PB83-243436
    Evaluation of  a Fathead Minnow
    "Pimephales promelas'  Embryo-Larval Test
    Guideline Using Acenaphthene and Isophorone
    (U.S.) Environmental  Research Lab.-Duluth, MN
    Jul 83


              s^
U.S. Dcȣrtmsnt of Commsrce
Flafei?.! Tocfiaica! Information Service

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                                     TECHNICAL REPORT DATA
                              (Please rsad Instructions on the reverse before completing)
1, REPORT NO.
    EPA-GOO/3-83-062	
A, TITLti AND SUBTITLE

 Eval.nation of a Fathead Minnow lllmc^h£l_es_ 1H£HLCLL;L;2. Embryo-
 Larva].  Test Guideline  Using Acenaphthent! and 'Isophorone
              S. REPORT DATE
                July 1983
              6. PERFORMING ORGANIZATION CODi
              3, RECIPIENT'S ACCESSION NO.
                            2 A 3 4 3  6
7. AUTHOB(S)
                                                              8. PERFORMING ORGANIZATION REPORT NO.
 A. E.  Lcmke, E. Durhan,  and T. Fclhabcr
9, PERFORMING ORGANIZATION NAME AND AODBESS

 U.S.  Environmental  Protection Agency
 Environmental Research  Laboratory-Dul.uth
 6201  Congdon Boulevard
 Duluth,  UN  5ri804
              10. PROGRAM ELEMENT NO.


              11. CONTRACT/GRANT NO.
12. SPONSORING AGI5NCV NAME AND ADDRESS
  Environmental  Research Laboratory
  Office of Research  and Development
  U.S.  Environmental  Protection Agency
  Duluth, MN 55804
                                                               13, TYPE OF REPORT AND PERIOD COVERED
              14. SPONSORING AGENCY CODE
                EPA/600/03:
16, SUPPLEMENTARY NOTES
10. ABSTRACT
 A set of  4  embryo-larval  bioas.says (2 each  with isophorone  and acenaphthene,
 respectively,  were conducted with the fathead  minnow, Piniephales prome.las.  The
 objective of  the study was  to evaluate a specific method  for  this type of  test.
 The no effect  levels when compared to the controls were 0.208 and 0.226 mg/1
 acenaphthene  and 19.5 and 6.89 mg/1 isophorone, respectively.   The only problem'
 encountered was in the feeding regime which may have a possibility .for improvement
 as control weights varied..
17.
                                 KEY WORDS AND DOCUMENT ANAtYSIS
                   DESCRIPTOHS
18. DISTRIBUTION STATEMENT
REI.KASK  TO PUBLIC
                                                b.lOENTIFIERS/OPEN ENDED TEHMS
                                                19. SECURITY CLASS ('fhll Report/
                                                 UNCLASSIFIED
2O. SECURITY CLASS (Thit'
 UNCLASSIF] ICO
                                                                             e. COSATI Field/Group
                            21. NO. OF PAGES
                                  29
EPA Form 3220-1 (Rev. 
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                      NOTICE

Tills document has been reviewed in accordance with
U.S. Environmental Protection Agency policy and
approved for publication.   Mention of trade names
or commercial products does not constitute endorse-
ment or recommendation for use.
                       1.1

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                                                    EPA-600/3-83-062
                                                    July 1983
Evaluation of a Fathead Minnow Piinephalcs promelas Embryo-Larval  Test

             Guideline Using Acenaphtbene and  Isophorone
        Arraond  E.  Lemke,  Elizabeth Durban,  and Taryl  Felhaber
                U.S. Environmental Protection Agency

             Environmental Research Laboratory-Duluth

                      6201 Congdon Boulevard

                     Duluth, Minnesota  55804

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     Evaluation  of a Fathead Minnow Plinophales promelas Embryo-Larval Test




                  Guideline Using Acenaphthcnie and Isophorone









                                An;1-:-: ,1  E ,  Lemke




                               Eli i-.'ibeth Durban




                                Taryl Felhaber









     Toxicity testing  in  biological  aquatic  systems  lias been used for more




than 20  years.   Various kinds  of tests have  been conducted including static,




flow-through, short-term,  long-terra, and  static  renewal tests.   Species




tested include  most  of the common  species of fish and  many species of




invertebrates.   A large bulk of  the  testing  has  been on Daphnia magna and the




fathead  minnow.   There is  a general  consensus that much of the  testing is




imprecise and perhaps  inaccurate.   Determination of  expected accuracy and




precision of such  testing  was  necessary before the use o£  such  tests could be




required by EPA.




     The testing  plan  being reported here was to provide each of several




laboratories with  two  chemicals  and  a  set of guidelines, ask them to perform




two tests with  each  chemical,  and  report  as  the  primary criteria the




no-effect level of each chemical on  the early life-history stages of the




fathead minnow.   A description of  this  criteria  is in  Appendix  .1.  Partici-




pating laboratories  were required  to provide all other necessary items for




following the guidelines,  including  water, chemical  expertise,  fish  and




testing personnel.   An absolute minimum of consultation assistance was




provided by the test set manager.   It  was decided that the guidelines must




stand by themselves  eventually and this was  best  determined  by  minimizing any




assistance Crotn the'  project chief.

