"
  doned), U.S. EPA-44Q/3-77-Q27, Office of Water Planning and Standards,
  Water Planning Division, Washington, D.C.

EPA77b    U.S. Environmental  Protection Agency, Office of Air and Waste Man-
  agement, Office of Air Quality Planning and Standards, 1977, "Compilation
  of Air Pollutant Emission Factors," Third Edition.

Fe31      Fenneman, N.H,, 1931, "Physiography of Western United States," N~>*
  York, McGraw Hill, 534 p.

FBD77-78  Ford, Bacon and Davis Utah Inc., 1977-78, series of reports to the
  U.S. EROA, Grand Junction Office on the "Phase II - Title I Engineering
  Assessment of Inactive Uranium Mill Tailings".

Fu73      Fulkerson, W. and Goeller, H.E. (Editors), 1973, "Cadmium, The
  Dissipated Element," Oak Ridge Natl. Lab - National Science Foundation
  Environmental Program, QRNL-NSF-EP-21, ORNL, Oak Ridge, Tennessee.

Fu77      Fuller, W. H., 1977, "Movement of Selected Metals, Asbestos, and
  Cyanide in Soil:  Applications to Waste Disposal Problems," U.S.  Environ-
  mental, Protection Agency Report, EPA 600/2-77-020.

Fu78      Fuller, W. H, , 1978, "Investigation of Landfill Leachate Pollutant
  Attenuation by Soils," U.S.  Environmental Protection Agency Report,
  EPA 600/2-78-158.

Ga77a     Gableman, J~,W, , 1977, "Migration of Uranium and Thorium - Exploration
  Significance,*1 Series in Geology No.  3, American Association of Petroleum
  Geologists,  Tulsa, Oklahoma.

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                                                                      3-?47

Ga?7b   Gabin, V.L. and  Lesperance, I.E., 1977, "New Mexico Climatological
  Data; Precipitation, Temperature, Evaporation, and Wind, Monthly and Annual
  Means,  1950-1975," W.K. Summers and Associates, Socorro, New Mexico.

6e77      Gesell, T, F.  and Cook, L.M,, 1977, "Environmental Radioactivity in
  the South Texas, USA Uranium District," in International Symposium on Areas
  of High Natural Radioactivity, Pocos de Caldas, Brazil, June 16-20, 1975.

Go61      Gordon, E". D,, 1961, "Geology and Groundwater Resources of the Grants-
  Bluewater Area, Valencia County, New Mexico," New Mexico State Engineer,
  Technical Report 20, prepared in cooperation with the U.S. Geological Survey.

tV67      Gregors-Hansen, Birte, 1967, "Application of Radicactivation Analysis
  for the Determination  of Selenium and Cobalt in Soils and Plants," Transactions,
  8th International Congress of Soil Scientists, Bucharest, Volume 3, 63-70.

Ha68      Havlik, B., Grafova, J., and Nycova, B., 1968, "Radium-226 Liberation
  from Uranium Ore Processing Mill Waste Solids and Uranium Rocks into Surface
  Streams - I, The Effect of Different pH of Surface Waters," Health Physics,
  Volume  14, 417-422.

Ha78   •   Harp, D. L., 1978, "Historical Examination of Water Quality Impact
  from the Shirley Basin Uranium Operation," Wyoming Department of Environmental
  Quality, Cheyenne, Wyoming,

Ha61      Hartraan, H., 1961, "Mine Ventilation and Air Conditioning," The
  Ronald Press Co., New York.

He60      Hem, J.D., 1960, "Some Chemical Relationships Among Sulfur Species
  and Dissolved Ferrous Iron,"  U.S.  Geological  Survey, Water Supply Paper
  1459-C,  pp.  57-73.

He69      Heier,  K.  S.  and Billings,  G.  K-,  1969,  "Potassium,"  Handbook of
  Geochemistry, Springer-Verlog,  Berlin, Chapter 19.

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                                                                      3-248
He78      Hendricks, 0. W., 1978, Director, U.S.  EPA Office of Radiation
  Programs, Las Vegas, written communication (Review of Cotter Uranium Mill
  Reports), to Paul B. Smith, Regional Representative, Radiation programs,
  U.S. EPA, Denver, June 1978.

He79      Henry, C. D., 1979, "Trace and Potentially Toxic Elements Associ-
  ated with Uranium Deposits in South Texas  (draft)," Bureau of Economic
  Geology, University of Texas at Austin.

Hi68      Hill, R.  D,, 1968, "Mine Drainage Treatment, State of the Art and Re-
  search Needs," U.S. Department of the Interior, Federal  Water Pollution
  Control Administration.

Hi69      Hilpert,  L.S., 1369, "Uranium Resources of Northwestern New Mexico,'*
  U.S. Geological  Survey Report, Geological Survey Professional Paper 603.

Hi73      Hill, R.  0., 1973, "Water Pollution from Coal  Mines,"  Proceedings,
  45th Annual  Conference,  Water Pollution Control Association of Pennsylvania,
  University Park,  Pennsylvania.

Hi77      Hiss, W,  I,, 1977, "Uranium Mine Waste  Water - a Potential Source of
  Groundwater in Northwestern New Mexico,"  U.S.  Geological  Survey open file
  report 77-625, 10 p.

Ho72      Howard,  J.  H., 1972, "Control  of Geochemical Behavior of Selenium in
  Natural Waters by Adsorption on Hydrous  Ferric  Oxides,"  jji Trace Substances
  in Environmental  Health  (Hemphill,  D.D. , Editor),  5th Annual  Conference,
  June 29 - July 1, 1971,  University of Missouri-Columbia, Columbia, Missouri,
  (pp. 485-495) 559 p.

Ho73     -Hodson,  W.  G., Pearl,  R.  H.  and  Druse,  S.  A.,  1973,  "Water Resources
  of the Powder River Basin and Adjacent Areas, Northeast  Wyoming," USGS Hydro-
  logic Investigations' Atlas HA-465.

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                                                                      3-249

 Hu76       Hubbard,  S.  J.,  1976,   "Evaluation  of Fugitive  Dust  Emissions  from
   Mining:   Task 1  Report -  Identification of  Fugitive  Dust  Sources Associated
   with  Mining," Report Prepared  by  PEDCo  -  Environmental  Specialists, Inc.,
   for U.S.  Environmental Protection Agency, Contract No.  68-02-1321, Task  36.

 ICRP64     International Commission  on  Radiological Protection, 1964, "Recom-
   mendations  of the ICRP (as amended 1959 and revised  1962},"  ICRP Publication
   6, Pergamon Press,  London.

 ICRP66     International Commission  on  Radiological Protection, Committee II
   Report,  1966, "Deposition and  Retention Models  for Internal  Oosiroetry of
   the Human Respiratory Tract,"  Health Physics  12, 173.

 It75       Itln, S.C.,  1975, "The Public Health  Significance of Abandoned
   Open  pit Uranium  Mines in South Texas," Master's Thesis, University of Texas
   (unpublished).

 Ja79a      Jackson,  B,, Coleman,  W.,  Murray, C., and Scinto, L., February 1979,
   "Environmental Study on Uranium Mills,  Part 1,  Final Report,"  Thompson,
   Woodridge,  and Ramo, Inc., Prepared  for U.S.  Environmental Protection
   Agency,   Effluent Guidelines Division,  Washington, D.C., Contract No.  68-
   03-256Q.

 Ja79b      Jackson,  P. 0., et.  a!.,  1979,  "Radon-222 Emissions  in Ventilation
   Air Exhausted from Underground Uranium  Mines,"  Battelle Pacific Northwest
   Laboratory  Report, PNL-2888 Rev.,  NUREG/CR-0627,

 Je68       Jenne, E. A., 1968,  "Controls on Mn, Fe, Co, Ni, Cu,  and Zn Con-
   centrations  in Soils and Water; the  Significant Role of Hydrous Mn and Fe
  Oxides,"  i_n  Trace Inorganics in Water,  A symposium by the Division of Water,
  Air, and Waste Chemistry at the 153rd Meeting of the ACS,  Miami Beach,  Florida,
  April  1967,  Advances in Chemistry  Series No. 73, ACS.

Jo63      John, E.  C. and West, S.W.,  1963, "Groundwater in the Grants  District,"
  New Mexico State Bureau of Mines and Mineral Resources Memoir 15.

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                                                                      3-250
Ka75      Kallus, M.F., 1975, "Environmental Aspects of Uranium Mining
  and Milling in South Texas", U.S.  Environmental Protection Agency Report,
  EPA-906/9-75-004.

Ka?6      Kallus, M.F., 1976, "Environmental Impacts of Uranium Mining in South
  Texas," in Geology of Alternate Energy Resources in the South-Central United
  States (M.O. Campbell, Editor) Houston Geological Society, 1977.

Ka77      Kaufmann., R. F. and Bliss, J. D., 1977, "Effects of Phosphate Mineral-
  ization and the Phosphate Industry on Radium-226 in Groundwater of Central
  Florida," U.S. Environmental Protection Agency, Office of Radiation Programs
  Report, EPA/520-6-77-010,

Ka?8a     Kaufmann, R. F., 1978, U.S. EPA Office of Radiation Programs, Las
  Vegas, written communication (Review of October 1977 Environmental Re-
  port on Split Rock Mill, Jeffrey City, Wy) to Paul  B.  Smith,  Regional
  Representative, Radiation Programs, U.S. EPA, Denver,  January 1978.

Ka78b     Rasper, D., Martin, H. and Munsey, L.» 1978, "Environmental  Assess-
  ment of In Situ Mining," Report prepared by PRC Toups  Corp.  for the U.S.
  Department of the Interior, Bureau of Mines,  Contract  No.  JQ265Q22.

Ka79      Kaufmann, R, F., 1979, U.S. EPA Office of Radiation Programs, Las
  Vegas, written communication (Review of Dawn Mining Company Tailings
  Disposal  Activities), to Edward Cowan, Regional Radiation Representative,
  U.S.  EPA Region X, November 1979.

Kab79     Kaback, D. S.» 1979, "The Effect of Uranium Mining and Milling on the
  Incidence of Molybdenosis in Cattle of South Texas  (abs.)" jm Abstracts
  with Programs, 1979 annual meeting, Geological  Society of America, Volume 11,
  Number 7,  August 1979.  GAAPBC 11(7) 313-560.

Ke76      Reefer, W. Rfand Hadley,  R.  F., 1976,  "Land and Natural Resource
  Information and Some Potential Environmental  Effects of Surface Mining of
  Coal  in the Gillette Area, Wyoming,"  U.S.  Geological Survey Circular 743.

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                                                                       3-251
Ke77      Kerr-McGee Nuclear Corporation, 1977, "Environmental Report, South
  Powder River Basin Mill, Converse County, Wyoming",

Ki67      Kittle, D.F., Kelley, V.C. and Melancon, P.E., 1967, "Uranium
  Deposits of the Grants Region," _in New Mexico Geological Society Eighteenth
  Field Conference, Guidebook of the Defiance - Zuni - Mt. Taylor Region of
  Arizona and New Mexico, pp. 173-183.

K178      Klute, A. and Heerman, D. F., 1978, "Water Movement in Uranium Mill
  Tailings Profiles," U.S. Environmental Protection Agency, Technical Note
  ORP/LV-78-8,

Ku79      Kunkler, J.L.» 1979, "Impacts of the Uranium Industry on Water
  Quality," Working Paper No. 22, San Juan Basin Regional Ur^ium Study,
  U.S. Department of Interior, Albuquerque, New Mexico.

La72      Lakin, H. W., 1972, "Selenium Accumulation in Soils and Its Absorp-
  tion by Plants and Animals," Geological Society of America Bulletin, Vol.
  83, pp. 181-190.

La78      Larson, W.C., 1978, "Uranium In Situ Leach Mining in the United
  States," U.S. Department of the Interior, Bureau of Mines Information
  Circular 8777.

La79      Lappenbusch, W.  1979, U.S. EPA Office of Drinking Water, Washington,
  0. C. , written communication to Dr.  Frank Traylor,  State of C.olorado, Depart-
  ment of Health, Denver,  July 6, 1979.

Lo64      Lowder, W.M., Condon,  W.J.  and Beck, H.L., 1964, "Field Spectro-
  metric Investigations of Environmental Radiation in the U.S.A.," j_n the
  Natural  Radiation Environment,  University of Chicago Press, Chicago, IL,
  pp.  597-616.

Lo76      Lowham, H.W.,  1976, "Techniques for Estimating Flow Characteristics
  of Wyoming Streams," USGS Water Resources Investigation No. 76-112.

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                                                                      3-252
Ly78      Lyford, F. P. and Frenzel, P.P., 1978, "Ground Water in the San Juan
  Basin, New Mexico and Colorado:   The Existing Environment," San Juan Basin
  Regional Uranium Study, Albuquerque, New Mexico, Working Paper No. 23.

Ly79      Lyford, F. P. and Frenzel, P. F., 1979, "Modeled effects of uranium
  mine dewatering on water resources in Northwestern New Mexico," San Juan
  Basin Regional Uranium Study, Albuquerque, New Mexico, Working Paper No. 37.

Ma69      Masuda, K. , Yamamoto, T., and Kitamura, N., 1969, "Studies on
  Environmental Contamination by Uranium, 4.  Some Aspects on the Eliminating
  Factor of Uranium in Streams," Report Summaries of 12th annual  meeting of
  the Japan Radiation Research Society, 442.

Mi76      Miller, H. T. , 1976, "Radiation Exposures Associated with Surface
  Mining for Uranium," 21st Annual Meeting of the Health Physics  Society,
  San Francisco, California.

Mo74      Moran, R.  E. and Wentz, D. A.,  1974, "Effects of Metal-Mine Drainage
  on Water Quality in Selected Areas of Colorado, 1972-73," U.S.  Geological
  Survey in Cooperation with the Colorado Water Pollution Control Commission,
  Colorado Water Conservation Board, Denver, Colorado.

NAS72     Natiortal Academy of Sciences -  National Academy of Engineering, 1972,
  "Water Quality Criteria 1972," Ecological  Research Series,  EPA-R3-73-033.

NAS79     National Academy of Science,  1979,  "Continuation Report of Drinking
  Water and Health - Draft,"  Report to Office of Drinking Water,  Safe Drinking
  Water Committee, U.S. EPA,  421 p.

NCRP75    National Council  on Radiation Protection  and  Measurements,  1975,
  "Natural  Background Radiation in the  United States,"  NCRP Report No,  45.

NM79      New Mexico Energy Resources  Board,  1979,  "The Uranium Industry in
  New Mexico -   Its  Demands on State Resources," Draft.

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                                                                       3-253
Ni76       Nichols, H.  L., 1976,  "Moving the  Earth," third edition, North
  Castle  Books, Greenwich, Connecticut.

Ni79       Nielson, K.  K., Perkins, R. W., Schwendiman, L.C. and Enderlin, W. I.,
  1979, "Prediction  of the Net Radon Emission from a Model Open Pit Uranium
  Mine,"   Battelle Pacific Northwest Laboratory Report, PNL-2889 Rev.,
  NUREG/CR-0628,

NRC76      U.S. Nuclear Regulatory Commission, Office of Nuclear Material
  Safety  and  Safeguards, 1976, "Final Generic Environmental Statement  on
  the Use of  Recycle Plutonium in Mixed Oxide Fuel in Light Water Cooled
  Reactors,"  NUREG-0002, Vol. 3.

NRC77a     U S. Nuclear Regulatory Commission, Office of Nuclear Material Safety
  and Safeguards, 1977, "Draft Environmental Statement Related to Operation of
  Sweetwater  Uranium Project," NUREG-Q4Q3, Docket No. 40-8584.

NRC77b     U.S. Nuclear Regulatory Commission, Office of Nuclear Material Safety
  and Safeguards, 1977, "Final Environmental Statement Related to Operation of
  Bear Creek  Project," NUREG-0129, Docket No. 40-8452.

NRC78a     U.S. Nuclear Regulatory Commission, Office of Nuclear Material Safety
  and Safeguards, 1978, "Draft Environmental Statement Related to Operation of
  White Mesa  Uranium Project," Docket No. 40-8681, NUREG-0494.

NRC785     U.S. Nuclear Regulatory Commission, Office of Nuclear Material Safety
  and Safeguards, 1978, "Draft Environmental Statement Related to Operation of
  Highland Uranium Solution Mining Project,"  Docket No.  40-8102,  NUREG-0407.

NRC78c     U.S. Nuclear Regulatory Commission, 1978,  "Draft Environmental
  Statement Related  to Operation of the Morton Ranch Uranium Mill,  United
  Nuclear Corporation," NUREG-0439.

NRC78d    U.S. Nuclear Regulatory Commission, 1978,  "Final Environment^
  Statement - Highland Uranium Solution Mining Project,"  NUREG-0489.

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                                                                      3-254
 NRC79a     Nuclear  Regulatory  Commission, Office  of Nuclear Material  Safety
  and Safeguards,  1979} "Draft Environmental  Statement on the Shootering
  Canyon Uranium Project  (Garfield County, Utah)," NUREG-0504.

 NRC79b     U.S. Nuclear Regulatory Commission, 1979, "Draft Generic Environ-
  mental Impact Statement on  Uranium Milling," Volume I, Appendices, NUREG-
  0511,

 Qa72       Oakley,  D, T., 1972, "Natural Radiation Exposure in the United
  States,"  U. S.  Environmental Protection Agency Report, ORP/SIO 72-1.

 Pa?3       Page, A.  L. and Bingham, F, T., 1973,  "Cadmium Residues in the
  Environment" jm  Residue Reviews, Vol. 48, Francis A. Gunther (Ed.),
  Springer-Verlag  Publishers.

 Pa74       Paone, J., Morning, J.  and Giorgetti,  L., 1974, "Land Utilization
  and Reclamation  in the Mining Industry, 1930-71,"  U.S. Bureau of Mines
  Information Circular 8642.

 Pe52      Peele, R., 1952, "Mining Engineers Handbook,"  John Wiley and Sons,
  Inc., London,

 Pe79      Perkins, B, L., 1979, "An Overview of the New Mexico Uranium Indus-
  try," New Mexico Energy and Minerals Department Report, Santa Fe, New
  Mexico.

 Ph64      Phair, G. and Gottfried, D., 1964,  "The Colorado Front Range, Colo-
  rado,  U.S.A. as a Uranium and Thorium Province," i_n the Natural Radiation
  Environment, University of Chicago Press, Chicago,  IL, pp.  7-38*

Ra78      Rachal, E. A,,  1978, "Survey of Fugitive Dust from Coal Mines,"
  U.S.  Environmental Protection Agency Report, EPA-9Q8/1-78-QQ3.

Ra77      Rankl,  J.G. and Barker,  O.S., 1977,  "Rainfall  and Runoff Data from
  Small  Basins in Wyoming,"  Wyoming Water Planning Program/USGS Report No. 17.

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                                                                       3-255
Re76      Reed, A. K., Meeks, H.C., Pomeroy, S.E. and Hale, V.Q.,  1976,
  "Assessment of  Environmental Aspects of Uranium Mining and Milling," U.S.
  Environmental Protection Agency Report, EPA-600/7-76-036.

Ri78      Ridgley, J., Green, M., Pierson, C., Finch, W. and Lupe,  R. ,  1978,
  "San Juan Basin Regional Uranium Study, Working Paper No. 8, Summary of the
  Geology and Resources of Uranium in the San Juan Basin and Adjacent Region,
  New Mexico, Arizona, Utah and  Colorado,"  U.S. Department of the Interior,
  U.S. Geology Survey Report.

Ro64      Roserifeld,  I. and Beath, D.A. , 1964, "Selenium: Geobotany, Bio-
  chemistry, Toxicity, and Nutrition,"  Academic Press PublisherSj New York.

Ro78      Rogo^ski, A.S., 1978,  "Water Regime in Strip Mine Spoil," i_n Sur-
  face Mining and Fish/Wildlife  Needs in the Eastern United States, Proc. of
  a Symposium, Eds. 0. E. Samuel, J.  R.- Stauffer and W. T.  Mason, U.S. De-
  partment of the Interior, Fish and Wildlife Service, FWS/OBS-78/81, 137.

Ru58      Rushing, D.E., 1958, Unpublished Memorandum, U.S. Public Health
  Service, Salt Lake City, Utah.

Ru76 '     Runnels, D. D., 1976,  "Wastewaters in the Vadosa Zone of Arid  Re-
  gions:   Geochemical Interactions," Proc.  3rd National Ground Water Quality
  Symposium, Las Vegas, Nevada,  Sept.  15-17, 1976, Ground Water 14, No.  6,
  374.

Sc74      Schaiger, K. J., 1974, "Analysis of Radiation Exposures on or  Near
  Uranium Mill Tailings Piles,"  U.S.  Environmental  Protection Agency,
  Radiation Data Repts.  15, 441-425.

Sc79      Schwendiman, L.  C., Battelle Pacific Northwest Laboratories, 1979,
  a letter to Harry Landon, Office of Nuclear Regulatory Research, U.S.
  Nuclear Regulatory Commission.

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                                                                     3-256

Se75      Sears, M. B., Blanco,  R.  E.» Dahlman, R. C.,  Hill,  G.  S,,  Ryan, A.D.
  and Witherspoon, J,  P., May 1975,  "Correlation of  Radioactive  Waste Treatment
  Costs and the Environmental Impact of Waste  Effluents in  the Nuclear Fuel
  Cycle for Use in Establishing  'As  Low As  Practicable1  Guides - Milling of
  Uranium Ores," Oak  Ridge National  Laboratory, ORNL-TM-4903, Vol. 1.

Sh62      Shearer, S.  D. , 1962,  "The Teachability of radium-226  from uranium
  mill waste  solids and river sediments," Ph.D. Dissertation, University of
  Wisconsin,  Madison,-  Wisconsin,

Sh64      Shearer, S.  D., and tee,  G. F., 1964, "teachability of Radium-226
  from Uranium Mill Solids and River Sediments," Health Physics, 10, 217-227.

Si66      Sigler, W.  F., Helm, W, T., Angelovic, J.  W. ,  Linn, W. D. and
  Martin, S.  S., 1966, "The effects  of uranium mill  wastes  on stream biota,"
  Bulletin 462, Utah  Agricultural Experiment Station, Utah  State University,
  Logan, Utah.

Si77      Sill, C. W. , 1977, "Workshop on Methods for Measuring  Radiation in
  and Around  Uranium  Mills,"  (Edited by Harward, E. D.), Atomic Industrial
  Forum Inc., Program Report, Vol. 5, No.  9,  221, Washington, D.C,

So79      Sorenson, J.B. and Marston, K.L., 1979, "Uranium  Mining and Milling and
  Environmental Protection:   Mitigation of Regulatory Problems," San Juan Basin
  Regional Uranium Study, Albuquerque, New Mexico, Working  Paper No.  35.

St79      Stein, R. B., 1979, "Modeling Future U-CL  Search  Costs," Engineering
  and Mining  Journal  179, No. 11, 112.

St^8      Stone and Webster Engineering Corp., 1978, "Uranium Mining and Milling -
  The Need, The"Processes, The Impacts, The Choices,"   A contract prepared for
  the Western Interstate Energy Board, U.S.  Environmental Protection Agency
  Report, EPA-908/1-78-OQ4.

Sw76      Swift,  J. J. , Hardin,  J, M. and Galley, H.W.,  1976, "Potential Radio-
  logical  Impact of Airborne Releases and Direct Gamma  Radiation to Individuals
  Living Near Inactive Uranium Mill  Tailings Piles,"  EPA-520/1-76-001.

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                                                                       3-257
 Ta58      Tanner,  A.B.,  1958,  "Meteorological  Influence on Radon Concen-
   tration in Drill  Holes,"  AIME Trans,  214,  706.

 Ta78      Tanner,  A.  B.,  1978, "Radon Migration in the Ground:   A Supple-
   mentary Review,"   U.S.  Geological  Survey Open-File  Report 78-1050.

 Ta64      Taylor,  S.  R,,  1964, "Abundance of Chemical  Elements  in the  Con-
   tinental  Crust:   A New Table,"   Geochim. Cosmochim.  Acta 29,  1273.

 Th79      Thomasson,  W.  N.,  1979,   "Draft Environmental  Development  Plan for
   Uranium Mining, Milling and  Conversion," U.S.  Department of Energy.

 Th78      Thompson,  W.E., et.  a!.,  1978,  "Ground-Water Elements of in-Situ
   Leach Mining  of Uranium,"  A  contract  prepared by Geraghty and Miller,  Inc.,
   for  the U.S.  Nuclear Regulatory  Commission,  NUREG/CR-Q311.

 Tr79      Travis, C.  C,,  Watson, A.  P., McDowell-Boyer,  L.  M.,  Cotter, S.  J.,
   Randolph,  M,  L. and Fields,  D. E,,  1979, "A  Radiological  Assessment  of Ra-
   don-222 Released  from Uranium Mills and Other Natural  and Technologically
   Enhanced  Sources,"  Oak  Ridge National Laboratory, NUREG/CR-0573 (ORNL/
   NUREG-55).

 Tu69     Turekian,  K. K., 1969, "Handbook of  Geochemistry," Springer-Verlog,
   New York,  pp. 314-316.

 TVA76     Tennessee Valley Authority, 1976,  "Final  Environmental  Statement -
   Morton  Ranch  Uranium Mining".

 TVA78a    Tennessee Valley Authority, Department of the  Interior,  1978,  "Final
   Environmental Statement - Dal ton Pass Uranium Mine".

 TVA78b    Tennessee Valley Authority, Department of the  Interior,  1978,  "Draft
   Environmental Statement - Crownpoint Uranium Mining  Project".

TVA79     Tennessee Valley Authority, 1979,  "Draft Environmental  Statement -
  Edgemont Uranium Mine".

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                                                                      3-258
Tw79      Tweeton, 0, R., et. al., 1979, "Qeoehemical Changes During In Situ
  Uranium Leaching with Acid," SME-AIME Preprint.

UGS54     Utah Geological Society, 1954, Guidebook to the Geology of Utah,
  No. 9, University of Utah, Salt Lake City, Utah.

We?4      Wentz, D. A,, 1974, "Effect of Mine Drainage on the Quality of
  Streams in Colorado, 1971-72," U.S. Geological Survey in Cooperation with
  the Colorado Water Pollution Control Commission, Colorado Water Conser-
  vation Board," Denver, Colorado, Circular No. 21.

Wh76      Whicker, F. W. and Winsor, T.F., 1976, "Interpretation of Radio-
  logical Analyses of Soil and Vegetation Collected from 1971 through 1975
  at the Shirley Basin Uranium Mine,"  Utah International Inc.,  San Fran-
  cisco, California.

Wo71      Woolson, E. A., Axley, J.  H., anu Kearney, P.  C.  1971, "The Chem-
  istry and Phytotoxicity of Arsenic in So:Is;  I.  Contaminated Field Soils,"
  Soil Scientists Society of America Proceedings, /ol.  35.

Wo79      Wogman, N. A., 1979, "Environmental Study of Active and Inactive
  Uranium Mines, Mills and their Effluents," Battelle Pacific Northwest
  Laboratory Report, PNL-3069.

Wy76-78   Wyoming Department of Environmental Quality,  Land Quality Division,
  1976-1978, Guidelines Nos. 1-6.

Wy77      Wyoming Mineral Corporation, 1977,  "Environmental Report - Irigaray
  Project, Johnson County, Wyoming,"  Wyoming Mineral  Corporation, 3900  So.
  Wadsworth Blvd. , Lakewood, Colorado 80235.

Ya73      Yamamoto, T., Yunoki,  E.,  Yamakawa, M., and Shimizu, M., 1973,
  "Studies on Environmental  Contamination by Uranium,  3.   Effects of Carbonate
  Ion on Uranium Adsorption to and Desorption from Soils,"   Journal  of  Radiation
  Research,  14,  219-224.

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         SECTION 4





DESCRIPTION OF       MINES

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                                                                 4 -
   4.0   Description  of  Model  Mines
        Section 1.3  describes uranium mines  and  their operations,  and  Section 3
   describes  the potential  sources of  contamination  at the principal  types  of
   active  and  inactive mines.   These  discussions  include an  analysis  of  the
   potential  sources  of contamination,  quantities of contaminants associated
   with  the different sources, variations  in the sources, and estimates of  the
   values  needed to  define the  impact  that these  sources may impose upon  the
   environment  and  nearby populations.  We attempted  to define these  terras  and
   mining  parameters in a way that would  reflect a general view of the uranium
   mining  industry  and permit a  generic assessment.   The  parametric values that
   we  have chosen  for  this assessment are listed  below.   The sections of this
   report  from  which  they we»*e derived are  given  in parentheses.

   4.1   Surface Mine
        The model open  pit  (surface) mine will be located  in Wyoming.   It is  the
   mine  defined in  Section 3.3 as  the "average large  mine."  However,  to define
   the total  Impact  of all 63 open pit  mines operating in the United  States  in
   1978  we used the parameters developed in  Section 3.3 for the "average mine."
Parameter
Ore, MT/yr
Sub-ore, MT/yr
Overburden, MT/yr
  Production Parameters (1.3.1, 3.3.1)
       Average La rge Hi ne
            5.1 x 105
            5.1 x 105
            4.0 x 107
                                   Average Mine
                                     1,2 x 105
                                     1.2 x 105
                                     6.0 x 106
Parameter
Mining days
  per year
Mine life, yr
Ore stockpile
  residence time,
Overburden
  management
days
Mining Parameters^3.3.1)
Average la rge Mine
          330

           17

           41

        Case  2*
Average Mine
     330

      17

      41

     Case 2*
  *Case 2—Backfilling concurrent with mining - assumes 7 pits opened in 17-yr.
  mine  life  and  the equivalent  of  one-pit overburden  (2.4 yr.  production)
  remains on the surface.

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                                                                4-2
 Parameter
 Average  grade,
  percent UgOg
 Th-232 concentration,
 Activity ratio
   (dust/ore)
 Mineralogy
 Density, MT/m3
 Surface 'area o
   stockpile, m
Area of pad, m
Stockpile height, m
Thickness of ore
  zone, m
  Ore Parameters (3.3.1.2)
      Average Urge Mine

           0.1

          10

           2.5
      Sandstone
           2.0

       6,200
       5,300
           9.2

          12
      Average Mine

           0.1

          10

           2.5
      Sandstone
           2.0

      3,590
      3,340
           3.1

          12
Parameter
Average grade,
 ' percent ILQg
Th-232 concentration,
  pCi/g
Activity ratio
  (dust/sub-ore)
Mineralogy
Density, MT/m3
Surface area of
              2
  stockpile, m
Stockpile height, m
Area of pad, hectares
Sub-Ore Parameters  (3.3.1.3)
      PeerageLarge Mine

           0.015
flverageMine

     0.01S

     2
2.5
Sandstone
2.0
120,000
30
11
2.5
Sandstone
2.0
36,000
30
3

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                                                                 4  -  3
Parameter
Average grade,
  percent U3CL
Th-232 concentration,
  pCI/g
Mineralogy
Density, MT/ra3
Surface area of
         2
  dump, m
Dump height, m
Area of terrain,
  hectares
                        Overburden Parameters  (3,3.1.1)
                          Average Large Mine

                               0.0020

                               1
                             Sedimentary
                               2.0

                           1.1  x  106
                             65

                             104
Average Mine

     0.0020

     1
  Sedimentary
     2.0
3.5 x"10
    30

    33
        5
                  Wastewater Discharge Parameters
Parameters  (mg/j, except as noted)
Discharge volume,
  m /ruin
Total uranium
Radium-226, pCi/£ ^
Total suspended solids
Zinc
Cadmium
Arsenic
                                                  Average Mine
                                                  2.94
                                        (Assumed value of 3.0)
                                                  0.07
                                                  0.41
                                                 20.88
                                                175
                                                  0.071
                                                  0.004
                                                  0.005
       (a)
          Concentration of Ra-226 and  its  daughters  are reduced to  10^  of the
 amount  actually  released  due  to  irreversible  sorption  and  precipitation.
       ^Concentration  of sulfate  is reduced  to 20% of  the amount  actually
 released due to Irreversible  sorption and  precipitation.

-------
                                                                 4-4
                           Ai rborneSource Terms (3.3.4)
        Section 3,3.4  identifies  and  describes  potential  sources  of  airborne
   contamination at  surface mines.   The principal  sources  are dusts  produced
   by mining operations and wind  erosion and Rn-222 released by exposed uranium
   in the  pit  and overburden,  sub-ore,  and  ore  piles.  The  tables  of Section
   3.3.4 present the  average annual  emissions of contaminants from  these sources
   during active mining.
                          Source
                Combustion Products
                Vehicular Dusts
                Dust from Mining  Activities
                Wind Suspended Dust
                Rn-222  Emissions
   4.2   Underground  Hi_n_e
        The model  underground mine, defined  in Section  3.4  as  the  "average  large
   mine," will  be  located  in New Mexico,  However,  to determine  the  total impact
   of  all  305  underground uranium  mines  in   the  United  States we  used  the
   parameters developed in  Section 3.4 for the "average mine."
Parameter
Ore, MT/yr
Sub-ore, MT/yr
Waste rock, MT/yr
Production Parameters (1.3.1, 3.4.1)
     Average Large Mine
          2__5
          2 x 105
        2,2 x 104
Average Mine
1.8 x 104
1.8 x 104
2.0 x 103
Parameter
Mining days per year  -
Mine life, yr
Ore stockpile residence
  time, days
Waste rock management
      Mi n i ncj Parameters (1.4.1!
          Ave rage  Larc[g_ _H i _ne
               330
                17

                41
          No backfill
Average Mine
     330
      17

      41
  No backfill

-------
                                                                 4-5
 Parameter
 Average grade,
   percent U30g
 Th-232 concentration,
   pCi/g
 Activity ratio
   (dust/ore)
 Mineralogy
 Density, MT/m
 Surface area  of
              2
   stockpile,  m
 Stockpile height, m
              2
 Area  of pad,  m
  Ore Parameters  (3.4.1.2)
      Average Large Mine

           0.10

          10

           2.5
      Sandstone
           2.0

       5,300
           3.1
       5,480
           Average  Mine

               0.10

               10

               2.5
           Sandstone
               2.0

             680
               3.1
             620
Parameter
Average  grade,
  percent U3Gg
Th-232 concentration,
  pCi/g
Activity ratio
  (dust/sub-ore)
Mineralogy
Density, MT/m
Surface area of
         2
  dump, m
Dump height, m
              ?
Area of pad, ra
Sub-Ore Parameters(3.4,1.3)
 Average Large Mine

      0.035
      2.5
 Sandstone
      2.0

104,900
     12
 99,400
     Average Mine
     0.035
     2.5
Sandstone
     2.0

18,800
     6
17,700

-------
                                                                 4-6
                       Maste Rock  Parameters  (3.4,1.1)
 Parameters
 Average  grade,
  percent U30g
 Th-232 concentration,
  pCi/g
 Mineralogy
 Density, MT/m3   -
 Surface area  of
         2
  dump, :n
 Dump h&vjht,  m
                  2
 Area or  terrain, m
Average Large Mine

     0.0020

     1
  Sedimentary
     2.0

14,100
    12
12,800
Average Mine

     0.0020
   Sedimentary
     2.0

 2,700
     6
                  Viastewater Discharge Parameters (3.4.2.2)
Parameter  (mg/jj except as noted)
Discharge  volume,
  m /min
Total Uranium
Radium-226, pCi
Lead-210,  pCi/s
Total suspended solids
Zinc
Barium
Cadmium
Arsenic
Molybdenum
Selenium
                         Average Mine
                         2.78
                      (assume value of 2.0)
                         1.41
                         1.37
                         1.46
                        27.8
                       116
                         0.043
                         0.81
                         0.007
                         0.012
                         0.29
                         0.076
       U)
          Concentrations of  Ra-226 and  its  daughters are  reduced  to  10  per-
  cent of  the amount  actually  released  due to irreversible  sorption  and  pre-
  cipitation.
       *  ^Concentrations of  sulfate are  reduced  to 20  percent of  the  amount
   actually released due to irreversible sorption and precipitation.

