United States      Office of Air Quality      EPA-450/2-89-002
Environmental Protection  Planning And Standards     April 1989
Agency        Research Triangle Park, NC 27711
AIR
SEPA
      LOCATING AND
      ESTIMATING AIR
     EMISSIONS FROM
        SOURCES OF
        CHROMIUM
         SUPPLEMENT

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                                            EPA-450/2-89-002
                                                August  1989
  LOCATING  AND  ESTIMATING  AIR EMISSIONS  FROM

             SOURCES OF CHROMIUM
                 SUPPLEMENT
                     By

         Midwest Research  Institute
                  Suite 350
         401 Harrison Oaks Boulevard
         Gary, North Carolina  27513

   EPA Project Officer:  Dallas U.  Safriet
    U. S.  Environmental  Protection Agency
         Office of Air and Radiation
Office of Air Quality Planning and  Standards
Research  Triangle Park,  North Carolina  27711
                 August  1989

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This report has been reviewed by the Office of Air Quality Planning And
Standards,  U.  S. Environmental Protection Agency, and approved for
publication.   Any mention of trade names or commercial products is not
intended to constitute endorsement or recommendation for use.
                             EPA-450/2-89-002

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                             TABLE OF CONTENTS

                                                                      Page

LIST OF FIGURES	    ill

LIST OF TABLES	    111

SECTION 1.0  PURPOSE OF DOCUMENT	      1

SECTION 2.0  OVERVIEW OF DOCUMENT CONTENTS	      3

SECTION 3.0  CHROMIUM EMISSION SOURCES	      5

             3,1  CHROMIUM ELECTROPLATING AND CHROMIC ACID
                    ANODIZING OPERATIONS	      5
                  3.1.1  Background Information	      5
                  3.1.2  Uncontrolled Chromium Emissions	     17
                  3.1.3  Emission Reduction Techniques	     21
                  3.1.4  Nationwide Emission Estimates	     23

             3.2  COOLING TOWERS	     26
                  3.2.1  Background Information	     26
                  3.2.2  Potential Emission Reduction Techniques...     29
                  3.2.3  Cooling Tower Emissions	     34
                  3.2.4  Nationwide Emissions Distribution by
                           Industry	     38

SECTION 4.0  SOURCE TEST PROCEDURES	     41

             4.1  CHROMIUM ELECTROPLATING	     41
             4.2  COOLING TOWERS	     41

SECTION 5.0  REFERENCES	     43

APPENDIX A.  ADDITIONAL CHROMIUM ELECTROPLATING EMISSION DATA
             OBTAINED AND EVALUATED DURING DEVELOPMENT OF THIS
             REPORT	    A-l
                                    11

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                              LIST OF  FIGURES

                                                                       Page
 Figure  1.   Flow diagram for  a typical chromic  acid anodizing
             process	      11

 Figure  2.   Internals of crossflow and counterflow cooling  towers...      30

 Figure  3.   Designs of various drift eliminators.....	      33

                              LIST OF TABLES

                                                                       Page

 TABLE 1.    TYPICAL OPERATING PARAMETERS FOR HARD CHROMIUM
              ELECTROPLATING		......       7

 TABLE 2.    TYPICAL OPERATING PARAMETERS FOR DECORATIVE CHROMIUM
              PLATING	       9

 TABLE 3.    CHROMIC ACID/SULFURIC ACID ETCH  SOLUTION	       9

 TABLE 4.    TYPICAL OPERATING PARAMETERS FOR CHROMIC ACID
              ANODIZING	      13

 TABLE 5.    HEXAVALENT AND TRIVALENT           DEPOSIT COMfQSITIONS       16

 TABLE 6.    UNCONTROLLED EMISSION  DATA FOR TOTAL AND HEXAVALENT
              CHROMIUM FROM CHROMIUM PLATING OPERATIONS		      18

 TABLE 7.    TANK PARAMETERS AND PROCESS OPERATING PARAMETERS
              MONITORED DURING CHROMIUM PLATING TESTS	      20

 TABLE 8.    PERFORMANCE LEVELS OF  INDIVIDUAL CONTROL DEVICES	      24

 TABLE 9,    NATIONWIDE        OF OPERATIONS AND ESTIMATED HEXAVALENT
              CHROMIUM EMISSIONS FROM CHROMIUM ELECTROPLATING AND
              CHROMIC ACID ANODIZING OPERATIONS	      25

 TABLE 10.   MODEL COMFORT COOLING TOWERS AND HOURLY BASELINE Cr+6
              EMISSIONS	.	..........	      28

 TABLE 11.   EMISSION FACTORS FOR HEXAVALENT CHROMIUM FROM
              COOLING TOWERS	      36

TABLE 12.   NATIONWIDE COOLING TOWER CHROMIUM EMISSIONS SUMMARY	      40

TABLE A-l.  ADDITIONAL CHROMIUM  ELECTROPLATING EMISSION DATA
              OBTAINED AND EVALUATED DURING DEVELOPMENT OF  THIS
              REPORT.	    A-l
                                    111

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                          1.0  PURPOSE OF  DOCUMENT

      The U. S. Environmental Protection Agency (EPA), States, and local
air pollution control agencies are becoming increasingly aware of the
presence of substances in the ambient air that may be toxic at certain
concentrations.  This awareness, in turn, has led to attempts to identify
source/receptor relationships for these substances and to develop control
programs to regulate emissions.  Unfortunately, very little information is
available on the ambient air concentrations of these substances or on the
sources that may be discharging them to the atmosphere.
      To assist groups interested in inventorying air emissions of various
potentially toxic substances, EPA is preparing a series of documents that
compiles available information on the sources and emissions of these
substances.  This document was prepared as a supplement to a previous EPA
document that addressed chromium emissions, "Locating and Estimating A1r
Emissions From Sources of Chromium," EPA-450/4-84-Q07g.  The supplement
updates technical information and presents new emission data upon which
emission factors are based for chromium emissions from cooling towers and
chromium electroplating operations.  The reader should use both the
original document and this supplement to obtain the most complete
assessment of emissions from these two sources of chromium emissions.  The
information in this supplement was obtained by EPA's Emission Standards
Division for use in development of National Emission Standards for a
Hazardous Air Pollutant (NESHAP) for chromium used in electroplating
operations and for regulation of chromium emissions from comfort cooling
towers under the Toxic Substances Control  Act.
      The reader is strongly cautioned against using the emissions
information contained in the original  document or this supplement to
develop an exact assessment of emissions from any particular facility.
Because of insufficient data, no estimate can be made of the error that
could result when these factors  are used to calculate emissions  from any
given facility.   It is possible, in some extreme cases,  that orders-of-
magnitude differences could result between actual  and calculated
emissions, depending on differences in source configurations,  control
equipment, and operating practices.   Thus, in situations where an accurate

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assessment of chromium emissions is necessary, source-specific Information
should be obtained to confirm the existence of particular emitting
operations, the types and effectiveness of control measures, and the
impact of operating practices.  A source test and/or material balance
should be considered as the best means to determine air emissions directly
from an operation.
      Possible sources of plant-specific information that would be useful
in estimating air emissions of hexavalent chromium include the National
A1r Toxics Information Clearinghouse database maintained by EPA or the
Toxics Release Inventory (TRI) data resulting from Section 313 of the
Superfund Amendments and Reauthorizatlon Act (SARA).  In the absence of
specific Information about the locations of facilities, State Departments
of Commerce, trade associations, or references such as the Thomas Register
ofAmerican Manufacturers may be sources of information.

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                    2.0  OVERVIEW OF DOCUMENT CONTENTS

      This section outlines the information presented in the remaining
sections of this report and indicates whether the information  is new or
whether it is a revision of information presented in the original
document.
      Section 3.1 presents process descriptions for five kinds of
plating/anodizing operations.  New information is Included for decorative
chromium electroplating of plastics, chromic acid anodizing, and trivalent
chromium plating.  Additional process information 1s provided to
supplement the discussion of hard and decorative chromium electroplating
presented in the original document.   New emission data are presented for
hard and decorative chromium electroplating operations; the results of an
engineering mass balance to obtain an emission estimate for chromic acid
anodizing are also presented.  A significant change from the original
document is 1n the format of the chromium emission factors for hard and
decorative plating operations, which have changed from kilograms per hour
per square foot of tank area to milligrams per ampere-hour.  Supplemental
information has been included on emission control techniques for reduction
of chromic acid mist from plating operations.   New information Is
presented on nationwide chromium emission estimates for three types of
plating operations:  hard plating, decorative  plating, and chromic acid
anodizing.
      Section 3.2 presents updated information about the distribution of
industrial process cooling towers that  use chromium-based water treatment
chemicals and presents new information  about comfort cooling towers.  New
information also is presented on emission reduction techniques for
chromium emissions from cooling towers.   New emission data are presented
for cooling towers equipped with low- and high-efficiency drift
eliminators.   A significant change from the original document Is in the
format of the chromium emission factor,  which  has changed from picograms
per joule of  thermal  energy input to the power plant associated with the
cooling tower to percentage of the recirculating  chromium that is
emitted.  New information is presented  on nationwide chromium emission
estimates for industrial  cooling towers  in eight  Industries,

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      Section 4.0 summarizes the procedures used for source sampling and
analysis of chromium In emission streams from electroplating operations
and cooling towers.

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                      3.0  CHROMIUM EMISSION  SOURCES

3.1  CHROMIUM ELECTROPLATING AND CHROMIC ACID ANODIZING OPERATIONS
3.1.1  Background Information
      Plating and anodizing operations range  in size from small shops,
with one or two tanks that are operated only  a few hours per week, to
large shops with several tanks that are operated 24 hours per day, 7 days
per week.  Many plating and anodizing operations are captive shops that
perform chromium electroplating or chromic acid anodizing as one operation
within or for a manufacturing facility, while others are job shops that
provide custom plating or anodizing services  for many different clients.
Captive and job shops may perform hard or decorative chromium plating or
chromic acid anodizing or any combination of  these three operations.
      The estimated number of electroplating  shops nationwide is
1,540 hard chromium plating facilities and 2,800 decorative chromium
plating facilities.   The estimated number of chromic acid anodizing shops
                  2
nationwide is 680.   Electroplating and anodizing shops typically are
located in or near industrial centers in areas of high population
density.  States with large numbers of chromium electroplaters include
California, Illinois, Massachusetts,  Michigan, New York, Ohio, and
Pennsylvania.
      3.1.1.1  Hard Chromium Electroplating of Metals.   In hard plating, a
relatively thick layer of chromium is deposited directly on the base metal
(usually steel) to provide a surface  with wear resistance,  a low
coefficient of friction, hardness,  and corrosion resistance, or to build
up surfaces that have been eroded by  use.   Hard plating is used for items
such as hydraulic cylinders and rods,  industrial  rolls,  zinc die castings,
plastic molds, engine components, and marine hardware.
      Tanks used for hard chromium electroplating usually are constructed
of steel and lined with  a polyvinyl chloride sheet or  plastisol.   The
anodes, which are insoluble,  are made of a lead alloy  that  contains either
tin or antimony.  The substrate to  be plated,  the cathode,  is suspended
from a plating rack that is connected  to the cathode bar of the
rectifier.   The plating  rack  may be  loaded in  the tank manually,  by a
hoist,  or by an automatically controlled hoist system.

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      The plating tanks typically are equipped with some type of heat
exchanger.  Mechanical agitators or compressed air supplied through pipes
on the tank bottom provide uniformity of bath temperature and
composition.  Chromium electroplating requires constant control of the
plating bath temperature, current density, plating time, and bath
composition.
      Hexavalent chromium plating baths are the most widely used baths to
deposit chromium on metal.  Hexavalent chromium baths are composed of
chromic acid, sulfuric acid, and water.  The chromic acid is the source of
the hexavalent chromium that reacts and deposits on the metal and that is
emitted to the atmosphere.  The sulfuric acid in the bath catalyzes the
chromium deposition reactions.  Typical operating parameters are given in
Table 1."
      The evolution of hydrogen gas from chemical reactions at the cathode
consumes 80 to 90 percent of the power supplied to the plating bath,
leaving the remaining 10 to 20 percent for the deposition reaction.  When
the hydrogen gas evolves, it entrains chromic acid and causes misting at
the surface of the plating bath,
      3.1.1.2  Decorative Chromium Electroplating of Metals.  In decorative
plating, the base material (e.g., brass, steel, aluminum, or plastic)
generally is plated with a layer of nickel followed by a relatively thin
layer of chromium to provide a bright surface with wear and tarnish
resistance.  Decorative plating is used for items such as automotive trim,
metal furniture, bicycles, hand tools, and plumbing fixtures.  The purpose
of decorative chromium plating is to achieve a combination of the
following surface properties:
      1.  Blue-white color;
      2.  High reflectivity;
      3.  Tarnish resistance;
      4.  Corrosion resistance;
      5.  Wear resistance; and
      6.  Scratch resistance.
      Decorative electroplating baths operate on the  same principle as
that described for the hard chromium plating process:   the metal  substrate
is immersed in a plating solution,  and direct current  is passed  from the

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  TABLE 1.   TYPICAL OPERATING PARAMETERS FOR HARD CHROMIUM ELECTROPLATING
Plating thickness, vm (mil)                               1.3-762  (0.05-30)
Plating time, mina                                                20-2,160
Chromic acid concentration, g/£ (oz/gal)b                  225-375  (30-50)
Temperature of solution, °C (°F)                           49-66  (120-150)
Voltage, volts                                                          c
Current, amperes (A)                                                    d
Current density, A/nt2 (A/ft2)6                                1,600-6,500
                                                                  (150-600)
?min. = minutes.
 g/s, = grams per liter,  oz/gal = ounces per gallon.
^Depends on the distance between the anodes and the items being plated.
 Depends on the amount of surface area plated.
eA/m  = amperes per square meter (square foot) of surface area plated.

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anode through the plating solution causing the desired metal  (copper,
nickel, chromium) to deposit out of the solution onto the metal substrate
(cathode).
      Decorative chromium plating requires shorter plating times and
operates at lower current densities than does hard chromium plating to
achieve the desired properties of the chromium plate.  Some decorative
chromium plating operations use fluoride catalysts instead of sulfuric
acid because fluoride catalysts, such as fluosilicate or fluoborate, have
been found to produce higher bath efficiencies.   Typical operating
parameters are shown in Table 2.
      3.1.1.3  Decorative Chromium Electroplating of Plastics.  Most plastics
that are electroplated with chromium are formed from the polymer composed
                                               a
of acrylonltrile, butadiene, and styrene (ABS).   The process for chromium
electroplating of ABS plastics consists of the following steps:
      1.  Chromic acid/sulfuric acid etch;
      2.  Dilute hydrochloric acid dip;
      3.  Colloidal  palladium activation;
      4.  Dilute hydrochloric acid dip;
      5.  Electroless nickel plating or copper plating;  and
      6.  Chromium electroplating cycle.
      After each process step, the plastic is rinsed with water to prevent
carry-over of solution from one bath to another.  The chromic acid/
sulfuric acid etch solution (see Table 3)  renders the ABS surface
hydrophilic and modifies the surface to provide adhesion for the metal
coating.   The dilute hydrochloric acid dips  are used to clean the surface
and remove palladium metal  from the plating rack, which  is insulated with
a coating of polyvinyl  chloride.   The colloidal  palladium activation
solution deposits a  thin layer of metallic palladium over the plastic
surface. °  The metallic palladium induces the deposition of copper or
nickel,  which will  not deposit directly onto  plastic. The electroless
nickel  and copper plate are applied to impart electrical  conductivity to
the part;  otherwise, the insulating surface of the plastic could not be
electroplated with chromium.  The electroless nickel  plating or copper
electroplating baths develop a film on the plastic about  1.0 micrometer
(urn)  (3.9xl(T5 inch  [in.])  thick.   The plating time for  electroless nickel
                                    8

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  TABLE 2.  TYPICAL OPERATING PARAMETERS FOR DECORATIVE CHROMIUM PLATING
Plating thickness, wm (mil)                         0.003-2.5 (0.0001-0.1)
Plating time, min                                                   0.5-5
Chromic acid concentration, g/i (oz/gal)                   225-375 (30-50)
Temperature of solution, °C (°F)                           38-46 (100-115)
Voltage, volts                                                          a
Current, A                                                              b
Current density, A/m2 (A/ft2)c                          540-2,400 (50-220)
^Depends on the distance between the anodes and the items  being plated.
D0epends on the amount of surface area being plated,
cAmperes per square meter (square foot) of surface area plated.
            TABLE 3.  CHROMIC ACID/SULFURIC ACID ETCH SOLUTION
      Concentrated sulfuric  acid,  g/a  (oz/gal)               172 (23)
      Chromic acid,  q/l  (oz/gal)                             430 (57)
      Temperature, °C (°F)                            60-65  (140-149)
      Immersion time, min                                       3-10

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pitting and electroless  copper plating ranges from  10 to  15 minutes  and  15
to 30 minutes, respectively, at temperatures ranging  from 25° to  35*C  (77°
to §5°F),  The components of the plating baths  Include the metal  salt
(nickel or copper), a reducing agent, a complexlng  agent, a stabilizer,
and a pH buffer system.11  The electroplating of  plastics follows the  same
cycle as that described  for decorative chromium electroplating.
      3.1.1.4  ChromicAcid Anodizing.  Chromic acid  anodizing is used primarily
on aircraft parts and architectural structures  that are subject to high
stress and corrosion.  Chromic acid anodizing is  used to  provide an  oxide
layer on aluminum that imparts the following properties:
      1.  Corrosion protection;
      2,  Electrical insulation;
      3.  Ease of coloring; and
      4,  Improved dielectric strength.
Figure 1 presents a flow diagram for a typical  chromic  acid anodizing
process.
      There are four primary differences between  the  equipment used  for
chromium electroplating  and that used for chromic acid  anodizing:
(a) chromic acid anodizing requires the rectifier to  be fitted with  a
rheostat or other control mechanism to permit starting  at about 5 V,
(b) the tank is the cathode in the electrical circuit,  (c) the aluminum
substrate acts as the anode, and (d)  sldewall shields typically are used
instead of a liner in the tank to minimize short  circuits and to decrease
the effective cathode area.    Types of shield materials used are
herculite glass, wire safety glass, neoprene, and vinyl chloride
polymers.
      The following pretreatment steps typically are used to clean the
aluminum before anodizing:
      1.  Alkaline soak;
      2.  Desmut;
      3.  Etching; and
      4.  Vapor degreasing.
The pretreatment steps used for a particular aluminum substrate  depend
upon the amount of smut and the composition of the aluminum.   The aluminum
substrate Is rinsed between pretreatment  steps to remove cleaners.
                                    10

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             SUBSTRATE TO BE PLATED
               PRETREATMENT STEPS

               Alkaline soak
               DesmuI
               Etching
               Vapor degreasina
                          RINSE
            CHROMIC ACID  ANODIZING
CHROMIC ACID
  EMISSIONS
                          RINSE
                     SEALING
                  FINAL PRODUCT
Figure 1.   Flow diagram for a typical  chromic acid anodizing process
                                 11

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      The alkaline soak is the primary preparatory step in cleaning  the
aluminum; Its purpose Is to dislodge soil from the aluminum surface.  The
solutions for alkaline cleaning are typically made up of compounds such as
sodium carbonate, sodium phosphate, and sodium hydroxide and usually
contain a small amount of silicate to prevent metal attack.    The
alkaline soak consists of immersing the metal in the alkaline solution
that  1s mildly agitated with air.
      The purpose of desiutting is to remove soil or grease films that
cleaners and etchants leave behind.  Desmuttlng baths typically consist of
a cold nitric add solution mixed with water at a concentration ranging
from  5 to 50 percent acid by volume.  The nitric acid bath also is used
either as a bleaching treatment to remove dyes from faulty coatings or as
part  of the technique of producing multicolor coatings.    Other
desmuttfng treatments use combinations of chromic, phosphoric, and
sulfurlc acids depending upon the amount of smut to be removed or the
aluminum composition.
      When a dull finish is desired, the aluminum is etched before
anodizing.  Etching baths consist of a dilute solution of soda ash,
caustic soda, or nitric acid.16  The degree of etching desired and the
composition of the aluminum being treated determine the concentration of
the etch solution, temperature of the bath, and duration of the etch.
      The vapor degreasing step removes any residual  oil or grease on the
surface of the aluminum prior to the anodizing operation.
      Typical operating parameters for chromic acid anodizing baths are
presented in Table 4.  *    The voltage is applied step-wise (5 V* per*
minute) from 0 to 40 V and maintained at 40 V for the remainder of the
anodizing time.   A low starting voltage (i.e.,  5 V) minimizes current
surge that may cause "burning"  at contact points between the rack and the
aluminum part.   The process is  effective over a wide range  of voltages,
temperatures, and anodizing times.  All  other factors being equal, high
voltages tend to produce bright transparent films,  and lower voltages tend
to produce opaque films.     Raising the bath temperature increases current
density to produce thicker films  in a given time period.  Temperatures up
to 49°C (120°F)  typically  are used to produce films that are  to  be colored
by dyeing.     The amount of current varies depending  on  the size  of the
                                    12