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     Participants were asked to provide a detailed  description of all the




.activities.  Included in this do':ail was to be any  other  endpoints  such as 96




or 30-day LCSOs which were gathered as part of determining the no-effect




level.  Each participant was asked to also include  a  thorough  discussion  of




interpretation and/or technique problp.ni;> which were encountered during the




conduct of the four required tests.  The laboratory operator:;  were  also




encourageo to make suggestions for rectifying any of  the  problems which they




encountered.  This report describes the participation  of  the Environmental




Research Laboratory-Duluth in this interl.nboratory'comparison  test.

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 METHODS AND MATERIALS




      The water  supply was  sand  filtered Lake  Superior  water;  hardness  45-47




 mg/1 as CaCO-j,  alkalinity  40-42 tng/1 as CaC03,  pH  7,8.   Other chemical




 parameters of. the water are as  described  in Bicsinger  and  Christensen  (1972).




 All water was heated in the head  box by stainless  st'.'.c:l  immersion  coil and




 aerated vigorously  to bring all gases  into equilibrium with  the  atmosphere.




 Water was delivered  to the diluter . through a  rigid PVC pipe  and  controlled  by




 a stainless steel and anodized  aluminum liolcnoid valve.  Experimental  water




 temperatures were monitored continuously  in three  randomly assigned  chambers




 and taken twice weekly in  all chambers with a calibrated thermcmeter.




 Reported temperatures are  for the calibrated  thermometer readings.




      The diluter (DeFoe, 1975)  utilized in this work provided useful




' flexibility in  making up the required  solutions on a continuing  basis.  Toxic




 materials can be added directly by changing syringe sizes  or  by  making




 different" concentrations in solvent of the desired materials.  This  equipment




 was constructed of glass with silicons glue joints and teflon tubing.   Teflon




 has been shown  to be i-iuch  less  adsorptive than other plastics  and  does not




 contain plasticizets which may  leak out and cause  toxicity.




      Test chambers ware of glass with  a minimum of silicone  glass  and  ceramic




 glue.   Chamber size was 46 cm x 16 cm  x 18 cm containing 10  cm water with an




 8  nn frpphoarH.   W^it^r v;olum.(^ was approximately S*25 liters.   Cycle  tiiue of




 the diluter was about 420  cycles in 24 hours and during  each  cycle,  0,5




 liters  was  delivered to each chamber resulting in  a 25 fold  turnover in  eacli




 chamber per 24 hours.




 Toxic  Solutions




     Acenaptliene was dissolved in dimethylformamide (CMF)  at  the required




 amount  to add 16 .11! of  solvent-toxicant solution to each liter of  water.  At




                                       3

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 the highest concentrations some acenapthene was noted coning out of solution




 at  the injection point.   This floating material was not sampled  when the




 analysis for active ingredient was accomplished.




      Isophoronc was added directly into the dilutor mixing chambers at eac'.i




 concentration.   It  is fairly water soluble and  no residues were  noted at any




 test  concentrations.




 Test  Organisms




      Embryos of the fathead  minnow Pimephales  promelas were removed from the




 cement asbestos spawning tile by gentle rolling (Cast and Brungs,  1973).  A




 dissecting  microscope was utilized to  pick embryos  that were undergoing cell




 division.   Embryos  were  assigned in groups of  five  in a stratified random




 fashion to  the  screen bottomed glass embryo cup. The cups were  set in petri




 dishes  containing sufficient dilution  water to  keep the embryos  covered




 during the  distribution.   Transfers were made  by carefu.l  manipulation using




 an  eye  dropper  with an enlarged  opening.   Embryo numbers  varied  from 15-35




 per cup but  were equal for any single  test.  Embryo numbers were varied by




 embryo  availability and  by choice  to test  the effect  of this parameter.




      After  all  embryos were  transferred,  the incubation cups were  moved to




 the test chambers with minimum air exposure  (less than 10 seconds) and hung




 on  an  oscillating rockerarm  apparatus.   This equipment cycled  the  embryo cups




 vertically causing  gentle  movement of  the  test  water  and  maintained all test




 parameters  in close proximity to  the embryos.   The  fish in these tests were




 fed beginning the first  day  of hatching.   Tills  was  done to prevent starvation




of  the  earliest hatchllngs.   The  first  feeding  was  put directly  i.ito the




embryo  cups.  On the  fourth  day  of  exposure all  live  embryos were  released




 into  the test chambers by  unhooking  the  incubation  cups from the aeration




apparatus and then  submerging  by  tipping into the chamber.   Larvae were



                                      A

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allowed  Co  swim out of  their own volition and the  cups  were  removed. 24  hours



later.   This  procedure  minimized handling which  is  very stressful  on newly



hatched  larvae.   However, this procedure resulted  in varying numbers of



larvae  in each chamber,  as hatching success vaiied .



