Pvrethrins (PC 069001)

MRIDs 50475402/50475401

Analytical method for pyrethrins in water
Reports:

Document No.

Guideline:

Statements:

Classification:

PC Code:
EFED Final
Reviewers:

CDM/CSS-
Dynamac JV

ECM: EPAMRID No. 50475402. DeVellis, S.R. 2017. Validation of an
Environmental Chemistry Method for the Determination of Pyrethrins in
Groundwater and Surface Water. Smithers Viscient Study No.: 14118.6100.
Report prepared by Smithers Viscient, Wareham, Massachusetts; sponsored
and submitted by Pyrethrin Steering Committee/Joint Venture (PJV) c/o
Consumer Specialty Products Association, Inc., Washington, D.C.; 65 pages.
Final report issued June 9, 2017.

ILV: EPAMRID No. 50475401. Jutson, J.I. 2017. Independent Laboratory
Validation of: Validation of an Environmental Chemistry Method for the
Determination of Pyrethrins in Groundwater, Surface Water, Soil and
Sediment. Concord Biosciences Study No.: 036079 and Document No.:
036079-1. Report prepared by Concord Biosciences, LLC, Concord, Ohio;
sponsored and submitted by Pyrethrin Steering Committee/Joint Venture
(PJV) c/o Consumer Specialty Products Association, Inc., Washington, D.C.;
154 pages. Final report issued December 15, 2017.

MRIDs 50475402 & 50475401
850.6100

ECM: The study was conducted in accordance with the USEPA FIFRA (40
CFR Part 160) and OECD Good Laboratory Practices (GLP; p. 3 of MRID
50475402). Signed and dated No Data Confidentiality, GLP and Quality
Assurance statements were provided (pp. 2-4). A certification of the
authenticity of the report was included with the QA statement.

ILV: The study was conducted in accordance with the USEPA FIFRA GLP
(p. 3 of MRID 50475401). Signed and dated No Data Confidentiality, GLP
and Quality Assurance statements were provided (pp. 2-4). A certification of
the authenticity of the report was not included.

This analytical method is classified as unacceptable. An updated ECM was
not submitted incorporating the fact that the source of the acetonitrile was
critical. ILV performance data at the LOQs was unacceptable in both water
matrices. ILV linearity was not satisfactory for Pyrethrin I in ground water.
ECM linearity was not satisfactory for all analyses.

069001

Zoe Ruge, Physical Scientist

Mohammed Ruhman, Ph.D.,
Senior Scientist

Lisa Muto, M.S.,
Environmental Scientist

Signature:



Date:

9/27/18

Signature:



Date:

9/27/18

Signature:



Date:

4/26/18

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Pvrethrins (PC 069001)

MRIDs 50475402/50475401

Reviewers:

Kathleen Ferguson, Ph.D., Signature:
Environmental Scientist

Date:

/

--'7°

/

4/26/18

This Data Evaluation Record may have been altered by the Environmental Fate and Effects
Division subsequent to signing by CDM/CSS-Dynamac JVpersonnel. The CDM/CSS-Dynamac
Joint Venture role does not include establishing Agency policies.

Executive Summary

This analytical method, Smithers Viscient Study No. 14118.6100, is designed for the quantitative
determination of Pyrethrin I (pyrethrin I, jasmolin I, and cinerin I) at the LOQ of 0.10 |ig/L and of
Pyrethrin II (pyrethrin II, jasmolin II, and cinerin II) at the LOQ of 0.0818 |ig/L in water using
LC/MS/MS. Analytes were identified using one ion transition; a confirmation method is usually not
required when LC/MS or GC/MS is used as the primary method for quantifying residues. The
LOQs are less than the currently known lowest toxicological level of acute concern in water (0.76
|ig /L), however they are greater than the currently known chronic levels of concern (0.04 |ig /L). It
is suggested that the registrant adjust the ECM so that the LOQ is lower than the currently known
chronic value of 0.04 |ig/L in the new submitted study. The ECM and ILV used one characterized
surface water and one characterized ground water matrices; matrices differed between the ECM and
ILV. The ILV validated the ECM in the second trial for pyrethrins in water with insignificant
modifications of the analytical instrumentation and parameters; however, the failure of the first ILV
trial was due to Sigma-Aldrich acetonitrile, not Fisher acetonitrile, being used. The ECM did not
contain a statement that the use of Fisher-brand acetonitrile was critical; an Updated ECM should be
submitted specifying the source of the acetonitrile as Fisher as critical. All ECM data was
satisfactory regarding accuracy and precision for all analytes, but ILV performance data at the
LOQs was unacceptable in both water matrices. All ECM and ILV data was satisfactory regarding
specificity for all analytes; however, linearity was not satisfactory for some of the ECM and ILV
analyses.

