J technical FACT SHEET BUILDING A SCIENTIFIC FOUNDATION FOR SOUND ENVIRONMENTAL DECISIONS Rapid Radiochemical Method Phosphorus-32 (32P) in Water Samples EPA's rapid radiochemical methods expedite analytical turnaround time for selected radionuclides while providing quantitative results that meet measurement quality objectives. Methods are applicable to samples where contamination is from either known or unknown origins. This fact sheet is intended for radioanalytical laboratory personnel, decision makers within the incident command structure, additional reoccupancy decision makers (e.g., state and local public health), and other field environmental response personnel. Method Summary: The method uses rapid radiochemical separation techniques for determining 32P in water samples following a radiological or nuclear incident, A100 mL water sample is filtered and phosphate carrier is added, The solution is passed through a cation exchange resin and then a high performance, gel-type cation resin to remove interferences from cation radionuclides. The eluent is treated with a mixture of hydrogen peroxide and concentrated nitric acid, reduced in volume, by heating, and quantitatively transferred to a liquid scintillation vial for counting. The Cerenkov photons from the 32P beta (1710 keV, Emax) decay are detected using a calibrated liquid scintillation counter, Following counting of the sample, an aliquant of the final solution is used for yield determination by the inductively coupled plasma-atomic emission spectrometry (ICP-AES) method, Time to Process: 8 hr Includes radiochemical processing and counting The rapid method takes approximately half the time as other P-32 methods. Method Application The method is specific for 32P in drinking water and other aqueous samples, Application of this method should be validated by the laboratory using the protocols provided in Method Validation Guide for Qualifvino Methods Used bv Radiolociical Laboratories Particioatinciin Incident Response Activities, or the protocols published bv a recognized standards organization for method validation, Measurement Quality Objectives Required method uncertainty: 150 pCi/L Analytical action level (AAL): 12,000 pCi/L Required relative uncertainty: 13% above AAL Minimum detectable concentration (MDC): 3 pCi/L Sample quantity: 100 mL; 500 mL (MDC) Count time: Less than 30 minutes; 100 minutes (MDC) Equipment and Supplies Balances: Analytical —0.001 g readability or better; toploader —0,1 g readability | Hot plate or other suitable device for reducing sample volume | Laboratory supplies: glass beakers — 250, 400 mL; glass stirring rods; graduated cylinders —25, 50,100, 250,1,000 mL; pipettes — volumetric/automatic — assorted volumes down to the microliter range; scintillation vials — 22 mL glass; volumetric flasks —25,100, 200, 500,1,000 mL | Liquid scintillation counter: detector capable of measuring Cerenkov radiation | Inductively Coupled Plasma-Atomic Emission Spectrometer (ICP-AES) Sample Preservation Analysis within 3 days of sampling: No preservation required Holding time >3 days: Adjust pH to <2 with concentrated nitric acid Waste Generated per Sample 2 mL of gel-type cation resin 10 mL of cation exchange resins ~ 2 mL extraction chromatographic resin ~ 20 mL of acidic waste Isotopes of uranium, neptunium, and thorium, if present in the sample originally will be contained in extraction chromatographic resin Contacts Proaram: Kathv Hall Technical: John Griaas 513-379-5260 334-270-3450 hall.kathy@epa.gov griggs.john@epa.gov Method Access: https://www.epa.aov/sites/production/files/2015- 06/documents/p-32 epa-600-r-11-1811 11-10-11.pdf U.S. Environmental Protection Agency Office of Research and Development, Homeland Security Research Program EPA/600/S-17/057 March 2017 ------- |