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      TABLE 4.  TYPICAL OPERATING  PARAMETERS FOR CHROMIC
                        ACID AKODIZING
Chromic acid concentration, g/a (oz/gal)    50-100 (6.67-13.3)
Temperature, JC (°F)                             32-35 (90-95)
Plating time, min                                       30-60
pH                                                   0.5-0.85
Current density, A/m2 (A/ft2)3           1,550-7,750 (144-720)
Voltage (step-wise), volts                              30-40
Film thickness, ym (mil)                  0.5-1.27 (0.02-0.05)
aAmperes per square meter (square foot) of surface area
 plated.
                               13

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aluminum parts; however, the current density typically ranges from 1,550
to 7,750 A/m2  (144 to 720 A/ft2).
      The postanodizing steps Include sealing and air drying.  Sealing
causes hydration of the aluminum oxide and fills the pores in the aluminum
surface.  As a result, the elasticity of the oxide film increases, but the
hardness and wear resistance decrease.    Sealing is performed by
immersing aluminum in a water bath at 88° to 99°C (190° to 21Q°F) for a
                      2 U
minimum of 15 minutes.    Chromic acid or other chromates may be added to
the solution to help improve corrosion resistance.  The aluminum is
allowed to air dry after it is sealed.
      3.1.1.5  Trivalent Chromium Plating.  Trivalent chromium
electroplating baths have been developed primarily to replace decorative
hexavalent chromium plating baths.  Development of a trivalent bath has
proven to be difficult because trivalent chromium solvates in water to
form complex stable ions that do not readily release chromium.  The
trivalent chromium baths that have been developed are proprietary baths.
      There are two types of trivalent chromium processes on the market:
single-cell and double-cell.  The major differences in the two processes
are that (1) the double-cell process solution contains minimal-to-no
chlorides whereas the single-cell process solution contains a high
concentration of chlorides; and (2) the double-cell process utilizes lead
anodes that are placed in anode boxes that contain a dilute sulfuric acid
solution and are lined with a permeable membrane whereas the single-cell
process utilizes carbon or graphite anodes that are placed in direct
contact with the plating solution.
      The advantages of the trivalent chromium processes over the
hexavalent chromium process are (1) fewer environmental  concerns,
(2) higher productivity, and (3)  lower operating costs.   In the trivalent
chromium process, hexivalent chromium is a plating bath  contaminant.
Therefore, the bath does not contain any appreciable amount of hexavalent
chromium,  which is more toxic than trivalent  chromium.   The total chromium
concentration of trivalent chromium solutions is approximately one-fifth
that of hexavalent chromium solutions.     As  a result of the chemistry of
the trivalent chromium electrolyte, misting does not occur during plating,
as it does during hexavalent chromium plating.   Use of trivalent  chromium
                                    14

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also reduces waste disposal problems and costs.  Waste treatment of
hexavalent chromium is a two-stage process.  The hexavalent chromium is
first reduced to the trlvalent chromium ion; then it can be precipitated
as chromium hydroxide.  Trivalent chromium plating solution wastewaters
are already in the reduced trivalent state and require only the chromium
hydroxide precipitation step.
      Productivity is increased when trivalent chromium processes are used
because less stripping and replating of parts are required, more parts can
be placed on a rack, and more racks can be placed on a workbar.
      The cost of operating a trivalent chromium process is less than that
of a hexavalent chromium process because of the lower wastewater treatment
costs and lower operating costs due to a reduction in rejects and high
productivity.
      The disadvantages of the trivalent chromium process are that the
process is more sensitive to contamination than the hexavalent chromium
process and the trivalent chromium process cannot plate the full range of
plate thicknesses that the hexavalent chromium process can.28  Because it
is sensitive to contamination, the trivalent chromium process requires
more thorough rinsing and tighter laboratory control than the hexavalent
chromium process.  Trivalent chromium baths can plate thicknesses ranging
up to 0.13 to 25 micrometers (urn) (0.005 to 1.0 mils).28  The hexavalent
chromium process can plate thicknesses up to 762 ym (30 mils).  Therefore,
trivalent chromium solutions cannot be used for most hard chromium plating
applications.
      The plating efficiency of a trivalent chromium bath,  approximately
20 to 25 percent, is slightly higher than that of a hexavalent chromium
plating bath.29  The color, hardness, and corrosion resistance of triva-
lent chromium deposits are comparable to those of hexavalent chromium
deposits.30  However,  the composition of the trivalent chromium deposit is
significantly different than that of the hexavalent chromium deposit.
Table 5 presents the composition of trivalent and hexavalent chromium
deposits.31
                                    15

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     TABLE 5.  HEXAVALENT AND TRIVALENT CHROMIUM DEPOSIT COMPOSITIONS
Chromium deposit      Carbon,  % wt       Oxygen,  % wt        Chromium,  $ wt
Hexavalent                 0.0               0.4               99+
Trivalent                  2.9               1.6               95+
                                    16

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3.1.2  Uncontrolled Chromium Emissions
      Emissions of chromic acid mist from the electrodeposltion of
chromium from chromic add plating baths occur because of the inefficiency
of the hexavalent chromium plating process; only about 10 to 20 percent of
the current applied actually is used to deposit chromium on the item
plated.  Eighty to ninety percent of the current applied is consumed by
the evolution of hydrogen gas at the cathode with the resultant liberation
of gas bubbles.  Additional bubbles are formed at the anode due to the
evolution of oxygen.  As the bubbles burst at the surface of the plating
solution, a fine mist of chromic acid droplets is formed.
      3.1.2.1  Hard Chromium and Decorative Electroplating Operations.
Uncontrolled emission data for 10 hard chromium plating operations and
2 decorative chromium plating operations are presented in Table 6.  These
data were obtained from 11 EPA tests and 1 non-EPA test.  Table 7 presents
tank parameters and process operating parameters monitored during each of
the 12 tests.  The process parameters monitored during testing include
current supplied to the plating baths, voltage, chromic acid concentration,
and temperature of the plating baths.  The chromic acid concentration and
temperature did not vary significantly within each type operation for the
emission tests and appeared to be representative of typical  operating
values for conventional hard and decorative chromium plating operations.
The amount of current supplied during testing varitd considerably because
of the different types and quantities of parts plated.
      Based on the existing test data, an uncontrolled emission factor of
10 milligrams of hexavalent chromium per ampere-hour (mg/Ah) (0.15 grain
per ampere-hour Igr/AhJ) is considered to be representative  of uncon-
trolled emissions from a hard chromium electroplating operation, and an
uncontrolled hexavalent chromium emission factor of 2 mg/Ah  (0.03 gr/Ah)
is considered representative of uncontrolled emissions from  a decorative
chromium electroplating operation.
      The emission factor for uncontrolled chromium emissions from
decorative chromium plating operations is based on EPA-approved  test data
from two plants whose tanks represent the extremes in tank size  for
decorative chromium plating.   Although the sizes  of these tanks  may not be
                                    17

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                        TABLE 6.  UNCONTROLLED EMISSION DATA  FOR  TOTAL AND HEXAVALENT CHROMIUM FROM
                                               CHROMIUM PLATING OPERATIONS8
CD
Process conditions
Plant
Total tank
No. of surface area,
tanks m2 (ft2)
Ampere-
hours
Actual
gas flow
rate,
m /m i n
(ftVmin)
Mass emission
rate, kg/h (tb/h)
Total Cr
Crto
Process Cr emission
rate, mg/A*h (gr/A«h)
Hard chromium plating
Plant Ab'32
Plant Bc'33
Plant Cd'34
Plant Dc'35
Plant Ec'36
Plant Ff«37
Plant Qc«38
Plant Hc'39
Plant l'-40
Plant Jc'41
Average
I 5.8
(63)
2 2.5
(27)
1 8. 4
(90)
1 5.2
(56)
1 3.4
(37)
1 1.8
(20)
1 1.4
(1.5)
1 5.5
(60)
2 9.0
(99)
3 6.6
(?D

14,000
14,400
20 ,000
19,800
11,700
12,200
8,900
3,440
8,530
8,790

226
(7,970)
152
(5,390)
339
(12,000)
177
(6,260)
190
<6,670)
128
(4,540)
95
(3,360)
242
(8,540)
290
(10,300)
512
(18,100)

0.029
(0.064)
0.008
(0.018)
e
0.076
(0,167)
e
e
e
0.009
(0,019)
0.100
(0.221)
0.044
(0,097)

0.026
(0.057)
0.015
(0.033)
0.039
(0.085)
0,076
(0.168)
0.031
(0.069)
0.083
(0.183)
0.024
(0.053)
9
9
0.090
(0.199)
0.046
(0.102)

4.0 (0,06)
3,2 (0.05)
4.6 (0,07)
9.1 (0.14)
6.3 (0,10)
16.3 (0.25)
6.5 (O.!0)
3.6 (0.06)h
22.5 (0.35)
15.5 (0.24)

9.8 (0.15)
                                                                                                          (continued)

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TABLE 6.
Process conditions
No, of
Plant tanks
Decorative chromium plating
Plant Kc»42 1
Plant Lc>43 1
Average
Total tank
surface area, Ampere-
m2 (ft2) hours
22.6 97,000
(240)
2.9 6,500
(30.8)
(continued)
Actual
gas flow
rate,
nr /m 1 n
(ft3/min)
683
(24,100)
70
<2,470)

Mass emission
rate, kg/h fib/h)
Total Cr Crt&
e 0.066
(0.145)
e 0.004
(0.008)

Process Cr*6
rate, mg/A«h
2.0 (0.
1.3 (0.
1.6 (0.

emission

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             TABLE  7.   TANK PARAMETERS AND PROCESS  OPERATING PARAMETERS MONITORED DURING CHROMIUM  PLATING TESTS
ho
C3
Average process parameters won i tored
Tank parameters


Plant
Hard chromium plating
Plant A32
Plant B33
Plant C34
Plant D35
Plant E36
Plant F37
Pi ant G38
Plant H39
Plant I40
Plant J41
Decorative chromium plating
Plant K42
Plant L43

No, of
tank(s)

1
2
4
1
1
1
1
1
2
3

1
1
Total tank
surface area,
«2 (ft2)8

5.8 163)
2.5 (27)
8.4 (90)
5.2 (56)
3.4 (37)
1.8 (20)
1.4 (15)
5.5 (60)
9.0 (99)
6.6 (71)

22.6 (240)
2.9 (3!)
Total tank
capacity ,
9, (gal)b

10,710 (2,830)
4,130 (1,090)
35,000 (9,250)
15,820 (4,180)
9,270 (2,450)
4,810 (1,270)
5,720 (1,510)
7,190 (1,900)
11,210 (2,960)
6.090 (1,610)

61,170 (16,160)
3,060 (1,020)

Current,
amperes

6,220
1,610
2,860
8,390
4,970
2,640
3,480
2,480
1,140
1,150

21,320
2,700

Voltage,
volts

9,0
12.3
7.9
7.4
7.0
4,9
4.9
6,6
7.7
6.1

22.4
5.1
Chromic
acid
concen-
tration.
fl/t
(oz/gal)

254 (34)
208 (28)
250 (33)
156 (21)
250 (33)
210 (28)
210 (28)
210 (28)
225 (30)
173 (23)

300 (40)
241 (32)

Bath
temp.,
•C CF)

52 (125)
62 (145)
54 (130)
52 (125)
54 (130)
56 (133)
55 (131)
60 (140)
59 (138)
49 (120)

54 (130)
48 (119)
           am  = square meters,  ft* - square feet.
             = liters, gal = gallons.

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typical of the sizes of other decorative plating tanks, there  1s
Insufficient evidence to show that emissions are directly proportional to
tank size.  In any case, the uncontrolled emissions have been  normalized
to account for tank size using the ampere-hours term in the emission
factor.  Because the data are limited, a conservative approach was taken
in selecting the emission factor for decorative plating.  Thus, a value of
2 mg/Ah was selected instead of the average value for the two  tests,
      3.1.2.2  Chrora1c Acid Anod1zing Operat1ons•  Uncontrolled emission
data for chromic acid anodizing operations were not obtained through an
EPA source test at an anodizing facility.  Instead, an estimate of the
amount of hexavalent chromium emissions was made by performing a mass
balance on a scrubber used to control emissions from a chromic acid
anodizing operation.  Outlet scrubber water grab samples were  analyzed to
determine the amount of hexavalent chromium in the sample, and a mass
balance was performed on the scrubber to determine the inlet hexavalent
chromium emission rate.  The results of this mass balance indicate that an
uncontrolled of emission factor of 6.0x10*"  kilogram of hexavalent
chromium per hour per square meter of tank surface area (1.2xl(T  pound
per hour per square foot of tank surface area) 1s appropriate to
characterize emissions from chronic acid anodizing.    Alternatively, if
the tank surface area is unknown, uncontrolled emission rates can be used
to approximate the level of uncontrolled chromium emissions.  The results
of the mass balance at the small anodizing operation (tank capacity
-1,900 liters [500 gallons])  and results from a non-EPA emission test at a
large chromic acid anodizing  operation (tank capacity -17,600 liters
[4,600 gallons]) indicate uncontrolled emission rates range from 0.0012 to
0.0028 kg/h (0.0026 to 0.0062 lb/h),  respectively.1"*  At this time,  there
are insufficient data from anodizing  operations to determine conclusively
that one emission factor format  is more appropriate than the other.
3.1.3  Emi ss i on Reduction Techn1ques
      The principal techniques  used to control  emissions of chromic  acid
mist from decorative and hard chromium plating and chromic acid anodizing
operations include add-on control  devices and chemical  fume
suppressants.   The control  devices most frequently used  are mist
eliminators and wet scrubbers that are operated at relatively low pressure
                                    21

-------
drops.  Because of the corrosive properties of chromic acid, control
devices typically are made of polyvinyl chloride (PVC) or fiberglass.
      Chemical fume suppressants are added to decorative chromium plating
and chromic acid anodizing baths to reduce chromic acid mist.  Although
chemical agents alone are effective control techniques, many plants use
them in conjunction with a control device.
      Chevron-blade and mesh-pad mist eliminators are the types of mist
eliminators most frequently used to control chromic acid mist.  The most
important mechanism by which mist eliminators remove chromic acid droplets
from gas streams is the inertia! impaction of droplets onto a stationary
set of blades or a mesh pad.  Mist eliminators typically are operated as
dry units that are periodically washed down with water to clean the
impaction media.
      The wet scrubbers typically used to control emissions of chromic
acid mist from chromium plating and chromic acid anodizing operations are
single and double packed-bed scrubbers.  Other scrubber types used less
frequently include fan-separator packed-bed and centrifugal-flow
scrubbers.  Scrubbers remove chromic acid droplets from the gas stream by
humidifying the gas stream to increase the mass of the droplet particles,
which are then removed by impingement on a packed bed.  Once-through water
or recirculated water typically is used as the scrubbing liquid because
chromic acid is highly soluble in water.
      Chemical fume suppressants are surface-active compounds that are
added directly to chromium plating and chromic acid anodizing baths to
reduce or control misting.   Fume suppressants are classified as temporary
or as permanent.  Temporary fume suppressants are depleted mainly by the
decomposition of the fume suppressant and dragout of the plating solution,
and permanent fume suppressant are depleted mainly  by dragout of the
plating solution.  Fume suppressants,  which are manufactured in liquid,
powder, or tablet form, include wetting agents that reduce misting by
lowering the surface tension of the plating or anodizing bath,  foam
blankets that entrap chromic acid mist at the surface of the plating
solution,  or combinations of both a wetting agent and foam blanket.
                                    22

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      The performance capabilities of the control devices used  to control
chromic acid mist are presented in Table 8,  Thi air pollution  control
devices tested include four mist eliminators, three packed-bed  scrubbers,
and one packed-bed scrubber in conjunction with a mist eliminator used to
control emissions from hard chromium plating operations.  In addition, one
emission test was conducted at a decorative chromium plating facility to
determine the performance of chemical fume suppressants in controlling
chromic add mist.
      The average hexavalent chromium removal efficiency of mist
eliminators was 98 percent for mist eliminators with double sets of
blades, 90 percent for mist eliminators with single sets of blades, and
98 percent for mesh pad units.  The average hexavalant chromium removal
efficiency of scrubbers was 98 percent.  The hexavalant chromium removal
efficiency of the scrubber 1n conjunction with the mist eliminator was
95 percent.
      For decorative chromium plating operations, the performance
efficiency of both chemical fume suppressants tested (a foam blanket and a
combination of a foam blanket and wetting agent) was greater than
99 percent.  This performance efficiency is achievable as long  as vendor
recommendations on the makeup and use of the fume suppressants  are
followed rigorously.
3.1.4  Nationwide Emission Estimates
      Table 9 presents the estimated number of operations and the
nationwide annual emission rate for each type of operation.   The
assumptions regarding the existing control  levels for each type operation
were derived from data obtained during the  development of the NESHAP for
chromium electroplating operations.  The nationwide emission rate for hard
chromium electroplating operations was based on the assumption that
30 percent of operations are uncontrolled,  30 percent of operations are
controlled by mist eliminators with single  sets of  blades (90 percent
efficient), and 40 percent are controlled by single packed-bed scrubbers
(97 percent efficient).   The nationwide emission rate for decorative
chromium electroplating operations was based on the assumption that
15 percent of operations are uncontrolled,  80 percent are controlled by
chemical fume suppressants (97 percent efficient),  and  5  percent are
                                    23

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                                               TABLE  8.    PERFORMANCE  LEVELS  OF  INDIVIDUAL  CONTROL  DEVICES
            Plant  Plant
            code   name
                             Description of control device
                                                                                                Mo. of
                                                                                                runs
                                                                                                Concen-
                                                                                             tration, ii
Mass enisslon
  rate,  fcg/h
                                                                                   averaged   Inlet     Outlet    Inlet
                                                                                                                          Outlet
Efficiency,
 percent*
                                                                                                                                                               Process
                                                                                                                                                   __
                                                                                                                                                   Inlet
                                                                                                                                                            Outlet
ro
            HARD CHROMIUM MATING

            Chevron-blade raist eliminators
A
8
0
Single set of overlapping-type blades
Single set of overlapptng-type blades
Double set of overlapping -type b'ades
4
3
3
2.030
1.760
7.690
0.306
0.149
0,1 Z4
0.0260
0.0151
0.0763
0,0033
0,0013
0.0012
87.9
91.3
9B.4
3.96
3.16
9.06
0. §5
0.2?
0,15
Mesh-pad nisi »li«1nators
F
S,
tf
Ec
Packed-bed
1
J
C

DECORATIVE:
Two oesh pads in series
Two aesh pads in series
One aesh pad
Two seti of chevron-blade* followed by two mesh pads
scrubbers
Single packed-bed scrubber
Double packed-bed scrubber
Double packed-bed scrubber fol lowed by chevron-blade «ist
elininJtor *ith 3 double set of wave-type blades
CHROMIUM PLATING
S
3
3
3

11
3
6


11.400
4,410
0.609
3.070

5.510
1,670
2.040


0,0326
0,0435
0.025?
0.040

0.0302
0.0523
0.081


0.0829
0.0241
0.008?
B.0313

0,0900
0,0464
0.0388


0,0002
0.0003
0,0005
0,0004

0,0005
0.0015
0.001S


99.7
98.9
94. S
98. J

99.4
96,2.
95. 4d


16,3
6.52
3.60
6,33

22.5
15,5
4.5?


