SOP HW-17 Revision #3.1 December 2010 Page 1 of 13 Validating Chlorinated Herbicides GC, SW-846, Method 8151A % PREPARED BY: Russell Arnone, Chemist Hazardous Waste Support Section Peer Reviewed by: Concurred by: Approved by: Date: Date: Muhammad Sheikh, Chemist Hazardous Waste Support Section Michael Mercado, Acting Chief Hazardous Waste Support Section Robert Runyon, Chief Hazardous Waste Support Branch Annual Review Date: Date: Reviewed by: Date: Reviewed by: Date: ------- GC, SW-846, Method 8151 A/Herbicides SOP HW-17 EPA/Region II TABLE OF CONTENTS 1. Traffic Reports and Laboratory Narratives 3 2. Holding Times 3 3. Surrogate Recovery ( Form I I/Equivalent) 4 4. Matrix Spikes (Form Ill/Equivalent) 5 5. Blanks (Form IV/Equivalent) 6 6. Contamination 7 7. Calibration and GC Performance 8 8. Laboratory Control Samples 8 9. Equivalent-Herbicides-1 (Form VI) 9 10. Continuing Calibration (Form VII) 10 11. Analytical Sequence Check (Form VIII) 11 12. Herbicides Identification 11 13. Compound Quantitation and Reported Detection Limits 13 14. Chromatogram Quality 14 15. Field Duplicates 16 ------- USEPA Region II SW846 Method 8151 A/Chlorinated Herbicides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A 1.0 Traffic Reports and Laboratory Narrative 1.1 Are Traffic Report Forms present for all samples? jj _ _ ACTION: If no, contact lab for replacement of missing or illegible copies. 1.2 Do the Traffic Reports or SDG Narrative indicate any problems with sample receipt, condition of the samples, analytical problems or special circumstances affecting the quality of the data? _ jj _ ACTION: If any sample analyzed as a soil, other than TCLP, contains 50%-90% water, all data should be qualified as estimated (J). If a soil sample, other than TCLP, contains more than 90% water, all data should be qualified as unusable (R). ACTION: If samples were not iced (4°C) upon receipt at the laboratory, flag all positive results "J" and all non-detects "UJ". 2.0 Holding Times 2.1 Has the technical holding times, determined from date of sample receipt to date of extraction, been exceeded? _ jj _ Note: Samples may be analyzed for herbicide ester and acid. Check Laboratory SDG Narrative. Note: Aqueous samples must be extracted within 7 days. Extracts must be analyzed within 40 days following extraction. Soil/Concentrated Waste samples must be extracted within 14 days and extracts analyzed within 40 days following extraction. ACTION: If technical holding times are exceeded, flag all positive results and non-detects(U)as estimated ("J") and document in the narrative that holding times were exceeded. Samples extracted more than 28 days from sample receipt, either on the first analysis or Herbicides- 3 - ------- USEPA Region II Date:December 2010 SW846 Method 8151 A/Chlorinated Herbicides SOP: HW-17, Rev 3.1 YES NO N/A upon re-analysis, flag all positive results as Estimate ("J") and non-detects as unusable (R). 3.0 Surrogate Recovery (Form I I/Equivalent) 3.1 Are the Herbicide Surrogate Recovery Summaries (Form I I/Equivalent) present for each of the following matrices? a. Aqueous JJ _ b. Soil U _ 3.2 Are all the samples listed on the appropriate Surrogate Recovery Summary for each of the following matrices? a. Aqueous JJ _ b. Soil/Concentrated Waste JJ _ ACTION: Contact lab for explanation/resubmittals. If missing deliverables are unavailable, document effect in data assessments. 3.3 Were outliers marked correctly with an asterisk? JJ ACTION: Circle all outliers with red pencil. Note: recommend surrogate is 2,4-Dichlorophenylacetic acid (DCAA) 3.4 Did the laboratory provide their developed in-house QC limits/recoveries? U ACTION: If no, use 70 -130% recovery to qualify data ACTION: No qualification is done if the surrogate is diluted out. If recovery for the surrogate is below the QC limit, but above 10%, flag all results for that sample "J". If recovery is < 10%, qualify postive results "J" and flag non-detects "R". If recovery is above the QC limits limit, qualify positive values "J". Herbicides- 4 - ------- USEPA Region II SW846 Method 8151 A/Chlorinated Herbicides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A Note: In-house QC limits must be examined for reasonableness, e.g. 10-170% may be appropriate for analytes not present in the sample. Note: Matrix effect is indicated if the LCS data are within limits but surrogate data exceeds QC limits. 3.5 Were surrogate retention times (RT) within the windows established during the initial 5-point calibration analysis? jj _ _ ACTION: If the RT limits are not met, the analysis may be qualified unusable (R) for that sample on the basis of professional judgement. 3.6 Are there any transcription/calculation errors between raw data and Form I I/Equivalent? _ jj _ ACTION: If large errors exist, call lab for explanation/resubmittal. Make any necessary corrections and document effect in data assessments. 