Environmental Radiation Data REPORT 149 J anuary-March 2012 United States Environmental Protection Agency Office of Radiation and Indoor Air ------- This page intentionally left blank 11 ------- Contents Page List of Tables v Preface vii Acknowledgments ix Data Reporting Conventions xi 1. Air Program 1 Airborne Particulates and Precipitation 1 Plutonium and Uranium in Airborne Particulates 17 2. Water Program 19 3. Milk Program 23 Pasteurized Milk 23 in ------- This page intentionally left blank iv ------- List of Tables Table Page 1 Reporting Units and Minimum Detectable Concentrations xiii 2 Gross Beta in Airborne Particulates: January 2012 2 3 Gross Beta in Airborne Particulates: February 2012 6 4 Gross Beta in Airborne Particulates: March 2012 10 5 Specific Gamma in Precipitation: January 2012 14 6 Specific Gamma in Precipitation: February 2012 15 7 Specific Gamma in Precipitation: March 2012 16 8 Tritium in Drinking Water: January-March 2012 20 9 Radionuclides in Pasteurized Milk: January-March 2012 24 v ------- This page intentionally left blank vi ------- Preface Environmental Radiation Data (ERD) contains data from the RadNet monitoring system (formerly ERAMS), which is operated by the Office of Radiation and Indoor Air's National Analytical Radiation Environmental Laboratory (NAREL) in Montgomery, Alabama. ERD is published in both hard-copy and electronic formats. Electronic reports are available online at http://www.epa.gov/narel. RadNet data are also available online in a searchable database at: http://www.epa.gov/enviro/facts/radnet The United States Environmental Protection Agency established RadNet in 1973 with an emphasis on identifying trends in the accumulation of long-lived radionuclides in the environ- ment. RadNet is comprised of a nationwide network of sampling stations that provide air particulate, precipitation, drinking water, and milk samples. Sampling locations are selected to provide population and geographic coverage for the United States. The radiation analyses performed on RadNet samples may include gross alpha and gross beta analysis, gamma analyses, and radionuclide-specific analyses for isotopes of uranium, plutonium, strontium, iodine, radium, and tritium. This monitoring effort also provides informa- tion on natural background levels and possible accidental releases into the environment. vii ------- This page intentionally left blank viii ------- Acknowledgments All sampling for the RadNet monitoring system (formerly ERAMS) is performed by volunteer collectors who are frequently members of health departments or related environmental agencies of their respective states. The National Analytical Radiation Environmental Laboratory (NAREL), on behalf of the U.S. Environmental Protection Agency, would like to acknowledge the time and effort of these volunteer collectors, who are so essential to the successful operation of RadNet. The efforts of the sample collectors are especially appreciated during times of emergency operation when sampling frequencies are increased and schedules are sometimes demanding. IX ------- This page intentionally left blank x ------- Data Reporting Conventions Every laboratory measurement involves uncertainty. When there is little or no radioactivity in a sample, one consequence of measurement uncertainty is the possibility of obtaining a measured value that is less than zero. Such a negative result occurs when random effects in the measure- ment process cause the measured value for the sample to be less than that of the blank or back- ground, which is subtracted from it. From April 1991 to December 1995, negative results were reported as "not detected" or "ND," and gamma analysis results that were less than their estimated measurement uncertainties were also reported as "ND." In January 1996, both of these practices were discontinued. Although negative activities are physically impossible, the inclusion of negative results in the report allows better statistical analysis of the data. Results of gamma analyses are still reported as "ND" when gamma-emitting