0,04
0.0?
0.18
0,08

0,14
0.56
0.14


Fuse suppressants
i

1, Foan blanket
2. Foaa blanket in combination with wetting agent
3
3
0,916
0.916
0.0041
0.0021
0.0036
0,0036
0.00002
0,00001
.99.5
*39,6
1.34
1,34
0.006
0,003
                                                                              Therefore, they may not agree with iNe values obtained by calculating the efficiency frcn the  average
Efficiencies are based on the average of efficiencies froa eich  run,
.Inlet and outlet rate.
Ttesulti are for total chroniun,   He»avalent chroaiuo analyses  were not performed.
CA moisture extractor preceded the cmt el initiator unit.  However, the eoission  data for the combined control  techniques were attributed  to the nist el mind tor unit  only.
 Any  droplets, caught by the moisture extractor would have been  collected by the  list eliminator unit, if  the nolsture extractor was eiiainated froo the systea,
"The  efficiency presented ii the  contained efficiency of bath units.

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          TABLE 9.   NATIONWIDE NUMBER OF OPERATIONS AND ESTIMATED
        HEXAVALENT CHROMIUM EMISSIONS FROM CHROMIUM ELECTROPLATING
                  AND CHROMIC ACID ANODIZING OPERATIONS
Operatfon
No. of plants
  nationwide
   Nationwide
Cr+  emissions,
Mg/yr (tons/yr)
Hard chromium plating

Decorative chromium plating
                      2
Chromic acid anodizing
    1,540

    2,800

     680
   145  (160)

     10 (11)

   3.6  (3.9)
                                    25

-------
controlled by single packed-bed scrubbers  (95 percent efficient).  The
nationwide annual emission rate for chromic add anodizing operations was
based on the assumption that 40 percent of operations are uncontrolled,
10 percent are controlled by mist eliminators with single sets of blades
(90 percent efficient), 30 percent are controlled by chemical fume
suppressants (97 percent efficient), and 20 percent are controlled by
single packed-bed scrubbers (95 percent efficient).
3,2  COOLING TOWERS
3.2.1  Background Information
      Cooling towers are devices that cool warm water by contacting it
with ambient air that is drawn or forced through the tower.  This cool
water is used to remove heat from a process or an HVAC chiller and is then
recirculated to the cooling tower.  Chemicals are added to this
recirculating water to inhibit heat exchanger corrosion.  One of the many
classes of corrosion inhibitors used is chromium based.  Air emissions of
chromium occur when water droplets (and the chemicals they contain)
entrained in the air stream that 1s drawn through the tower are emitted to
the atmosphere.  These droplet emissions are referred to as "drift."  All
cooling towers that are used to remove heat from an Industrial process or
chemical reaction are referred to as industrial  process cooling towers
(IPCT's).  Towers that are used to cool heating, ventilation, and air
conditioning (HVAC)  and refrigeration systems are referred to as comfort
cooling towers (CCT's).
      3.2.1.1  Industrial  Process Cooling Towers.  Major users of IPCT's
that also use chromium-based water treatment chemicals are chemical
manufacturing plants, petroleum refineries, and  primary metals
facilities.   Several  miscellaneous manufacturing industries (textiles,
tobacco products, tire and rubber products, and  glass products)  and
utilities use chromium-based water treatment chemicals to a lesser
degree.  It  is estimated that IPCT's are used at approximately 190 petro-
leum refineries,  1,800 chemical manufacturing plants,  240 primary metals
plants, and  730 plants In  the miscellaneous industries/   In addition,
the percentage of cooling  towers using chromium-based  water treatment
chemicals in each industry Is estimated as  70 percent  at petroleum
refineries,  40 percent at  chemical  manufacturing plants, 20 percent  at
                                    26

-------
primary metals facilities, 15 percent at plants 1n the tire and rubber
                                                                        i» S
industry, and 5 percent at plants in the other miscellaneous industries.
In the utilities Industry, 1t was reported that chromium-based water
                                                          |, g
treatment chemicals are used at two electric power plants.    When
combined with data from plant responses to EPA information requests in
each of these Industries, these estimates result 1n a total of about
2,855 IPCT's using chromium-based water treatment chemicals:  476 at
petroleum refineries, 2,039 at chemical plants, 224 at primary metals
plants, 110 at miscellaneous plants, and 6 at utilities.  The nationwide
baseline Cr+6 emissions from these towers are estimated to be 85 megagrams
per year (Mg/yr) (94 tons per year [tons/yr])."5
      3,2.1.2  Comfort Cooling Towers.  Comfort cooling towers are used 1n
all States in the U.S., primarily in urban areas.  Major users of CCT's
with HVAC systems include hospitals, hotels, educational facilities,
office buildings, and shopping malls.  Refrigeration systems that may
operate with CCT's Include ice skating rinks, cold storage (food) ware-
houses, and other commercial operations.  The EPA estimates that the
nationwide population of CCT's is 250,000 units and that 15 percent of
CCT's (about 37,500) use chromium-based water treatment chemicals.  These
CCT's are estimated to emit between 7.2 and 206 Mg/yr (8 to 227 tons/yr)
of chromium."*   Chromium use in CCT's appears to be distributed randomly
across the country.
      In the preparation of the proposed rule for CCT's under the Toxic
Substances Control  Act (TSCA) (see 52 FR 10206), EPA developed model tower
parameters and estimates of chromium emissions per model tower to
represent the population of CCT's 1n the U.S.  Table 10 presents the model
parameters and baseline (i.e., low efficiency drift eliminator [LEDE])
emission estimates.
      The emission estimates in Table 10 are based on an emission factor
developed from EPA- and industry-sponsored cooling tower emission tests.
Because the emission factors developed to estimate Cr+6 emissions from
cooling towers are independent of tower operating parameters (redrculatlon
rate, chromate concentration, cooling range), the factors are applicable
to both CCT's and IPCT's.  Section 3.2.3.1 of this document discusses
specific emission factors to use for estimating Cr+  emissions from
cooling towers on a case-by-case basis.   [Note:  The proposed TSCA rule

                                    27

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                       TABLE 10.  MODEL COMFORT COOLING TOWERS AND HOURLY BASELINE Cr*6 EMISSIONS
ho
Co
Model
tower
1
2
3
4
5
6
Model
building
^ize»2
mr (ft2)
673
(7,240)
1,460
(15,720)
3,405
(36,650)
6,224
(66,990)
12,338
(132,800)
37,626
(405,000)
Model tower
cooling requirements
W (Btu/h)
95,400
(325,800)
207,100
(707,400)
482,900
(1,649,000)
882,900
(3,015,000)
1,750,000
(5,976,000)
5,338,000
(18,230,000)
Tons
27
59
137
251
498
1,520
Flow
Recircu-
lation
rate
246
(65)
534
(141)
1,250
(330)
2,280
(602)
4,520
(1,194)
13,800
(3,642)
rates, a/m1n
(gal/min)
Evapora- Slowdown
tion rate rate
2.08
(0.55)
4.54
(1.20)
10.6
(2.80)
19.4
(5.12)
38.4
(10.15)
117,0
(30.96)
0.53
(0.14)
1.14
(0.30)
2.65
(0.70)
4.85
(1.28)
9.61
(2.54)
29.3
(7.74)
Chromium
emissions
per tower,
mg/h (lb/1,000 h)
19.9
(0.044)
43.2
(0.095)
101
(0.222)
184
(0.406)
365
(0.804)
1,110
(2.45)
        Assumptions:
        Wet bulb temperature = 23.9°C (75°F)
        Hot water temperature « 29.4°C (85°F)
        Cooling range = 5.6DC (10°F)  z                      2
        Cooling requirements = 142 W/m  floorspace (45 Btu/ft /h)
        Cycles of concentration = 5
        Latent heat/total heat =0.8
        Chromate concentration = 10 ppm
        Chromium emission factor = 0.0003 mg Cr"*" /(ppm Cr* )(liter H20)
                                               (2.504x10   Ib Cr* /ppm Cr* /gal H20)

-------
would prohibit the use of chromium-based chemicals in CCT's.   If
promulgated, this rule would hive the effect of reducing Cr*   emissions
from CCT's to zero.]
      3.2.1.3  Cooling Tower Fundamentals.  Schematics of typical cooling
                                    j. a
tower designs are shown in Figure 2.    The major cooling tower components
include the fan(s), fill material, water distribution deck or  header,
drift eliminator, structural frame, and cold water basin.  Other
components that affect tower operation include the pumps and pipes
necessary to circulate the cooling water through the cooling tower and
heat exchanger loops.
      Most IPCT's are designed with induced-draft airflow, but many have
forced-draft airflow, and some (especially in the utilities industry) have
natural-draft airflow.  Induced draft is provided by a propeller-type
axial fan located in the stack at the top of the tower.  Forced-draft
towers are usually smaller than induced-draft towers and have either
centrifugal fans located at the base of the tower, which is constructed as
a plenum to provide positive-pressure airflow through the fill material,
or axial fans located on the side of the tower.  Natural-draft airflow
relies on air currents created by temperature differences between the air
in the tower and the atmosphere.  When the cooling demands are minimal and
the air temperature is low enough, water can be circulated through the
tower and cooled sufficiently without using the fans.  In these instances,
a natural draft is created in the cooling tower.
      The direction of the airflow through a mechanical draft tower is
either crossflow or counterflow.   Crossflo/ refers to horizontal airflow
through the fill,  and counterflow refers to upward vertical  airflow.   Fill
material is used to maintain an even distribution of water across the
horizontal plane of the tower and to create as much water surface as
practical to enhance evaporation and sensible heat transfer.
3.2.2  Potential  Emission Reduction Techniques
      Techniques to control  chromium emissions from cooling  towers Involve
two different strategies:   modification of chromium addition  to the
recirculating water,  and improved reduction of drift.  The first technique
involves reducing  the concentration of  chromium in the  water  treatment
program, thereby reducing  the concentration of chromium in the drift
                                    29

-------
                              ilR
                            OUTLE"
                            A    A
               WATER
               INLET
              WATER  OUTLET
                              FAN

                                WATER
                                NLET
                             DRIFT
                        "ELIMINATORS
                    MECHANICAL   DRAFT
                    CROSS-FLOW  TOWER
                           AIR
                          OUTLET
                        A
                     f
               «««««««]—	DRIFT

                             ELIMINATORS
        AjR
        INLET
                                        FAN
                                  FILL
               s
               0
                                             INLET
Figure 2.
WATER  OUTLET

       MECHANICAL  DRAFT
       COUNTER-FLOW  TOWER
Internals of crossflow and counterflow cooling towers
    (reprinted from Reference No.  48).
                              30

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 emitted.  The second technique involves retrofitting  towers  that normally
 have LEDE's with high-efficiency drift eliminators  (HEDE's)  to reduce
 drift emissions to the lowest possible rate.
      3.2.2.1  Alternative Hater Treatment Programs.   Responses to 28 EPA
 information requests and a survey of the Chemical Manufacturers Associa-
 tion indicate that the average chromate concentration for  those IPCT's
                                                    ** 5  ** 9
 using chromium-based corrosion inhibitors 1s  13 ppm.   »    One potential
 chromium emission reduction technique involves alternative water treatment
 programs such as programs with lower chromate levels  or nonchromate
 treatments.
      A low-chromate treatment program would reduce Cr+s emissions from
 IPCT's by limiting the chromate concentration in cooling water.  Water
 treatment programs are available that maintain average chromate concentra-
 tions of 0.5 to 4 ppm 1n the recirculating water, but these  programs have
 not always been successful in Industrial applications.  Low-chroitte
 programs that have provided acceptable results 1n a number of cases
 maintain chromate concentrations in the range of 4 to 6 ppm,
      Because of National Pollution Discharge Elimination  System (NPDES)
 chromium restrictions and other regulations, nonchromium treatments are
 now more widely used than chromium treatments.  The most common
 nonchromium treatment program is phosphate based, but others include
 molybdates, zinc, and ill-organic treatments (primarily organo-phosphorus
 compounds).  However, these alternative programs may  not perform corrosion
 inhibition functions as well  or as cheaply as chromates depending on the
 individual cooling tower system.   The performance of  any treatment program
 is dependent on water quality parameters (pH, alkalinity,  hardness, and
 conductivity) and operating conditions (water temperature, flow velocity,
 inhibitor concentration,  and  the presence of contaminants  such as H2S,
 S02i NH3t and N02)  that are specific to each cooling  system.
      3.2.2.2  Low- and High-Efficiency Drift Eliminators.  Water droplets
 entrained in the air and  the  dissolved and suspended  solids contained 1n
 the droplets that are emitted from cooling towers are referred to as
drift.   Drift eliminators can be  installed at the exit of the fill
 sections to reduce  the amount of  drift 1n the exiting airflow.
Historically, the purpose of  drift reduction has been to alleviate  the
                                    31

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nuisance deposition of water drift and its dissolved solids on nearby
buildings or on personal property such as automobiles.  More recently, the
concern has focused on the environmental Impact caused by the compounds
contained 1n the drift and, thus, on the deposition of these compounds.
Drift eliminators are designed with pressure drops lower than those of
other air pollution control equipment and rely primarily upon the
impaction of water droplets on drift eliminator surfaces to reduce the
concentration of drift from the exit air of cooling towers.  The drift
eliminator blades are configured to force directional changes in the
airflow such that the momentum of the water droplets causes them to
Impinge onto the blade surfaces.  The number of directional airflow
changes, the spacing between the blade surfaces, the angle of directional
change, and the capability to return the collected water to a quiescent
area of the plenum are the major design features (parameters) in drift
eliminators that affect efficiency.  Drift eliminators are constructed of
wood, PVC, metal, asbestos-cement, polystyrene, or cellulose.  The
material most often specified is PVC.
      Figure 3 presents schematics of the three major drift eliminator
designs:  herringbone (blade-type), waveform, and cellular (or honey-
comb).  Low-efficiency drift eliminators Include herringbone, some
waveform (sinusoidal), and some cellular designs.  Herringbone designs are
constructed to create two or three major directional  changes in the
airflow.  The blades are sloped 1n opposing directions in a manner that
provides drainage of the accumulated drift into the fill area.  The blades
typically are constructed of wood, but other materials (e.g., metal and
asbestos cement board) also are used.  Waveform drift eliminators are
configured in a sinusoidal wave pattern such that two major directional
changes in the airflow are created.  The sinusoidal blades are constructed
of asbestos cement board or PVC material.  Cellular drift eliminators are
configured with thinner blades in a honeycomb pattern.  The airflow
passages in the cellular drift eliminators, which are narrower than
passages in other designs, reduce the distance a droplet must travel
across the stream to Impact on the surface.  Drainage of the collected
water to prevent reentrainment is not a design criteria of LEDE's.
                                    32

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                                             Lacit
                           HERRINGBONE
                          (BLADE-TYPE)
                          ELIMINATOR
                          WAVEFORM
                          ELIMINATOR
                                               Pfcmrte
                           CELLULAR
                           ELIMINATOR
Figure 3.   Designs of various drift  eliminators  (reprinted
                  from Reference  No.  50),
                             33

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      High-efficiency drift eliminators include a few of both cellular and
sinusoidal designs.  The cellular HEDE's that achieve the higher
efficiencies are designed with complex configurations that contain
numerous, closely constructed airflow passages.  Thin materials of
construction are used to reduce the area of blockage to the airflow and
minimize the pressure drop that is created by the eliminator.  For
sinusoidal drift eliminators, the blades are placed closer together in
high-efficiency designs than in low-efficiency designs, and the exit is
configured with a tip for draining captured water that would otherwise be
partially reentrained in the airflow.  Typically, drainage of water into a
quiescent area of the tower is a major design consideration of HEDE's.  A
few drift eliminators installed in towers built in recent years are more
likely to be higher efficiency waveform or cellular units, but the vast
majority of older tov/ers still have lower efficiency herringbone and
waveform eliminators.
      The performance of a drift eliminator is affected primarily by the
droplet or particle size and the airflow velocities through the drift
eliminator.  Small  droplets are created both from evaporation of larger
droplets and the physical  breakage of larger droplets into small
droplets.  Parameters that affect the rate of evaporation and the size of
droplets created include the water distribution system, the type of fill,
the type of tower,  the meteorological conditions,  and the temperature of
the recirculating water.
      A drift eliminator manufacturer indicates that HEDE's can remove
80 to 90 percent or more of the drift discharged from low-efficiency
herringbone drift eliminators.   *     These drift eliminator efficiencies,
however, are based  on data collected with  a test method that has not been
submitted to EPA for approval.
3.2.3  Cooling Tower Emissions
      Three series  of emission  tests were  conducted  by EPA on IPCT's
equipped with low-  and high-efficiency drift eliminators.   The  results  of
these tests are presented  in the  next section.
                                    34

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      3.2.3.1  Drift and Chromium Emissions.  The drift rate (rate of
water lost by entrainment in the cooling air drawn through the tower) is
often expressed as the percentage of the recirculating water flow rate
that is emitted.  Likewise, the chromium emission rate can be expressed as
a percentage of the recirculating chromium rate.  However, the chromium
emission rate from towers should not be confused with the drift rate.
Based on test results, a drift eliminator manufacturer claims that the
achievable drift rates range from 0.001 to 0.06 percent of the
recirculating water.  The approximate dividing line between drift rates
for higher and lower efficiency drift eliminators is 0.008 percent.  Those
achieving a lower percentage are "higher efficiency," and those that
cannot achieve 0.008 percent are "lower efficiency."50"5
      Drift can be estimated by measuring the emission rate of an element
(such as sodium, calcium, manganese, chromium, lithium or bromine) and
assuming that the percentage of water emitted as drift is the same as the
percentage of the recirculating element emitted.  However, a claimed drift
rate may or may not be equivalent to the element's emission rate depending
on the way the drift rate was measured.  Also, drift rate measurement
results are highly dependent on the measurement method; therefore,
achievable drift rate claims may not be comparable if they are based on
different measurement methods.
      The EPA-sponsored emission tests of IPCT's at three facilities used
an isokinetic test method for chromium which is still under development.
Emission factors relating the chromium emission rate to the chromium
recirculation rate were developed from each of these emission tests.  The
average baseline (LEDE) and controlled (HEDE) emission factors for each
test site are presented in Table 11.  In addition, five industry-sponsored
drift performance tests conducted by Midwest Research Institute and two
chromium emission tests conducted by Mobil are included.  The emission
factors express the emission rate as a percentage of the recirculating
rate (milligrams of chromium emitted per milligram of chromium
recirculating in the tower multipled by 100).  The most comprehensive
emission tests were conducted at Plant B.  At this plant, two towers of
similar design located side-by-side were tested simultaneously under the
same meteorological conditions.  One tower was equipped with an LEDE and
the other was equipped with an HEDE.