      Feeding  wr.s  accomplished by putting an aliquot of.  settled  brine shrimp



nauplii  Artomia sal ina  (Jungle brand) into each  flow splitter of  the diluter



assuring equal distribution to each duplicate.   Feeding was  done  at  the



beginning,  middle, and  end of an 8 hour period  5 days  per  week  with  two



feedings approximately  1 hour opart 2 days on weekends.  Sufficient  shrimp



were  added  so at  least  some were not eaten.  No  siphoning  of tanks was  done



the first week after hatching, thus preventing handling injury.and allowing



any micro organisms in  the water to grow.  After 1  week approximately 5 grams



per day of  a very  fine  trout starter was added daily to each tank  and tanks



were  siphoned every other day.  Fish were killed and individually  we'.ghed  to


  ~"\
10    grams  on the  28th  day post hatch.  All weights were recorded  and an



analysis of variance and Dunnetts test were performed  to determine difference



from  the regular  and solvent control with the acenaphthene and  with  only the



regular control in the  isophorone tests.



Ch emiea1 Analysis



      Chemical analyse,1;  for the toxicants were performed  on all  chambers



initially (1st day) and  finally (last day) for each test.  Also twice weekly



analyses w,?.re performed with duplicates alternating.  All  results  reported



were  as active ingredient analyzed.  Dissolved oxygen analysis  was performed



once  a week at each concentration with duplicates  alternating.  Hardness,



alkalinity,  and pit analysis were performed twice during  each test.

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      Analysis  for aeenaphthene was accomplished by using a Balrd AtomLc Model




 SFR  100  spectrofluorlineter.   The fluorlmeter was chosen as the instrument




 because  it  is  very sensitive to the aromatic rings of the aeenaphthcne




 molecule.   This  structure  fluorcsces readily and no concentration or cleanup




 of  the samples was needed.   Water  samples  were taken and mixed at a ratio of




 75°7  test  solution, 25%  isopropanol.  This  mixture was alloweu to equilibrate




 until all of  the  air  bubbles were  gone  (2-16 hours).  Appropriate amounts of




 this  solution  were analyzed  and the results  recorded.




      Standards were made by  adding weighed amounts of acenaplit'icnc to




 dr'.methyl  formaroi.de solvent and injecting appropriate aliquots into clean room




 temperature  lake  water.  A standard curve  was produced and used  as a




 comparison.  Spiked samples  were prepared  similarly from control water




 obtained  from  the experimental equipment.




      Operating parameters  for the  fluoriraeter:




 Excitation Wavelength:  290  nm




 Emission Wavelength;  336 nm




 Excitation Slit Width:  10 nm




 Emission Slit  Width:  20 nm




      The isophorone was analyzed by gas chromatography.   Weighed amounts of




 isophorone were added to hexane and used for standards.   The  procedure for




 analysis was as follows:  50  ..1! of  isophorone water solution  was sampled from




 the test tanks and  added to  50 ml  redistilled haxaue in  100 nil volumetric




 flasks.   Test  samples and spiked recovery  samples  were extracted by stirring




 for 1.5 hours  on  an electric  stirrer with  a  teflon stirring bar,   A 5 pi




aliquot of the hexane layer  was injected onto the  GC column by automatic




sampler.   The  mean  retention  .time was 5.4  minutes  under  the following




operating conditions:



                                      6

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Instrument:  Hewlett Packard 571DA gas ehromatograph with a KID detector




Column:  6  ft. x 2 mm ID glass column packed with H)% carbowax 20 M on 80/100




         Gas Chrom Q




Carrier ftas:  Nitrogen




Detector Temp.:  250° 0




Injr.ctor Temp.:  7.50° C




0» en Temp,:  140° C 150 thermal.




All samples were injected twice and the mean of the two  infections was




reported.  The precision of the instrument was periodically checked by




duplicate analyses.

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 RESULTS  •




 General Parameters




      Temperature of the test  chambers was  maintained between 2<'t.2°C and




 25.6°C at  all times.   No excursions  beyond these limits were noted in any of




 the  four tests.   Mean temperature  was 25.1*0.   Dissolved oxygen was always




 maintained  at plus 90% of saturation, mainly  because of the, high turnover




 rate in the test chambers.  Hardness was  always between 47-48 mg/1 as CaCOj




 and  alkalinity at 38-40 mg/1  as  CaC03,  and pH  was 7.5-7,8,




      The chemical analysis  for  acenaphthene tests 1  and 2 are found in Table




 1.   !">at a presented are analyzed  concentrations in mg/1 of material.  There




 were no large excursions from the  tesc  parameters due to equipment'.




 malfunction during the acenaphthene  tests.




      The isophorone chemical  analyses for  tests 1 and 2, respectively, are




 presented  in Table ?..   All  concentrations  are  in rag/1,  Concentration 4 in




 test  2  had  a complete  failure of the toxicant  airiition equipment during a 16




 hour  period in the middle of  the test which i.s reflected in the mean and




 standard deviation of  test  2,




 Reprodiicibi 1 i t y




     The spilt sample  precision was  98,4%  _+ l.ITi n ~ 8 for the acenaphthene,




 and  95.3% -t- 6.9% n = 8  for  the isophorone.  Spike recoveries were 99% +• 5%




 for  acenaphthcae and 99.5%  +  7.2%  for isophorone tent 1 and 106,8% t 7. IX for




 isophorone  test  1  and  2,  respectively.  All reported data on .the tests were




 adjusted for  recoveries  prior to running the statistical evaluations for the




 test data.    No data were discarded.




