NERL Research Abstract

EPA's National Exposure Research Laboratory
GPRA Goal 2 - Clean and Safe Water

Significant Research Findings

Identification of New Disinfection By-Products
Formed by Alternative Disinfectants

Purpose	Trihalomethanes (THMs) and other halogenated by-products can be formed

during chlorination of drinking water. Several drinking water treatment plants
in the U.S. have altered their treatment methods and adopted alternative
disinfectants to comply with an EPA regulation that limits levels of THMs in
drinking water. The alternative disinfectants currently being used (including
ozone, chloramine, and chlorine dioxide) are effective and do not produce
significant levels of THMs. However, limited information exists concerning
disinfection by-products (DBPs) that are produced from alternative
disinfectants, resulting in significant uncertainty regarding human exposure to
DBPs. These alternative disinfectants may produce compounds more or less
harmful than those produced by chlorine. The purpose of this research is to
identify unknown DBPs formed by alternative disinfectants and in combination
with chlorine. This abstract presents a summary of all research NERL has
conducted on DBPs from alternative disinfectants.

Drinking water was collected from full-scale treatment plants using ozone and
chloramine, and from pilot plants using chlorine dioxide, ozone, and titanium
dioxide with UV light—with and without secondary chlorine or chloramine
disinfection. Elevated bromide levels was also investigated using drinking
water disinfected with ozone. Disinfection by-products were extracted using
XAD resins. A combination of analytical techniques, including gas
chromatography (GC)/high resolution mass spectrometry (MS), GC/chemical
ionization MS, and GC/infrared spectroscopy, were used to identify new DBPs
found in drinking water samples. Liquid chromatography (LC)/MS was used to
identify polar DBPs that are difficult to extract from water. Derivatization
techniques, including pentafluorobenzylhydroxylamine (PFBHA), 2,4-
dinitrophenylhydrazine (DNPH), and BF3/methanol methylations were also
utilized to aid in the extraction and identification of DBPs.

Major	Many new DBPs were identified using the combination of spectroscopic

Findings techniques. Several DBPs were not present in the spectral library databases,

Research
Approach

National Exposure Research Laboratory - September 2000


-------
and, therefore, required information obtained from high resolution MS,
chemical ionization MS, infrared spectroscopy, and much scientific reasoning.
Many identifications were confirmed through the analysis of purchased or
synthesized standards. Elevated levels of bromide in the source water had a
substantial effect on DBPs formed by ozone-chlorine and ozone-chloramine
treatments, shifting the speciation from mostly chlorine-containing species
(e.g., trichloronitromethane) to bromine-containing species
(tribromonitromethane). Elevated bromide levels had a very minor effect on
ozone DBPs formed; only one compound, dibromoacetonitrile, was formed by
ozone treatment alone (for pilot plant samples of Mississippi River-treated
water). Comparing the DBPs found for the different treatments, Ti02/UV
formed the least amount of by-products, with only a single diketone formed in
the treatment studied. Chlorine dioxide and ozone produced the least halogen-
containing by-products (only two for chlorine dioxide and one for ozone, under
high bromide conditions), whereas chlorine and chloramine formed many
halogenated by-products. Most of the by-products were the same for chlorine
and chloramine, but chloramine produced lower levels compared to chlorine.
This effect has been seen by others when comparing THMs and haloacetic acids
formed by the two disinfectants.

Research

Collaboration

and

Publications

Much of this research is the result of a collaboration with a research group at
EPA's National Risk Management Research Laboratory (NRMRL). Scientists
from NRMRL were responsible for performing some of the treatments studied.
Scientists from EPA's NERL were responsible for the identification work. A
research brief will be published that summarizes all of the results and compares
DBPs for the different disinfectants studied. As this represents results of a
large volume of research, there have been several peer-reviewed journal articles
published using portions of the work. There have also been presentations
resulting in additional publications (two are listed here).

Patterson, K.S., Richardson, S.D., Lykins, B.W., Jr. Mutagenicity of drinking water following
disinfection. Journal of Water Supply: Research and Technology-AQUA 44: 1-9,
1995.

