EPA/600/A-97/079
7A.11
LABORATORY OBSERVATIONS OF THE RISE OF BUOYANT THERMALS
               CREATED BY OPEN DETONATIONS
                                          Roger S. Thompson*
                                   U.S. Environmental Protection Agency
                                  Research Triangle Park, North Carolina

                                           William H. Snyder
                                           University of Surrey
                                        Guildford, Surrey, England

                                             Jeffrey C. Weil
                                 National Center for Atmospheric Research
                                           Boulder, Colorado
1. INTRODUCTION

    The most common  method of disposing of obsolete
munitions is  by open  detonation in an  earthen  pit.
Typically, small quantities (up to 500 Ibs.) are destroyed
in a detonation that creates a buoyant, turbulent cloud or
thermal which contains  contaminants and rises through
the atmosphere.  The  detonations are scheduled for
daytime  when the  atmospheric  conditions can  be
described as a convective boundary layer surmounted by
a temperature inversion. Detonating larger quantities
would result in more complete combustion  and more
economic disposal of the munitions. The environmental
effects of detonating larger quantities are being evaluated
with new dispersion models  (Weil, et al,  1996) which
require new experimental data and descriptive algorithms
for their development and testing.
    Laboratory experiments were carried out in a water
tank  at  the  Fluid  Modeling  Facility of  the U.S.
Environmental Protection Agency to study the rise and
growth of buoyant thermals and their penetration through
elevated density changes and into elevated stable  layers.
A dense  volume of salt water (herein referred to as a
thermal) was released at the top of the tank and observed
as it fell 1) through water of constant density, 2) through
a constant-density layer into  a layer of greater density
with a step-change at  the interface,  or 3) through a
constant-density layer into a layer with a linear increase
of density  with depth.   The falling volume  of water
simulated  a   buoyant   thermal   rising  through   the
atmosphere where density decreases with height.  These
density profiles are first approximations to the profiles
observed during convective atmospheric conditions.
    Visual observations  and video recordings were used
to determine the rise and growth of the thermals as well
as estimates of the fraction of the thermal that penetrated
a step-change interface.  Observations and concentration
measurements were  used to  determine the maximum

* Corresponding author address: Roger S, Thompson,
MD-81, National Exposure Research Laboratory, U.S.
Environmental Protection Agency, Research Triangle
Park, NC 27711; thompson.roger@epamail.epa.gov.
                                 penetration distance and equilibrium height of thermals
                                 that encounter an elevated linear gradient.
                                    A criterion  was obtained for  predicting  when  a
                                 thermal will penetrate a  step-change  in density  as  a
                                 function of its initial buoyancy, the magnitude of the  step-
                                 change and the  height of the interface. The maximum
                                 penetration  distance and equilibrium  heights for the
                                 elevated gradient cases are presented graphically.

                                 2. EXPERIMENTAL DETAILS

                                    The experiments were conducted in the towing tank
                                 at the EPA Fluid Modeling Facility. The tank is 3.6 m wide
                                 and was filled to a level of 108 cm using salt water. By
                                 varying the salinity, the desired density stratification was
                                 obtained. Thermals were simulated with the release of a
                                 150 cm3 mixture of salt water and blue food dye from a
                                 10-cm-diameter hemispherical cup. The  cup was lowered
                                 into the water until the surface of the fluid in the cup was
                                 level  with the water surface in the tank.  By quickly
                                 rotating the cup, its fluid was released  with  roughly the
                                 initial shape of a thermal created by a detonation.  This
                                 technique has been  used  by  Richards (1961)  and
                                 Saunders (1962) who performed similar experiments.
                                    Releases into neutral and step-change environments
                                 were made first.  A video camera was used to record a
                                 time history of the trajectory and growth  of each thermal;
                                 a mirror to the side at 45° provided a side view in addition
                                 to the direct front view.   Several frames of the video
                                 recording  of each  thermal were input to  a  personal
                                 computer and analyzed to determine the depth of the
                                 leading edge, the depth of the centroid, the horizontal
                                 dimension (diameter),  and vertical thickness from both
                                 front and side views.  These dimensions were used to
                                 compute the volume of the thermal by approximating its
                                 shape as an oblate spheroid. For the experiments with a
                                 neutral layer followed by a linear increase in density, a
                                 visual observation of the maximum penetration distance
                                 was made.   In addition,  the equilibrium height of the
                                 thermal was computed from the concentrations of dye
                                 samples collected with an array of sample ports that were
                                 moved through the thermal after it reached its equilibrium
                                 height.

