402-R-01-904 ENVIRONMENTAL RADIATION DATA REPORT 108 October - December 2001 United States Environmental Protection Agency Office of Radiation and Indoor Air ------- (This page intentionally left blank) ------- Contents Page List of Tables v Preface vii Acknowledgments ix Data Reporting Conventions xi 1. Air Program 1 Airborne Particulates and Precipitation 1 Plutonium and Uranium in Airborne Particulates 12 2. Drinking Water Program 17 3. Milk Program 33 Pasteurized Milk 33 in ------- (This page intentionally left blank) ------- List of Tables Table Page 1 Reporting Units and Minimum Detectable Concentrations xiii 2 Gross Beta in Airborne Particulates: October 2001 2 3 Gross Beta in Airborne Particulates: November 2001 4 4 Gross Beta in Airborne Particulates: December 2001 6 5 Gross Beta and Specific Gamma in Precipitation: October 2001 8 6 Gross Beta and Specific Gamma in Precipitation: November 2001 9 7 Gross Beta and Specific Gamma in Precipitation: December 2001 10 8 Tritium in Precipitation: October - December 2001 11 9 Plutonium and Uranium in Airborne Particulates: January - December 2001 Composites 13 10 Tritium in Drinking Water: October - December 2001 16 11 Plutonium and Uranium Analyses of Selected Drinking Water Composite Samples: January - December 2001 18 12 Iodine-131 in Drinking Water: January - December 2001 19 13 Alpha, Beta, and Sr-90 Concentrations in Drinking Water: January - December 2001 Composites 21 14 Radium-226, -228 and Gamma-Emitting Radionuclides in Drinking Water: January - December 2001 Composites 24 15 Radionuclides in Pasteurized Milk: October - December 2001 28 ------- (This page intentionally left blank) ------- Preface Environmental Radiation Data (ERD) is compiled and published quarterly by the Office of Radiation and Indoor Air's National Air and Radiation Environmental Laboratory (NAREL) in Montgomery, Alabama, and contains data from the Environmental Radiation Ambient Monitoring System (ERAMS). ERD is published in both hard-copy and electronic formats. Electronic reports are available online at www.epa.gov/narel. The United States Environmental Protection Agency established ERAMS in 1973 with an emphasis on identifying trends in the accumulation of long-lived radionuclides in the environment. ERAMS is comprised of a nationwide network of sampling stations that provide air particulate, precipitation, drinking water, and milk samples. Sampling locations are selected to provide population and geographic coverage for the United States. The radiation analyses performed on these samples include gross alpha and gross beta analysis, gamma analyses, and radionuclide-specific analyses for uranium, plutonium, strontium, iodine, radium, and tritium. This monitoring effort also provides ancillary information on natural background levels and on routine and accidental releases into the environment from stationary sources. The radiochemical procedures used by NAREL to analyze the ERAMS samples are contained in the NAREL Radiochemistry Procedures Manual. Station operation and sample collection are in accordance with procedures contained in the ERAMS Manual (EPA 520/5-84-007, 008, 009). vn ------- (This page intentionally left blank) ------- Acknow ledgmen ts All sampling for the Environmental Radiation Ambient Monitoring System (ERAMS) is performed by volunteer collectors who are frequently members of health departments or related environmental agencies of their respective states. The National Air and Radiation Environmental Laboratory (NAREL), on behalf of the U.S. Environmental Protection Agency, would like to acknowledge the time and effort of these volunteer collectors, who are so essential to the successful operation of ERAMS. The efforts of the sample collectors are especially appreciated during times of emergency operation when sampling frequencies are increased and schedules are sometimes demanding. IX ------- (This page intentionally left blank) ------- Data Reporting Conventions Every laboratory measurement involves uncertainty. When there is little or no radioactivity in a sample, one consequence of measurement uncertainty is the possibility of obtaining a measured value that is less than zero. Such a negative result occurs when random effects in the measurement process cause the measured value for the sample to be less than that of the blank or background, which is subtracted from it. From April 1991 to December 1995, negative results were reported as "not detected" or "ND," and gamma analysis results that were less than their estimated measurement uncertainties were also reported as "ND." In January 1996, both of these practices were discontinued. Although negative activities are physically impossible, the inclusion of negative results in the report allows better statistical analysis of the data. Results of gamma analyses are still reported as "ND" when gamma-emitting radionuclides are not detected. Measurement Uncertainty Each measured valuey is reported with an expanded uncertainty U=k uc(y), which is determined from the combined standard uncertainty uc(y) and the coverage factor h = 2. The interval from y - Utoy + Uis estimated to have a level of confidence of approximately 95%. Significant Figures Expanded uncertainties are reported to two significant figures. Measurement results are rounded to the corresponding number of decimal places. Detection Capability The minimum detectable concentrations (MDCs) for each radionuclide