EPA/600/A-97/079 7A.11 LABORATORY OBSERVATIONS OF THE RISE OF BUOYANT THERMALS CREATED BY OPEN DETONATIONS Roger S. Thompson* U.S. Environmental Protection Agency Research Triangle Park, North Carolina William H. Snyder University of Surrey Guildford, Surrey, England Jeffrey C. Weil National Center for Atmospheric Research Boulder, Colorado 1. INTRODUCTION The most common method of disposing of obsolete munitions is by open detonation in an earthen pit. Typically, small quantities (up to 500 Ibs.) are destroyed in a detonation that creates a buoyant, turbulent cloud or thermal which contains contaminants and rises through the atmosphere. The detonations are scheduled for daytime when the atmospheric conditions can be described as a convective boundary layer surmounted by a temperature inversion. Detonating larger quantities would result in more complete combustion and more economic disposal of the munitions. The environmental effects of detonating larger quantities are being evaluated with new dispersion models (Weil, et al, 1996) which require new experimental data and descriptive algorithms for their development and testing. Laboratory experiments were carried out in a water tank at the Fluid Modeling Facility of the U.S. Environmental Protection Agency to study the rise and growth of buoyant thermals and their penetration through elevated density changes and into elevated stable layers. A dense volume of salt water (herein referred to as a thermal) was released at the top of the tank and observed as it fell 1) through water of constant density, 2) through a constant-density layer into a layer of greater density with a step-change at the interface, or 3) through a constant-density layer into a layer with a linear increase of density with depth. The falling volume of water simulated a buoyant thermal rising through the atmosphere where density decreases with height. These density profiles are first approximations to the profiles observed during convective atmospheric conditions. Visual observations and video recordings were used to determine the rise and growth of the thermals as well as estimates of the fraction of the thermal that penetrated a step-change interface. Observations and concentration measurements were used to determine the maximum * Corresponding author address: Roger S, Thompson, MD-81, National Exposure Research Laboratory, U.S. Environmental Protection Agency, Research Triangle Park, NC 27711; thompson.roger@epamail.epa.gov. penetration distance and equilibrium height of thermals that encounter an elevated linear gradient. A criterion was obtained for predicting when a thermal will penetrate a step-change in density as a function of its initial buoyancy, the magnitude of the step- change and the height of the interface. The maximum penetration distance and equilibrium heights for the elevated gradient cases are presented graphically. 2. EXPERIMENTAL DETAILS The experiments were conducted in the towing tank at the EPA Fluid Modeling Facility. The tank is 3.6 m wide and was filled to a level of 108 cm using salt water. By varying the salinity, the desired density stratification was obtained. Thermals were simulated with the release of a 150 cm3 mixture of salt water and blue food dye from a 10-cm-diameter hemispherical cup. The cup was lowered into the water until the surface of the fluid in the cup was level with the water surface in the tank. By quickly rotating the cup, its fluid was released with roughly the initial shape of a thermal created by a detonation. This technique has been used by Richards (1961) and Saunders (1962) who performed similar experiments. Releases into neutral and step-change environments were made first. A video camera was used to record a time history of the trajectory and growth of each thermal; a mirror to the side at 45° provided a side view in addition to the direct front view. Several frames of the video recording of each thermal were input to a personal computer and analyzed to determine the depth of the leading edge, the depth of the centroid, the horizontal dimension (diameter), and vertical thickness from both front and side views. These dimensions were used to compute the volume of the thermal by approximating its shape as an oblate spheroid. For the experiments with a neutral layer followed by a linear increase in density, a visual observation of the maximum penetration distance was made. In addition, the equilibrium height of the thermal was computed from the concentrations of dye samples collected with an array of sample ports that were moved through the thermal after it reached its equilibrium height. ------- 3, RESULTS The variables used to describe the position of a thermal are defined in Fig. 1 in an atmospheric setting where z is measured upward from the earth's surface. The height of the centroid of the thermal is zc and the distance to the virtual origin, below the surface, where