-------
                                                               4-7

                        Ai rborneSourceTerms  (3,4.4)
     Section  3,4.4  identifies  and  describes  potential  sources of  airborne
contamination  at underground mines.   The principal sources are  contaminated
dusts  due  to  mining operations and  wind  erosion and Rn-222 that is  released
from  the  mine exhaust vents during  mining  and from waste  rock,  sub-ore,  and
ore  pile  surfaces.   Average  annual  emissions  of contaminants  from  these
sources during active fliining operations are presented in  the following  tables
of Section 3.4.4.

                  Source                             Table
             Combustion Products                     3.52
             Vehicular Dusts                         3.56
             Dust from Mining Activities             3.54
             Wind Suspended Dust                     3.55
             Rn-222 Emissions                        3.51

4.3  In Situ Leach Mine
     The following parameters are for a model  (hypothetical) in situ solution
mine as defined in Section 3.5;
   1.   Size of deposit = 52.6 hectares
   2.   Average thickness of ore body = 8 m
   3.   Average ore grade = 0.06 percent U30g
   4.   Mineralogy = Sandstone
   5.   Ore density = 2 MT/m3
   6.   Ore body depth = 153 m
   7.   Mine life = 10 years (2-yr leach period in each  of 5 sectors)
   8.   Well  pattern = 5 spot
                       Injection wells - 260
                       Production wells =  200
                       Monitoring wells =   80
   9.    Annual  U30g production » 227 MT
  10.    Uranium leaching   efficiency = 80  percent
  11.    Lixiviant - Alkaline-
  12.    Lixiviant flow capacity a 2,000 i/m1n
  13.    Lixivitnt bleed =  50 A/min  (2.5 percent)
  14.    Uranium 1n Lixiviant *  183 mg/g,
  15.    Calcite.(CaC03)  removal  required = 2 kg calcite  per kg  U_0g

-------
                                                               4-8
      Data were insufficient to estimate aqueous releases of contaminants from
 these type mines.   However,  since  these facilities  are planned  to  operate
 with no  aqueous discharges, releases of contaminants via this pathway, except
 for possible  excursions,  should be small.  Annual  releases of contaminants to
 the atmosphere were computed  in  Section 3.5.3 for  the  model  mine and listed
 in Table  3.59.   These  estimated annual  airborne releases  will  be  used  to
 compute  dose  and  indicate  adverse  health effects  that might be  associated
 with  in  situ  leach mining.

 4.4  jn_actjve Gurface  Mine
      The model  inactive  surface  mine  will  be  located  in  Wyoming.    It  is
 defined   in   Suction  3.7.1.   The model  mine  parameters are  listed  below.

                             Mine  Parameters
                   1.   Period  of  active  mining  =  17  years
                   2.   Total waste rock  production =  8.88 x 10  MT
                                                       4
                   3.   Total ore  production = 3.59 x 10   MT
                                                                3
                   4.   Density of  ore  and waste rock  = 2.0 MT/m
                   5.   Size of abandoned  pit:
                       Volume  = 4.62 x  105 m3
                                                       4   2
                       Ground  surface  area = 2.03  x  10  m
                       Pit  bottom  area =  6.00 x 103 m2
                       Depth = 36.7  m
                   6.   Surface area  and  composition  of waste  rock pile  =
                                4  2
                       6.33 x  10   m  uniformly  covered to a depth of
                       0.36 m  with sub-ore
                   7.   Reclamation = none
                            Airborne Source Terms

     Sections  3.7.1.1  and 3.7.1.2  identify and describe potential sources of
airborne  contamination  at inactive  surface uranium  mines.   The  principal
sources are  contaminated, wind-suspended  dust  from the waste  rock  pile and
Rn-222 released  from exposed  ore and sub-ore bearing surfaces  in the pit and
the waste  rock pile.  Tables 3.70 and  3.74  show average annual emissions of
contaminants from these sources.

-------
                                                               4-9
4.5   Inactive  Underground  Mine
      The  model  inactive  underground  mine  will  be  located  in  New Mexico.  It is
defined in  Section  3.7.2,  and its  parameters are  listed below.

                             Mine  Parameters
                   1.    Period of active mining -  15 yrs
                                                              4
                   2.    Total waste rock production =  1.00 x 10  MT
                                                       4
                   3.    Total ore production = 3.14 x  10  MT
                   4.    Density of ore and waste rock  =2.0 MT/m
                   5.    Surface area and composition of waste rock pile =
                                3  2
                        4.08 x 10  m  uniformly covered to a depth of
                        0.78 m with sub-ore
                   6.    Mine entrance and exhaust  vents not sealed
                            Airborne Source Terms

     Sections  3.7.2.1  and 3.7.2.2  identify and  define  potential  sources of
airborne contamination  at inactive  underground uranium mines.  The principal
sources are  contaminated, wind-suspended  dust from the waste  rock  pile and
Rn-222  released  from the  unsealed  mine entrance and exhaust  vents  and the
waste rock pile.   Tables 3.76 and 3.77  list  average annual  emission of con-
taminants from these sources.

-------
     SECTION 5





POTENTIAL PATHWAYS

-------
                                                            5-1
 5.0  Potential Pathways

 5.1  General
 5.1.1  Vegetation
      Airborne  participate  radioactivity  may  be  deposited  directly on  the
 edible foliar surfaces of crops  or on the  soil and  then migrate through the
 soil  into the plant's root  system and into an edible  crop.  Such crops may be
 consumed directly by man or  by  animals which are  ultimately consumed by man.
 The  use  of  contaminated  water  (either groundwater  or  surface) to  irrigate
 crops  may also lead  to the  ingestion of radionuclides from either the direct
 consumption  of the crop or  the crop-to-animai-to-man  pathway.
      The reconnaissance surveys  of some inactive uranium mine  sites indicated
 that  no crops for  human  consumption  were being farmed  at or  near any of the
 sites.   Although  the  potential for man's  ingestion  of radionuclides in edible
 crops  due to the  direct deposition or the root uptake of either  airborne par-
 ticulates or contaminated mine water  is a greater  possibility  near  the active
 mines,  farming in such areas  is  not extensive.
      Almost  every inactive and active mine  site visited  had  range cattle and/
 or  sheep  grazing  on  the  natural  vegetation  growing  at  the site;  hence,  the
 possible  consumption  of such animals  could  be a  potential  pathway for  man's
 ingestion of radionuclides released into  the  environment surrounding  the mine
 sites.

 5.1.2   Wildlife
     There are numerous  species  of mammals,  birds, reptiles, and  amphibians
 at  both active and  inactive uranium mine  sites.   Though mining may  destroy
 their  natural  habitat,   there  are no  significant radiological  impacts on
 wildlife  in  these areas.  Dewatering  and  drainage from active mines sometimes
 create  ponds or  streams  that may  be used  by migratory waterfowl  and  local
wildlife  as  a source  of water,  but,  when mining  is completed,  the ponds dry
 up, probably without  leaving any  permanent or  significant  radiological impact
on wildlife.   The small  lakes formed in  inactive surface mine pits,  however,
may remain  for a long "period of  time and  have  a significant  environmental
 impact.   It  would  be  expected  that  sedimentation  and eutrophication of the
lakes  would  progressively diminish the impact with time by  reducing  the con-
tact of ore  bodies with the biosphere.  The potential  food pathway  of  animal-

-------
                                                            5-2
 to-man via wildlife hunting  at  these sites is also minimal.   Hunting 1s poor
 and  hunting restrictions are usually observed at the mine sites.

 5.1.3  Land Use
      Most uranium  mining  activities have  been conducted in  areas  away from
 population centers.  Most  mines are  located on  private property or are  on
 Federal  lands  such as  national  forests.    The  predominant   land  use  is  as
 rangeland  (or forest) and  only minor areas  are cropland.  The  fraction of land
                                                                             -3
 used  for vegetable crop production  for Wyoming and New Mexico is  1.59 x 10
              _g
 and  1.38 x 10 -,  respectively.   This fraction is  based  on the assumption that
 the  statewide  fractions apply  to  uranium mining  areas within  each state.
 Average  population densities are typically  rural,  i.e.,  less than  one person
           p
 per  2.6  km .

 5.1.4  Population Near Mining Areas
      Uranium  mines occur in  clusters throughout  many western states and are
 somewhat scattered throughout the eastern  states.   In  order  to estimate the
 number of persons residing within 50 miles (80km) of  a  mine, we used county
 populations  where there either  is  or  has  been mining.  Table 5.1 lists the
 states and their respective  mining  counties  plus  the numbers of inactive and
 active surface and underground uranium mines in  each county. We derived the
 county population  statistics from  U.S.  Department  of Commerce  census  data
 (DOC78), which are  January  1, 1975 estimates.   The  county areas were  obtained
 from  the same reference.
                         2
     The area, 20,106 km  , within  a  circle with  a  radius  of 80 km usually
 exceeds  the area  of most  counties.   Because  of  this,  the number of persons
 residing  within  80 km of a mine will  be underestimated  using county popula-
 tion  statistics.   In other words,   we  consider the estimates of populations
 within the  mining  regions to  be  somewhat  low.
     Persons  residing  in a mining   area  are likely  to be exposed from more
 than one mine  because of the  aforementioned clustering.   To account for  this,
 Table  5.1 -lists the product (person-mines)  for  both active and inactive  uran-
 ium mines.   The  total  number of  person-mines for inactive mines  Is approxi-
mately 82,000,000 persons.  The total number  of person-mines  for active mines
 is  approximately  14,000,000  persons.    The  combined  equivalent  population
exposed  to inactive and active  uranium  mining  is  approximately 96,000,000
persons.

-------
Table 5.1     Number of uranium mines and population statistics  for counties
              containing uranium nines
State County
!
Alaska Southeast'3'
Arizona Apache
Coehlse
Co con i no
filla
Graham
Maricopa
Mohava
Nivajo
Pfrrta
Santa Cm*
Yavapa 1
California Imperial
Inyo
tern
Lassen
Number of
Uranium Mines
Inactive Active
I
140
2
113
18
1
3
5
3S
2
3
3
2
1
6
2
0
0
0
0
0
0
0
0
1
1
0
0
0
0
0
0
Population
Density County Area
2 2
(persons/km ) (tai)
0,03
1.1
3.8
1.0
2.4
i,4
41,
0.76
2.3
19.
4.3
1.8
6,8
0.77
17
1.4
44,501
28,930
16,203
48,019
12,297
11,961
23,711
34,232
2S.666
23,931
3,227
20,956
10,984
26,237
21,113
11,816
County
Population
(persons)
1,282
32,304
81,918
48,326
29,255
16,578
i?l,Z28
25,857
5i»649
443,958
13,966
37,005
74,492
17,259
349,874
16,796
Person-Mines Person-Mines
Inactive Active
1,282
4,522,560
123,836
5,460,838
526,590
16,578
2,913,684
129,285
2,088,715
887,916
41,898
111,015
148,984
17.2S9
2,099,244
33,592
0
0
0
0
0
0
0
0
59,649
443,958
0
0
0
0
0
0

-------
Table 5.1
(Continued)
State County
i
California Madera
Mono
Riverside
San Bernarduv
Sierra
Tuolurnne
Colorado Boulder
Clear Creek
Custer
Dolores
Eagle
El Paso
Fremont
Garfield
Gilpin
Grand
Number of
Uranium Mines
Inactive Active
1
1
5
3
4
1
7
4
3
6
2
1
25
10
4
4
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
Population
Density
(persons /km'
7.5
0.51
25.
14
1.2
4.6
68
4.8
0.59
0.62
1.7
42
6.6
2.3
5.0
0.86
County Area
!) (to)2
5,556
7,840
18,586
52,103
2,481
5.832
1,937
995
1,909
2,657
4,353
5,587
4,022
7,759
383
4,802
County ,
Population
(persons)
41,519
4,016
456,916
696,871
2,842
25,996
131,889
4,819
1,120
1.641
7,498
235,972
26,545
17,845
1,915
4,107
Person-Mines Person-Mines
Inactive Active
41,519
4,016
2,284,580
2,090,613
2,842
25,996
923,223
19,276
3,360
9,846
14,996
235,972
663,625
178,450
7,660
16,428
0
0
o •
0
0
0
0
0
0
0
0
0
0
0
0
0

-------
Table 5.1
(Continued)
(
State County
Colorado Gunnison
Hinsdale
Huerfano
Jefferson
La Plata
Larimer
Mesa
Moffat
Montezuma
Hontrose
Park
Pitkin
Pueblo
Rio Blanco
Saguache
San Juan
Number of
Uranium Mines
Inactive Active
1
1
2
13
3
5
185
18
6
479
7
1
1
26
13
2
0
0
0
1
0
0
20
3
I
63
0
0
0
0
1
0
Population
Density
( persons/km )
1.2
0.19
1.6
120
5.4
17
7,3
0.77
2.7
3.5
0.77
3.5
20
0.77
0,39
0.77
County Area
(to)2
8,339
2,729
4,077
2,018
4,358
6,762
8,549
12,284
5,423
5,796
5,599
2,520
6,228
8,45t
8,142
1,012
County
Population
( persons \
10, DOS
519
6,590
235,368
23,533
114,954
62,407
9,459
14,642
20,286
4,311
8,820
124,560
6,507
3f175
779
Person-Mines
Inactive
10,006
519
13,180
3,059,784
70,599
574,770
11,545,295
170,262
87,852
9,716,994
30,177
8.S20
124,560
169,182
41,275
1,558
Person-Mines
Active
0
0
0
235,368
0
0
1,248,140
28,377
14,642
1,278,018
0
0
0
0
3,175
0

-------
Table 5.1
(Continued)
State
Col arado

Idaho

Montana





Nevada





County
San Miguel
Teller
Custer
Lemhi
Broadwater
Carbon
Fallen
Hill
Jefferson
Hadfson
Clark
Elko
Humboldt
Lander
Lincoln
Lyon
Number of
Uranium Hines
Inactive Active
339
3
5
1
1
11
1
1
3
1
2
3
1
2
2
2
25
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0
Population
Density
{persons/km*
0.7?
3.9
0.23
0.39
0.82
1.5
0.96
2.3
1.5
0.55
16,2
0.31
0.25
0.39
0.19
1.9
Coynty Area
1 (te)2
3,322
1,432
12,?66
11,862
3,090
5,325
4,229
7,581
4,278
9,138
20,393
44,452
25,128
14,558
27,114
5,257
County
Population
(persons)
E.557
5,584
2,967
6,395
2,526
7,797
4,050
17,358
6,839
5,014
330,714
13,958
6,375
2,992
2,64?
10,508
Person-Mines Person-Mines
Inactive Active
866,823
16,752
14,835
6,395
2,52$
85,767
4,050
17,358
20,517
5,014
661.428
41,874
6,375
5,984
5,294
21,016
63,925
0
0
0
0
0
0
0
0
0
0
0
0
0
0
0

-------
Table 5.1
(Continued)
State
Nevada


New Jersey
New Mexico












County
Mineral
; Hye
Was hoe
Sussex
Catron
Dona Ana,
Grant
Harding
Hidalgo
McKinley
Mora
Quay
R1o Arriba
Sandoval
San Juan
San Miguel
Santa Fe
Number of
Uranium Mines
Inactive Active
2
1
6
I
4
1
3
1
1
73
1
3
8
3
41
3
2
0
0
0
0
0
0
0
0
0
35
0
0
0
0
0
0
0
Population
Oens i ty
o
{persons/km )
0.71
0.12
8,9
73
0.12
7.1
2.1
0.25
0.53
3.5
0.93
1.5
1.9
2.3
4.6
1.8
13
County Area
(ta»)2
9,751
46,786
16,487
1,364
17,863
9,852
10,282
5,527
8,927
14,138
5,025
7,446
15,133
9,619
14,245
12,279
4,926
County
Population
(persons)
7,051
5,5§9
144,750
99,299
2,198
69,773
22,030
1,348
4,734
49,483
4,573
10,903
28,752
22,123
65,527
21,§S1
64,038
Person-Mines
Inactive
14,102
5,599
868,100
99,299
8,792
69,773
66,090
1,348
4,734
3,612,259
4,673
32,709
230,016
66,369
2,686,S07
$5,853
128,076
Person-Mines
Active
0
0
0
0
0
0
0
0

1,731,905
0
0
0
0
0
0
0

-------
Table 5,1
(Continued)
State
Mew Mexico



North Dakota


Oklahoma

Oregon

South Dakota





County
Sierra
Socorro
Taos
Valencia
Billings
Slope
Stark
Cad do
Custer
Crook
Lake
Butte
Custer
Fall River
Harding
Lanrence
Pennlngton
Number
Uranium
Inactive
6
7
I
19
9
1
3
2
1
1
2
3
ID
93
28
2
5
of
Mines
Active
0
Q
0
4
0
3
0
0
0
0
0
0
0
0
0
0
0
Population
Density
2
{ persons/km )
0.6?
0.57
3,0
3.1
0.39
0.39
5.8
8.8
8.3
1.3
0.34
1.3
l.Z
1.9
0.39
8.4
8.3
County Area
(km)2
10,790
17,102
5,843
14,649
2,950
3,172
3,408
3,294
2,538
7,703
21,318
5,827
4,032
4,514
6,946
2,072
7,198
County
Population
(persons)
7,189
9,763
17,516
45,411
1,153
1,360
19,650
28,931
21,040
9,985
7,158
7,825
5,196
8,066
1,879
17,453
59,349
Person-Mines
Inactive
43,134
68,341
17,516
862,809
10,377
1,360
58,950
57,862
21,040
9,985
14,316
23,475
51,960
750,138
$2,612
34,906
296,745
Person-Mines
Active
0
0
0
181,644
0
0
0
0
0
0
0
0
0
0
0
0
0

-------
Table 5.1
(Continued)
State County
Texas • Briseoe
Burnet
Crosby
Sana
Gonzales
Karnes
lite Oak
Utah Beaver
Box El
-------
Table 5.1
(Continued)
State
Utah





Washington


Wyoming






Cou n ty
Pmte
San Juan
Sevier
Umtah
Mash ing ton
Wayne
Pend Orel lie
Spokane
Stevens
Albany
8ig Horn
Camp be 1 1
Carbon
Converse
Crook
Fremont
Number
Uranium
Inactive
10
241
2
14
6
32
3
9
1
4
9
55
16
31
23
65
of
Mines
Active
0
24
0
0
0
0
0
0
z
0
0
0
3
5
0
13
Population
Bens i ty
2
(persons/km }
0,77
0.77
2.3
1.5
2.7
0.39
1.9
67
3.5
2.3
1.5
1.2
0,77
0.77
0.77
1.2
County Area
(km)2
1,952
i§,961
4, §96
11,621
8,281
6,438
3,631
4,553
6,4
-------
                Table S.I
(Continued)
Stite County
Wyoming Johnson
i Nitrona
Niobrara
Sublett«
Sweetwater
Washakie
Weston

Rum her
Uranium
Inactive
15
16
13
1
4
2
1

Of
Mines
Active
0
2
0
0
I
0
0

Population
Dans i tv
y
(persons/km )
0,39
3,9
0,39
0.39
1.2
1,5
1,0
Average Population
Density Area
2
4.4 persons /km 1
County Area
(km)2
10,813
13,835
6,770
12,554
27,011
5,858
6»Z34
County
Population Person-Mines Person-Mines
(persons) Inactive Active
4,217 63,255
53,956 863,296
2,640 34,320
4,899 4,899
32,413 129,652
8,78? 17,574
6,307 6,307
Total County Total Person-Mines
(tan)2 Population (Inactive)
,492,136 6,625,099 82,327,885
0
107,912
0
0
64,826
0
0
Total Person-Nines
(Active)
14,035,161
Note.--Population statistics from (OOC78).
   Congressional  District.

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                                                            5-12
 5.1.5  Population  Statistics  of  Humansand  BeefCattle
      Table 5,2 lists some  population  statistics for humans in New Mexico and
 Wyoming,  humans in all  uranium  mining  states, and  beef  cattle  in New Mexico
 and Wyoming.
        Table   5.2    Population  statistics  for  humans  and  beef cattle
     TotalHuman  andBeef  Cattle  Population Within 80  km Radius  of  Mines
               New Mexico          Wyoming        All  Uranium Mining States

 Human          447,412              224,195              6,625,099
 Beef cattle    753,000              905,000              	
  Average  Human and Beef Cattle  Population Densities Within 80 km Radius
                 of Uranium Mines  (number/km r'
Human
Beef Cattle
2.4
4.1
1.3
5.1
4.4
              taken from Table  5.1:  New Mexico - 183,646 km2; Wyoming • 177,422
  2                                          2
km, and the total county area  = 1,492,136 km ,
5.2  ProminentEnylronmental Pathways and Parameters for Aqueous Releases
     From a computer code prepared within EPA, we calculated annual committed
dose equivalents  to  individuals and annual collective  dose  equivalents  to a
population for these  assessments.   Table 5.3 lists the aqueous pathways that
were  initially-considered  potential  pathways of  exposure.  As  indicated  in
Table  5,3,  these pathways  result  in computation of dose  equivalents  due  to
inhalation, ingestion, ground surface exposure, and air submersion. For above
surface crop  ingestion, milk  ingestion,  and beef  ingestion  (pathways 3,  4,
and 5), we considered  only uptake through  the plant  root systems to predict

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                                                            5-13
 concentrations  of radlonuelides  in  crops,  since essentially all irrigation is
 ditch   irrigation.    Appendix  J  contains  a  detailed  explanation  of  the
 environmental  transport  and  dosimetry models used in these analyses.

     The  maximum individual  for the  aquatic pathways  is  the  individual  at
 maximum risk.   He  is exposed to  radionuclides  discharged  in  mine  effluent
 through pathways 2 through  10 of Table  5.3.   The water contributing radionu-
 cl ides  to  these pathways comes from  a creek into which  a mine  discharges.  The
 average individual  is exposed to the average risk of all  persons  included in
 the  population  of the assessment area.   He is  exposed  to  radionuclides dis-
 charged in mine  effluent  through  pathways 2  through 8 and 10  of Table 5.3.
 The  water  contributing  radionucl ides  to  these pathways  is  taken  from  the
 regional  river after  the  creek water has  been diluted in this  river.   The
 population  considered in the assessment of the aquatic pathways  is  obtained
 by  multiplying the  regional assessment area  size by the  population  density
 within  this area.  This assessment  area contains the drainage  basin  for  the
 mine effluent stream, the creek and the regional  river discussed  in  defining
 the maximum and average  individuals.

 5.2.1   IndividualCommitted  Dose Equivalent Assessment
     Section  6  of this  report contains  the computed dose equivalents  to  the
 maximum individual   and  to  the  average  individual.  For  the maximum  indi-
 vidual,' we  included  all  pathways in  Table  5.3 except drinking  water  (pathway
 1).  It is  known that the releases  to the aquatic  environment occur  through
 discharge  of mine  water  to surface  streams.   Potentially,  drinking  water
 could be one  of the most significant  pathways  for the maximum  individual dose
 equivalents,  if surface  water containing mine wastes was drunk.   However,  it
 appears that all  drinking water for  both the New Mexico  and the  Wyoming  sites
 conies   from  wells   (Robert  Kaufmann,  1979,  U.S.  Environmental  Protection
 Agency,  Las  Vegas,  NV,   personal  communication).   Thus,  the  only  way mine
 discharges  can  enter  human drinking water is by  percolating through the  soil.
 Since  we  do  not  know   the  soil  chemistry for  these  sites  well  enough  to
 predict  the  ion-exchange- parameters  for   the  soil,  we  can  not  predict,
 realistically,  the  quantity  of  mine-related  radionuclides  that would  ^ach
 the groundwater.   We expect that these ion-exchange factors  would  be  large
 for  several  of  the  radionuclides  conn'dered  in  these  analyses  and that
groundwater concentrations of radionuclides discharged  in mine  water

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                                                            5-14
would  be  quite  small  compared to concentrations  In  the surface water down-
stream from  the  mines.  Further study is  needed before dose equivalents  for
the  maximum  individual by drinking  groundwater can be adequately addressed.
     The following are other assumptions used to calculate  maximum individual
dose equivalents:
     1.   Ground surface concentrations of radionuclldes (used for
          pathways 6 through 8) are  for 8.5 years,  the assumed
          midpoint of mine life.  The assumed period of mine oper-
          ation is 17 years.  The organ annual dose equivalents for
          the external surface exposure pathway are based on the
          ground concentrations after the 8.5 years buildup time.
     2.   For inhaled or ingested radionuclides» the dose equivalents
          are the annual committed dose equivalents that will be
          accumulated over 70 years after intake for an adult.
     We calculated dose  equivalents  to the average individual in the assess-
ment area by  taking  the population dose equivalents (discussed in Subsection
5.2.2) and dividing by the population living in the area.

Table 5.3  Aquatic environmental transport pathways initially considered

Pathway No.                                   Pathway

     1              Drinking water ingestion
     2              Freshwater fish ingestion
     3              Above surface crops ingestion - irrigated cropland
     4              Milk ingestion -  cows  grazing on irrigated pasture
     5              Beef Ingestion -  cows  grazing on irrigated pasture
     6              Inhalation - material  resuspended which was deposited
                    during  irrigation
     7              External  dose due to ground contamination by material
                    originally deposited  during irrigation
     8              External  dose due to  air submersion in  resuspended
                    material  originally deposited during irrigation
     9              Milk ingestion -  cows  drinking  contaminated
                    surface water
    10              Beef ingestion -  cows  drinking  contaminated surface
                    water

-------
                                                            5-15
 5.2.2  Collective  (Population)  Dose Equivalent Assessment
      For the population dose  equivalent assessment calculations,  we concluded
 that the  pathways  of  concern  are pathways  2,  3» 4, 5,  6,  7t 8» and  10  of
 Table 5.3  (detailed  discussion in Appendix  J,  subsection J2).  The  size  of
                                                 2               2
 the assessment areas  for New  Mexico is 19,037 km  and  13,650  km  for  Wyoming.
 We used the following considerations  to calculate  population  dose equivalents
 for the assessment  area:
      1.   Ground surface concentrations of radionuclides  are  for  8.5
           years, the  assumed  midpoint mine life.   (The period of
           mine operation is 17  years.)   The organ  annual  collective
           dose equivalent rates for the external surface  exposure
           pathway are based on  the ground  concentrations  after the
           8.5  year  buildup time.

      2,    For  inhaled or ingested  radionuclides, the dose  equivalents
           are  the annual  collective dose equivalents that  will  be ac-
           cumulated over the  70 years  after intake for adults.

      3.    The  population  distributions  around the  sites are based
           on estimates  by county planners  (John  Zaboroc,  1979,
           Converse  Area Planning Office, Douglas,  Wyoming, personal
           communication)  and  agricultural  personnel (Tony  Romo, 1979,
           Valencia  County Agent, Los  Lunas, New Mexico, personal
           communication)  for  1979.  The populations, assumed  to remain
           constant  in time, were estimated  to be 16,230 and 64,950
           persons in  the  Wyoming and  New Mexico assessment areas,
           respectively,

      4.    Average agricultural  production data for the county  which con-
           tains a major  portion of  the  assessment  area are used.

      5.    The  population  in the assessment  area eats food  from the as-
           sessment area.  We assume that any  imported  food is  free ot
           radionuclides.

     As  mentioned  previously. Appendix J  contains the details regarding the
models and values for parameters used in these analyses.

-------
                                                            5-16
5.3  j^gnimentEnvironmentalPathways and Paraffieters  for Atmospheric Releases
     We  used  the  AIRDOS-EPA  (Mo79)  computer  code to calculate radionyclide
air  and  ground  concentrations,  ingestion and  inhalation intakes, and working
level exposures; and we used the DARTAB (BeSO) computer code to calculate dose
and  risk  from  the AIRDOS-EPA Intermediate output  using dose and risk factors
from the  RADRISK (Du80)  computer code.  We calculated working levels associ-
ated with  Rn-222 emissions assuming  that Rn-222  decay  products  were 70 per-
cent in  equilibrium  with  Rn-222» a value considered  representative of indoor
exposure conditions (Se78).  Appendix K contains a detailed discussion of the
application of the AIRDOS-EPA and RA0RISK computer codes.
     Figure  5.1  shows  the general airborne  pathways evaluated  for uranium
mines.    We  calculated doses due to  air immersion,  ground  surface exposure,
inhalation, and ingestion of radionuclides,  but w= did not address the resus-
pension pathway, since  the AIRDOS-EPA code  did nat provide a method for cal-
culating  resuspended  air  concentrations  or  subssquent  redeposftlon to  the
ground  surface.   We  used  the  modification  to  the AIRDOS-EPA computer  code
made by  Nelson  (Me80)  to  include the  effect  of environmental  removal  of
radioactivity from the  soil.   For ingestion,  transfers associated  with  both
root uptake and foliar deposition on  food  and forage are considered,

5.3.1  IndividualCommittedDoseEquivalentAssessment
     We assessed  the  maximum individual  on the following  basis:

     1.    The maximum individual  for each  source category is intended
          to represent an  average of the  individuals living  close  to
          each  model  uranium mine.  The  individual  Is assumed  to be
          located about 1600 meters from the  center of the model site.
     2.    Ground  surface concentrations  of radionuclides  used  in the
          assessment  are  those  that would occur during the midpoint  of
          the active  life  of the  model uranium mine.  Buildup  times
          used  in the  assessment  are 8.5 years  for  active  surface and
          underground  mines, 5 years for the  in situ leach mine, and
          26.5 years  for the inactive  surface  and underground mines.
          The 26.5-year  buildup time for the  inactive mines  is chosen
          to represent the midpoint of the 53-year  exposure  time that
         a  resident  living  a lifetime in the  region around  the model
         mine is estimated  to experience.  The organ dose equivalent
         rates for the external  surface exposure  pathway are  based  on

-------
                                      Airborne Radionuehdes and Trace Metal Contaminants
                             Inhalation
Soil
Vegetation
"*"   Ingestion
                                                                      Animals
                                                                                                                               Ul
                                                                                                                               I
' Figure 5 1 Potential airborne pathways in the vicinity of uranium mines.

-------
                                                           5-18
          "the concentrations for the indicated buildup time,

     3.   For inhaled or ingested radionuclides, the dose equivalent
          rates are actually the 70-year committed dose equivalent
          rates for an adult receptor, i.e., the internal dose equiva-
          lent that would be delivered up to 70 years after an intake.
          The individual dose equivalent rates in the tables are in
          units of mrem/yr.

     4.   The individual is assumed to home grow a portion of his or
          her diet consistent with the rural setting for each model
          uranium mine site.  Appendix K contains the actual  fractions
          of home-produced food consumed by individuals for the model
          mine sites.  The portion of the individual's diet that was
          not locally produced is assumed to be imported and uncontam-
          inated by the assessment source.

5.3.2  ColTective (Population) Dose Equivalent Assessment

     The collective dose equivalent assessment to the population out to 80 km
from the facility under consideration is performed as follows:
     1.   The population distribution around the model  mine sites is
          based on the 1970 census.   The population is assumed to re-
          main constant in time.
     2.   Ground surface concentrations  and organ dose equivalent rates
          for the external  surface exposure pathway (as for the individ-
          ual  case) are those that would occur over the active life of
          the  model  mine.
     3.   Average agricultural  production data for the state  in which  the
          model  uranium mine is  located  are assumed.
     4.  Jhe  population in the  assessment area eats  food from the  assess-
          ment area to the  extent that the calculated production allows,
          and  any balance  is assumed  to  be imported without contamination
          by the  assessment source.
     5.    Seventy-year committed  dose equivalent  factors  for  an adult
          receptor (as for  the  individual  case) are used  for  ingestion
          and  inhalation.

-------
                                                            5-19
5.4  Mine Wastes Used  In  the Construction of Habitable  Structures
     Using  uranium  mine  wastes  under  or  around  habitable  structures  or
building  habitable structures on  land contaminated  with uranium mine wastes
can  result  in  increased  radiation exposures  to individuals occupying  these
structures.   The  radium-226  present  in these  wastes  elevates  the concen-
trations  of radon-222 and  its  decay  products and  produces  increased  gamma
radiation inside  these structures.  The health  risk to  individuals occupying
these  structures  is  generally  much  greater  from  inhaling  radon-222  decay
products than the  risk received  from gamma radiation.
     Radon-222,  formed from the decay of radium-226,  is  an  inert gas  that
diffuses  through the soil and migrates  readily  through foundations, floors,
and  walls  and   accumulates  in  the  inside  air  of  a  structure.   Breathing
radon-222  and  its  short-lived  decay  products  (principally  polonium-218,
bismuth-214, and polonium-214) exposes the lungs to radiation.
     The  radon-222  decay  product concentration  (working  level)  inside  a
structure  from   radon-222  gas  diffusing  from underlying  soil  is extremely
variable  and  influenced   by  many complex factors.   These  would  include the
radium-226  concentration of  the soil,  the  fraction of  radon-222 emanating
from the  soil,   the  diffusion  coefficient  of radon-222  in  soil,  the rate of
influx  of  radon-222  into  the  structure,   the  ventilation  rate  of  the
structure,  and   the   amount  of  plate-out  (adsorption)  of  radon-222  decay
products on inside surfaces.
     'The potential risks of fatal lung cancer that could occur to individuals
living in homes  built on land contaminated by uranium  mine wastes have been
estimated using  measurements and calculational  methodology  relating radon-222
decay product concentrations inside homes to  the  radium-226 concentrations in
outside  soil  (He78,  Wi78).   These  estimates  are  shown  in Section  6.1.5.

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                                                           5-20
5.5  References
Be80    Begovich, C.L., Eckerman, K.F., Schlatter, E.G. and Qhr, S.Y., 1980,
     "DARTAB: A Program to Combine Airborne Radionuclide Environmental Exposure
     Data with Dosimetric and Health Effects Data to Generate Tabulations of
     Predicted Impacts," Oak Ridge National Laboratory Rept., QRNL-5692 (Draft).
DQC78   U.S. Department of Commerce, Bureau of Census, 1978, "County and
     City Data Book, 1977,"  (U.S. Government Printing Office, Washington,
     D.C.).
Du80   Dunning, D.E. Jr., Leggett, R.W., and Yalcintas, M.G., 1980, "A Com-
     bined Methodology for Estimating Dose Rates and Health Effects from
     Exposure to Radioactive Pollutants," Oak Ridge Natioial Laboratory
     Rept., OiNL/TM-7105.
6e78   George, A.C. and Breslin, A.J., 1978, "The Distribution of Ambient Radon
     and Radon Daughters in Residential Buildings in the New Jersey-New York
     Area," presented at the symposium on the Natural Radiation Environment III,
     Houston, Texas, April 23-28.
He78   Healy, J.W. and Rodgers, J.C., 1978, "A Preliminary Study of Radium-
     Concentrated Soil," Los Alamos Scientific Laboratory Report, LA-7391-
     MS,
Mo79   Moore, R.E., Baes, C.F. Ill, McDowell-Boyer, L.M., Watson, A.P.,
     Hoffman, F.  0., Pleasant, J.C. and Miller,  C.W., 1979, "AIRDOS-EPA:
     A Computerized Hethodology for Estimating Environmental Concentrations
     and Dose to Man from Airborne Releases of Radionuclides," U.S. Environ-
     mental  Protection Agency Report, EPA 520/1-79-009 (Reprint of ORNL-
     5532).
Ne80   Nelson, C.B., 1980, "AIRDOS-EPA Program Modifications," internal
     memorandum dated February 12, 1980, U.S.  Environmental Protection
     Agency, Office of Radiation Programs,  Washington, D.C,.
Wi78  Windham,  S.T., Phillips,  C.R.,  and Savage,  E.D., 1978, "Florida
     Phosphate Land Evaluation Criteria,"  U.S.  Environmental  Protection
     Agency Draft Report,  unpublished.