are shown in Table 1. The MDC is defined as the minimum concentration that gives a 95% probability of detection when the detection criteria are chosen to give only a 5% probability of false detection in a blank sample. XI ------- (This page intentionally left blank) ------- Table 1 Reporting Units and Minimum Detectable Concentrations for Radionuclide Analyses Radionuclide Gross Alpha Gross B eta Tritium * Plutonium-238, 239/240 f Uranium-234,235,238 Radium-226 Strontium-90 t Iodine-131 Cesium-137 t Barium- 140 Potassium Potassium-40 Media Water Air Water Precipitation Water Milk Air Water Air Water Water Milk Water Milk (gamma) Water (gamma) Water Milk Water Milk Water Milk Water Water Reporting Unit pCi/L pCi/m3 pCi/L pCi/L pCi/L pCi/L aCi/m3 pCi/L aCi/m3 pCi/L pCi/L pCi/L pCi/L pCi/L pCi/L pCi/L pCi/L pCi/L pCi/L pCi/L g/L g/L pCi/L Minimum Detectable Concentration 2 0.0015 2 2 150 150 0.75 0.1 0.75 0.1 0.02 2 1 4 4 0.3 5 5 15 15 0.06 0.06 50 * The MDC for air is based on an assumed total sample volume of 120,000 nf. Measurement by alpha spectrometry includes combined activities of 239Pu and 240Pu, since the relative contributions of these two isotopes cannot be determined. f The MDC for air is based on an assumed total sample volume of 120,000 m3. J Activity as of the day of counting. Xlll ------- (This page intentionally left blank) ------- 1. Air Program Airborne Participates and Precipitation Gross beta radioactivity measurements and certain specific analyses are performed on air particulates and precipitation samples as indicator measurements in assessing the general (national) impact of all contributing sources on environmental levels of radiation. Airborne particulates are collected continuously at field stations representing wide geographic coverage throughout the United States. Filters (10-cm diameter synthetic fiber) from air samplers are changed twice weekly and field measurements are made with a G-M survey meter 5 hours after collection to allow natural radon isotopes and their progeny to decay. Field estimates are reported to appropriate EPA officials by telephone or mail depending on the activity levels found. The filters are sent to NAREL for more sensitive analysis in a low background beta counter. Gamma scans are performed on all filters showing gross beta activity greater than 1 pCi/m3. The laboratory obtained values are usually lower than the field estimates because of the decay of naturally occurring radionuclides during the time between the two measurements. Precipitation samples are collected at most field stations that collect air filters. These samples are also sent to NAREL where they are composited monthly for gamma scans, tritium, and gross beta activity measurements. A compilation of individual measurements is available from the National Air and Radiation Environmental Laboratory, 540 South Morris Avenue, Montgomery, AL 36115-2601. ------- Table 2 Gross Beta in Airborne Particulates October 2001 Location AL: Montgomery/408 AL: Montgomery /4 1 1 AR: Little Rock AZ: Phoenix CA: Berkeley CA: Los Angeles CO: Denver CT: Hartford DE: Wilmington FL: Jacksonville FL: Miami HI: Honolulu IA: Iowa City ID: Boise ID: Idaho Falls IN: Indianapolis KS: Topeka ME: Augusta MI: Lansing MN: Minneapolis MN: Welch/510 MS: Jackson NC: Charlotte NC: Wilmington ND: Bismarck NH: Concord NJ: Trenton NV: Las Vegas NY: Albany NY: New York City NY: Yaphank OH: Painesville OH: Ross OR: Portland PA: Harrisburg PA: Pittsburgh SC: Barnwell SC: Columbia Number of Samples 9 9 7 5 9 9 9 9 9 9 5 6 9 3 9 9 6 8 9 3 9 9 7 5 7 9 1 9 4 9 8 8 9 8 9 9 1 7 5 -hour Field Estimate Max Min Avg (pCi/m3) 0.1 0.0 0.0 0.2 0.0 0.1 0.1 0.0 0.0 0.9 0.2 0.6 0.2 0.0 0.1 0.3 0.0 0.2 1.2 0.2 0.7 0.2 0.0 0.1 0.3 0.1 0.2 0.2 0.0 0.1 0.0 0.0 0.0 0.1 0.1 0.1 0.3 0.0 0.2 0.5 0.1 0.3 0.4 0.0 0.2 0.6 0.1 0.2 0.2 0.0 0.1 0.3 0.1 0.2 0.8 0.1 0.4 0.7 0.0 0.3 0.1 0.0 0.1 1.7 0.2 0.8 0.4 0.1 0.2 0.2 0.1 0.2 0.2 0.0 0.1 0.3 0.0 0.1 0.2 0.0 0.1 0.3 0.1 0.2 0.2 0.1 0.1 0.9 0.1 0.4 0.0 0.0 0.0 0.4 0.1 0.2 NAREL Lab Measurement Max Min Avg (pCi/m3) 0.014 0.005 0.008 0.019 0.004 0.009 0.016 0.006 0.010 0.028 0.014 0.023 0.014 0.007 0.010 0.024 0.013 0.018 0.020 0.006 0.012 0.015 0.004 0.007 0.020 0.005 0.010 0.012 0.003 0.007 0.006 0.003 0.004 0.006 0.002 0.003 0.014 0.007 0.010 0.013 0.006 0.010 0.013 0.004 0.009 0.015 0.005 0.009 0.015 0.007 0.010 0.022 0.004 0.008 0.014 0.004 0.008 0.014 0.008 0.011 0.018 0.008 0.012 0.020 0.006 0.011 0.019 0.007 0.010 0.009 0.005 0.007 0.014 0.004 0.010 0.015 0.003 0.009 0.004 0.004 0.004 0.018 0.007 0.013 0.015 0.004 0.010 0.026 0.005 0.011 0.017 0.005 0.009 0.015 0.004 0.009 0.025 0.005 0.011 0.008 0.003 0.005 0.020 0.004 0.010 0.016 0.005 0.010 0.011 0.011 0.011 0.017 0.006 0.009 ------- Table 2 (continued) Gross Beta in Airborne Particulates October 2001 Location TN: Knoxville TN: Nashville TN: Oak Ridge/Bethel TN: Oak Ridge/K25 TN: Oak Ridge/Melton TN: OakRidge/Y12 E TN: OakRidge/Y12 W TX: Austin TX: El Pa so UT: Salt Lake City VA: Lynchburg WA: Olympia WA: Spokane Number of Samples 9 5 9 9 9 9 8 9 9 9 9 8 8 5 -hour Field Estimate Max Min Avg (pCi/m3) 0.9 0.0 0.2 0.3 0.1 0.2 1.1 0.3 0.6 1.5 0.4 0.8 1.4 0.3 0.7 1.9 0.0 0.8 0.9 0.2 0.4 0.3 0.0 0.1 0.9 0.3 0.6 0.6 0.1 0.3 1.0 0.4 0.7 0.1 0.0 0.1 0.5 0.1 0.2 NAREL Lab Measurement Max Min Avg (pCi/m3) 0.028 0.007 0.013 0.018 0.005 0.009 0.016 0.005 0.011 0.015 0.006 0.010 0.015 0.006 0.010 0.017 0.006 0.011 0.018 0.005 