The Impact of Climate Change
on Regional Air Quality

C. Nolte1', E, Cooter1, R. Gilliam1, W. Benjey1, J. Swall1, A. Gilliland1, L. Mickley2, P. Adams3

'NOAA Air Resources Laboratory, Atmospheric Sciences Modeling Division, in partnership
with EPA/ORD/NERL, RTP, NC, 2Harvard University, 3Carnegie Mellon University

Introduction

•	The Climate Impact on Regional Air Quality (CIRAQ) project seeks to assess how near-term (ca. 2050) climate change will affect air quality in the U.S.

•	A Global Climate Model (GCM) simulation for the period 1950-2050 has been linked with regional scale models to simulate regional climate and air quality.

•	A principal goal of CIRAQ is to determine the relative importance of climate change and changes in anthropogenic emissions to future U.S. air quality. In this first phase of the project,
anthropogenic emissions are held constant. In subsequent work changes to anthropogenic emissions will be considered.

1. Global and Regional Climate Modeling

•NASA Goddard Institute for Space Studies GISSII' GCM downscaledto 36 km grid
covering continental U.S. using Penn State/NCAR Mesoscale Model (MM5).

•C02 consistent with IPCC greenhouse gas emissions scenario A IB, corresponding to high
economic growth with balance between fossil fuel and alternative energy sources.

Modeled differences (Future-
Current) in mean summer (JJA) 2-m
temperature (K) for the ten year
meteorology simulations. The
largest increases are seen in
southern Texas and New Mexico
and the Pacific Northwest, while the
Upper Midwest is predicted to cool
slightly.

2. Air Quality Modeling

•Regional air quality simulations conducted using EPA Community Multiscale Air
Quality (CMAQ) model version 4.5 for two 5-year periods (1999-2003 and 2048-2052).

•Monthly averaged outputs from Harvard/Carnegie Mellon global tropospheric
chemistry models coupled to GISS II' provided chemical boundary conditions.

•Anthropogenic emissions held constant at 2001 levels; biogenic emissions and response
to temperature simulated using Biogenic Emissions Inventory System (BEIS) 3.13.

Difference In mean peak 1-h 03

- Curram tw Jun I Aug)*

Difference in mean 8-h max 03

Ci*f*m tn Jutl I /Vr}31

Modeled differences (Future - Current) in maximum 1-h and 8-h ozone
(03) concentrations (ppb), averaged over summer (JJA) for the two 5-
year periods. The largest increases are seen in Southern CA, Seattle,
east central Texas, and a strip from North Carolina through New Jersey.

3. Change in Frequency and Duration of Ozone Episodes

•The bar charts below show the number and duration of ozone episodes (8-h max > 80
ppb) for current (1999-2003) and future (2048-2052) years, broken down by geographic
region.

•	The number of high ozone episodes increases in the future simulations in both the
Western and Southeastern U.S.

•	Additionally, the duration of ozone episodes increases in the future simulations in the
Western and Southeastern US.

•	The number of future ozone episodes in the future simulations does not increase
substantially in the Northeast U.S., if interannual variability is considered

West

Northeast

Southeast

4. Changes in Particulate Matter (PM2.S) Concentrations

•The differences between modeled PM2 5 concentrations averaged over the two 5-year
periods and the frequency and duration of PM25 episodes are shown below.

•Compared to the current period, concentrations are broadly lower and the frequency of
PM episodes decreases in the future.

•Subsequent work will investigate the change in concentration of the individual
components of PM25 (sulfate, nitrate, ammonium, and organic and elemental carbon).

Difference in mean PMIS

= ESS

fpiti-do	(ConMCuSv# D«y»]

Summary and Future Work

•Regional climate and air quality simulations have been developed for both the current climate and under one future greenhouse gas emissions scenario.

•For this modeling system, summer ozone concentrations are predicted to increase in California and much of the Southern and Eastern U.S., with a greater frequency of ozone episodes. The
spatial pattern of this change appears to be consistent with the pattern of the temperature increase predicted by the regional climate model, though a more quantitative analysis is needed.

•These modeling results will be evaluated against observations for the current climate to assess the degree of uncertainty in the air quality predictions for the future climate period.

References

L.R. Leung and W.I. Gustafson, Jr., Geophys. Res. Lett. 32, doi: 10.1029/2005GL022911, 2005.
L.J. Mickley, D.J. Jacob, B.D. Field, andD. Rind Geophys. Res. Lett. 31, doi:10.1029/2004/GL021216,
2004.

^Contact email: nolte.chris@epa.gov





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*The research presented here was performed under the Memorandum of Understanding between the U.S. Environmental Protection Agency (EPA) and the U.S. Department of Commerce's National Oceanic and Atmospheric Administration (NOAA)
and under agreement number DW13921548. This work constitutes a contribution to the NOAA Air Quality Program. Although it has been reviewed by EPA and NOAA and approved for publication, it does not necessarily reflect their policies or views.


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