-------
            SECTION 6





HEALTH AND ENVIRONMENTAL EFFECTS

-------
                                                                  6 - 1
 6.0  Health and Environmental  Effects
 6.1  Health Effects and Radiation Dosimetry
 6.1.1  Radioactive Airborne Emissions
      We  used  data  on  radioactive  emissions  (Section  3}  to  estimate  the
 public health impact of these  emissions.   Our assessments include estimates
 of the following radiation exposures and  health risks:

    1.   Dose equivalent rates  and working level exposures to the
         most exposed individuals (maximum individual) and to the
         average exposed individuals in the regional  population
         (average individual)
    2.   Collective dose equivalent rates  and working level  exposures
         to the regional  population
    3.   Lifetime fatal  cancer  risks to the maximum and average indi-
         viduals in the  regional  population
    4.   Genetic effect  risk to the descendants of the maximum and
         average individuals in the regional  population
    5.   The number of fatal  cancers committed in  the regional  popu-
         lation per year of model  mine operation
    6.   The number of genetic  effects committed to the descendants of
         the regional population  per year  of model  mine operation

      The somatic health impact risks estimated in this report are for  fatal
 cancers  only.   For whole  body exposure,  the risk  of  nonfatal cancer  is
 about the  same  or slightly less than for  fatal cancer.  Thus, for  whole
 body  doses, it is conservatively  estimated  that  one nonfatal  cancer  could
 occur for each additional  fatal  cancer.   The somatic health  impact  for  the
 regional  population (additional  cancers  per  year)  is calculated at  equi-
 librium  for continuous  exposure  and this  is  equal  to the  additional  cancers
 committed   over  all  time  per year  of  exposure;  thus  we used  the  term
 committed  additional cancers {see Appendix  L),
      The  genetic effect risks  estimated  in  this  report are for  effects  in
descendants of an irradiated  parent  or parents.   Genetic effects per year
 in  the  regional  population due  to  radionuclide releases  from  the mines  are
calculated  for an equilibrium exposure  situation.  The calculated  genetic
effects  per year at equilibrium  is  equal  to the genetic effects committed
over  all  time from one  vear exposure.   Thus,  the calculated  additional

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               Table 6.1      Annual-release rates (C1) used in the dose equivalent and  health
                              effects computations for active uranium mines
Classifi-
cation
Mining
activities
Ore
Sub-ore
Overburden/
waste rock
Vehicular
dust
Total
Average Surface Mine^
Location
Pit/mine site
Pile site
Pile site
Pile site
Mining area
All sources
U
4.3E-3
1.01E-2
4.2E-4
2.25E-3
9.9E-4
1.81E-2
Th
2.2E-4
1.42E-4
8.4E-6
1.50E-4
3.7E-4
8.90E-4
Rn-222
1.99E+2
4.2E+1
5.0E-H
4.0E+1
0
3.31E+2
Average Large Surface Mine * '
U
2.57E-2
4.42E-2
1.51E-3
1.34E-2
5.86E-3
9.07E-2
Th
1.44E-3
6.20E-4
3.00E-5
8.94E-4
2.17E-3
5.15E-3
Rn-222
7.97E+2
9.6E+1
1.66E+2
2.02E+2
0
1.26E+3
;?(Release rates taken from Tables 3.32 to 3.35.
l°JRelease rates taken from Tables 3.51 and 3.54 to 3.56.
                                                                                                          cr>

                                                                                                          ro

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Table 6.1 (cont.)
Average Underground Mine ^ '
U
2.22E-4
9.63E-4
1.04E-3
9.6E-6
6.5E-5
2.30E-3
Th ,
2.8E-6
1.35E-5
8.4E-6
6.4E-7
2.4E-5
4.93E-5
Rn-222
3.08E+2
7.7
6.1E+1
5.0E-1
0
3.77E+2
Average Larqe Underground Mine * '
U
2.41E-3
1.07E-2
5.95E-3
5.10E-5
1.29E-4
1.92E-2
Th
3.10E-5
1.50E-4
4.8E-5
3.40E-6
4.80E-5
2.80E-4
Rn-222
3.42E+3
6.83E-H
3.38E+2
2.6
0
3.83E+3
fcl
In Situ Leach Mine VCJ
U
l.OE-1 ,
N.A. ^
N.A.
N.A.
N.A.
l.OE-1
Th
0
N.A.
N.A.
N.A.
N.A.
0
Rn-222
6.50E+2
N.A.
N.A.
N.A.
N.A.
6.50E+2
     (c)

     (d)
Release rates taken from Table 3.59.

N.A.-  Not Applicable.
Note.--Columns labeled U and Th Include each daughter of the decay chain in secular equilibrium.
                                                                                                               I
                                                                                                               OJ

-------
                                                                 6-4
Table 6.2   Annual release rates (Ci) used in" the dose equivalent and health
            effects computations for inactive uranium mines
Location
Pit/vents-
portals
Waste rock/
sub-ore pile
Surface Mine ^ Underground Mine \ '
U Th Rn-222 U Th Rn-222
0 0 8.1 0 0 7.55

1.48E-3 1.1E-5 1.74E+1 2.38E-4 1.7E-6 1.7

     ^  '
          Release rates taken from Tables 3.70 and 3.74.
          Release rates taken from Tables 3.76 and 3.77.
Note. — Column headings U and Th include each daughter of the decay chain
       in secular equilibrium.

-------
                                                                  6-5
genetic  effects are  committed  effects  to  all  future  generations  for  one
year of exposure to the regional  population.
     We  calculated  individually each major  source of radionuclide  airborne
emissions  for each  model  uranium mine  site  so  that we could determine  the
extent that  each source contributed  to  the total health impact.  Tables  6.1
and 6.2 contain the annual release rates for each source classification  (or
location)  that  we  used   to  calculate dose equivalent  rates  and health
effects for  active and inactive uranium mines.
     The  estimated -annual  working level exposures from Rn-222 emissions by
the model  uranium mines  are listed  in Table  6.3.  The  working level ex-
posures  presented  for the maximum individual are  the  Rn-222 decay product
levels to  which an individual would  be continuously exposed for an entire
year. Working level  exposure to  the  regional population  is the sum of  the
exposures  to  all  individuals  in the  exposed  population  from  the annual
release from the model mine.
     We  estimated  radiological  impacts of  radioactive  airborne emissions
from  the  model uranium mines with  the A[RDOS-EPA  (Mo79),  RADRISK (Du80),
and DARTAB  (Be80)  computer codes.  Appendixes K and L contain explanations
of our use of these computer codes.
     Where  emissions  for  U-238 plus daughters  and Th-232  plus daughters
were reported (Section  3), a source term for both the parent and important
daughters  were input into  the AIRDOS-EPA code.   For  example,  a  reported
emission  rate of 0.01 Ci/yr  of U-238 plus daughters (U  in Tables  6.1 and
6.2) would  be input  into  the AIRDOS-EPA code as  0.01  Ci/yr of U-238, 0.01
Ci/yr of  U-234,  0.01  Ci/yr of Th-230,  0.01  Ci/yr  of Ra-226, 0.01 Ci/yr of
Pb-214,  0.01  Ci/yr  of Bi-214,  0.01  Ci/yr  of Pb-210,  and 0.01 Ci/yr of
Po-210.  A  reported  emission  rate  of  0.01 Ci/yr of Th-232 plus daughters
(Th in Tables 6.1  and 6.2) would be input into the AIRDOS-EPA code as 0.01
Ci/yr of Th-232, 0.01  Ci/yr of Ra-228, 0.01 Ci/yr of Ac-228, 0.01 Ci/yr of
Th-228, 0.01  Ci/yr of  Ra-224, 0.01 Ci/yr of  Pb-212, 0.01 Ci/yr of Bi-212,
and 0.0036  Ci/yr of  Tl-208.  The Tl-208 source term 1s  approximately one-
third that of Bi-212 because of the branching ratio.
     The  maximum individual, average individual, and population dose equiv-

-------
                              Table 6.3   Annual working level exposure from radon-222
                                          emissions from model uranium mines
Source
s
Average Surface Mine
Average Large
Surface Mine
Average Underground
Mine
Average Large
Underground Mine
Inactive Surface
Mine
Inactive Underground
Mine
In Situ Leach Mine
Maximum
Individual
(WL}(a)
2.3E-4

8.4E-4

4.6E-4

4.7E-3

1.8E-5

1.1E-5
4.5E-4
Average
Individual
(WL)
4.5E-7

1.7E-6

2.1E-6

2.1E-5

3.5E-8

5.1E-8
8.9E-7
Regional
Population
(person-WL)
6.5E-3

2.5E-2

7.5E-2

7.6E-1

5.0E-4

1.8E-3
1.3E-2
(a)
    Working level.
                                                                                                              en

-------
                                                                  6  -  7
  Table 6.4  Annual radiation dose equivalents due to atmospheric radioactive
             particulate and Rn-222 emissions from a model average surface
             uranium mine
Organ
Red marrow
Endosteal
Pulmonary
Muscle
Liver
Stomach wall
Pancreas
LLI^ wall
Kidney
Bladder wall
ULI(b) wall
SItc^ wall
Ovaries
Testes
Spleen
Uterus
Thymus
Thyroid
Weighted mean
Maximum
Individual
(mrem/yr)
2.4
3.4E+1
1.2E+1
5.5E-1
1.6
9.7E-2
5.2E-1
4.6E-1
4.2
3.0E-1
2.1E-1
9.4E-2
5.1E-1
5.4E-1
6.4
5.1E-1
5.2E-1
5.4E-1
4.9
Average
Individual
(mrem/yr)
5.4E-3
7.5E-2
6.3E-3
2.0E-3
6.3E-3
8.9E-5
1.9E-3
1.6E-3
1.8E-2
9.7E-4
5.2E-4
1.2E-4
1.9E-3
1.9E-3
2.8E-2
1.9E-3
1.9E-3
1.9E-3
5.5E-3
Population
(person-rem/yr)
7.7E-Z
1.1
9.0E-2
2.7E-2
9.1E-2
1.3E-3
2.7E-2
2,3E-2
2.5E-1
1.4E-2
7.4E-3
1.7E-3
2.7E-2
2.7E-2
4.0E-1
2.7E-2
2.7E-2
2.7E-2
7.8E-2
> ' I AlaJdy 1 Jl r«no -ir»-f-£ie'4->i««* *.ia 1 1
uppsr larytj  inucsuine
Small intestine wall.

-------
                                                                6-8
Table 6.5  Annual radiation dose equivalents due to atmospheric radio-
           active participate and Rn-222 emissions from a model average
           large surface uranium mine
Organ
Red marrow
Endosteal
Pulmonary
Muscle
Liver
Stomach wall
Pancreas
LLI wall
Kidney
Bladder wall
ULI wall
SI wall
Ovaries
Testes
Spleen
Uterus
Thymu s
Thyroid
Weighted mean - -
Maximum
Individual
(mrem/yr)
1.35E+1
1.9E+2
6.6E+1
3.0
8.9
5.4E-1
3.0
2.5
2.1E+1
1.7
1.1
5.2E-1
2.8
3.0
3.5E+1
2.8
2.9
3.0
2.7E+1
Average
Individual
(mrem/yr)
2.7E-2
3.8E-1
3.1E-2
9.5E-3
3.2E-2
4.5E-4
9.6E-3
8.2E-3
9.0E-2
4.9E-3
2.6E-3
6.0E-4
9.6E-3
9.5E-3
1.4E-1
9.6E-3
9.6E-3
9.6E-3
2.7E-2
Population
(person-rem/yr)
3.9E-1
5.4
4.5E-1
• 1.4E-1
4.6E-1
6.4E-3
1.4E-1
1.2E-1
1.3
7.0E-2
3.8E-2
8.6E-3
1.4E-1
1.4E-1
2.0
1.4E-1
1.4E-1
1.4E-1
3.8E-1

-------
Table 6.6  Annual radiation dose equivalents due to atmospheric radio-
           active participate and Rn-222 emissions from a model average
           underground uranium mine
Organ
Red marrow
Endosteal
Pulmonary
Muscle
Liver
Stomach wall
Pancreas
LLI wall
Kidney
Bladder wall
ULI wall
SI wall
Ovaries
Testes
Spleen
Uterus
Thymus
Thyroid
Weighted mean -
Waximum
Individual
(mretn/yr)
5.1E-1
7.2
2.9
1.2E-1
3.5E-1
2.0E-2
1.1E-1
9.4E-2
9.1E-1
6.4E-2
4.3E-2
2.0E-2
1.1E-1
1.1E-1
1.4
1.1E-1
1.1E-1
l.IE-1
1.1
Average
Individual
(mrem/yr)
8.3E-4
1.2E-2
5.0E-3
' 2.3E-4
7.2E-4
2.8E-5
2.2E-4
1.8E-4
2.0E-3
1.2E-4
7.3E-5
2.8E-5
2.2E-4
2.3E-4
3.1E-3
2.2E-4
2.2E-4
2.3E-4
2.0E-3
Population
(person-rem/yr
2.9E-2
4.1E-1
1.8E-1
8.3E-3
2.7E-2
l.OE-3
8.0E-3
6.5E-3
7.4E-2
4.4E-3
2.7E-3
l.OE-3
8.0E-3
8.0E-3
l.IE-1
7.9E-3
8.QE-3
8.1E-3
7.1E-2

-------
                                                                6-10
Table 6.7 Annual radiation dose equivalents due to atmospheric radioactive
          particulate and Rn-222 emissions from a model average large
          underground uranium mine
Organ
Red marrow
Endo steal
Pulmonary
Muscle
Li ver
Stomach wall
Pancreas
LLI wall
Kidney
Bladder wall
ULI wall
SI wall ,
Ovaries
Tes tes
Spleen
Uterus
Thymus
Thyroid
Weighted mean
Maximum
Individual
(mrem/yr)
4.2
6.0E+1
2.5E+1
9.7E-1
2,9
1.7E-1
9.4E-1
7.8E-1
7.7
5.4E-1
3.6E-1
1.6E-1
9.2E-1
9.4E-1
1.2E+1
9.2E-1
9.4E-1
9.4E-1
9.8
Average
Individual
(mrem/yr)
6.9E-3
9.6E-2
4.7E-2
1.9E-3
6.0E-3
2.3E-4
1.8E-3
1.5E-3
1.7E-2
l.OE-3
6.0E-4
2.3E-4
1.8E-3
1.8E-3
2.6E-2
1.8E-3
1.8E-3
1.9E-3
1.8E-2
Population
(person-rem/yr
2.5E-1
3.5
1.7
6.9E-2
2.2E-1
8.5E-3
6.8E-2
5.5E-2
6.2E-1
3.6E-2
2.2E-2
8.4E-3
6.6E-2
6.8E-2
9.2E-1
6.6E-2
6.7E-2
6.8E-2
6.2E-1

-------
                                                                6-11
Table 6,8 Annual radiation dose equivalents due to atmospheric radioactive
          particulate and Rn-222 emissions from a model inactive surface
          uranium mine
Organ
Red marrow
Endosteal
Pulmonary
Muscle
Liver
Stomach wall
Pancreas
LLI wall
Kidney
Bladder wall
ULI wall
SI wall
Ovaries
Testes
Spleen
Uterus
Thymus
Thyroid
Weighted mean
Maximum
Individual
(mrem/yr)
2.1E-1
2.9
9.5E-1
5.6E-2 •
1.4E-1
1.5E-2
5.4E-2
4.4E-2
3.5E-1
3.3E-2
2.4E-2
1.4E-2
5.2E-2
5.5E-Z
5.3E-1
5.2E-2
5.3E-2
5.5E-2
3.9E-1
Avtrage
Individual
(mrem/yr)
4.8E-4
6.8E-3
5.0E-4
1.8E-4
5.5E-4
1.1E-5
1.8E-4
1.4E-4
1.5E-3
9.2E-5
4.7E-5
1.3E-5
1.8E-4
1.8E-4
2.3E-3
1.8E-4
1.8E-4
1.8E-4
4.7E-4
Population
(person-rem/yr
6.9E-3
9.8E-2
7.2E-3
2.6E-3
7,8E-3
1.6E-4
2.6E-3
2.0E-3
2.1E-2
1.3E-3
6.7E-4
l.BE-4
2.5E-3
2.6E-3
3.3E-2
2.5E-3
2.5E-3
2.6E-3
6.8E-3

-------
                                                                6-12
Table 6.9 Annual radiation dose equivalents due to atmospheric radioactive
          particulate and Rn-222 emissions from a model inactive underground
          uranium mine
Organ
Red marrow
Endosteal
Pulmonary
Muscle
Liver
Stomach wall
Pancreas
LLI wall
Kidney
Bladder wall
ULI wall
SI wall
Ovaries
Testes
Spleen
Uterus
Thymus
Thyroid
Weighted mean ..
Maximum
Individual
(mrem/yr)
' 5.8E-2
8.0E-1
2.7E-1
1.6E-2
3.9E-2
4.0E-3
1.5E-2
1.2E-2
9.7E-2
9.1E-3
6.6E-3
3.7E-3
1.4E-2
1.5E-2
1.5E-1
1.4E-2
1.5E-2
1.5E-2
1.1E-1
Average
Individual
(mrem/yr)
9.3E-5
1.3E-3
3.4E-4
2.9E-5
7.9E-5
5.2E-6
2.8E-5
2.2E-5
2.1E-4
1.6E-5
l.OE-5
4.9E-6
2.7E-5
2.8E-5
3.2E-4
2.7E-5
2.8E-5
2.8E-5
1.5E-4
Population
(person-rem/yr
3.4E-3
4.6E-2
1.3E-2
l.OE-3
2.8E-3
1.8E-4
l.OE-3
8.0E-4
7.6E-3
5.8E-4
3.7E-4
1.8E-4
9.7E-4
l.OE-3
1.2E-2
9.8E-4
l.OE-3
l.OE-3
5.7E-3

-------
                                                                6-13
Table 6.10  Annual  radiation dose equivalents due to atmospheric radioactive
            participate and Rn-222 emissions from a hypothetical in situ
            uranium solution mine
Organ
Red marrow
Endosteal
Pulmonary
Muscle
Liver
Stomach wal 1
Pancreas
LLI wall
Kidney
Bladder wall
ULI wall
SI wall
Ovaries
Testes
Spleen
Uterus
Thymus
Thyroid
Weighted mean
Maximum
Individual
(mrem/yr)
1.6E-1
2.8
3.9E+1
8.4E-3
1.9E-2
1.6E-2
7.6E-3
6.1E-1
3.3E-1
4.8E-3
2.0E-1
3.6E-2
7.3E-3
8.9E-3
4.6E-2
7.4E-3
7.9E-3
8.4E-3
1.2E+1
Average
Individual
(mrem/yr)
2.7E-4
5.0E-3
2.0E-2
2.2E-5
5.4E-5
5.7E-5
2.1E-5
2.5E-3
l.OE-3
1.2E-5
8.1E-4
1.4E-4
2.1E-5
2.2E-5
1.8E-4
2.1E-5
2.1E-5
2.1E-5
6.2E-3
Population
(person-rem/yr
3.8E-3
7.1E-2
2.9E-1
3.1E-4
7.7E-4
8.1E-4
3.0E-4
3.5E-2
1.5E-2
1.6E-4
1.2E-2
2.0E-3
3.0E-4
3.1E-4
2.5E-3
3.0E-4
3.0E-4
3.1E-4
8.8E-2

-------
                                                                    6-14
   alent rates*  due  to atmospheric  radioactive participate and  Rn-222 emis-
   sions from the model  uranium mine  sites are presented in Tables 6.4 through
   6.10. The  Rn-222  dose equivalent rate  is  only for the  inhalation  and  air
   immersion pathways and excludes  Rn-222 daughters.  The  impact  from Rn-222
   daughters is  addressed  separately with  a  working level  calculation.   The
   dose  equivalent estimates  are for the  model  sites described  for  use with
   the AIRDQS-EPA code  in Appendix  K.   Assumptions about food  production  and
   consumption  for the maximum  individual  were  selected for a  rural  setting.
   The maximum  -individual  dose  equivalent  rate  occurred  about  1600  meters
   downwind  from the center of  the  model  site.   The  term  "population" refers
   to  the population  living  within a radius  of 80 kilometers of  the  source.
   Population dose equivalents  are  the sum of  the exposures  to all  individuals
   in  the exposed  population  for  the  annual  release  from the model  uranium
   mine.
        Dose equivalent  rates  in  Tables  6,4  through 6.10  indicate  that the  red
   marrow,   endosteal  cells,   lung,   kidneys,  and   spleen  are  generally  the
   highest exposed  target organs.  A  dose  equivalent rate is presented  for  the
   "weighted mean" target organ,  but this  calculated  result was not  used  in
   the health effect calculations.   We  calculated  "weighted mean"  dose equiv-
   alents  by using  organ  dose  equivalent  weighting factors (see Appendix  L)
   and summing  the results.   The weighted  mean  dose equivalent rate was pre-
   sented instead  of the total  body dose equivalent rate.
        Individual  lifetime fatal  cancer risks  and estimated additional fatal
   cancers to the  regional population due  to atmospheric  radioactive emissions
   from  the  model  uranium mine sites are presented  in  Tables  6.11 and 6.12.
   The  individual  lifetime risks  in Table  6.11 are  those  that would  result
   from  one  year  of  exposure (external  and internal)  and  the working  levels
   estimated  for those  individuals.   Except for the  in  situ leach mine,  the
   individual  lifetime  risks  in Table 6.12  are  those  that would result  from a
   lifetime  of  exposure (71 years  average  life expectancy).  The individual
   lifetime  risks in Table 6.12 for  the  in situ  leach  mine  are based on an
  exposure  time of 18  years,  which is the expected life, including  restor-
  ation, of this type of model uranium mine.
     *The dose equivalent rates were not used to calculate risk and are only
presented for perspective purposes.  Risks of health impact were calcu-
lated directly from external and internal radionuclide exposure data.

-------
                                                                  6-15
     Table 6.11   Individual  lifetime  fatal  cancer  risk  for one year  of  exposure
                  and estimated  additional fatal  cancers  to the regional  popula-
                  tion due  to annual radioactive  airborne emissions from model
                  uranium mines
Source
Maximum
Exposed
Individual
Average
Exposed
Individual
Regional
Population
Average  surface mine

     Participates and Rn-222       6.7E-7
     Radon-222 daughters           5.5E-6
     Total                         6.2E-6

Average  large surface mine

     Participates and Rn-222       3.7E-6
     Radon-222 daughters           1.9E-5
     Total                         2.3E-5

Average underground mine

     Particulates and Rn-222       1.6E-7
     Radon-222 daughters           1.1E-5
     Total                         1.1E-5

Average large underground mine

     Particulates and Rn-222       1.4E-6
     Radon-222 daughters           1.1E-4
     Total                         1.1E-4

Inactive surface mine

     Particulates and Rn-222       8.5E-8
     Radon-222 daughters           4.2E-7
     Total                         4.7E-7

Inactive underground mine

     Particulates and Rn-222       1.5E-8
     Radon-222 daughters           2.7E-7
     Total      -                  2.8E-7

In situ leaching  facility -

     Particulates and Rn-222       1.6E-6
     Radon-222 daughters           1.1E-5
     Total                          1.3E-5
 7.5E-10
 1,1E-8
 1.2E-8
3.7E-9
4.1E-8
4.5E-8
2.8E-10
4.9E-8
4.9E-8
2.5E-9
5.0E-7
5.0E-7
6.4E-11
8.3E-10
8.9E-10
2.0E-11
1.2E-9
1.2E-9
8.7E-10
2.1E-8
2.2E-8
 1.1E-5
 1.6E-4
 1.7E-4
 5.4E-5
 5.9E-4
 6.4E-4
l.OE-5
1.7E-3
1.7E-3
9.0E-5
1.8E-2
1.8E-2
9.1E-7
1.2E-5
1.3E-5
7.4E-7
4.4E-5
4.5E-5
1.2E-5
3.0E-4
3.1E-4

-------
                                                                  6-16
      Table 6.12  Individual  lifetime fatal  cancer risk due  to  lifetime exposure
                  to radioactive  airborne emissions from model  uranium mines
      Source
                            Maximum
                            Exposed
                          Individual
 Average
 Exposed
Individual
                                                                  (c)
 Average  surface mine^  '
      Particulates  and  Rn-222
      Radon-222  daughters
      Total
 Average  large  surface
      Particulates  and  Rn-222
      Radon-222 daughters
      Total
Average underground
      Particulates  and  Rn-222
      Radon-222  daughters
      Total

Average large underground mine
      Particulates  and  Rn-222
      Radon-222  daughters
      Total

Inactive surface mine*  '
      Particulates  and  Rn-222
      Radon-222  daughters
      Total

Inactive underground mine^
      Particulates  and  Rn-222
      Radon-222  daughters
      Total

In situ leaching facility* '
      Particulates  and  Rn-222
      Radon-222  daughters
      Total
                      (a)
                            1.4E-5
                            1.2E-4
                            1.3E-4
                           6.6E-5
                           3.5E-4
                           4.2E-4
                           3.5E-6
                           2.0E-4
                           2.0E-4
                           2.5E-5
                           1.9E-3
                           1.9E-3
                           3.9E-6
                           3.0E-5
                           3.4E-5
                           1.1E-6
                           1.9E-5
                           2.0E-5
                           1.6E-5
                           2.0E-4
                           2.2E-4
 1.6E-8
 2.3E-7
 2.5E-7
 6.6E-8
 7.4E-7
 8.1E-7
 5.8E-9
 9.0E-7
 9.1E-7
 4.4E-8
 8.6E-6
 8.6E-6
4.5E-9
5.9E-8
6.3E-8
 1.4E-9
 8.5E-8
 8.6E-8
8.7E-9
3.8E-7
3.9E-7
     * 'Considers exposure for 17 years to active mining and 54 years to
inactive mine effluents. -
     (b)

     (c),
Considers exposure for 71 years to inactive mine effluents.
        Considers the average individual in the regional population within an
80-km radius of the model mine.
     (d)
          Considers 10-year operation and 8-year restoration.

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                                                            6-17
Table 6.13     Genetic effect risk to descendants for one year of parental
               exposure to atmospheric radioactive airborne emissions from
               model uranium mines
Source
Descendants of
Maximum Exposed
Individual
{effects/
birth)
Descendants of
Average Exposed
Individual
(effects/
birth)
Descendants of
Regional
Population
(effects/yr)
Average surface mine
Average, large surface mine
Average underground mine

Average large underground mine
Inactive surface mine
Inactive underground mine
In situ leach facility
6.3E-7
3.7E-6
1.4E-7
t
1.1E-6
6.0E-8
1.6E-8
8.0E-9
2.6E-9
1.3E-8
2.9E-10

2.4E-9
2.4E-10
3.4E-11
2.7E-11
1.6E-5
7.9E-5
4.4E-6

3.6E-5
1.4E-6
5.0E-7
1.6E-7

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                                                                      18
     Table 6.14     Genetic effect risk to descendants for a 30-year parental
                    exposure to atmospheric radioactive airborne emissions from
                    model uranium mines
                                                     Effects/birth
     Source
 Descendants of
Maximum Exposed
   Individual
Descendants of
Average Exposed
  Individual^
Average surface mine* '
Average large surface mine'
Average underground mine
Average large underground mine^ '
Inactive surface mine^ '
Inactive underground mine^
In situ leach facility^ '
1.2E-5
6.4E-5
2.6E-6
2.0E-5
1.8E-6
5.0E-7
1.4E-7
4.6E-8
2.21-7
5.4E-9
4.0E-8
7.2E-9
5.8E-10
4.8E-10
    • ^'Considers exposure to 17 years active mining and 13 years inactive
mine effluents.
     (b)
        Considers exposure for 30 years to inactive mine effluents.
     (c)
     x 'Considers the average individual  in the regional  population within an
80-km radius of the model  mine.
     (d)
        Considers 10-year operation and 8-year restoration.

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                                                                  6-19
      Genetic effect risks due to atmospheric radioactive emissions from the
 model uranium mine  sites  are presented in Tables 6.13 and 6.14.   The risks
 to descendants in Table  6.13 are those that, would  result from one year of
 exposure to the parent or parents of first generation individuals.   The de-
 scendant risks in Table  6.14 are those that would result from 30 years ex-
 posure to  the  first generation  parent  or parents,  except for the  in  situ
 leach mine where we used  an 18-year exposure time.   The 30-year time period
 represents  the  mean  years of  life where  gonadal   doses are  genetically
 significant.
      We estimated  the health impact  risks  v/ith  the DARTAB code  using ex-
 posure data  from the AIRDOS-EPA code.   The dose equivalent and  risk  con-
 version factors that we used with the  DARTAB code are tabulated in Appendix
 L.   The sou-atic  risk  conversion  factors are based on  a  lifetime (71 years
 average lifetime)  exposure time,  and  the  genetic  effect ri<»k  conversion
 factors are based on  a 30-year  exposure time.   When  the  exposure time for
 calculated risks was only  one year,  we calculated the  risk by multiplying
 the risk calculated by OARTAB with the ratio of  the  one year  exposure  time
 to the exposure  times used to  calculate the risk conversion  factors (1/71
 for somatic effects and  1/30  for genetic  effects to  descendants  of maximum
 and average exposed individuals).*  Appendix L  contains a discussion of the
 health risk assessment methodology.
      We developed  several  tables to  present the calculated health  impact
 risk.   The  percentage  contributions to the fatal cancer risks  for indi-
 vidual  sources  at each model uranium mine site are contained  in  Table  6.15
 for the maximum  individual  and  Table 6.16 for  the average individual.   The
 fatal  cancer risks  by  source term for one  year  of exposure which  we  used  to
 calculate  percentage contributions  are contained in  Tables  L.4  to L,6  in
 Appendix  L.  Tables  L.7 to  L.9 contain  genetic  risks  by source  term  at  each
 model  uranium  mine site.   The   percent  of  the  fatal cancer  risk due  to
 radon-222  daughter  concentrations at model  uranium mine  sites  is  indicated
 in  Table  6.17.  The percent  of the  fatal cancer risk  for  principal  nuclides
 and  pathways due to radioactive  particulate and Rn~222 emissions at  each
 model uranium mine site are  contained in Table 6.18.
     *A  correction  factor  was  not needed  for OARTAB  calculated genetic
effects committed per year to the regional population.

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     Table  6.15      Percent  of the fatal  cancer risk for the maximum Individual
                    due  to the sources  of radioactive emissions  at model  uranium
         '           mines
Percent of fatal cancer risk ' ' '
Mining
Mine type Activities
Average surface mine
Average large surface mine
Average underground mine
Average large underground mine
Inactive surface mine
Inactive underground mine
In situ leach facility
56 (95)
59 (93)
80 (=100)
89 (=100)
28^ (100)
77(c) (100)
100 (87)
Ore
18 (66)
14 (41)
3 (79)
2 (76)
0
0
0
Sub-ore
14 (98)
12 (98)
17 (97)
9 (96)
0
0
0
Spoils
12 (89)
14 (86)
<1 (96)
<1 (96)
72 (84)
23 (77)
0
Vehicular
Dust
<1 (0)
1 (0)
<1 (0)
<1 (0)
0
0
0
       Table L.  4, Appendix L,


          in parentheses are percent contribution of radon-222 daughters.
^Emissions from abandoned pit (surface mine) or vents and portals (underground mine).
                                                                                                       IN3
                                                                                                       o

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     Table 6.16     Percent  of  the fatal  cancer risk for the average individual
                    In the regional  population due to the sources  of radioactive
                    emissions  at model  uranium mines
Percent of fatal cancer "isle3' '
Mine type ,
Average surface mine
Average large surface mine
Average underground mine
Average large underground mine
Inactive surface mine
Inactive underground mine
In situ leach facility
Mining
'Activities
58 (97)
60 (96)
81 {a 100)
89 (slQQ)
29^ (100)
80^ (100)
100 (96)
Ore
16 (78)
11 (64)
2 (93)
2 (91)
0
0
0
Sub-ore
14 (99)
12 (99)
16 (99)
9 (99)
0
0
0
Spoils
12 (93)
16 (92)
<1 (99)
<1 (99)
71 (90)
20 (92)
0
Vehicular
Dust
<1 (0)
1 (0)
<1 (0)
<1 (0)
0
0
0
(a)
(b)
(c)
See Table L.5» Appendix L.
Values in parentheses are percent contribution of radon-222 daughters.
Emissions from abandoned pit (surface mine) or vents and portals (underground mines).
                                                                                                          ro

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                                                                   6-22
          Table 6,1?     Percent of fatal cancer risks due to radon-222
                         daughter concentrations at model uranium mine
                         s i tes
           Source                   Percent fatal cancer risk
                                                             (a)
Average surface mine                              89
Average large surface mine                        84
Average underground mine                          99
Average large underground mine                    99
Inactive surface mine                             88
Inactive underground mine                         95
In situ leach facility                            8?
     ^'Remainder due to radioactive particulate and Rn-222 emissions.

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            Table 6.18     Percent of  the  fatal  cancer risk  for  principal  nucl ides  and  pathways  slue  to  radioactive
                           jj£tjc_u!ate  and Rn-22?  emissions  at model  urajjuinipnes_
Percent of fatal cancer risk
Internal Pathways
Mine Type
Average
Surface Mine /
•
Average Large
Surface Mine
j
Average
Underground Mine

Average Large
Underground Mine

Inactive . ,
Surface Mine18'

Inactive , ,
Underground Mine* '
In situ
Leaching Facility

Receptor
Max. Individual
Av. Individual
or population
Max. Individual
Av, Individual
or Population
Max, Individual
Av. Individual
or Population
Max. Individual
Av. Individyal
or Population
Hax, Individual
Av. Individual
or Population
Max. Individual
Av. Individual
or Population
Max. Individual
Av, Individual
or Population
Principal Nyclides
U-238(20.0), 0-234(22.1), Th-230{31.7T,
Ra-226[7.94), Po-210{7.33)
(J-Z38C9.I7), 0-234(10.1), Th-Z30(22.7) ,
fta-226{21.3), Pb-210(6.92), Po-2IO(22,4)
11-238(20.0), 11-234(22.2), Th-230(3l.8),
fta-226{7.98)
U-238(i.l9), 0-234(10,1), Th-23Q(22.7),
Ra-226(21.4), Pb-210{6.94)» Po-2lO(22.4)
U-238(17.9), U-234{19.8). Th-230(28.4),
Ra-226<7.14), Po-210(6.59), Rn-222(13.6)
U-238(12.0), U-234(13.2), Th-230{20.1),
Ra-226{7.24), Po-210(7.31), Rn-Z2Z{34.6)
U-238(17.5), U-234(19.3), Th-230(27.7),
Ra-226{6.97), Po-210{6.43), Rn-222(16.0)
U-238(1I.2), U-234C12.4), Th-230(18.8),
«a-226{6.76), Po-210{6.83), Rn-222(39.2)
U-238(19.5), U-234(2l.6}» Th-230(31.0),
«a^226{9.4), 81-214(5.31). Po-210(7.17)
U-238(8.76), U-234(9.68), Th-230{2L7)
R3-226E26.1), Pb-210(6.77), Po-210(2l.4)
U-238(19.6), U-234(21.6), Th-230(31.1),
Ra-226{9.45), Bi-214{5.33), Po-210C?.21)
U-238{17.0), U-234(18.8), Th-230(28.5J»
Ra-226{12,7), Bi-214{4.81), Po-210{10.4)
U-238(45.2), 0-234(50.0), U-235(2,2I)
U-238(43.3), U-234(47.BS, U-235(2.12)
Inges-
tion
15.8
60.1
15.9
60.5
14.0
16.9
13.6
15.7
1S.8
6Z.2
16.9
26.3
0.46
3.50
Inhal-
ation
80.2
38.1 |
80.0
37.7
82.5
80.6
82.9
82.0
75.4
34.3
75.2
66.6
99.5
96.5
External
Air
Immersion
0.003
0.005
0.002
0.004
0.025
0.063
0,029
0.071
0.002
0.003
0.001
0.004
0.002
0.009
Pathways
Ground
Surface
4.02
1.81
4.05
1.83
3.52
2.43
3.39
2.25
7.85
3.48
7.88
7.09
0.039
0.038
'Spoils source term only.