4.0 Matrix Spikes (Form Ill/Equivalent) 4.1 Is the Matrix Spike/Matrix Spike Duplicate Recovery Form (Form Ill/Equivalent) present? jj _ _ 4.2 Were matrix spikes analyzed at the required frequency for each of the following matrices? Note: At a minimum, analysis of at least one matrix spike and one duplicate unspiked sample or one matrix spike/matrix spike duplicate pair with each batch of up to 20 samples. a. Aqueous jj _ _ b. Soil/Concentrated Waste jj _ _ ACTION: If any matrix spike data are missing, take the action specified in 3.2 above. Herbicides- 5 - ------- USEPA Region II SW846 Method 8151 A/Chlorinated Herbicides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A 4.3 Did the laboratory provide their developed in-house QC limits/recoveries? U ACTION: If no, use 70 -130% recovery to qualify data ACTION: No action is taken on MS/MSD data alone. However, using informed professional judgement, the data reviewer may use the matrix spike results in conjunction with other QC criteria (e.g. LCS) to determine the need for qualification of the data. 5.0 Blanks (Form IV/Equivalent) 5.1 Is the Method Blank Summary (Form IV) present? jj _ _ 5.2 Frequency of Analysis: has a reagent/method blank been analyzed for each SDG or every 20 samples of similar matrix or concentration or each extraction batch, whichever is more frequent? jj _ _ ACTION: If any blank data are missing, take the action specified above in 3.2. If blank data is not available, reject (R) all associated positive data. However, using professional judgement, the data reviewer may substitute field blank data for missing method blank data. 5.3 Has a Herbicide instrument blank been analyzed at the beginning of every analytical sequence of 10 samples? jj _ _ ACTION: If any blank data are missing, call lab for explanation/resubmittals. If missing deliverables are unavailable, document the effect in data assessments. 5.4 Chromatography: review the blank raw data - chromatograms, quant reports or data system printouts. Is the chromatographic performance (baseline stability) for each instrument acceptable for Herbicides- 6 - ------- USEPA Region II Date:December 2010 SW846 Method 8151 A/Chlorinated Herbicides SOP: HW-17, Rev 3.1 YES NO N/A Herbicides? JJ _ ACTION: Use professional judgement to determine the effect on the data. Contamination NOTE: "Water blanks", "distilled water blanks" and "drilling water blanks" are validated like any other sample and are not used to qualify the data. Do not confuse them with the other QC blanks discussed below. Herbicides- 7 - ------- USEPA Region II SW846 Method 8151 A/Chlorinated Hericides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A 6.1 6.2 Do any method/instrument/reagent/cleanup blanks have positive results for Herbicides? When applied as described in table below, the contaminant concentration in the method blank is multiplied by the sample dilution factor and corrected for % moisture when necessary. Do any field/rinse blanks have positive Herbicides results? ACTION: Prepare a list of the samples associated with each of the contaminated blanks. (Attach a separate sheet) NOTE: All field blank results associated to a particular group of samples (may exceed one per case or one per day) may be used to qualify data. Blanks may not be qualified because of contamination in another blank. Field blanks must be qualified for surrogate, calibration, or any QC problems. ACTION: Follow the directions in the table below to qualify TCL results due to contamination. Use the largest value from all the associated blanks. Li U Sample cone > CRQL Sample cone < CRQL & Sample cone > CRQL but < 5x blank is < 5x blank value & > 5x blank value Flag sample result Report CRQL & with a "U": No qualification qualify "U" is needed NOTE: If gross blank contamination exists, all data in the associated samples should be qualified as unusable (R). 6.3 Are there field/rinse/equipment blanks associated with every sample? jj _ _ ACTION: For low level samples, note in data assessment that there is no associated field/rinse/equipment blank. Herbicides- 8 - ------- USEPA Region II SW846 Method 8151 A/Chlorinated Hericides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A Exception: samples taken from a drinking water tap do not have associated field blanks. 7.0 Calibration and GC Performance 7.1 Are the Gas Chromatograms and Data Systems printouts for both columns present for all samples, blanks, QC Check references, and matrix spikes? LJ _ _ ACTION: If no, take action specified in 3.2 above. 7.2 Are Form Vl/Equivalent present and complete for each column and each analytical sequence? LJ _ _ ACTION: If no, take action specified in 3.2 above. 7.3 Are there any transcription/calculation errors between raw data and Forms VI? _ LJ _ ACTION: If large errors exist, call lab for explanation/resubmittal, make necessary corrections and document effect in data assessments. 