radionuclides are not detected. Measurement Uncertainty Each measured value y is reported with an expanded uncertainty U=k uc(y), which is determined from the combined standard uncertainty uc(y) and the coverage factor k = 2. The interval from y- Utoy+ Uis estimated to have a level of confidence of approximately 95 %. Significant Figures Expanded uncertainties are reported to two significant figures. Measurement results are rounded to the corresponding number of decimal places. Detection Capability The minimum detectable concentrations (MDCs) for each radionuclide are shown in Table 1. The MDC is defined as the minimum concentration that gives a 95 % probability of detection when the detection criteria are chosen to give only a 5 % probability of false detection in a sample that is analyte-free. XI ------- This page intentionally left blank Xll ------- Table 1 Reporting Units and Minimum Detectable Concentrations for Radionuclide Analyses Radionuclide Media Reporting Unit IMinimum Detectable Concentration Gross Alpha Water pCi/L 2 Gross Beta Air pCi/m3 0.0015 Water pCi/L 2 Precipitation pCi/L 2 Tritium Water pCi/L 150 * Plutonium-23 8,23 9/240 Air aCi/m3 0.75 Water pCi/L 0.1 f Uranium-234,235,238 Air aCi/m3 0.75 Water pCi/L 0.1 Radium-226 Water pCi/L 0.02 Strontium-90 Milk pCi/L 2 Water pCi/L 1 t Iodine-131 Milk (gamma) pCi/L 4 Water (gamma) pCi/L 4 Water pCi/L 0.3 Cesium-137 Milk pCi/L 5 Water pCi/L 5 { Barium-140 Milk pCi/L 15 Water pCi/L 15 Potassium Milk g/L 0.06 Water g/L 0.06 Potassium-40 Water pCi/L 50 * The MDC for air is based on an assumed total sample volume of 120,000 m3. Measurement by alpha spectrometry includes combined activities of 239Pu and 240Pu, since the relative contributions of these two isotopes cannot be determined. ¦f The MDC for air is based on an assumed total sample volume of 120,000 m3. } Activity as of the day of counting. Xlll ------- This page intentionally left blank xiv ------- 1. Air Program Airborne Particulates and Precipitation Gross beta radioactivity measurements and certain specific analyses are performed on air partic- ulates and precipitation samples as indicator measurements in assessing the general (national) impact of all contributing sources on environmental levels of radiation. Continuous air samplers collect airborne particulates at field stations representing wide geographic coverage throughout the United States. Filters (10 cm diameter synthetic fiber) from air samplers are changed routinely, and generally field measurements are made with a dual-phosphor scintillation counter at least 5 hours after 222 collection to allow Rn progeny to decay. Field estimates are reported to appropriate EPA officials by telephone or mail depending on the activity levels found; however, as of the first quarter of 2012, NAREL no longer reports field estimates in Environmental Radiation Data. The filters are sent to NAREL for more sensitive analysis in a gas proportional counter. Gamma scans are performed on all filters showing gross beta activity greater than 1 pCi/m3. All stations routinely submit precipitation samples as rainfall, snow, or sleet occurs. The precip- itation samples are composited at NAREL into single monthly samples for each station. Each month that precipitation occurs, an aliquant of the composited sample is analyzed for gamma- emitting radionuclides. NAREL discontinued gross beta analysis of precipitation in January 2010 and discontinued tritium analysis of precipitation in January 2012. 