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 3,  RESULTS

     The  variables used to describe the position of a
 thermal are defined in Fig. 1 in an atmospheric setting
 where z is measured upward from the earth's surface.
 The height of the centroid of the thermal is zc and the
 distance to the virtual origin, below the surface, where the
 thermal can be considered to have originated at a point is
 Zy. The height to the step-change interface or base of the
 elevated linear gradient is z.,. For the tank experiments,
 z was  measured positive downward  from the  water
 surface.  To keep an atmospheric perspective, we will
 discuss the laboratory results as if the tank were inverted;
 that is, the falling volume of fluid will be described as a
 rising thermal with its properties defined in  terms of its
 height.
   Figure 1. Variables to describe the rise of a
   thermal in the atmosphere.
    Thermals with  high buoyancy compared to the
density difference  at the  interface  will  completely
penetrate into the  upper -layer  and continue to rise
indefinitely; Thermals with less buoyancy may, because
of their momentum,  penetrate beyond :he interface only
to have a fraction return to the interface as the momentum
fades.   The  weakest thermals will not  penetrate the
interface at all. In describing the final fraction of a thermal
that penetrates a step change Pf, Richards (1961) defined
a  parameter S  as a measure of the  strength of the
interface relative to the buoyancy of the thermal.  By
adapting his expression to the  atmosphere,  we  get
S=V(p,-p2)/B, where V is the volume of the thermal when
it is centered on the interface (we  use the volume when
the centroid  is at z,), p,-p2 is the density difference
between the lower and upper layers and B is the mass
deficit of the thermal at its release (initial volume times its
density subtracted from that of an equal volume of the
surrounding fluid).  In the water tank, B is replaced by M,
a  similarly  defined  mass excess, and  the  density
difference  is  reversed.    A  comparison   of   our
determinations of Pf with those of  Richards is shown in
Fig. 2 where it is seen that our results have a similar slope
but are offset to larger values of S.   Based on  the
following intuitive  argument,  our  results  seem  more
reasonable. As a thermal with a value of S less than 1
approaches the interface, its average density is less than
that in the upper layer.  Given this and its momentum, the
thermal may be expected to continue rising, resulting in
essentially total penetratbn.   Our results are in better
agreement with this argument; Richards' results suggest
Pf of only 0,5 when S=0.9.
    Figure 2. Final penetration versus Richards' S (uses-
    measured volume). Open symbols and dashed line
    are from Richards (1961).

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     Because the volume of the thermal when it  is
 centered on  the  interface  is not known prior to the
 detonation, Richards' formula is not  very  useful  in
 modeling applications.  To obtain a predictive formula, we
 define  a parameter  A=Vp(p1-p2)/B, where V. is the
 predicted volume of the thermal when its centroid is at the
 interface.  An expression for Vp as a function of z was
 obtained from values computed from the video recordings
 of the thermals.  As shown  in Fig, 3, for thermals in a
 neutral environment  and those encountering a  step-
 change in density  with a P( 2 0.5, the volume can be
 described by 0.058(zc-»-zv)3.  Thermals that have a lower
 final  penetration,  P,  < 0.5,  have a somewhat larger
 volume.   Using the  volume formula  above  in  our
 expression for A (with zc=z1, i.e. Vp=0.058(z1-*-zv)3) we
 obtain  the results shown in  Fig. 4.  A vertical line at
 4=1.35 divides  the data into cases with  large P, and
 cases with low P, and leads to the simple criterion ,that
 thermals penetrate for A < 1.35 and do not penetrate for
 A a 1.35.
    50000
             '• step-change environment; P(>0.5
             . o step-change environment; P, < 0.5
              1 neutral environment
    10000
 o

1
     1000
           30
                          40         50

                          zc+zv, cm
60
 Figure 3, Average measured volumes for all releases
 into step-change and neutral environments.
    When  a thermal in  the  tank  enters an  elevated
gradient  (layer  of  linearly  increasing  density),  its
momentum causes it to overshoot its equilibrium height.
It will then  reverse  direction and  soon approach an
equilibrium position.  The maximum penetration distance
1 •
9

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.7 •
.6 •
.5 •
.4 •
.3 •

.2 -

.1 •

i t ' 	
* ••*
• <
•
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4

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	 1 I 	
1 1 1
»*
1* •
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m mm .... ' •
                                                                       Figure 4. Final penetration versus A.
type. After the thermal was seen to reach its equilibrium
height, an array of 100 sample tubes was drawn through
the thermal collecting water samples that were analyzed
for dye concentration.  From these concentrations, the
vertical distribution of the  dye in the  thermal was
determined and used to calculate the height of its centroid
zeq.  The values of these variables are shown in  Fig. 5
plotted against PT, a measure of the initial buoyancy of
the thermal divided by the strength of the density gradient,
This   nondimensional  parameter   is   defined   by
pT=FT1M/[(z1+zv)N1/2Jt where FT is the buoyancy of the
thermal and N is the Brunt- Valsala frequency of the stable
layer.   In the water tank, FT=Bg/p,  where g is the
acceleration due to gravity, p, is the density of the neutral

layer, and jV2=-&| -£•  , where —£. is the density gradient

in the stable layer. While in the atmosphere, Fr=	—.
        where QT is the heat content of the thermal, cp is the
        specific  heat of air, pa is the density of air, 8a is the
        potential temperature of the ambient air, and
                   , where — is the gradient of the potential
                          dz
of the leading  edge of the thermal zmx was  visually    temperature in the stable layer. The solid line through the
observed and recorded during each experiment of this      P°ints for z™ IS the theoretical prediction of Saunders

