United States Environmental Protection Agency	Office of Research and Development

National Exposure Research Laboratory
Research Abstract

Government Performance Results Act Goal: Safe Food

Significant Research Findings:

Immunochemical Methods

Scientific Problem The immunochemistry program of the U.S. Environmental Protection

and Policy Issues	Agency's (EPA) National Exposure Research Laboratory's (NERL)

Human Exposure Research Branch is addressing the need for rapid,
cost-effective monitoring methods to assess human exposures to low
levels of environmental contaminants such as pesticides.

Immunochemical methods such as immunoassays can provide
information regarding the presence and concentration of contaminants
that might impact human health and the environment. One way to reduce
uncertainties in the determination of low-level, non-occupational
exposures is to better characterize potential routes of exposure through
extensive environmental monitoring and dietary studies. The
information from these assessment studies is then used to ultimately
mitigate or reduce exposures. A large number of multi-media samples
(e.g. air, water, soil, dust, and food) are required for sampling and
laboratory analysis, which can often be slow and expensive; however,
time and budget constraints limit the number of samples that can be
analyzed. Since analytical methods are the foundation of the overall
exposure assessment and risk management process, reliable and cost-
effective monitoring methods such as immunoassays are key to safe
guarding human and environmental health.

Research Approach The need for new methods is determined through extensive literature

searches and discussions with Program Offices and NERL researchers
responsible for measurement studies. After target chemicals and
matrices have been identified, immunoassays are either developed or
adapted for particular applications. The experimental design and
statistical approach is specific for each chemical and is dependent upon
the data quality objectives of the particular study. The guidance in "A
User's Guide to Environmental Immunochemical Analysis"
(EPA/540/R-94/509) is followed throughout the methods development
process. Immunoassays for parent compounds, environmental
degradation products, and biomarkers of exposure are ultimately
configured for appropriate environmental and biological matrices to
support an integrated multimedia approach to environmental monitoring

National Exposure Research Laboratory — October 2001


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and risk assessment. Research results are published in the peer
reviewed literature and presented at scientific meetings.

Results and	Immunoassays to detect the pesticide chlorpyrifos (0,0-diethyl-0-

Implications	[3,5,6-trichloro-2-pyridyl]-phosphorothioate and its metabolite TCP

(3,5,6-trichloro-2-pyridinol) in food, track-in dirt, house dust and urine
have been developed. The assay format is an indirect competitive
enzyme-linked immunosorbent assay (ELISA) which utilizes a color
endpoint. Based on a 96-well microplate format, the ELISA has a high
sample capacity. A streamlined approach for the immunoassay
determination of chlorpyrifos and TCP residues in various food
matrices was developed to analyze samples from dietary exposure
surveys. Sample preparation is based on a sonic extraction followed by
dilution to reduce interfering components. Recoveries range from 74-
95% for various food commodities. Cleanup by solid phase extraction
can be employed for more difficult food matrices. Samples can also be
prepared using accelerated solvent extraction or supercritical fluid
extraction techniques prior to detection by ELISA. Chlorpyrifos levels
of 5-400 ppb can be determined based on a 10 g sample. Initial
evaluations indicate the ELISAs perform favorably with gas
chromatography/mass spectrometry (GC/MS) procedures; however, for
the ELISAs, sample preparation is minimal with a high sample
throughput and lower cost.

This immunochemistry program is conducted in-house with technical
support through the Senior Environmental Employee Program
(Cooperative Agreement #826228). An extramural component is
conducted through Battelle, Columbus, Ohio (Contract #69-D-99-011).
Examples of recent publications and presentations from this program
include:

Chuang, J.C., Hart, K., Chang, J.S., Boman, L.E., Van Emon, J.M., and Reed, A.W.
"Evaluation of Analytical Methods for Determining Pesticides in Baby
Foods and Adult Duplicate Diet Samples," Analytica Chimica Acta,
(accepted 2002).

Van Emon, J.M. "Immunochemical Applications in Environmental Science,"
Journal of AO AC International, Vol. 84, No. 1, (2001), 125-133.
Van Emon, J.M., Brumley, W.C., Reed, A.W., and Chuang, J.C., "Human Exposure
Assessment Using Immunoassay," presented at the 221st American
Chemical Society, San Diego, CA, April 1-5, 2001.

Van Emon, J.M., and Reed, A.W., "Immunoassay Analysis for Chlorpyrifos in
Foods," presented at the 37th Pesticide Residue Workshop and Florida
Foodborne Pathogen Analysis Conference, St. Petersburg Beach, FL, July
16-21, 2000.

Chuang, J.C., Pollard, M.A., Misita, A.M., and Van Emon, J.M., "Evaluation of

Analytical Methods for Determining Pesticides in Baby Food," Analytica
Chimica Acta 399, (1999) 135-142.

Research
Collaboration and
Publications

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Van Emon, J.M., Gerlach, C.L., Reed, A.W., and Hardwick, B.C., "Foliar
Dislodgeable Residue Analysis: A New Scientific Approach to a
Regulatory Concern," Food Technol. Biotechnol. 36, (1998),119-124.

Future Research

Contacts for

Additional

Information

All journal articles and abstracts from the immunochemistry program
were reviewed and approved in accordance with ORD's scientific peer
review procedures.

The TCP and chlorpyrifos ELISAs will be used to analyze samples from
on-going and planned NERL exposure studies. Additional evaluations
with GC/MS will be conducted based on the parameters of precision,
accuracy, sample throughput and cost. ELISA development for
compounds identified through the literature survey recently completed
will be initiated. Probable candidates include the pyrethroids for
various food matrices as well as their urinary biomarkers of exposure.
Selective antibodies will also be configured for immunoaffinity
chromatography columns. Immunoaffinity chromatography will be used
for sample preparations prior to ELISA detection and coupled on-line
with liquid chromatography/MS. As the need for rapid, low-cost
analytical methods continues, immunochemical methods will be
developed and applied.

Questions and inquiries can be directed to:

Jeanette M. Van Emon, Ph.D.

US EPA, Office of Research and Development
National Exposure Research Laboratory
Las Vegas, NV 89193-3478

Phone: 792/798-2154

E-mail: vanemon.jeanette@epa.gov

Federal funding for this research was administered under EPA
cooperative assistance agreement #826228 with the Senior
Environmental Employee Program and under EPA contract #69-D-99-
011 with Battelle, Columbus, Ohio.

National Exposure Research Laboratory — October 2001


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