0.012 0.011 0.004 0.008 0.021 0.013 0.017 0.015 0.006 0.011 0.014 0.005 0.009 0.006 0.002 0.004 0.015 0.006 0.008 ------- Table 3 Gross Beta in Airborne Particulates November 2001 Location AK: Fairbanks AL: Montgomery/408 AL: Montgomery /4 1 1 AR: Little Rock AZ: Phoenix CA: Berkeley CA: Los Angeles CO: Denver CT: Hartford DE: Wilmington FL: Jacksonville FL: Miami HI: Honolulu IA: Iowa City ID: Boise ID: Idaho Falls IN: Indianapolis KS: Topeka ME: Augusta MI: Lansing MN: Minneapolis MN: Welch/510 MS: Jackson NC: Charlotte NC: Wilmington ND: Bismarck NH: Concord NV: Las Vegas NY: Albany NY: New York City NY: Yaphank OH: Painesville OH: Ross OR: Portland PA: Harrisburg PA: Pittsburgh SC: Barnwell SC: Columbia Number of Samples 1 8 8 8 4 8 8 8 9 9 9 4 7 9 5 8 8 7 7 8 4 7 8 2 2 8 9 9 4 9 7 9 9 8 9 9 1 5 5 -hour Field Estimate Max Min Avg (pCi/m3) 0.0 0.0 0.0 0.1 0.0 0.1 0.2 0.0 0.1 0.0 0.0 0.0 1.2 0.2 0.6 0.5 0.0 0.1 0.4 0.1 0.2 1.5 0.4 0.8 0.2 0.0 0.1 0.4 0.1 0.2 0.1 0.0 0.1 0.0 0.0 0.0 0.2 0.0 0.1 0.8 0.0 0.3 0.9 0.0 0.4 0.5 0.1 0.2 0.2 0.0 0.1 0.6 0.1 0.2 0.5 0.1 0.3 3.4 0.0 0.9 1.1 0.0 0.4 0.1 0.0 0.0 3.0 0.3 1.3 0.2 0.1 0.1 0.2 0.0 0.1 0.3 0.0 0.1 0.6 0.0 0.2 0.5 0.1 0.2 0.2 0.0 0.1 1.4 0.1 0.6 0.0 0.0 0.0 0.6 0.1 0.3 NAREL Lab Measurement Max Min Avg (pCi/m3) 0.023 0.023 0.023 0.025 0.006 0.014 0.026 0.006 0.015 0.032 0.007 0.018 0.026 0.014 0.021 0.014 0.003 0.007 0.031 0.007 0.015 0.021 0.008 0.013 0.012 0.006 0.008 0.020 0.008 0.013 0.021 0.006 0.011 0.008 0.004 0.006 0.004 0.002 0.003 0.032 0.009 0.016 0.023 0.004 0.012 0.021 0.008 0.013 0.026 0.005 0.013 0.032 0.008 0.016 0.018 0.004 0.009 0.036 0.006 0.015 0.034 0.013 0.021 0.040 0.004 0.020 0.030 0.003 0.016 0.008 0.008 0.008 0.010 0.008 0.009 0.024 0.009 0.017 0.023 0.005 0.011 0.022 0.004 0.011 0.020 0.010 0.014 0.021 0.006 0.012 0.014 0.005 0.009 0.028 0.008 0.014 0.036 0.009 0.016 0.026 0.002 0.007 0.026 0.007 0.016 0.034 0.008 0.015 0.014 0.014 0.014 0.026 0.012 0.016 ------- Table 3 (continued) Gross Beta in Airborne Particulates November 2001 Location TN: Knoxville TN: Nashville TN: Oak Ridge/Bethel TN: Oak Ridge/K25 TN: Oak Ridge/Melton TN: OakRidge/Y12 E TN: OakRidge/Y12 W TX: Austin TX: El Paso UT: Salt Lake City VA: Lynchburg WA: Olympia WA: Spokane Number of Samples 7 7 7 7 7 7 6 8 7 8 7 6 8 5 -hour Field Estimate Max Min Avg (pCi/m3) 1.1 0.0 0.3 0.2 0.1 0.2 1.7 0.2 0.7 1.6 0.2 0.7 0.9 0.2 0.5 2.1 0.2 0.9 0.7 0.1 0.4 0.4 0.0 0.2 2.2 0.6 1.1 0.5 0.0 0.2 1.4 0.3 0.9 0.2 0.0 0.1 0.2 0.0 0.1 NAREL Lab Measurement Max Min Avg (pCi/m3) 0.061 0.010 0.026 0.033 0.007 0.016 0.031 0.009 0.015 0.048 0.009 0.019 0.030 0.008 0.014 0.033 0.009 0.016 0.043 0.010 0.019 0.026 0.006 0.013 0.025 0.010 0.016 0.018 0.002 0.013 0.033 0.007 0.015 0.019 0.003 0.006 0.039 0.002 0.011 ------- Table 4 Gross Beta in Airborne Particulates December 2001 Location AK: Fairbanks AL: Montgomery/408 AL: Montgomery /4 1 1 AR: Little Rock AZ: Phoenix CA: Berkeley CA: Los Angeles CO: Denver CT: Hartford DE: Wilmington FL: Jacksonville FL: Miami HI: Honolulu IA: Iowa City ID: Idaho Falls IN: Indianapolis KS: Topeka ME: Augusta MI: Lansing MN: Minneapolis MN: Welch/510 MS: Jackson NC: Charlotte NC: Wilmington ND: Bismarck NH: Concord NV: Las Vegas NY: Albany NY: New York City NY: Yaphank OH: Painesville OH: Ross OR: Portland PA: Harrisburg PA: Pittsburgh SC: Barnwell SC: Columbia TN: Knoxville Number of Samples 1 8 3 7 4 8 9 7 7 9 8 4 6 8 9 9 9 6 7 5 6 8 6 3 4 9 7 4 5 9 7 9 7 8 9 1 6 5 5 -hour Field Estimate Max Min Avg (pCi/m3) 0.0 0.0 0.0 0.1 0.0 0.0 0.1 0.0 0.1 0.0 0.0 0.0 0.9 0.3 0.6 0.3 0.0 0.1 0.3 0.0 0.2 1.1 0.3 0.5 0.1 0.0 0.1 0.3 0.1 0.2 0.1 0.1 0.1 0.0 0.0 0.0 0.1 0.1 0.1 0.7 0.1 0.4 0.4 0.0 0.2 0.2 0.0 0.1 0.2 0.1 0.1 0.3 0.1 0.2 0.5 0.1 0.4 0.2 0.1 0.1 0.3 0.0 0.1 1.0 0.4 0.7 0.5 0.0 0.2 0.2 0.1 0.1 0.1 0.0 0.1 0.3 0.0 0.1 0.1 0.0 0.1 0.3 0.1 0.1 0.2 0.0 0.1 0.6 0.1 0.3 0.0 0.0 0.0 0.4 0.1 0.2 0.4 0.1 0.2 NAREL Lab Measurement Max Min Avg (pCi/m3) 0.019 0.019 0.019 0.015 0.004 0.010 0.018 0.009 0.014 0.025 0.012 0.015 0.028 0.007 0.018 0.013 0.002 0.005 0.014 0.004 0.008 0.020 0.007 0.011 0.014 0.006 0.009 0.020 0.011 0.015 0.011 0.004 0.009 0.007 0.002 0.004 0.003 0.001 0.002 0.026 0.013 0.018 0.037 0.003 0.018 0.018 0.010 0.013 0.026 0.009 0.014 0.019 0.007 0.011 0.020 0.013 0.017 0.031 0.013 0.020 0.026 0.010 0.019 0.017 0.007 0.013 0.017 0.005 0.011 0.012 0.007 0.010 0.036 0.011 0.027 0.015 0.009 0.012 0.011 0.005 0.008 0.017 0.012 0.015 0.024 0.006 0.012 0.019 0.006 0.011 0.015 0.007 0.012 0.019 0.011 0.014 0.032 0.001 0.007 0.020 0.011 0.015 0.019 0.009 0.015 0.009 0.009 0.009 0.014 0.005 0.009 0.027 0.008 0.015 ------- Table 4 (continued) Gross Beta in Airborne Particulates December 2001 Location TN: Nashville TN: Oak Ridge/Bethel TN: Oak Ridge/K25 TN: Oak Ridge/Melton TN: OakRidge/Y12 E TN: OakRidge/Y12 W TX: Austin TX: El Pa so UT: Salt Lake City VA: Lynchburg WA: Olympia WA: Spokane Number of Samples 5 8 8 8 8 8 4 6 9 5 8 9 5 -hour Field Estimate Max Min Avg (pCi/m3) 0.2 0.1 0.1 0.7 0.1 0.3 0.9 0.1 0.3 0.4 0.1 0.2 0.6 0.1 0.2 0.3 0.1 0.2 0.1 0.0 0.1 1.6 0.6 1.1 0.2 0.0 0.1 1.1 0.2 0.7 0.2 0.0 0.1 0.1 0.1 0.1 NAREL Lab Measurement Max Min Avg (pCi/m3) 0.017 0.006 0.014 0.019 0.006 0.011 0.020 0.006 0.011 0.018 0.006 0.010 0.019 0.006 0.011 0.023 0.008 0.015 0.014 0.008 0.011 0.024 0.011 0.015 0.047 0.004 0.016 0.016 0.007 0.011 0.015 0.001 0.005 0.028 0.002 0.009 ------- Table 5 Gross Beta and Specific Gamma in