                                    35

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         TABLE 11.  EMISSION FACTORS FOR HEXAVALENT CHROMIUM FROM
                           COOLING TOWERS*3-
Test site
Chromium emission
factor, percent*
Standard deviation
(percent relative
standard deviation,
percent)
EPA-sponsored tests
A (HEDE)
C (HEDE)
B (HEDE)
B (LEDE)
A (LEDE)
Industry-sponsored tests
MRI No. 3 (HEDE)
MR I No. 4 (HEDE)
Mobil -PTR Tower No. 5
(LEDE)
Mobil -North Tower No. 6
(LEDE)
MRI No. 1 (LEDE)
MRI No. 2 (LEDE)
MRI No. 5/6 minerals
test (LEDE)
0.0037
0.028 w/outliers
0.0038
0.0087
0.0267
0.0318
0.141 w/outl1ers
0.01
0.007
0.0334
0.0321
0.0305
0.034
0.018
0.021 w/outliers
0.0020 (54)
0.035 w/outl1ers
0.0044 (116)
0.0037 (43)
0.0168 (63)
0.0292 (92)
0.192 w/outHers
NA (--)
NA (-)
0.0306 (92)
0.0156 (49)
NA (-)
NA (-)
0.0045 (25)
0.0094 w/outliers
(126)



(136)






(45)
^Percentage  of  recirculatlng  chromium  that  is  emitted.
                                    36

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      Since the completion of the emission tests at Plant  Bf  additional
methods development Investigations have been conducted.  These
Investigations have revealed that the chromium sampling method  1s  subject
to substantial error due to potentially severe problems associated with
chromium recovery and cross-over contamination from sample run  to  sample
run.  The extent to which these problems appear in the test results
obtained at Plants A, C, and Mobil is uncertain.  As a result,  the data
presented in Table 11 should be used with caution.
      The EPA believes that the tests at Plant B provide the  best
available data on the relative performance of HEOE's.  The EPA  Method  13-
type testing at Plant B Indicated a Cr"1"6 emission factor of 0.03 percent
of the recirculatlng Or"1"6 for LEDE's and 0.0087 percent for HEDE's.  As
discussed in Section 3.2.1.2, these factors can be used for both IPCT's
and CCT's,
      The current factors are based on the assumption that the  ratio of
hexavalent to total chromium in the emissions is the same  as  that  in the
cooling water.  The test program conducted by the Agency has  not
conclusively identified the speciation of emissions (i.e., Cr"1"  versus
Cr*3),  For purposes of estimating Cr"1"5 emissions, the conservative
assumption is that all of the chromium is Cr+ .
      3.2.3.2  Samp1e Calcu1at1on of Chrornlurn Emissions.   The chromium
emission rate for any tower can be estimated by multiplying the emission
factor by the recirculatlng rate of water and the chromium concentration
in the recirculating water as shown in Equation (1).
                              ECr = K-R.CCr                            (1)
where:
      E^r = chromium emission rate,  mg Cr/tnin
        K = chromium emission factor,  percent of recirculating chromium
            that is emitted
        R = recirculating r§:e of cooling water, liters/min
      C£P = concentration of chromium in the recirculating water, mg
            Cr/liter = ppin (multiply CrQi» concentration by 0.448 to obtain
            Cr concentration)
For example,  the following calculation estimates the emissions from a
10,000-gallon-per-minute (gal/min)  IPCT with a recirculatlng chromate
                                    37

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concentration of 10 parts per mill ton (ppm), equipped with a low-
efficiency drift eliminator.
        R - (10,000 gal/min)(3.785 liters/gallon) - 37,850 liters/minute
      C£r = 10 ppm as CrO^ =4,48 ppm Cr
        K = the emission factor for towers with low-efficiency drift
            eliminators; use K = 0,03 percent.
      ECr - K-R-CCr = (O.Q3X)(37,850)(4.48) = (0.0003)(37,850)(4.48) =
            50,9 mg Cr emitted/mln
To estimate the emissions from the same IPCT equipped with a high-
efficiency drift eliminator, use K = 0.0087.
Therefore:

ECr = K«R'CCf = (0.0087%)(37,850)(4.48) = (0.000087)(37,850)(4.48) =
                          14.8 rag Cr emitted/min
Thus, the emission reduction achieved by a HEDE compared to a LEOE 1s:
                       50.9-14.8.,, nn   71 na~-an*.
                       	cn-q—xlOO = 71 percent.
                           50.9

      The following example calculation estimates the emissions from a
500-gal/min CCT with a reeirculatinf chromate concentration of 10 ppm,
equipped with a low-efficiency drift eliminator.
        R = (500 gal/min)(3.785 liters/gal) = 1,892.5 liters/min
      CCr = 10 ppm as CrO,, = 4.48 ppm Cr
        K » 0.03 percent
      ECf • K-R-CCr = (0.03*)(1,892.5)(4.48) =
            (0.0003)(1,892.5)(4.48) - 2.5 mg Cr emitted/min

3.2,4  Nationwide EmissionsDistribution by Industry
      In developing the NESHAP for chromium emissions from IPCT's, EPA has
generated industry-by-industry estimates of the total number of cooling
towers, the number of towers using chromate treatments, and chromium
emissions.  Table 12 presents these estimates as currently known.   The
data show that the industries of greatest concern are chemical manufac-
turing (43 Mg/yr [47.5 tons/yr]),  petroleum refining (31.8 Mg/yr
[35.1 tons/yrj), and primary metals production (8.4 Mg/yr [9.3 tons/yr]).
                                    38

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Together, these Industries represent 98.2 percent of nationwide chromium
emissions from IPCT's.1**  Tab1<
chromium emissions from CCT's.
emissions from IPCT's.    Table 12 also presents nationwide estimates of
                                    39

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   TABLE 12.  NATIONWIDE COOLING TOWER CHROMIUM EMISSIONS SUMMARY
                                                                    «*7
Industry
Chemical manufacturing
Petroleum refining
Primary metals
Tobacco products
Tire and rubber
Textile finishing
Glass manufacturing
Utilities
Subtotal (IPCT only)
Comfort cooling towers
TOTAL
Total No.
of cooling
towers
5,096
680
1,118
336
267
, 1,018
58
775
9,348
250,000
259,350
No. of
cooling towers
using chromate
2,039
476
224
16
40
51
3
6
2,855
37,500
40,360
Cr+6
Mg/yr
43.13
31.82
8.39
0.23
0.18
0.08
0.01
0.95
84,8
33
118
emissions4
Tons/yr
47.54
35.08
9.25
0.26
0.20
0.09
0.01
1.05
93.5
34
128
aBased on use of low-efficiency drift eliminators.
                                    40

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                        4.0  SOURCE TEST PROCEDURES

 4.1   CHROMIUM ELECTROPLATING
       During the standards support study for hexavalent chromium  emissions
 from  hard  and decorative chromium electroplating facilities,  samples  to  be
 analyzed for hexavalent and total chromium were obtained  in accordance
 with  EPA Method 5  (40 CFR Part 60-Appendix A), also referred  to as
 Modified Method 13-B in test reports.  The only modification  to the sample
 collection method was the elimination of the filter and the replacement  of
 H20 in the impingers with 0.1 Normal sodium hydroxide.  Method 5  provides
 detailed procedures and equipment criteria and other considerations
 necessary  to obtain accurate and representative emission  samples.  In
 order  to sample for chromium emissions, Methods 1 through 4 must  also be
 used.
       After collection, the samples were analyzed for hexavalent  and  total
 chromium (total chromium is the sum of hexavalent chromium plus other
 chromium).  Concentrations of hexavalent chromium were determined using
 spectrophotometric analysis while total chromium was determined using
 inductively coupled argon plasmography (ICAP).  At the present time,
 sample analysis has been performed in accordance with the tentative method
 "Detection of Hexavalent Chromium from Stationary Sources (December 13,
 1984)," and a draft method:  "E.P.A.  Protocol for Emission Sampling for
 Both Hexavalent and Total  Chromium (February 22, 1985),"
 4.2  COOLING TOWERS
       During the standards support study for chromium emissions from
 cooling towers, testing was conducted according to two draft test methods
 developed from previously  conducted methods development testing:
 "Method 	—Determination of Chromium Emissions from Cooling Towers"  and
 "Method 	—Direct Measurement of Gas Velocity and Volumetric Flowrate
 Under  Cyclonic Flow Conditions (Propeller Anemometer),11  The cooling  tower
method  is similar to EPA Method  13 (40 CFR Part 60-Appendix A) with the
 following exceptions:   (1)  a Teflon™  filter is used in place of a paper
filter, (2) a propeller anemometer is used in place of the pitot tube  for
gas velocity and flowrate  measurements,  (3)  the determination of the
measurement site does  not  follow EPA  Method  1,  and  (4)  the chemical
                                    41

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 analysis for total chromium In the emission samples is performed using
 Neutron Activation Analysis (NAA), Graphite Furnace Atomic Absorption
 (GFAA), or ICAP.  In conjunction with the emissions testing, repre-
 sentative cooling tower water samples were collected to determine the
 ratio of hexavalent to total chromium in the cooling water; these samples
 were analyzed for total chromium by NAA, GFAA, or ICAP and for hexavalent
 chromium by the dlphenylcarbazide colorimetric method (in "EPA Draft
 Method-Determination of Hexavalent Chromium Emissions from Stationary
 Sources," December 13, 1984).  The ratio was used to calculate the amount
 of hexavalent chromium in the cooling tower emissions.
      Preliminary material balance calculations were performed on the
 cooling water at several towers to compare the apparent chromium loss In
 the drift emissions with the emission measurements obtained during the
 standards support study.  Variables used in these calculations included!
 cooling water flow rates to the towers, riser cells, and/or fan cells;
 blowdown rates; makeup water flow rates; addition(s) of chemicals to the
 cooling water; and chemical analysis of the cooling water samples taken
 during testing.
      Two major modifications were made to the draft test method for
 cooling towers based on problems encountered and knowledge gained during
 the testing program.  Initially, the draft method specified the use of NAA
 to determine the total chromium content of the Impinger train samples and
 the cooling water samples.  Because of the length of time required for
 sample analysis and the limited availability of commercial NAA services,
 two additional analytical  techniques, GFAA and ICAP, were utilized and
were added as options to the draft test method.  Unlike NAA,  both of these
 techniques require acid solubllization of the chromium in the sample prior
to analysis.   In assessing the chromium recovery efficiency for the
concentrated implnger samples  from the first test, it was discovered that
a significant residue remained in the beakers used to concentrate the
samples.   The concentration procedure was modified to require an add
rinse of  the beakers used  for  sample concentration with the rinse being
added to  the concentrated  sample.
                                    42

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                             5.0  REFERENCES
 1.  Nemo from Hester, C., MRI, to Smith, A., EPA/ISB.  Bases for Risk
     Assessment Inputs for Chromium Electroplating Operations.  June
     1988.  pp. 6-7, 10.
 2.  Memo from Hester, C., MRI, to Smith, A., EPA/ISB.  Bases for Risk
     Assessment Inputs for Chromic Acid Anodizing Operations.  June
     1988.  pp. 8-9.
 3.  Logozzo, A., and Schuwartz, M.  Hard Chromium Plating.  American
     Electroplaters Society, Inc.  p. 9.
 4.  Vervaert, A.  Preliminary Assessment of Chromium from Chromium
     Electroplating Facilities.  Research Triangle Park, North Carolina.
     U. S. Environmental Protection Agency,  p. 3.
 5.  Decorative Chromium Electroplating.  American Electroplaters
     Society.  1980.  p. 2.
 6.  Dennis, J., and Such, T.  Nickel and Chromium Plating, Butterworth
     and Company.  University Press.  Cambridge, England, Second
     Edition.  1986.  p. 179.
 7.  Reference 4, p. 2.
 8.  Reference 6, p. 287.
 9.  Reference 6, p. 289.
10.  Reference 6, p. 290.
11.  Reference 6, pp. 272, 294-295.
12.  Locating and Estimating Air Emissions From Sources of Chromium.
     U. S. Environmental Protection Agency, Research Triangle Park, North
     Carolina.  EPA Publication No.  450/4-84-007g.  July 1984.  p.  83.
13.  Graham, K.  Electroplating Engineering Handbook.  Reinhold Book
     Corp.,  New York.  1962.  p. 427.
14.  Reference 13, p. 432.
15.  Reference 13, p. 432.
16.  Reference 13, pp.  162, 427.
17.  Brace,  A.  The Technology of Anodizing Aluminum.  Robert Draper,
     Ltd.   Teddington,  1968.  p. 54.
18.  Darrin, M.,  and Tubbs, I.   "Dyeing Chromic Acid Anodized Aluminum."
     Metal Finishing.  September 1984.   p. 550.
                                    43

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19.  Schwartz, M.  Anodized Aluminum and Its Alloys.  American
     Electroplaters Society.  1985.  p. 15.

20.  Wernick, S., and Pinner, R.  "Surface Treatment and Finishing of
     Light Metals."  Metal Finishing.  June 1955.  p. 92.

21.  Reference 13, p. 429.

22.  Reference 13, p. 429.

23.  Brimi, M., and Luck, J.  Electrofinishing.  American Elsevier
     Publishing Company.  New York.  1981.  p. 77.

24.  Reference 13, p. 430.

25.  Snyder, D.  "Trivalent Chromium Plating:  The Second Decade."
     Product Finishing.  March 1988.  p. 57.

26.  Reference 25, pp. 59-60.

27.  Reference 25, p. 63.

28.  Reference 25.  p. 65.

29.  Trivalent Chromium Cost Enclosure:  Harshaw/Filtrol Partnership.
     Prepared for U. S. Environmental Protection Agency, Research Triangle
     Park, North Carolina, by Dennis Maserik, Manager of Technical
     Services.  June 22, 1987.  p. 3.

30.  Tomaszewskl, T., and Fischer, R.  "Trivalent Chromium:  A
     Commercially Viable Alternative."  Occidental Chemical Crop.  p. 5.

31.  Reference 30, p. 5-6.

32.  Chromium Electroplaters Test Report:   Greensboro Industrial  Platers,
     Greensboro, North Carolina.  Entropy Environmentalists, Inc.,
     Research Triangle Park, North Carolina.  Prepared for U. S.
     Environmental Protection Agency, Research Triangle Park, North
     Carolina.  EMB Report 86-CEP-l.  March 1986.

33.  Chromium Electroplaters Test Report:   Consolidated Engravers
     Corporation, Charlotte, North Carolina.  Peer Consultants, Inc.,
     Rockville, Maryland.  Prepared for U.  S. Environmental Protection
     Agency, Research Triangle Park, North Carolina.  EMB
     Report 87-CEP-9.  May 1987.

34.  Chromium Electroplaters Test Report:   Roll Technology, Greenville,
     South Carolina.  Peer Consultants,  Inc., Dayton, Ohio.  Prepared for
     U.  S. Environmental Protection Agency, Research Triangle Park, North
     Carolina.  EMB Report 87-CEP-6.  September 1987.
                                    44

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35.  Chromium Electroplaters Test Report:  Able Machine Company, Taylors,
     South Carolina.  PEI Associates, Inc., Cincinnati, Ohio.  Prepared
     for U. S. Environmental Protection Agency, Research Triangle Park,
     North Carolina.  EMB Report 86-CEP-3.  June 1986.

36.  Chromium Electroplaters Test Report:  Roll Technology Corporation,
     Greenville, South Carolina.  Peer Consultants, Dayton, Ohio.
     Prepared for U. S. Environmental Protection Agency, Research Triangle
     Park, North Carolina.  EMB Report 88-CEP-13.  August 1988.

37.  Chromium Electroplaters Test Report:  Precision Machine and
     Hydraulic, Inc., Worthington, West Virginia.  Peer Consultants,
     Dayton, Ohio.  Prepared for U. S. Environmental Protection Agency,
     Research Triangle Park, North Carolina.  EMB Report 88-CEP-14.
     September 1988.

38.  Chromium Electroplaters Test Report:  Hard Chrome Specialists, York,
     Pennsylvania.  Peer Consultants, Dayton, Ohio.  Prepared for U. S.
     Environmental Protection Agency, Research Triangle Park, North
     Carolina.  EMB Report-89-CEP-15.  January 1989.

39.  Emission Test Report:  Norfolk Naval Shipyard, Norfolk, Virginia.
     Naval Energy and Environmental Support Activity, Port Hueneme,
     California.  Source Emission Testing of the Building 195 Plating Shop
     at Norfolk Naval Shipyard, Portsmouth, Virginia.  March 11-18,
     1985.  NEESA 2-124.  May 1985.

40.  Chromium Electroplaters Test Report:  Piedmont Industrial Platers,
     Statesville, North Carolina.  Entropy Environmentalists, Inc.,
     Research Triangle Park, North Carolina.  Prepared for U. S.
     Environmental Protection Agency, Research Triangle Park, North
     Carolina.  EMB Report 86-CEP-04.  September 1986.

41.  Chromium Electroplaters Test Report:  Steel  Heddle, Inc., Greenville,
     South Carolina.  PEI Associates, Inc., Cincinnati, Ohio.  Prepared
     for U. S. Environmental Protection Agency, Research Triangle Park,
     North Carolina.  EMB Report 86-CEP-2.  June 1986.

42.  Chromium Electroplaters Test Report:  CMC Delco Products Division,
     Livonia, Michigan.  Peer Consultants, Inc.  Rockville, Maryland.
     Prepared for U. S. Environmental Protection Agency, Research Triangle
     Park, North Carolina.  EMB Report 87-CEP-7.   May 1987.

43.  Draft Chromium Electroplaters Test Report:  A Plant in the Midwest.
     Prepared for U. S. Environmental Protection Agency, Research Triangle
     Park, North Carolina.  April 1988.

44.  Memo from Barker,  R., MRI,  to Vervaert, A.,  EPA/ISB.   Engineering
     Analysis - Reliable Plating and Polishing Company.  May 1987.
     pp. 5-7.
                                    45

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45.  Chromium Emissions from Industrial Process Cooling Towers-Background
     Information for Proposed Standards.  Draft.  Prepared for U. S,
     Environmental Protection Agency.  Research Triangle Park, North
     Carolina.  May 1988.

46.  Telecon.  P. BelHn, MR!, with C. Bergesen, Utility Data Institute
     (UOI).  March 5, 1986.  UOI study on chromate use in electric
     utilities industry.

47.  Chromium Emissions from Comfort Cooling Towers-Background Information
     for Proposed Standards,  Prepared for U. S. Environmental Protection
     Agency.  Research Triangle Park, North Carolina.  March 1988.
     EPA-450/3-87-010a.

48.  Holmberg, J. D.t and 0. U Kinney.  Drift Technology for Cooling
     Towers.  The Marley Company, Mission, Kansas.  1973.

49.  Letter and attachments.  Mayer, A., Chemical Manufacturers
     Association, to Cuffe, S., EPA:ISB.  September 27, 1986.  Summary of
     CMA member survey on corrosion inhibitors used in process cooling
     towers including average ppm in recirculating water.

50.  Telecon:  C, Clark, MRI, with J. Holmberg, Marley Cooling Tower
     Company.  April 2, 1985.  Drift eliminator efficiency.

51.  Telecon:  P. Bell in, MRI, with J. Holmberg, Marley Cooling Tower
     Company.  July 19, 1985.  Drift eliminator efficiency.

52.  Kelly, G. M.  A System Efficient Approach to Cooling Tower Energy
     Modifications.  Cooling Tower Institute Technical Paper.
     No. TP-85-18.  New Orleans, Louisiana.  January 1985.

53.  Emission Test Report:  National Bureau of Standards, Gaithersburg,
     Maryland.  EMB Report 85-CCT-4.  October 1986.