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Table 1. Analytical Method Summary.

Analyte(s)

by
Pesticide1

MRID











Limit of
Quantitation
(LOQ)

Environmental
Chemistry
Method

Independent
Laboratory
Validation

EPA Review

Matrix

Method
Date

Registrant

Analysis

Pyrethrin I

50475402

50475401

Unacceptable

Water2-3

9/6/17

Pyrethrin
Steering
Committee/J
oint Venture
(PJV) c/o

LC/MS/

0.10 ng/L



Consumer

MS



Pyrethrin II











Specialty
Products
Association
Inc.



0.0818 ng/L

1	Pyrethrins = Pyrethrin Concentrate (BAS 383 HB I), which consists of six different esters grouped as such: Pyrethrin I
(pyrethrin I, jasmolin I, and cinerin I) and Pyrethrin II (pyrethrin II, jasmolin II, and cinerin II). Pyrethrin Concentrate
(% purities) = 29.46% Pyrethrin I, 24.02% Pyrethrin II, 53.48% Total Pyrethrins.

2	In the ECM, surface (river) water (pH 7.6, 85 mg equiv. CaCCh/L. 0.53 mmhos/cm conductivity) obtained from
Taunton River, Taunton, Massachusetts, and ground (well) water (pH 6.24, 84 mg equiv. CaCCh/L. 20 mg/L
alkalinity, 642 |iS/cm conductivity) obtained from Rock Creek, Ohio, were used. Water characterization was
performed by Agvise Laboratories, Northwood, North Dakota.

3	In the ILV, surface (river) water (EFS-629; pH 8.3, 104 mg equiv. CaCCh/L. 24 ppm total dissolved solids) obtained
from Grand River, Madison, Ohio, and ground (well) water (EFS-625; pH 8.0, 242 mg equiv. CaCO.VL. 348 ppm
total dissolved solids) obtained from Rock Creek, Ohio, were used. Water characterization was performed by Agvise
Laboratories, Northwood, North Dakota.

I. Principle of the Method

Samples (40.0 mL) were fortified as necessary with 0.04 mL or 0.40 mL of the fortification solution
pyrethrins (0.100 mg/L:0.0818 mg/L of Pyrethrin LPyrethrin II) in acetonitrile (pp. 13-17 of MRID
50475402). The water samples were extracted twice with 5.00 mL of dichloromethane. The
extraction procedure was not described. The dichloromethane layers were removed, placed in a 45-
mL glass vials, and evaporated under a gentle stream of nitrogen set at 40°C to ca. 100 |iL. The
residue was reconstituted with 7.50 mL of acetonitrile via vortex-mixing for 30 seconds and
sonication for five minutes. An aliquot of purified water (7.50 mL) was added in the same manner,
bringing the final composition of the samples to acetonitrile:water (50:50, v:v). LOQ samples were
analyzed via LC/MS/MS. For lOxLOQ fortifications, the samples were further diluted 1:10 with
acetonitrile:water (50:50, v:v) before analysis via LC/MS/MS.

Samples were analyzed by an Agilent 1200 HPLC system coupled with an MDS Sciex 4000
QTRAP® MS (Version 1.6.2; Agilent Poroshell 120 EC-C8 column, 3.0 mm x 50 mm, 2.7 |am
column; column temperature 25°C) using a mobile phase gradient of (A) 0.1% formic acid in water
(B) 0.1% formic acid in acetonitrile [percent A:B at 0.01-0.50 min. 98.0:2.0, 2.00 min. 30.0:70.0,
5.00-6.00 min. 2.0:98.0, 6.10-7.00 min. 98.0:2.0] with MS/MS detection and Multiple Reaction
Monitoring (MRM; TEM 550°C; pp. 11, 17-18 of MRID 50475402). Ion source was positive ESI
for all analytes. One ion transition was monitored for each analyte: m/z 329.0—>-161.30 for pyrethrin
I, m/z 331.40—>163.20 for jasmolin I, m/z 317.40—>149.30 for cinerin I, m/z 373.40—>-161.10 for
pyrethrin II, m/z 375.30—>163.20 for jasmolin II, and m/z 361.30—>149.00 for cinerin II.
Approximate retention times were reported as 4.2 minutes for pyrethrin I, 4.5 minutes for jasmolin

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I, 4.2 minutes for cinerin I, 3.6 minutes for pyrethrin II, 3.8 minutes for jasmolin II, and 3.6 minutes
for cinerin II for ground water and surface water. Injection volume was 100 |iL.