Precipitation October 2001 Location AL: Montgomery AR: Little Rock CA: Berkeley CT: Hartford DE: Wilmington FL: Jacksonville FL: Miami HI: Honolulu IA: Iowa City ID: Idaho Falls KS: Topeka ME: Augusta MI: Lansing MN: Minneapolis NC: Charlotte NC: Wilmington ND: Bismarck NH: Concord NY: Albany NY: Yaphank OH: Painesville OR: Portland PA: Harrisburg TN: Knoxville TN: Nashville TX: Austin UT: Salt Lake City VA: Lynchburg WA: Olympia Gross B eta Activity pCi/L ± 2w 0.38 0.33 1.52 0.80 0.82 2.07 0.61 1.62 0.59 1.21 0.80 5.94 0.67 1.37 0.84 2.40 1.73 2.87 0.55 2.05 1.20 0.69 1.40 36.7 0.37 0.29 2.79 11.87 0.06 0.29 0.38 0.45 0.33 0.32 0.43 0.31 0.47 0.32 0.43 0.41 0.59 0.32 0.36 0.33 0.44 0.46 0.46 0.30 0.41 0.35 0.40 0.37 1.4 0.28 0.38 0.52 0.81 0.35 Gamma-Emitting Radionuclides Nuclide pCi/L±2w Pb212 K40 Be7 Pb212 Pb214 Be7 Be7 Ra224 Be7 Bi214 K40 Bi214 Pb212 Ra224 Bi214 Pb214 Be7 Bi214 T1208 3.1 5.6 46 13 ND ND ND 49 30 ND 5.3 6.5 ND ND ND 12.3 7.5 ND 31 18 ND 39 35 ND ND 52 74 ND 35 19 6.5 3.0 11 15 ND 28.0 7.8 5.0 7.0 52 74 7.1 6.5 8.9 6.5 ND ND 58 21 7.8 7.4 1.8 1.3 Note: ND = Not Detected ------- Table 6 Gross Beta and Specific Gamma in Precipitation November 2001 Location AL: Montgomery AR: Little Rock AZ: Phoenix CA: Berkeley CO: Denver CT: Hartford DE: Wilmington FL: Jacksonville FL: Miami HI: Honolulu IA: Iowa C ity ID: Idaho Falls KS: Topeka ME: Augusta MI: Lansing MN: Minneapolis MN: Welch NC: Wilmington NH: Concord NY: Albany OH: Painesville OR: Portland SC: Barnwell SC: Columbia TN: Knoxville TN: Nashville TX: Austin UT: Salt Lake City VA: Lynchburg WA: Olympia Gross Beta Activity pCi/L ± 2w 0.53 1.04 4.84 0.33 4.10 1.21 1.38 1.89 1.60 0.79 0.70 0.92 1.05 5.63 1.69 4.28 8.06 0.71 7.57 1.75 2.29 1.76 7.82 9.85 38.9 0.35 0.43 1.10 12.83 0.20 0.31 0.41 0.64 0.35 0.56 0.36 0.37 0.43 0.40 0.41 0.32 0.41 0.35 0.58 0.39 0.52 0.68 0.32 0.66 0.39 0.43 0.45 0.68 0.74 1.4 0.29 0.38 0.42 0.84 0.34 Gamma-Emitting Radionuclides Nuclide pCi/L±2w Be7 Be7 Pb212 Pb212 Be7 Be7 Pb212 Pb212 T1208 Be7 Be7 Be7 Be7 K40 Be7 K40 ND ND 65 37 ND ND ND 33 36 4.9 5.8 ND ND ND ND 4.0 6.6 42 32 ND 42 21 2.4 2.9 ND 6.2 6.1 2.0 3.5 50 42 42 36 70 22 59 42 ND ND 29 39 ND 28 20 ND ND 19 29 Note: ND = Not Detected ------- Table 7 Gross Beta and Specific Gamma in Precipitation December 2001 Location AL: Montgomery AR: Little Rock AZ: Phoenix CA: Berkeley CO: Denver CT: Hartford DE: Wilmington FL: Jacksonville FL: Miami HI: Honolulu IA: Iowa C ity ID: Idaho Falls KS: Topeka MN: Minneapolis NC: Charlotte NC: Wilmington NH: Concord NY: Albany NY: Yaphank OH: Painesville OR: Portland PA: Harrisburg SC: Columbia TN: Knoxville TN: Nashville TX: Austin UT: Salt Lake City VA: Lynchburg WA: Olympia Gross Beta Activity pCi/L ± 2w 0.74 1.14 2.85 0.32 0.74 2.59 1.61 0.88 1.08 1.12 0.27 0.82 3.98 2.39 1.88 -0.02 3.41 0.24 1.96 2.61 0.59 1.62 3.63 1.68 0.39 0.37 1.39 30.7 0.41 0.39 0.37 0.48 0.29 0.32 0.50 0.46 0.41 0.46 0.37 0.38 0.35 0.58 0.49 0.45 0.36 0.52 0.38 0.46 0.48 0.31 0.43 0.55 0.46 0.35 0.35 0.37 1.3 0.29 Gamma-Emitting Radionuclides Nuclide pCi/L±2w Be7 Be7 Be7 Pb212 T1208 Ra224 T1208 T1208 Be7 Be7 K40 Pb212 Be7 T1208 Bi212 Pb212 29 21 ND ND ND ND 52 38 61 41 4.5 6.5 2.0 3.3 ND ND ND 30 28 2.2 2.8 2.5 3.3 25 19 62 33 ND ND ND 20 37 5.3 6.2 35 32 2.4 3.5 ND 32 48 ND 3.6 5.6 ND ND ND ND Note: ND = Not Detected 10 ------- Table 8 Tritium in Precipitation October - December 2001 Location AL: Montgomery AR: Little Rock AZ: Phoenix CA: Berkeley CO: Denver CT: Hartford DE: Wilmington FL: Jacksonville FL: Miami HI: Honolulu IA: Iowa City ID: Idaho Falls KS: Topeka ME: Augusta MI: Lansing MN: Minneapolis MN: Welch NC: Charlotte NC: Wilmington ND: Bismarck NH: Concord NY: Albany NY: Yaphank OH: Painesville OR: Portland PA: Harrisburg SC: Barnwell SC: Columbia TN: Knoxville TN: Nashville TX: Austin UT: Salt Lake City VA: Lynchburg WA: Olympia October 2001 pCi/L ± 2w -45 81 -22 77 NS 57 80 NS 52 85 2910 160 -31 81 -23 81 3 78 -48 80 8 78 -52 80 17 84 -48 80 28 83 NS 41 83 43 84 35 79 520 100 -54 81 5 82 -12 82 280 89 57 85 NS NS -12 82 -17 82 20 79 29 78 53 84 73 80 November 2001 pCi/L ± 2u -43 78 0 76 -54 74 -32 75 -46 74 188 89 -69 77 26 81 -61 77 -24 75 48 78 -43 74 -24 75 690 110 -11 79 54 78 112 85 NS -82 76 NS -9 78 -6 80 NS 610 110 -37 75 NS 56 83 -4 80 -20 79 -47 78 -13 75 -4 76 211 90 1950 140 December 2001 pCi/L ±2w -82 76 32 79 5 78 30 80 37 80 121 86 9 80 122 86 7 81 -8 78 45 80 30 79 65 81 NS NS 12 78 NS -24 80 4 80 NS 126 86 24 81 13 81 -15 79 30 80 50 83 NS -6 80 -50 78 17 81 30 79 13 78 -45 78 -30 76 Note: NS = No Sample 11 ------- Plutonium and Uranium in Airborne Particulates Environmental radiation levels of plutonium and uranium are determined by the analysis of annually composited samples (air filters) collected from the continuously operating airborne particulate samplers. Concentrations of plutonium-238, combined plutonium-239 and 240, and uranium-234, 235, and 238 are determined by alpha spectrometry following chemical separation. The volume of air represented by the annual composite typically ranges from 120,000 to 500,000 cubic meters. Plutonium and uranium results are published when they become available. Beta Activity in Precipitation All stations routinely submit precipitation samples as rainfall, snow, or sleet occurs. The precipitation samples are composited at the NAREL into single monthly samples for each station. Each month that precipitation occurs, an aliquant of the composited sample is analyzed for gross beta, tritium, and gamma-emitting nuclides. 