     The test  concentrations  all were nominally  at a 0.5 factor  from each




other with   the exception of: isophorone  test 1  in  which the difference between




the tor  two concentrations was only  0.33%.




                                      R

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Biolog i c_n 1  Re s u 11 a




     The no-effect  level  for  acenaphthmie  when compared  to the solvent




control was between  0.133  and  0.2fj3  mg/1.  for  test  1  and  between 0.146 and




0.285 mg/1  for test  2  (Steele  and  Torrie,  1960).




     The no—effect  levels  when compared against  the  normal control  were 0.133




to 0.263 mg/1 for test  1 and  between 0.593 and 1,02  mg/1 for  test  2.   In both




tests with  acenupthene  the solvent control fish  were the largest.   Also, the




two lowest  concentrations  were, larger than the normal, control  fish.   This




appears to be a usual occurrence  in  hioassay  testing.




     The no-effect  levels  for  isophorone hased on  growth were  between 15.6




and 22.7 mg/1 for test  1 and  between 4.2 «-md  8.8 mg/1 for test 2,   The total




growth of the test  fish was also higher in test  2  with  the controls  in test 1




averaging 0.141 grams and  those in test ''.  averaging  0.202 grains.




     The effect of egg  numbers was also tested as  part  of the  work.   The




final low mean weight in the  second  acenaphthene test and the  first




isophorone test was  at  first  thought  to he caused  by the larger number of




fish used as opposed to the first  acenaphthene test.   To test  this  theory a




test was conducted using 35 embryos  per hatching cup (70 per  concentration).




The test was begun so that  the larvae  began to feed  on  Tuesday allowing 4




jays of full feed before the weekend.  Th?.s(?  fish  weiru. thp heaviest  of the




four tests.

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 DISCUSSION




      No apparent difference in the testing procedures were found.  All




 procedures and practices were as similar as possible.  Water temperatures,




 flow rates,  food sources, food rearing practices, feeding rates, source of




 fi.sh and  all  similar factors were very similar if not identical.  One




 procedure not  noted in the protocol  was that  of feeding dttv.iriR the first 48




 hours  post hatch.   In test 1 the eggs  hatched on Saturday and Sunday so they




 were only fed  twice.  In test 2  they hatched  mid-week and were fed three




 times  a day during the first 2 days  of life.   The'presence of a wider




 variation in  size  in test 2  perhaps  reflects  this as the standard deviation




 was  almost double  0.026 vs.  0.017 in tests 2  and 1,  respectively.  This




 variation in  growth rate was already noted by observation after about 2 weeks




 of testing.   The guidelines  called  for at  least  one  concentration to be equal




 to the  control  in  growth of  the  test animals  and at  least one concentration




 to be  significantly lower in growth,  if growth  was  used as an end point.




 This  requirement was wet in  all  four of the reported tests.   Variation in




mean growth between tests made the use of  a control  absolutely necessary.




One  cannot compare weights of  two separate tests'but each test must  be




compared  to its  own control.




     If solvents are used, more  reproducibi1ity  is  obtained  when toxicnc




effects are compared to  solvent  controls rather  than to the  normal  controls.




The  acenaphthene tests  are nearly  identical if  iud$;erf  against the solvent




control and about  three  times different  when  iud»eu  against  the normal




control.   The extra growth usually found with usable solvents may make the




results appear less  toxic  if only comparison  to  a normal  control  is  made.




The difference noted  results  from the  anparent stimulation of growth  by the




solvent DMF which  at  low  levels  acts us  a  nutrient source for bacteria.   This




                                     10

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in turn nourished microorganisms which  the  newly  hatched  fry  used  as  food.




This throe-fold difference  is  also  found  in  the  isophorone  test.   Numbers  of




fish as noted previously are not n  factor  if  all  life  sustaining  parameters




are maintained at a high level.




     Feeding of the newly hatched  fry still,  could  be  improved.   If natural




waters are used, certain unknown factors may  interfere.   The  two  lowest




growth tests were adjacent  to  each  other  in  time.,  but  none  of  the  usual  test




parameters were different in any of the tests.




     The protocol as written in the guideline document  appears  quite  easy  to




follow and has a limited amount of  "art".  This.is  particularly  true  if  no




sorting or thinning of the hatched  fry  is done.   If any further  work  is  to be




done, it should be in the area of  feeding during  the  first  week  post  hatch




because the growth differences noted took place during  this time  span.
                                     11

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REFERENCES




Biesinger, K. K., nntl G. M, Christiansen.  1972.  Effects of various metals on




     survival, growth, reproduction and metabolism of Dnphnia magna.  J.




     Fish. Res. Hoard Can. 29:  1691-1700.




DeFoe, D. L.  1975.  Multichannel toxicant injection system for flow-through




     bioassays.  J. Fish. Res.  Board Can. 32: 544-546.




Cast, M., and W. A. Brungs.  1973.  A procedure for separating eggs cC the




     fathead minnow.  Prog. Fish-Cult. 35: 54.