7.4 Were the retention time windows calculated using the average absolute retention time (at least three measurements) + three times the standard deviation of the absolute retention time, for each standard? (Refer to Method 8000A, section 7.5). LJ _ _ 7.5. Was a LCS check standard analyzed prior to environmental samples? LJ _ _ 7.5.1 If yes, was the surrogate recovery >50%? LJ _ _ 7.5.2 Was the LCS check standard re-extracted/re-analyzed, if surrogate recovery was <50%, or any one analyte was < 40%, or two analytes < 70% ? LJ _ _ Action: If No/' to any of the above, then qualify positive hits as estimated "J" and non-detects as rejected "R" in the original analysis of all samples in the associated analytical sequence. Herbicides- 9 - ------- USEPA Region II SW846 Method 8151 A/Chlorinated Hericides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A 7.6 Do all standard retention times, including each Herbicides in each level of Initial Calibration fall within the windows established during the initial calibration analytical sequence? (For Initial Calibration Standards, Form Vl/Equivalent - Herbicides -1). jj _ _ ACTION: If no, all samples in the entire analytical sequence are potentially affected. Check to see if the chromatograms contain peaks within an expanded window surrounding the expected retention times. If no peaks are found and the surrogate is visible, non- detects are valid. If peaks are present and cannot be identified through pattern recognition or using a revised RT window, qualify all positive results and non-detects as unusable (R). 7.7 Are the linearity criteria for the Initial Calibration analyses within limits for both columns? (% RSD must be < 20.0% for all analytes). jj ACTION: If no, qualify all associated positive results generated during the entire analytical sequence "J" and all non- detects "UJ". When RSD >90%, flag all non-detect results for that analyte R (unusable). 7.8 Are there any transcription/calculation errors between raw data and Form VII - Herbicides-2? _ jj ACTION: If large errors exists, call lab for explanation/resubmittal, make any necessary corrections and document effect in data assessments. 7.9 Is the resolution between any two adjacent peaks in the QC Reference Check Mixture > 60.0% for both columns? (Form Vl-Herbicides- 4) JJ Herbicides- 10 - ------- USEPA Region II SW846 Method 8151 A/Chlorinated Hericides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A ACTION: If no, positive results for compounds that were not adequately resolved should be qualified "J". Use professional judgement to determine if non-detects which elute in areas affected by co-eluting peaks should be qualified "N" as presumptive evidence of presence or unusable (R). 10 Is Form VII -Continuing Calibration present and complete for each analytical sequence for both ACTION: If no, take action as specified in 3.2 above. 11 Have all samples been injected within a 24 hr. period beginning with the injection of the first ACTION: If no, use professional judgement to determine the severity of the effect on the data and qualify accordingly. 12 Do all analyte retention times for the Mid-concentration Check standard (Form VII Herb-2) fall within the windows established by the initial calibration sequence? JJ ACTION: If no, beginning with the samples which followed the last in-control standard, check to see if the chromatograms contain peaks within an expanded window surrounding the expected retention times. If no peaks are found and the surrogates are visible, non-detects are valid. If peaks are present and cannot be identified through pattern recognition or using a revised RT window, qualify all positive results and non-detects as unusable (R). columns? U standard? U Herbicides- 11- ------- USEPA Region II SW846 Method 8151 A/Chlorinated Hericides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A 7.13 Are RPD values for all verification calibration standard compounds < 25.0% jj _ _ ACTION: The "associated samples" are those which followed the last in-control standard up to the next passing standard containing the analyte which failed the criteria. If %D is 25 -50% qualify as "J" If %D is 51-100% qualify as "NJ" If %D is >100% qualify as "R" If %D is >100% with visible interferences/qualify as "JN" 8.0 Analytical Sequence Check (Form VIM) 8.1 Is Form VIII present and complete for each column and each period of analyses? JJ ACTION: If no, take action specified in 3.2 above. 8.2 Was the proper analytical sequence followed for each initial calibration and subsequent analyses? (see SAS Client Request/section 8/paragraph 6) JJ ACTION: If no, use professional judgement to determine the severity of the effect on the data and qualify it accordingly. Generally, the effect is negligible unless the sequence was grossly altered or the calibration was also out of limits. 9.0 Herbicides Identification 9.1 Is Form X complete for every sample in which a Herbicide was detected? £J _ ACTION: If no, take action specified in 3.2 above. 9.2 Are there any transcription/calculation errors between raw data and Form X. _ JJ Herbicides- 12 - ------- USEPA Region II SW846 Method 8151 A/Chlorinated Hericides Date: December 2010 SOP: HW-17, Rev 3.1 ACTION: If large errors exist, call lab for explanation/resubmittal, make necessary corrections and note errors in data assessment. 