the thermal can be considered to have originated at a point is Zy. The height to the step-change interface or base of the elevated linear gradient is z.,. For the tank experiments, z was measured positive downward from the water surface. To keep an atmospheric perspective, we will discuss the laboratory results as if the tank were inverted; that is, the falling volume of fluid will be described as a rising thermal with its properties defined in terms of its height. Figure 1. Variables to describe the rise of a thermal in the atmosphere. Thermals with high buoyancy compared to the density difference at the interface will completely penetrate into the upper -layer and continue to rise indefinitely; Thermals with less buoyancy may, because of their momentum, penetrate beyond :he interface only to have a fraction return to the interface as the momentum fades. The weakest thermals will not penetrate the interface at all. In describing the final fraction of a thermal that penetrates a step change Pf, Richards (1961) defined a parameter S as a measure of the strength of the interface relative to the buoyancy of the thermal. By adapting his expression to the atmosphere, we get S=V(p,-p2)/B, where V is the volume of the thermal when it is centered on the interface (we use the volume when the centroid is at z,), p,-p2 is the density difference between the lower and upper layers and B is the mass deficit of the thermal at its release (initial volume times its density subtracted from that of an equal volume of the surrounding fluid). In the water tank, B is replaced by M, a similarly defined mass excess, and the density difference is reversed. A comparison of our determinations of Pf with those of Richards is shown in Fig. 2 where it is seen that our results have a similar slope but are offset to larger values of S. Based on the following intuitive argument, our results seem more reasonable. As a thermal with a value of S less than 1 approaches the interface, its average density is less than that in the upper layer. Given this and its momentum, the thermal may be expected to continue rising, resulting in essentially total penetratbn. Our results are in better agreement with this argument; Richards' results suggest Pf of only 0,5 when S=0.9. Figure 2. Final penetration versus Richards' S (uses- measured volume). Open symbols and dashed line are from Richards (1961). ------- Because the volume of the thermal when it is centered on the interface is not known prior to the detonation, Richards' formula is not very useful in modeling applications. To obtain a predictive formula, we define a parameter A=Vp(p1-p2)/B, where V. is the predicted volume of the thermal when its centroid is at the interface. An expression for Vp as a function of z was obtained from values computed from the video recordings of the thermals. As shown in Fig, 3, for thermals in a neutral environment and those encountering a step- change in density with a P( 2 0.5, the volume can be described by 0.058(zc-»-zv)3. Thermals that have a lower final penetration, P, < 0.5, have a somewhat larger volume. Using the volume formula above in our expression for A (with zc=z1, i.e. Vp=0.058(z1-*-zv)3) we obtain the results shown in Fig. 4. A vertical line at 4=1.35 divides the data into cases with large P, and cases with low P, and leads to the simple criterion ,that thermals penetrate for A < 1.35 and do not penetrate for A a 1.35. 50000 '• step-change environment; P(>0.5 . o step-change environment; P, < 0.5 1 neutral environment 10000 o 1 1000 30 40 50 zc+zv, cm 60 Figure 3, Average measured volumes for all releases into step-change and neutral environments. When a thermal in the tank enters an elevated gradient (layer of linearly increasing density), its momentum causes it to overshoot its equilibrium height. It will then reverse direction and soon approach an equilibrium position. The maximum penetration distance 1 • 9 • .8 - .7 • .6 • .5 • .4 • .3 • .2 - .1 • i t ' * ••* • < • * 4 *• < • l 1 I 1 1 1 »* 1* • • • « * Y i i »* * m mm .... ' • Figure 4. Final penetration versus A. type. After the thermal was seen to reach its equilibrium height, an array of 100 sample tubes was drawn through the thermal collecting water samples that were analyzed for dye concentration. From these concentrations, the vertical distribution of the dye in the thermal was determined and used to calculate the height of its centroid zeq. The values of these variables are shown in Fig. 5 plotted against PT, a measure of the initial buoyancy of the thermal divided by the strength of the density gradient, This nondimensional parameter is defined by pT=FT1M/[(z1+zv)N1/2Jt where FT is the buoyancy of the thermal and N is the Brunt- Valsala frequency of the stable layer. In the water tank, FT=Bg/p, where g is the acceleration due to gravity, p, is the density of the neutral layer, and jV2=-&| -£• , where —£. is the