Steel, R. G. D., and J. H. Torric.  1960.  Principles and procedures of




     statistics with special reference to the biological sciences.  New York:




     McGraw Hill.

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                                        Table  1




                             Aeenaphthetie  Chemical  Analysis




                             Mean  and  Standard  Deviation

Test 1
Test 2
Control
Not
Found
Not
Found
Solvent
Control
Not
Found
Not
Found

0
+ 0
0
+0
#1
.069
.009
.070
.005
Conccntrat
#2
0
+0
0
+0
.133
.004
.146
.016
ion mg/1
#3
0.263
+0.061
0.285
+0.032
Anal
0
+ 0
0
+ 0
yzcd
r?4
.474
.120
.593
.179

1
+0
1
+0
«
.029
.200
.022
.529
N =

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                                 Table 2




                       Isophorone Chemical Analysis




                       Mean and Standard Deviation

Test 1

Test 2

Control
Not
Found
Mot
Found

2
+0
2
±°
#1
.14
.26
.18
.17
Concentration ing/1
#2 «
4
±°
4
+0
.18
.23
.15
.22
8
+0
8
+ 2
.29
.34
.78
.81
Analyzed
ff4
15.61
+ 0.92
14.51
+ 1 . 44

22
+0
27
+5
«
.66
.87
.63
.41
N = 8
                                    J4

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                                          Table  3




                                      Toxicity Results




                   Weights of Surviving Fish and Comparison  with  Controls

Aeenaphthene
1

Aeenaphthene
2

Isophorone
I

Isophorone
2


X
SO
N
3c
SD
N
X
SD
N
X
SD
H
Control
0.1-%
0.032
31
0.122
0,042
45
0.141
0.047
54
0.202
0.041
68
Solvent Cone.
Control 1
0.218 0
0.034 0
33
0.180 0
0.048 0
50
None 0
0

None 0
0

.200
.037
40
.167
.054
35
.145
.066
52
.239
•.046
69
Cone.
2
0.200
0.034
39
0.176
0.056
49
0.144
0.060
62
0.204
• 0.0 ';7
63
Cone.
3
0.152ab
0.030
50,
0.155b
0.039
40
0.143
0.052
36
0.1793
0.045
71
Cone.
4
0.140ab
0.028
35
0.126b
0.033
52
0,140
0.040
48
0.162®
0.039
71
Cone .
5
0.073ab
0.023
31
0.079ab
0.010
29
0.1153
0.031
63
0.171a
0.041
59
a = 1 tail test different froa normal control 0.99% level




b = i tail test different from solvent control 0.99% level




c = 1 tail test different from solvent control 0.95% level

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                                 Appendix  1




  Guidelines  for  Conducting  Flow-Through  Karly  Life Stage Toxicity Tests  with




        Fathead Minnows  for  Use  in  the USE PA, OTS-01U) Round  Robin Tost









 1.    In  an Early  L^fe Stage Toxicity Tost  with  fathead  minnows,  organisms1,  are




      exposed  to  toxicant  during  part of  the  embryonic  stage,  all of  the




      larval stage  and part  of the  juvenile stage.'  The  organisms are examined




      for  statistically  significant reductions  in  survival and weight  in  order




      to  determine  lower and upper  chronic  endpoints.







      A lower  chronic endpoint is the highest tested  concentration (a)  in an




      acceptable chronic test, (b) which did  not cause the occurrence  (which




      wes  statistically  significantly different  from  the control  at  the 95%




      level) of any specified adverse effect, and  (c) below  which no  tested




      concentration caused such an occurrence.







      An upper chronic endpoint is the lowest tested  concentration (a)  in an




      acceptable chronic, test, (b) which caused  the occurrence (which was




      statistically significantly different  from the  control  at the 95% level)




     of any specified adverse effect  and (c) above which  all  tested




     concentrations caused  such an occurrence,







2,   Not enough information is currently available concerning early  life




     stage tests  with fathead minnows to allow precise  specification of




     details   for  all. aspects of the test.  Enough  such  tests  have been




     conducted ~nd enough  aspects have  been studied, howuver,  to indicate




     that these Guidelines are appropriate.  A prudent  course  of action  for




     anyone planning to  conduct  such, tests  would be to  initially conduct a




                                     16-          . • •

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     test with no  toxicant  to  gain  experience  nut)  to  determine  if  the




     requirements  of  sections  10,  11,  19,  20,  26 and  27  can  bo  mot:  using  the.




     planned water, food, procedures,  etc.   If a solvent may bo: used  In  the




     preparation of a stock solution,  it would also be  prudent  to  test: one  or




     more concentrations of one  or  more solvents at the  same time  (sec




     Section A),   General infc""mat i.on  on such  things  as  apparatus,  dilution




     wj.i~.er, toxicant,  randomization of test  chatrbers  and organisms,  and




     methods for chemical analyses, can be  found in Draft  #10 of the  proposed




     ASTM Standard Practice for  Conducting  Acute Toxicity  Tests with  Fishes,




     Macroinvertehrates, and Amphibians.