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                                                                  6-24
      The fatal  cancer health  risk  at each of the  model  uranium mine sites
 is  dominated  by the  lung  cancer  risk from radon-222 daughter exposures (see
 Table 6.17).    Radioactive particulates  and Rn-222 contributed  to  a  Tittle
 over 10 percent of  the total  fatal  cancer health  risk  at the model  surface
 mines and at the  in  situ  leaching  facility (see Table  6.11).   Essentially
 all  the risks  from  the model  underground mines  are due  to radon-222  daugh-
 ter exposures.   The fatal cancer health risks from the  active  model  under-
 ground  mines  are greater  than  the risks  from the active  model  surface mines
 because of the -larger quantity  of  Rn-222 released.  The  risks  are similar
 at  inactive surface  and underground  mines.
      The largest  fatal cancer risk  is  f'*om  the average  large  underground
 mine (see Tables 6.11 and 6.12)—an  estimated 1.9E-3 lifetime  fatal  cancer
 risk to the maximum exposed individual  for a lifetime exposure.  The life-
 time fatal cancer  risk to the  average individual in the  regional  population
 is  estimated  to be  8.6E-6  for a lifetime  exposure period.  The number  of
 estimated  additional  fatal  cancers  in the  regional population per year  of
 mine operation  is  estimated to be 1.8E-2.
      For the  active  surface mines,  about 60  percent of the  radon  daughter
 impact  is from  the  exposed  pit surfaces  (see Table L.4).  For the  active
 underground mines,  the predominate  radon daughter  impact  is  from mine vent
 air.  For  the inactive surface mine,  about  70 percent of  the  radon  daughter
 impact  is  from  waste rock pile exhalation and about 30 percent was  from the
 pit  interior  surfaces.   About  80 percent  of  the radon  daughter  impact for
 the  inactive underground mine  was due to  radon releases  from  the mine  vents
 and  entrance.   The release of  radon from  the pregnant leach surge tanks was
 the  predominate source of  the radon  daughter  health impact risk  for the
 model  in  situ  leach  mine.    Detailed  percentages  of  the  lifetime   fatal
 cancer  risks  by source term  for each model uranium mine are contained  in
 Tables  6,15 and 6.16.
     The  health impact from particulate  radionuclides and Rn-222 was pre-
 dominately due  to U-238 and daughter radionuclides  (see Table 6.18).  Thor-
 ium-232  and daughters  were  only minor contributors to  the particulate and
 Rn-222 fatal cancer risk with  Rn-222 only contributing significantly  (14  to
40 percent) at  active  underground mines.   The majority  of the exposure  to
individuals around  the model  uranium mines is  received from the  internal
pathways.   Inhalation  was the most  important internal  pathway except for
the   average  individual and  regional  population  impact  at  surface  mines

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                                                                  6-25

 where ingestfon was the major pathway (see Table 6,18),  For active surface
 mines,  about 52 percent of the participate and Rn-222 impact to the maximum
 individual   was  from  the  ore  source  term,  and  about 25  percent of  the
 health  impact was  from  the  mining activities source term  (see Table  1.4).
 For active underground  mines,  between  28 and 46 percent of the particulate
 and Rn-222 impact  was  from  the ore source term  and  between 25 and 41 per-
 cent of the particulate and  Rn-222 impact was from the  sub-ore  source  term.
 The predominant  source  of the  particulate and  Rn-222  impact  from  the  in~
 active  mines was particulate  radionuclides in wind-suspended dust  from  the
 waste rock  pile.  The  release  of particulate  radionucl1des  from the uranium
 recovery plant was the  predominant  source of the particulate health impact
 risk for the model  in  sity leach mine.
      For perspective,  the calculated fatal cancer risks can be compared  to
 the estimated cancer  risk from  all  causes.   The  American Cancer  Society
 estimates  the risk of cancer  death  from  all  causes to  be 0,15  (Ba7i).   The
 maximum exposed  individual around the  model  average  large  underground mine
 is  estimated  to  incur an additional lifetime fatal  cancer risk of 0.0019
 (1.3 percent) due  to  radioactive airborne emissions from  the  model mine.
 There  is  a  regional  population of 36,004 persons for the model   average
 large underground mine site located in New Mexico.  The cancer death rate
 for the State of New  Mexico  for whites of both  sexes  was  154.5 deaths  per
 year for 1973 to 1976  per 100,000 people  (NCI78),  Applying this statistic
 to  the  regional  population, about 56 cancer  deaths are estimated  to occur
 each year in  the  regional  population from  all   causes.   Applying the  approxi-
 mate  fatal  cancer  risk  coefficient of 0.15  to  the regional population of
 36,004  persons,  about  5,400 people  in the regional area would normally die
 of  cancer.   About 0.018 additional cancer deaths  (0.00033  percent) in the
 regional  population are estimated  per  year  of  operation  from  radioactive
 airborne emissions  at  the model average large  underground mine.
     The risk  of genetic effects from  radiation  exposure at model  uranium
 mine  sites  is very small  compared to  the  normal  occurrence of hereditary
 disease. The national  incidence of genetic effects is 60,000 per 10  births
 (MAS72). The normal occurrence of hereditary disease for the descendants of
 the  regional  population  of 14,297 at the  model  average large surface mine
 in  Wyoming  is 0.06 effects  per birth  and 12.1 effects  per year,  based on
202  live  births  per year  in  the regional population.  (We present  sta-
tistics  for  the  site  of the average large surface mine since  the largest

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                                                                  6-25
 genetic risk  for all the  evaluated model  uranium  mines occurred  at  this
 site [see Tables 6.13 and  6.14]).   We  estimated the genetic  effect  risk to
 the descendants  of  the  maximum  exposed individual  to be  an  additional
 6.4E-5 effects/birth (0.1 percent  increase)  for a 30-year exposure  period.
 The genetic  effect  risk to  the descendants of the average exposed indi-
 vidual in the regional population  is  estimated to be an additional 2.2E-7
 effects/birth (0.00036  percent  increase)  for  a  30-year exposure  period.
 The number  of  additional genetic  effects  committed to the descendants  of
 the regional population  per year  of operation  of  the average large  surface
 mine is estimated to be  7.9E-5.   The  additional committed genetic  effects
 constitute a very  small  increase  to  the 12.1  effec.,s  that will normally
 o(-ur  each year  in  the live  births  within the regional population.

 6 1,2      Nonradioactjve  Airborne  Emissions
     To calculate atmospheric  concentrations at  the  ""ocation of the  maximum
 individual,  we used  the data on  nonradioactive air pollutant emissions from
 Section 3.   We compared  these pollutant  air concentrations with calculated
 nonoccupational  threshold limit values,  natural background concentrations,
 and average  urban  concentrations  of  selected  airborne  pollutants  in  the
 United States.
     The  "natural"   background  atmospheric concentration has  been  defined
 (Va7J)  as  the concentration of  pollutants in areas absent of activities by
 man which  cause  significant pollution.   Variations in background levels may
 result  from  differences   in  mineral content of  the  soil, vegetation,  wind
 conditions,  and  the  proximity to the ocean or metropolitan areas.   Based on
 an  extensive literature  survey and  consideration of the abundance and dis-
 tribution of the  chemical elements  in the ocean and earth's crust, a set of
 "natural"  background airborne  concentrations  has  been developed  for  the
 United  States   (Va71).    Natural  background airborne  concentrations  for
 selected pollutants  are   listed  in the second  column of Table 6.19.  Also
 listed  in  the. table  are  average concentrations of  airborne  pollutants in
 urban  areas.   The latter are arithmetic  mean  concentrations  obtained  from
 measurements taken over a period of several years (Va71).

6.1.2.1  Combustion Products
     Airborne  concentrations  of combustion  products released from  diesel
and gasoline-powered  equipment were estimated for the site of  the maximum

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                                                                     27
           Table 6.19  Natural background concentrations and average urban
                      concentrations of selected airborne pollutants in
                      the United States
                              Natural Background -          Average Urban   -
Pollutant                     Concentration, p g/m        Concentration, p g/rn"


Gases

CO                -            100                           7000
NO                             40                            141
NH*                            10                             80
SO                              5                             62
CO*                       594,000, ,                          NR
Hydrocarbons                   NRW                         500


Suspended particles
Total
As
Ba
Cd
Co
Cr
Cu
Hg
Fe
Pb
Mg '
Mn
Mo
Ni
Se
Sr
Th
U
V
Zn
Zr
20 - 40
0.005
0.005
0.0001
0.0001
0.001
0.01
0.0005
0.2 - 0.5
0,001
0.1
0.01
0,0005
0,001
0,001
0.005
0.0005
0.0001
0.001
0.01
0.001
105
0.02 ( 1)
NR
0.002
0.0005
0.015
0.09
0.1
1.58
0.79
NR
0.1
0.005
0.034
NR
NR
NR
NR
0.05
0.67
NR
   NR - Not Reported.
Source: Va71; except for CG~,  Ba76,

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                                                                  6-28
 individual.   The  concentrations  were  computed  using  the  annual  release
 rates  given in Tables  3,30  and  3.52 with dispersion  parameters  applicable
 for the model underground  (New  Mexico)  and  surface (Wyoming) mining  areas
 (Appendix   K).   The  estimated  combustion  product concentrations  are  low
 compared  to  the  natural  background  and  average urban  concentrations  (see
 Table  6.20).   A conservative threshold  limit  value (TLV) was computed,  as
 described  in Section  6.1.2.3 for S02>  CO,  and N02.   Of these pollutants,
 only  the nitrogen  oxide  concentrations  at  the average large surface  mine
 exceed  the  ngnoccupational   TLV.   Considering  these  comparisons  and  the
 conservative  nature  of  the analyses,   combustion products  released  from
 heavy  uranium  mining  equipment  do  not  appear  to pose a  health  hazard.

 6,1.2.2   Nonradioactive  Gases
     Airborne concentrations of  the three  principal  nonradioactive  gases
 released  from  the  hypothetical  in  situ  leach mining  site  were computed
 using  the source  terms from Table  3.59  and the meteorological   parameters
 and dispersion  model  described in Appendix  K.   Table  6.21  shows the  esti-
 mated  atmospheric  concentrations at  the  location  of  a maximum individual;
 occupational  threshold limit values  (TLV's);  adjusted TLV's  applicable  to
 nonoccupational exposures; and the percent the  estimated concentrations are
 of  the  adjusted  TLV's.  The  occupational  TLV's  have been  conservatively
 adjusted. They  were  adjusted on  the basis of  a 168-hr  week,  instead of a
 40-hour week  and a safety factor of  100.
     The  results  of  this analysis indicate  that  two  of the estimated  con-
 centrations  fall  below their respective  TLV's,  and   the concentration  of
 ammonium  chloride  is  approximately equal  to its  TLV.  Considering the
 conservative  nature  of the adjusted nonoccupational TLV on which the com-
 parisons were made,  none of  the nonradioactive gases  appear  to   be at con-
 centrations that might pose a serious health hazard.   The ammonia level  is
 about  80  percent of  the estimated  "natural"  background concentration and
 only  about  10  percent  of  the  average  urban  concentration  (Table  6.19).

 6.1.2.3   Irace Metals  and Parttculates in the  Form of Dust
     We identified seventeen trace metals and  particulates in the  form  of
dust as potential  airborne emissions from uranium  mines.  Table  6.22 pre-
 sents   projected airborne  concentrations of  the metals and  particulates  at
 the site of  the maximum individual for six mine classifications.  As might

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     Table  6.20   Combustion  product  concentrations at the site of the maximum individual

                 with  comparisons, pg/m

Pollutant
Particulates
of combustion
S0x
CO
NOX
Hydrocarbons
Average
underground
mine
1.4E-3
1.2E-2
9.7E-2
1.6E-1
1.6E-2
Average large
underground
mine
1.6E-2
1.3E-1
1.1 E+0
1.8E+0
1.8E-1
Average
surface
mine
9.7E-2
5.5E-1
4.3E+0
7.1E+0
7.1E-1
Average large
surface
mine
4.5E-1
2.2E+0
USE-f-1
3.0E+1
3.1E+0
Natural
background
concentration
NR(C)
5E+Q
l.OE+2
4.0E+1
NR
Average
urban
concentration^ '
NR
6.2E+1
7.0E+3
1.4E+2
5.0E+2
Non-
occupational
TLV(b)
NR
3.1E+1
1.3E+2
2.1E+1
NR
U)

(b)

(c)
See Table 6.19.
Nonoccupational TLV = TLV (mg/m3) x 40 hr/168 hr x 10"2 x 103 pg/mg (ACGIH76).
   NR - Not reported.
                                                                                                             i
                                                                                                            r\>

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                                                                 6-30
Table 6.21     A comparison of the airborne concentrations of nonradioactive
               gases it the hypothetical  in situ leach site with threshold
               1imit values


Contaminant
NH3
NH4C1
co2
Atmospheric
Concentration' '
Ug/m3)
8.1
24
60

TLV{bJ
(mg/m )
18
10
9000
Non-
(c)
occupations 1 v '
TLV (yg/m )
43
24
21,400
Percent of
Nonoccupational
TLV
19
100
0.3
     (a)
     (b)
Location of maximum individual.
        Source:  ACGIH76.
     ^Nonoccypational  TLV = TL¥  (mg/rn3)  x  40  hr/168  hr  x  10~2  x  103  pg/mg,

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                                                                  6-31

 be expected, large surface mine emissions usually have the greatest concen-
 trations, and  those  from Inactive underground mines  the  least.   Projected
 metal concentrations  range from a low  of  about  5 x  10"  ygm/m   of cobalt
                                                              3
 frum  inactive  underground  mines  to  a  high of about  1 ygm/m  of potassium
 from large surface mines.
      Table 6.23 shows where  particulates (dust)  or trace metal air concen-
 trations are  estimated  to exceed  natural  background or  average  urban  air
 concentrations (Table 6.19).   Several  trace metal  air concentrations exceed
 "natural" background; however,  only the  estimated  air concentration of par-
 ticulates (dust)  exceeds  the air  concentration  of airborne pollutants  in
 urban areas.
      We   evaluated  the  significance  of  these  concentrations  by  comparing
 them  with  threshold  limit  values (TLV's)  for workroom  environments  pub-
 lished  by  the  American  Conference of  Governmental   Industrial  Hygienists
 (AC6IH76).   These TLV's, which are  for  occupational  workers and a  40-hour
 workweek, were  adjusted  by multiplying  by  40/168 to convert  them  to  con-
 tinuous  exposure values and dividing by 100 to make  them  applicable to  the
 general  public.  Table  6.24 is  a  tabulation  of  the adjusted  TLV's,  the  pro-
 jected concentrations of metals and  particulates  (from Table 6.22),  and  the
 ratio of  these concentrations  to  the  adjusted TLV's.   The sums of  these
 ratios provide  a  measure of whether  a   mixture  of the metals would be a
 significant  problem,  a  sum  greater than  one  indicating that  the "composite"
 TLV  has  'been exceeded.
      Table  6.24 shows that in  no  case  does a single  metal  exceed  its TLV,
 nor  do any of  the mixtures  exceed a "composite"  TLV.  Although TLV's were
 not  available  for potassium and  strontium,  their  low  toxicity  and  low con-
 centrations  make it unlikely that their  addition  to  the  sums  would  change
 this  conclusion.   For the  worst case,  large surface  mines, the  sum of
 ratios is only  about  17  percent of the limit.
      Particulates, on the other hand, present a different  picture.  The TLV
 for  nonspecific particulates,  nuisance  dust, was  chosen for comparison. It
 can  be seen  that^the TLV is exceeded by  a factor  of six at  the large model
 surface  mine and nearly exceeded at the  average model surface mine.  About
 50%  of the  exposure  to  dust is from vehicular traffic,  and about 30% re-
 sults  from mining activities within the pit.
      In summary, specific trace metal airborne emissions from uranium mines
do not appear   to  present a significant  hazard,   either  singly or as com-

-------
Table 6.22     Stable truce metal airborne concentrations  at  the  site of  the maximum
 '              individual, ug/m
Trace
metal
AS
fia
Co
Cu
Cr
Fe
Hg
K
Hg
Mn
Ho
Ni
Pb
St
Sr
V
Zn
Part(b
Av§. undsr-
ground mine
3.1E-5
5.1E-4
4.0E-6
3.3E-5
5.0E-S
9.7E-3
7.2E-6
1.3E-2
9.4E-4
7.1E-4
3.3E-5
4.9E-6
4.1E-5
3.1E-5
1.7E-4
4.7E-4
2.6E-5
J 1.2
Avg. large
underground mine
1.9E-4
i.ae-3
3.1E-5
l.SE-4
1.4E-4
4.1E-2
1.5E-5
6.3E-2
6.91-3
2.8E-3
2.3E-4
3.9E-5
2.0E-4
2.2E-4
5.5E-4
3.0E-3
9.6E-5
3.9
Avg. surface
mine
2.6E-4
7.0E-3
1.1E-5
4.4E-4
1.1E-3
1.4E-1
1.8E-4
1.7E-1
2.SE-3
I.IE-2
1.4E-4
1.4E-5
5.4E-4
1.2E-4
3.4E-3
2.2E-3
4.6C-4
2.3E*1
Avg. large Inactive under-
surface mine ground mine
1.5E-3
4.2E-2
4.7E-S
?.6E-3
6.9E-3
B.5E-1
1.1E-3
1.0
l.OE-2
6.8E-2
6.7E-4
5.8E-5
3.2E-3
5.9E-4
2.1E-2
1.8E-2
2.8E-3
1.4E+2
3.1E-6
3.6E-S
4.5E-7
2.2E-6
8.9E-7
6.3E-4
N^a)
9.8E-4
1.3E-4
3.7E-5
4.5E-6
8.9E-7
3.1E-6
4.SE-6
4.9E-6
5.4E-5
1.3E-6
3.9E-2
Inactive surface
mine
1.5E-5
1.6E-4
2.9E-6
I.1C-5
3.6E-6
2.7E-3
NA
4.4E-3
6.2E-4
1.7E-4
2.0E-5
3.6E-6
1.4E-5
1.9E-S
2.3E-5
2.5E-4
S.2E-6
1.7E-1
 *b'
      - Not available.
   Part. - Particulates (dust).

-------
                                                                 6-33
Table 6.23     Comparison of stable trace metal airborne concentrations at the
               location of the maximum individual with natural background con-
               centrations and average urban concentrations of these airborne
               pollutants
ExceedNatural Background
                         (a)
Exceed Average Urban Concentration
                                  (a)
Average Large Surface Hjne
Ba» Cr (possible), Fe, Hg (possible),
Mn» Ho, Pb» Sr, V,
participates
     Participates
Average Surface Mine
Ba, Cr (possible), Mn, V
     None
Average Large Unde rground Ml ne
V
     None
Average Underground Mine
None
     None
     (a)
          See Tables 6.19 and 6.22.

-------
Table 6 24     Comparison of trace metal airborne concentrations at ^.he site of the maximum individual  with threshold limit values

               (TLV's) in the workroom environment adjusted for continuous exposure to the general  public,  ug/«
Trace
metal
As
Ba
Co
Cu
Cr
fs
Hg
i.'
Kg
Mn
Mo
Ni
Pb
Se
Sr
V
Zn
Total
. , • Average
Adjusted^ ' Underground Mine
TLV
1.2
1 2
0 24 i
0.48
1 2
12
0.12
w(-b}
24
12
12
0.24
0,36
0.48
NA
1.2
12
of ratios
Participates:
Oust 24(c)
Cone Cone /TLV
3 1E-5
S.1E-4
4.0E-6
3 3E-5
5E-5
9.7E-3
7.2E-6
1.3E-2
9.4E-4
7. 11-4
3.3E-5
4.9E-6
4.1E-S
3.1E-5
1.7E-4
4.7E-4
2.6E-5

1. 2E+Q
3E-5
4E-4
2E-5
7E-5
4E-5
8E-4
6E-5
__-
4E-5
6E-5
3E-6
2E-5
1E-4
6E-5
—
4E-4
2£-6
2E-3
5E-2
Average Large
Underground mine
Cone. Cone /TLV
1.9E-4
1.8E-3
3.1E-S
1.5E-4
1.4E-4
4.1E-2
1.5E-5
6.3E-2
6 9E-3
2.8E-3
2.3E-4
3.9E-5
2.0E-4
2.21-4
5.5E-4
3.0E-3
9.6E-5

3.9E+0
2E-4
2E-3
l£-4
3E-4
1E-4
3E-3
1E-4
— -
3E-4
2£-4
2E-5
2E-4
6E-4
5E-4
—
2E-3
8E-6
1E-2
2E-1
Average
Surface Mine
Cone. Cone. /TLV
2.6E-4
7 OE-3
1.1E-5
4 4E-4
1 1E-3
1.4E-1
1.8E-4
1 7E-1
2.5E-3
1.1E-2
1.4E-4
1.4E-5
5.4E-4
1.2E-4
3.4E-3
2.2E-3
4 6E-4

2.3E+1
2E-4
61-3
5E-5
9E-4
91-4
1E-2
2E-3
--
1E-4
9C-4
IE- 5
6E-5
2E-3
2E-4
—
2E~3
4E-5
3E-2
1E+0
Average Large
Surface mine
Cone Cone /TL','
1.5E-3
4 2E-2
4.7E-5
2.6E-3
6 9E-3
8.5E-1
1.1E-3
l.OE+0
l.OE-2
6.8E-2
6.7E-4
5.BE-5
3 2E-3
5.9E-4
2.1E-2
1.8E-2
2.8E-3

1.4E+2
1E-3
4E-2
2£-4
5E-3
6E-3
7E-2
9E-3
—
4E-4
6E-3
6E-5
2E-4
9E-3
1E-3
..
2E-2
2E-4
1.7E-1
6E+0
Inactive
Unde^g round mine
Cone Cone. /TLV
3 1E-6
3 6E-5
4 5E-7
2.2E-6
8 9E-7
6.3E-4
NA
9 8E-4
1 3E-4
3. 7£-5
4.5E-6
8.9E-7
3.1E-6
4.5E-6
4.9E-6
5.4E-5
1.3E-6

3.9E-2
3E-6
3E-5
2E-6
5E-6
7E-7
5E-5
	
	
SE-6
3E-6
4E-7
4E-6
9E-6
9E-6
—
4E-5
1E-7
2E-4
2E-3
Inactive
Surface mine
Cone.
1.5E-5
1 6E-4
2.9E-6
1.1E-5
3 6E-6
2 7E-3
NA
4.4E-:
6.2E-4
1.7E-4
2 OE-5
3.6E-6
1.4E-5
1.9E-5
2.3E-5
2.5E-4
5.2E-6

1.7E-1
Conc./TLtf
1E-&
1E-4
IE- 5
2E-5
3E-6
2E-4
._
--
3E-5
ie-5
2E-6
2E-5
4E-5
4E-5
..
2E-4 a
4E-7 S
7E-4
7E-3
     '"'Adjusted TIV = Occupational TLV (mg/m3) x 40 hr/lfiShr x 103  fig/mg x 1/100.
     (b)
     (c)
NA ~ Not available.
Limit for nuisance dust - total mass.
     Source: Morkroom TLV's from ACGIH76.

-------
                                                                  6-35

 posite mixtures, when  evaluated against  adjusted threshold  limit values.
 However,  particulate  emissions,  at  least for surface  mines,  require further
 evaluation.  If  model  predictions can  be  verified by  measurement, control
 measures  are  indicated.

 6.1.3      Radioactjye Aquatic  Emissions
     We  used  the  data  on  radioactive  releases from mine dewatering  (Sec-
 tions  3.3.3  and 3.4.3)  to estimate  the  public  health  impact of mining
 operations  at a typical active  underground  mining site (New Mexico)  and  a
 typical  active  surface mining site  (Wyoming),   The health  risks  estimated
 in  this  section are of  fatal  cancers  and  genetic  effects to  succeeding
 generations.   Dose equivalents  and  health  risks  per  year  of active  mine
 operation are  estimated for the  maximum  and  average individuals  and for the
 population  of each assessment area.  These  calculated  dose  equivalents and
 health risk estimates are believed to be higher than  the actual  dose equiv-
 alents and health risks because  of the conservative ass .ptions  required to
 predict  movement of  radionuclides  in surface  waters  (see  Section J.2 of
 Appendix  J).   Very  few data  are  available on aquatic  releases from  inactive
 mines; hence,  the significance of these  releases,  particularly for  Colorado
 and  Utah  where  inactive   mines are  numerous, could  not  be  determined.
     The  individual  and population dose equivalents  presented in this  sec-
 tion are  computed  using the models and parameters discussed in Appendix J.
 The  health  risk  estimates are generated   by  the  following   procedures:
   a.   For inhalation or ingestion of radionuclides, the quantity
        of radionuclides taken into the body is  determined as part
        of the dose equivalent calculations.  This quantity  is mul-
        tiplied  by a  health  risk  per unit intake conversion  factor.
   b.   For external  irradiation  from ground deposited  radionuclides
        or from  air submersion,  the dose equivalents are calculated
        and multiplied by a  health risk per  unit dose equivalent con-
        version  factor.
 The  health risk per  unit  intake and  health  risk per unit external   dose
 equivalent  conversion factors  for  aquatic  releases  are listed  in Tables
 J.13 and  J.14,  Appendix J.  This appendix  also discusses  the health  risk
 assessment methodology  used to obtain the risks presented in this section.
Uranium and Ra-226  releases are  given for both active mining sites.  It is
assumed that the stated  uranium  releases are entirely  U-238 and that U-234
is in  equilibrium  with the U-238 but that  Th-230 precipitates  out of the

-------
                                                              6-36
Table 6.25     Annual radiation dose equivalent rates due to aquatic releases
               from the New Mexico model underground mine
Organ
Endosteal
Red Marrow
Lung
Liver
Stomach Wall
LLI Wall^
Thyroid
Kidney
Muscle
Ovaries
Testes
Weighted Mean
Maximum Individual
Dose Rate (mrem/y)
5.6E+1
2.0
1.3
5.5E-1
1.9E-1
9.4E-1
4.5E-1
2.8E-H
4.9E-1
4.1E-1
4.7E-1
2.2
Average Individual
Dose Rate (mrem/y)
5.0
1.6E-1
2.1E-3
2.9E-2
3.8E-3
6.6E-2
2.5E-2
2.4
2.5E-2
2.4E-2
2.4E-2
1.5E-1
Population Dose
Rate (person-rem/y
3.2E+2
1.1E+1
1.4E-1
1.9
2.5E-1
4.3
1.6
1.6E+2
1.6
7.8E-1
7.8E-1
9.9
         large  intestine  wall

-------
                                                                    6-37
Tible 6.26     Annual radiation dose equivalent  rates  due  to  aquatic releases
               from the Wyoming model  surface mine
Organ
Endo steal
Red Marrow
Lung
Liver
Stomach Wall
LLI Wall{a)
Thyroid
Kidney
Muscle
Ovaries
Testes
Weighted Mean
Maximum Individual
Dose Rate (mr&n/y)
• 6.8E-1
3.8E-2
2.3E-2
3.0E-2
l.OE-2
2.9E-2
1.8E-2
4.0E-1
1.9E-2
1.5E-2
1.8E-2
4.0E-2
Average Individual
Dose Rate (rnrem/y)
2.1E-1
7.4E-3
l.OE-4
2.8E-3
2.8E-4
7.7E-3
1.4E-3
1.1E-1
1.5E-3
1.5E-3
1.4E-3
7.1E-3
Population Dose
Rate (person-rern/y
3.4
1.2E-1
1.7E-3
4.5E-2
4.6E-3
1.3E-1
2.3E-2
1.8
2.4E-2
1.2E-2
1.2E-2
1.2E-1
     ^a'Lo,wer large intestine wall

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Table 6.27     Individual lifetime fatal cancer risk and committed fatal cancers to the population
               residing within the assessment areas

Source


Underground
mine site
(New Mexico)
Surface mine
Site (Wyoming)
Maximum exposed individual Average exposed individual
lifetime fatal cancer risk lifetime fatal cancer risk
for operation of the mine for operation of the mine

1 yr. 17 yrs. 1 yr. 17 yrs.

3.3E-7 5.6E-6 2.0E-8 3.4E-7


7.1E-9 1.2E-7 9.6E-10 1.6E-8

Cpmraitted fatal cancers
for the assessment area
population for operation
of the mine
1 yr. 17 yrs.

1.3E-3 2.2E-2


1.6E-5 2.7E-4

        'The average  individual  risk  is the  cumulative  population  risk divided by  the  population
residing within the  assessment  area.
                                                                                                                   CJ
                                                                                                                   CD

-------
                                                                  6-39
 Also, it fs  assumed  that  Rn-222,  Pb-214,  Bi-214, Pb-210, and Po-210 are in
 equilibrium with the Ra-226.   For example,  a reported release rate of 0.01
 Ci/yr of U-238 would be reflected  in  the analyses as 0.01  Ci/yr of U-238
 and  0.01  Ci/yr  of U-234.   In like manner,  a release  of 0.001  Ci/yr  of
 Ra-226 would be  reflected  in the  analyses as  0.001 Ci/yr  Ra-226,  0.001
 Ci/yr Rn-222, 0.001 Ci/yr Pb-214, 0.001 Ci/yr Bi-214, 0.001  Ci/yr Pb-210,
 and 0.001 Ci/yr Po-210.
      The maximum individual,  average individual,  and population annual  dose
 equivalent  rates 
-------
                                                                  6-40
 (Table 6.27).  This  represents  a 0.00023 percent  increase  in  the expected
 fatal  cancer occurrences  in  the assessment area population  as  a  result of
 operation of  the  underground mine  in New  Mexico  over  its  17-year active
 life.   For  the Wyoming  assessment  area  (16,230  persons), the  estimated
 increase  in the expected  fatal  cancer deaths due  to  operation  of the sur-
 face mine for 17 years is  0.000011 percent.
     Table 6.28 presents  the genetic risks to succeeding  generations,  for
 exposure  to both  individuals  and the population  within the assessment area,
 caused by  mine dewatering  radionuclide  releases.   The  genetic  risks  to
 succeeding generations of maximum and  average exposed individuals (columns
 2 and  3,  respectively) and the committed  genetic  effects to the  descendants
 of the present population within the assessment area (column 4)  are shown
 for one year of releases.  The  mechanics and assumptions  used  to estimate
 the genetic  effects  are  similar to  those used to  estimate fatal  cancer
 risks  (see Appendix  J).   For both  the model  underground  (New  Mexico)  and
 surface (Wyoming) mines the majority of the risk  is from releases  of U-238,
 U-234,  and  Po-210.
     The  risks  of  additional  genetic  effects  due to   the discharge  of con-
 taminated mine water  from  model  uranium mine sites  are very small  when com-
 pared  to  the normal  occurrence of hereditary diseases.  As  given in  Section
 6.1.1,  the  natural   incidence  of genetic  effects is  60,000  per  million
 births  (NAS72),  or 0.06 effects  per birth.  This natural  incidence  rate  is
 equivalent to 848 effects  per year per  million persons,  considering  a  birth
 rate of 0.01413  births per person-year.   Taking  the  New Mexico site  as  an
 example,  the  normal  incidence  of genetic  effects  for the assessment area
 population  (64,950  persons)  during  the 17 years of  operation  of  the mine
 would be 936 genetic  effects.  The increase in genetic effects committed  to
 the  assessment  area  population  during the 17 years  of  operation  is  0.015
 genetic effects  committed.   Thus,  the genetic  effects committed  due   to
 aquatic wastes  released  during the  operation of the New Mexico  underground
mine are  only^ 0.0016% of the  genetic effects  which occur due  to  other
causes  during the  mine operating life.   For the  Wyoming site (16,230 per-
 sons),   the  genetic  effects committed due to aquatic wastes released during
the  operation  of  the model  surface  mine are only 0.0001% of  the  genetic
effects which occur  due  to other causes during the mine operating life.  It

-------
Table 6.28     Genetic risks to succeeding generations of an individual  and committed genetic effects
               to descendants of the present population residing within the assessment area
     Source
Genetic effects committed to succeeding
generations of an individual for operation
of the mine for 1     '
                    Maximum Individual
                         Average Individual
                    Genetic effects committed to the
                    descendants of the present population
                    for operation of the mine for 1 year
Underground mine
site (New Mexico)
     4.5E-7
3.3E-8
9.0E-4
Surface mine
site (Wyoming)
     1.4E-8
2.0E-9
1.4E-5
     ^Genetic effects assume 1 birth per person.

-------
                                                                  6-42
 should  be  noted  that genetic  effect  risks  to  descendants of  individuals
 cannot  be added  to somatic  effect  risks  for these individuals.

 6.1.4      Ngnradioactive  Aquatic Emissions
     Data on  nonradlological  emissions  from uranium mines  via the  water
 pathway are  limited.   Table 6.29  presents available estimates of  concen-
 trations  of  four  trace  metals plus  sulfate and  suspended solids  in  dis-
 charge  streams from  the  model surface  mine located  in Wyoming and  seven
 trace metals plus sulfate and  suspended  solids  from the model  underground
 mine  located  in  New Mexico.  These  concentrations  are  calculated  after
 dilution  in the first order tributaries  (Appendix J) and represent  average
 concentrations  for the assessment  areas.   The  concentrations presented  in
 Table 6.29 are conservative since, with  the  exception of sulfates,  loss  of
 contaminants due  to precipitation, adsorption, and infiltration to  shallow
 aquifers  are not  considered.  The concentrations  are calculated  by diluting
 discharges  from a  mine into  the first  order surface streams with no  losses.
 For sulfate,  a more realistic approach is taken since only 20 percent  of  it
 Is  assumed  to  remain  in  solution  in  the  surface  stream,  as discussed  in
 Section 3.3.3.1.4.
     Also  presented  in Table 6.29  are recommended  agricultural  water  con-
 centration  limits for livestock  and   irrigation  for  several  of  these  ele-
 ments  (EPA73).   Drinking  water limits  are  not presented  because  public
 water supplies are normally derived   from  groundwater  rather than  surface
 water,  so drinking water  would not be a pathway  of concern for  the  average
 individual  in the assessment  area.  Though drinking water would  be a po-
 tentially  significant  pathway  for the maximum individual,  the  data  avail-
 able for  this analysis did not allow  a  reliable  prediction of groundwater
 concentrations due to  mine dewatering  (Appendix  J).  For  this  reason, the
 impact  of nonradioactive  waterborne emission on  the  maximum  exposed  indi-
 vidual   could not  be  evaluated.   The  ratios  of   the  average  water concen-
 trations  to  these  limits  are also  listed in  Table  6.29 and show that only
molybdenum  from   the  underground  mine approaches its  limit  (irrigation).
 Also,  the  sums  of the ratios being less than one indicate that mixtures of
 the metals  would  not  exceed a "composite limit"  for  an average individual
 in the  assessment area.

-------
Table 6,29     Comparison of nonradiological  waterborne emissions  from uranium mines  with
               recommended agricultural  water quality limits
Recommended Limits, mg/t


Livestock
Parameter
Arsenic
Barium
Cadmium
Molybdenum
Selenium
Zinc
Uranium
Sulfate
Total suspended solids
Totals

0.2
0.05
NA
0.05
25
NA
NA
NA


Model Surface Mine Model Underground Mine
Avg. Water Ratio Ratio, Avg./ Avg. Mater
Irrigation Cone., mg/t Avg. /Livestock Irrigation Cone., mg/i

0.1
NA
0.01
0.01
0.02
2.0
NA
NA
NA

Limit Limit
1.4E-4 0.0007 0.0014 3.1Er4
2.0E-2
1.1E-4 0.0022 0.011 1.6E-4
7.0E-3
1.6E-3
4.8E-4 0.00002 0.00024 1.1E-3
2.0E-3 3.5E-2
4.9 2.9
5.8E-1 6.8E-1
0.0029 0.013
Ratio' Ratio, Avg./
Avg. /Livestock Irrigation
Limit Limit
0.0016 0.0031
0.0032 0.016
0.70
0.032 0.08
0.00004 0.00055



0.037 0.80
lit
(b)
NA - Not available.
Excluding molybdenum.