In the ILV, the ECM was performed as written, except for insignificant modifications of the
analytical instrumentation and parameters (pp. 15-16, 24; Table A-9, p. 36 of MRID 50475401).
Details for the dichloromethane extraction procedure were provided. The ILV reported that
Shimadzu Nexera UPLC system (System X) coupled with an AB Sciex 4000 MS was used (TEM
500°C). All monitored ion transitions were the same as those of the ECM. Retention times were not
reported. A critical component of the method was elucidated by the ILV through the failure of the
LOQ fortification in the first trial (p. 18; Appendix E, pp. 127-130). The Study Monitor informed
the ILV that Fisher acetonitrile must be used for the sample processing since problems have
occurred when other sources of acetonitrile have been used for pyrethrins. After switching from
Sigma-Aldrich to Fisher brand acetonitrile, the ILV successfully validated the ECM.

In the ECM and ILV, the method Limits of Quantification (LOQs) in water were 0.10 |ig/L for
Pyrethrin I (pyrethrin I, jasmolin I, and cinerin I) and 0.0818 |ig/L for Pyrethrin II (pyrethrin II,
jasmolin II, and cinerin II; pp. 19-22, 25-26 of MRID 50475402; pp. 6, 25 of MRID 50475401). In
the ECM and ILV, the method Limits of Detection (LOD) were 0.0132 |ig/L in ground water and
0.0138 |ig/L in surface water for Pyrethrin I and 0.0181 |ig/L in ground water and 0.00986 |ig/L in
surface water for Pyrethrin II.

II. Recovery Findings

ECM (MRID 50475402): Mean recoveries and relative standard deviations (RSD) were within
guideline requirements (mean 70-120%; RSD <20%) for analysis of Pyrethrin I (pyrethrin I,
jasmolin I, and cinerin I) at 0.10 |ig/L (LOQ) and 1.0 |ig/L (lOxLOQ) and for analysis of Pyrethrin
II (pyrethrin II, jasmolin II, and cinerin II) at 0.0818 |ig/L (LOQ) and 0.818 |ig/L (lOxLOQ) in
water matrices (Tables 1-4, pp. 29-32). Analytes were identified using one ion transition; a
confirmation method is usually not required when LC/MS or GC/MS is used as the primary method
for quantifying residues. Surface (river) water (pH 7.6, 85 mg equiv. CaC03/L, 0.53 mmhos/cm
conductivity) obtained from Taunton River, Taunton, Massachusetts, and ground (well) water (pH
6.24, 84 mg equiv. CaC03/L, 20 mg/L alkalinity, 642 |iS/cm conductivity) obtained from Rock
Creek, Ohio, were used (p. 12). Water characterization was performed by Agvise Laboratories,
Northwood, North Dakota.

ILV (MRID 50475401): Mean recoveries and RSDs were within guideline requirements for
analysis of Pyrethrin I at 1.0 |ig/L (lOxLOQ) and for analysis of Pyrethrin II at 0.818 |ig/L
(lOxLOQ) in water matrices (Tables 1-2, pp. 20-21; Tables A-l to A-4, pp. 29-31; DER Attachment
2). Analysis of Pyrethrin I at 0.10 |ig/L (LOQ) and Pyrethrin II at 0.0818 |ig/L (LOQ) were
unacceptable in both water matrices: Pyrethrin I (ground water, mean 67.8% and RSD 34.6%;
surface water, RSD 44%) and Pyrethrin II (ground water, RSD 28.1%; surface water RSD 35%).
LOQ recovery statistics were reviewer-calculated based on all reported recovery values (n = 6 or 7).
The study author only used five values for statistics. Recovery values which were deemed outliers
were omitted, and the samples were replaced with additional samples. LC/MS/MS Analytes were
identified using one ion transition. Surface (river) water (EFS-629; pH 8.3, 104 mg equiv. CaC03/L,
24 ppm total dissolved solids) obtained from Grand River, Madison, Ohio, and ground (well) water
(EFS-625; pH 8.0, 242 mg equiv. CaC03/L, 348 ppm total dissolved solids) obtained from Rock

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Pvrethrins (PC 069001)

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Creek, Ohio, were used (p. 14; Appendix A, pp. 91-92). Water characterization was performed by
Agvise Laboratories, Northwood, North Dakota. The ILV validated the ECM in the second trial for
pyrethrins in water with insignificant modifications of the analytical instrumentation and
parameters; however, through the failure of the LOQ fortification in the first trial, the ILV learned
that Fisher acetonitrile must be used for the sample processing since problems have occurred when
other sources of acetonitrile have been used for pyrethrins (pp. 15-16, 18, 24-25; Appendix E, pp.
127-130). After switching from Sigma-Aldrich to Fisher brand acetonitrile, the ILV successfully
validated the ECM. The ECM did not contain a statement that the use of Fisher-brand acetonitrile
was critical; an Updated ECM should be submitted specifying the source of the acetonitrile as
Fisher as critical.