54.  Emission Test Report:  Exxon Company Petroleum Refinery, Baytown,
     Texas.  EMB Report 85-CCT-3.  November 1986.

55.  Emission Test Report:  Southeastern Manufacturing Facility.   EMB
     Report 87-CCT-5.   Draft.  September 1987.

56.  Abstracts of six confidential  emission test reports conducted by MRI
     for industrial clients.

57.  Letter and attachments.  Hawes, R., Mobil Oil Corp., to Randall, D.,
     MRI.   August 24,  1987.  Emission test results.
                                    46

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                                  TECHNICAL REPORT DATA
1 • ^££QRT ^O. * A -. i 2, i3, RECIPIENT'S ACCESSION NO.
A.
TITLE AND SUBTITLE
Locating And Estimating Air Emissions From Sources
of Chromium (Supplement)
7. AUTHOR(S)
Jeff Shular. Robin Barker, Bruce Nicholson,
David Randall
9.
12
IS
16
PiRFORMING ORGANIZATION NAME AND ADDRESS
Midwest Research Institute
401 Harrison Oaks Boulevard
Cary, North Carolina 27513
. SPONSORING AGENCY NAME AND ADDRESS
U. S. Environmental Protection Agency
OAR, QAQPS, AQMD, PCS (MD-15)
Research Triangle Park, North Carolina 27711
S, REPORT DATE
August
6, PERFORMING ORGANIZATION CODE !
8. PERFORMING ORGANIZATION SEPOHT NO, 1
1
50. PROGRAM ELEMENT NO.
1 1 . CONTRACT/GRANT NO,
68-02-4395
13. TYPE OF REPORT AND PERIOD COVERED
Final
»4. SPONSORING AGENCY CODE
, SUPPLEMENTARY NOTES
EPA Project Officer: Dallas W. Safriet
. ABSTRACT j
t
  To assist  groups  inventorying  air emissions of potentially toxic substances,  EPA     j
  is preparing a  series of documents that compiles available Information on  sources
  and emissions of  toxic  substances.  This document deals specifically with  methods  to
  estimate chromium (Cr+6) emissions from cooling towers and electroplating  operations.'
17. KEY WORDS AND DOCUMENT ANALYSIS
a. DESCRIPTORS
Chromium (Cr+6)
Estimating Air Emissions
Air Toxic
Cooling Towers
Electroplating
18. DISTRIBUTION STATEMENT
Unlimited
I
b.IOENTIFtEHB/OPIN ENDED TERMS

19. SECURITY CLASS (This Rtportt
Unclassified
2Q. SECURITY CLASS IThispage)
Unclassified
c. COSATI [-'ietd/Gioup
i
\
"i
21, NO. Of PAGES i
50
22. PBICB i
EPA Form 2220-1 (R>«, 4-77)  PREVIOUS EDITION is OBSOLETE

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                                            EPA-4SQ/2-89-Q02
                                                 August 1989
  LQCATINS AND ESTIMATING AIR EMISSIONS FROM

             SOURCES OF CHROMIUM
                  SUPPLEMENT
                     By

         Midwest Research  Institute
                  Suite 350
         401 Harrison Oaks Boulevard
         Cary, North Carolina  27513

   EPA Project Officer:  Dallas M. Safriet
    U, S. Environmental  Protection Agency
         Office of Air and Radiation
Office of Air Quality Planning and Standards
Research Triangle Park,  North Carolina  27711
                 August  1989

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This report has been reviewed by the Office of Air Quality Planning And
Standards,  U.  S. Environmental Protection Agency, and approved for
publication.   Any mention of trade names or commercial products is not
intended to constitute endorsement or recommendation for use.
                             EPA-450/2-S9-002

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                             TABLE OF CONTENTS

                                                                      Page

 LIST OF FIGURES	     111

 LIST OF TABLES	     111

 SECTION 1.0  PURPOSE OF DOCUMENT	      1

 SECTION 2.0  OVERVIEW OF DOCUMENT CONTENTS.....	      3

 SECTION 3.0  CHROMIUM EMISSION SOURCES		      5

             3.1  CHROMIUM ELECTROPLATING AND CHROMIC ACIO
                    ANODIZING OPERATIONS	      5
                  3.1.1  Background Information.	      5
                  3.1,2  Uncontrolled Chromium Emissions....	     17
                  3.1.3  Emission Reduction Techniques	     21
                  3,1.4  Nationwide Emission Estimates	     23

             3.2  COOLING TOWERS.......................	     26
                  3.2.1  Background Information..	     26
                  3.2.2  Potential Emission Reduction Techniques...     29
                  3.2,3  Cooling Tower Emissions.,	     34
                  3.2.4  Nationwide Emissions Distribution by
                           Industry	     38

SECTION 4.0  SOURCE TEST PROCEDURES,.	     41

             4.1  CHROMIUM ELECTROPLATING	     41
             4.2  COOLING TOWERS,...	     41

SECTION 5.0  REFERENCES....	     43

APPENDIX A.  ADDITIONAL CHROMIUM ELECTROPLATING EMISSION  DATA
             OBTAINED AND EVALUATED DURING DEVELOPMENT OF THIS
             REPORT	    A-1
                                    11

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                              LIST OF FIGURES

                                                                       Page

 Figure  1.  Flow diagram for a typical chromic  add  anodizing
             process	      11

 Figure  2.  Internals of crossflow and counterflow cooling  towers...      30

 Figure  3.  Designs of various drift  eliminators	      33

                              -LIST OF TABLES

                                                                       Page

 TABLE 1.    TYPICAL OPERATING PARAMETERS FOR HARD CHROMIUM
              ELECTROPLATING	       7

 TABLE 2.    TYPICAL OPERATING PARAMETERS FOR DECORATIVE CHROMIUM
              PLATING	       9

 TABLE 3.    CHROMIC ACID/SULFUR1C ACID ETCH  SOLUTION..	       9

 TABLE 4.    TYPICAL OPERATING PARAMETERS FOR CHROMIC ACID
              ANODIZING..	      13

 TABLE S.    HEXAVALENT AND TRIVALENT CHROMIUM DEPOSIT CQMJ  OSITIQNS       16

 TABLE 6.    UNCONTROLLED EMISSION DATA FOR TOTAL AND HEXAVALENT
              CHROMIUM FROM CHROMIUM PLATING OPERATIONS	      18

 TABLE 7.    TANK PARAMETERS AND PROCESS OPERATING PARAMETERS
              MONITORED DURING CHROMIUM PLATING TESTS	..........      20

 TABLE 8.    PERFORMANCE LEVELS OF INDIVIDUAL CONTROL DEVICES	      24

 TABLE 9.    NATIONWIDE NUMBER OF OPERATIONS AND ESTIMATED HEXAVALENT
              CHROMIUM EMISSIONS FROM CHROMIUM ELECTROPLATING AND
              CHROMIC ACID ANODIZING OPERATIONS	      25

TABLE 10.   MODEL COMFORT COOLING TOWERS AND HOURLY BASELINE Cr*S
              EMISSIONS.	      28

TABLE 11.   EMISSION FACTORS FOR HEXAVALENT CHROMIUM FROM
              COOLING TOWERS...................	      36

TABLE 12.   NATIONWIDE COOLING TOWER CHROMIUM EMISSIONS SUMMARY	      40

TABLE A-l.  ADDITIONAL CHROMIUM ELECTROPLATING  EMISSION DATA
              OBTAINED AND EVALUATED DURING DEVELOPMENT OF  THIS
              REPORT	,	    A-l
                                    111

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                          1.0  PURPOSE OF DOCUMENT

       The  U.  S.  Environmental  Protection Agency  (EPA),  States,  and local
 air  pollution control  agencies are becoming Increasingly  aware  of the
 presence of  substances 1n  the  ambient  air that may  be toxic  at  certain
 concentrations.   This  awareness,  1n turn,  has led to attempts to  Identify
 source/receptor  relationships  for these  substances  and  to develop control
 programs to  regulate emissions.  Unfortunately,  very little  information 1s
 available  on  the ambient air concentrations of these substances or on the
 sources that  may be discharging them to  the atmosphere.
       To assist  groups Interested 1n Inventorying air emissions of various
 potentially toxic substances,  EPA 1s preparing a series of documents  that
 compiles available Information on the  sources and emissions  of  these
 substances.   This document was prepared  as  a supplement to a previous  EPA
 document that addressed chromium emissions,  "Locating and  Estimating  A1r
 Emissions  From Sources of Chromium," EPA-450/4-84-007g.   The supplement
 updates technical  Information  and presents  new emission data upon  which
 emission factors are based for chromium  emissions from cooling  towers  and
 chromium electroplating operations.  The reader  should use both the
 original document and  this supplement to obtain  the most complete
 assessment of emissions from these two sources of chromium emissions.   The
 Information 1n this supplement was obtained by EPA's Emission Standards
 Division for  use  in development of National Emission Standards for a
 Hazardous Air Pollutant (MESHAP)  for chromium used in electroplating
 operations and for regulation of  chromium emissions from comfort cooling
 towers under  the Toxic Substances Control Act.
      The reader  1s strongly cautioned against using the emissions
 Information contained 1n the original  document or this  supplement to
 develop an exact assessment of emissions from any particular facility.
 Because of Insufficient data, no  estimate can be made of the error that
could result when these factors are used to calculate emissions  from any
given facility.   It is  possible,  in some extreme cases,  that orders-of-
magnitude differences could result between actual and calculated
emissions,  depending  on differences  1n source configurations, control
equipment,  and operating practices.  Thus, in situations where an  accurate

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assessment of chromium emissions is necessary, source-specific information
should be obtained to confirm the existence of particular emitting
operations, the types and effectiveness of control measures, and the
impact of operating practices.  A source test and/or material balance
should be considered as the best means to determine air emissions directly
from an operation.
      Possible sources of plant-specific information that would be useful
in estimating air emissions of hexavalent chromium include the National
Air Toxics Information Clearinghouse database maintained by EPA or the
Toxics Release Inventory (TRI) data resulting from Section 313 of the
Superfund Amendments and Reauthorization Act (SARA).   In the absence of
specific information about the locations of facilities, State Departments
of Commerce, trade associations, or references such as the Thomas Register
of AmericanManufacturers may be sources of information.

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                     2.0   OVERVIEW  OF  DOCUMENT  CONTENTS

      This section outlines the  Information presented in  the  remaining
sections of this report and indicates whether  the information is  new  or
whether 1t is a revision  of information presented 1n the  original
document.
      Section 3.1 presents process descriptions for five  kinds  of
plating/anodizing operations.  New information is included  for  decorative
chromium electroplating of plastics, chromic acid anodizing,  and  trivalent
chromium plating.  Additional process information is provided to
supplement the discussion of hard and decorative chromium electroplating
presented in the original document.  New emission data are  presented  for
hard and decorative chromium electroplating operations; the results of  an
engineering mass balance to obtain an emission estimate for chromic acid
anodizing are also presented.  A significant change from the  original
document is 1n the format of the chromium emission factors for  hard and
decorative plating operations, which have changed from kilograms per  hour
per square foot of tank area to milligrams per ampere-hour.   Supplemental
information has been Included on emission control  techniques  for" reduction
of chromic acid mist from plating operations.   New information  1s
presented on nationwide chromium emission estimates for three types of
plating operations:  hard plating,  decorative  plating,  and chromic acid
anodizing.
      Section 3.2 presents updated  information about the distribution of
industrial process cooling towers that use chromium-based water treatment
chemicals and presents new information about comfort cooling towers.  New
information also is presented on emission reduction techniques for
chromium emissions from cooling towers.   New emission data are presented
for cooling towers equipped with low-  and high-efficiency drift
eliminators.   A significant change  from the original  document is in the
format of the chromium emission factor,  which  has  changed from picograms
per joule of thermal  energy input to the power plant  associated with the
cooling tower to percentage of the  recirculatlng chromium that is
emitted.   New information is presented on nationwide  chromium emission
estimates for industrial  cooling towers  in eight industries.

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      Section 4.0 summarizes the procedures used for source sampling and
analysis of chromium in emission streams from electroplating operations
and cooling towers.

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                       3.0  CHROMIUM  EMISSION SOURCES

3.1  CHROMIUM  ELECTROPLATING AND CHROMIC ACID ANODIZING OPERATIONS
3.1.1  Background  Information
      Plating  and  anodizing operations range in size from small shops,
with one or two tanks that are operated only a few hours per week, to
large shops with several tanks that are operated 24 hours per day, 7 days
per week.  Many platlnf and anodizing -operations are captive shops that
perform chromium electroplating or chromic tcld anodizing as one operation
within or for  a manufacturing facility, while others are job shops that
provide custom plating or anodizing services for many different clients.
Captive and job shops nay perform hard or decorative chromium plating or
chromic add anodizing or any combination of these three operations.
      The estimated number of electroplating shops nationwide is
1,§4Q hard chromium plating facilities and 2,800 decorative chromium
plating facilities.1  The estimated number of chromic add anodizing shops
nationwide 1s  680.2  Electroplating and anodizing shops typically are
located 1n or  near Industrial centers 1n areas of high population
density.  States with large numbers of chromium electroplaters include
California, Illinois, Massachusetts,  Michigan, Mew York, Ohio, and
Pennsylvania.
      3.1.1.1  HardChromium Electroplatinfl of Metals.   In hard plating, a
relatively thick layer of chromium 1s deposited directly on the base metal
(usually steel) to provide a surface  with wear resistance, a low
coefficient of friction, hardness, and corrosion resistance, or to build
up surfaces that have been eroded by  use.   Hard plating is used for items
such as hydraulic cylinders and rods, industrial  rolls,  zinc die castings,
plastic molds, engine components, and marine hardware.
      Tanks used for hard chromium electroplating usually are constructed
of steel  and lined with a polyvlnyl chloride sheet or plastisol.   The
anodes, which are Insoluble,  are made of a lead alloy that contains  either
tin or antimony.  The substrate to be plated, the cathode,  is suspended
from a plating rack that 1s connected to the cathode  bar of  the
rectifier.   The plating rack  may be loaded in the tank manually,  by  a
hoist,  or by an automatically controlled hoist system.

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      The plating  tanks typically are equipped with  some type of heat
exchanger.  Mechanical agitators or compressed air supplied through pipes
on the tank bottom provide uniformity of  bath temperature and
composition.  Chromium electroplating requires constant control of the
plating bath temperature, current density, plating time, and bath
composition.
      Hexavalent chromium plating baths are the most widely used baths to
deposit chromium on metal.  Hexavalent chromium baths are composed of
chromic add, sulfuric acid, and water.   The chromic add is the source of
the hexavalent chromium that reacts and deposits on the metal and that is
emitted to the atmosphere.  The su If uric  add in the bath catalyzes the
chromium deposition reactions.  Typical operating parameters are given in
Table I.1*
      The evolution of hydrogen gas from  chemical reactions at the cathode
consumes 80 to 90  percent of the power supplied to the plating bath,
leaving the remaining 10 to 20 percent for the deposition reaction.  When
the hydrogen gas evolves, it entrains chromic acid and causes misting at
the surface of the  plating bath.
      3.1.1.2  Decorative Chromium Electroplating of Metals.  In decorative
plating, the base material (e.g., brass,  steel, aluminum, or plastic)
generally is plated with a layer of nickel followed by a relatively thin
layer of chromium to provide a bright surface with wear and  tarnish
resistance.  Decorative plating is used^for items such as^utomotive trim,
metal furniture, bicycles, hand tools, and plumbing fixtures.   The  purpose
of decorative chromium plating is to achieve a combination of the
following surface properties:
      1,  Blue-white color;
      2.  High reflectivity;
      3.  Tarnish resistance;
      4.  Corrosion resistance;
      5.  Wear resistance; and
      6.  Scratch resistance.5
      Decorative electroplating baths  operate  on  the  same  principle  as
that  described for the hard  chromium plating process:   the metal substrate
is immersed in a plating  solution,  and direct  current  is passed from the

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  TABLE 1.  TYPICAL OPERATING PARAMETERS FOR HARD CHROMIUM ELECTROPLATING
Plating thickness, va (roll)                               1.3-762  (0.05-30)
Plating time, m1na                                                20-2,160
Chromic acid concentration, g/4 (oz/gal)b                  225-375  (30-50)
Temperature of solution, °C (°F)                           49-66  (120-150)
Voltage, volts                                                          c
Current, amperes (A)                                                    d
Current density, A/m2 (A/ft2)6                                1,600-6,500
                                                                  (150-600)
?m1n. = minutes.
°g/i » grams per liter,  oz/gal = ounces per gallon.
^Depends on the distance between the anodes and the Items being plated.
Depends on the amount of surface area plated.
eA/m  = amperes per square meter (square foot) of surface area plated.

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anode through the plating solution causing the desired metal  (copper,
nickel, chromium) to deposit out of the solution onto the metal substrate
(cathode).
      Decorative chromium plating requires shorter plating times and
operates at lower current densities than does hard chromium plating to
achieve the desired properties of the chromium plate.  Some decorative
chromium plating operations use fluoride catalysts Instead of sulfuric
add because fluoride catalysts, such as fluosHlcate or fluoborate, have
been found to produce higher bath efficiencies.5  Typical operating
parameters are shown in Table 2.
      3.1.1.3  Decorative Chromium Electroplating of Plastics.  Most plastics
that are electroplated with chromium are formed from the polymer composed
of acrylonitrlle, butadiene, and styrene (ABS).a  The process for chromium
electroplating of ABS plastics consists of the following steps:
      1.  Chromic acid/sulfuric acid etch;
      2.  Dilute hydrochloric acid dip;
      3.  Colloidal palladium activation;
      4.  Dilute hydrochloric acid dip;
      5.  Electroless nickel plating or copper plating;  and
      6.  Chromium electroplating cycle.
      After each process step, the plastic 1s rinsed with water to prevent
carry-over of solution fromjme bath to another.  The chromic add/
sulfuric acid etch solution (see Table 3)  renders the ABS surface
hydrophlllc and modifies the surface to provide adhesion for the metal
coating.   The dilute hydrochloric acid dips  are used to clean the surface
and remove palladium metal  from the plating rack, which  is Insulated with
a coating of polyvinyl  chloride.  The colloidal  palladium activation
solution deposits a thin layer of metallic palladium over the plastic
surface.    The metallic palladium Induces the deposition of copper or
nickel, which will not  deposit directly onto  plastic. The electroless
nickel  and copper plate are applied to Impart electrical  conductivity to
the part; otherwise, the insulating surface of the plastic could not be
electroplated with chromium.  The electroless nickel  plating or copper
electroplating baths develop a film on the plastic about  1.0 micrometer
(wm) (3.9xlO"s inch [in.])  thick.  The plating time for  electroless nickel

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  TABLE 2.  TYPICAL OPERATING PARAMETERS FOR DECORATIVE CHROMIUM PLATING
Plating thickness,  pm (rail)                          0.003-2.5  (0.0001-0.1)
Plating time, min                                                   0.5-5
Chromic add concentration,  g/i  (oz/gal)                    225-375  (30-50)
Temperature of solution,  d.C  (°F)                            38-46 (100-115)
Voltage, volts                                                          a
Current, A                                                              b
Current density,  A/m2 (A/ft2)c                          540^2,400 (50-220)
^Depends on the distance  between the anodes  and the  items being  plated.
 Depends on the amount of surface area being plated.
 Amperes per square meter (square foot) of surface area plated.
            TABLE 3.   CHROMIC ACID/SULFURIC ACID ETCH SOLUTION
      Concentrated sulfuHc add, g/a (oz/gal)              172 (23)
      Chromic  add, g/a (oz/gal)                            430 (57)
      Temperature, 'C  (°F)                           60-65 (140-149)
      Immersion time, min                                      3-10

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 plating and electroless copper plating ranges from 10 to 15 minutes and 15
 to 30 minutes, respectively, at temperatures ranging from 25° to 35°C (77°
 to 95°F).   The components of the plating baths Include the metal salt
 (nickel or copper), a reducing agent, a complexing agent, a stabilizer,
 and a pH buffer system.11  The electroplating of plastics follows the same
 cycle as that described for decorative chromium electroplating.12
       3.L.I.4  Chromic Acid Anodizing.  Chromic acid anodizing is used primarily
 on aircraft parts and architectural  structures that are subject to high
 stress and corrosion.  Chromic add  anodizing 1s used to provide an oxide
 layer on aluminum that Imparts the following properties:
       1.  Corrosion protection;
       2.  Electrical Insulation;
       3.  Ease of coloring; and
       4.  Improved dielectric strength.1
 Figure 1 presents a flow diagram for a typical  chromic add  anodizing
 process.
       There are four primary differences  between the equipment used for
 chromium electroplating and that used for chromic 'add anodizing:
 (a)  chromic add anodizing requires  the .rectifier to be fitted with a
 rheostat or other control  mechanism  to permit starting at about 5  V,
 (b)  the tank Is the cathode 1n the electrical  circuit,  (c) the aluminum
 substrate  acts as the anode, and (d)  sldewall  shields typically are used
Jnstead^of a liner in the  tank-to minimize short circuits and._to decrease
 the  effective cathode area.    Types  of shield  materials  used  are
 hercullte  glass,  wire safety glass,  neoprene,  and vinyl chloride
   ,       is
 polymers.
       The  following pretreatment steps typically  are  used  to clean  the
 aluminum before anodizing:
       1.   Alkaline soak;
       2.   Oesmut;
       3.   Etching;  and
       4.   Vapor degreasing.
 The  pretreatment  steps  used  for  a particular aluminum substrate depend
 upon the amount of  smut and  the  composition of the aluminum.  The aluminum
 substrate  is  rinsed  between  pretreatment steps to remove cleaners.
                                     10

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             SUBSTRATE TO BE PLATED
               PRETREATMENT STEPS

               Alkslln* sock
               O«tm«Jt
               Etching
               Vapor d«gr«*ains
                          RINSE
            CHROMIC ACID ANODIZING
                         RINSE
                     SEALING
                 FINAL PRODUCT
CHROMIC ACID
  EMISSIONS
Figure 1.   Flow diagram for a typical Chromic add  anodizing process.
                                 11