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                                                                  6-44
      Because of  the  limited number  of  data available, it is  difficult'to
 evaluate the significance  of these discharges.  Although molybdenum  could
 be  a  problem,  it is not possible  to  quantify the risk from molybdenum to
 the maximum  individual  without  having  estimates  of  drinking water  con-
 centrations.  Uranium, the  metal  estimated  to be in highest concentration
 (Table 6.29), has no established  limits based on chemical toxicity  in the
 United States.  In Canada,  the  maximum acceptable concentration for uranium
 in  drinking  water based  on chemical  toxicity  has  been set  at  0.02  tng/£
 (0.04  mg/day),-considering  a continuous  lifetime  intake  rate of 2  liters of
 water  per day (HWC78).  It  is  reasonable  to assume that  limits for uranium
 in  water  used  for  irrigation  and  to  water  livestock would  exceed  the
 drinking water  limit. Hence, based on  the estimated uranium concentrations
 at  surface  (0.002 mg/£ } and underground  (0.035 mg/x, ) uranium mines,  the
 water  would probably be  icceptable  for irrigation  and livestock watering.
 The other constituents,  such as solids  and  sulfates,  for which limits  are
 not available, have minimal  or  no toxic  properties.
     It   is   premature  to   conclude   the  health  hazard  caused  by   non-
 radiological  waterborne emissions  from uranium mines.   Before definitive
 conclusions  can  be   reached,  additional   information  is  needed.   Of  par-
 ticular  interest would be data  on water  use  patterns in the vicinity of  the
 mines  and the degree to which the mine discharges may infiltrate ground-
 water  supplies.

 6.1.5     Solid Wastes
 6.1.5.1   Radium-226  Content
     Solid  wastes, consisting  of  sub-ore, waste  rock,  and  overburden, at
 active   and   inactive  uranium  mines  contain   elevated  concentrations  of
 radium-226.*  The  sub-ore may contain as much as  100  pCi/g  of  radium-226.
 Even though the overburden and waste rock contain lower concentrations than
 the sub-ore,  most of these wastes contain concentrations  of  radium-226 in
quantities  greater than  5  pCi/g  (see  Sections  3.3.1, 3.4.1,  3.7.1,  and
 3.7.2).
* The  radium-226  concentration in natural soil  and  rock  is about 1 pCi/g.

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                                                                 6-45
     Uranium mine wastes containing radium-226 in quantities greater than  5
pCi/g have been designated as "hazardous wastes" in a recently proposed EPA
regulation  (43FR58946,  December 18, 1978)  under the Resource Conservation
and Recovery Act (RCRA).  This is primarily due  to the fact that the use of
these  wastes  under  or around  habitable  structures could  significantly
increase  the  chance  of  lung  cancer to  individuals  occupying  these struc-
tures.

6.1.5.2   Estimates of Potential Risk
     We  have  estimated  the risk  of fatal  lung  cancer that could  occur to
individuals living  in houses built on  land  contaminated by uranium  mine
wastes  (Table  6.30).   Risks  were  estimated  for homes  built on  land  con-
taining  radium-226  soil  concentrations  ranging  from 5  to 30 pCi/g,   The
relationship between  the indoor radon-222 decay product  concentration and
the radium-226 concentration  in  soil  under a structure is  extremely  vari-
able and  depends upon many complex factors.  Therefore,   the  data  in  Table
6.30 only  illustrate  the  levels  of risks  that  could occur to  individuals
living in structures  built on contaminated land.  These  data  should not be
interpreted as establishing a firm relationship  between  radium-226 concen-
trations in soil  and indoor radon-222 decay product concentrations.

   Table 6.30     Estimated lifetime risk of fatal  lung cancer  to
                  individuals  living in homes built on land
                  contaminated by uranium mine wastes

Ra in Soil
(pCi/g)
5
10
20
30

Indoor Working Levels
(ML)
0.02
0.04
0.08
0.12
Lifetime Risk of
Fatal Lung Cancer'3'
(per 100 persons)
2.5
5.0
10
15
       Based  on an  individual  being  inside  the  home  75  percent  of  the  time,

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                                                                  6-46
      The  working  level  concentrations  In Table  6.30  were derived  from
 calculations  made  by  Healey  (He78),   who  estimated  that  1  pCi/g  of
 radium-226  in  underlying  loam-type  soil  would  result  in  about 0.004  WL
 inside a house with an  air change rate  of  0.5  per hour.  These calculated
 working levels are  in  reasonable  agreement with measurements made  by EPA
 (Fig. 6.1) at 21  house  sites  in Florida (S.T. Windham,  U.S. Environmental
 Protection  Agency,  Written Communication,  1980).    The  Florida data  were
 derived from  the  average  radium-226 concentration  in  soil   (core  samples
 were taken to a maximum depth of three  feet  at  each site) and  the  average
 radon-222  decay product  concentration inside each structure.

 6.1.5.3   Usjng Radium Bearing Wastes In  The Construction of  Habitable
           Structures
      Wastes  containing  elevated  levels   of  radium-226  have  been used  at  a
 number of  locations  in  the  construction  of  habitable structures.  In Grand
 Junction,  Colorado,   uranium  mill  tailings were widely  used as landfill
 under and  around the foundations  of homes and  other structures causing  high
 radon-222  decay product  concentrations  inside many structures.   To  remedy
 this  situation,  Public  Law 92-314 was passed in 1972  to establish  a  fed-
 eral-state remedial  action program to correct the affected structures.   In
 Mesa  County, Colorado, which includes Grand  Junction, uranium mill tailings
 were  identified at about 6,000 locations.  About  800  of these locations are
 expected  to  receive  corrective action  because the radon  decay   product
 concentrations inside  buildings constructed  at these  locations exceeded the
 remedial action criteria  (DOE79).  According to the criteria,  dwellings and
 school houses would be  recommended for remedial action  if the indoor radon
 decay  product concentration exceeded  0.01 WL above background; other struc-
 tures  would  be recommended  for remedial action  if  the indoor radon decay
 product concentration exceeded 0.03 WL above background.
      In central Florida, structures have been built  on reclaimed phosphate
 land.   The  reclaimed  land is  composed of phosphate mining wastes that con-
 tain elevated radium-226  concentrations.  EPA estimates that  about 1,500 to
 4,000  residential  or commercial  structures  are  located  on  7,500 acres of
 the  total   50,000  acres of  reclaimed  phosphate-mined  lands (EPA79).   A
 survey of 93 structures built on reclaimed phosphate land showed that about
40 percent  of  the structures  had  indoor radon-222  decay  product  concen-
trations in  excess of 0.01  WL and about 20 percent  had  concentrations in

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                                                                                6-47
    0.1
O)

cu
en
c
   0.01
o
o
TJ
C
  0.001
   I       I       i       I

        10             15

Radtum-226 in soil (pCi/g)
                                                              20
            Figure 6,1  Average indoor radon-222 decay product

                      measurements (tn working levels) as a function of

                      average radium-226 concentration in soil

-------
                                                                  6-48
 excess  of  0.03  WL  (EPA79).   Lifetime  residency  in  a  structure with  a
 radon-222 decay product concentration  of 0.03 WL could result in twice the
 normal 3 to 4 percent risk of  fatal  lung  cancer.
 6.1.5.3.1 Use of Uranjum MineHastes
      We do not  know  to  what extent  the wastes from uranium mines have been
 removed from mining sites  and  used  in local and  nearby  communities.   How-
 ever, while  surveying in  1972  for locations with  higher-than-normal  gamma
 radiation in  the  Western  States  to locate uranium mill  tailings  material
 used  in local communities,  EPA and  AEC identified more  than  500 locations
 where "uranium  ore"  was believed to  be   the  source of  the elevated  gamma
 radiation (ORP73).  The specific type of ore (mill-grade,  sub^ore, low-grade
 waste rock) was not determined as this was beyond the  scope of the survey.
 At  some locations, however, surveyors  attempted  to characterize the ore  by
 using such  terms  as  "ore  spillage,"   "ore  specimens,"  "low-grade  crushed
 ore," or "mine  waste dump  material.11   Some  locations  were identified  as
 sites of former  ore-buying  stations  (ORP73).
      Since  it  is  unlikely  that  valuable mill-grade  ore  would have  been
•widely available  for off-site use, we   suspect  that  uranium  mine  waste
 (perhaps sub-ore)  may be the  source of the elevated  gamma  radiation levels
 at  many of  the  locations  where large  quantities  of ore material  are  pre-
 sent.  Table  6,31 shows  the locations  where higher-than-normal  gamma  radi-
 ation levels  were detected during these  surveys  and the suspected  sources
 of  the elevated  levels.

 6.2   En v ir onmen t ajJEjff e cts
 6.2.1     General Considerations
      Minerals  are  necessary to  augment   man's  existence  and  welfare;  in
 order to obtain  them,  some  form of mining  is necessary.   The very nature  of
 mining  requires  disturbing  the land surface,  but may  be considered  tran-
 sitory.   To  discuss  the  environmental   effects of  uranium mining  in  partic-
 ular,  it is convenient to divide the  mining operations  into three  phases,
 The first  phase  includes the exploration  for,  and the  delineation  of, the
 ore body.   This  involves,  in   most  cases, substantial  exploratory and de-
 velopment drilling.  The  second phase involves  the preparation  of the mine
 site  and  the  mining process itself.  This phase  includes the construction
 of  service areas,  dewatering   impoundments, and  access  roads,  digging or
drilling  of mine entries,  etc.  During  the actual  mining  process, waste

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                                                                         6-49
          Table  6.31
Gamma  radiation  anomalies and  causes


Location
Arizona , ,
Cane Valleyw
Cameron
Cutter
Tuba Ci ty
State Total
Colorado^
Cameo
Canon City
Clifton
Coll bran
Craig
Debeque
Delta
Dove Creel'
Durango
Fruita
Gateway
Glade Park
Grand Valley
Gunnison
Lead vi lie
Loma
Mack
Mesa
Mesa Lakes
Mol ina
Naturita
Nucla
Palisade
Plateau City
Rifle
Sal Ida
Slick Rock
Uravan
Whitewater
State Total
Idaho
!Ba"ho City
Lowman
Salmon
Number of
Anomalies
Detected

19
3
5
17
44

3
187
1083
145
86
109
43
83
354
1276
17
1
110
47
91
199
90
123
3
43
33
13
939
28
810
64
9
209
55
6253

3
12
77
Cause of Anomaly
Uranium Radioactive
Tailings

15


7
22

1
36
159
4
8
2
1
59
118
58
12
1
10
3
18
10
6
I


10
3
107
1
168
6
3
208

1013


9
1
Ore

4
1
4

9


24
31
2
7

3
17
18
47
1

2
8
2
3
2
1


15
6
36

20
2
5

4
256



2
Source



1

1



3




2
49
1
1


1

1
1



5

3

7

1


75




Natural
Radioactivity




3
3


99
14

46
1
29
2
67
26



28
65
4




1
2
14

1
52


2
453

2
3
65

Unknown


2

7
9

2
28
876
139
25
106
10
3
102
1144
3

98
7
6
181
82
120
3
43
2
2
773
27
614
4

1
49
4456

1

9
State Total
92
10
70
10

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                                                                          6-50
T ab1e  6.31  (egntin ued)


Location
New Mexico
(Tfuewater
Gatnerco
Grants
Milan
Shiprock
State Total
Oregon
Lakeview
New Pine Creek
State Total
South Dakota
EJgemont
Hot Springs
Provo
State Total
Texas
Camp be 11 ton
Coughran
Falls City
Fashing
Floresville
George West
Karnes City
Kenecfy
Panna Mana
Pawnee
Pleasanton
Poth
Three Rivers
Til den
Whitsett
Number of
Anomalies
Detected

2
5
101
41
9
158

18
4
, 22

55
45
4
104

7
1
5
1
IS
10
10
22
3
1
21
15
5
11
I


Cause of Anomaly

Uranium Radioactive Natural
Tailings

1

7
5
8
21





43

3
46



2



2
1




1


Ore

1

49
23
1
74

2
1
3

2
3

5

1


1



1

1
1




Source Radioactivity


5
1 25
4 1
0
5 31

10

10

1 1
17
1
2 18

6
1
3

14
10
6
13
3

2 17
14
2
11
1
Unknown



19
8

27

6
3
9

8
25

33





2

2
7


1
1
2


State Total
129
101
15

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                                                                         6-51
Location
Utah
Blanding
Bluff
Ci sco
Crescent Junction
Green River
Magna
Mexican Hat
Mexican Hat
(Old Mill)
Hoab
MonticeTIo , »
Salt Lake City^ '
Thompson
Number of
Anomalies
Detected

38
2
2
2
23
27
5

- 14
125
59
225
30

Tailings

10



1
1


10
15
31
70
26

Uranium
Ore

21
1
2
1
14
1
4

1
76
16
10
3
Cause of
Anomaly
Radioactive Natural
Source Radioactivity






1
1

2
7
3
5
0

3



1
21


I
6

76


Unknown

4
1

1
7
3



21
9
64
1
State Total
State Total
552
164
 150
                      19
 16
                                             108
                                   16
                                                                                   111
Washington
C res ton
Ford
Reardan
Spring dale

3
1
10
2

3
1
10
2
Hudson
Jeffery City
Lander
Riverton
Shirley Basin
8
28
86
86
9

13
4
15
9
2
9
8
14


1
1
1

5
3
53
33

1
2
2Q
23

State Total
Totals
 217
7587
  41
1323
          33
537
                   107"
                                             94
                                            904
                                                                                    46
                                                                                  4716
             EPA report ORP/LV-75-2, August 1975.  Cane Valley was not included in initial
gamma survey program.
        Excluding Grand Junction where non-tailings anomalies were not sub-categorized
according to source.
     frl
     v 'Salt Lake City was not completely surveyed.
     Source: ORP73.

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                                                                  6-52
 plies  are  produced, mine  vents  drilled or  reamed,  and  pits opened  and
 sometimes closed.   In  the  third  or retirement  phase,  the site is  subject to
 deterioration  from  weathering  ad  infinitum.   The  extent  of the  deter-
 ioration  depends  somewhat  on the  amount and quality  of reclamation  con-
 ducted  during this phase.
 6,2.2      Effects  of Mine  Dewatering
     Both surface  and underground mines  are dewatered  in order to  excavate
 or sink shafts and  to  penetrate and remove  the  ore body.   Dewatering  is  by
 ditches,  sumpst and drill  holes within  the  mine or  by  high  capacity  wells
 peripheral  to the  mine and  associated  shafts.   Dewatering  rates up to  4 x
   5 3
 10  m /day  have been reported in the literature.  Average discharge for  the
 surface   and  underground  mines  modeled  herein  are  3.0 and  2.0  m  /min-
 ute/mine, respectively.   Between 33  and  72  new  mines are projected in  the
 San Juan  Basin of New Mexico alone.   Total  annual discharge  is expected  to
                 9   3
 exceed  1.48 x 10  m  ,  Calculated  effects include decreased flow in  the  San
             3                                3
 Juan (0.05 m /min} and the  Rio  Grande  (0.85 m /mm)  rivers.   Future mining
 will be  primarily  underground and  the average mine depth will  increase  275
 percent,  i.e.,  from 248 m  to 681 m.  Average mine discharge  is expected  to
                     3               3
 increase  from 2.42 m /min to  13.8 m  /min.
     Aside  from the hydraulic  and  water  quality effects  of discharging
 copious quantities of mine water to  typically ephemeral  streams, dewatering
 impacts are receiving  increasing scrutiny because of the observed and cal-
 culated  impacts on  regional  water  availability  and  quality.  Declines  of
 water  levels  in regionally-significant  aquifers  of New Mexico and  reduced
 base flow to  surface streams  are expected.  Water quality effects  relating
 to   inter-aquifer  connection  and  water  transfer as  a  result  of  both de-
 watering  and  exploratory drilling  have  not been evaluated  in any uranium
 mining  area.  In several  Texas uranium  districts,  the  effects  of massive
 dewatering  associated  with surface mining are beginning to receive atten-
 tion, but definitive studies have not yet  begun and regulatory  action  is
 not  expected  in the near future.   With respect to  in situ  leach mining,
 dewatering  is not necessary and hence is not a concern.  There is, however,
 some question concerning  the practice of  pumping large volumes of ground-
water to  restore  aquifers.  It is  likely  that both dewatering and aquifer
restoration practices will come under increasing State  regulation in water-
short areas,  particularly  in areas  of  designated   groundwater  basins  or
where aquifers  connect with  fully-appropriated  surface  streams.   The un-
certainties surrounding environmental impacts of mining  in this area can  be

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                                                                  6-53
 expected to  increase,  and additional, comprehensive  investigations  of the
 effects of mine dewatering  and  wastewater discharge are needed.   Expansion
 in Wyoming  and  Texas  surface and  in situ leaching operations  is  similar,
 and these areas  should  be included  in future  investigations.
      Uranium  in  water  removed  from  mines  through  deliberate pumping  or
 gravity flow is  extracted for sale  when  the concentration is  2 to  3 mg/£  or
 more.   If  there  is subsequent  discharge to  surface  water,   radium-22^  is
 also removed  down  to  concentrations of  2  to 4 pCi/t,  to comply with  NPDES
 permit conditions.  .Use  of  settling  ponds at the mines  also  reduces  total
 suspended solids  and may reduce  other dissolved constituents  as a  result  of
 aeration and coprecipitation. Seepage from such settling ponds  is  believed
 to be low and, therefore, environmentally insignificant  relative to ground-
 water.  Management of waterborne solid wastes is inconsistent  from  one mine
 to another.  In  some  cases,  the  solids are collected  and put in with  mill
 tailings, but in most  cases  they remain  at the mine portal and are covered
 over.
      For surface versus  underground  mines, we  recognize certain  inconsis-
 tencies  in  the  parameters  chosen  to   calculate  contaminant  loading  of
 streams.   Contaminant  loadings  from a  model  surface   uranium mine  were
 calculated  for uranium,  radium, TSS,  sulfate, zinc, cadmium, and  arsenic.
 As  noted  in  Section  3.3.1, molybdenum,  selenium,  manganese,  vanadium,
 copper,   zinc,  and  lead  are commonly  associated  with  uranium deposits!
        t
 however,  there tfere  too  few data  for the  latter elements  to  develop  an
 "average"  condition.   In  addition,   barium,  iron, and magnesium can  be
 abundant  in  New  Mexico uranium  deposits.   There were  insufficient  data for
 these  elements  in  the  case of  surface  uranium  mines  1n  Wyoming,   hence
 contaminant  loadings were not  calculated.   Regional  differences dictate
 which  parameters  are  monitored for baseline  definition  and NPDES purposes.
 Not  all  potential  contaminants  are  important  in  every  region.  For  this
 reason  and  others,  State and industry monitoring programs are inconsistent
 with  respect to  parameters.   Since the  scope of this  study did not permit
 extensive field surveys,  maximum reliance was  placed on  published,  readily-
 available data.
     In terms  of parameters and concentrations,  NPDES  permit limits are in-
consistent from  one EPA Region to another and  from one  facility to another
in a given Region.  In  part,  this reflects previous screening  of the efflu-
ent discharge  data  and  natural  variations  in the  chemistry of ore bodies.

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                                                                  6-54
 However,  the  inconsistencies  in   parameters  included  and  concentration
 limits are sufficiently large  as  to suggest Devaluating NPDES permits and
 specifying more  consistent  limits  that  more  closely reflect  contaminant
 concentrations and  volumes  of mine  discharge.
      Infiltration of most  of  the mine discharge in Wyoming  and  New Mexico
 is confirmed  by field  observations  from these States.   The modeling results
 agree with  these  field  data.   Furthermore,  the  modeling  results,  i.e.,
 maximum  infiltration,  are  consistent  with those in the  generic  assessment
 of uranium milling  (NRC79).   Potable  aquifers  are defined  under  the  Safe
 Drinking  Water Act as  those  which  contain  less  than   10,000  mg/£  TOS.
 Shallow  groundwater throughout the  uranium  regions  of the U.S.  meets  this
 criterion.
      Considering  that  essentially all  of  the mine  effluent infiltrates and
 is a  source of recharge to  shallow  potable aquifers, NPOES limits should  be
 influenced by the drinking  water regulations and ambient groundwater qual-
 ity.  The latter is essentially  never  considered  with  respect to mine  dis-
 charges. Extensive  use of soils in  both the  saturated  and unsaturated zones
 as sinks for  significant masses of  both water  and toxic  chemical  constit-
 uents originating  in the mine  discharge necessitates  further evaluation  of
 the  fate  of  these  elements.   Present  understanding  of  fractionation and
 resuspension  processes  affecting  stable  and  radioactive  trace  elements
 greatly  limits accurate prediction  of  health and  environmental  effects  of
 mine  discharge.

 6.2.3     Eros ionpfjifned.Lands and Associa ted Wastes
      Increased  erosion and sediment  yield  result  from  mining  activities
 ranging  from  initial exploration through  the  postoperative phase.    Access
 roads and  drilling pads and  bare piles  of  overburden/waste  rock and sub-ore
 constitute  the most significant  waste  sources.  Dispersal is  by  overland
 flow  originating  as  precipitation  and  snowmelt.  To a lesser extent, wind
 also  transports wastes and  sub-ore to the  offsite environment.  Underground
 mining  is much less  disruptive  to  the  surface  terrain  than  1s  surface
 mining.  Documentation  of  the  processes  and removal  rates  is  scarce  and
 consists  of  isolated studies  in Texas, Wyoming, and  New Mexico.  Conser-
 vatively  assuming that  sediment yields characteristic  of the  areas con-
 taining  the  mines  also apply  to  the  mine  wastes, yields of  overburden,
                                                3
waste  rock, ore,  and sub-ore amount to 90,000 m  per year.  Total  sediment

-------
                                                                  6-55
yield  from  all  mining  sources,  including  exploration  and  development
                                    fi   1
activities,  is estimated  at  6.3  x  10  ra .
     Actual  erosion  rates from specific sources  could  be  considerably  above
or  below  this value  owing to such  variables as pile  shape and  slope, degree
of  induration and grain size, vegetative cover,  and  local climatic  patterns
and cycles.  Slope  instability  does  present  serious  uranium mine  waste
problems  throughout  the mountainous uranium mining  areas of Colorado  (S.M.
Kelsey,  State  of Colorado,  written communication,  1979).   Field obser-
vations  in  four western  states  confirm  that  some erosion  characterizes
essentially  every pile but  that  proper  reclamation,  particularly grading
and plant cover, provides marked  Improvement and may  actually reduce  sedi-
ment loss  to below ore-mining levels.   Unstabilized  overburden,  waste  /ock,
and sub-ore  piles revegetate rather slowly, even in  areas of ample  rainfall
such as south Texas;
     Stable  trace metals  such as  molybdenum, selenium, arsenic, manganese,
vanadium,  copper, zinc,  and lead  are commonly associated with uranium ore
and may  cause deleterious  environmental  and  health effects.   Mercury and
cadmium are  rarely  present.  There is  no apparent relationship  between the
concentration of  trace metals and  ore grade.  In New Mexico ores, selenium,
barium, iron, potassium,  magnesium, manganese, and  vanadium are most  abun-
dant.  Presently, very  few  data  are available  to  characterize the  trace
metal .concentrations in overburden rock.  Results  of  trace metal   analyses
of  a  few  grab  samples from  several uranium  mines  in New Mexico and one in
Wyoming show that except for selenium, vanadium,  and arsenic, no signif-
icant  trend  attributable  to uranium  mining  was  present  (N.A.  Wogman,
Battelle   Pacific  Northwest  Laboratory,   Written  Communication,  1979),
Considering the background concentration for these elements and  the limited
number of  analyses,  the inference of offsite contamination  based  on  these
elements is  indefinite.
     Ore  storage  piles, used to hold ore at the mine for periods averaging
one  month,  are  .potential  sources  of contamination  to the  environment via
dusts  suspended   and  transported  by  the  wind,  precipitation  runoff, and
Rn-222 exhalation--all  of  which  can   be  significantly  reduced by proper
management.  Similarly,  spoil piles  remaining  as  a result of overburden,
waste rock,  or  sub-ore  accumulations  left on the land surface after mining
constitute a source of contaminants for transport by wind and water.  Waste
particles   enriched  in  stable and radioactive  solids and  Rn-222 can  be

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                                                                  6-56
 transported  by wind  and precipitation  runoff.   Such transport can  be  re-
 duced  through proper grading and  installation  of soil covers  protected  by
 vegetation or rip-rap.
     Soil  samples  collected from  ephemeral  drainage  courses  downgrade  from
 inactive  uranium  mines  in  New Mexico  and Wyoming  generally revealed  no
 significant  offsite movement of  contaminants (See Appendix  G}.   For  the  New
 Mexico  mines studied, Ra-226 was  elevated  to  about twice  local background
 at  distances of 100  to  500 meters from  the mine.  Water and  soil  samples
 from a  surface mining site in  Wyoming showed  no  significant  offsite move-
 ment of mine-related pollution  although  some local transport of stockpiled
 ore was evident  in drainage areas on and immediately adjacent to one mine
 pit.   The strongest  evidence  that mine wastes  are a source  of local  soil
 and water contamination is  the radiochemical  data and  uranium in  partic-
 ular.   Substantial disequilibrium between  radium and uranium may indicate
 leaching  and remobilization of  uranium, although  disequilibrium in  the ore
 body is also  suspect.

 6.2.4     Land Disturbance from  Exploratory  and  Devejopment Drill ing
     About  1.3 x  10  exploratory and  development drill  holes  have been
 drilled  through  1977 by the uranium  mining industry (see Section  3.6.1).
 Using  the estimated  land  area  of 0.51  hectares  disturbed  per drill hole
 (Pe79),  about 6.5 x  10   hectares  of  land  have  been  disturbed by drilling
 through 1977,  To  further  refine  the  estimates  of land areas disturbed, we
 reviewed  some recent drilling  areas  at  three  mine sites.   From observing
 187 recent  drill   sites, it  was concluded that  0.015 ±  0.006 hectares per
 drill  pad were physically  disturbed.  The  error term for the estimates is
 at  the  95 percent confidence  level.   The land  area  disturbed  by  roads to
 gain access  to the drill sites  was  also  estimated from aerial photography
 and amounts  to 0.17  ± 0.11 hectares.  The  error term for this estimate is
 also at  the  95  percent confidence level.  The total area  disturbed  per
 drill  site (drill   pad and access roads) is 0.19  ±  0.11 hectares.  Using the
 latter  estimates   from aerial  photography,  the  total land  area  disturbed
                                                                   2
 from all  drilling  through 1977  ranges from about 1000 to  4000 km  with a
                      2
mean of  about 2500  km  .  Drilling wastes  removed from  the  boreholes can
disturb additional land  areas  through  wind and water  erosion.  Ore  and
sub-ore  remaining  in  the  drilling  wastes  can, in  a  radiological  sense,
disturb land  areas around  the drill site  from  erosion.   The extent of the

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                                                                             57
 J *•„„* ^f^lfft CS    **« -i^J *iJ! Sfcl Ii/ A-**J j^. :^ ' "'-nJii fi
Figure 6 2  Example of natural reclamation of drill sites

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                                                                  6-58
 radiological  contamination at drill sites is not known and cannot presently
 be estimated.
      Some reversal  of the initial environmental damage at older drill sites
 was also observed  from  aerial  photographs.  Figure  6.2  contains  a typical
 medium-to-large surface uranium  mine  and some adjacent drilling areas that
 show the effects of weathering.  New drill sites are in the upper left-hand
 corner  of  the  photograph.   The  access  roads and  drill  pads  are  plainly
 visible. It also appears  that  exposed drilling wastes remain  at  the drill
 site.  The area left of center in the photograph shows drill  sites that are
 probably  Intermediate  in  age.  The  drilling wastes  remaining  have very
 little voluntary vegetation growing  on them, and appear  to  have  been sub-
 ject  to  wind erosion.  Weathering  of  the drill  puds  and access roads  is
 obvious, as they are  hardly discernible.  It appears, in these cases, that
 weathering may  be  considered  a natural reclamation  phenomenon.   Old  drill
 holes are located  in the lower left corner of the photograph.  The drilling
 wastes appear  to  be  isolated  dots;  the  drill  pads  and  roads are  almost
 indistinguishable  from the surrounding terrain.   It appears  that weathering
 and volunteer plant growth tend to obscure scarring  caused by roads  located
 in  relatively  level  areas.   In  Figure 6.3,  an underground  mine  site,  the
 access roads  to the  adjacent  drill   sites  required extensive  excavation
 because   of  the  topography.   These more severe excavation "scars"  will
 probably  remain  for a  long period of time.
      In  summarys the  average  number of drill  holes  per mine can be  esti-
 mated  by dividing  the total number of holes  drilled through 1977 by  the
 number of active and inactive mines in existence  in  1977;

         1.3 x  106 drill  holes   y    400 drill  holes.                 (6.1)
              3300 mines                    mine
    The total  land area  physically disturbed from  drilling  per mine is
        4°° drill holes  x 0.19 hectares x km2	  = 0.76  km
            <™™**™"™~~™~™11™™~™~''''~~'"~™   ~ J™~""^                      "  «
             -- mine         drill  hole     100 hectares    mine        (6.2)

 In  some   instances,  weathering  and  volunteer  plant growth (natural  recla-
mation)  tend  to restore the land  areas disturbed by drilling.  In  others,
especially  on rugged  topography where extensive  excavation has  occurred,
weathering may promote extensive  erosion  rather than natural -reclamation.
Any  ore   or sub-ore remaining  at the  drill  sites  is  subject  to erosion.

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                                                                  6-59
 6.2.5     Land Disturbance frog^ Mining
 6.2.5.1   Underground Mines
      At underground mines,  some  land area must be disturbed to accommodate
 equipment, buildings,  wastes,  vehicle  parking,  and  so  on.   The disturbed
 area may  range  widely  between  mines in the  same  area or in different geo-
 graphical  areas.   The  land  area  disturbed  by 10 mines  was  estimated from
 aerial  photographs.   Nine of the mines were in  New Mexico  and  one  was in
 Wyoming.   The disturbed  land area averaged  9.3 hectares  per mine site and
 ranged  from 0.89  to  17 hectares.   Access  roads for each mine site consumed
 about  1.1  hectares on the  average  and  ranged from 0.20  to  2.59 hectares,
 Subsidence or  the collapse  of  the underground workings also causes some
                                         2
 land disturbances.  An estimated  2.8 km  of  land has  subsided  as a  resul';
 of uranium mining  in New Mexico  from 1930-71  (Pa74).   A crude  estimate cf
 the  land  disturbed from  subsidence  per mine  can  be made by dividing the
 subsided  area  by  the  number of  inactive  underground mines  in New Mexico.
 This amounts  to about 1.5  hectares  per mine.  The total area  (mine  site,
 access  roads,  and subsidence) disturbed  by an underground mine is estimated
 to be 12 hectares.

 6.2.5.2   Surface Mines
     An estimate of land  disturbed  from surface  mining was  also  made from
 aerial  photographs of eight  mining  sites  in  New Mexico and  two  in Wyoming.
 The  area  estimates are for  a single  pit or a group  of interconnected  pits,
 including  the  area covered  by mine  wastes.   The average  disturbed area was
 estimated  to be  about  40.5  hectares and  ranged  from 1.1 to  154  hectares.
                                                          2
 Access  roads for the pits  averaged 2.95  hectares (0.03 km ) and ranged from
 0.18  to 18 hectares.   The total  area disturbed per mine site is about  44
 hectares.

 6.2.6      Retirement Phase
     The actual  exploration  and  mining  of  the uranium  ore  constitutes a
 very  small  portion of  the total  existence time of  a mine when considered
 over a  large  time  frame.  The natural forces  of erosion  and  weathering,  as
well  as plant  growth,  will  eventually change any  work or alterations that
man  has made on the  landscape.  For example, underground mines may  even-
tually  collapse  and fill  with  water if they are  in  a water table;  waste
piles erode and disperse in  the environment;  the sharp  edges  of pits become

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                                                       6-60
Figure 6.3  Inactive underground mine site.

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                                                                  6-61

 smooth from wind and water erosion; lakes that are produced in pits fill up
 with sediment; vents and mine entries collapse, etc.
      Perhaps  one  of  the  more  important  considerations  associated  with
 allowing a mine site to  be naturally reclaimed is the dispersal  of the mine
 wastes.   Their  removal  from  underground  and subsequent  storage on  the
 surface constitute  a  technological enhancement of  both  radioactive  mater-
 ials and  trace metals,  creating  a low-level radioactive materials disposal
 site.    It  appears  that  containment  of  the  wastes would be  preferred  over
 their dispersal. .Wastes from  underground mines deposited  near  the entries
 are  subject to substantial erosion.  - Figure 6.3 is  an aerial  photograph of
 an inactive underground uranium mine.   The large light area is  the  waste
 pile and the  small  pile nearby is a  heap-leach area.   Erosion is  occurring
 on both.  A possible  solution  to this problem is to minimize the  amount of
 wastes  brought  to  the  surface  by  backfilling  mined-out areas.  Another
 technique   to  minimize  the  dispersal of wastes  into  the  environment  by
 containment is to stabilize them.   Unfortunately,  a  substantial  quantity of
 wastes  from  past  mining  activities  have been  dumped  in  depressions  and
 washes,  which, in essence, enhances  their dispersion  into  the environment.
 In retrospect,  the  wastes should  have  been stored  in areas  where minimal
 erosion  would   occur  and then  covered with  sufficient  topsoil  to promote
 plant  growth.
      In  surface  mining, radiological  containment can  be  accommodated  by
 keeping  the topsoil, waste rock,  and sub-ores segregated during their  re-
 moval.   When backfilling, the materials  can be returned to the pit in  the
 order  they were removed  or in  an order  that would enhance  the radiological
 quality  of  the  ground surface.  In  this  manner,  the  wastes would be con-
 tained  and essentially removed from  the  biosphere.   Figure 6.4  shows some
 examples of  inactive and active surface mines.   Some weathering  and natural
 revegetation are  noticeable around  the inactive  pits.  Revegetation, on  the
 other  hand,  appears  to be relatively  sparse  at  other inactive  pits.
     Erosion in  inactive mining areas  in  New Mexico and Texas  can result  in
 deep  gullying  of mine waste  and overburden piles.   The mine wastes blan-
 keting the  foreground  oT Figure 6.5 are incised  by an  ephemeral  stream that
 has  been subsequently crossed  by  a  roadbed in  the  immediate  foreground.
 This particular mine,  located in the Mesa Montanosa area immediately south
 of Ambrosia  Lake, New Mexico, was  active  from  1957 to 1964.   Thus, erosion
occurred in  about 15 years.  In the  background  is a large mine  waste pile,

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                                                                  6-62
 the toe of which is being undercut by the same ephemeral  stream (Fig. 6.6).
 No  deliberate  revegetation  of the  mine wastes  dumped  in either  discrete
 piles or  spread  over the landscape  (Fig.  6.7}  is occurring,  due  in large
 part  to   the  unfavorable  physical   and  chemical  characteristics   of  the
 wastes.   The wastes are  devoid of organic matter and  are  enriched  in  stable
 and radioactive trace  elements,  some of which  are toxic  to plant  life.   Low
 rainfall   and  poor moisture  retention  characteristics  further  suppress
 vegetative growth.   As shown  in  Fig.  6.7, there  is  a  sharp contrast between
 the vegetative cover  on  mine  wastes versus that on  the  undisturbed  range-
 land  in the background.  Waste  rock from many if  not most of  the  mines  in
 New Mexico, Utah, and Colorado  is weakly cemented sandstone with  numerous
 shale partings.   Physical  breakdown  to  loose,  easily-eroded soil unsuitable
 for plant  life  is  common  (Fig.  6.8),   and  transport by overland  flow and
 ephemeral  streams occurs  both during  and  long  after the  period of  active
 mining  (Fig.  6.9).
      Depending  on the  degree of reclamation, if  any,  -inactive surface mines
 in  Texas  vary considerably in the degree of erosion  and  revegetation.  For
 example,  the deep gullying shown  in  Fig.  6.10 developed  in a period  of one
 year.   The mine wastes in this case  were not  contoured or  covered  to mini-
 mize  gamma  radiation, excessive  erosion,  or  revegetation.  In  fact,  the
 wastes were disturbed  and shifted very recently  in the course  of construc-
 ting  the  holding pond (for mine  water  pumped  from  an  active  mine  to the
 right  of  the  picture)  in  the background.  Drainage in  this  instance is
 internal,  i.e.,  to  a  holding  pond.   In the background are  more recent mine
 waste  piles  also  showing  deep  gullying,  scant  vegetation,  and  lack  of
 protective  soil covering.  Mine wastes  in Texas are not completely  returned
 to  the mine  primarily because of the  excessive cost.   As in  the case of
 most  mining operations,  the bulking  factor makes it physically impossible
 to completely dispose  of  the wastes  in  the mines.
     Surface mines  in  Texas,  particularly the older  ones,  also have  assoc-
 iated  overland  flow to  the  offsite  environment.  Shown  in Fig,  6.11 is a
 principal  channel  floored by unstabilized  mine  wastes  and draining  toward
 nearby  grazing  lands.   Numerous  deer and doves  also were observed in  the
 area  and  are activefy  pursued by  sportsmen.   The unstabilized mine in this
 photograph  was  last active several years ago,  but most activity stopped in
 1964.   Vegetation  has been  very slow to reestablish and is  essentially
limited to a very  hardy, drought-resistant .willow shown  in  the center of
the picture.