3.   Tests should  he  conducted with at least  five  toxicant co?icentrat ions  in




     a geometric series and  at least one control treatment.   The




     concentration of  toxicant in  each treatment,  except  for highest




     concentration and the  control  treatment,  should  usually be 50  percent  of




     that, in the next  higher one.







4.   If a solvent  other than water  is  used  to  prepare test solutions,  a




     solvent control  (at the highest solvent concentration present  in  any




     other treatment)  using  twice  as many  test organisms and  test  chambers  as




     the other treatments is required  in addition  to  the regular control,




     unless such a control  has already been  tested in the  same  water vith  the




     same species of  fish,   food, and test procedure and  the  water quality has




     not changed significantly,  A  concentration of solvent  is  acceptable




     only if it is (or has   been) shown that  concentration  or  a  higher  one




     does not cause an increase  or  decrwase  in survival  or weight  at  the  end




     of the test that  is statistically significantly different  from  the.




     control at the 95% level using a  two-tailed test.




                                     17

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*5 .   For each  treatment  (toxicant  concentration  and  control)  there1,  must:  be  at




     least two replicate test chambers each  containing  one  or more  embryo




     cups with at  least  60 embryos divided equally between  the  embryo  cups  at




     the beginning of the test.







6,   Two test  chambers have been used routinely:




     a.  Twenty fish have been tested in -3 ehftmber which  is 16  cm x 44 cm x




         18 cm high with a 16 cm x 18 cm 40-inesh stainless  steel  screen  ft cm




         from one end, with a water depth of  12.8 cm and  with a flow rate of




         190 ml/minute,




     b.  Fifteen fish have been tested in a  chamber  which  is  6,5 cm x  18.0  cm




         x 9.0 cm high with a 6.5 cm x 9.0 era 40~mesh stainless steel  screen




         2.5 cm from one end, with n water depth of  4.5 cm  and  with  a  flow




         rate of 15 ml/minute.




     All of the above are inside dimensions.  In both test  chambers  the  water




     depth is controlled by a standnipe located  in the  smaller  screened




     compartment  with the test solution entering at  the other end of the test




     chamber.







7.   Embryo cups  should be glass cylinders about 4.5 cm inside  diameter  and




     about 7 cm high with 40-mesh nylon or stainless steel  screen glued  to




     the botton.   The embryo cups must be suspended  in  the  test  chamber  in




     such a way as to insure that the organisms are  plways  submerged and that




     test solution regularly flows into and out of the cup  without  agitating




     the organisms too vigorously,   A rocker arm apparatus  dtivtni by a 2




     r.p.ra.  motor and having a vertical-travel distance of  2.5  - 4.0 cm has




     been successful ly used,  as have self-starting siphons  that  cause  the




     level  o£ solution in the test  chamber to rise and  fall.




                                    . 18

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8.    Any  water  in  which  fathead minnows will  survive,  grow,  and reproduce

      sat isfactorily  should  be  an  acceptable dilution  water for early life

      ,'itage  toxicity  tests with  fathead minnows.


9,    A  16-hr  light and 8-hr  dark  photoperiod  should  be provided.   A 15- to

      30-mimite  transition period  at "lights on"  and  "lights  off"  may be

      desirable.  Light intensities  from 10 to  100  lumens  at  the water surface

      have been  used  successfully, but the intensity  should be about the same

      for  all  test  chambers.  Lights should he  provided by wide—spectrum

      (color Rendering Incex  > 90) fluorescent  lamps.


10.   Tests should be conducted at 25° C.  The  temperature in each test

      chamber  should  be between 24 and 26° C at all times  and must be between

      20 and 28° C  at all times.   If the water  is heated,  precautions should

      be taken to assure that supersaturation of dissolved gases is avoided

      and  total  dissolved gases should be measured  at  least once during  the

      tekt in  the water entering the control treatment.
                                              £

11.   The dissolved oxygen concentration should be  between 75 percent and 100

      percent  saturation at all times in all test chambers.  At  no time  during

      the  test should one test chamber have a dissolved  oxygen concentration

      that is more than 1.1 times the dissolved oxygen  concent rat ion occurring

      in another chamber at the same time,


12.  The  flow rate of test solution through the test chambers must be great

     enough to maintain the dissolved oxygon concentration (sec- sections 11

     and 22) and to  insure that the toxicant concentrations  are not decreased

     significantly due  to uptake by test organisms and  material on the  sides

     aiifi bottoms of the chambers .

                                 ' '   19

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13.  A test begins when embryos  in embryo  cups  are  placed  in  test  solution




     and ends 3?, days  later,







14.  Embryos and Fish  should not  be  treated  Co  cure or  prevent  disease  or




     fungus before or  during a test.







15.  Embryos should be obtained  From  a  fatbend  minnow stock culture




     maintained at 25° C and a dissolved oxygen concentration  between 75




     percent and 100 percent saturation with  a  16-hr light: and  3-hr  dark




     photoperiod.  Frozen adult brine shrimp  has been success fully used  as a




     food for adult fathead minnows.  The  maximum production  of embryos  by




     fathead minnows has been obtained  in  a  30  cm x 60  cm x 30  cm  deep




     chamber with a water depth of 15 cm when 15 cm x 30 cm quadrants are




     formed with stainless steel  screen and one male, one female and one  or




     two substrates are placed in each  quadrant.  Half-round  spawning




     substrates (Benoit and Carlson,  1977) with an  inside diameter of 7.5 cm




     and a length of 7.5 cm have  been used successfully.