1 ------- Table 2 Gross Beta in Airborne Particulates January 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) AK: Anchorage 5 0.007 0.002 0.004 AK: Fairbanks 6 0.021 0.011 0.017 AK: Juneau 7 0.007 0.001 0.003 AL: Birmingham 9 0.013 0.006 0.010 AL: Montgomery/408 9 0.018 0.009 0.012 AR: Fort Smith 4 0.029 0.011 0.016 AR: Little Rock 6 0.019 0.005 0.009 AZ: Phoenix 8 0.025 0.007 0.016 AZ: Phoenix/956 8 0.021 0.009 0.014 AZ: Tucson 7 0.015 0.006 0.009 AZ: Yuma 3 0.017 0.006 0.012 CA: Anaheim 7 0.016 0.005 0.011 CA: Bakersfield 6 0.093 0.009 0.037 CA: Eureka 2 0.004 0.002 0.003 CA: Fresno 2 0.012 0.012 0.012 CA: Los Angeles 3 0.010 0.007 0.009 CA: Richmond 5 0.021 0.003 0.012 CA: Riverside 8 0.013 0.004 0.009 CA: Sacramento 9 0.021 0.004 0.011 CA: San Bernardino Cty. 7 0.014 0.004 0.010 CA: San Diego 4 0.010 0.004 0.007 CA: San Francisco 9 0.014 0.001 0.006 CA: San Jose 7 0.021 0.002 0.008 CO: Denver 8 0.012 0.005 0.009 CO: Grand Junction 6 0.021 0.009 0.016 CT: Hartford 9 0.010 0.004 0.008 DC: Washington 9 0.020 0.005 0.009 DE: Dover 6 0.015 0.005 0.007 FL: Jacksonville 9 0.009 0.004 0.006 FL: Miami 3 0.005 0.004 0.005 FL: Orlando 9 0.010 0.004 0.007 FL: Tallahassee 3 0.011 0.008 0.009 FL: Tampa 6 0.009 0.005 0.007 GA: Atlanta 2 0.008 0.007 0.008 GA: Augusta 6 0.005 0.004 0.004 HI: Hilo 9 0.004 0.002 0.003 HI: Honolulu 9 0.003 0.002 0.002 IA: Des Moines 6 0.024 0.005 0.013 2 ------- Table 2 (continued) Gross Beta in Airborne Particulates January 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) IA: Mason City 6 0.018 0.006 0.012 ID: Idaho Falls 7 0.015 0.004 0.009 IL: Aurora 9 0.031 0.006 0.014 IL: Chicago 9 0.030 0.006 0.011 IN: Fort Wayne 1 0.011 0.011 0.011 IN: Indianapolis 8 0.025 0.007 0.012 KS: Kansas City 9 0.017 0.005 0.009 KS: Topeka 8 0.028 0.005 0.011 KS: Wichita 7 0.022 0.005 0.010 KY: Lexington 6 0.021 0.010 0.014 KY: Louisville 8 0.023 0.005 0.009 LA: Baton Rouge 9 0.008 0.003 0.005 LA: Shreveport 7 0.010 0.004 0.007 MA: Boston 9 0.006 0.003 0.005 MA: Worcester 7 0.014 0.006 0.009 MD: Baltimore 9 0.024 0.004 0.010 ME: Orono 3 0.010 0.007 0.009 ME: Portland 3 0.006 0.004 0.006 MI: Detroit 8 0.016 0.006 0.009 MI: Grand Rapids 6 0.017 0.007 0.012 MI: Lansing 9 0.041 0.016 0.027 MN: Duluth 4 0.018 0.006 0.009 MN: St. Paul 5 0.012 0.006 0.009 MO: Jefferson City 8 0.019 0.003 0.008 MO: Springfield 7 0.019 0.005 0.011 MO: St. Louis 2 0.013 0.011 0.012 MS: Jackson/Deq 9 0.013 0.004 0.008 MT: Billings 2 0.008 0.005 0.007 NC: Charlotte 8 0.009 0.006 0.007 NC: Raleigh 5 0.009 0.003 0.006 NC: Wilmington 4 0.007 0.005 0.006 ND: Bismarck 8 0.020 0.003 0.009 NE: Kearney 7 0.019 0.003 0.008 NE: Lincoln 7 0.022 0.004 0.012 NE: Omaha 3 0.012 0.007 0.009 NH: Concord 4 0.007 0.006 0.006 NJ: Edison 4 0.005 0.004 0.005 NJ: Trenton 9 0.018 0.007 0.010 3 ------- Table 2 (continued) Gross Beta in Airborne Particulates January 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) NM: Albuquerque 4 0.013 0.005 0.009 NM: Carlsbad 6 0.014 0.008 0.010 NM: Navajo Lake St Park 5 0.020 0.009 0.013 NV: Las Vegas/913 3 0.012 0.006 0.010 NV: Reno 7 0.024 0.003 0.011 NY: Albany 9 0.015 0.005 0.010 NY: Lockport 9 0.013 0.005 0.007 NY: New York City 4 0.010 0.007 0.008 NY: Rochester 3 0.005 0.003 0.004 NY: Syracuse 1 0.007 0.007 0.007 NY: Yaphank 7 0.006 0.004 0.005 OH: Cincinnati 9 0.022 0.004 0.010 OH: Cleveland 8 0.021 0.004 0.009 OH: Painesville 7 0.013 0.006 0.009 OH: Toledo 8 0.025 0.009 0.013 OK: Oklahoma City 9 0.016 0.004 0.008 OK: Tulsa 8 0.020 0.004 0.009 OR: Corvallis 7 0.004 0.001 0.003 OR: Portland 9 0.004 0.001 0.002 PA: Harrisburg 7 0.009 0.004 0.006 PA: Philadelphia 4 0.011 0.005 0.007 PA: Pittsburgh 6 0.014 0.006 0.009 PR: San Juan 9 0.003 0.001 0.002 RI: Providence 4 0.008 0.003 0.005 SC: Barnwell 1 0.009 0.009 0.009 SC: Columbia 3 0.013 0.011 0.012 SD: Pierre 9 0.020 0.003 0.009 SD: Rapid City 7 0.016 0.004 0.008 TN: Knoxville 7 0.012 0.005 0.007 TN: Memphis 4 0.021 0.007 0.011 TN: Nashville 4 0.009 0.007 0.008 TN: Oak Ridge/Bethel 7 0.018 0.007 0.011 TN: Oak Ridge/K25 7 0.018 0.008 0.012 TN: Oak Ridge/Melton 7 0.021 0.009 0.014 TN: Oak Ridgc/Y12 E 7 0.019 0.008 0.012 TN: Oak Ridge/Y12 W 7 0.019 0.008 0.012 TX: Austin 3 0.011 0.009 0.010 TX: Dallas 8 0.014 0.005 0.009 4 ------- Table 2 (continued) Gross Beta in Airborne Particulates January 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) TX: El Paso 7 0.022 0.009 0.015 TX: Ft. Worth 4 0.010 0.008 0.009 TX: Harlingen 7 0.010 0.006 0.008 TX: Houston 9 0.012 0.004 0.006 TX: Laredo 3 0.022 0.007 0.013 TX: Lubbock 5 0.009 0.001 0.006 TX: San Angelo 6 0.015 0.006 0.008 TX: San Antonio 9 0.017 0.005 0.010 UT: Salt Lake City 8 0.022 0.004 