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                                                                      6 -  63

                                                                     ,-«  -c>s>  -y" a/ i«f*
Figure 6,4  Example of active and inactive surface mining activities

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                                                             6-64


Figure 6,5 Mine wastes eroded by ephemeral streams In the Mesa
           Montanosa area, New Mexico.

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                                                                   6-65

                           i^^wr^K^1 'sSH^s i*"*^* •J^^llSr;*^3;'f»*5^' -?*v^>T*
Figure 6 6  Basal erosson of a uranium  mine waste pile by an ephemeral
           stream in the Mesa Montanosa area, New Mexico.

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                                                                  6-66
Figure 6.7  Scattered piles of mine waste at the Mesa, Top Mine, Mesa
           Montanosa, New Mexico, Note the paucity of vegetation. Colum-
           nar object in background »s a ventilation shaft casing
Figure 6.8  Close-up view of easily eroded sandy and silty mine waste from
           the Mesa Top Mine, Mesa Montanosa, New Mexico

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                                                                      6-67
figure 6.9  Gullying and sheet erosion of piled arid spread mine wastes at
          the Dog Incline uranium mine, Mesa Montanosa, New Mexico,

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                                                                         6-68
                                »^t^r&*3^is£!!*&7* I-.-- r."ft*--: isr


Figure 6.10  Recent erosion of unstabtlized overburden piles at the inactive
             Galen mine, Karnes County, Texas
Figure 6.11   Unstabilrzed overburden piles and surface water erosion at the
            Galen Mine, Karnes County, Texas.

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                                                                  6-69
      Mines  stabilized  within the last few years feature improved final con-
 touring  and  use  of  topsoil  and seeding  to  stimulate revegetation.   The
 reclaimed  spoil  piles are  then available  for grazing.  Because  backfill
 cannot be  complete (due  to  economic  and bulking factors),  part of the mine
 pit remains  as shown  in Figs,  6.12  and 6.13, which are of  the same mine. The
 aerial view  shows  extensive  patches of light colored soil devoid of vegeta-
 tion.  Here  topsoil  is missing  and  revegetation is minimal despite  the 5
 years elapsed since mining.   Figure 6.13 is a  closeup of one portion of the
 mine showing  deep  gullying, a  thin  layer of dark  topsoil  over relatively
 infertile  sand  and  silt, and  the  vertical mine  walls.  Excavations  like
 this must be  fenced.  They  are a hazard  to :livestock  and  people.   It is
 likely that  erosion  will  continue to spread  away  from the mine;  but  the
 rate and consequence  is unknown.
      Although a  mine  site can  be  reclaimed to  produce an acceptable aesthe-
 tic  effect,  it may not  be suitable  in  a  radiological  sense.   At the conclu-
 sion of  surface mining,  the  remaining pit will contain exposed  sub-ore on
 some of  the  pit walls  and pit floor.   Because most mines  at  least partly
 fill  with  water and  the ore zone  is  thereby covered, gamma radiation  and
 radon diffusion  should  be  markedly reduced.  Although water  accumulation in
 the  pit  would be expected to  have  elevated concentrations  of  trace metals
 and   radioactive  materials,   this  condition  would   probably  be  temporary
 because of the eventual covering  of the  pit by sedimentation from  inflow of
 surface  water and  materials  sloughed  from the  pit walls.   The  natural
 reclamation  process  could be enhanced by  tapering the pit wjlls  to a more
 gradual slope and  depositing the materials  on the pit floor.   If  sub-ores
 are  allowed  to remain near  the  surface, gamma  exposure  rates may  be suffi-
 cient to prevent unlimited land  use and,  even  if  enough stabilizing mater-
 ials  were used to  suppress  the  gamma  radiation, radon exhalation  probably
 could  prevent unrestricted land use also.   Some of the possible  radiation
 problems could be reduced  by  separating  the waste  rock  and sub-ore when
 hauled to the surface.   The waste rock could  then be  used as a  blanket  for
 the  sub-ore.  Away  from  the  pit proper»  surface gamma readings must  be
 below 62 yR/hr to comply with Texas State  regulations. It is reasoned that,
 since  background is  about 5y R/hr, surface gamma radiation  of  57 yR/hr  or
 less would  cause a  total body dose of  500 mrem/yr  or  less.
     A number of the older  mines in  Texas  were  active  in  the late  1950*5
and  early  1960's—before there were  requirements for stabilization.  Such

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                                                                        6-70
Figure 612  Aerial view of the Manka Mine, Karnes County, Texas. Note
            the extent of the mine pit and associated waste piles with poor
            vegetative growth on bare wastes or those with insufficient top-
            soil cover.
 Figure 613  Overburden pile showing the weak vegetative cover and
            gullying associated with improper stabilization at the Manka
            Mine, Karnes County, Texas. Mine stabilized  m 1974

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                                                                  6-71
mines,  one  of which is shown in Fig. 6.14,  are  relatively  shallow,  contain
shallow  pools of  water,  and have  high associated  gamma  radiation on  the
order  of 80  to  100 ^R/hr and  as  much  las 140 to  250 pR/hr in some areas.
The  particular mine in Fig. 6.14  has maximum readings of  400wR/hr on  the
mine waste  piles.   In  addition, the mine  was used  for illegal disposal  of
toxic  wastes, primarily  styrene,   tars,  and  unidentified  ceramic  or  re-
fraction nodules.   Some of the drums containing  the  wastes  are shown in  the
rear center and right of the photograph.
     Mine wastes  may be  used  for construction  and  other  purposes if they
are  not  controlled or  restricted (see  Sections  5.4  and 6.1.5.3.1).  These
wastes  have  been  used  for fill  in  a yard  and park  (Appendix G).  Possibly
they have  also been used  1n a school   area  and  fairgrounds (Th79).  Their
use  in  dwelling construction  has  also been reported  (Ha74).   It is also
common  practice  to use mine  wastes  for  road  ballast and fill  in areas
around  mine  sites.  This  type  of  usage  is  evident from  the  roads Immed-
iately  adjacent  to and  located north  and  northeast of the mine shown  in
Fig. 6.3.
     In summary,  only about six percent of the land  used for uranium mining
has  been reclaimed from 1930-71 (Pa74),  For the  most  part, the wastes  at
the  mine sites are spreading  as  a result  of  weathering   and erosion.   It
appears that  the wastes can be controlled or disposed  of  by altering some
mining, practices,  which would  require  very little effort or expense on the
part of  the  mining industry.  Any reclamation of  the mine  sites should  be
keyed to  long-term, natural reclamation  that will  continue indefinitely.
Careful   planning   can  hasten the  natural   reclamation  process and  insure
long-term stability of the mine sites.   Measures should be  taken  to prevent
the removal  of mine wastes.

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                                                                       6-72


iiJtvsp&ap*
       Figure 614  Inactive Hackney Mine, Karnes County, Texas. Drums in back-
                 ground contained toxic liquid wastes and styrene. Mine was
                 active in late 1950's and early 1960,

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                                                                   6-73
6.3   References

ACGIH76   American  Conference of Governmental  and  Industrial Hygienists, 1976,
      "TLV's  - Threshold  Limit Values  for  Chemical  Substances and Physical Agents
      in  the  Workroom  Environment with Intended Changes for 1976,"  American Con-
      ference of Governmental and Industrial Hygienists, Cincinnati, Ohio.

Ba76   Baes, C.F.,  Goeller, H.E., Olson,  J.S.  and  Rotty, R.M. , 1976, "The Global
      Carbon  Dioxide Problem," Oak Ridge National Laboratory Report, ORNL-5194.

Ba79   Battist, L., Buchanan, J., Conge!, F.,  Nelson, C., Nelson, M., Peterson, H. ,
      and  Rosenstein,  M., 1979, Ad Hoc Population Dose Assessment Report, "Popu-
      lation  Dose and  Health Impact of the Accident at the Three Mile Island Nu-
      clear Station,"  A preliminary assessment  for  the period March 28 through
      April 7, 1979  (Superintendent of Documents, U.S. Government Printing Office,
      Washington, D.C.).

Be80    Begovich, C.  L., Eckeroan, K.F.,  Schlatter,  E.C. and Ohr, S.Y., 1980, "DAR-
      TAB: A  Program to Combine Airborne Radionuclide Environmental Exposure Data
      with Dosimetric  and Health Effects Data to Generate Tabulations of Predicted
      Impacts", Oak  Ridge National Laboratory Report, ORNL-5692 (Draft).

DOE79  U.S. Department of Energy, 1979,  "Progress Report on the Grand Junction
      Uranium Mill Tailings Remedial Action Program," DOE/EV-0033.

DOI68  U.S. Department of the Interior,  Federal Water Pollution Control Admin-
      istration, 1968, "Water Quality  Criteria:   Report of the National  Technical
      Advisory Committee to the Secretary of the Interior."

Du80   Dunning, D.E.  Jr., Leggett,  R.W. and Yalcintas, M.G.,  1980,  "A Combined
     Methodology for  Estimating Dose  Rates and Health Effects From Exposure to
      Radioactive Pollutants," Oak Ridge National Laboratory Report,  ORNL/TM-
     7105.

EPA73   U.S.  Environmental  Protection Agency,  1973, "Water Quality Criteria-1972,"
     U.S.  Environmental Protection Agency Report, EPA-R3/73-033.

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                                                                    6 - 74

 EPA79   U.S.  Environmental  Protection Agency,  1979,  "Indoor Radiation Exposure
      Due to Radium-226 in Florida Phosphate Lands,"  EPA-520/4-78-013.

 Ha74   Hans,  J.  and Douglas,  R.,  1974, "Radiation Survey of Dwellings  in  Cane
      Valley,  Arizona and Utah,  for the Use of  Uranium Mill  Tailings,"  Office
      of Radiation Programs, U.S.  Environmental  Protection Agency.

 He78   Healy, J.W,  and Rodgers, J.C., 1978, "A Preliminary Study  of Radium-Con-
      centrated Soil,""LA-739]-M$.

 HWC78   Health and Welfare  Canada, 1978,  "Guidelines  for Canadian Drinking Wate',
      Quality," Canadian Government Publishers  Centre,  Supply and  Services Canadf
      Hull,  Quebec,  Canada,  K1ADS9.

 Mo79   Moore, R.E., Baes, C,f.  Ill,  McDowell-Boyer,  L.M,,  Watson,  A.P., Hoffman,
      P.O.,  Pleasant,  J.C. and Miller, C.W.,  1979,  "AIRDOS-EPA:  A Computerized
      Methodology for Estimating Environmental  Concentrations and  Dose  to Man
      from Airborne  Releases of  RadionucTides,"  U.S. Environmental  Protection
      Agency Report, EPA 520/1-79-009 (Reprint  of  ORNt-5532).

 NAS72   National  Academy of Sciences, National  Research  Council,  1972, "The Ef-
      fects  on Populations of  Exposure to  Low Levels of Ionizing Radiation,"
      Report of the  Advisory Committee on  the Biological  Effects of Ionizing
      Radiations  (BEIR Report).

 NCI78   National  Cancer Institute, 1978,  "SEER  Program:  Cancer Incidence and
      Mortality in the United  States  1973-1976," Prepared by  Biometry Branch,
      Division of  Cancer Cause and  Prevention, National Institutes  of Health,
      National  Cancer  Institute, Bethesda, Maryland.

NRC79    U.S.  Nuclear  Regulatory Commission,  1979, "Draft Generic Environmental
      Impact Statement on Uranium Milling, Volume I, Appendices," NUREG-0511.

ORP73   Office of Radiation Programs,  1973,  "Summary Report  of Radiation Surveys
     Performed in Selected Communities," U.S. Environmental  Protection Agency.

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                                                                   6 - 7'5

Pa74   Paone, J,,  Morning, J.  and Giorgetti, L.,  1974, "Land Utilization and Rec-
     lamation in the Mining Industry, 1930-71,"  U.S.  Bureau of Mines, Washington,
     D.C.

Pe79   Perkins, B.L., 1979, "An Overview of the New Mexico Uranium Industry," New
     Mexico Energy and Minerals Department, Santa Fe,  New Mexico.

Th79   Thrall, J., Hans,  J. and Kallemeyn, V.,  1980,  "Above Ground fiamnia-
     Ray Logging of Edgemont,  South Dakota and  Vicinity," U.S.  Environmental  Pro-
     tection Agency, Office of Radiation Programs - Reot.,  QRP/LV8Q-2.

Va?l   Vandergrift, A.E., Shannon,  L.J., Gorman,  P.G. ,  Lawless,  E.W,,  Sallee, E.E.
     and Reichel,  M,, 1971, "Participate Pollutant System Study -  Volume 1  -  Mass
     Emissions,"   EPA Contract to Midwest Research Institute,  Kansas City,  Missouri,
     Contract No.  CPA 22-69-104.

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         SECTION 7





SUMMARY AND RECOMMENDATIONS

-------
                                                                  7-1
 7.0   Summary and  Recorofngndatlons
 7.1   Overview
      This  report describes  the  potential  health and environmental  effects
 caused  by  uranfym mines.   It considers  all  contaminants—solid,  liquid,  and
 airborne—and  presents doses  and health effects  caused by wastes  at  both
 active  and inactive mines.   In addition to  outlining  the various methods  of
 mining  uranium,  the report graphically  depicts mine locations and  lists  the
 U.S.  total  of 340 active and 3,389  inactive urainum mines (Appendixes E  and
 F)    according    to   mine   name,   owner,   location    (state,    county,
 section-township-range),  and total  ore production.  Table 7.1 summarizes
 the 'nine lists.
      Several  facts  and limitations helped  shape the  method and approach  of
 this  study.   Little information  on uranium mines is  available; measurement
 info,(nation that  is available on uranium mine wastes 's frequently influ-
 enced   (biased)   by nearby  uranium  mills;  there  are  inherent  variations
 between uranium  mines, especially  between  in situ mines, that complicate
 generic assessments  of uranium  mine wastes; and,  finally, the  law (P.L.
 95-c04)  that  mandated  this  study allotted only a short time  in  which  to
 complete it.  To  accommodate these  facts in our study  plan, we  decided  to
 develop  conceptual  models  of  uranium  mines  and  to  make  health  and
 environmental   projections  from  them,   based  upon  available data  from  the
 litprature; to employ conservative (maximizing) assumptions when necessary;
 and to  supplement available information with  information from discussions
 with  persons  inside  and  outside  the  agency and  by doing several  field
 studies  in Texas,  New Mexico,  and Wyoming.   Table  7.2 summarizes  the
 sources  of uranium  mine  contaminants  that  were  modeled  in  this  study.

 7.2  Sources and Concentrations of Contaminants
 7.2.1    Surfaceand Underground Mines
     We calculated  released  radioactivity   for two models of active  under-
 ground and  surface uranium mines.  The average-large mine, the  first  model,
 reflects new  and  predicted  future  mines.   The  average mine,  the  second
model,  reflects  the regional  impact  of multiple  mines.  The quality  and

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      Table  7.1   Distribution of United States uranium mines  by type of mine and state
Active
State
Alaska
r
Arizona
California
Colorado
i
Florida
Idaho
Minnesota
Montana
Nevada
New Jersey
New Mexico
N. Dakota
Oklahoma
Oregon
S. Dakota
Texas
Utah
Washington
Wyoming
Unknown
Total
Surface -
0

1
0
5

0
0
0
0
0
0
4
0
0
0
0
16
13
2
19
0
60
Under-
ground
0

1
0
106

0
0
0
0
0
0
35
0
0
0
0'
0
108
0
6
0
256
• In situ
leaching
0

0
0
0

0
0
0
0
0
0
0
0
0
0
0
8
0
0
3
0
11
Others
0

0
0
4

0
0
0
0
0
0
3
0
0
0
0
1
3
0
2
0
13
Surface
0

135
13
263

0
2
0
9
9
0
34
13
3
2
111
38
378
13
223
6
1252
Inactive
Under-
ground
1

189
10 .
902

0
4
0
9
12
1
142
0
0
1
30
0
698
0
32
5
2036
All
Other(a)
0

2
0
52

1
0
1
0
0
0
12
0
0
0
0
4
17
0
10
2
101
                                                                                                       I
                                                                                                      ro
Includes mine water, heap leach dumps, miscellaneous,  and unknown.

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                                                        7-3
      Table 7.2,  Sources of contaminants at uranium mines

Source
Waste Rock (Overburden) Pile
Wind suspended dust "
Rn-222 emanation
Precipitation runoff
Sub-Ore Pile
Wind suspended dust
Rn-222 emanation
Precipitation runoff
Ore Stockpile
Wind suspended dust
Rn-222 emanation
Precipitation runoff
Abandoned Mine Area Surfaces
Rn-222, emanation
Mining Activities
Dusts
Combustion products
Rn-222
Waste water
Surface discharge
Seepage
Active
Underground

M
M
C

M
M
C

M
M
C

M

M
M
M

M
C
Note, — M» Source model edjC, considered but
Active
Su rf ace

M
M
C

H
M
C

M
M
C

M

K
M
M

M
C
not modeled due
Inactive
Underground

M
M
C

M
M
C

M
M
C

M

NA
NA
NA

NA
C
to lack of
Inactive
Surface

M
M
C

M
M
C

M
M
C

M

NA
NA
NA

NA
C

information^ NA»  not applicable.

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                                                                      7-4
 flow  rates  that were determined  for  water discharges from typical  surface
 and underground mines in Wyoming  and  New Mexico,  respectively, were  used to
 calculate  chemical  loading  of streams in  three hydrographic units:   sub-
 basin  (containing the mines),  basin,  and  regional  basin.  Infiltration  of
 mine  water to potable  groundwater and suspension/solution of contaminants
 in  flood  waters  are the  main components  of the  aqueous  pathway.   Crude
 dilution  and infiltration models were used  to  evaluate aqueous discharge
 from  active  mines.   Off-site movement from  inactive  mines  is primarily  by
 overland  flow,  the contamination  significance of which  was evaluated with
 limited field and literature surveys.
     Concentrations  of  radionuclides  and  stable elements in  waste rock,
 sub-ore, and ore, selected from only a few measurements, are shown in Table
 7.3.  Average annual airborne emissions for the sources listed in Table  7.2
 were computed for active and inactive mines using the concentrations listed
 in Table  7.3 and the geological  and meteorological  information appropriate
 for each  region.   Source  terms were maximized by assuming  no dust control
 and no  spoils  pile restoration.  Annual emissions of airborne contaminants
 estimated  for the  various  sources  are  given in the following  tables   of
 Section 3.
                       Tables on Active Mines
Tables on Inactive Mines
Source
Combustion Products
Vehicular Dusts
Dust from Mining
Activities
Wind Suspended Oust
Radon-222 Emissions
Su rf ace
3.30
3.32

3.33
3.34
3.35
Underground
3.52
3.56

3.54
3.55
3.51
Surface Underground

—

—
3.70 3.76
3.74 3.77
     Annual emissions  in  mine  water discharged to the surface by the model
average underground and surface mines are listed below.

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                                                                         7-5
     Parameter
Surface Mine
 ._{Wyoming.)
Underground Mine
  {New Mexico)
3
Flow rate, m /min
Uranium-238, Ci/yr
Uranium-234, Ci/yr
Radium-226, Ci/yr^
Radon-222 and each
short-lived daughter, Ci/yr
Lead-210, C1/yr
Poloniura-210, Ci/yr
Arsenic, Kg/yr
Barium, Kg/yr
Cadmium, Kg/yr
Molybdenum, Kg/yr
Selenium, Kg/yr
Sulfate, MT/yr^
Zinc, Kg/yr
Total suspended solids,_MT/yr
3.0
0.037
0.037
0.00065

0.00065
0.00065
0.00065
7.9
ND^
6.3
ND
ND
276
112
33.0
2.0
0.49
0.49
0.0014

0.0014
0.0014
0.0014
13
850
7
300
70
12?
45
29
     'a'No data available.
     ^ Mhe values shown for radium-226 and sulfate are 10 percent and 20 per-
cent, respectively, of those released on an annual basis.  Radium 1s assumed
to be irreversibly sorbed, and sulfate readily infiltrates.

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                                                                      7-6
Table 7.3.  Concentration of contaminants in waste rock (overburden), ore, and
            sub-ore
Nonradioactive
Stable
Element

Arsenic
Barium
Cadmium
Cobalt
Copper
Chromium
Iron
Mercury
Magnesium
Concentration
Waste Rock
-
9
290
NA
NA
18
<51
6,000 15
<8
NA 3
> uq/g
Ore and
Sub-ore
86
920
ND
16
61
20
,700
ND
,500
Stable
Element

Manganese
Molybdenum
Potassium
Lead
Ruthenium
Selenium
Strontium
Vanadium
Zinc
Concentration
Waste Rock

485
2.5
7,000
22
NA
2
150
100
20
» uq/g
Ore and
Sub-ore
960
115
25,000
78
ND
no
130
1,410
29
                                   Radioactive
Radioactive
Contaminant
U-238 and each daughter
Th-232 and each daughter

Waste rock
6
1
Concentration,
Sub-ore
(a)
2
pCi/g
Ore
285
10
            concentration of U-238 and each daughter was assumed to be 99 pCi/g
at active underground mines, 40 pCi/g at active surface mines, and 110 pCi/g
at inactive mines of both types.

Note.—NA, Not~available; ND, Not detected.

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                                                                         7-7
  7.2.2
In Situ Leach Mines
       The sources of airborne releases that we assessed at our model  in  situ
  leach  mine were the  uranium recovery  and  packaging unit,  the evaporation
  ponds, and the surge tank.  The annual  releases for  these sources are listed
  below.
     Source
                            Annual  Airborne Release Rate
Recovery Plant
     Uranium-238
     Uranium-234
     Uranium-235
     Thorium-230
     Radium-226
     Leid-210
     Polontum-210
     Ammonia
     Ammonium chloride
     Carbon dioxide
                                      0.10 C1
                                      0.10 C1
                                      0.0048 C1
                                      0.0017 Ci
                                      0.00010  Ci
                                      0.00010  Ci
                                      0.00010  Ci
                                      3.2  MT
                                     12 MT
                                   680 MT
Surge Tank
     Radou-222
                                   650 Ci
Storage Ponds
     Ammonia
     Ammonium chloride
     Carbon dioxide
                                   100 MT
                                   300 MT
                                    80 MT
       Since  in  situ  mining  is  site  specific  and  relatively new,  little
  information is available on  its  wastes.   Thus,  only airborne releases were
  assessed  quantitatively;  liquid  and solid  wastes  were discussed  quali-
  tatively.
       Several chararcteristics  of in situ mining,  especially regarding its
  liquid and  solid  wastes,  tend  to minimize  its  release of contaminants.

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                                                                       7-8
 First,  only a  small  fraction  of Ra-226 is leached  (2.5  percent assumed);
 second,  all liquid  wastes are  impounded  with no planned  releases;  third,
 much  of the liquid waste  evaporates,  except at a few  sites in Texas where
 the wastes are  injected  into  deep wells;  and,  finally,  at in  situ mines
 solid  wastes  accumulate at a  much lower rate than they do at  conventional
 mines.   Aquifer  restoration  and  underground  excursion   of  the  leaching
 solution  were also discussed  qualitatively.  Although restoration has  not
 yet been  done at a commercial  scale  site,  preliminary  experiments  indicate
 that   proper  aquifer   restoration is  possible.   During   the   restoration
 process,  Rn-222  will  continue to be  purged from the aquifer and should be
 considered  a possible source of  exposure.

 7.2.3     Uranium Exploration
     During  exploration  and  developmental  drilling,  dusts  are produced,
 Rn-22H  and  combustion  products   from drilling  equipment  are released,  and
 approximately  0.2  hectares of land surface are disturbed per drill   hole.
 The  average mine site  produces  an estimated 6,100 kg of airborne dust,  20
 kg  of  which is ore and subore.   About 3400  Ci of Rn-222 are released  annu-
 ally  from  all development holes drilled since  1948  (4.5  x 10 ), which  is
 similar  to  that  released from  one operating  mine.  Combustion  product
 releases are small .
7. '3
     Exposures  were assessed  for  a hypothetical most  exposed individual
living  about  1600  m   (1-mile)  from  the  center of  the mine  and  for  a
population  residing within  an  80-km  (50-mile)  radius  of  the  mine.  The
meteorological and geological parameters used were those appropriate to the
respective sites.
     Aqueous releases were modeled through a basin, sub-basin, and regional
basin hydrographic area.  Dilution by precipitation, snowmelt, and periodic
flooding  (typical  of semiarid  regions)  was analyzed  but not  used  in the
model.   For  the  model  we  assumed  that  the  average  annual   release  of
contaminants is diluted by the average annual flow rate of the stream being
considered.  The pathways that we assessed are listed below.

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                                                                    7-9
   Air Pathways
Water Pathways
   Breathing
   a.   Radioactive particulates
        and radon-222
   b.   Radon-222 daughters
1.   Breathing
     a.   Resuspertded contaminants
          deposited from irrigation
          water
   External Exposure
   a.   Submersion-
   b.   Surface deposited
        radioactivity
     External Exposure
     a.    Submersion in resyspended
          contaminants deposited
          from irrigation water
   Eating
   a.   Above-surface foods
        grown in the area
   b.   Milk and beef cattle
        grazing in the area
     Egting
     a.    Above-surface foods grown
          in the area
     b.    Milk and beef cattle grazing
          in the area and drinking
          contaminated water
     c.    Fish
     In  addition  to the  risks caused by wastes  at  or discharged directly
from the  mines,  we assessed the risks to occupants of habitable structures
built  on land  containing  uranium  mine wastes.   The radium-226  in these
wastes increases the concentrations of radon-222 and its decay products and
the gamma radiation inside these structures.
7.4  Potential Health Effects
7.4.1     Radioactive Ajrborne.Emissions
     The  risks of  fatal  cancer  were  estimated for  radioactive  airborne
emissions.  They  include the lifetime risk to the most and average exposed
individuals in the  regional  population and the  number  of additional  fatal
cancers in  the  regional  population caused per year of model mine operation
(see Table 7.4),

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                                                                       7-10
      The  major fatal cancer risk  at  each of  the model  uranium  mines  is  the
 risk of lung cancer from  Rn-222 daughter exposures  (Tables  6.11  and  6.12).
 At  surface  and  in situ mines,  radioactive particulates  plus  Rn-222 con-
 tribute only a little over  10 percent of the total  fatal  cancer  risk.   The
 principal  radionuclides in  the  airborne particulate  emissions  are  U-238,
 U-234,  Th-230, Ra-226,  and  Po-210,  The contribution  from Th-232 and  its
 daughters  is minor.   At underground mines,  essentially  all the risks  are
 due  to  Rn-222  daughter exposures.   Fatal cancer risks at active underground
 mines are greater than  those at active surface mines because of  the  larger
 quantity  of  Rn-222 daughter products  released.   For  inactive  mines,  the
 risks are  similar  at surface and underground sites.
      Most  of the exposure to individuals around the model uranium mines is
 received  internally, usually by breathing.  However,  the  average person in
 the  region  around  surface mines  receives  most  of  his  exposure by  eating
 contaminated foods.   The  largest  contributors  to  the  radioactive partic-
 ulate plus Rn-222  impact are ore and  overburden at active  surface mines  and
 ore  and sub-ore at  the active  underground mines.  For  the model  in situ
 mine,  the uranium processing plant  was the main  source  of  particulate
 radionuclides.
      Of all  evaluated model  uranium mines,  the  average   large underground
 mine  (Table   7.4)  causes  the  largest  fatal  cancer  risk and  the  largest
 number  of additonal cancers  in  the  regional population.   Compared to the
 natural occurrence of fatal cancer  from all  causes (Table  7.5), we estimate
 an increase  of 1.3 percent (0.0019)  in fatal cancers  over the lifetime of
 the  maximum   individual  and a  0.0003  percent  (0.018)  increase in  fatal
 cancers in the regional  population per year.  Increases  in expected fatal
 cancers are  less at all  other model mine sites.
     Compared   to   a  normal  occurrence   of  genetic   effects   of  0.06
 effects/birth  and  12.1  effects/year  in the regional  population  (Wyoming),
 the  computed risk  of additional  genetic effects from radiation exposure at
 the  model  uraninum  mines is  very small.   The  average large  surface mine
 produces the largest  increase  in genetic effects. We  estimate  the  genetic
 risk  to the  descendants  of the most exposed individual to be an additional
6.4E-5  effects/birth (0.1  percent increase)  for  a 30-year  parental  ex-
posure; 2.2E-7  effects/birth (0.00036 percent increase) to the descendants
of the  average  exposed  individual   in the regional  population for the same

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              Table  7.4       Summary  of  fatal cancer  risks from radioactive air-
                            borne  emissions  of model uranium mines
Source
Average Surface
Mine
Average Large
Surface Mine
Average Under-
ground Mine
Average Large
Underground Mine
Inactive Surface
Mine
Inactive Under-
ground Mine
In Situ Leach Mine
Most exposed
individual life-
time fatal cancer
risk (a)
1.3E-4
4.2E-4
2.0E-4
1.9E-3
3.4E-5
2.0E-5
2.2E-4
Average exposed
individual life-
time fatal cancer
risk (a)
2.5E-7
8.1E-7
9.1E-7
8.6E-6
6.3E-8
8.6E-8
3.9E-7
Fatal cancers
cancers caused in
regional population
per year
1.7E-4
6.4E-4
1.7E-3
1.8E-2
1.3E-5 '
4.5E-5
3.1E-4
  ^ 'Lifetime exposures were calculated as follows;
Surface and underground mines:  Exposure for 17 years to active mining and 54 years to
inactive mine effluents.
Inactive mines:   Exposure for 71 years to inactive mine effluents.
In situ leach mine:  Exposure for 10-year operation and 8-year restoration.

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                                                                         7-12
      Table  7.5  Percent  additional  lifetime fatal  cancer risk for a
                lifetime exposure to the individual  and  the  percent
                additional  cancer deaths in the regional  population
                per year of exposure estimated  to  occur  as a result
                of uranium  mining
Source
Average surface mine
Average large surface
mine
Average underground
mine
Average large
underground mine
Inactive surface mine
Inactive underground
Most
Exposed
Individual
8.7E-2
2.8E-1
1.3E-1
1.3
2.3E-2
1.3E-2
Average
Exposed
Individual
1.7E-4
5.4E-4
6.1E-4
5.7E-3
4.2E-5
5.7E-5
Regional
Population
7.9E-6
3.0E-5
3.1E-5
3.3E-4
6.1E-7
8.3E-7
mine

In situ leach mine
1.5E-1
2.6E-4
1.4E-5
  Note.--Comparisons are based on the risks given in Table 7.4, a national
cancer risk from all causes of 0,15, and an estimate of the cancer death rate
from all causes to the regional populations of New Mexico (5,400 deaths) and
Wyoming (2,140 deaths).

-------
                                                                 7-13
exposure  period;  and  7.9E-5 additional  genetic effects  committed  to  the
descendants  of the  regional  population per  year of  mine operation.    The
latter  increase  is very small compared to the 12.1 effects that will norm-
ally occur each year in the live births of the regional population.

7.4.2   Nonradioactive Airborne Emissions
     Atmospheric   concentrations  of  nonradioactive  air  pollutants  were
calculated  at the  location  of the  most  exposed individual.   The concen-
trations  were  compared  with calculated  nonoccupational  threshold  limit
values, natural background concentrations, and average urban concentrations
of selected airborne pollutants in the United States.
     Of  the pollutant  sources  investigated, three  produced  insignificant
health  hazards:
   1.   airborne stable trace metals
   2.   airborne combustion products from heavy equipment operation
   3,   nonradioactive gas emissions at in situ leach mines
     However,  at active surface mines, dust  particulates (produced  mainly
by  vehicular  traffic) equal  or  exceed conservatively  calculated nonoccu-
pational  threshold limit  values  and, therefore,  are  a potential  nuisance.

7:4.3     Radioactive Aqueous Emissions
     The only water from active uranium mines is that pumped from the mines
and  released  to surface  streams.   The largest  radiation dose*  from  this
water to  individuals in  the  assessment regions  is to  the endosteal  cells
(bone)  (see  Tables 6.25  and  6.26).   It primarily comes  from  eating foods
grown on  land  irrigated  by streams fed by discharged mine water.   Signifi-
cant, but  of  lesser  importance,  are exposures due to  breathing  wind  sus-
pended material from irrigated land,  eating fish caught in streams near the
site, and  external gamma  radiation  from  land irrigated  by streams  fed by
mine water discharges.  We  estimate  only  a small risk from eating beef and
milk from cattle grazing  on irrigated pasture and drinking water contami-
nated  by  mine discharges  (< 2  percent  of  the  total  risk  from  aqueous
emissions).   The radionuclides of major importance in the risk analyses are
U-238 and U-234.
     *In Section  7,  "dose"  is  to be  read as  "dose  equivalent"--absorbed
radiation (dose) multiplied by a quality factor.

-------
                                                                       7-14
      The risks of fatal cancer  were estimated for radioactive aqueous dis-

 charges to  surface  streams from  active uranium mines.  The  estimates in-

 cluded, for the 17-years  of  active mine operation, the  cumulative  risk to

 the most  and  average exposed  individuals  fn  the  assessment area  and the

 number  of  fatal  cancers caused  to persons residing within  the  assessment

 area (Table 7.6).  Aqueous emissions  from  inactive mines and  from  in situ

 leach mines were  not modeled  due  to  a  lack  of data.   However,  we  believe

 aqueous source terms  from  these  mines  would be low.

      Drinking  water  may  be an  important source of exposure for the most

 exposed individual living near  a  uranium mine.  However, we did  not  esti-

 mate it because we could  not  quantify radionuclide concentrations  in pot-

 able groundwater with available  information.  Also, mine water probably  is

 not consumed directly by man.
      Table  7.6       Summary  of  the  fatal  cancer  risks caused  by  radioactive

                     aqueous  emissions  from model uranium mines
 Source
Most exposed
individual's life-
time fatal cancer
risk for 17 years
of mine operation
Average exposed
individual's life-
time fatal  cancer
risk for 17 years
of mine operation
Fatal cancers
caused in the
assessment area
population from
17 years of
mine operation
 Underground     5.6E-6(3.7E-3%)
 mine site
 (New Mexico)

 Surface mine    1.2E-7(8.0E-5*)
 site
 (Wyoming)
                               (a)
                         3.4E-7(2.3E-4%)      2.2E-2(2.3E-4X)



                         1.6E-8{1.1E-5X)      2.6E-4(1.1E-5X)
      ll "risks" in this table are  in addition to the 0.15 risk of fatal
cancer from all causes.


     Although  aqueous  discharges  from  the model underground  mine produce
greater  risks  than  those from the  model surface mine, primarily because of

greater  releases of U-238 and U-238 daughters,  aqueous  releases at either

mine cause  only very  small  cancer risks  (see  Table  7.6)  beyond  the  0.15

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                                                                       7-15

 natural  risk  of  fatal  cancer.   For example,  in New  Mexico  (assessment
 population  64,950) and  Wyoming (assessment  population  16,230), 9,742  and
 2,434  deaths from cancer  from  all  causes are projected to  occur.   Aqueous
 mine discharges  in  these areas will  add only 0.022 and 0.00026 estimated
 deaths,  respectively,  to these  totals.
     The largest increase in  estimated genetic effects occurs  at the under-
 ground  mine site.  However,  compared  to  the natural  occurrence of  heredi-
 tary disease,  the overall risk  of additional genetic effects  due to radio-
 nuclides discharged  in water from  the model  mines  is very small.  Based  on
 a  natural  occurrence  of 0.06  effects/birth,  there will  be  936   genetic
 effects  in  the  regional  population of New  Mexico  during  17 years   of mine
 operation.  In  contrast,  there will  be only  0.015 additional effects to all
 the  descendants  of the regional population  because of the 17-year exposure
 period.