16.  The afternoon before a test  -is to begin, all of the substrates  should be




     removed from an appropriate  number of tanks in the stock culture unit




     and should be replaced about the time the  lights are turned on  the next




     morning.   Enough  (at least three) substrates with embryos  on  them should




     be I'eitiuved six hours later and soaked in dilution water  for two hours.




     For  each  individual substrate the ^-nbryos should be gently separated




     (Cast  and  Hrungs,  1973)  and  removed ;;nd visually examined  using a




     dissecting scope  or a magnifying viewer.  Empty shells and undeveloped




     and  onaque embryos should  be discarded.   If less than 50 percent of  the




     embryos  from a substrate appear to he healthy  and  ft?rtile, all the




                                     20

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     embryos from that .substrate should be discarded.  Single embryos with no




     fungus or partial shells attached are preferable, although embryos with




     partial shells attached and clumps of two or throe embryos (with or




     without separation) have been used success fully,  An approximately equal




     number of acceptable embryos from one substrate should be impartially




     distributed to each embryo cup and the process repeated for at least two




     more substrates until the proper number of embryos have been placed  in




     each cup to give at least 60 embryos per treatment.  The embryo cups




     should be standing in dilution water when the embryos are being




     distributed and then the cups should be randomly placed in the test




     chambers.







17.   Twenty to 7.4 hours after the.y are placed in the embryo cups, the embryos




     should be  visually examined under a dissecting scope or magnifying




     viewer and all  dead embryos should be counted and discarded.  Embryos




     that are alive  but heavily fungused should also be counted and




     discarded.   Forty to 48 hours after the start of the exposure all dead




    , and  heavily fuugused embryos should be counted and removed.   The




     remaining  healthy, fertile embryos should be impartially reduced to  the




     desired number  of test  organisms (,-tt  least 30 par treatment).  IE more




     than about  35  percent  of embryos in the control treatment  arc discarded




     within the  firnt  48  hours  of the test because they are  dead  or heavily




     fungused,  it  will probably be cost-eftective to restart the  test.  In




     addition,  if  toxicant  related  effect;, are seen at 48 hours,  it will




     probably be  cost  effective to  restart the test since all of  the toxicant




     concentrations  will  probably cause adverse effects.   Each  day thereafter




     dead embryos  should  be  counted  and  discarded.




                                     21

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 18.   In  each  treatment, when hatching  is  about  90 percent complete or 48 hr

      after  first hatch  In  tli.it  treatment,  the  live young fish ahould.be

      counted  and the  live  fish  that  arc visibly (without the use of a

      dissecting scope or magnifying  viowfir)  lethargic or grossly abnormal in

      either swimming  behavior or  physical  appearance should be counted.  All

      of  the normal and  abnormal  live  fish  should  he  released into the test

      chambers.  Unhatched  embryos should  be  left  in  the cups'and released

      into the test chamber when  they hatch.  The  ra: £9 of time-to-hatch (to

      the nearest day) in each cup should  be  recorded.


 19.   A test should be terminated  if  t'-c average percent of embryos (based on

      the number of: embryos after  thinning) that  produce live fry for release

      into test chambers in any control treatment  is  less than 50 peicent or

      if  the percent hatch  in any control embryo  cup  is more than 1.6 times

      that in  another control embryo cup,


20.   The flow rate, size of the  test chamber and  the amount of food added

      should be such that the average weight of  the control  fish  at the end o£

      the test would not be significantly greater  if  only half as many fish

     were tested per test chamber.


21,   Each test chamber containing live fish over  two days old must be fed

      live newly hatched brine sliLintp at least two  times a day at least six

     hrs apart (or three times a day aboui. four hours apart)  on  days 2-5

     after hatch and  at least five days a week  thereafter.   They must be fed

     at least  once a  day on all other days.  Other food mny. als\t be provided

     in addition to the above.   The amount of food provided to each chanihor

     may be proportional to the mi'sber an.d size; of fish in  the chamber, but

     each chamber  wist be treated in a comparable manner.   Quantifying the
                                     22 '-.'.-•

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      amount  of  live  newly hatched brine shrimp to be fed is difficult, but




      the  fish should  not  be  excessively overfed or underfed.   A largo buildup




      of  food on the.  bottom of the charnbaer  i.a  a sign of Recessive




      overfeeding,  A  sign of not  feeding enough of the light  kind of food is




      that  in a  sideview  the  abdomen does not  protrude.







22.   Test  chambers should be clc.ined often  enough to maintain the dissolved




      oxygen  concentration (see  sections 11  and 12) and to insure that the




      toxicant concentrations are  not decreased significantly  due to sorption




      by matter  on !:he  bottom and  sides.   In most  tests  if the organisms are




      not  ove.rfe:! too  much and  the flow rate is not too low,  removing debris




      from  the bottom  once or twice  a week should  he adequate.  With some




      toxicants  that promote  growth  of bacteria the sides and  bottoms should




      be cleaned more  often.   Debris  can  be  removed with a large pipette and




      rubber  bulb or by siphoning  into a white  bucket.   A dark tip on the




      pipette or siphon should help  fish  avoid  being sucked  up,  but  the




      pi "•(••  te or bucket should be  examined Co  insure that no  live fish is




      d iscarded.