9.3 Are retention times (RT) of sample compounds within the established RT windows for both columns? Was GC/MS confirmation provided instead of confirmation by a second dissimilar column? Action: Qualify as unusable (R) all positive results which were not confirmed by second GC column analysis or by GC/MS. Also qualify as unusable (R) all positive results not meeting RT window unless associated standard compounds show a similar RT shift. The reviewer should use professional judgement to assign an appropriate quantitation limit. 9.4 Is the percent difference (% D) calculated for the positive sample results on the two GC columns < 25.0%? ACTION: If the reviewer finds neither column shows interference for the positive hits, the data should be flagged as follows: % Difference Qualifier 25-50 % J 50-90 % JN > 90 % R NOTE: The lower of the two values is reported on Form I. If using professional judgement, the reviewer determines that the higher result was more acceptable, the reviewer should replace the value and indicate the reason for the change in the data assessment. YES NO N/A u _ _ u _ _ Herbicides- 13 - ------- USEPA Region II Date:December 2010 SW846 Method 8151 A/Chlorinated Hericides SOP: HW-17, Rev 3.1 YES NO N/A 9.5 Check chromatograms for false negatives. Were there any false negatives? _ jj _ ACTION: Use professional judgement to decide if the compound should be reported. 10.0 Compound Quantitation and Reported Detection Limits 10.1 Are there any transcription/calculation errors in Form I results? Check at least two positive values. Were any errors found? _ jj _ NOTE: The reviewer should use professional judgement to decide whether a much larger concentration obtained on one column versus the other indicates the presence of an interfering compound. If an interfering compound is indicated, the lower of the two values should be reported and qualified as presumptively present at an approximated quantity (NJ). This necessitates a determination of an estimated concentration on the confirmation column. The narrative should indicate the presence of interferences during the evaluation of the second column confirmation. 10.2 Are the CRQLs adjusted to reflect sample dilutions and, for soils, % moisture? JJ ACTION: If errors are large, call lab for explanation/resubmittal, make any necessary corrections and document effect in data assessments. ACTION: When a sample is analyzed at more than one dilution, the lowest CRQLs are used (unless a QC exceedance dictates the use of the higher CRQL data from the diluted sample analysis). Replace concentrations that exceed the calibration range in the original analysis by crossing out the "E" value on the original Form I and substituting it with data from the analysis of diluted sample. Specify which Form I is to be used, then draw a red "X" across the entire page of all Form I's that should not be used, including any in the summary package. Herbicides- 14 - ------- USEPA Region II SW846 Method 8151 A/Chlorinated Hericides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A ACTION: Quantitation limits affected by large, off-scale peaks should be qualified as unusable (R). If the interference is on-scale, the reviewer can provide an approximated quantitation limit (UJ) for each affected compound. 10.3 Have all data (Forms and associated chromatograms and quantitation reports) been submitted for original, diluted or re-extraction/re-analysis samples? JJ 11.0 Chromatogram Quality 11.1 Were baselines stable? jj _ 11.2 Were any electropositive displacement (negative peaks) or unusual peaks seen? _ JJ ACTION: Address comments under System Performance of data assessment. Explain use of professional judgement where used to qualify data. Herbicides- 15 - ------- USEPA Region II SW846 Method 8151 A/Chlorinated Hericides Date: December 2010 SOP: HW-17, Rev 3.1 YES NO N/A 12.0 Field Duplicates 12.1 Were any field duplicates submitted for Herbicides analysis? U _ _ Note: Check whether SAS Client Request required field duplicates. ACTION: Compare the reported results for field duplicates and calculate the relative percent difference. ACTION: Any gross variation between field duplicate results must be addressed in the reviewer narrative. However, if large differences exist, identification of field duplicates should be confirmed by contacting the sampler. Herbicides- 16 - ------- SOP HW-17 Revision #3.1 December 2010 Page 1 of 13 Validating Chlorinated Herbicides GC, SW-846, Method 8151A PREPARED BY: uk Russell Arnone, Che Iter Hazardou Peer Reviewed by: Concurred by: Approved by: s Waste Support Section LL )V^/ Muhammad Shaikh, Chemist Hazardous Waste Support Section fichael Wercado-,-Acting Chief Hazardous Waste StyppqftSection Robert Runyo?CChief y Hazardous Waste Support Branch Date: '2 / Date: |W zff/tr, Date: Date: / Annual Review Reviewed by: Date: Reviewed by: Date: ------- |