 7.4.4  Nonradi oactiveAqueous Emissions^
     Aqueous  concentrations  of nonradioactive  pollutants  were calculated
 for  stream  water we assumed  was used  by  the average individual within the
 assessment  area.  The  pathways considered are those listed in Section 7.3.
 Drinking  water  might  be  a significant pathway  for  the  most exposed indi-
 vidual.   However, we  could  not make a  reliable  prediction  of increased
 groundwater  concentrations  due  to  mine dewatering with the available data.
     A  comparison of  the water concentrations  of  several  pollutants with
 recommended  EPA  limits for livestock and irrigation usage (see Table 6.29)
 showed that only molybdenum  from the underground mine approaches its limit
 for  irrigation.  The  sums of  the ratios of the average water concentrations
 to the  recommended limits  are less than one, indicating  that mixtures of
 the  metals  would not  exceed  a  "composite limit"  for  an  average individual
 in  the  assessment  areas.  Constituents  such as  solids  and  sulfates,  for
which limits are unavailable, have minimal or no toxic properties.
     More  .information  is  needed  before  definitive  conclusions   can  be
 reached about health hazards  caused by nonradioactive waterborne emissions.
Uranium,  the metal estimated to be  in  highest  concentration,  has  no es-
tablished  limits based  on chemical  toxicity in  the United States.   Of
particular  interest would be  data  on water use patterns  near the mines and
the  degree  to  which mine discharges may  infiltrate  groundwater supplies.

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                                                                       7-16

 7.4.5   Solid  Wastes
     We estimated the  risk of  fatal  lung  cancer to individuals living  in
 houses  built  on land contaminated  by  uranium mine wastes as  a  function  of
 the Ra-226  concentration  in the  wastes (see  Table 7.7). How much mine  waste
 has been used  for  homesite land fill   as well  as its level(s) of contami-
 nation  are unknown.   Because of the  cost,  it is unlikely that mill-grade
 ore would  be available  for  off-site   use.    It  is more  likely  that  waste
 rock,  perhaps mixed  with  some  sub-ore,  would be  the  material  used. Con-
 sidering  the Ra-226  content of  sub-ores and the  likelihood  of its  being
 diluted with  waste rock  and  native soil, mine wastes in residential  areas
 would probably contain  between 5 to 20 pCi/gm  of  Ra-226,

     Table  7.7      Estimated lifetime risk  of fatal  lung cancer to the
                    average person  living in a  home built on land contami-
                    nated by  uranium mine wastes

     226Ra  in Soil        Indoor  Working Levels         Lifetime Risk of
     (pCi/g)                        (WL)                Fatal Lung Cancer^
5
10
20
30
0.02
0.04
0.08
0.12
0.025
0.050
0.10
0.15
         on the average individual being inside his home 75 percent of the
time.
7.5  Environmental Impacts
     We  evaluated  the environmental  effects  of uranium  mining,  including
exploration, by  reviewing  completed studies,  extensive communications with
State  and  Federal  agencies,  field studies in Wyoming and  New Mexico, re-
connaissance  visits  " to  Wyoming,   Colorado,  New  Mexico,  and Texas,  and
imagery  collection and  interpretation.   Underground and surface mines were
examined to develop a sense of an average or typical condition with respect
to mine  size,  land  areas  affected,  quality  and quantity  of airborne and

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                                                                       7-17
waterborne  releases,  and general, qualitative appreciation  for the effects
of  such operations on  surface  streams,  groundwater, disturbed land areas,
and  natural  recovery  processes.   In  many  instances,  conditions  can be
documented, but  the significance  remains  highly  subjective and thus weakens
the  justification for  corrective action, particularly for inactive nines.

7.5,1   Land and  Water Contamination
     We conclude that (1) U.S.  uranium mills make little use of mine water;
(2)  mine drainage .is  to  the  environment,  with occasional  use  for agri-
culture,  sand backfilling,  construction,  and potable supply;  (3)  active
surface  mines in Wyoming  and  underground  mines  in  New Mexico  have the
greatest  discharge  to  the offsHe environment;  (4) inactive surface mines
do  not appear to adversely affect  groundwater  quality,  although water in
such  mines  is typically contaminated and runoff from surface accumulation
of overburden and sub-ore may  be  a  source of surface water contamination;
and  (5)  selected inactive underground mines in Colorado and possibly adja-
cent  portions of Utah  may discharge water enriched  in  radionuclides and
trace  elements.   Since  the mining industry now uses terrestrial ecosystems
extensively as sinks for mining-related contaminants, an appropriate govern-
ment agency should monitor active mines for groundwater quality, sorption of
contaminants  on  stream  sediments,  and  the  flushing  action of  flooding
events.
     Before and  during  surface  and underground uranium mining, contaminated
mine water  is frequently discharged to arroyos  and pasture  lands adjacent
to the mines.   Less frequently, mine water is used  in nearby uranium mills,
in which  case ultimate disposal  is  to  the mill  tailings  pile  where evap-
oration and  seepage occur.  However, despite  this  practice  of mine  water
discharge to  land and  despite  the existence of over  3,000  active  and in-
active  mines  and the  accelerating  level  of exploration  and mining,  there
are many  more studies  and surveys on the interaction  of  uranium mills and
water  resources  than  there are on uranium mines and water resources.   With
few  exceptions,  monitoring mine  water  quality  has been  related to  NPDES
permits.
     When mines discharge water to open  lands and water courses,  90 percent
or more of  it infiltrates the  soil and the balance evaporates.   Stable and
radioactive  contaminants  subject to sorption  are selectively concentrated

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                                                                       7-18

 in  nearby  soils,  which become a  local  sink.   Mobile constituents such  as
 sul fate and chloride probably percolate  to  the water table along with  the
 bulk  of the water, which  recharges  nearby shallow aquifers downgrade from
 the mines.  Although  many areas  In New Mexico, Texas, Colorado, Wyoming,
 and  Utah   have   received   mine  water  discharge,  studies  of contaminant
 accretion   on  soils  and  deterioration  of  groundwater  quality  have been
 rather   limited.   Widespread  contamination  of  groundwater  has  not been
 documented, but  there are  indications that  local surface water and ground-
 water quality have  been  adversely  effected in Colorado, Wyoming, and Texas.
 Studies underway in  New Mexico reveal,  in  at  least  two mining districts,
 groundwater deteriorating  because of mine drainage.  Significant increases
 in  ambient uranium  and radium occurred  in  the Shirley  Basin uranium dis-
 tri :t of Wyoming because of  initial  strip mining and mill processing and,
 to  e  lesser extent, in  situ  leaching.   The  long-term significance of soil
 loading with  stable and radioactive contaminants and their cycling through
 the terrestrial  ecosystem,  including  the human  food chain,  has  not been
 determined  for uranium mining operations.
      Discharges  from model active surface and  underground mines  average 2
      3
 to  3  m  /minute.   In most cases, complete  infiltration takes place in stream
 beds  within 5 to  10 kilometers of  the mines.  However, when discharges from
 several  mines  are  combined or if single mine  discharge  is  several  cubic
 meters   per  minute  or  more,  infiltration  and  storage   capacity  of  the
 alluvium in nearby channels is exceeded and perennial  flows are created for
 distances  of  20  to 30 kilometers.   For  example,  underground  uranium  mines
 in  the  Grants Mineral  Belt  of  New Mexico  currently discharge 66 m  per
                             3
 minute.  Of  this,  only  12 ro  per minute are  used  in uranium mills;  the
 balance  is discharged  to  nearby  washes or arroyos.   Fourteen of the  20
 active  uranium  mills make  no use of mine water, which  is associated with
 essentially  every active underground mine  and  most  active  surface mines,
 particularly in Texas and Wyoming.
     Annual  contaminant  loading  from continuous discharge at a  rate  of 3
 •3
m / minute  from  one surface mine  in the Wyoming model area and dilution  in
 flood flows with  recurrence intervals of 2 to 25 years produce the loading
and stream  concentration  values  in Table 7.8.  Chemical loading was calcu-
lated on a mass-per-time  basis  to estimate the  effects of  mine  drainage.

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                                                                       7-19
 For  assessing  environmental  impacts,  we  assume  that  most  contaminants
 remain on  or  near the land  surface  and are available for  resuspension  in
 periodic  flash flooding in  the  sub-basin.   Sorption,  precipitation,  and  so
 on are  assumed  to  render  90 percent  of  the  radium-226 unavailable  for
 further  transport.  Eighty percent of  the  sulfate is  assumed  to  infiltrate
 and also  becomes  unavailable  for  further transport in  flood  waters.
      Stream concentrations  for  uranium,  zinc,  cadmium,  and  arsenic are
 likely to  be  less than those shown  because  there will  not be 100 percent
 resuspension  of  sbrbed  contaminants, and  flood  events with lesser  return
 periods  are also likely to  disperse contaminants.   The  loading data are
 believed  to be  quite  realistic;  it  is the  temporal  distribution and re-
 distribution  of  the contaminants  that constitute  a  significant unknown.
 These preliminary results  indicate  contamination  of surface  water with
 uranium,  radium,  sulfate,  and, to a lesser  extent, with cadmium and arsenic
 in  stream  waters near  the mine outfall.    Subsequent  dilution  of  these
 initial  concentrations  will  occur as  the  flow  merges  with  that  of pro-
 gressively  larger streams  in the  downgrade direction,  but  cadmium  and
 sulfate  may exceed  the drinking  water standard  in  flood  waters  as  far as
 the regional  basin.   Impoundment of these  initial  flows can  be expected
 considering  water management  practices  in semiarid  rangeland  areas like
 Wyoming.   Therefore,  further pathway  investigations,  based  on field  data,
 are needed.
      For  the model underground mining area, we  selected  the Ambrosia Lake
 District  of New Mexico.  We assumed that 14 mines discharged an average of
 2 m /minute and that loading took place for two years prior to each flood.
 We  then   calculated  concentrations   in  flood  water  for  eight  different
 cases-for  2,  5,  10,  and 25 year  floods  (larger  numbers  indicating  larger
 floods),  with  concentrations  for  each flood being  calculated  on  the  basis
 of  both a  1-day and 7-day flood duration (see Table 7.9).  Based upon  these
 assumptions  and  calculations,  it appears  that  concentrations  in  flood
waters,  particularly in  the  basin,  may exceed  established  or  suggested
 standards  for   uranium,  .radium*  cadmium,  arsenic,  selenium,  barium,  and
 sulfate.    However,  precipitation and  sorption,   in  addition  to  dilution
farther downstream,  probably  will reduce  these concentrations  enough  so
that quality standards  for drinking  and irrigation water  can  be  met.  But

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Table 7.8   Summary of contaminant loading and stream water quality from a model  surface  uranium mine
Annual Loading
  Per Mine
   (Kg/yr)
                              Drinking Water
                                Standard
Concentrations in Basin and Regional  Basin
Flood Flows for Floods of 2, 25,  and 100
Years Return Period, mg/t


Uranium s 0.015/3. 5/0. 21^
110
Radium-226 5
0.00065 Ci/yr pCi/£
TSS
32,955
Sul fate 250
2.76 x 105
Zinc 5.0
112.0
Cadmium 0.01
6.31
Arsenic 0.05
7.88
^- ' I nsirHf nsi i/aliiac? c hnuin ¥f\v* v*arl-i lint anH eiil^
Basin
Mi n Max
0.36 0.76

2.1 4.5
pCi/£ pCi/l.
107 228

900 1909

0.366 0.774

0.02 0.044

0.025 0.054


Regional
Min '
0.26

1.6
pCi/£
79

668

0.271

0.015

0.019

^i-iii Od r»e»¥*/"*£inf'
Basin
Max
0.44

2.6
pCi/£
131

1098

0.445

0.025

0.031


of the amount actually released by a mine.  Irreversible sorption and precipitation affect radium and
sulfate  infiltrates to the water table.
      * '0.015 mg/l :  Suggested maximum daily limit based on radiotoxicity for potable water consumed at a
rate  of  2  liters per day on a continuous basis.  3.5 mg/t :  Suggested maximum daily limit based on chemical
toxicity and intake of 2 liters in any one day.  0.21 mg/£ :  Suggested maximum daily limit based on chemical
toxicity and intake of 2 liters per day for 7 days.
                                                                                                                     f\5
                                                                                                                     O

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               laoie  /.y    nummary or contaminant  loading ana stream water quality rrum
                           a  model underground  uranium mine
Annual Loading,
Per Mine(a)
(Kg/yr)
Uranium 1480
Radium-226
0.0014 Ci/yr
Lead-210
0.0014 Ci/yr
Cadmium 7
Arsenic 13
Selenium 80
Molybdenum 300
Barium 850
Zinc 45
Sulfate 1.22 x 105
TSS 29,000
Drinking
Water
Standard
(mg/ £ )
0.015/3. 5/0. 21(b)

5 pCi/£

—
0.01
0.05
0.01
—
1.0
5.0
250
•*-""-*
Concentrations in Basin and Regional Basin for 1-day and
7-day Floods of 2 to 25 Years Return Period, mg/l

Min
6.9

6.7 pCi/£

71.2 pC1/£
0.03
0.061
0.37
1.4
4.0
0.21
574
130
Basin
Max
7.1

6.9 pd/£

73.4 pCi/t
0.03
0.063
0.38
1.4
4.2
0.22
584
140
Regional
Min
0.045

0.044 pCi/£

0.470 pCi/£
0.0002
0.00039
0.0026
0.0089
0.26
0.0014
3.7
0.89
Basin
Max
0.046

0.044 pCi/£

0.0472 pCi/£
0.0002
0.00041
0.0026
0.0093
0.27
0.0014
3.8
0.92
     (a)Loading values shown for radium and sulfate are reduced to 10 percent and 20 percent,  respectively,
of the amount actually released by a mine.  Irreversible sorption and precipitation affect radium and sulfate
infiltrates to the water table.
     ^ '0.015 mg/l :  Suggested maximum daily limit based on radiotoxicity for potable water consumed at a
rate of 2 liters per day on a continuous basis.  3.5 ng/i : Suggested maximum daily limit based on
chemical toxicity and intake of 2 liters in any one day.  0.21 mg/l :  Suggested maximum daily limit
based on chemical toxicity and intake of 2 liters per day for 7 days.
                                                                                                                  ro

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                                                                       7-22
 more theoretical  and  field  evaluations  are  needed  to confirm  this.
      In situ  leaching  has contaminated  local  groundwater reservoirs.   We
 expect that this will continue  because leach solution excursions  from  the
 well field  do  occur and  because  injected  constituents,  especially ammonium,
 can not be  fully recovered.  The  NRC  and  agreement States  recognize  this
 situation  but consider  the adverse  impacts  outweighed by the benefits  of
 recovering  additional uranium and  developing a relatively new technology.
 7.5.2   Effects of Mine Dewatering
     Underground  mines  and  most surface mines  are  dewatered  to allow  for
 excavation  or shaft  sinking and ore  removal.   The  resulting  low concen-
 tration and, oftentimes,  large  volume  effluent  discharges  introduce sub-
 stantial  masses  of  stable and radioactive trace elements to local soil  and
 water  systems.   This extensive  use of soils  in  both  the  saturated  and
 unsaturated  zones a.s  water and contaminant sinks requires further study to
'determine the environmental  fate  of those elements.  In  addition to local
 effects,  the long-term  impacts on  regional water availability and quality
 are  also  important.   The NPDES limits  relating  to  surface  discharges are,
 in terms  of  parameters and concentrations, different from one EPA region to
 another and  should be  reevaluated   to  more  closely reflect  the impact of
 contaminant  concentration  and   mine discharge.   In  general,  the  uncer-
 tainties  about the  environmental  impact of mine dewatering  can be expected
 to  increase; and additional,  comprehensive  investigations  of  its effects
 are  necessary.

 7.5.3   Erosion of MinedLands and AssociatedWastes
     From  initial  exploration  through retirement,  mining,  particularly
surface mining, increases erosion and sediment yield.  The most significant
waste   sources  are  access  roads,   drilling  pads,   and  piles  of  over-
burden/waste  rock  and sub-ore.   Sediment  and associated contaminants are
dispersed mostly  through the  overland  flow of  precipitation  and snowmelt
water.   Erosion  rates  vary considerably with  the  characteristics of  the
source area,  i.e., pile  geometry, soil  and rock characteristics, amount and
type of  vegetative  cover,  topography,  and  local  climate.  There  is  some

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                                                                       7-23

 erosion  of all mine waste  sources,  although studies of ephemeral  drainage
 courses  downgrade  from  inactive mines  in New Mexico  and Wyoming  usually
 reveal  only local  soil and water contamination and no  significant  off-site
 dispersal  of  contaminants.   Proper  reclamation,  particularly grading  and
 revegetation,  markedly reduce  erosion and, consequently, contaminant trans-
 port.

 7.5.4      Exploratory  and Development Drilling
     The  uranium industry  has drilled approximately 1,300,000 exploratory
 and  development drill  holes through  1977.   This amotr.ts to about 430  drill
 holes  per  mine if  averaged over all  active and inactive mines.  During  the
 r-;urse  of  drilling, some land areas  are  disturbed to provide access  roads
 *c  the drill  sites and pads for the drill-rig placements.   This has dis-
 turbed  about  2500  km2 (960 mi2)  of  land for all  drilling  through  1977.
     Drilling  wastes  accumulate  at each drill site.  Although these wastes
 are  sometimes  placed in trenches and  backfilled after drilling, the  general
 industry  practice  (observed  from  field  studies  and  aerial  photography),
 apparently,  is to  allow  the wastes  to remain on the  surface,  subject to
 erosion.   The  extent  of  radiological contamination  from erosion  of  the
 remaining  ore  and sub-ore at development drill holes is not known.
     The average  drilling  depth has  increased with time  and  will probably
 continue ,to do so in the future.  Deeper drilling  will tend to increase  the
 probability  that several aquifers  may be penetrated  by  each  drill  hole.
 Aquifers with  good quality  water may be  degraded by  being connected,  via
 the  drill  holes,  with aquifers  of poor quality water.  Current regulations
 require  drill  holes to  be plugged  to prevent interaquifer  exchange,  but
 often  only the first  one  and  one-half  meters  of the   borehole  will  be
 plugged, and regulations do not effect past drill   holes. Finally, it appears, from
 mine site  surveys  and aerial  photography, that very few  drill  sites have
 been reclaimed.

 7.5.5     Underground  Mining
     The land  disturbed by individual underground  mines varies from  0.89 to
 17 hectares (2.2  to 42 acres) with  an average of  9.3 hectares (23  acres).
 In  addition,   access  roads to  the  mines  consume  about 1.1  hectares (2.7
acres), and  mine subsidence disturbs about  1.5  hectares  (3.7  acres).   A

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                                                                       7-24

 total  of about 12 hectares  (30 acres) of land are  disturbed by  an  average
 underground  mine.
     All  underground uranium mining  through  1977  has produced  about  2,9  x
 10  MT or about  1.8  x  10  m  of wastes.   Some  of these wastes, the  sub-
 ores,  contain  elevated concentrations of  naturally  occurring radionuclides.
 The  sub-ores usually are removed  last in the mining  process  and dumped on
 top  of the  waste  rock where they are subject  to erosion.  Some radiation
 surveys conducted around waste  piles  indicate that  the sub-ores are eroding
 and  contaminating  land in addition to that  disturbed by the mining activ-
 ities.
     During  our field studies  in  Texas,  New Mexico, Wyoming, and Colorado,
 we saw very  few mine  sites  where  reclamation  had been completed or was in
 progress—especially at the  inactive  mine sites.

 7.5,6  .Surface Minjng
     The  cumulative  waste from  surface mining uranium between 1950 and 1978
                          9              93
 amounts to about  1.7 x 10   MT  (1.1  x 10  m ).  Overburden is usually used
 to backfill  mined-out pits  during contemporary mining.   At older inactive
 mines,  the  mine  wastes were  either   used  for  pit  backfill or  completely
 disregarded.   Erosion of these waste piles may cause substantial environ-
 mental problems.
     The  amount of  land  physically  disturbed at a  surface mine  is  highly
 variable. The  area  disturbed  at ten   surface mines  was  estimated to range
 from  1.1  to 154 hectares  (2.7 to 380 acres), averaging  about  41 hectares
 {101  acres)  per  mine site.   Access   roads disturb  about 3 hectares  (7.4
 acres) per mine site, bringing the total  average  area physically disturbed
 to  about  44 hectares  {109  acres).   Field  surveys  of inactive mine sites
 indicate  that  mine   wastes  (sub-ores) erode ,and  contaminate  land  areas
 greater than those physically disturbed.  The land contamination  appears to
 have been caused  by erosion of ore  stockpiles,  erosion of sub-ores,  and
dust losses  from the actual  mining process.
     Very few  if any  inactive  mine  sites were reel aimed.  Reclamation of
any mine site will  have to address the radiological  aspects  of the mine and
 Its wastes.

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                                                                      7-25
 7.6  Regu 1 atory Perspect1ve
     Except for in situ leach mining, licensed by the Nuclear Regulatory
 Commission (NRC), uranium mining is not licensed, per se» by a Federal
 agency.  However, three Federal statutes have particular relevance to
 uranium mining.  First, the Federal Water Pollution Control Act as
 amended O972) requires a permit for discharges to navigable waters.
 Second, the Clean Air Act amendments of 1977 require a permit for
 pollutant air  emissions.  Third, proposed regulations under the Resource
 Conservation Recovery  Act of 1977 Identify hazardous wastes and
 stipulate their disposal for uranium mining.  When promulgated,  these
 latter regulations will  strengthen current Federal  and State reclamation
 requirements.
     In situ yrar.Iym mining is licensed by those states having
 agreement-state status with NRC.  National Pollution Discharge
 Elimination System (NPDES) permits are issued by EPA approved states.   No
 state issues mining licenses per se.   However,  most  states require mining
 and reclamation plans, including bonding fees,  for at least
 state-controlled lands.  Most reclamation requirements provide erosion
 control through  slope and vegetation standards.   Arizona is the only
 uranium mining state without reclamation requirements.

 7', 7  Cone 1 usions andRecommendations
     The evaluation of the potential  impacts of uranium mining was
 performed largely by means of analytical studies of  model  facilities.   We
 believe that the results give an adequate representation of the
 industry.   In order to determine the  extent  of  possible  problems,  our
 studies were specifically designed to give conservative  results.  It
 should be recognized that actual mines may operate under conditions
producing substantially smaller Impacts than the results presented.
     Compared to uranium milling, health and environmental  effects of
mining are"not as well understood,  despite the  existence of over
3000 active and inactive mines.   We have noted  throughout this report
Instances of the absence or Inadequacy of pertinent  information.

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                                                                      7-26

7.7.1  Conclusions

7.7.1.1  Solid Wastes
     Solid uranium mining wastes are potentially hazardous when used as
building materials or when buildings are constructed on land containing
such wastes.  The hazard arises principally from increased risk of  lung
cancer due to, radon-222.  In a 1972 survey of communities in uranium
mining regions, EPA and the former Atomic Energy Commission found more
than 500 locations where such wastes had been used.

7.7.1.2  A1rborneEff1uents
     a)  Individuals living very near active underground mine exhaust
vents would have an increased risk of lung cancer caused by exposure to
radon-222 emissions.  Surface mines and in situ mines are less hazardous,
ami inactive mines do not have significant radon-222 emissions.   Other
airborne radioactive emissions from all types of mines are judged to be
smaller.
     b)   The number of additional cancers committed per year in  the
regional populations due to radionuclide air emission from the
approximately 340 active mines and 3300 inactive mines was estimated to
be about 0.6 cancers in 1978.  This number of estimated additional
cancers is small, about one-third of the estimated additional  cancers in
•regional populations due to radon emissions from the 24 inactive  uranium
mill tailings piles addressed by Title I of the Uranium Mill  Tailings
Radiation Control Act (EPA 80).   (These mill  tailings piles represent
about 13 percent of all tailings currently existing  due to U.S. uranium
mifling and mining).  These potential  effects are not of sufficient
magnitude to warrant corrective measures,  especially considering  the
large number of sites involved.
     c)  The following were judged to cause an insignificant health risk
for all types of mines:
          1.  airborne nonradioactive trace metals.
          2.  airborne combustion products from heavy-duty
          equipment operations.
          3.  nonradioactive emissions from in situ  leach sites.

-------
                                                                      7-27
     d)  Airborne dust near large surface mines (primarily caused by
vehicular traffic) may exceed the National Ambient Air Quality Standard
for particulate matter.

7.7.1.3  Wa terborne Effluents
     a)  We estimate that an insignificant health risk accrues to
populations from waterborne radioactivity from an average existing mine.
     b)  Uranium mine dewatering and water discharges,  which are
                                       i
increasing as more and deeper mines are created,  may in the future have
significant effects on water quality.  Current treatment practices are
controlling the release of radioactivity  into surface waters.
     c)  Water in inactive surface and underground mines usually contains
radionuclides and trace elements in concentrations comparable to
groundwater in contact with ore bodies.  Some abandoned underground mines
in certain areas of Colorado and Utah probably discharge such waters to
nearby streams and shallow aquifers.   Available data is not sufficient  to
conclude whether or not there is a problem.
     d)  We could not determine, using models,  that there is no health
hazard to individuals who drink water drawn  from  such surface or
underground sources.   Water discharges from  active mines to nearby
streams and stream channels may extensively  recharge shallow aquifers,
many of which are either now used or  could be used for drinking water.
Such determinations must be made on a site-specific  basis,  and take
account of the additive effects of multiple  mines.   These studies can be
made easily a part of State or utility surveillance programs.

7.7.1.4  Exploratory  and Development  Drilling
     Harm from effluents due to exploratory  and developmental  drilling  is
probably small compared to effects of operating mines.   Under  current
regulations and practices, however, aquifers penetrated at different
levels can mix, creating the potential  for degrading high quality
groundwater.

-------
                                                                      7-28

 7.7.2   Recommendations to Congress

     1)  Based on this study, we do not believe at this time that
 Congress needs to enact a remedial action program like that for uranium
 mill tailings.  This is principally because uranium mine wastes are lower
 in radioactivity and not as desirable for construction purposes as
 uranium mill taiTings.  Nonetheless, some mining waste materials appear
 to have been moved from the mining sites but not to the extent that mill
 tailings were. .
     2)  Some potential problems were found that might require regulatory
 action  but none of these appear to require new Congressional action at
 this time.

 7.8  Other Findings

     1)  Regulations may be needed to control  wastes at active uranium
 mines to preclude off-site use and to minimize the health risks from
 these materials.   These regulations would need to address the use of the
 materials for construction purposes as well  as ultimate disposal  of the
 materials.
     EPA proposed such regulations in 1978 under the Resource
 Conservation and Recovery Act (RCRA).   In 1980,  Congress amended  RCRA  to
 require further EPA studies before promulgating  general  regulations for
 mining wastes.  An EPA study by the Office of  Solid Wastes on all  types
 of mines, including uranium mines, is currently  being conducted.   The
 amendment did not restrict EPA's authority to  regulate use of uranium
 mine wastes in construction or reclamation of  lands containing such
 wastes.
     2)  Standards are needed to control  human exposure  from radioactive
 air emissions from uranium mines.   This is principally because of
potential exposure to individuals living  near  large underground uranium
mines rather than concerns regarding the  exposure  of  regional
populations.   We  have proposed such standards  under Section 112 of  the
Clean Air Act.

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                                                                      7-29
     3)  EPA has conducted two field studies in 1972 and 1978 which
define possible sites at which mine wastes may have been used in
construction or around buildings.  The information developed in these
studies has been sent to State health departments.   The States should
conduct follow-up studies, as appropriate, to determine whether there are
problems at these sites.
     4)  The adequacy with which NPDES permits protect individuals who
may obtain drinking water near the discharge points for uranium mine
dewatering should be evaluated by States.   Under the Public  Water  Systems
provision of the Safe Drinking Water Act,  radionuclide sfarjdajcds now
exist for drinking water.
     5}  Some site specific studies should be considered by  States to
determine the extent to which inactive uranium mines are significant
water pollution sources.
     6)  States with uranium mines should  determine the feasibility of
control of fugitive dust from large surface mines and incorporate  the
recommendations in State Implementation Plans.
     7)  States should require borehole plugs in drilling operations  that
will prevent interaquifer mixing (exchange)  and also seal drilling  holes
at the surface.

7.9  References

EPA80 U.S.  Environmental Protection Agency,  1980,  "Draft Environmental
     Impact Statement for Remedial  Action  Standards for Inactive Uranium
     Processing Sites (40 CFR 192),  "EPA 520/4-80-011.

-------
               APPENDIX A

FEDERAL LAWS, REGULATIONS, AND GUIDES FOR
             URANIUH MINING

-------
 Table  A.l    Federal  laws,  regulations,  and  guides  for  uranium mining
General
Conservation-
Water Preservation
Federal Agency Use Statutes
/
Depti of Int. 1 2,3,4,6,7
BIA(a)
BLM(a) 5
Dept. of Energy 2
Dept. of Agr, 1 2,8d
USFS(a)
EPA 1 2
AIR-OAQPS^
Water
Surface OWPS
Ground OSW(a)
Land-QSW
Radiation-QRP^
U.S. Array
Corps. Qf Engrs. 1 2
Dept. of Labor 2
MSHA(a)
OSHA(a)
Nuclear Reg.
Mining
Permits Environmental Quality
Exploration Mining Water Land
Rights Rights Air Surf UG Solids Reclam.

8 8 2,8
99 9
10 10 10
9 9
11 11 2
2,8d
12,13 13 12
16 19 2
14

17
19
18 18 18 18
15 15 15 15 15

16 2

2 23(b) 23(b) 23(b) 23{l

Health
and
Safety



20


20


22
21
J) 23(b)
wBIA-Bureau of Indian Affairs
   BLM-Bureau of Land Management
   USGS-United States Geological Survey
   USFS-United States Forest Service
OWPS-Office of Water Planning and Standards
OSW-Office of Solid Waste
ORP-Office of Radiation Programs
MSHA-Mining Safety and Health Administration
               .... — - ^ ™  -_, ™_ ___.,.__                    tl*^«»l»llilil!l^,y«'*. \fV \A\ l\A IICUI VII m^tll M]t3bfOiriUM
^b,OAQPS-Office of Air Quality, Planning and Standards  QSHA-Qccupational  Safety and Health Administration
   Nuclear Regulatory  Commission (NRG) regulations and guides for milling  do apply to in situ extraction
   or mining but not conventional  surface or underground mining where NRC  has  no authority.

-------
Table A.I (continued)— Key to Federal laws, regulations and guides cited
 1,  See Appendix B and Appendix C for U.S. Constitution Citations, Federal  Laws,  and Interstate Compacts
 2.  National  Environmental Policy Act of 1969 (Public Law 92-190)
 3.  Endangered Species Act of 1973 (Public Law 93-205) (Supplants Endangered Species Conservation Act of 1969)
 4.  National  Historic Preservation Act of 1966 (Public Law 89-655) (Supplants Antiquities Act of 1906)
 5.  Federal Land Management and Policy Act of 1976
 6.  Reservoir Salvage Act of 1960 (16 USCA 469-469C)
 7.  Historic Sites Acts of 1935 (16 USCA 21-50)
 8.  a.  U.S.  Mining Law of 1872 (30 USC 21-50)
     b.  Mineral Leasing Act of 1920 (30 USC 181 et seq)
     c.  Mineral Leasing Act for Acquired Lands (Amended) (30 USC 351-359)
     d.  Materials Act of 1947 (Amended) (30 USC 601-602)
     e.  Reorganization Plan of 1946 (60 Stat. 1099)
 9.  Indian Land - 30 CFR 231
10.  Public Land - 30 USC 22 (43 CFR 3810, 3746, 3501, 3814.1)
11.  Withdrawn Public Land - 42 USC 2097
12.  National  Forest Land - 16 USC 478 (43 CFR 3811.1 and 36 CFR 252)
13.  National  Forest Management Act of 1976 (16 USC 1600) - Regulations for land and resource management
     planning under this Act In the National Forest System are given in Federal Register Volume 44,
     Number 181, September 17, 1979
14.  Clean Air Act as Amended (42 USC 1857 et seq)
15.  Public Health Services Act (Reorganization No. 3, 1970; Section 301 - Environmental Monitoring)


-------
Table A.I (continued)—Key to Federal laws, regulations and guides cited

16.  Marine Protection Research and Sanctuaries Act of 1972

17.  Federal Water Pollution Control Act as Amended {33 USC 466 et seq)

18.  Resource Recovery and Conservation Act of 1976 (Proposed 40 CFR 250.46-4)

19.  Safe Drinking Water Act Amended (Public Law 95-523 and Public Law 95-190); (Could affect raining operation
     where injection of wastes is utilized)

20.  Atomic Energy Act Amended (Public Law 86-373; 42 USC 2Q21(h)» Federal Radiation Guidance functions from
     prior Federal Radiation Council)

21.  Occupational Safety and Health Act of 1970

22.  MSHA formed by transferring MESA from DO! to DOL pursuant to the Federal Mine Safety and Health Act of 1977,
     Public Law 91-173 as amended by Public Law 95-164

23.  Nuclear Regulatory Commission Guides and Regulations for Benefication Processes

     a.  Regulatory Guide 3.5, Standard Format and Content of License Applications for Uranium Hills
         (Nov. 1977)
     b.  Regulatory Guide 3.8, Preparation of Environmental Reports for Uranium Mills (Sept. 1978)
     c.  Regulatory Guide 3.11, Design, Construction, and Inspection of Embankment Retention Systems for
         Uranium Mills (Dec. 1977)
     d.  Regulatory Guide 4.14, Measuring, Evaluating, and Reporting Radioactivity in Releases of Radioactive
         Materials in Liquid and Airborne Effluents from Uranium Mills (June 1977)
     e.  Regulatory Guide 4.15, Quality Assurance for Radiological Monitoring Programs (Normal Operations) -
         Effluent Streams and the Environment (Feb. 1979)
     f.  Regulatory Guide 8.11, Applications of Bioassay for Uraniurn (June 1975)
     g.  Regulatory Guide 8.13, Instruction Concerning Prenatal Radiation Exposure
     h.  Standards for Protection Against Radiation (10 CFR 20)
     i.  Domestic Licensing of Source Material (10 CFR 40)
     j.  Licensing and Regulatory Policy and Procedures for Environmental Protection (10 CFR 51)
     k.  Proposed Regulations: Uranium Mill Tailings Licensing (10 CFR Parts 40,150) - 44 F.R,
         50012, August 24, 1979

-------
Table A.I (continued)—Key to Federal laws, regulations, and guides cited

     1.  Staff Technical Positions:  Tailings Management - "Current U.S.  Nuclear Regulatory Commission
         Licensing Review Process:  Uranium Mill Tailings Management"; Environmental Monitoring - "Pro-
         posed Branch Position for Operational Radiological Environmental Monitoring Programs for
         Uranium Mills"
     m.  Proposed Regulatory Guide 3.11.1, Operational Inspection and Surveillance of Imbankment Reten-
         tion Systems for Uranium Mill Tailings {April 1979}

-------
                 APPENDIX B
FEDERAL WATER PROGRAMS AND RIGHTS ACTIVITIES
   AND THEIR LEAD ADMINISTRATIVE AGENCIES

-------
      DM 2000, INC
      1833Hormel
    San Antonio, Texas 78219
  (210)222-9124 FAX (210)222-9065
      THIS
      PAGE
    FOUND
    MISSING
FROM DOCUMENTS
 WHILE SCANNING

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                    APPENDIX C
CONGRESSIONALLY APPROVED INTERSTATE MATER COMPACTS

-------
                                                                      C-l
                         Interstate water compacts
              Name                                                    Year

Arkansas River Compact                                                1948
Arkansas River Basin Compact                                          1965
Bear River Compact                                                    1955
Belle Fourche River Compact                                           1943
Canadian River Compact                                                1950
Colorado River Compact                                                1922
Connecticut River Flood Control Compact                               1951
Costi11 a Creek Compact                                                1963
Delaware River Basin Compact                                          1961
Great Lakes Basin Compact                                             1955
Klamath River Basin Compact                                           1957
La Plata River Compact                                                1922
Merrimack River Flood Control Compact                                 1956
New England Interstate Water Pollution Control Compact                1947
New York Harbor (Tri-State) Interstate Sanitation Compact             1935
Ohio River Valley Water Sanitation Compact                            1939
Pecos River Compact                                                   1948
Potomac River Basin Compact                                           1939
Red River of the North Compact                                        1937
Republican River Compact                                              1942
Rio Grande Compact                                                    1938
Sabine River Compact                                                  1953
Snake River Compact                                                   1949
South Platte River Compact                                            1923
Susquehanna River Basin Compact                                       1970
Tennessee River Basin Water Pollution Control  Compact                 1955
Thames River Flood Control Compact                                    1957
Upper Colorado River Basin Compact                                    1948
Wheeling Creek Watershed Protection and Flood  Prevention
     District Compact                                                 1967
Yellowstone River Compact                                             1950

     Source:   Environmental Study on Uranium Mills,  TRW,  Inc.,  USEPA Contract
No. 68-03-2560,  February 1979.