0.011 VA: Harrisonburg 8 0.011 0.006 0.008 VA: Lynchburg 9 0.010 0.007 0.008 VA: Richmond 3 0.015 0.006 0.010 VA: Virginia Beach 8 0.007 0.003 0.005 VT: Burlington 9 0.009 0.005 0.008 WA: Olympia 5 0.004 0.002 0.003 WA: Richland 7 0.010 0.003 0.006 WA: Seattle 4 0.003 0.001 0.002 WA: Spokane 7 0.009 0.003 0.006 WI: Madison 9 0.027 0.006 0.012 WI: Milwaukee 7 0.020 0.005 0.010 WV: Charleston 6 0.027 0.007 0.013 5 ------- Table 3 Gross Beta in Airborne Particulates February 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) AK: Anchorage 6 0.008 0.001 0.003 AK: Fairbanks 6 0.009 0.002 0.005 AK: Juneau 7 0.004 0.001 0.002 AL: Birmingham 8 0.012 0.006 0.010 AL: Montgomery/408 8 0.018 0.008 0.012 AR: Fort Smith 4 0.015 0.009 0.012 AR: Little Rock 7 0.011 0.004 0.008 AZ: Phoenix 7 0.022 0.006 0.016 AZ: Phoenix/956 8 0.017 0.005 0.012 AZ: Tucson 8 0.013 0.005 0.010 AZ: Yuma 1 0.004 0.004 0.004 CA: Bakersfield 7 0.033 0.004 0.015 CA: Fresno 5 0.017 0.004 0.010 CA: Los Angeles 4 0.018 0.007 0.013 CA: Richmond 4 0.010 0.003 0.006 CA: Riverside 7 0.012 0.004 0.009 CA: Sacramento 8 0.015 0.002 0.006 CA: San Bernardino Cty. 9 0.016 0.004 0.010 CA: San Diego 9 0.018 0.003 0.009 CA: San Francisco 8 0.010 0.002 0.004 CA: San Jose 8 0.022 0.002 0.007 CO: Denver 8 0.028 0.004 0.016 CO: Grand Junction 5 0.018 0.005 0.012 CT: Hartford 7 0.010 0.005 0.007 DC: Washington 8 0.013 0.008 0.009 DE: Dover 7 0.009 0.006 0.007 FL: Jacksonville 8 0.009 0.004 0.007 FL: Miami 2 0.004 0.003 0.004 FL: Orlando 8 0.009 0.006 0.007 FL: Tallahassee 4 0.012 0.006 0.009 FL: Tampa 7 0.008 0.004 0.007 GA: Atlanta 2 0.007 0.006 0.006 GA: Augusta 6 0.011 0.005 0.008 HI: Hilo 8 0.004 0.002 0.003 HI: Honolulu 8 0.003 0.002 0.002 IA: Des Moines 7 0.014 0.006 0.010 IA: Mason City 7 0.012 0.007 0.010 ID: Idaho Falls 8 0.022 0.003 0.010 6 ------- Table 3 (continued) Gross Beta in Airborne Particulates February 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) IL: Aurora 8 0.015 0.009 0.012 IL: Chicago 8 0.012 0.007 0.010 IN: Indianapolis 8 0.012 0.008 0.010 KS: Kansas City 7 0.018 0.002 0.008 KS: Topeka 8 0.019 0.006 0.011 KS: Wichita 7 0.019 0.004 0.011 KY: Lexington 8 0.017 0.011 0.014 KY: Louisville 7 0.010 0.005 0.007 LA: Baton Rouge 8 0.007 0.003 0.005 LA: Shreveport 8 0.011 0.003 0.006 MA: Boston 8 0.008 0.005 0.006 MA: Worcester 7 0.014 0.009 0.010 MD: Baltimore 1 0.010 0.010 0.010 ME: Orono 4 0.010 0.008 0.009 ME: Portland 7 0.015 0.005 0.008 MI: Bay City 48708 4 0.011 0.008 0.009 MI: Detroit 8 0.011 0.007 0.009 MI: Grand Rapids 7 0.013 0.007 0.010 MI: Lansing 8 0.037 0.020 0.027 MN: Duluth 4 0.012 0.007 0.009 MN: St. Paul 4 0.012 0.007 0.010 MO: Jefferson City 8 0.013 0.003 0.007 MO: Springfield 6 0.019 0.005 0.010 MO: St. Louis 5 0.011 0.007 0.008 MS: Jackson/Deq 8 0.013 0.005 0.009 MT: Billings 3 0.020 0.006 0.013 NC: Charlotte 8 0.010 0.006 0.008 NC: Raleigh 4 0.008 0.005 0.007 NC: Wilmington 5 0.008 0.006 0.006 ND: Bismarck 5 0.014 0.009 0.011 NE: Kearney 8 0.012 0.003 0.008 NE: Lincoln 8 0.015 0.004 0.009 NE: Omaha 2 0.008 0.007 0.007 NH: Concord 7 0.010 0.006 0.008 NJ: Edison 7 0.008 0.004 0.006 NJ: Trenton 6 0.012 0.010 0.011 NM: Albuquerque 4 0.012 0.007 0.010 NM: Carlsbad 4 0.022 0.009 0.013 7 ------- Table 3 (continued) Gross Beta in Airborne Particulates February 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) NM: Navajo Lake St Park 4 0.019 0.006 0.013 NV: Las Vegas/913 8 0.020 0.004 0.011 NV: Reno 8 0.024 0.005 0.011 NY: Albany 7 0.014 0.010 0.011 NY: Lockport 6 0.009 0.006 0.008 NY: New York City 5 0.009 0.007 0.008 NY: Yaphank 8 0.008 0.004 0.005 OH: Cincinnati 7 0.014 0.006 0.009 OH: Cleveland 8 0.011 0.006 0.008 OH: Painesville 8 0.013 0.008 0.011 OH: Toledo 7 0.015 0.010 0.012 OK: Oklahoma City 8 0.016 0.004 0.009 OK: Tulsa 7 0.025 0.005 0.011 OR: Corvallis 8 0.011 0.001 0.004 OR: Portland 8 0.009 0.001 0.004 PA: Philadelphia 4 0.008 0.006 0.006 PA: Pittsburgh 5 0.011 0.009 0.010 PR: San Juan 7 0.003 0.002 0.002 RI: Providence 4 0.009 0.006 0.007 SC: Barnwell 2 0.010 0.008 0.009 SC: Columbia 3 0.011 0.005 0.009 SD: Pierre 