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       The alkaline soak is the primary preparatory step in cleaning the
 aluminum; its purpose is to dislodge soil from the aluminum surface.  The
 solutions for alkaline cleaning are typically made up of compounds such as
 sodium carbonate, sodium phosphate, and sodium hydroxide and usually
 contain a small amount of silicate to prevent metal attack.15  The
 alkaline soak consists of immersing the metal 1n the alkaline solution
 that 1s mildly agitated with air.
       The purpose of desmuttlng is to remove soil or grease films that
 cleaners and etchants leave behind*  Oesrauttlng baths typically consist of
 a cold nitric add solution mixed with water at a concentration ranging
 from 5 to 50 percent acid by volume.  The nitric acid bath also is used
 either as a bleaching treatment to remove dyes from faulty coatings or as
 part of the technique of producing multicolor coatings.1   Other
 desinutting treatments use combinations of chromic, phosphoric, and
 sulfyHc acids depending ypon the amount of smut to be removed or the
 aluminum composition.
       When a dull finish 1s desired, the aluminum is etched before
 anodizing.  Etching baths consist of a dilute solution of soda ash,
 caustic soda, or nitric add.18  The degree of etching desired and the
 composition of the aluminum being treated determine the concentration of
 the itch solution, temperature of the bath, and duration of the etch.
	The^vapor_degreas1ng step removes any residual  oil or grease on the
 surfflcs of the ilucilnunt "rior to the anodlzln'* operation,
       Typical operating parameters for chromic acid anodizing  baths are
 presented in Table 4.I9f2°  The voltage is applied step-wise (5 V per
 minute) from 0 to 40 V and maintained at 40 V for the  remainder of the
 anodizing time.   A low starting voltage (i.e.,  5  V) minimizes  current
 surge that may cause "burning"  at contact points  between the rack and  the
 aluminum part.  The process  Is  effective over a wide range  of  voltages,
 temperatures, and anodizing  times.  All  other factors  being equal,  high
 voltages tend to produce bright transparent  films,  and  lower voltages  tend
 to produce opaque films.     Raising  the bath temperature increases  current
 density to produce thicker films  in  a given  time  period.  Temperatures up
 to 49°C (120aF)  typically  are used to produce films that are to be  colored
 by dytlng.     The amount of current  varies depending on  the  size  of the
                                     12

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      TABLE 4.  TYPICAL OPERATING PARAMETERS FOR CHROMIC
                        ACID ANODIZING
Chromic add concentration, g/8, (oz/gal)    50-100 (6.67-13.3)
Temperature, 3C (°F)                             32-35 (90-95)
Plating time, mln                                       30-60
pH                                                   0.5-0.85
Current density, A/m2 (A/ft2)a           1,550-7,750 (144-720)
Voltage (step-wise), volts                              30-40
Film thickness, um (mil)                   0.5-1.27 (0.02-0.05)
aAmperes per square meter (square foot)  of surface area
 plated.
                              13

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aluminum parts; however, the current density typically ranges from 1,550
to 7,750 A/ra2  (144 to 720 A/ft2).
      Tht pastanoeHzIng steps Include sealing and  air drying.  Sealing
causes hydration of the aluminum oxide and fills the pores in the aluminum
surface.  As a result, the elasticity of thi oxide film increases, but the
hardness and wear resistance decrease.    Sealing  1s performed by
Immersing aluminum 1n a water bath at 88° to 99°C  (190° to 210'F) for a
minimum of 15 minutes.    Chromic acid or other chromates lay be added to
the solution to help improve corrosion resistance.  The aluminum Is
allowed to air dry after 1t is sealed.
      3.1.1.5  Trtvalent Chromium Plating.  THvalent chromium
electroplating baths have been developed primarily to replace decorative
hexavalent chromium plating baths.  Development of a trivalent bath has
proven to be difficult because trivalent chromium  solvates in water to
form complex stable Ions that do not readily release chromium.  Thi
trivalent chromium baths that have been developed  are proprietary baths.
      There are two types of trivalent chromium processes on the market:
single-cell and double-cell.  The major differences in the two processes
are that (I) the double-cell process solution contains minloial-to-no
chlorides whereas the single-cell process solution contains a high
concentration of chlorides; and (2) the double-cell process utilizes lead
anodes that are placed in anodeboxes-that^contain a dilute sulfuric acid
solution ind are llney with i permeable tlelbfane whereas the single-cell
process utilizes carbon or graphite anodes that are placed in direct
contact with the plating solution.25
      The advantages of the trivalent chromium processes over the
hexavalent chromium process are (1) fewer environmental  concerns,
(2) higher productivity, and (3)  lower operating costs.   In the trivalent
chromium process, hexavalent chromium 1s a plating bath  contaminant.   .
Therefore, the bath does not contain any appreciable amount of hexavalent
chromium, which is more toxic than trivalent chromium.   The total  chromium
concentration of trivalent chromium solutions 1$. approximately one-fifth
that of hexavalent chromium solutions.     As a result of the  chemistry of
the trivalent chromium electrolyte, misting does not occur during plating,
as 1t does during hexavalent chromium plating.   Use of trivaltnt  chromium
                                    14

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 also reduces waste disposal  problems  and  costs.   Waste treatment of
 hexavalent chromium  Is  a  two-stage process.   The hexavalent  chromium  is
 first reduced to the  trivalent  chromium ion;  then it  can  be  precipitated
 as chromium hydroxide.  Trivalent chromium plating solution  wastewaters
 are already 1n the reduced trivalent  state and require.only  the  chromium
 hydroxide precipitation step.
      Productivity 1s Increased when  trivalent chromium processes  are  used
 because less stripping  and replatlng  of parts are required,  more parts can
 be placed on a rack,  and  more racks can be placed on  a workbar.
      The cost of operating  a trivalent chromium process  is  less than  that
 of a hexavalent chromium  process because  of the  lower wastewater treatment
 costs and lower operating costs due to a  reduction in rejects and  high
 productivity.
      The disadvantages of the  trivalent  chromium process are that the
 process 1s more sensitive to contamination than  the hexavalent chromium
 process and the trivalent chromium process cannot plate the  full range of
 plate thicknesses that the hexavalent chromium process can.    Because 1t
 1s sensitive to contamination,  the trivalent  chromium process requires
 more thorough rinsing and tighter laboratory  control  than the hexavalent
 chromium process.  Trivalent chromium baths can  plate thicknesses ranging
 up to 0.13 to 25 micrometers (ym) (0.005 to 1.0  mils).28  The hexavalent
 chromium process can plate thicknesses up to  762  urn (30 mils).  Therefore,
 trivalent chromium solutions cannot be used for most  hard chromium plating
 applications.
      The plating efficiency of a trivalent chromium bath, approximately
 20 to 25 percent, 1s slightly higher than that of a hexavalent chromium
 plating bath.     The color, hardness,  and corrosion resistance of triva-
 lent chromium deposits are comparable  to those of hexavalent chromium
 deposits.  °   However, the composition  of the trivalent chromium deposit is
 significantly different than that of the hexavalent chromium deposit.
Table 5 presents the composition of trivalent and hexavalent chromium
deposits.
                                    15

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     TABLE 5.  HEXAVALENT AND TRIVALENT CHROMIUM DEPOSIT COMPOSITIONS
Chnwrfym deposit      Carbon, % wt       Oxygen,  % wt        Chromium,  % vt
Hexavalent                 0.0                Q.4               99+
Trfvilent                  2.9                1.6               95+
                                   16

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 3.1.2  Uncontrolled Chromium  Emissions
       Emissions of chromic acid mist  from the electrodeposition of
 chromium  from chromic acid plating  baths  occur because  of  the inefficiency
 of the hexavalent chromium plating  process;  only  about  10  to  20 percent of
 the current  applied actually  is used  to deposit chromium on the item
 plated.   Eighty to ninety percent of  the  current  applied is consumed by
 the evolution of hydrogen gas at the  cathode with the resultant, liberation
 of gas bubbles.  Additional bubbles are formed at the anode due to the
 evolution of oxygen.  As the  bubbles  burst at the surface  of  the plating
 solution, a  fine mist of chromic acid droplets is formed.
       3.1.2.1  Hard Chromium  and Decorative  Electroplating Operations.
 Uncontrolled emission data for 10 hard chromium plating operations and
 2 decorative chromium plating operations  are presented  in  Table 6.   These
 data were obtained from 11 EPA tests  and  1 non-EPA test.   Table 7  presents
 tank parameters and process operating parameters  monitored during  each of
 the 12 tests.  The process parameters monitored during testing  include
 current supplied to the plating baths, voltage, chromic acid  concentration,
 and temperature of the plating baths.  The chromic acid concentration  and
 temperature did not vary significantly within  each type operation  for  the
 emission  tests and appeared to be representative of typical operating
 values for conventional  hard and decorative  chromium plating operations.
 The amount of current supplied during testing  varied considerably  because
 of the different types and quantities of parts plated.
       Based on the existing test data, an  uncontrolled emission factor of
 10 milligrams of hexavalent chromium  per ampere-hour (mg/Ah)  (0.15 grain
 per ampere-hour [gr/Ahl) 1s considered to  be representative of uncon-
 trolled emissions from a hard chromium electroplating operation, and an
 uncontrolled hexavalent  chromium emission  factor of 2 mg/Ah (0.03 gr/Ah)
 Is considered representative of uncontrolled emissions from a decorative
chromium electroplating  operation.
      The emission factor for uncontrolled chromium emissions  from
decorative chromium plating operations is  based on EPA-approved test data
from two plants  whose  tanks represent  the  extremes in tank  size for
decorative chromium plating.   Although the sizes of these tanks may not be
                                    17

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                        TABLE 6.  UNCONTROLLED EMISSION DATA  FOR  TOTAL AND HEXAVALEKT CHROMIUM FROM
                                               CHROMIUM PLATING OPERATIONS8
00
Plant
Hard chroaiitm plating
Plant Ab'32
Plant Bc'33
Plant C11'34
Plant Dc'35
Plant EC-M
Plant Ff'37
Plant 6C'38
Plant Hc»39
Plant I1'40
Plant Jc'41
Average
Process conditions
Total tank
No. of surface area, Aapero-
tanks m2 «t2)| hours
1 5.8 14,000
2 2.5 14,400
(S'7)
4 8.4 20,000
1 5.2 19,800
1 3,4 11,700
(37)
1 1.8 12,200
(30) ;
1 1.4 8,900
(1,5)
» 5.5 3,440
2 9.0 i 8,530
(99)
3 6.6 8,790
on
Actual
gas flow
rate,
(ft3/«ln)
226
(7,970)
152
(5,390)
339
(12,000)
177
190
120
(4,540)
95
242
(8,540)
290
(10.300)
512
(18,100)
Mass emission
rate, kg/lt (Ib/h)
Total Cr
0.029
(0.064)
0.008
(0.018)
«
0.076
(0.167)
e
e
e
0.009
(0.019)
0.100
(0,221)
0.044
(0.097)
cP*
0.026
(0.057)
0.015
(0.033)
0.039
(0.085)
0.076
(0.168)
0.031
(0.069)
0.083
(0.183)
0.024
(0.053)
9
9
0.090
(0.199)
0.046
(0,102)
Process Cr emission
rate, aig/A»h (gr/A«h)
4.0 (0.06)
3.2 (0.05)
4.6 (0.07)
9.1 (O.14)
6.3 (0.10)
16.3 (0.25)
6.5 (0.10)
3.6 <0,06)h
22.5 (0.35)
15.5 (0.24)
9,8 (0.15)
                                                                                                           (continued)

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                                                   TABLE  6.   (continued)
Process conditions
Plant
No, of
tanks
Total tank
surface area,
a2 (ft2)
Ampere- .
hours
Actual
gas flow
rate,
(ft5/m!n)
Mass emission
rate, kg/h (Ib/h)
Total Cr Cr*6
Process Cr emission
rate, mg/A«h (gr/A-h)
Decorative chromium plating
Plant Kc»**

Plant Lc>43

Average
i 22.6
(240)
I 2.9
(30.6)

97,000

6.500


683
(24,100)
10
(2,410)

e 0.066
(0.145)
a 0.004
(0.006)

2.0 CO.OJ)

1.3 (0.02)

1.6 (0.02)
 All tests were perforated by EPA except for the Plant  H test  which was performed by the Naval Energy and Environmental  Support
 Activity, Port Hueneme, California.
 Ampere-hour and BBSS emission rate values are based on an  average of four test runs.
^Ampere-hour and mass emission rate values are based on an  average of three test runs.
^Ampere-hour and mass emission rate values are based on an  average of six test runs,
^Tota I chronlun emissions Mare not determined.
 Ampere-hour and mass emission rate values are based on an  average of five test runs.
^Hexavalent chromium emissions nere not reported.
"Not Included In average value because data are based  on total chromium.
 Ampere-hour and mass emission rate values are based on an  average of II test runs.

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             TABLE 7.  TANK  PARAMETERS AND PROCESS OPERATING  PARAMETERS MONITORED DURINS CHROMIUM PLATING TESTS
ro
o
Average process


Tank paraaeters
Total tank Total tank
, No. of surface area, capacity, Current,
Plant tank(s)
Hard chromium plating
Plant A32 1
Plant B33 2
Plant C34 4
Plant O31
Plant E36
Plant F37
Plant G38
Plant H39
Plant I40 2
Plant J41 3
Decorative chromium plating
Plant K42 I
Plant L43 1
or (ft2)* t (gal)b amperes

5.8 (63) 10,710 (2,830) 6,220
2.5 (27) 4,130 (1,090) 1,610
8.4 (90) 35,000 (9,250) 2,860
5.2 (56) 15,820 (4,180) 6,390
3.4 (37) 9,270 (2,450) 4,970
1,8 (20) 4,810 (1,270) 2,640
1.4 (15) 5,720 (1,510) 3,480
5.5 (60) 7,190 (1,900) 2,480
9.0 (99) 11,210 (2,960) 1,140
6.6 (71) 6,090 (1,610) 1,150

22.6 (240) 61,170 (16,160) 21,320
2.9 (JO 3,860 (1,020) 2.700


Voltage,
volts

9.0
12.3
7.9
7.4
7.0
4.9
4.9
6.6
7.7
6.1

22.4
5.1
parameters monitored
Chronic
acid
concen-
tration.
fl/l
(oz/gal)

254 (34)
208 (28)
250 (33)
156 (21)
250 (33)
210 (28)
210 (28)
210 (28)
225 (30)
173 (23)

300 (40)
241 (32)

Bath
temp..
'C (*F)

52 (125)
62 (145)
54 (130)
52 (125)
54 (130)
56 (133)
55 (131)
60 (140)
59 (13S)
49 (120)

54 (130)
48 (119)
           "nr* = square meters, ft* » square feet.
            £ - liters, gal = gallons.

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 typical  of  the  sizes  of  other decorative  plating  tanks,  there is
 insufficient  evidence to show that emissions  are  directly  proportional  to
 tank  size.  In  any  case, the uncontrolled emissions  have been normalized
 to  account  for  tank size using the ampere-hours term in the  emission
 factor.  Because  the  data are limited, a conservative  approach was  taken
 in  selecting  the  emission factor for decorative plating.   Thus, a value of
 2 mg/Ah  was selected  instead of the average value for  the  two tests.
       3.1.2.2  Chromic Acid Anodizing Operations.  Uncontrolled emission
 data  for chromic  acid anodizing operations were not  obtained  through an
 EPA source  test at  an anodizing facility.  Instead,  an estimate of  the
 amount of hexavalent  chromium emissions was made  by  performing a mass
 balance  on  a  scrubber used to control emissions from a chromic add
 anodizing operation.   Outlet scrubber water grab  samples were analyzed  to
 determine the amount  of  hexavalent chromium in the sample, and a mass
 balance  was performed on  the scrubber to determine the Inlet  hexavalent
 chromium emission rate.   The results of this mass balance  indicate that an
 uncontrolled  of emission  factor of 6.0x10'* kllograa of hexavalent
 chronlUB per  hour per square meter of tank surface area (1.2x10'* pound
 per hour per  square foot of tank surface area) 1s appropriate to
 characterize  emissions froa chromic acid anodizing/1*  Alternatively, if
 the tank surface area  1s unknown,  uncontrolled emission rates can be used
 to  approximate  the  level of uncontrolled chromium emissions.   The results
 of  the mass balance at the small  anodizing operation (tank  capacity
 -1,900 liters [500 gallons])  and  results from a non-EPA emission test at a
 large chromic acid anodizing operation  (tank  capacity -17,600 liters
 [4,600 gallons]) indicate uncontrolled  emission rates range from 0.0012 to
 0.0028 kg/h (0.0026 to 0.0062 lb/h),  respectively/"   At  this time,  there
 are Insufficient data from anodizing  operations to determine  conclusively
 that one emission factor format  is  more appropriate than  the  other.
 3.1.3  Emission Reduction Techniques
      The principal  techniques used to  control emissions  of chromic  acid
mist from decorative and hard chromium  plating and chromic  acid anodizing
operations Include add-on control devices  and  chemical  fume
 suppressants.   The control devices most  frequently used are mist
eliminators and wet  scrubbers that are  operated at relatively low pressure
                                    21

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drops.  Because of the corrosive properties  of chromic  acid,  control
devices typically are made of polyvinyl chloride  (PVC)  or  fiberglass.
      Chemical fume suppressants are added to decorative chromium  plating
and chromic acid anodizing baths to reduce chromic acid mist.  Although
chemical agents alone are effective control  techniques, many  plants use
them in conjunction with a control device.
      Chevron-blade and mesh-pad mist eliminators are the  types of mist
eliminators most frequently used to control  chromic acid mist.  The most
important mechanism by which mist eliminators remove chromic  acid droplets
from gas streams is the inertial impaction of droplets  onto a stationary
set of blades or a mesh pad.  Mist eliminators typically are  operated as
dry units that are periodically washed down with water  to  clean the
impaction media.
      The wet scrubbers typically used to control emissions of chromic
acid mist from chromium plating and chromic acid anodizing operations are
single and double packed-bed scrubbers.  Other scrubber types used less
frequently include fan-separator packed-bed and centrifugal-flow
scrubbers.  Scrubbers remove chromic add droplets from the gas stream by
humidifying the gas stream to Increase the mass of the droplet particles,
which are then removed by Impingement on a packed bed.  Once-through water
or recirculated water typically is used as the scrubbing liquid because
chromic acid is highly soluble in water.
      Chemical fume suppressants are surface-active compounds that are
added directly to chromium plating and chromic acid anodizing baths to
reduce or control misting.   Fume suppressants are classified as temporary
or as permanent.   Temporary fume suppressants are depleted  mainly by the
decomposition of the fume suppressant and  dragout of the plating  solution,
and permanent fume suppressant are depleted mainly by dragout of  the
plating solution.  Fume suppressants,  which are manufactured in liquid,
powder,  or tablet form, include wetting  agents  that  reduce  misting by
lowering the surface tension of the plating or  anodizing bath, foam
blankets that entrap chromic acid  mist  at  the surface  of the plating
solution,  or combinations of both  a wetting agent and  foam  blanket.
                                    22

-------
       The  performance  capabilities  of the  control  devices  used to control
 chromic  add mist  are  presented  in  Table 8.   The  air  pollution control
 devices  tested  include four mist  eliminators,  three packed-bed scrubbers,
 and  one  packed-bed scrubber in conjunction with a mist  eliminator used  to
 control  emissions  from hard chromium  plating operations.   In  addition,  one
 emission test was  conducted at a  decorative chromium  plating  facility to
 determine  the performance of chemical  fume suppressants in controlling
 chromic  add mist.
       The  average  hexavalent chromium removal  efficiency of mist
 eliminators was 98 percent for mist eliminators with  double sets  of
 blades,  90 percent for mist eliminators  with single sets of blades*  and
 98 percent for mesh pad units.  The average hexavalant  chromium removal
 efficiency of scrubbers was 98 percent.  The hexavalant chromium  removal
 efficiency of the scrubber in conjunction with the mist eliminator was
 95 percent.
       For  decorative chromium plating operations* the performance
 efficiency of both chemical fume  suppressants tested  (a foam blanket  and a
 combination of a foam blanket and wetting agent) was greater than
 99 percent.  This performance efficiency 1s achievable  as  long as  vendor
 recommendations on the makeup and use of the fume suppressants are
 followed rigorously.
 3.1.4  Nationwide Emission Estimates
      Table 9 presents the estimated number of operations and the
 nationwide annual  emission rate for each type of operation.  The
 assumptions regarding the existing control  levels  for each type operation
were derived from data obtained during the  development of the NESHAP for
 chromium electroplating operations.   The nationwide emission rate for hard
chromium electroplating operations was based  on the assumption that
30 percent of operations are uncontrolled,  30  percent  of operations are
controlled by mist eliminators  with  single  sets of blades (90  percent
efficient), and  40 percent are  controlled by  single packed-bed scrubbers
 (97 percent efficient).  The nationwide emission rate  for decorative
chromium electroplating operations was based on the assumption that
15 percent of operations  are  uncontrolled,  80  percent  are  controlled  by
chemical  fume suppressants (97  percent efficient),  and 5 percent are