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 (1962) with his constants evaluated using the empirical
 results of this study. It is seen to provide a good fit to the
 data.  We know of no theoretical expression for zeq, but
 given the prediction of zmx, a corresponding value of zeq
 can be estimated from the empirical expression
 (Zeq-z1)/(z1+ztf)=0.47[(zmx-z1)/(zl+zv)]1^2  shown  as  a
 dashed line in Fig. 5.
 N
 •f
       1.5
 N
        .5 •
               dp/dz = 0.0001 gm/cm
               dp/dz = 0.0004 gm/cm4
dp/dz = 0.0001 gm/cm4
dp/dz = 0.0004 gm/cm4.
 5. ACKNOWLEDGEMENTS

    The authors wish to acknowledge Mr. Van Hursey
 and Mr. G. Leonard Marsh of Geophex, Ltd. for their
 support in the laboratory setup, data collection and data
 analysis portions of this experimental study.

 6. REFERENCES

 Lawson, R.E. Jr., Snyder, W.H., and Shipman, M.S. 1998;
 A laboratory model of diffusion in the convective boundary
 layer. Preprints 10th Joint Conference on Applications of
 Air Pollution Meteorology with the AWMA, Amer. Meteor,
 Soc., Boston.

 Richards, J.M., 1961: Experiments on the penetration of
 an interface by buoyant thermals. J. Fluid Mech., 11, 369-
 384.

 Saunders,  P.M., 1962; Penetrative convection in stably
 stratified fluids. Tellus, 14,178-194.

 Weil, J.C., Templeman, B.T., Banta, R., and Mitchell, W.
 1996; Dispersion model development for open burn/open
 detonation  sources. Preprints 9th Joint Conference  on
Applications of Air Pollution Meteorology with AWMA,
Amer. Meteor. Soc., Boston, 610-616.
                                                      DISCLAIMER: The information in this document has been
                                                      funded by the U.S. Environmental Protection Agency. It
                                                      has  been  subjected  to  the  Agency's  peer  and
                                                      administrative review  and approved for publication.
                                                      Mention of trade names or commercial products does not
                                                      constitute commercial endorsement or recommendation
                                                      for use.
 Figure 5.  Maximum penetration height beyond interface
 (solid symbols) and equilibrium height of centroid (open
 symbols) for elevated gradient environments.
4. SUMMARY AND DISCUSSION

    Laboratory results have been presented that can be
used  in  the development of dispersion  models for
assessing the impact of detonation of surplus munitions.
In  particular,  a  simple  criterion  for  predicting  the
penetration of a thermal through a step-change in density,
data to support a theoretical prediction of the maximum
height, and an empirical expression for the equilibrium
height of thermals that encounter an elevated temperature
gradient will provide basic algorithms for such models.
Further work is underway in a convection tank (Lawson,
et  at., 1998)  with  a heated  floor and an  elevated
temperature  gradient  to  more closely   model  the
convective nature of the atmosphere.

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• • . TECHNICAL
REPORT DATA
1. REPORT NO. 2.
EPA/600/A-97/079
4. TITLE AND SUBTITLE
Laboratory observations of the rise of buoyant thermals created
detonations
by open
7. AUTHOR(S)
'Thompson, R.S., 2W.H. Snyder, and 3J.C. Weil
9. PERFORMING ORGANIZATION NAME AND ADDRESS
'Same as Block 12
2Universtiy of Surry
Guilford, Surrey, England
'National Center for Atmospheric Research
Boulder, CO
12. SPONSORING AGENCY NAME AND ADDRESS
National Exposure Research Laboratory
Office of Research and Development
U.S. Environmental Protection Agency
Research Triangle Park, NC 277 1 1

5. REPORT DATE
6. PERFORMING ORGANIZATION CODE
8. PERFORMING ORGANIZATION REPORT NO.
10.PROGRAM ELEMENT NO.
1 1 . CONTRACT/GRANT NO.
13.TYPE OF REPORT AND PERIOD COVERED
14. SPONSORING AGENCY CODE
EPA/600/9
IS. SUPPLEMENTARY NOTES
16. ABSTRACT
The most common method of disposing of obsolete munitions is by open detonation in an earthen pit. Typically, small quantities
(up to 500 Ibs.) are destroyed in a detonation that creates a buoyant, turbulent cloud or thermal which contains contaminants that
rises through the atmosphere. The detonations are scheduled for daytime when the atmospheric conditions can be described as a
convective boundary layer surmounted by a temperature inversion. Detonating larger quantities would result in more complete
combustion and more economic disposal of the munitions. The environmental effects of detonating larger quantities are being
evaluated with new dispersion models (Weil, et al, 1996) which require new experimental data and descriptive algorithms for
their development and testing.
17. KEY WORDS AND DOCUMENT ANALYSIS
a. DESCRIPTORS
^IDENTIFIERS/ OPEN ENDED TERMS o.COSATl

18. DISTRIBUTION STATEMENT
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