12 ------- Table 9 Plutonium and Uranium in Airborne Particulates January - December 2001 Composites Location AK: Fairbanks AL: Montgomery/408 AL: Montgomery /4 1 1 AR: Little Rock AZ: Phoenix CA: Berkeley CA: Los Angeles CO: Denver CT: Hartford DE: Wilmington FL: Jacksonville FL: Miami HI: Honolulu IA: Iowa C ity ID: Boise ID: Idaho Falls IN: Indianapolis KS: Topeka ME: Augusta MI: Lansing MN: Minneapolis MN: Welch/510 MS: Jackson NC: Charlotte NC: Wilmington ND: Bismarck NH: Concord NJ: Trenton NV: Las Vegas NY: Albany NY: New York City NY: Syracuse NY: Yaphank OH: Painesville OH: Ross OR: Portland PA: Harrisburg PA: Pittsburgh SC: Barnwell SC: Columbia 238Pu aCi/m3 ± 2w 0.7 1.0 1.2 1.4 1.0 1.4 1.3 2.3 -2.3 4.5 0.9 2.2 1.3 3.3 -0.3 2.3 -0.8 1.3 -0.16 0.75 0.11 0.98 0.32 0.88 0.2 2.1 0.7 1.4 1.2 2.0 1.2 1.9 0.6 2.4 -0.15 0.53 0.3 1.4 0.2 1.9 0.6 1.6 -0.27 0.95 1.1 2.0 -0.2 1.1 0.5 1.4 0.3 1.3 -0.20 0.64 -0.7 1.9 0.3 3.2 0.3 1.1 0.5 1.1 0.6 1.7 -0.4 1.4 1.4 1.5 0.1 2.4 0.5 1.6 0.1 1.2 -0.2 1.7 0.21 0.58 0.54 0.95 239 240pu aCi/m3 ± 2w -0.10 0.35 -0.06 0.37 0.37 0.66 0.15 0.83 -0.9 1.7 -0.26 0.86 -0.81 0.96 0.6 1.0 0.00 0.69 0.00 0.34 -0.11 0.38 0.20 0.51 0.07 0.86 0.31 0.67 0.3 1.1 0.26 0.85 -0.20 0.71 0.00 0.48 -0.38 0.59 -0.09 0.58 0.00 0.57 0.8 1.5 -0.13 0.87 -0.09 0.41 -0.05 0.48 0.33 0.71 0.04 0.47 0.6 1.0 0.7 1.7 0.16 0.46 -0.10 0.66 0.12 0.77 0.21 0.80 0.18 0.52 -0.1 1.1 -0.27 0.84 0.28 0.61 0.07 0.79 -0.10 0.20 0.17 0.46 234U aCi/m3 ± 2w 8.5 1.8 11.7 3.1 8.9 2.4 25.7 5.6 52.4 9.5 10.0 2.2 32.5 6.8 28.7 5.2 12.0 3.0 18.9 3.7 22.1 4.1 12.8 2.7 8.8 2.4 12.4 4.1 30.1 5.4 51.1 9.6 16.6 4.7 20.2 5.4 31.2 6.6 9.9 3.6 13.2 3.7 25.7 8.0 15.4 3.3 16.1 3.4 14.6 2.8 19.9 5.6 13.0 2.4 52.2 8.9 62 11 22.7 4.8 28.4 5.3 24.4 4.6 10.7 2.6 11.3 3.3 27.4 7.0 10.4 2.6 17.3 3.7 35.9 6.4 11.0 2.2 30.1 5.0 235U aCi/m3 ± 2w 0.66 0.51 0.8 1.0 1.24 0.95 1.3 1.3 2.7 2.0 1.68 0.90 2.8 1.9 1.8 1.2 0.17 0.63 1.7 1.0 1.7 1.0 0.68 0.71 0.35 0.71 0.5 1.3 2.0 1.3 3.4 2.2 1.0 1.4 2.8 2.1 2.1 1.7 0.4 1.2 1.2 1.2 0.6 2.2 1.01 0.83 1.10 0.88 1.24 0.79 5.3 3.1 0.78 0.57 2.7 1.7 1.3 1.6 1.6 1.3 4.1 1.8 1.5 1.1 1.08 0.88 0.8 1.1 1.6 1.8 2.1 1.2 3.2 1.5 1.8 1.3 0.81 0.57 1.7 1.0 238U aCi/m3 ± 2w 8.5 1.8 8.9 2.6 8.9 2.4 r\ s- s- en 26.6 5.7 46.0 8.7 8.4 2.0 32.2 6.7 31.5 5.6 11.9 3.0 17.2 3.5 20.7 3.9 8.4 2.0 7.9 2.2 11.0 3.8 28.7 5.2 44.8 8.7 17.7 4.8 15.9 4.6 32.0 6.7 10.7 3.8 9.6 3.1 22.6 7.4 14.5 3.1 16.9 3.5 15.5 2.9 n/~ C 1 .6 5.3 10.5 2.1 49.0 8.5 44.8 8.9 23.5 4.9 i-\i-l 1-1 CO 27.7 5.2 23.6 4.5 10.2 2.5 10.8 3.2 34.2 8.0 9.3 2.5 14.4 3.3 29.2 5.5 10.2 2.1 26.5 4.6 Table 9 (continued) 13 ------- Plutonium and Uranium in Airborne Particulates January - December 2001 Composites Location TN: Knoxville TN: Nashville TN: Oak Ridge/Bethel TN: Oak Ridge/K25 TN: Oak Ridge/Melton TN: OakRidge/Y12E TN: OakRidge/Y12 W TX: Austin TX: El Pa so UT: Salt Lake City VA: Lynchburg WA: Olympia WA: Spokane 238Pu aCi/m3 ± 2w 1.6 2.9 0.2 1.4 0.5 1.5 -2.0 2.5 1.2 1.3 0.1 1.7 0.11 0.99 1.5 2.0 0.2 3.6 -0.1 1.5 0.38 0.83 0.15 0.70 0.7 3.1 239 240pu aCi/m3 ± 2w 0.0 1.4 0.16 0.60 0.9 1.0 -0.14 0.90 0.22 0.47 0.50 0.89 0.55 0.77 0.35 0.96 -0.5 1.1 0.17 0.78 0.25 0.53 -0.02 0.16 0.0 1.2 234U aCi/m3 ± 2w 15.1 6.5 18.8 3.7 9.9 2.6 90 12 7.6 2.2 34.2 6.7 98 14 18.3 3.6 88 17 36.8 6.5 144 18 6.5 1.5 23.6 5.5 235U aCi/m3 ± 2w -1.0 1.8 0.83 0.75 0.43 0.67 8.4 2.2 0.10 0.43 1.7 1.5 6.2 2.3 2.2 1.2 5.7 4.4 1.2 1.1 8.8 2.2 0.29 0.37 0.7 1.4 238U aCi/m3 ± 2w 22.1 7.9 15.0 3.1 9.3 2.6 308 39 5.3 1.8 15.1 4.0 56.1 9.1 16.7 3.4 74 16 34.0 6.2 18.1 3.2 5.5 1.4 25.8 5.8 Note: NA = No Analysis 14 ------- 2. Drinking Water Program The ERAMS drinking water program provides data on radionuclide concentrations in the nation's drinking water supplies. Samples are taken at 78 sites which are either major population centers or selected nuclear facility environs. Drinking water data are used to assess trends and anomalies in concentrations, and to compare with standards set forth in the EPA "National Interim Primary Drinking Water Regulations." These regulations provide for approval of supplies when the combined radium-226 and radium-228 levels do not exceed 5 pCi/L, when the gross alpha (excluding radon and uranium) levels do not exceed 15 pCi/L, when tritium levels do not exceed 20,000 pCi/L, when the strontium-90 levels do not exceed 8 pCi/L, and when the gross beta levels do not exceed 50 pCi/L. The analyses include (a) tritium on a quarterly basis; (b) gross alpha, gross beta, strontium-90, and gamma on annual composites; (c) radium-226 if the gross alpha exceeds 2 pCi/L and radium-228 if the radium-226 falls between 3 and 5 pCi/L; (d) iodine-131 on one quarterly sample per year for each station; and (e) an annual composite for plutonium-238, combined plutonium-239 and 240, and uranium-234, 235, and 238 for stations that demonstrate gross alpha levels greater than 2 pCi/L. 15 ------- Table 10 Tritium in Drinking Water October - December 2001 Location AK: Fairbanks AL: Montgomery AR: Little Rock CA: Berkeley CT: Hartford DE: Dover FL: Miami FL: Tampa GA: Baxley GA: Savannah HI: Honolulu ID: Idaho Falls IL: Morris IL: W. Chicago KS: Topeka MA: Lawrence MD: Baltimore MD: Conowingo ME: Augusta MI: Detroit MI: Grand Rapids MN: Minneapolis MN: RedWing MO: Jefferson City MS: Jackson MS: Port Gibson MT: Helena NC: Charlotte NC: Wilmington ND: Bismarck NH: Manchester NJ: Waretown NM: Santa Fe NV: Las Vegas NY: Albany NY: Syracuse OH: Cincinnati OH: Columbus OH: E. Liverpool OH: Painesville Date Collected 10/17/01 10/01/01 10/05/01 10/26/01 10/03/01 10/04/01 10/17/01 12/19/01 10/10/01 11/15/01 10/23/01 10/24/01 10/03/01 11/15/01 10/02/01 10/01/01 10/04/01 10/31/01 10/02/01 10/16/01 11/20/01 10/29/01 10/15/01 10/04/01 10/02/01 10/02/01 10/05/01 12/12/01 10/22/01 10/05/01 10/16/01 10/15/01 11/20/01 11/15/01 10/04/01 10/18/01 12/10/01 12/31/01 11/01/01 10/03/01 3H pCi/L ± 2w 1400 -57 -61 124 64 -73 -17 15 6 27 -24 76 2 59 9 91 102 135 15 123 107 177 -28 13 30 6 28 630 70 90 -48 -40 80 23 194 41 53 48 74 105 130 78 80 84 77 79 81 80 77 80 76 83 73 82 74 79 79 85 75 84 83 87 81 74 75 74 75 100 80 78 81 80 82 80 82 80 81 76 83 80 16 ------- Table 10 (continued) Tritium in Drinking Water October - December 2001 Location OH: Toledo OR: Portland PA: Columbia PA: Harrisburg PA: Philadelphia/Baxter PA: Philadelphia/Queen PA: Pittsburgh RI: Providence SC: Barnwell SC: Columbia SC: Jenkinsville SC: Seneca TN: Chattanooga TN: Knoxville TN: Oak Ridge - Anderson Co. #768 TN: Oak Ridge - RoaneCo. #4442 TN: Oak Ridge - Knox Co. #371 TN: Oak Ridge - RoaneCo. #360 TN: Oak Ridge - Anderson Co. #772 TX: Austin VA: Ashland VA: Lynchburg WA: Seattle Date Collected 10/04/01 10/05/01 11/02/01 11/01/01 10/18/01 10/18/01 11/01/01 10/01/01 10/22/01 10/03/01 10/24/01 10/16/01 10/03/01 10/01/01 10/17/01 10/18/01 10/26/01 10/26/01 10/30/01 10/15/01 10/03/01 10/03/01 11/19/01 3H pCi/L ± 2w 106 -9 67 111 960 32 92 18 -48 111 17 13 173 153 -13 96 2 29 -31 -9 670 9 12 87 73 82 85 110 84 83 75 75 79 79 82 82 81 77 82 77 79 75 77 100 74 80 17 ------- Table 11 Plutonium and Uranium Analyses Selected Drinking Water Composite Samples January - December 2001 Location CA: Los Angeles GA: Baxley IL: Morris IL: W. Chicago MN: RedWing NE: Lincoln NM: Santa Fe NV: Las Vegas SC: Jenkinsville 238Pu pCi/L ± 2w 0.004 0.027 -0.003 0.042 0.020 0.030 0.013 0.031 0.018 0.045 -0.014 0.015 0.009 0.030 -0.013 0.024 0.007 0.041 239 240pu pCi/L ± 2w 0.007 0.017 0.011 0.021 -0.0010 0.0068 0.0011 0.0097 -0.002 0.014 -0.004 0.011 0.0011 0.0097 0.002 0.011 0.005 0.021 234U pCi/L ± 2w 1.80 0.18 0.037 0.035 0.547 0.087 0.408 0.077 0.297 0.071 4.10 0.35 9.92 0.71 2.41 0.22 3.69 0.35 235U pCi/L ± 2w 0.067 0.033 0.002 0.019 0.025 0.021 0.025 0.022 -0.002 0.015 0.180 0.056 0.499 0.095 0.097 0.038 0.162 0.059 238U pCi/L ± 2w 1.14 0.14 0.032 0.029 0.057 0.027 0.070 0.031 0.066 0.034 2.98 0.27 6.12 0.47 1.39 0.15 1.99 0.22 Note: NA = No Analysis 18 ------- Table 12 Iodine-131 in Drinking Water January - December 2001 Location AK: Fairbanks AL: Dothan AL: Montgomery AL: Montgomery AL: Muscle Shoals AL: Scottsboro AR: Little Rock CA: Berkeley CA: Los Angeles CT: Hartford DE: Dover FL: Miami FL: Tampa GA: Baxley GA: Savannah HI: Honolulu IA: Cedar Rapids ID: Boise ID: Idaho Falls IL: Morris IL: W. Chicago KS: Topeka LA: New Orleans MA: Lawrence MD: Baltimore MD: Conowingo ME: Augusta MI: Detroit MI: Grand Rapids MN: Minneapolis MN: RedWing MO: Jefferson City MS: Jackson MS: Port Gibson MT: Helena NC: Charlotte NC: Wilmington ND: Bismarck NE: Lincoln NH: Manchester NJ: Trenton Date Collected 10/17/01 01/17/01 04/02/01 07/02/01 01/11/01 01/12/01 04/10/01 07/10/01 04/10/01 04/05/01 07/10/01 10/17/01 05/08/01 10/10/01 11/15/01 10/23/01 10/09/01 10/10/01 07/27/01 10/03/01 02/09/01 10/02/01 06/29/01 04/04/01 01/10/01 02/08/01 04/04/01 01/17/01 04/13/01 01/29/01 10/15/01 04/06/01 01/10/01 07/10/01 08/07/01 01/17/01 10/22/01 01/10/01 01/10/01 04/11/01 01/17/01 pCi/L 0.00 -0.04 -0.06 0.01 -0.07 0.03 -0.01 0.12 -0.04 0.19 -0.07 -0.10 -0.03 0.27 0.01 0.03 0.04 -0.07 0.04 -0.04 0.27 0.10 -0.01 -0.05 0.09 -0.24 0.09 -0.02 0.05 0.00 0.14 0.17 0.00 0.00 -0.02 -0.13 0.07 0.02 -0.12 -0.05 0.24 ±2w 0.31 0.18 0.22 0.11 0.19 0.16 0.14 0.25 0.15 0.22 0.26 0.29 0.14 0.51 0.24 0.33 0.18 0.56 0.11 0.22 0.45 0.20 0.16 0.26 0.19 0.58 0.21 0.28 0.20 0.19 0.88 0.24 0.20 0.25 0.17 0.17 0.19 0.16 0.18 0.31 0.18 Table 12 (continued) 19 ------- Iodine-131 in Drinking Water January - December 2001 Location NJ: Waretown NM: Santa Fe NV: Las Vegas NY: Albany NY: Niagara Falls NY: Niagara Falls NY: Syracuse OH: Cincinnati OH: E. Liverpool OH: Painesville OH: Toledo OK: Oklahoma City OR: Portland PA: Columbia PA: Harrisburg PA: Philadelphia/Baxter PA: Philadelphia/Queen PA: Pittsburgh RI: Providence SC: Barnwell SC: Columbia SC: Jenkinsville SC: Seneca TN: Chattanooga TN: Chattanooga TN: Knoxville TN: Oak Ridge - Anderson Co. #772 TN: Oak Ridge - Knox Co. #371 TN: Oak Ridge - Anderson Co. #768 TN: Oak Ridge - RoaneCo. #4442 TN: Oak Ridge - RoaneCo. #360 TX: Austin VA: Ashland VA: Lynchburg WA: Richland WA: Seattle Date Collected 01/17/01 11/20/01 07/09/01 01/11/01 04/19/01 09/29/01 07/19/01 12/10/01 03/02/01 01/08/01 04/05/01 01/10/01 04/05/01 02/08/01 02/08/01 10/18/01 10/18/01 03/02/01 04/09/01 07/09/01 04/05/01 01/18/01 07/25/01 04/03/01 10/03/01 04/09/01 02/22/01 02/22/01 03/08/01 10/18/01 10/26/01 10/15/01 07/12/01 10/03/01 07/16/01 11/19/01 13 pCi/L -0.08 -0.02 0.05 0.08 0.12 0.09 0.07 0.13 0.64 0.08 0.10 0.02 -0.05 0.46 0.12 0.57 2.00 0.23 0.32 -0.02 -0.10 0.10 0.04 0.02 0.11 0.02 0.01 0.08 0.01 -0.10 0.09 0.12 -0.06 -0.02 -0.08 -0.11 ±2w 0.16 0.29 0.15 0.15 0.15 0.12 0.17 0.18 0.14 0.11 0.21 0.17 0.24 0.52 0.47 0.19 0.30 0.15 0.24 0.15 0.26 0.15 0.15 0.14 0.18 0.16 0.16 0.17 0.14 0.18 0.30 0.37 0.22 0.18 0.16 0.28 20 ------- Table 13 