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                                   TABLE  8.    PERFORMANCE  LEVELS  OF  INDIVIDUAL CONTROL DEVICES
Plant  Plant
code  n
-------
  TABLE  9.   NATIONWIDE NUMBER OF OPERATIONS AND ESTIMATED
HEXAVALEMT CHROMIUM EMISSIONS FROM CHROMIUM ELECTROPLATING
          AND CHROMIC ACID ANODIZINS OPERATIONS
Qptratlon
No. of plants
  natlomddt
                                                     Nationwide
                                                   Cr   emissions,
                                                   Mg/yr (tons/yr)
Hard chromium plating
Decorative chromium plating
Chromic acid anodizing
    1,540
    2,800
     680
                                                     145 (160)
                                                       10 (11)
                                                     3.6 (3.9)
                           25

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controlled by single packed-bed scrubbers (95 percent efficient).  The
nationwide annual emission rate for chromic acid anodizing operations was
based on the assumption that 40 percent of operations are uncontrolled,
10 percent are controlled by mist eliminators with single sets of blades
(90 percent efficient), 30 percent are controlled by chemical fume
suppressants (97 percent efficient), and 20 percent are controlled by
single packed-bed scrubbers (9S percent efficient).
3.2  COOLING TOWERS
3.2.1 , Background Information
      Cooling towers are devices that cool warm water by contacting it
with ambient air that 1s drawn or forced through the tower.  This cool
water is used to remove heat from a process or an HVAC chiller and is then
recirculited to the cooling tower.  Chemicals are added to this
recirculatlng water to inhibit heat exchanger corrosion.  One of the many
classes of corrosion inhibitors used is chromium based.  A1r emissions of
chromium occur when water droplets (and the chemicals they contain)
entrained in the air stream that is drawn through the tower are emitted to
the atmosphere.  These droplet emissions are referred to as "drift."  All
cooling towers that are used to remove heat from an industrial process or
chemical reaction art referred to as Industrial process cooling towers
(IPCT's).  Towers that are used to cool heating, ventilation, and air
conditioning (HVAC) andrefrigeration systems are referred to_as comfort
cooling towers (CCT's).
      3.2.1.1  Industrial Process Cooling Towers.  Major users of IPCT's
that also use chromium-based water treatment chemicals are chemical
manufacturing plants, petroleum refineries,  and primary metals
facilities.  Several miscellaneous manufacturing industries (textiles,
tobacco products, tire and rubber products,  and glass products) and
utilities use chromium-based water treatment chemicals to a lesser
degree.  It is estimated that IPCT's ari used at approximately 190 petro-
leum refineries, 1,800 chemical manufacturing plants,  240 primary metals
plants, and 730 plants in the miscellaneous  industries.*   In addition,
the percentage of cooling towers using chromium-based  water treatment
chemicals in each Industry Is estimated as 70 percent  at petroleum
refineries, 40 percent at chemical  manufacturing plants, 20 percent at
                                    26

-------
primary metals facilities,  15  percent  at plants  in  the tire and rubber
                                                                         14 5
Industry, and 5 percent  at  plants  1n the other miscellaneous Industries.
In the utilities  industry,  it  was  reported  that  chromium-based  water
                                                           *f G
treatment chemicals are  used at  two electric  power  plants.    When
combined with data from  plant  responses  to  EPA Information  requests  in
each of these Industries, these  estimates result in a  total of  about
2,855 IPCT's using chromium-based  water  treatment chemicals: 476  at
petroleum refineries, 2,039 at chemical  plants,  224 at primary  metals
plants, 110 at miscellaneous plants, and 6  at utilities.  The nationwide
baseline Cr*6 emissions  from these towers are estimated to  be 85 megagrams
per year (Mg/yr)  (94 tons per  year [tons/yr]).1*5
      3.2.1.2  Comfort Cooling Towers.   Comfort  cooling towers  are used 1n
all States in the U.S.,  primarily  1n urban  areas.   Major users  of  CCT's
with HVAC systems Include hospitals, hotels,  educational facilities,
office buildings, and shopping malls.  Refrigeration systems that  may
operate with CCT's Include  Ice skating rinks,  cold  storage  (food)  ware-
houses, and other commercial operations.  The  EPA estimates that the
nationwide population of CCT's is  250,000 units  and that 15 percent of
CCT's (about 37,500) use chromium-based water  treatment chemicals.  These
CCT's are estimated to emit between 7.2  and 206  Mg/yr  (8 to 227  tons/yr)
of chromium.1*7  Chromium'use 1n CCT's appears  to be distributed  randomly
across the country.
      In the preparation of the proposed  rule  for CCT's under the Toxic
Substances Control Act (TSCA)  (see 52 FR  10206),  EPA developed model tower
parameters and estimates of chromium emissions per model tower to
represent the population of CCT's  in the  U.S.  Table 10 presents the model
parameters and baseline  (I.e., low efficiency drift eliminator [LEDE])
emission estimates.**
      The emission estimates in Table 10  are based on an emission factor
developed from EPA- and Industry-sponsored cooling tower emission tests..
Because the emission factors developed to estimate Cr+s emissions from
cooling towers are Independent of tower operating parameters (recirculation
rate, chroraate concentration, cooling range), the factors are applicable
to both CCT's and IPCT's.  Section 3.2.3.1 of this document discusses
specific emission factors to use for estimating Cr+fi emissions from
cooling towers on a case-by-case basts.   [Note:  The proposed TSCA rule

                                    27

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                       TAILE 10.  MODEL COMFORT COOLINS TOWERS  AMD  HOURLY BASELINE Cr*6 EMISSIONS
ro
Q3
Model
tower
1
2
3
4
5
6
Model
building
fiie^
" (ft*)
673
(7,240)
1.460
(15,720)
3,405
(36.650)
6.224
(66,990)
12,338
(132,800)
37,626
(405,000)
•
Flow
Model tower i Reclrcu-
coollng requirements latlon
W (Btu/h)
95,400
(325,800)
207,100
(707,400)
482.900
(1,649,000)
882,900
(3,015,000)
1,750,000
(5,976,000)
5,338,000 1
(18,230,000)
Tons rate
27 246
(65)
59 534
(141)
137 1,250
(330)
251 2,280
,(602)
498 4,520
(1,194)
,520 13,800
(3,642)
rates, t/nrin
(qal/mln)
E vapor a- Slowdown
tlon rate rate
2,08
(0.55)
4.54
(1.20)
10.6
(2.80)
19.4
(5.12)
38.4
(10.15)
117.0
(30.96)
0.53
(0.14)
1.14
(0,30)
2.65
(0.70)
4.85
(1.28)
9.61
(2.54)
29.3
(7.74)
Chromium
emissions
per tower,
mg/h (lb/1,000 h)
19.9
(0.044)
43.2
(0.095)
101
(0.222)
18-1
(0.406)
365
(0,804)
1,110
(2.45)
        Assumptions:
        Wet bulb temperature = 23.9°C (75°F)
        Hot water temperature » 29.4°C (85*F)   ;
        Cooling range = 5.6"C (10°F)
        Cooling requirements = 142 W/ra  floorspace (45 Btu/ft /h)
        Cycles of concentration = 5
        Latent heat/total heat = 0.8
        Chromate concentration = 10 ppin
        Chromium emission factor = 0.0003 mg Crl /(ppm Cr* )(Hter H20)
                                               (2.504x10"  Ib Cr* /ppm Cr* /gal  H20)

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 would  prohibit the  use  of  chrotnfurn-based  chemicals  in CCT's.   If
 promulgated,  this rule  would  have  the  effect  of  reducing  Cr*   emissions
 from CCT's  to zero.]
       3.2.1.3  Cooling  Tower  Fundamentals.  Schematics of typical  cooling
 tower  designs are shown in Figure  2.*8  The major cooling tower components
 include the fan(s), fill material, water  distribution deck or  header,
 drift  eliminator, structural  frame, and cold  water  basin.  Other
 components  that affect  tower  operation include the  pumps  and pipes
 necessary to  circulate  the cooling water  through the  cooling tower and
 heat exchanger loops.
       Most  IPCT's are designed with induced-draft airflow, but many have
 forced-draft  airflow, and  some (especially 1n the utilities industry) have
 natural-draft airflow.   Induced draft  1s  provided by  a propeller-type
 axial  fan located 1n the stack at the top of  the tower.   Forced-draft
 towers  are  usually  smaller than induced-draft towers  and  have either
 centrifugal fans located at the base of the tower,  which  1s constructed as
 a plenum to provide positive-pressure airflow through  the  fill material,
 or axial fans located on the  side of the  tower.  Natural-draft airflow
 relies  on air currents created by temperature differences  between  the air
 in the  tower  and the atmosphere.   When the cooling  demands are minimal and
 the  air  temperature is low enough, water  can  be  circulated through  the
 tower and cooled sufficiently without using the  fans.   In  these instances,
 a natural draft is created in the cooling tower.
      The direction of the airflow through a mechanical draft tower is
 either crossflow or counterflow.   Crossflo / refers to horizontal airflow
 through  the fill, and counterflow refers to upward vertical airflow.  Fill
 material 1s used to maintain an even distribution of water across the
 horizontal plane of the tower and to create as much water surface as
 practical to enhance evaporation  and sensible heat transfer.
 3.2.2  Potential Emission Reduction Techniques
      Techniques to control chromium emissions from cooling towers involve
two different strategies:  modification of chromium addition  to the
redrculating water, and Improved  reduction  of drift.   The first techniqua
 involves reducing the concentration of  chromium 1n the water  treatment
program, thereby reducing the  concentration  of chromium in the  drift
                                    29

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               WATER
               INLET
                              FAN

                               WATER
                               NLET
                             DRIFT
                        'ELIMINATORS
              WATER  OUTLET
                    MECHANICAL  DRAFT
                    CROSS-FLOW  TOWER
                           AIR
                         OUTLET

                        t      t
               «««««««j—	DRIFT

                            ELIMINATORS
                                       FAN
                                  WATER
Figure 2.
WATER  OUTLET

       MECHANICAL  DRAFT
       COUNTER-FLOW  TOWER
Internals of crossflow and counterflow cooling towers
    (reprinted from Reference  No. 48).
                             30

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 emitted.  The second  technique  involves  retrofitting  towers that normally
 have  LEDE's with high-efficiency  drift eliminators  (HEDE's) to reduce
 drift emissions to the  lowest possible rate.
      3.2.2.1  Alternative Water  Treatment  Programs.   Responses to 28 EPA
 information requests  and a survey of the Chemical Manufacturers Associa-
 tion  indicate that the  average  chromate  concentration for  those IPCT's
 using chromium-based  corrosion  inhibitors is 13 ppm." »*    One potential
 chromium emission reduction technique involves alternative water treatment
 programs such as programs with  lower chromate levels  or nonchromate
 treatments.
      A low-chromate  treatment  program would reduce Cr*6 emissions from
 IPCT's by limiting the  chromate concentration in cooling water.   Water
 treatment programs are  available  that maintain average chromate concentra-
 tions of 0.5 to 4 ppra in the recirculating water, but these programs  have
 not always been successful in industrial applications.  Low-chromate
 programs that have provided acceptable results in a number of  cases
 maintain chromate concentrations  In the  range of 4 to 6 ppm.
    ,  Because of National Pollution Discharge Elimination  System (NPDES)
 chromium restrictions and other regulations, honchromium treatments are
 now more widely used than chromium treatments.  The most common
 nonchromium treatment program is phosphate based, but others include
 molybdates, zinc, and all-organic treatments (primarily organo-phosphorus
 compounds).  However, these alternative  programs may  not perform corrosion
 inhibition functions as well  or as cheaply as chromates depending  on  the
 individual cooling tower system.  The performance of  any treatment  program
 is dependent on water quality parameters (pH, alkalinity,  hardness, and
 conductivity)  and operating conditions (water temperature,  flow  velocity,
 Inhibitor concentration, and  the presence of contaminants  such as H2S,
 S02, NH3,  and  N02)  that are specific to each cooling system.
      3.2.2.2   Low- and High-Efficiency Drift Eliminators.   Water droplets
 entrained in the air and the  dissolved and suspended solids contained  in
 the droplets that are emitted from cooling towers are referred to as
drift.  Drift  eliminators can be installed at the exit of the fill
sections to reduce  the amount of drift in the exiting airflow.
Historically,  the purpose of  drift reduction has  been to alleviate the
                                    31

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nuisance deposition of water drift and Its dissolved solids on  nearby
buildings or on personal property such as automobiles.  More recently, the
concern his focused on the environmental Impact caused by the compounds
contained 1n the drift and, thus, on the deposition of these compounds.
Drift eliminators are designed with pressure drops lower than those of
other air pollution control equipment and rely primarily upon the
Impact1on of water droplets on drift eliminator surfaces to reduce the
concentration of drift from the exit air of cooling towers.  The drift
eliminator blades are configured to force directional changes 1n the
airflow such that the momentum of the water droplets causes them to
Impinge onto the blade surfaces.  The number of directional airflow
changes, the spacing between the blade surfaces, the angle of directional
change, and the capability to return the collected water to a quiescent
area of the plenum are the major design features (parameters) 1n drift
eliminators that affect efficiency.  Drift eliminators are constructed of
wood, PVC, metal, asbestos-cement, polystyrene, or cellulose.  The
material most often specified 1s PVC.
                                                          *
      Figure 3 presents schematics of the three major drift eliminator
designs:  herrlngbont (blade-type), waveform, and cellular (or honey-
comb).  Low-efficiency drift eliminators Include herringbone, some
waveform (sinusoidal), and some cellular designs.  Herringbone designs are
constructed^to create two or_three major d1rect1ona]_changesj[n the	
airflow.  The hladef art sloped 1n opposing directions 1n a manner that
provides drainage of the accumulated drift Into the fill area.  The blades
typically are constructed of wood, but other materials (e.g., metal and
asbestos cement board) also are used.  Waveform drift eliminators art
configured 1n a sinusoidal wave pattern such that two major directional
changes 1n the airflow are created.  The sinusoidal blades are constructed
of asbestos cement board or PVC material*  Cellular drift eliminators are
configured with thinner blades 1n a honeycomb pattern.   The airflow
passages 1n the cellular drift eliminators,  which are narrower than
passages in other designs, reduce the distance a droplet must travel
across the stream to Impact on the surface.   Drainage of the collected
water to prevent reentralnment 1s not a design criteria of LEOE's.
                                    32

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                                       .wood
                                       Blooms
                      \'\\
                           HERRINGBONE
                          (BLADE-TYPE)
                          ELIMINATOR
                          WAVEFORM
                          ELIMINATOR
                          CELLULAR
                          ELIMINATOR
Figure 3.   Designs of various drift eliminators (reprinted
                 from Reference No. 50).
                             33

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       High-efficiency  drift  eliminators  Include a few of both  cellular and
 sinusoidal designs.  The cellular  HEDE's that  achieve the higher
 efficiencies  are  designed with complex configurations that contain
 numerous, closely constructed airflow passages.  Thin materials  of
 construction  are  used  to reduce the area of  blockage to  the airflow and
 minimize the  pressure  drop that is created by  the eliminator.  For
 sinusoidal drift  eliminators, the  blades are placed  closer together in
 high-efficiency designs  than 1n low-efficiency designs,  and the  exit 1s
 configured with a tip  for draining captured  water that would otherwise be
 partially reentrained  in the airflow.  Typically,  drainage of  water Into  a
 quiescent area of the  tower  1s a major design  consideration of HEDE's.  A
 few drift eliminators  installed 1n towers built 1n recent years  are more
 likely to be  higher efficiency waveform  or cellular  units,  but the vast
 majority of older touers still have lower efficiency herringbone and
 waveform eliminators.
      The performance  of a drift eliminator  is  affected  primarily  by the
 droplet or particle size and the airflow velocities  through  the  drift
 eliminator.   Small droplets  are created both from  evaporation  of. larger
 droplets and  the  physical  breakage of larger droplets  Into  small
 droplets.  Parameters  that affect the rate of evaporation  and  the  size  of
 droplets created  Include  the water distribution system,  the  type of  fill,
 the type of tower,^-the meteorological  conditions,  and the^temperatLire__of

      A drift eliminator  manufacturer Indicates that HEDE's  can remove
 80 to 90 percent or more of the drift discharged from low-efficiency
 herringbone drift eliminators.50'51  These drift eliminator efficiencies,
 however, are based on data collected  with a test method that has not been
 submitted to EPA for approval.
 3.2.3  Cooling. Tower Emissions
      Three series of emission  tests  were conducted by EPA on IPCT's
 equipped with low- and  high-efficiency  drift  eliminators.  The  results of
these tests  are presented 1n  the  next  section.
                                    34

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      3.2.3,1  Drift and Chromium  Emissions.   Thi  drift  rate (rate  of
water lost by entrairanent  in  the cooling  air  drawn through  the  tower)  is
often expressed as the percentage  of  the  recirculating water flow rate
that 1s emitted.  Likewise, the chromium  emission  rate can  be expressed as
a percentage of the recirculating  chromium  rate.   However,  the  chromium
emission rate from towers  should not  be confused with the drift rate.
Based on test results, a drift eliminator manufacturer claims that  the
achievable drift rates range  from  0.001 to  0,06 percent  of  the
recirculating water.  The  approximate dividing line between drift rites
for higher and lower efficiency drift eliminators  1s 0.008  percent.  Those
achieving a lower percentage  are "higher  efficiency," and those that
cannot achieve 0.008 percent  are "lower efficiency."
      Drift can be estimated  by measuring the  emission rate of  an element
(such as sodium, calcium,  manganese,  chromium, lithium or bromine)  and
assuming that the percentage  of water emitted  as drift is the same  as  the
percentage of the recirculating element emitted.   However,  a claimed drift
rate may or may not be equivalent  to  the  element's  emission rate depending
on the way the drift rate was measured.   Also, drift rate measurement
results are highly dependent  on the measurement method;  therefore,
achievable drift rate claims may not  be comparable  if they  are  based on
different measurement methods.
      The EPA-sponsored emission tests of IPCT's at  three facilities used
an 1sok1net1c test method for chromium which is still under development.
Emission factors relating the chromium emission rate to  the chromium
recirculation rate were developed from each of these emission tests.   The
average baseline (LEDE) and controlled (HEDE) emission factors  for each
test site are presented in Table 11.  In addition, five  industry-sponsored
drift performance tests conducted by Midwest Research Institute  and two
chromium emission tests conducted by Mobil are included.  The emission
factors express the emission rate as a percentage of the recirculating
rate (milligrams of chromium emitted per milligram of chromium
recirculating 1n the tower multipled by 100).  Tht most comprehensive
emission tests were conducted at Plant B.   At this plant, two towers of
similar design located  side-by-side were tested simultaneously under the
same meteorological  conditions.   One tower was equipped with an  LEDE and
the other was equipped  with an HEDE.