-------
         APPENDIX  0
STATE LAWS, REGULATIONS, AND GUIDES
        FOR URANIUM MINING

-------
                  Table D.I   State  laws,  regulations,  and  guides for uranium mining
General
State

COLORADO
Department of Health
Water Quality Control Div,
Air Quality Control Div.
Department of Natural Resources
Div. of Water Reserves (State
Board of Land Commissioners
Mined Land Reel am. Bd.
Division of Mines
MEW MEXICO
State Land Commission
Dept. of Energy and Minerals
Dept. of Natural Resources
Env. Improvement Div.
TEXAS
Dept. of Water Resources
R.R. Commission of Texas
General Land Office
Dept. of Health
Air Control Board
UTAH
State Engineer
Dept. of Social Services
Division of Health
Water Pollution Control Bd.
NRC
Agreement
State

Yes

-
-

-
-
-
-
Yes
_
-
-
-
Yes
-
-
-
-
-
No
-
-
-
-
NPDES
Permit
State

Yes

-
-

-
-
-
-
No
-
-
-
-
No
-
-
-
-
-
No
-
-
-
-
Water
Use

-

-
-

15
-
-
-
_
_
-
3
-
„
13
-
-
-
-
—
3,4
-
-
-
Permits
Exploration
Rights

-

-
-

-
1
2,3
-
—
1
-
T
-
_
-
1
14
-
-
_
-
-
-
-

Mining
Rights

-

-
-

_
1
2,3
_
_
1
-
-
-
_
3
1
14
_
-
—
-
_
_
-
Mining

Air

-


4,5

-
_
-
_
—
_
_
_
5,6,7
„
.
5
_
_
12
—
-
-
5
-
Environmental
Water
Surf



6,7,8,10
-

-
-
2,3
-
—
_
-
-
,8,9 10,12,13,
™
8,9
5
-
6,10
-
_
-
-
1
1
Quality

UG Sol

-

8,9,10
-

-
-
2,3
-
.
_
-
_
14 11
M>
-
2,7

-
-
.
-
-
1
1

Land
ids Reclam.

_

_
_

_
1
2,3
-
v a*
_ _
2
_
14
_ _
4,11 4
2
15
_
-
_> .•,
_
_
_
-
Safety

-

-
-

-
-
-
14
«*
-
9
.
16
—
_
_
_
10
-

-
,»
5
_
Dept. of Natural  Resources

-------
Table D.I (continued)
                                     GENERAL	   	Mining
                                  NRC        NPOES           	Permits	Environmental Qua 1ity	
                               Agreement     Permit  Water Exploration  Mining    A_1_r   	Water               Land
 State                            State      State    Use  Rlflhts       Rights          Surt         JJG      Solids Reel am.   Saf


 WASHINGTON                       Yes        Yes                          ...           -
  Dept. of Natural Resources      -          -          -1,2         1,2--           -22
  Dept. of Ecology                -          -          9-           -       -       -           ____
   Office of Water Programs       -          -          -                 -       -       8           (No)    -       -
  Dept. of Social Services & Health          -          -     -           __.-...
   Health Services Division       -          -          -     -           -       -       -           -       --         3
   Air Quality Division           -          -          -     -           -       7       -           -       -       -

 WYOMING                          No         Yes                          -                           -
  State Inspector of Mines        -          -          -    Ba          Sa                                           3d       8c
  State Engineers Office          -          -          1-           .__           ..__
  Dept. of Env. Quality           -          -          --           ___           ____
   Air Quality Div.               -          -          -                 -      3a,4     -           -
   Water Quality Div.             -          -          -                 -       -       2,5         5,6     -       .         .
   Land Quality Div.              -          -                3c         3c       -       -           -       3c,7    3c,7
   Solid Waste Management         -          -          -     -           __.           _3d__

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  Table D.I (continued)—Key to State laws, regulations,  and  guides  cited


                                        Col orado

1.   Mining Rules and Regulations, 1973, 1976; Uranium Mining Lease  and Prospecting  Permit;  State Board of
     Land Commissioners.

2,   Colorado Mined Land Reclamation Act, July 1, 1976; Mined Land Reclamation Board (Act,  32,  Title 34,
     C.R.S. 1973, as amended).

3,   Rules and Regulations, Colorado Mined Land Reclamation Board; effective July 1978.
         I
4,   Colorado Air Quality Control Act of 1979, adopted June 20, 1979,   Replaces Colorado Air Pollution
     Control Act of 1970.  Radioactive materials included in  list of air pollutants.

5.   Colorado Air Quality Control Regulations and Ambient Air Quality Standards, Colorado Air Pollution
     Control Commission.  Specifically, Regulation No. 1, Emission Control  Regulations for Particulates,
     Smokes, and Sulfur Oxides for the State of Colorado; and Regulation No, 3, Regulation Governing Air
     Contaminant Emission Notice, Emission Permit, and Fees for Direct Sources.

6,   Regulations Establishing Basic Standards and an Antidegradation Standard and Establishing a System
     for Classifying State Waters, for Assigning Standards, and for  Granting Temporary Modifications,
     Colorado Water Quality Control Commission, May 2E, 1979; effective July 10, 1979.

 7,  Regulations for Effluent Llmftati ons, Colorado Department of Health, Water Quality Control Commission;
     adopted March 18, 1975 effective August 21, 1975.

 8.  Regulations for the State Pischarge Permit System, Colorado Department of Health, Water Quality Control
     Commission; adopted November 19, 1974 effective January 31, 1975, amended February 7» 1978.

 9.  Rules  for Subsurface Pisposal Systems, Colorado Department of Health, Water Quality Control Commission;
     revised July 6, 1976, effective October 1, 1977.

10.  Guidelines  for Control of Water Pollution from Mine Drainage, November 10, 1979; Water Pollution Con-
     trol Commission (Ch 66, Act. 28, C.R.S. 1963 as amended 1970).

11.  Colorado Rules and Regulations Pertaining to Radiation Control, April 1, 1978, Uranium Mill Licensing
     Guide, May  1978; Radioactive Materials License; Radiation and Hazardous Wastes Control Division             G
     (Title 25,  Act. II, C.R.S.  1973, Radiation Control).                                                        »

-------
Table D.I (continued)—Key to State laws, regulations,  and  guides  cited,
         /

12,  Guidelines for the Design, Operation, and Maintenance  of Mill  Tailings  Ponds  to  Prevent  Water
     Pollution, March 13, 1968; Water Pollution Control  Commission  (Colorado Water Pollution  Control
     Act of 1966, Ch. 44, Session Laws 1966 as amended  by Ch. 217).

13,  Publication of a Regulation-Providing Tailings Piles from Uranium and Thorium Mills  be Adequately
     Stabilized or Removed, Colorado Department of Public Health;  effective  June 10,  1966,

14.  Colorado Division of Mines responsible for health  and  safety  standards  for uranium mines and mills.
     Regulations contained in Bulletin 20:  Section 108 - "Missed  Holes—Misfires,"  Section  110 -
     "Mucking,"  Section 12,2 "Radiation Control," Section  130 -  "Safeguards,"  Section 140  -  "Shafts
     and Raises,"

15,  Office of State Engineer, Division of Water Resources  (Article 16, Section 5  - Colorado  Constitution
     and Title 37, Article 90, Section 137 - Colorado Revised Statutes, 1973).
                                                                                                            o

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Table D.I (continued)—Key to State laws,  regulations,  and  guides  cited

                                          New Mexico

 1.   State Land.   Leased by State Land Commission, 19-8-14  NMSA 1978.

 2.   State and Private Land.  Mine plan filed and approved  by  State  Mining  Inspector,  67-5-1  et seq.
     NMSA 1978.

 3.   Water Permit issued by State Engineer; 72-5-1 et seq.  NMSA 1978 and 72-12-1  NMSA  1978 and Desert
     Lands Act of 1866 as amended and 43 USC 383.

 4.   NRC agreement State Under 42 USC 2021.  License  required  for  source material:  unrefined  and un-
     processed ore is not included.  Specific License required for Mills, 10 CFR  40.20 - 40.31,  Ad-
     ministered by Environmental Improvement Division (E1D).

 5.   New Mexico delegated responsibilities and powers under Clean  Air Act (40 CFR 52.1620).
     Ambient Air Quality Standards and Air Quality Control  Regulations,  State of  New Mexico Health
     Department,  Environmental Improvement Division;  reissued  November 1976.

 6.   Application for Permit and Certificate of Registration General  Form for Sources Located  Within
     the State of New Mexico, New Source Review Section, Air Quality Section, Environmental Improve-
     ment Division, revised February 1976.

 7.   Application for Permit to Construct or Modify and Certificate of Registration for Mineral Pro-
     cessing Plants Located within the State of New Mexico, New Source Review Section, Air Quality
     Section, Environmental Improvement Division, revised February 1976.

 8.   Supplementary Information and Notes for Use with Application  for Permit and  Certificate  of
     Registration for Mineral Processing Plants, State of New Mexico - Environmental Improvement
     Division, Air Quality Section, New Source Review Section.

 9.   Monitoring Air Quality in Mines and Mills Underground:  State Mine Inspector 69-5-7 NMSA 1978
     also MSHA (30 CFR 57.5-37) Restricted Areas:  Mills, EID, 74-2-13 NMSA 1978  Unrestricted Areas:
     EID per Clean Air Act (42 USC 7410) and State Radiation Protection Act (74-2-1 et seq. NMSA 1978).

10.   New Mexico Water Quality:  Not NPDES approved by EPA.   State  does not require permit per 74-6-5
     NMSA 1978 and parts 2-100 of N.M. Water Quality  Regulations if  EPA issues NPDES permit.

11.   Underground Water.  State EID regulates pollution of underground water per 74-6-1 et seq. NMSA 1978.
o
I
CJ1

-------
Table D.I {continued}—Key to State laws, regulations,  and guides cited

12.  Water Quality - Radioactivity:  Mines by EID according to Sec.  2-101{b)  of N.M.  Water Quality
     Regulations; Mil Is,by EID per NRC 10 CFR 20.106 and Appendix B.

13.  Water Quality Standards on Enforcement:   EPA enforces under NPDES system for effluent streams
     entering surface water of United States: EID enforces N.M. groundwater standards under N.M,  Water
     Quality Control Act, 74-6-1 et seq. NMSA 1978.
                     *.>
14.  Amended Water Quality Control  Commission Regulation, Parts 1,2,3, and 4, Water Quality Control
     Commission; January 11, 1977,  as amended June 14,  1977 and November 8, 1977.
     Water Quality Standards for Interstate and Intrastate Streams in New Mexico, Water Quality Control
     Commission under the authority of Paragraph C,  Section 74-6-4 of the New Mexico Water Quality Act
     (Chapter 326, Laws of 1973, as amended); adopted August 22, 1973, revised September 29, 1975,
     January 13, 1976, February 8, 1977 and March 14, 1978.

15,  New Mexico Environmental Improvement Agency Uranium Mill  License Application Guidelines,
     Radiation Protection Section; September 1977.

16.  (a) Radiation Protection Act, Chapter 185 Laws  of 1959 (as amended by Chapter 284 Laws of 1971
     and by Chapter 343 Laws of 1977).

     (b)  New Mexico Environmental  Improvement Agency Regulations for Governing the Health and Environ-
     mental Aspects of Radiation, Environmental Improvement Board, June 16, 1973.

-------
  Table D,l (continued)—Key to State laws,  regulations,  and  guides  cited


                                           Texas

'l.  Texas Uranium Surface Mining and Reclamation Act (May 1978),  Rules  of the Surface Mining and
     Reclamation Division.  The Railroad Commission of Texas, July 1,  1979.

 2,  Surface Mining Permit Rule 102 - Elements of Permit  Application,  Rule 250 Reclamation Plan; Rules
     of the Surface Mining and Reclamation Division.

 3,  Application for Permit to Conduct In Situ Uranium Mining, Instructions  and Procedural Information for
     Filing an Application for a Permit to Conduct In Situ Mining  of Uranium,  Texas Department of Water
     Resources.

 4.  Technical Report for In Situ Uranium Mining, Texas Department of Mater Resources.

 5.  Surface Mining Permit, Rule 108 - Permit Approval (Rules of the Surface Mining and Reclamation
     Division),  Permit shall be granted if application complies with Permit rules and all applicable
     Federal and State laws.  Permit may be approved conditioned upon approval of all  other required
     State permits or licenses.

 6.  Texas Department of Health (TDH) issues licenses for surface mining, in situ mining, milling and
     processing of uranium ores and leachates in accordance with NRC Agreement,

 7,  TDH implements U.S. Safe Drinking Water Act regarding public water supplies. The underground injection
     portion of SDWA is regulated by the Railroad Commission {Oil  and fias), Department of Water Resources
     (In situ mining of uranium, salt, and sulfur).

 8,  Texas Regulations for Control of Radiation and Texas Water Quality Standards apply to surface water ,
     throughout state,

 9,  Texas Department of Water Resources issues "no discharge" permits to all  uranium in situ extraction
     processes.

10.  Texas Radiation Control Act, 1971.  Texas Regulations for Control of Radiation (TDH).

11.  Texas Solid Waste Disposal Act, 1969 (Texas Department of Water Resources), Rules pertaining
     to Industrial Solid Waste Management, March 3, 1978.

12.  Texas Air Control Board.  Air Control Board H-76 bill introduced February 1, 1979 to include
     radioactive material  in the definition of air contaminant and allow Board to charge fees for
     permits and variances.

-------
Table 0.1 (continued)—Key to State laws, regulations,  and guides cited

13.  Texas Water Code, Chapter 2 - "Water Use" - Texas  Department of Water Resources.

14.  Rules and Regulations for Prospecting and Mining State-owned minerals.   General  Land Office Rules
     12.6.18.03,001-.006 {Feb. 17, 1976).

15.  Texas Uranium Surface Mining and Reclamation, General Land Office Rules 135,18.05.001-.005.
                                                                                                               C3
                                                                                                                I
                                                                                                               CO

-------
Table D.I (continued)—Key to State laws, regulations,  and guides  cited

                                     -    Utah

1.   Utah Water Pollution Control  Act,  Utah State Divison of Health.
     (a)  Wastewater Disposal Regulations, Part I, Definitions  and General  Requirements,  State  of Utah,
     Department of Social Services, Division of Health; adopted by Utah  Water Pollution  Control  Board,
     May 18, 1965, Utah State Board of Health, May 19,  1965, (Revised  by Utah Water  Pollution Control
     Committee, Nov. 2, 1978) under authority of 26-15-4 to 5 and  73-14-1 to ,13,  Utah  Code  annotated,
     1953, as amended.

     (b)  Wastewater Disposal Regulations, Part II, Standards of Quality for  Waters  of the  State, State
     of Utah Department of Social  Services, Division of Health; adopted  by Utah Water  Pollution Control
     Board May 18, 1965, Utah State Board of Health May 19, 1965,  revised by  action  of the  Boards June 2,  1967
     and June 21, 1967, further revised by action of the Utah Water Pollution Committee  September 13,  1973,  and
     by action of the Utah State Board of Health October 23, 1978.

     (c)  Wastewater Disposal Regulations, Part III, Sewers and Wastiwater Treatment works. Consideration of
     Waste stabilization Ponds (Lagoons) for Industrial Wastes  is  subject to  requirements determined from
     analysis of the engineers report and other available pertinent information  in addition to  sections  83-91.

     (d)  Wastewater Disposal Regulations, Part IV, Individual  Wastewater Disposal Systems.

     (e)  Wastewater Disposal Regulations, Part V, Small Underground Wastewater
     Disposal Systems.

2.   Changes and Additions to the General Rules and Regulations, adopted by the  Board  of Oil,  Gas and
     Mining; March 22, 1978, effective June 1, 1978.

     (a)  Rule M-3 — Notice of Intention to Commence Mining Operations.

     (b)  Rule M-1Q — Reclamation Standards.

3.   Water Laws of Utah and  Interstate Compacts and Treaties (Second Edition, 1964).

4.   State Engineer, H,B. No. 167 - "Temporary Applications to  Appropriate Water" -  introduced  in the
     1979 General Session, an act enacting Section 73-3-5.5, Utah  Code Annotated  1953.
                                                                                                             D

                                                                                                             ID

-------
Table 0.1 (continued)—Key to State laws,  regulations, and guides cittd

5,   Utah Radiation Protection Act; Utah  Code  Annotated,  1953; Title 26, Chapter 25 - Radiation Control.

6.   Utah Air Conservation Regulations, State  of Utah, Department of Social Services, Division of Health;
     adopted by the Utah Air Conservation Committee  and the Utah State Board of Health September 26, 1971;
     revised January 23, 1972; July 9,  1975;   May 22, 1977; February 1979; under authority of 26-15-5 and
     26-24-5 Utah Code annotated,  1953, as amended.

-------
Table D.I (continued)—Key to State laws, regulations,  and guides  cited

                                         Washington

1.   Mineral Leasing Laws, Revised 1965.  (Laws cover surface and  underground  but  not  in  situ  and  heap
     leaching).

2.   Rules and Regulations Relating to Protection and Restoration  of Lands  disturbed through  Surface
     Mining, October 20, 1970 (Surface - Mined Land Reclamation Act, Ch  64, '1970,  Sec.  5  ROW  78.44--
     only applies to surface mining on private and state-owned lands).

3.   Rules and Regulations for Radiation Protection, Chapter-402-22 WAC, Specific  Licenses.

4.   Rules and Regulations for Radiation Protection, Sec, 402-24-220 WAC, Concentrations  in Air and
     Water for Release to Restricted and Unrestricted Areas,   *

5.   Rules and Regulations for Radiation Protection, Chapter 402-24 WAC,
     Standards For Protection Against Radiation.

6.   Rules and Regulations for Radiation Protection, Chapter 402-52 WAC, Uranium and/or Thorium
     Mill Operation and Stabilization of Mill Tailings Piles.

7.   Clean Air Act, Revised Washington Administrative Code, Rev,,  Chapter 70.94, RCW,

8,   Water Quality Standards, State of Washington, Department of Ecology; June 19, 1973.   (Revised
     Dec. 19, 1977).  Water Pollution Control Act of 1970 (as amended).

9.   Department of Ecology - Water Use -
     (a)  Water Pollution Control:  Chapter 90,48 RCW
     (b)  Water Code - 1917 Act;  Chapter 90.03 RCW
     (c)  Regulations of Public Groundwaters:  Chapter 90.44 RCW.

-------
Table D.I (continued)—Key to State laws,  regulations,  and  guides  cited
                                        Wyomi ng
1*   Regulations and Instructions, Part I, Surface Water, Wyoming  State  Engineer's Office,  revised
     January 1974.
2.   Condensed Detailed Instructions for Preparation of Surface  Water Applications and Accompanying Maps
     for Facilities (pollution control  and others) for Mining  and  Other  Industrial Operations, revised
     4-28-78.  Effluent Limitations and Monitoring Requirements:  Wyoming's  BPT  for Uranium Mine  Waters.
3.   Wyoming Environmental Quality Act, as amended, Department of  Environmental  Quality:  1973 Cumulative
     Supplement, 1974 Session Laws, 1975 Session Laws,  1976 Session  Laws,  1977 Session Laws.
     (a)  Article 2 - Air quality Regulations.
     (b)  Article 3 - Water quality.
     (c)  Article 4 - Land Quality.  Buidelines No. 1-6 and 8.
     (d)  Article 5 - Solid Waste Management.
4.   Wyoming Air Quality Standards and Regulations, Department Environmental  Quality,  filed January 25,  1979.
5,   Water Quality Rules and Regulations, Department of Environmental Quality: Chapter I, Quality Standards for
     Wyoming Surface Waters, filed July 17, 1979; Chapter II,  Discharges/Permit  Regulations for Wyoming  1974;
     Chapter IV, Regulations for Discharge of Oil and Hazardous  Substances into  Water  of  the  State of Wyoming,
     June 13, 1978,
6.   Proposed Groundwater Regulations:  WQD Chapter VIII,  Quality  Standards  for  Groundwater of Wyoming (1979);
     WQD Chapter IX, Wyoming Groundwater Pollution Control  Permit  (1979).
7.   Wyoming Land Quality Rules and Regulations, Department of Environmental  Quality,  filed October 6, 1978,
     amended September 13, 1979.
8.   State of Wyoming Non-Coal Mining Laws, Safety Rules and Regulations,  Title  30—Mines and Minerals.
     (a)  Chapter 1 - General Provisions
     (b)  Chapter 2 - Bureau of Mining Statistics
     (c)  Chapter 3 - Mining Operations Generally (Article 4 - Safety Regulations)
      (d)  Chapter 3 - Mining Operations Generally (Article 5 - Open Cut Land Reclamation)
o
1

-------
      APPENDIX E
ACTIVE URANIUM       IN
   THE UNITED STATES

-------
                       ICTIVE PRAKIU*  MIHES  I»  THE UHITED STATED
                        SOURCE]   DOC,  GRAND  JUNCTION, COLORADO
CONTROLLER HA«E
                   COUNT*
RUTH 1 * 4
8ILVER CREEK IND
KAVAJO
BLUE ROCK UOCO HHA
BCHWARTZKAIDER M COTTER CORP
BLACC MA»A IHCE *NG CO
BOMAKZA
CEDAR PT.1-L.CHJ
ELIZABETH 17*11
HOBBARD HJ'STP PA
JULY
LA SAL 4
LIBERT* REtL
LUBSDE1- 1
MINERAL CHA.N io»
?LB-C-G-2»A
NLB-C-G-27
HE* VIBDE
OCTOBER ADIT
PACK RAT 1 * 2
RAJAH 30 SHAFT
RAJAH 67 » 61
ROSEBUD
THORNTON
ZEE LSE, -RAJAH 4
BESSIE 3*1
XARCE GROUP
SAGE-BUELLA
BROKEN BOX
VCA ilATURITA TA1
ADA*
APRIL
8LACK POINT
BLAC.KBURN
BLUE CAP
BOON DOCK
BREEZY
HUCKHORH-UREKA
CANON 4,5 * ^
CLIt FD"ELLER
COL1PAD1UX
CRIPPLE CREEK 2
DONALD L
ECHO 2 » 1
ECHO t
EOUIHOX
ATLAS MtUERALS
* S OAWSOK
GULF STATES CME«
HU5BARO *4NG,
V, C, MOORE3
PIOKC^JJ yRAV I we
MARIO" BIRCH
UNIOl CARBIDE CP
ATLAS-AHAIC
RALPN FOSTER
FOSTER H-COVTLSC
UNION CARBIOE CP
ATLAS-AHAX
UNION CtRBIOE
UNION CARBIDE
UMIOM CARBIOE CP
GRAHA" MKG,
C V HGOD«»BD
UNION CARBIDE
U«10V CARBIDE CP
UN10H CARBIOE CP
UNIOW CARPI&E CP
JOHK DUFUR
DURITA CORP,
CLEGHORI-tWASHP-lll'
ATLAS MINERALS
UNION CARBIDE CP
UNION CARBIDE
GEO--ENCRCY RES
EARL HOT!
U4JIOX CARBIDE CP
t * H IININC
C f COOPER
UNION CARPWr
UHOH CARBIDE CP
UNION CARBIDE CP
UNION CARBIDE
•UCHAEL GPEAGOR
GLEN GRIAGQ*
CLfCHORN + HSHP, UP
MESA
HESA
NtSA
NCSA
»E8A
NESA
KCSA
"ESA
KESA
NESA
MESA
HEE>
MESA
<*ESA
HESA
MESA
MESA ,
MESA
MESA
MESA'
HOf FAT
"OFFAT
HOFFAT
KONTEZUMA
"QNTEZUMA
MONTROSE
MOHTROSE
MONTR05F
MONTROSE
MOt-TROSE
HONIROSE
KONT»08E
HONfROSE
MQNIRDSE
HONTROSE
KONTOOSE
MONTRDSE
KOfTROSI
MONTROSE
KONTR04E
NONTROSE
1C. TOWMSKIP
RANGE
HERSD.
X1NIKG
TCTAtr PROBUCTIQN
MtTKOO (TONS IS Or 01/01/7
3

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20
36
2)
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12
36
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so
so
51
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51
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7
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7


41
45
4*
46
31

45
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41
41
47
47
47
4S
41
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N

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N
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N
1
n
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N
N
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H
K
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K
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H
H
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H
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h
K
H
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5

N
K
H
N
K
N
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13

71
11
JO
19
17
20
{1
20
19
20
tl


11
19
20
30
20
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.0
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.0
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• 0
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.0
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• 0
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22
22
22
22
22
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22
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22
32
32
22
22
32
22
06
06
06


22
22
22
23
24

33
32
33
22
22
J2
32
22
32
22
SURFACE
UNDERGRO
UHDERGRO
UHOERGRO
UfTDERGRO
UNDERGRO
UN0ERGRQ
UNDERCRQ
UNDERGRO
UNDESCRQ
UKDERGRO
UNOERSRO
UKDtRGRO
UNKNOKN
U*DERGRO
UHBMGRO
UNOeftGKO
UNDERGRO
UKDERGRD
UNOERGRO
UNOEHGRQ
UNDERORQ
UNDERGRO
SURFACE
suRf»CE
SURFACE
SURFACE
T»1L,DHP
UNOERCBO
UKOERCRO
UKDCRCRO
UKDERORO
UKDERGRO
auftncc
UNDERCftO
UMDERGRO
UNDERCRO
UNDEXGRO
UNDEAGRO
UKDIKORO
UNDEKSftQ
UNDEKCRO
UMDERGRO
UNOERCRD
1,000 •
100
>100,000
j.ooo «
>100,000
,000 >
,00g .
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• 000 -
,000 »
,000 -
,000 •
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too
>100,000
>100,000
1,000 •
1,000 »
HOOiOOO
>100, 000
100
1,000 •
noo.ooo
1,000 •
>100,OOC
>iOO,OOC
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• 1

100

100
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100
100
100
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100
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• I


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000
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000
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000
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100,000
100


- 1
100

100


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000

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<100
100
l.OOO •
100
100
1,000 -
1,000 -
100
1,000 -
1,000 -
1,000 -
1,000 -
1,000 •
1,000 -
1,000 -
1,000 •
1,000 •
1,000 •
- 1
1
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100,000
• 1
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100
100
- 1
100
100
100
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100
100
100
too
loo
100
1
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000
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000
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000
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000
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DEPIK
tri.j
                                                                                                      150
                                                                                                       SO
                                                                                                      ISO
                                                                                                      100
                                                                                                      400
                                                                                                      200
                                                                                                       50-
                                                                                                      250
                                                                                                       SO
                                                                                                      450
                                                                                                      150
                                                                                                      100
                                                                                                       SO
                                                                                                      100"
                                                                                                      400
                                                                                                      100
                                                                                                      450
                                                                                                      300
                                                                                                      iso
                                                                                                      sso
                                                                                                       50
                                                                                                      100
                                                                                                      450
                                                                                                      100
                                                                                                      100
                                                                                                       so
                                                                                                       50
                                                                                                        0
                                                                                                      330
                                                                                                       SO
                                                                                                        0
                                                                                                      200
                                                                                                      200
                                                                                                        0
                                                                                                        0
                                                                                                      100
                                                                                                       SO
                                                                                                      200
                                                                                                      100
                                                                                                      TOO
                                                                                                      1S»
                                                                                                       50
                                                                                                      too
                                                                                                      ISO
                                                                                                                           m-
                                                                                                                            i

-------
                                  active URANIUM MINE* IN TKZ UNITED STATES
                                   SQIfRCEl  DOE, 5«»ND JUNCTION, COLORADO
HAKE
           CONTROLLER  N*NE
                             COUNTlf
    COLORADO
                 CCQNT'Ol
EULA BELLE CRAIG
FARMER CIRL
FAVN SPRINGS «
CREAGOR CROUP
CREASY SPOC"
GUADALCANU
J M
JACK ICNirC
LONG PARK 11
LONG PARK IS
LONG PARK 1*
LUCKY GPQUP
fiYBt i « 6
HILL 2
MINERAL JOE CROU
MINERAL PARK 4,s
*LS»C-!>L-3J
MLB-C-JO-5
MLB-C-LP-23
KLB-C-SF-11
MLB-C-SR-12
XLB-C-SR-1 J
NLB-C-SR-St
Hi.B-c-5h.i6A
MONOGRAM CLAIH
NIL-TRACE
PEANUT MINES
PEGGY
PICKET COBPAL
PRINCESS
RAVEN
REX KINE
RIKSQCK 5
RINROCK BLUE"! 2
RIKROCK CROUP
RYE 1
SEPTEMBER NORN
BESMQ
SILVER DOLLAR
ST. PATRICK 9
SUNiEAN GROUP
URA
WAND* 3
MHITE FACE
TtLLDK BIRD 1
YELLO" SPOT CBOU
PITCH
UNION CARBIDE
HONOGRAH HSG,
UNION CARBIDE CP
ATLAS-AMAJt
nONEFH URAV INC
UNION CIRPIOC CP
UKIOH CARBIDE
WILLIAMS INC
UNION CARBIDE CP
UNION CARBIDE
UNION CARKIDE CP
ENERGY FUELS KUC
UNIOX CA'BIDE CP
UN10U CARBIDE CP
ATLAS HINrRALS
t ATLA8 MINERALS
1NCS NUC-COVTLSE
CATESrOJC-COVTLSE
INCC MKG-GOVTLSC
CAWSON »-FOVTtSE
•HABAKER-CQVTL3C
rLANGANp-covn.sr
kLEASE DAVSON
DYNOVE LTD
UNIOV CAR»IDE
UN10M CARBIDE CP
ATLAS-lilA]!
KEESHAH, GLEN
DON ANDPErfS
D K. »NDBr>S
rooTi KI^ERALS
CLECHOflf + HAS
UNION CARBIDE CP
UNION CMblDE CP
UHIOK CARBIDE CP
KATIVE RESERVE
UHIOK CARSIOE
ATLAS MINERALS
C + D EXPLORATIO
C H BUNKER
UNION CARBIDE
UNION CARPIDC C
PATTERSON, JAMES
UNION CARBIDE CP
R K DIETZ,
REED KIKIKG
HOHESTAKE HNG CO
MO"TROSE
KQNTROSE
MONTROSE
MO^TROSE
KQITROSE
XONTROSE
•Ot-TUQSE
MONTPQSC
MONTRQSC
KONTRQSE
MONTROSE
UnNTROSir
HO**TPt3SE
MOMTROSC
MONTRQ3E
«IOI»TROSC
NO«TROSE
MOKTROSC
10"TRQSE
KO''TeOSE
KONTOQSE
MONTSOSE
MONTROSE
NONTROSE
MONTPOSE
HONTRQSE
KONTROSE
MONTROSE
NONTKOSE
MOXTHOSE
HOMT»OSE
M01TROSE
NQHTROSE
MO--TRQSC
MO.NTRQSC
KO^TROSE
MO"TI«08E
HOCTBOSE
NOMTROSE
HONTROSE
HONTPOSE
MONTROSE
MONTNOSC
NOWTROBt
KOHTROSE
KONTRQSE
8AGUACHE
]2
27
3 j
11

27

21
21

31
in
26
J2
21
1!








It


t
24
17

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16

10
34

11
10
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47

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4

47
47
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41
46
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44

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47
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tl

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45

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47

47
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47

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H
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N
M

N

K
K

N
N
N
N
H
#








H

N
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N
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N

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N

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N

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N
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J2
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11

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47
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45

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41

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47
41
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41

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H
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N

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N
N
N
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M
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N
N
N

N

N
N

N
N

N
N
N
N
N
N

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17
11
tl
11

17

11
1

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19
n
>7
17
17









17

17
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7

11
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17
17
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17

i
,6
.0
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• 0
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.0
9
.0
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0
.0
.0
,0
.0
.0
.0
D
0
0
0
0
0
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6
0
.0
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.6
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• 0
.0
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.0
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.0
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H
H
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H

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MEDIC,
jj
22
21
22

22

23
22

22
22
12
25
21
32









32

23
29
32
Jl

32

33
23

23
22

22
33
22
22
22
33

32
MIMING
MllHDO
UHDCRSIO
UNDERCftO
UKDZRGRO
UNOERCHO
UNOEKGRO
UMBEASRO
UHDERCRO
(JNDERGRO
UNOCRCRQ
UkDfRG*0
WDIRGRQ
UKDERCRO
UNOE3GRO
UHDERQRO
UNDERCHO
UNDERCRO
UHptftGRD
UNOEftGRO
UdDERSRO
UNDERCPO
UNDERGRO
UKDERGRO
UHSCfiCRQ
UkDtttCRO
UNDEDCRQ
UNDERGRO
UNDEftflRO
UNDERCRO
UKDERGKQ
UHDERGRO
«»DEI>ORO
UNDCRGRO
UKDERGXO
UKDEx&RO
UNDERCRO
UMDERSRO
UNOERCRO
UK&ERCRO
UNDERCRO
VMDCRCRO
UNDERGRQ
UNDERCRO
UNOtRSRO
IINDERSRO
UNDtRCRO
IfNDCRSRO
UNXNOMX
UNUCRSRQ
TOTAL PRODUCTIOd
(TQHJ 11 or Oi/Dl/7
>100,000
,080 "
,OOD •
,000 •
,oao •
,000 -
too
,000 -
,000 »
,060 •
1,000 •
100
1,000 -
1,000 •
MOO, 000
1,000 -
>ioo,ooa
1,000 -
1,900 •
1,000 -
1,000 •
1,000 »
1,000 »
1,000 •
1,000 .
1,000 -
>100,000
1,000 -
1,900 •
1,000 *
too
,000 -
,000 •
,000 •
.000 -
,800 •
,000 •
,000 -
,000 •

1,000 •
1,000 -
MOO, COD
100
1,000 -
$,000 -

MOO. 000

100,000
100,000
100,000
100,000
100,000
- 1,000
100,000
100,000
100,000
100,000
- 1,000
100,000
100,000

100,090

169,000
100,000
100,000
100,000
100,000
100,000
too, ceo
100,000
100,000

100,000
100,000
100,000
- 1,000
100,000
100,000
100,000
100,000
100,000
100,000
100,060
100,000
<100
100,000
100,000

" 1.000
106,000
100,000
<100

DIPTH
tn.)
                                                                                                                ISO
                                                                                                                  0
                                                                                                                160
                                                                                                                ISO
                                                                                                                100
                                                                                                                3SO
                                                                                                                200
                                                                                                                 SO
                                                                                                                200
                                                                                                                300
                                                                                                                200
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-------
                                          ACTIVE UPHSIUH MiNea IN tni UNITED STATES
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