Drinking Water Alpha, Beta, and Sr-90 Concentrations January - December 2001 Composites Location AK: Fairbanks AL: Dothan AL: Montgomery AL: Muscle Shoals AL: Scottsboro AR: Little Rock CA: Berkeley CA: Los Angeles CO: Denver CO: Platteville CT: Hartford DE: Dover FL: Miami FL: Tampa GA: Baxley GA: Savannah HI: Honolulu IA: Cedar Rapids ID: Boise ID: Idaho Falls IL: Morris IL: W. Chicago KS: Topeka LA: New Orleans MA: Lawrence MD: Baltimore MD: Conowingo ME: Augusta MI: Detroit MI: Grand Rapids MN: Minneapolis MN: RedWing MO: Jefferson City MS: Jackson MS: Port Gibson MT: Helena NC: Charlotte Total Solids (mg/L) 68.8 93.0 36.3 40.8 52.3 16.8 23.7 35.3 64.2 5.3 21.5 54.8 56.4 143.4 81.3 68.2 78.9 70.3 30.7 63.7 84.8 114.6 108.1 86.3 86.2 58.4 73.3 45.3 44.7 64.1 42.0 74.6 91.0 48.5 88.7 58.7 28.1 Gross Beta pCi/L ± 2w 4.45 0.86 2.0 1.2 1.92 0.79 2.89 0.99 1.03 0.81 1.24 0.66 0.61 0.54 5.2 2.9 2.69 0.76 -0.7 2.1 0.43 0.70 3.1 1.4 2.6 1.1 3.8 1.7 3.64 0.98 2.31 0.92 2.65 0.90 2.47 0.86 0.70 0.54 4.2 1.2 14.1 3.4 11.4 2.4 7.6 2.1 4.0 1.2 2.83 0.94 2.41 0.90 1.4 1.1 1.16 0.81 2.16 0.82 1.91 0.82 3.47 0.84 15.6 2.2 7.4 1.7 2.74 0.86 4.2 1.9 3.36 0.78 1.73 0.73 Gross Alpha pCi/L ± 2w 0.0 1.4 -2.4 2.5 -0.3 1.1 -0.7 1.5 0.1 1.4 0.18 0.68 0.12 0.73 7.3 5.5 1.5 1.6 -0.3 2.5 -0.13 0.73 0.6 2.2 0.3 2.1 0.7 4.7 3.8 2.4 0.4 1.7 0.1 1.9 0.1 1.4 0.29 0.85 0.4 2.2 10.6 7.4 11.4 6.1 -0.4 4.3 0.9 2.2 0.5 1.8 0.1 1.3 -0.2 1.9 -0.5 1.2 -0.1 1.2 -0.1 1.4 0.4 1.1 31.6 5.8 -0.8 3.0 -0.5 1.3 0.0 4.5 0.3 1.3 -0.63 0.89 90Sr pCi/L ± 2w -0.07 0.23 0.05 0.26 -0.18 0.24 0.29 0.58 -0.20 0.45 0.16 0.26 -0.04 0.21 0.24 0.40 -0.14 0.20 0.26 0.23 0.17 0.27 -0.06 0.26 0.20 0.22 21 ------- Table 13 (continued) Drinking Water Alpha, Beta, and Sr-90 Concentrations January - December 2001 Composites Location NC: Wilmington ND: Bismarck NE: Lincoln NH: Manchester NJ: Trenton NJ: Waretown NM: Santa Fe NV: Las Vegas NY: Albany NY: N iagara Falls NY: Syracuse OH: Cincinnati OH: E. Liverpool OH: Painesville OH: Toledo OK: Oklahoma City OR: Portland PA: Columbia PA: Harrisburg PA: Philadelphia/Baxter PA: Philadelphia/Queen PA: Pittsburgh RI: Providence SC: Barnwell SC: Columbia SC: Jenkinsville SC: Seneca TN: Chattanooga TN: Knoxville TN: Oak Ridge - Anderson Co. #768 TN: Oak Ridge - Anderson Co. #772 TN: Oak Ridge - RoaneCo. #4442 TN: Oak Ridge - RoaneCo. #360 TN: Oak Ridge - Knox Co. #371 TX: Austin VA: Ashland VA: Lynchburg Total Solids (mg/L) 78.1 90.2 85.2 47.3 61.6 51.7 102.0 76.6 54.4 52.6 49.7 83.8 90.1 52.6 55.4 61.8 11.5 90.3 18.1 50.5 90.2 73.8 47.4 25.9 45.4 56.9 17.2 45.3 54.6 62.4 60.1 54.0 49.1 59.2 69.2 51.2 29.2 Gross Beta pCi/L ± 2w 4.3 1.0 3.6 1.2 15.1 2.3 0.25 0.76 0.76 0.82 1.89 0.81 11.4 2.0 5.3 2.3 0.40 0.78 1.81 0.86 1.17 0.80 3.9 1.1 3.8 1.2 2.1 1.0 2.57 0.85 3.44 0.91 0.63 0.51 2.44 0.98 0.62 0.82 1.8 1.3 3.9 1.6 2.3 1.1 1.46 0.82 0.68 0.70 2.76 0.89 3.7 1.1 0.13 0.68 2.28 0.80 1.28 0.79 1.95 0.68 1.82 0.69 2.66 0.72 2.22 0.68 1.60 0.65 4.1 1.1 2.1 1.1 0.00 0.71 Gross Alpha pCi/L ± 2w -0.1 1.7 0.3 2.7 9.3 4.6 -0.2 1.1 -0.7 1.5 0.8 1.4 12.5 5.1 2.3 5.1 0.0 1.2 0.0 1.5 0.0 1.2 0.6 2.1 0.6 2.2 0.1 1.7 0.5 1.4 -0.1 1.4 0.03 0.58 -1.5 1.8 0.38 0.94 -0.2 2.0 0.2 2.8 -0.5 1.9 0.3 1.2 0.47 0.98 -1.2 1.3 7.0 2.8 -0.18 0.71 -0.7 1.2 -0.2 1.4 0.8 1.4 0.3 1.3 0.4 1.2 0.0 1.1 0.0 1.2 0.5 1.8 -0.5 1.6 0.57 0.89 90Sr pCi/L ± 2w 0.15 0.24 0.29 0.22 0.38 0.26 0.09 0.25 0.32 0.26 -0.02 0.28 0.15 0.27 0.60 0.33 0.26 0.31 0.02 0.25 22 ------- Table 13 (continued) Drinking Water Alpha, Beta, and Sr-90 Concentrations January - December 2001 Composites Location WA: Richland WA: Seattle Total Solids (mg/L) 29.0 1.6 Gross Beta pCi/L ± 2w 1.34 0.60 -0.03 0.43 Gross Alpha pCi/L ± 2w 0.21 0.82 0.04 0.50 90Sr pCi/L ± 2w -0.01 0.20 -0.15 0.30 23 ------- Table 14 Drinking Water Radium and Gamma-Emitting Radionuclides January - December 2001 Composites Location AK: Fairbanks AL: Dothan AL: Montgomery AL: Muscle Shoals AL: Scottsboro AR: Little Rock CA: Berkeley CA: Los Angeles CO: Denver CO: Platteville CT: Hartford DE: Dover FL: Miami FL: Tampa GA: Baxley GA: Savannah HI: Honolulu IA: Cedar Rapids ID: Boise ID: Idaho Falls IL: Morris IL: W. Chicago KS: Topeka LA: New Orleans MA: Lawrence MD: Baltimore MD: Conowingo ME: Augusta MI: Detroit MI: Grand Rapids MN: Minneapolis MN: Red W ing MO: Jefferson City MS: Jackson MS: Port Gibson MT: Helena 226Ra pCi/L ± 2w NA NA NA NA NA NA NA 0.147 0.024 NA NA NA NA NA NA 1.69 0.19 NA NA NA NA NA 2.61 0.29 1.99 0.22 NA NA NA NA NA NA NA NA NA 3.72 0.42 NA NA NA NA 228Ra pCi/L ± 2w NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA 2.67 0.78 1.11 0.65 NA NA NA NA NA NA NA NA NA 4.12 0.86 NA NA NA NA Gamma-Emitting Radionuclides Nuclide pCi/L±2w ND Pb212 5.2 7.1 T1208 2.3 2.6 ND ND Pb212 5.2 6.5 ND ND ND ND ND ND Pb212 5.7 7.2 ND ND ND ND ND ND ND K40 28 39 ND ND ND ND Bi212 39 40 ND T1208 2.8 4.4 K40 8 13 ND ND K40 18 14 Pb212 5.2 6.9 ND K40 19 34 ND Note: ND = Not Detected NA = No Analysis Table 14 (continued) 24 ------- Drinking Water Radium and Gamma-Emitting Radionuclides January - December 2001 Composites Location NC: Charlotte NC: Wilmington ND: Bismarck NE: Lincoln NH: Manchester NJ: Trenton NJ: Waretown NM: Santa Fe NV: Las Vegas NY: Albany NY: Niagara Falls NY: Syracuse OH: Cincinnati OH: E. Liverpool OH: Painesville OH: Toledo OK: Oklahoma City OR: Portland PA: Co lumbia PA: Harrisburg PA: Philadelphia/Baxter PA: Philadelphia/Queen PA: Pittsburgh RI: Providence SC: Barnwell SC: Columbia SC: Jenkinsville SC: Seneca TN: Chattanooga TN: Knoxville TN: Oak Ridge - Anderson Co. #768 TN: Oak Ridge - Anderson Co. #772 TN: Oak Ridge - RoaneCo. #4442 TN: Oak Ridge - RoaneCo. #360 TN: Oak Ridge - Knox Co. #371 TX: Austin 226Ra pCi/L ±2w NA NA NA 0.181 0.028 NA NA NA 0.163 0.027 0.201 0.031 NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA 0.779 0.094 NA NA NA NA NA NA NA NA NA 228Ra pCi/L ±2w NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA NA Gamma-Emitting Radionuclides Nuclide pCi/L±2w K40 26 37 ND ND ND Pb212 5.0 6.0 K40 35 35 ND ND K40 56 64 ND ND Pb212 4.1 6.6 ND ND ND ND Pb212 4.0 6.2 ND ND ND Pb212 3.4 5.4 ND ND ND ND ND ND Pb212 4.3 6.7 ND ND ND T1208 3.0 4.8 ND ND K40 16 28 K40 22 36 Note: ND = Not Detected NA = No Analysis 25 ------- Table 14 (continued) Drinking Water Radium and Gamma-Emitting Radionuclides January - December 2001 Composites Location VA: Ashland VA: Lynchburg WA: Richland WA: Seattle 226Ra pCi/L ±2w NA NA NA NA 228Ra pCi/L ±2w NA NA NA NA Gamma-Emitting Radionuclides Nuclide pCi/L±2w ND ND ND ND Note: ND = Not Detected NA = No Analysis 26 ------- 3. Milk Program Pasteurized Milk Milk is a reliable indicator of the general population's intake of certain radionuclides since it is consumed fresh by a large segment of the population and can contain several of the biologically significant radionuclides that result from environmental releases from nuclear activities. A primary function of this program is to obtain reliable monitoring data relative to current radionuclide concentrations and determine any long-term trends. Quarterly samples are collected at approximately 55 sampling sites. The samples are composited, according to production, from the major milk suppliers representing more than 80 percent of the milk consumed in a given population center. The samples are analyzed for gamma-emitting nuclides, including iodine-131, barium-140, cesium-137, and potassium-40. Total potassium concentrations in g/L are determined from potassium-40 activities assuming natural isotopic abundances. During the third quarter collection, one-fourth of the samples are also analyzed for strontium-90 on a four year rotating schedule. 27 ------- Table 15 Radionuclides in Pasteurized Milk October - December 2001 Location AL: Montgomery AR: Little Rock AZ: Phoenix CA: Los Angeles CA: Sacramento CA: San Francisco DE: Wilmington FL: Tampa HI: Honolulu IA: Des Moines IL: Chicago IN: Indianapolis KS: Wichita KY: Louisville MA: Boston MD: Baltimore MI: Detroit MI: Grand Rapids MO: Jefferson City MS: Jackson NC: Charlotte NJ: Trenton NM: Albuquerque NV: Las Vegas NY: Buffalo NY: Syracuse OH: Cincinnati OH: Cleveland OR: Portland OR: Portland PA: Philadelphia PA: Pittsburgh TN: Chattanooga TN: Knoxville TN: Memphis TX: Ft. W orth TX: San Antonio VA: Norfolk VT: Montpelier Date Collected 10/10/01 10/15/01 12/19/01 10/11/01 10/23/01 10/10/01 10/09/01 10/09/01 10/15/01 10/15/01 10/22/01 10/12/01 10/22/01 10/31/01 12/28/01 10/05/01 10/08/01 10/08/01 10/09/01 10/08/01 12/26/01 10/11/01 10/09/01 10/25/01 10/12/01 10/09/01 11/05/01 10/03/01 10/02/01 11/01/01 10/09/01 10/11/01 10/08/01 10/08/01 10/15/01 10/10/01 10/22/01 12/19/01 10/03/01 K g/L ± 2w 1.62 0.13 1.48 0.12 1.44 0.12 1.60 0.12 1.55 0.12 1.53 0.12 1.69 0.13 1.54 0.13 1.62 0.12 1.55 0.13 1.56 0.12 1.54 0.12 1.58 0.12 1.64 0.12 1.58 0.13 1.58 0.13 1.63 0.13 1.50 0.16 1.43 0.11 1.61 0.13 1.57 0.12 1.57 0.12 1.54 0.12 1.58 0.12 1.64 0.13 1.53 0.16 1.57 0.12 1.60 0.13 1.61 0.13 1.58 0.12 1.56 0.13 1.57 0.12 1.57 0.13 1.60 0.12 1.47 0.16 1.54 0.12 1.43 0.12 1.55 0.12 1.75 0.14 137Cs pCi/L ± 2w ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND 140Ba pCi/L ± 2w ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND 131j pCi/L ± 2w ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND ND Note: ND = Not Detected 28 ------- Table 15 (continued) Radionuclides in Pasteurized Milk October - December 2001 Location WA: Spokane WA: Tacoma WV: Charleston Date Collected 10/12/01 11/13/01 10/04/01 K g/L ± 2w 1.57 0.13 1.78 0.14 1.63 0.13 137Cs pCi/L ± 2w ND ND ND 140Ba pCi/L ± 2w ND ND ND 131j pCi/L ± 2w ND ND ND Note: ND = Not Detected 29 ------- (This page intentionally left blank) ------- For More Information Environmental Radiation Data (ERD) is published quarterly by the U.S. Environmental Protection Agency's Office of Radiation and Indoor Air. Requests for information concerning the operation of ERAMS and the data that are generated should be directed as follows: For System Operations- For Analytical Information and Data- Rhonda Sears John Griggs National Air and Radiation Environmental National Air and Radiation Environmental Laboratory Laboratory 540 South Morris Avenue 540 South Morris Avenue Montgomery, Alabama 36115-2601 Montgomery, Alabama 36115-2601 e-mail: sears.rhonda@epa.gov e-mail: griggs.john@epa.gov Requests for information concerning publication and distribution of ERD should be directed to: Charles M. Petko Office of the Director National Air and Radiation Environmental Laboratory 540 South Morris Avenue Montgomery, Alabama 36115-2601 e-mail: petko.charles@epa.gov Requests for information concerning policies of the Office of Radiation and Indoor Air should be directed to: Bonnie Gitlin USEPA - ORIA Radiation Protection Division (MC6608J) 1200 Pennsylvania Ave., NW Washington, DC 20460 e-mail: gitlin.bonnie@epa.gov ------- (This page intentionally left blank) ------- |