density gradient in the stable layer. While in the atmosphere, Fr= —. where QT is the heat content of the thermal, cp is the specific heat of air, pa is the density of air, 8a is the potential temperature of the ambient air, and , where — is the gradient of the potential dz of the leading edge of the thermal zmx was visually temperature in the stable layer. The solid line through the observed and recorded during each experiment of this P°ints for z™ IS the theoretical prediction of Saunders ------- (1962) with his constants evaluated using the empirical results of this study. It is seen to provide a good fit to the data. We know of no theoretical expression for zeq, but given the prediction of zmx, a corresponding value of zeq can be estimated from the empirical expression (Zeq-z1)/(z1+ztf)=0.47[(zmx-z1)/(zl+zv)]1^2 shown as a dashed line in Fig. 5. N •f 1.5 N .5 • dp/dz = 0.0001 gm/cm dp/dz = 0.0004 gm/cm4 dp/dz = 0.0001 gm/cm4 dp/dz = 0.0004 gm/cm4. 5. ACKNOWLEDGEMENTS The authors wish to acknowledge Mr. Van Hursey and Mr. G. Leonard Marsh of Geophex, Ltd. for their support in the laboratory setup, data collection and data analysis portions of this experimental study. 6. REFERENCES Lawson, R.E. Jr., Snyder, W.H., and Shipman, M.S. 1998; A laboratory model of diffusion in the convective boundary layer. Preprints 10th Joint Conference on Applications of Air Pollution Meteorology with the AWMA, Amer. Meteor, Soc., Boston. Richards, J.M., 1961: Experiments on the penetration of an interface by buoyant thermals. J. Fluid Mech., 11, 369- 384. Saunders, P.M., 1962; Penetrative convection in stably stratified fluids. Tellus, 14,178-194. Weil, J.C., Templeman, B.T., Banta, R., and Mitchell, W. 1996; Dispersion model development for open burn/open detonation sources. Preprints 9th Joint Conference on Applications of Air Pollution Meteorology with AWMA, Amer. Meteor. Soc., Boston, 610-616. DISCLAIMER: The information in this document has been funded by the U.S. Environmental Protection Agency. It has been subjected to the Agency's peer and administrative review and approved for publication. Mention of trade names or commercial products does not constitute commercial endorsement or recommendation for use. Figure 5. Maximum penetration height beyond interface (solid symbols) and equilibrium height of centroid (open symbols) for elevated gradient environments. 4. SUMMARY AND DISCUSSION Laboratory results have been presented that can be used in the development of dispersion models for assessing the impact of detonation of surplus munitions. In particular, a simple criterion for predicting the penetration of a thermal through a step-change in density, data to support a theoretical prediction of the maximum height, and an empirical expression for the equilibrium height of thermals that encounter an elevated temperature gradient will provide basic algorithms for such models. Further work is underway in a convection tank (Lawson, et at., 1998) with a heated floor and an elevated temperature gradient to more closely model the convective nature of the atmosphere. ------- • • . TECHNICAL REPORT DATA 1. REPORT NO. 2. EPA/600/A-97/079 4. TITLE AND SUBTITLE Laboratory observations of the rise of buoyant thermals created detonations by open 7. AUTHOR(S) 'Thompson, R.S., 2W.H. Snyder, and 3J.C. Weil 9. PERFORMING ORGANIZATION NAME AND ADDRESS 'Same as Block 12 2Universtiy of Surry Guilford, Surrey, England 'National Center for Atmospheric Research Boulder, CO 12. SPONSORING AGENCY NAME AND ADDRESS National Exposure Research Laboratory Office of Research and Development U.S. Environmental Protection Agency Research Triangle Park, NC 277 1 1 5. REPORT DATE 6. PERFORMING ORGANIZATION CODE 8. PERFORMING ORGANIZATION REPORT NO. 10.PROGRAM ELEMENT NO. 1 1 . CONTRACT/GRANT NO. 13.TYPE OF REPORT AND PERIOD COVERED 14. SPONSORING AGENCY CODE EPA/600/9 IS. SUPPLEMENTARY NOTES 16. ABSTRACT The most common method of disposing of obsolete munitions is by open detonation in an earthen pit. Typically, small quantities (up to 500 Ibs.) are destroyed in a detonation that creates a buoyant, turbulent cloud or thermal which contains contaminants that rises through the atmosphere. The detonations are scheduled for daytime when the atmospheric conditions can be described as a convective boundary layer surmounted by a temperature inversion. Detonating larger quantities would result in more complete combustion and more economic disposal of the munitions. The environmental effects of detonating larger quantities are being evaluated with new dispersion models (Weil, et al, 1996) which require new experimental data and descriptive algorithms for their development and testing. 17. KEY WORDS AND DOCUMENT ANALYSIS a. DESCRIPTORS ^IDENTIFIERS/ OPEN ENDED TERMS o.COSATl 18. DISTRIBUTION STATEMENT 1 9, SECURITY CLASS (This Report) 21 .NO. OF PAGES 20. SECURITY CLASS (This Page) 22. PRICE ------- |