8 0.012 0.003 0.008 SD: Rapid City 6 0.016 0.006 0.011 TN: Knoxville 5 0.008 0.007 0.008 TN: Memphis 4 0.014 0.007 0.010 TN: Nashville 7 0.012 0.007 0.008 TN: Oak Ridge/Bethel 7 0.013 0.008 0.011 TN: Oak Ridge/K25 7 0.014 0.008 0.011 TN: Oak Ridge/Melton 7 0.015 0.007 0.011 TN: Oak Ridgc/Y12 E 7 0.016 0.009 0.012 TN: Oak Ridge/Y12 W 7 0.015 0.007 0.012 TX: Austin 3 0.011 0.008 0.010 TX: Dallas 7 0.015 0.003 0.010 TX: El Paso 2 0.025 0.015 0.020 TX: Ft. Worth 5 0.018 0.007 0.011 TX: Harlingen 7 0.012 0.005 0.009 TX: Houston 5 0.008 0.004 0.006 TX: Laredo 7 0.013 0.005 0.009 8 ------- Table 3 (continued) Gross Beta in Airborne Particulates February 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) TX: Lubbock 3 0.023 0.003 0.014 TX: San Angelo 8 0.012 0.003 0.008 TX: San Antonio 8 0.011 0.005 0.009 UT: Salt Lake City 8 0.034 0.005 0.015 VA: Harrisonburg 8 0.011 0.007 0.009 VA: Lynchburg 8 0.012 0.008 0.010 VA: Richmond 8 0.009 0.006 0.008 VA: Virginia Beach 7 0.008 0.005 0.006 VT: Burlington 8 0.009 0.006 0.008 WA: Olympia 7 0.008 0.001 0.003 WA: Richland 8 0.032 0.002 0.009 WA: Seattle 4 0.005 0.001 0.002 WA: Spokane 8 0.012 0.002 0.006 WI: Madison 8 0.014 0.007 0.012 WI: Milwaukee 7 0.011 0.006 0.009 WV: Charleston 6 0.012 0.007 0.009 9 ------- Table 4 Gross Beta in Airborne Particulates March 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) AK: Anchorage 8 0.010 0.003 0.006 AK: Fairbanks 4 0.011 0.007 0.010 AK: Juneau 7 0.004 0.001 0.002 AL: Birmingham 8 0.011 0.005 0.008 AL: Montgomery/408 9 0.013 0.006 0.009 AR: Fort Smith 4 0.007 0.005 0.006 AR: Little Rock 7 0.008 0.005 0.007 AZ: Phoenix 9 0.019 0.009 0.013 AZ: Phoenix/956 8 0.023 0.006 0.013 AZ: Tucson 9 0.013 0.005 0.009 AZ: Yuma 2 0.009 0.006 0.008 CA: Anaheim 8 0.012 0.003 0.007 CA: Bakersfield 6 0.013 0.003 0.007 CA: Eureka 2 0.003 0.002 0.003 CA: Fresno 2 0.006 0.004 0.005 CA: Los Angeles 4 0.011 0.005 0.007 CA: Richmond 4 0.006 0.002 0.004 CA: Riverside 8 0.011 0.004 0.006 CA: Sacramento 9 0.007 0.002 0.004 CA: San Bernardino Cty. 8 0.014 0.004 0.008 CA: San Diego 6 0.007 0.003 0.005 CA: San Francisco 9 0.003 0.001 0.002 CA: San Jose 8 0.006 0.002 0.003 CO: Denver 7 0.015 0.008 0.011 CO: Grand Junction 6 0.014 0.004 0.009 CT: Hartford 9 0.007 0.004 0.006 DC: Washington 9 0.010 0.006 0.008 DE: Dover 6 0.008 0.005 0.007 FL: Jacksonville 9 0.007 0.003 0.005 FL: Miami 4 0.003 0.002 0.003 FL: Orlando 9 0.008 0.003 0.006 FL: Tallahassee 4 0.008 0.005 0.007 FL: Tampa 5 0.007 0.005 0.005 GA: Atlanta 4 0.009 0.007 0.008 GA: Augusta 7 0.012 0.005 0.008 HI: Hilo 9 0.005 0.002 0.003 HI: Honolulu 9 0.006 0.001 0.003 IA: Des Moines 7 0.014 0.005 0.009 10 ------- Table 4 (continued) Gross Beta in Airborne Particulates March 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) IA: Mason City 5 0.012 0.004 0.008 ID: Idaho Falls 9 0.014 0.004 0.007 IL: Aurora 9 0.012 0.006 0.010 IL: Chicago 8 0.010 0.006 0.008 IN: Fort Wayne 1 0.009 0.009 0.009 IN: Indianapolis 9 0.011 0.007 0.009 KS: Kansas City 7 0.009 0.004 0.006 KS: Topeka 9 0.011 0.006 0.009 KS: Wichita 7 0.016 0.006 0.009 KY: Lexington 8 0.017 0.010 0.012 KY: Louisville 8 0.008 0.006 0.007 LA: Baton Rouge 9 0.005 0.003 0.004 LA: Shreveport 7 0.005 0.003 0.004 MA: Boston 9 0.007 0.005 0.006 MA: Worcester 7 0.013 0.006 0.010 ME: Orono 5 0.010 0.005 0.008 ME: Portland 8 0.009 0.006 0.007 MI: Bay City 48708 8 0.011 0.006 0.008 MI: Detroit 9 0.011 0.006 0.009 MI: Grand Rapids 7 0.010 0.008 0.009 MI: Lansing 9 0.030 0.013 0.021 MN: Duluth 5 0.011 0.005 0.007 MN: St. Paul 4 0.009 0.006 0.008 MO: Jefferson City 9 0.010 0.004 0.006 MO: Springfield 7 0.011 0.004 0.007 MO: St. Louis 2 0.009 0.007 0.008 MS: Jackson/Deq 9 0.010 0.005 0.007 MT: Billings 4 0.010 0.007 0.008 NC: Charlotte 9 0.009 0.005 0.007 NC: Raleigh 3 0.007 0.005 0.006 NC: Wilmington 4 0.006 0.005 0.006 ND: Bismarck 7 0.015 0.005 0.009 NE: Kearney 7 0.010 0.006 0.008 NE: Lincoln 9 0.012 0.006 0.009 NE: Omaha 4 0.011 0.008 0.010 NH: Concord 6 0.008 0.006 0.007 NJ: Edison 9 0.006 0.002 0.005 NJ: Trenton 7 0.011 0.007 0.009 11 ------- Table 4 (continued) Gross Beta in Airborne Particulates March 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) NM: Carlsbad 5 0.014 0.006 0.010 NM: Navajo Lake St Park 4 0.015 0.007 0.010 NV: Las Vegas/913 2 0.005 0.004 0.005 NV: Reno 9 0.013 0.001 0.007 NY: Albany 7 0.014 0.010 0.012 NY: Lockport 8 0.009 0.006 0.007 NY: New York City 4 0.008 0.006 0.007 NY: Rochester 6 0.011 0.006 0.009 NY: Yaphank 9 0.006 0.004 0.005 OH: Cincinnati 9 0.009 0.006 0.008 OH: Cleveland 6 0.009 0.006 0.007 OH: Painesville 7 0.010 0.006 0.008 OH: Toledo 8 0.013 0.008 0.011 OK: Oklahoma City 9 0.008 0.004 0.006 OK: Tulsa 4 0.007 0.004 0.006 OR: Corvallis 9 0.003 0.001 0.002 OR: Portland 9 0.004 0.002 0.002 PA: Philadelphia 5 0.008 0.006 0.007 PA: Pittsburgh 4 0.010 0.008 0.009 PR: San Juan 9 0.009 0.002 0.004 RI: Providence 1 0.007 0.007 0.007 SC: Barnwell 2 0.011 0.007 0.009 SC: Columbia 4 0.011 0.007 0.009 SD: Pierre 8 0.011 0.006 0.009 SD: Rapid City 6 0.012 0.008 0.009 TN: Knoxville 8 0.019 0.006 0.010 TN: Memphis 4 0.008 0.006 0.007 TN: Nashville 7 0.010 0.006 0.007 TN: Oak Ridge/Bethel 9 0.010 0.006 0.008 TN: Oak Ridge/K25 9 0.011 0.006 0.009 TN: Oak Ridge/Melton 9 0.011 0.007 0.009 TN: Oak Ridgc/Y12 E 9 0.012 0.007 0.009 TN: Oak Ridge/Y12 W 9 0.012 0.006 0.009 TX: Austin 3 0.013 0.006 0.008 TX: Dallas 9 0.011 0.004 0.007 TX: El Paso 6 0.017 0.010 0.014 TX: Ft. Worth 8 0.008 0.004 0.006 TX: Harlingen 4 0.007 0.004 0.006 12 ------- Table 4 (continued) Gross Beta in Airborne Particulates March 2012 NAREL Lab Number Measurement of Max IMin Avg Location Samples (pCi/m3) TX: Houston 8 0.013 0.005 0.008 TX: Laredo 8 0.011 0.005 0.008 TX: San Angelo 6 0.009 0.004 0.006 TX: San Antonio 9 0.012 0.004 0.007 UT: Salt Lake City 9 0.020 0.005 0.009 VA: Harrisonburg 9 0.013 0.005 0.009 VA: Lynchburg 9 0.013 0.007 0.009 VA: Richmond 8 0.008 0.005 0.007 VA: Virginia Beach 7 0.007 0.005 0.006 VT: Burlington 9 0.013 0.006 0.009 WA: Olympia 8 0.004 0.001 0.002 WA: Richland 9 0.006 0.002 0.004 WA: Seattle 5 0.003 0.002 0.002 WA: Spokane 8 0.007 0.002 0.004 WI: Madison 9 0.012 0.007 0.009 WI: Milwaukee 7 0.010 0.004 0.008 WV: Charleston 6 0.009 0.007 0.008 13 ------- Table 5 Specific Gamma in Precipitation January 2012 Location Nuclide pCi/L ± 2 M AL: Montgomery/408 ND AR: Little Rock ND CA: Richmond Be-7 300 260 Cs-134 33.2 7.1 Cs-137 56 10 Tl-208 10.1 8.1 K-40 320 280 Pb-212 62 43 CO: Denver Pb-211 25 22 Pb-212 2.8 2.5 CT: Hartford ND FL: Jacksonville ND GA: Atlanta ND HI: Honolulu ND ID: Idaho Falls ND MA: Boston K-40 17 13 MN: St. Paul ND NC: Charlotte Be-7 102 42 NC: Wilmington ND NY: Albany ND NY: Yap hank Be-7 44 39 OH: Painesville ND OR: Portland ND PA: Harrisburg ND TN: Knoxville Pb-212 2.1 2.0 TN: Nashville K-40 12 12 TN: Oak Ridge/K25 K-40 17 12 TN: Oak Ridge/Melton Be-7 35 24 Tl-208 0.67 0.65 TN: Oak Ridgc/Y12 E ND TX: Austin Ra-224 29 22 TX: El Paso K-40 13 12 UT: Salt Lake City Pb-212 3.6 2.5 VA: Lynchburg ND WA: Olympia Pb-212 2.1 2.0 14 ------- Table 6 Specific Gamma in Precipitation February 2012 Location Nuclide pCi/L ± 2 M AL: Montgomery/408 Be-7 40 31 AR: Little Rock ND CA: Richmond Cs-134 2.7 1.3 Cs-137 5.6 1.4 CO: Denver Tl-208 1.4 1.3 CT: Hartford Be-7 80 26 Pb-212 1.8 1.3 Tl-208 1.59 0.69 FL: Jacksonville K-40 21 13 GA: Atlanta ND HI: Honolulu ND ID: Idaho Falls K-40 14.4 8.7 Tl-208 0.79 0.63 MA: Boston Be-7 101 33 K-40 13 12 Pb-212 2.3 2.3 NC: Charlotte K-40 18 12 Pb-212 2.5 2.1 NC: Wilmington Be-7 29 28 K-40 21 13 NY: Albany Be-7 63 49 NY: Yap hank Be-7 49 28 K-40 14 13 OR: Portland Tl-208 1.32 0.94 TN: Knoxville ND TN: Nashville Be-7 105 41 K-40 21 12 TN: Oak Ridge/K25 Be-7 95 41 Pb-212 2.9 2.4 TN: Oak Ridge/Melton Be-7 112 39 K-40 23 12 Pb-212 2.6 2.5 TN: Oak Ridgc/Y12 E Be-7 47 33 TX: Austin K-40 15 13 UT: Salt Lake City ND VA: Lynchburg K-40 14 14 Pb-212 2.4 2.0 Ra-228 4.4 4.3 WA: Olympia Tl-208 1.6 1.1 15 ------- Table 7 Specific Gamma in Precipitation March 2012 Location Nuclide pCi/L ± 2 M AL: Montgomery/408 Be-7 36 30 Tl-208 1.5 1.3 AR: Little Rock ND CA: Richmond Be-7 30 21 Cs-137 1.17 0.92 CT: Hartford Be-7 40 25 FL: Jacksonville Ra-228 2.4 2.2 GA: Atlanta Be-7 78 32 HI: Honolulu ND ID: Idaho Falls Be-7 41 32 KS: Kansas City Be-7 41 30 MA: Boston Be-7 34 29 Tl-208 1.5 1.2 MN: St. Paul ND MN: Welch/510 ND NC: Charlotte Be-7 32 29 NC: Wilmington K-40 11 11 NH: Concord ND NY: Albany Be-7 64 29 NY: Yap hank Be-7 23 18 OH: Painesville Be-7 55 27 Pb-212 2.7 2.3 Tl-208 0.95 0.94 OR: Portland ND PA: Harrisburg ND TN: Knoxville Tl-208 2.1 1.2 TN: Nashville ND TN: Oak Ridge/K25 Pb-212 3.3 2.1 TN: Oak Ridge/Melton Be-7 37 30 K-40 15 12 TN: Oak Ridge/Y12 E Be-7 33 29 Pb-212 3.8 2.6 Tl-208 1.6 1.3 TX: Austin ND UT: Salt Lake City ND VA: Lynchburg K-40 11 10 Tl-208 1.2 1.0 WA: Olympia Tl-208 1.9 1.3 16 ------- Plutonium and Uranium in Airborne Particulates Environmental radiation levels of plutonium and uranium are determined by the analysis of annually composited samples (air filters) collected from the airborne particulate samplers. Plutonium and uranium results are published in the ERD for the third quarter of the following year. Concentrations of plutonium-238, combined plutonium-239 and 240, and uranium-234, 235, and 238 are determined by alpha-particle spectrometry following chemical separation. The volume of air represented by the annual composite typically ranges from 120,000 to 500,000 cubic meters. 17 ------- This page intentionally left blank 18 ------- 2. Drinking Water Program The RadNet drinking water program provides data on radionuclide concentrations in the nation's drinking water supplies. Sampling sites are either major population centers or selected nuclear facility environs. Drinking water data are used to assess trends and anomalies in concentrations. The analysis scheme for RadNet samples is similar to that of EPA's "National Interim Primary Drinking Water Regulations." The analyses include (a) tritium on a quarterly basis; (b) gross alpha, gross beta, and gamma on annual composites; (c) radium-226 if the gross alpha exceeds 2 pCi/L and radium-228 if the radium-226 falls between 3 and 5 pCi/L on annual composites; (d) iodine-131 on one quarterly sample per year for each station; (e) plutonium-238, combined plutonium-239 and 240, and uranium-234, 235, and 238 for stations that demonstrate gross alpha levels greater than 2 pCi/L on annual composites; and (f) strontium-90 on one-fourth of the annual composites on a four year rotating schedule. Composite results are published in the ERD for the third quarter of the following year. RadNet drinking water data should not be used to monitor compliance with drinking water regu- lations or for comparisons to those data since different procedures for collection and analysis may be used. 19 ------- Table 8 Tritium in Drinking Water January-March 2012 Date 3H Location Collected pCi/L ± 2u AK: Fairbanks 01/03/12 -27 77 AL: Dothan 01/05/12 -2 77 AL: Montgomery 01/30/12 -58 77 AL: Muscle Shoals 01/12/12 -18 90 AL: Scottsboro 01/11/12 -47 87 AR: Little Rock 01/06/12 -16 77 CA: Richmond 01/06/12 9 78 CO: Denver 01/06/12 -7 77 CT: Hartford 01/04/12 -23 77 DE: Dover 01/09/12 -41 88 FL: Tampa 01/03/12 2 78 GA: Baxley 03/13/12 -23 78 GA: Savannah 01/03/12 -52 75 HI: Honolulu 03/09/12 66 75 IA: Cedar Rapids 01/04/12 -36 91 ID: Boise 01/03/12 -11 77 ID: Idaho Falls 01/06/12 134 96 IL: Morris 03/20/12 7 79 KS: Topeka 01/26/12 2 79 LA: New Orleans 03/29/12 80 76 MD: Baltimore 01/09/12 -12 89 MD: Conowingo 01/03/12 -45 78 MI: Detroit 02/27/12 57 81 MN: St. Paul 01/10/12 -20 89 MN: Welch 01/10/12 -35 88 MO: Jefferson City 01/06/12 -18 76 MS: Jackson 01/11/12 -22 90 MS: Port Gibson 01/11/12 19 96 ND: Bismarck 02/15/12 -40 77 NE: Lincoln 01/12/12 -61 87 NH: Concord 02/14/12 -7 78 NJ: Trenton 01/30/12 20 80 NJ: Waretown 01/30/12 18 80 NY: Albany 01/26/12 -14 89 NY: New York City 01/09/12 45 92 NY: Niagara Falls 01/03/12 16 79 NY: Syracuse 01/31/12 18 81 OH: Cincinnati 01/03/12 56 80 OH: Columbus 02/03/12 -25 78 OH: E. Liverpool 02/01/12 -34 77 20 ------- Table 8 (continued) Tritium in Drinking Water January-March 2012 Date 3H Location Collected pCi/L ± 2u OH: Painesville 02/15/12 72 82 OH: Toledo 02/08/12 -7 79 OR: Portland 03/29/12 94 76 PA: Columbia 01/03/12 13 79 PA: Harrisburg 01/03/12 -10 90 PA: Pittsburgh 01/31/12 -29 78 RI: Providence 01/03/12 -38 76 SC: Barnwell 01/25/12 -16 89 SC: Columbia 01/17/12 10 90 SC: Jenkinsville 01/11/12 22 91 SC: Seneca 01/16/12 0 90 TN: Knoxville 01/04/12 -45 77 TN: Oak Ridge/#360 01/05/12 25 79 TN: OakRidge/#371 01/05/12 -34 76 TN: Oak Ridge/#4442 01/05/12 23 79 TN: Oak Ridge/#768 01/05/12 -59 75 TN: Oak Ridge/#772 01/05/12 -12 89 TX: Austin 01/26/12 27 80 VA: Ashland 02/17/12 3220 220 VA: Lynchburg 01/05/12 13 79 WA: Richland 01/10/12 -2 90 WI: Madison 01/05/12 38 79 21 ------- This page intentionally left blank 22 ------- 3. Milk Program Pasteurized Milk Milk is a reliable indicator of the general population's intake of certain radionuclides since it is consumed fresh by a large segment of the population and can contain several of the biologically significant radionuclides that result from environmental releases from nuclear activities. A primary function of this program is to obtain reliable monitoring data relative to current radio- nuclide concentrations and determine any long-term trends. Milk samples are collected quarterly at each of the sampling sites. The samples are analyzed for gamma-emitting nuclides, including iodine-131, barium-140, cesium-137, and potassium-40. Total potassium concentrations in g/L are determined from potassium-40 activities assuming natural isotopic abundances. During the third quarter collection, one-fourth of the samples are also analyzed for strontium-90 on a four year rotating schedule. 23 ------- Table 9 Radionuclides in Pasteurized Milk January-March 2012 Date K 137Cs 140Ba 131 j Location Collected g/L ± 2 h pCi/L ± 2m pCi/L ± 2u pCi/L ± 2u AR: Little Rock 01/31/12 1.66 0.19 ND ND NR AZ: Phoenix 03/30/12 1.68 0.19 ND ND ND CA: Los Angeles 03/08/12 1.66 0.19 ND ND ND CA: San Francisco 01/11/12 1.92 0.23 2.9 2.5 ND ND CT: Hartford 02/15/12 1.66 0.20 ND ND NR DE: Wilmington 01/23/12 1.65 0.20 ND ND ND FL: Plant City 01/24/12 1.73 0.20 2.7 2.2 ND ND HI: Hilo 01/24/12 1.74 0.20 ND NR NR IA: Des Moines 01/30/12 1.65 0.19 ND NR NR KS: Wichita 02/14/12 1.73 0.20 ND ND NR KY: Louisville 01/11/12 1.66 0.19 ND ND ND MA: Boston 03/29/12 1.67 0.20 ND ND ND MD: Baltimore 01/09/12 1.58 0.19 ND ND ND MI: Detroit 01/31/12 1.62 0.19 ND NR NR MO: Jefferson City 03/07/12 1.69 0.19 ND ND ND NJ: Trenton 01/06/12 1.63 0.20 ND ND ND NM: Albuquerque 03/07/12 1.51 0.18 ND ND ND NV: Las Vegas 01/09/12 1.77 0.20 ND NR NR NV: Reno 01/12/12 1.67 0.19 ND ND ND NY: Buffalo 02/22/12 1.65 0.19 ND ND NR NY: Syracuse 01/09/12 1.61 0.19 ND ND ND OH: Cincinnati 01/09/12 1.69 0.19 ND ND ND OH: Cleveland 02/14/12 1.70 0.19 ND ND NR PA: Pittsburgh 01/10/12 1.71 0.19 ND ND ND TN: Chattanooga 01/05/12 1.72 0.20 ND ND ND TN: Knoxville 01/18/12 1.57 0.19 ND ND ND TN: Memphis 01/23/12 1.58 0.19 ND ND ND TX: San Antonio 01/31/12 1.58 0.19 ND NR NR WA: Spokane 01/24/12 1.63 0.19 ND NR NR WA: Tacoma 03/31/12 1.73 0.20 ND ND ND WV: Charleston 01/09/12 1.73 0.20 ND ND ND Note: ND = Not detected NR = No result (not analyzed within 5 half-lives of collection) 24 ------- For More Information Environmental Radiation Data (ERD) is published quarterly by the U.S. Environmental Protection Agency's Office of Radiation and Indoor Air. Requests for information concerning the operation of RadNet and the data that are generated should be directed as follows: Requests for information concerning the operation of RadNet, the data that are generated, or publication and distribution of ERD should be directed to: Charles M. Petko Office of the Director National Analytical Radiation Environmental Laboratory 540 South Morris Avenue Montgomery, Alabama 36115-2601 email: petko.charles@epa.gov Requests for information concerning policies of the Office of Radiation and Indoor Air should be directed to: Jonathan Edwards USEPA - ORIA Radiation Protection Division (MC6608J) 1200 Pennsylvania Ave. N.W. Washington, DC 20460 email: edwards.jonathan@epa.gov *** 25 ------- This page intentionally left blank 26 ------- |