23.   Temperatures should  bs  recorded in  till test  chambers once  at  the




     beginning of the test and  once  near  the middle of  the  test.   In




      addition,  temper ature should he recorded  at  least  hourly in one test




     chamber throughout the  test.   The  dissolved  oxygen concentration should




     be measured in each  treatment  nt  least once  a week during  the  test.




      Hardness,  pH,  alkalinity,  and  acidity  should  be measured once  a week in




     the control treatment and  one P.  in  the  highest toxicant concentration.




     The concentration of toxicant:  should be measured  at  least  twice a week




      in each treatment.




                                      23

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 24.  Dead  fish should be removed and recorded when  observed,   Ac  a minimum




     11, 18, 25 and  32 days aft«r  Che beginning  of  the test,  the  live  fish




     should be counted and the  fish that are visibly (without  the use  of  a




     dissecting scope or magnifying viewer)  lethargic  and  grossly abnormal in




     cither swimming behavior or physical  appearance should  be counted,







 25.  The fish should not be fed for the  last 24  hours  prior  to terinination on




     day 32.  At terminal'inn the weight  (wet, blotted  dry) of  each fish  that




     was alive at the end of the test should he  determined.   If the fish




     exposed to toxicant appear to ba edematous  compared  to  control fish,




     determination of dry, rather  than wet, weight  is  desirable.







 26.  A test is not acceptable if the average survival  of  the  controls  at  the  .




     end of the test is less than 80 percent or  if  survival  in any control




     chamber is less than 70 percent.







 27.'  A test is not acceptable if the relative standard  deviation  (RSD  =  100




     times  the standard deviation divided by the mean)  of  the  weights  of  the




     fish that were alive at the end of  the test in  any control test chamber




     is greater than 40 percent.







28.  Data to be statistical!'/ analyzed are:




     (A)  percent  of healthy,  fertile embryos at /sO-'iS  hours




     (H)  percent  of embryos that  produce live fry  for  release into test




         chambers




     (C) percent  of embryos that  produce live, normal .fry for release  into




         test  chambers




     (D) percent  of embryos that  produce life fish  at  end of  test




     (E)  percent  of "mbryos  that  produce live,  normal  fish at  end  of  test




                                     24

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     (F)  weights of  individual  fish  thnt  were  alive  at  end  of  test.




     Although  item A  is based on  the  number  of  embryos  initially  placed  in




     embryo cups, items B, C, D,  and  K  are based  on  the  number  of  embryos




     after thinning.







29.  Dichotomous data  (live-dead, normal-abnormal) should  be analyzed  using




     contingency tables (Sokal and  Kohl, f,  Biometry,  1969,  p.  587)  or  log




     linear techniques.  For weight data the  individual  fish a;.:  used  as the




     replicates unless a two-tailed V test indicates  that  differences  between




     replicate test chambers are  not  negligible.  Weight data may  be  analyzed




     using (Steel and Torrie, Principles end  Procedures  of Statistics,  1960,




     p. Ill) should be used to identify treatments producing weights  that are




     statistically significantly  lower than  those of  the controls  at  the 95




     percent level.







30.  Although the results of -the  analyses of  all  six  types of. data in  section




     28 should be reported, the lower and upper chronic  endpoints  are  only




     baaed on statistically significant reductions in survival  and weight at




     the end  of the  test  (items D and F),  Item A is  apparently relatively




     insensitive and item B is included in item D.  In addition, abnormal




     fish  seem to weigh less  than normal fish and so will  be covered  in  item




     F.  A1.no, since The  c'.ist incL ion between  normal and  abnormal is




     subjective,  this  kind  of data is expected to be  less reproducible from




     one investigator  to  another  than the other kinds oC data.  Although




     items 1)  and  F are considered primary,  the other  items are  included




     because,  tlioy may  provide useful  in format i.on.

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                                  References




 Benoit, D. A., and H. W. Carlson,  1977.  Spawning Success of Fathead Minnows




      on Selected Artificial Substrates.  Prog. Kish-Cult. 39: 67-69.




 Flickinger,, S. A.  1969.  Determinations of Sexes in the Fathead Minnow,




      Trans. Am. Fish. Soc.  98: 526-527.




 Cast, M. H. ,  and W. A. Brungs.  1973.  A Procedure for Separating figgs oE the




      Fathead Minnow.   Prog. Fish-Cult. 35: 54;




 May,  R. C.  1970.  Feeding Larval Marine Fishes in the Laboratory:  A Review.




      Calif. Mar. Res. Comm.,  California Cooperative Oceanic Fisheries




      Investigations Report  14: 76-83.
This tentative  procedure  was  written  by  Clisrl.es  Stephan with the help of many




members of the  staCf of the Environmental  Research  Laboratory in Dul.uth,




Minnesota,




                                      26

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