Richardson, S.D., Thruston, A.D., Jr., Chen, P.H., Collette, T.W., Schenck, K.M., Lykins,
B.W., Jr. Identification of Drinking Water Disinfection By-Products from Chlorine
Dioxide, Ozone, Chloramine, and Chlorine. EPA Research Brief. In preparation.

Richardson, S.D., Caughran, T.V., Poiger, T., Guo, Y., Crumley, F.G. Application of DNPH
derivatization with LC/MS to the identification of polar carbonyl disinfection by-
products in drinking water. Ozone Science & Engineering: In press.

Richardson, S.D., Thruston, A.D., Jr., Caughran, T.V., Chen, P.H., Collette, T.W., Schenck,
K.M., Lykins, B.W., Jr., Rav-Acha, C., Glezer, V. Identification of new drinking
water disinfection by-products from ozone, chlorine dioxide, chloramine, and
chlorine. In: Environmental Challenges for the Next Millennium: The 7th
International Conference of the Israel Society for Ecology and Environmental Quality
Sciences. Water, Air, and Soil Pollution. In press. (Invited article).

Richardson, S.D., Caughran, T.V., Poiger, T., Guo, Y., Crumley, F.G. Identification of polar

National Exposure Research Laboratory - September 2000


-------
drinking water disinfection by-products using LC/MS. Natural Organic Matter and
Disinfection By-products, American Chemical Society. In press. (Invited article).

Richardson, S.D., Thruston, A.D., Jr., Collette, T.W., Patterson, K.S., Lykins, B.W., Jr.,

Majetich, G., Zhang, Y. Multispectral identification of chlorine dioxide disinfection
by-products in drinking water. Environmental Science & Technology 28: 592-599,
1994.

Richardson, S.D., Thruston, A.D., Jr., Collette, T.W., Patterson, K.S., Lykins, B.W., Jr.,

Ireland, J.C. Identification of Ti02/UV disinfection by-products in drinking water.
Environmental Science & Technology 30: 3327-3334, 1996.

Richardson, S.D., Thruston, A.D., Jr., Caughran, T.V., Chen, P.H., Collette, T.W., Floyd, T.L.,
Schenck, K.M., Lykins, B.W., Jr. Identification of new ozone disinfection by-products
in drinking water. Environmental Science & Technology 33: 3368-3377, 1999.

Richardson, S.D., Thruston, A.D., Jr., Caughran, T.V., Chen, P.H., Collette, T.W., Floyd, T.L.,
Schenck, K.M., Lykins, B.W., Jr. Identification of new drinking water disinfection by-
products formed in the presence of bromide. Environmental Science & Technology
33: 3378-3383, 1999.

Richardson, S.D., Thruston, Jr., A.D., Caughran, T.V., Chen, P.H., Guo, Y., Collette, T.W.,
Floyd, T.L., Schenck, K.M., Lykins, B.W., Jr. Identification of new drinking water
disinfection by-products formed in the presence of bromide. Natural Organic Matter
and Disinfection By-Products, American Chemical Society, 1999. (Invited article).

Future
Research

National Exposure Research Laboratory - September 2000

Many new DBPs are being measured in a nationwide study and are also being
researched in preliminary health effects studies. The nationwide study will
provide an opportunity to analyze a wide range of drinking waters for new
DBPs. New research is also being conducted that identifies chlorine dioxide
DBPs formed under high bromide conditions (through a collaboration with
researchers at the Israel Ministry of Health). This is an important area that has
never been studied, yet many people in the U.S., particularly in Texas, drink
water treated under these conditions. Research also continues in this area of
polar drinking water DBPs. A collaboration with researchers at the University
of Torino (Italy) has been initiated to investigate another derivatization
procedure that previously has been shown useful for identifying poly-hydroxy,
poly-amino, and poly-carboxy polar compounds in water. This method will be
developed (to lower detection limits), and real drinking water will be analyzed.
Also, there is on-going research focusing on how some polar (and other) DBPs
are formed (mechanisms of formation), with the goal of learning how to control
the formation of any DBPs determined to be toxic.

Inquiries about new disinfection by-products may be directed to:

Dr. Susan Richardson

U.S. Environmental Protection Agency

960 College Station Road

Athens, GA 30605-2700

Phone: (706)355-8304

E-mail: richardson.susan@epa.gov


-------