United States Environmental Protection Agency	Office of Research and Development

National Exposure Research Laboratory
Research Abstract

Government Performance Results Act (GPRA) Goal #4.5.2
Annual Performance Measure #230

Significant Research Findings:

Research to Support the National Children's Study

Scientific	To help understand how the environment affects children's health, a National

Problem and	Children's Study (NCS) is planned as authorized by the Children's Health Act

Policy Issues	(2000). The NCS is an interagency effort sponsored by the Department of Health

and Human Services (DHHS) and the EPA. The goal of the NCS is to recruit and
follow 100,000 children from birth to adulthood. A study of this size requires
cost-effective methods that can measure large numbers of samples and provide
results of the needed quality. The research described below was conducted to
provide such methods to the NCS. The methods developed will also assist the
EPA in meeting goals under the Food Quality Protection Act and other programs
concerned with the effect of environmental contaminants on human health.

Research	EPA's National Exposure Research Laboratory (NERL) conducted several

Approach	projects designed to develop or evaluate techniques for the NCS. Each project was

reviewed annually by NCS staff. The project reports and publications have been
subjected to the appropriate level of EPA and/or external peer review.

Development of Exposure Assessment Study Designs

The objective of this project was to develop cost-effective and optimally-designed
statistical sampling strategies. When one is collecting detailed information about a
small number of people and then using statistics to extrapolate this to a larger
population, it is very important to know that you have sufficient numbers in the
statistically selected population, those that represent the group of concern, for the
statistics to accurately describe the larger population. To control costs, it is
equally important that the small group not contain more people than needed.

Demonstration of Low-Cost, Low-Burden, Exposure-Monitoring Methods

The objective of this project was to develop and evaluate low-cost, low-burden
methods for collecting high quality environmental and biological samples and
survey information from study participants without the presence and/or assistance
of field sampling technicians. Innovative sampling methods and approaches were
developed for collecting the exposure and survey data. Pilot studies were
conducted to evaluate how well participants managed to employ the methods and
approaches and then complete these activities without direct contact from an
investigator in the field.

Methods Development

The objective of this project was to identify, develop, and improve methods for
classifying subjects by level of exposure to chemicals in order to focus resources


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on the most highly exposed individuals. The approach included a literature search
to identify potential sampling devices or methods, and laboratory studies to
evaluate known methods of collecting long-term integrated air samples (semi-
permeable membrane devices) and analytical methods for rapidly screening these
samples for organophosphorus pesticides.

Results and	Development of Exposure Assessment Study Designs

Impact	Guidance and examples were provided for developing statistically valid designs

for individual studies and to ensure that the studies collect the required data at
minimum cost.

Demonstration of Low-Cost, Low-Burden, Exposure-Monitoring Methods

In the pilot studies, some types of samples (e.g., hair and vacuum cleaner dust)
were successfully collected by over 90 percent of the participants. Other more
complicated sampling procedures (e.g., collecting air samples) had a lower success
rate. Participant compliance with sample-collection instructions was generally
good. Follow-up interviews helped identify the weak points in the procedures and
indicated areas where additional participant training would improve the success
rate for sample collection. The results from these studies provide the NCS with
low-cost alternatives to investigator-administered questionnaires and sample
collection protocols. Recommendations for improving participant success in these
procedures was also provided to the NCS.

Methods Development

Procedures for classifying exposure levels were developed.

NERL conducted the research with contract support from Research Triangle
Institute and an interagency agreement with the U.S. Geological Survey.

The following publications describe the study design and results:

Fortmann, R. Demonstration of Low Cost, Low Burden, Exposure Monitoring Strategies for Use
in Longitudinal Cohort Studies. Presented at: National Children's Pilot Study Review, Research
Triangle Park, NC, November 21, 2003 and at the National Children's Study Assembly Meeting,
Atlanta, GA, December 17, 2003.

Robertson, G.L., Hern, S.C., and Rogers, K.R. Methods studies for the national children's study:
molecularly imprinted polymers. Presented at: National Children's Study Assembly Meeting,
Atlanta, GA, December 17, 2003

Robertson, G.L., Hern, S.C., and Rogers, K.R. Methods studies for the national children's study:
semipermeable membrane device (SPMD). Presented at: National Children's Study Assembly
Meeting, Atlanta, GA, December 17, 2003.

McKinney, J.D., Hern, S.N., and Robertson, G.L. Identification of time-integrated sampling and
measurement techniques to support human exposure studies. EPA 600/R-04/043.

Mishra, N.N., Pedersen, J.A., and Rogers, K.R. "Highly sensitive assay for anticholinesterase
compounds using 96 well plate format." In: Chemicals in the Environment: Fate, Impacts, and
Remediation, Chapter 16 M. L. Phillips (Ed.), Washington, DC: American Chemical Society 2001,
289-305.

Research
Collaboration and
Research
Products


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Weetall, H., Mishra, N.N., Mahfouz, A., and Rogers, K.R. An approach for screening
cholinesterase inhibitors in drinking water using an immobilized enzyme assay. Analytical Letters,
37,1297- 1305 (2004).

Weetall, H., and Rogers, K.R. Preparation and characterization of molecularly imprinted
electropolymerized carbon electrodes. Talanta 62 (1):329-335 (2004). EPA/600/.T-04/040.

Rench, J.D. et al. Demonstration of Low Cost, Low Burden, Exposure Monitoring Strategies for
Use in Longitudinal Cohort Studies - Final Report. U.S. EPA Report EPA/600/R-04/109. Office of
Research and Development, Research Triangle Park, NC.

Strauss, W., Lehman, J., Morara, M., Ryan, L. (2003) Development of Exposure Assessment Study
Design for the National Children's Study: . Prepared by Battelle Memorial Institute for USEPA
National Exposure Research Laboratory, September 30, 2003.

Future Research Most of the specific research under this project has been completed. Work to
determine the uptake rates for semi-permeable membrane devices is in progress
and will be completed by September of 2005.

Contacts for	Questions and inquiries can be directed to

Additional

Information	Gary L. Robertson

U.S. EPA, Office of Research and Development
National Exposure Research Laboratory
P.O. Box 93478, Las Vegas, NV 89193
702-798-2215

E-mail: robertson.garv@epa.gov
Kim R. Rogers, Ph.D.

U.S. EPA, Office of Research and Development
National Exposure Research Laboratory
P.O. Box 93478, Las Vegas, NV 89193
702-798-2299

E-Mail: : rogers.kim@epa.gov
Roy Fortmann, Ph.D.

U.S. EPA, Office of Research and Development
National Exposure Research Laboratory
MD E-205-04, 109 TW Alexander Dr."

Research Triangle Park, NC 27711
919-541-1021

E-Mail: fortmann.rov@epa.gov
Halfk Ozkaynak, Ph.D.

U.S. EPA, Office of Research and Development
National Exposure Research Laboratory
E 205-05

Phone: 919/541-5172

E-mail: ozkavnak.haluk@epa.gov


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Federal funding for this research was administered under EPA contract 68-D-99-
012 with Research Triangle Institute, EPA Task Order Contract T019, 68D99-
011 with Battelle Memorial Institute., and EPA interagency agreement DW
14937889 with the U.S. Geological Survey.


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