                                    35

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         TABLE 11.  EMISSION FACTORS FOR HEXAVALENT CHROMIUM  FROM
                           COOLING TOWERS33-5'
Test site
Chromium emission
factor, percent3
Standard deviation
(percent relative
standard deviation,
percent)
EPA-sponsored tests
A (HEDE)
C (HEDE)
B (HEDE)
B (LEDE)
A (LEDE)
Industry-sponsored tests
MRI No. 3 (HEDE)
MRI No. 4 (HEDE)
Mob11-PTR Tower No. 5
(LEDE)
Mob 11 -North Tower No. 6
(LEDE)
MRI No. 1 (LEDE)
MRI No. 2 (LEDE)
MRI No. 5/6 minerals
test (LEDE)
0.0037
0.028 w/outl1ers
0.0038
0.0087
0.0267
0.0318
0.141 w/outT1ers
0.01
0.007
0.0334
0.0321
0.0305
0.034
0.018
0.021 w/ou tilers
0.0020 (54)
0.035 w/outl1ers
0.0044 (116)
0.0037 (43)
0.0168 (63)
0.0292 (92)
0.192 w/outl1ers
NA (-.)
NA (-)
0.0306 (92)
0.0156^(49)"
NA <--)
NA (-)
0.0045 (25)
0.0094 w/outllers
(126)



(136)






(45)
Percentage of redrculatfng chromium that Is emitted.
                                   36

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       Since the completion of the emission  tests  at  Plant  B,  additional
methods  development  Investigations have  been conducted.  These
Investigations have  revealed that the chromium  sampling method  1s  subject
to  substantial error due to potentially  severe  problems associated with
chromium recovery and cross-over contamination  from  sample run  to  sample
run.   The extent to  which these problems appear in the test results
obtained at Plants A, C, and Mobil is uncertain.  As a result,  the data   .
presented 1n Table 11 should be used with caution.
       The EPA believes that the tests at Plant  B  provide the  best
available data on the relative performance  of HEDE's.  The EPA  Method  13-
type testing at Plant B Indicated a Cr+6 emission factor .of 0.03 percent
of  the reclrculatlng Cr+a for LEDE's and 0.0087 percent for HEDE's. As
discussed in Section 3.2.1.2, these factors can be used for both IPCT's
and CCT's.
       The current factors are based on the  assumption that the  ratio of
hexavalent to total  chromium 1n the emissions is  the same  as  that  in the
cooling  water.  The  test program conducted  by the Agency has  not
conclusively Identified the spedatlon of emissions  (I.e., Cr"*"6 versus
Cr+3).   For purposes of estimating Cr+6 emissions, the conservative
assumption is that all  of the chromium 1s Cr+s.
       3.2.3.2  Sample Calculation of Chromium Emissions.  The chromium
emission rate for any tower can be estimated by multiplying the emission
factor by the reclrculatlng rate of water and the chromium concentration
1n the reclrculatlng water as shown in Equation (1).
                              ECr = K-R-CCr                           (1)
where:
      E(-r = chromium emission rate,  mg Cr/min
        K = chromium emission factor,  percent of reclrculatlng chromium
            that  1s emitted
        R = reclrculatlng ra;e of cooling water, llters/min
      ^Cr a concentration of  chromium  in  the reclrculatlng  water,  mg
            Cr/liter »  ppm (multiply CrOi, concentration  by  0.448 to obtain
            Cr concentration)
For example,  the  following  calculation estimates the  emissions from a
10,000-gallon-per-minute  (gal/min)  IPCT with a  recirculatlng  chromate
                                    37

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concentration of  10  parts per million  (ppm),  equipped  with  a low-
efficiency drift  eliminator.
         R =  (10,000  ga1/m1n)(3.785  liters/gallon)  = 37,850  liters/minute
       CQ,. «  10  ppm as  CrOu  =4.48 ppm  Cr
         K «  the emission factor for  towers  with  low-efficiency drift
             eliminators; use K = 0.03  percent.
       ECr =  K»R-CCp  =  (0.0356)(37.850)(4.48) = (0.0003)(37,850)(4.48)  =
             50.9  mg  Cr emitted/m1n
To estimate  the emissions from the same IPCT  equipped  with  a high-
efficiency drift  eliminator, use K = 0.0087.
Therefore:

ECr =  K»R-CCr - (0.0087«)(37,850)(4.48) » (0.000087)(37,850)(4.48) -
                          14.8 mg Cr em1tted/min
Thus,  the emission reduction achieved  by a  HEDE  compared  to a LEDE is:

                        50-g"^g'8xlOO = 71  percent.

       The following  example calculation estimates  the emissions from  a
500-gal/min  CCT with a reclrculating chromate concentration of  10 ppm,
equipped with a low-efficiency drift eliminator.
   ~'  R~=~(50
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Together, these Industries represent 98.2 percent of nationwide chromium
emissions from IPCT's."5  Tab1<
chromium emissions from CCT's.
emissions from IPCT's.    Table 12 also presents nationwide estimates of
                                   39

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TABLE 12.  NATIONWIDE COOLING TOWER CHROMIUM EMISSIONS
Industry
Chemical manufacturing
Petroleum refining
Primary metals
Tobacco products
T1re and rubber
Textile finishing
Glass manufacturing
Utilities
Subtotal (IPCT only)
Comfort cooling towers
TOTAL
Total No.
of cooling
towers
5,096
680
1.118
336
267
1,018
58
775
9,348 .
250,000
259,350
No. of
cooling towers
using chromate
2,039
476
224
16
40
51
3
6
2,855
37,500
40,360
Cr+6 emissions3
Mg/yr
43.13
31.82
8.39
0.23
0.18
0.08
0.01
0.95
84.8
33
118
Tons/yr
47.54
35.08
9.25
0.26
0.20
0.09
0.01
1.05
93.5
34
128
    on use  o£ low-efficiency  drift  eliminators.
                                 40

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                        4.0  SOURCE TEST PROCEDURES

 4.1   CHROMIUM  ELECTROPLATING
       During the  standards  support  study for  hexavalent chromium emissions
 from hard  and  decorative chromium electroplating  facilities,  samples  to be
 analyzed for hexavalent and total chromium were obtained  1n accordance
 with EPA Method 5 (40 CFR Part 60-Append1x A), also referred  to  as
 Modified Method 13-B 1n test reports.  The only modification  to  the sample
 collection method was the elimination of the  filter and the replacement of
 H20  in the Impingers with 0.1 Normal sodium hydroxide.  Method 5 provides
 detailed procedures and equipment criteria and other considerations
 necessary  to obtain accurate and representative emission  samples.  In
 order to sample for chromium emissions, Methoas 1 through 4 must also be
 used.
       After collection, the samples were analyzed for hexavalent and  total
 chromium (total chromium 1s the sum of hexavalent chromium plus  other
 chromium).  Concentrations of hexavalent chromium were determined using
 spectrophotometric analysis while total chromium was determined  using
 inductively coupled argon plasmography (ICAP).  At the present time,
 sample analysis has been performed In accordance with the tentative method
 "Detection  of  Hexavalent Chromium from Stationary Sources (December 13,
 1984)," and a  draft method:  "E.P.A. Protocol for Emission Sampling for
 Both  Hexavalent and Total  Chromium (February 22, 1985)."
 4.2   COOLING TOWERS
       During the standards support study for chromium emissions  from
 cooling towers, testing was conducted according to two draft test methods
 developed from previously  conducted methods development testing:
 "Method 	—Determination of Chromium Emissions from Cooling Towers"  and
 "Method 	—Direct Measurement of Gas Velocity and Volumetric Flowrate
 Under  Cyclonic Flow Conditions  (Propeller Anemometer)."   The cooling   tower
method  1s similar to EPA Method  13 (40 CFR Part 60-Appendix A) with the
following exceptions:   (1)  a Teflon™ filter 1s used in place of a paper
filter, (2) a propeller anemometer 1s used in place of the pltot  tube  for
gas velocity and flowrate  measurements,  (3)  the determination  of  the
measurement site does  not  follow EPA Method  1, and (4)  the chemical
                                    41

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 analysis  for total  chromium  in  the  emission  samples is  performed  using
 Neutron Activation  Analysis  (NAA),  Graphite  Furnace Atomic Absorption
 (GFAA), or  ICAP.   In conjunction with  the  emissions testing,  repre-
 sentative cooling tower  water samples  were collected to determine the
 ratio  of  hexavalent to total chromium  in the cooling water; these samples
 were analyzed  for total  chromium by NAA, GFAA,  or  ICAP  and for  hexavalent
 chromium  by the diphenylcarbazlde colorimetrlc  method (1n  "EPA  Draft
 Method-Determination of  Hexavalent  Chromium  Emissions from Stationary
 Sources," December  13, 1984).   The  ratio was used  to calculate  the amount
 of  hexavalent  chromium 1n the cooling  tower  emissions.
       Preliminary material balance  calculations were performed  on the
 cooling water  at several towers to  compare the  apparent chromium  loss in
 the drift emissions with the emission  measurements  obtained during the
 standards support study.  Variables used in  these  calculations  Included:
 cooling water  flow  rates to the towers, riser cells,  and/or fan cells;
 blowdown  rates; makeup water flow rates; addition(s)  of chemicals to  the
 cooling water; and  chemical analysis of the  cooling  water  samples taken
 during  testing.
      Two major modifications were made to the  draft  test method  for
 cooling towers based on problems encountered and knowledge gained during
 the testing program.  Initially, the draft method specified the use of NAA
 to determine the^total chromium content of theJmptnger^train samples and
 the cooling water samples.  Because of the length of time required for
 sample  analysis and the limited availability of commercial  NAA services,
 two additional analytical techniques,  GFAA and  ICAP, were utilized and
were added as options to the draft  test method.   Unlike NAA, both of these
techniques require acid solubilization of the chromium  in the sample prior
to analysis.  In assessing the  chromium recovery efficiency for the
concentrated 1mp1nger samples from  the first  test,  1t was discovered that
a significant residue remained  1n the  beakers used  to concentrate the
samples.  The concentration  procedure  was modified  to require  an add
rinse of the beakers used for sample concentration  with  the rinse being
added to the concentrated sample.
                                    42

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                              5.0  REFERENCES
 1.  Memo from Hester, C., MRI, to Smith, A., EPA/ISB.  Bases for Risk
     Assessment Inputs for Chromium Electroplating Operations.  June
     1988.  pp. 6-7, 10.
 2.  Memo from Hester, C., MRI, to Smith, A., EPA/ISB.  Bases for Risk
     Assessment Inputs for Chromic Acid Anodizing Operations.  June
     1988.  pp. 8-9.
 3.  Logozzo, A., and Schuwartz, M.  Hard Chromium Plating.  American
     Electroplaters Society,  Inc.  p. 9.
 4.  Vervaert, A.  Preliminary Assessment of Chromium from Chromium
     Electroplating Facilities.  Research Triangle Park, North Carolina.
     U. S. Environmental Protection Agency,  p. 3.
 5.  Decorative Chromium Electroplating.  American Electroplaters
     Society.  1980.  p. 2.
 6.  Dennis, J., and Such, T.  Nickel and Chromium Plating, Butter-worth
     and Company.  University Press.  Cambridge, England, Second
     Edition.  1986.  p. 179.
 7.  Reference 4, p. 2.
 8. .Reference 6, p. 287.
 9.  Reference 6, p. 289.
10.  Reference 6, p. 290,
11.  Reference 6t pp. 272, 294-295.
12.  Locating and Estimating Air Emissions From Sources of Chromium.
     U. S. Environmental Protection Agency, Research Triangle Park,  North
     Carolina.  EPA Publication No.  450/4-84-007g.  July 1984.  p.  83.
13.  Graham, K.  Electroplating Engineering Handbook.  Reinhold Book
     Corp.,  New York.  1962.   p.  427.
14.  Reference 13, p. 432.
15.  Reference 13, p. 432.
16.  Reference 13, pp.  162, 427.
17.  Brace,  A.  The Technology of Anodizing Aluminum.  Robert Draper,
     Ltd.  Teddington,  1968.   p.  54.
18.  Darrln, M.,  and Tubbs, L.  "Dyeing  Chromic Acid Anodized Aluminum."
     Metal Finishing.  September  1984.   p.  550.
                                    43

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 19.   Schwartz,  M.   Anodized Aluminum and Its Alloys,   American
      Electro?laters Society.  1985.   p.  15.

 20.   Wernick, S.t  and Pinner,  R.   "Surface Treatment  and Finishing of
      Light Metals."  Metal  Finishing.  June  195S.   p.  92.

 21.   Reference  13, p. 429.

 22.   Reference  13, p. 429.

 23.   Briml, M., and Luck,  J.  Electrof1n1shing.  American Elsevler
      Publishing Company.   New  York.   1981.  p.  77.

 24.   Reference  13, p. 430.

 25.   Snyder, 0.  "THvalent Chromium Plating:  The  Second  Decade."
      Product Finishing.  March 1988.  p. 57.

 26.   Reference  2§, pp.  59-60.

 27.   Reference  25, p. 63.

 28.   Referance  25.  p,  65.

 29.   Trfvilint  Chromium Cost Enclosure:   Harshaw/Flltrol  Partnership.
      Prepared for  U.  S. Environmental Protection Agency,  Research Triangle
      Park, North Carolina,  by  Dennis Haserlk, Manager  of Technical
      Services.   June 22, 1987. p. 3.

 30.   Tomaszewski,  T., and  Fischer, R.  "Trivalent Chromium:   A
      Commercially  Viable Alternative."  Occidental  Chemical  Crop.  p. 5.

-31.   Reference^, p, 5=6. — - -   			"      		•

 32.   Chromium Eleetraplaters Test Report;  Greensboro  Industrial  Platers,
      Greensboro, North Carolina.   Entropy Environmentalists,  Inc.,
      Research Triangle Park, North Carolina. Prepared for U.  S.
      Environmental Protection  Agency, Research Triangle  Park,  Korth
      Carolina.   EMB Report  86-CEP-l.   March  1986.

 33,   Chromium Electroplaters Test Report:  Consolidated  Engravers
      Corporation,  Charlotte, North Carolina. Peer  Consultants,  Inc.,
      Rockvllle, Maryland.   Prepared  for  U. S. Environmental  Protection
      Agency, Research Triangle Park,  North Carolina.   EMB
      Report S7-CEP-9. May  1987.

 34.   Chromium Electroplaters Test Report:  Roll  Technology,  Greenville,
      South Carolina.  Peer  Consultants,  Inc., Dayton,  Ohio.   Prepared for
      U. S. Environmental Protection  Agency,  Research Triangle  Park, North
      Carolina.   EMB Report  87-CEP-6.   September  1987.
                                     44

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35.  Chromium Electroplaters Test Report:  Able Machine Company, Taylors,
     South Carolina.  PEI Associates,  Inc., Cincinnati, Ohio.  Prepared
     for U. S. Environmental Protection Agency, Research Triangle Park,
     North Carolina.  EMB Report 86-CEP-3.  June 1986.

36.  Chromium Electroplaters Test Report:  Roll Technology Corporation,
     Greenville, South Carolina.  Peer Consultants, Dayton, Ohio.
     Prepared for U. S. Environmental Protection Agency, Research Triangle
     Park. North Carolina.  EMB Report 88-CEP-13.  August 1988.

37.  Chromium Electroplaters Test Report:  Precision Machine and
     Hydraulic, Inc., Worthington, West Virginia.  Peer Consultants,
     Dayton, Ohio.  Prepared for U. S. Environmental Protection Agency,
     Research Triangle Park, North Carolina.  EMB Report S8-CEP-14.
     September 1988.

38.  Chromium Electroplaters Test Report:  Hard Chrome Specialists, York,
     Pennsylvania.  Peer Consultants, Dayton, Ohio.  Prepared for U. S.
     Environmental Protection Agency, Research Triangle Park, North
     Carolina.  EMB Report-89-CEP-15.  January 1989.

39.  Emission Test Report:  Norfolk Naval Shipyard, Norfolk, Virginia.
     Naval Energy and Environmental Support Activity, Port Hueneme,
     California.  Source Emission Testing of the Building 195 Plating Shop
     at Norfolk Naval Shipyard, Portsmouth, Virginia.  March 11-18,
     1985.  NEESA 2-124.  May 1985.

40.  Chromium Electroplaters Test Report:  Piedmont Industrial Platers,
     Statesvllle, North Carolina.  Entropy Environmentalists, Inc.,
     Research Triangle Park, North Carolina.  Prepared for U. S.
     Environmental Protection Agency, Research Triangle Park, North
     Carolina.  EMB Report 86-CEP-04.  September 1986.

41.  Chromium Electroplaters Test Report:  Steel Heddle, Inc., Greenville,
     South Carolina.  PEI Associates, Inc., Cincinnati, Ohio.  Prepared
     for U. S. Environmental Protection Agency, Research Triangle Park,
     North Carolina.  EMB Report 86-CEP-2.  June 1986.

42.  Chromium Electroplaters Test Report:  GMC Delco Products Division,
     Livonia, Michigan.   Peer Consultants, Inc.   Rockville,  Maryland.
     Prepared for U. S.  Environmental Protection Agency, Research Triangle
     Park, North Carolina.  EMB Report 87-CEP-7.  May 1987.

43.  Draft Chromium Electroplaters Test Report:   A Plant in  the Midwest.
     Prepared for U. S.  Environmental Protection Agency, Research Triangle
     Park, North Carolina.  April  1988.

44.  Memo from Barker,  R., MRI,  to Vervaert,  A., EPA/ISB.   Engineering
     Analysis - Reliable Plating and Polishing Company.   May 1987.
     pp. 5-7.
                                    45

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45.  Chromium Emissions from Industrial Process Cooling Towers-Background
     Information  for Proposed Standards.  Draft.  Prepared for U. S.
     Environmental Protection Agency.  Research Triangle Park, North
     Carolina.  May 1988.

46.  Telecon.  P. Bell in, MRI, with C. Bergesen, Utility Data Institute
     (UOI).  March 5,  1986.  UDI study on chromate use in electric
     utilities industry.

47.  Chromium Emissions from Comfort Cooling Towers-Background Information
     for Proposed Standards.  Prepared for U. S. Environmental Protection
     Agency.  Research Triangle Park, North Carolina.  March 1988.
     EPA-450/3-87-010a.

48.  Holmberg, J. 0., and 0. L. Kinney.  Drift Technology for Cooling
     Towers.  The Marley Company, Mission, Kansas.  1973.

49.  Letter and attachments.  Mayer, A., Chemical Manufacturers
     Association, to Cuffe, S., EPA:ISB.  September 27, 1986.  Summary of
     CMA member survey on corrosion inhibitors used in process cooling
     towers Including average ppm in recirculating water.

50.  Telecon:  C. Clark, MRI, with J. Holmberg, Marley Cooling Tower
     Company.  April 2, 1985.  Drift eliminator efficiency.

51.  Telecon:  P. BelUn, MRI, with J. Holmberg, Marley'Cooling Tower
     Company.  .July 19, 1985.  Drift eliminator efficiency.

52.  Kelly, G. M.  A System Efficient Approach to Cooling Tower Energy
     Modifications.  Cooling Tower Institute Technical Paper.
     No. TP-85-18.  New Orleans, Louisiana.  January 1985.

53.  Emission Test Report: "National Bureau of Standards, Galthersburg,  --
     Maryland.  EM3 Report S5-CCT-4.  October 1985.

54.  Emission Test Report:  Exxon Company Petroleum Refinery, Baytown,
     Texas.  EMB Report 85-CCT-3,  November 1986.

55.  Emission Test Report:  Southeastern Manufacturing Facility.   EMB
     Report 87-CCT-5.   Draft.   September 1987.

56.  Abstracts of six  confidential  emission test reports  conducted by MRI
     for Industrial  clients.

57.  Letter and attachments.  Hawes, R.,  Mobil 011  Corp.,  to  Randall, D.,
     MRI.   August 24,  1987.   Emission test results.
                                    46

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                                            TECHNICAL REPORT DATA
1 W^-2-89-002 I2'

4. TITLE AND SUBTITLE
Locating And Estimating Air Emissions From Sources
of Chromium (Supplement)
7. AUFHOR(S)
Jeff Shular. Robin Barker, Bruce Nicholson,
David Randall
9. PERFORMING ORGANIZATION NAME AND ADDRESS
Midwest Research Institute
401 Harrison Oaks Boulevard
Cary, North Carolina 27513
12. SPONSORING AGENCY NAME AND ADDRESS
U. S. Environmental Protection Agency
OAR, OAQPS, AQMD, PCS (MD-15)
Research Triangle Park, North Carolina 27711
13. SUPPLEMENTARY NOTES
EPA Project Officer: Dallas W. Safriet
S. REPORT DATE
AuqUSt 1989
6. PERFORMING ORGANIZATION COOE
S. PERFORMING ORGANIZATION REPORT NO.
10. PROGRAM ELEMENT NO.
11. CONTRACT/CHANT NO,
68-02-4395
13. TYPE OF REPORT AND PERIOD COVERED
Fi na 1
14. SPONSORING AGENCY CODE

IS. ABSTRACT
To assist groups Inventorying air emissions of potentially toxic substances, EPA
is preparing a series of documents that compiles available Information on sources
and emissions of toxic substances. This document deals specifically with methods to
estimate chromium (Cr+6) emissions from cooling towers and electroplating operations.
17. KEY WORDS AND DOCUMENT ANALYSIS
1. DESCRIPTORS
Chromium (Cr+6)
Estimating Air Emissions
Air Toxic
Cooling Towers
Electroplating
18. OISTRIBUTION STATEMENT
Unlimited
b. IDENTIFIERS/OPEN ENDED TERMS

19, SECURITY CLASS (Tttit Rtporti
Unclassified
20. SECURITY CLASS (Thit page I
Unclassified
c. COSATl Held/Group

21. NO. OF PAGES
50
22. PRICE
EPA ton* 2330-1 (R»». 4— 77)    PREVIOUS SOI TION 1 1 OBSOLETE

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