Table 2. Initial Validation Method Recoveries for Pyrethrins as Pyrethrin I and Pyrethrin II
in Water.1'2'3

Analyte

Fortification

Number

Recovery

Mean

Standard

Relative Standard

Level (jig/L)

of Tests

Range (%)

Recovery (%)

Deviation (%)

Deviation (%)



Ground (Well) Water

Pyrethrin I

0.10 (LOQ)

7

86.4-98.6

91.8

4.21

4.59

1.0

5

92.3-94.1

93.2

0.763

0.819

Pyrethrin II

0.0818 (LOQ)

7

81.9-99.6

92.3

7.03

7.61

0.818

5

93.1-102

95.9

3.76

3.92



Surface (River) Water

Pyrethrin I

0.10 (LOQ)

7

80.6-94.4

87.3

4.39

5.03

1.0

5

65.3-92.8

80.8

10.9

13.5

Pyrethrin II

0.0818 (LOQ)

7

88.7-99.5

92.8

3.84

4.13

0.818

5

78.7-94.9

86.2

7.46

8.66

Data (uncorrected recovery results, pp. 20-21) were obtained from Tables 1-4, pp. 29-32 of MRID 50475402.

1	Pyrethrin I (pyrethrin I, jasmolin I, and cinerin I) and Pyrethrin II (pyrethrin II, jasmolin II, and cinerin II).

2	One ion transition was monitored for each analyte: m/z 329.0—>161.30 for pyrethrin I, m z 331.40—>163.20 for
jasmolin I, m/z 317.40—>149.30 for cinerin I, m/z 373.40—>161.10 for pyrethrin II, m/z 375.30—>163.20 for jasmolin
II, and m/z 361.30—>149.00 for cinerin II.

3	Surface (river) water (pH 7.6, 85 mg equiv. CaCCh/L. 0.53 mmhos/cm conductivity) obtained from Taunton River,
Taunton, Massachusetts, and ground (well) water (pH 6.24, 84 mg equiv. CaCCh/L. 20 mg/L alkalinity, 642 |iS/cm
conductivity) obtained from Rock Creek, Ohio, were used (p. 12). Water characterization was performed by Agvise
Laboratories, Northwood, North Dakota.

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Pvrethrins (PC 069001)

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Table 3. Independent Validation Method Recoveries for Pyrethrins as Pyrethrin I and
pyrethrin II in Water.1'2'3						

Analyte

Fortification
Level (jig/L)

Number
of Tests

Recovery
Range (%)

Mean
Recovery (%)

Standard
Deviation (%)

Relative Standard
Deviation (%)



Ground (Well) Water

Pyrethrin I

0.10 (LOQ)4

6

20.2-81.9

67.8

23.5

34.6

1.0

5

94.6-100

97.7

2.4

2.5

Pyrethrin II

0.0818 (LOQ)4

6

30.6-80.3

70.7

19.9

28.1

0.818

5

87.9-107

95.3

8.1

8.5



Surface (River) Water

Pyrethrin I

0.10 (LOQ)4

7

67.0-213

112

49

44

1.0

5

87.1-104

93.6

7.8

8.3

Pyrethrin II

0.0818 (LOQ)4

7

76.2-202

117

41

35

0.818

5

91.5-105

98.9

5.8

5.9

Data (uncorrected recovery results, Tables A-l to A-4, pp. 29-31) were obtained from Tables 1-2, pp. 20-21 and Tables
A-l to A-4, pp. 29-31 of MRID 50475401 and DER Attachment 2.

Red values indicate discrepancies with meeting guideline requirements.

1	Pyrethrin I (pyrethrin I, jasmolin I, and cinerin I) and Pyrethrin II (pyrethrin II, jasmolin II, and cinerin II).

2	One ion transition was monitored for each analyte: m/z 329.0—>161.30 for pyrethrin I, m z 331.40—>163.20 for
jasmolin I, m/z 317.40—>149.30 for cinerin I, m/z 373.40—>161.10 for pyrethrin II, m/z 375.30—>163.20 for jasmolin
II, and m/z 361.30—>149.00 for cinerin II.

3	Surface (river) water (EFS-629; pH 8.3, 104 mg equiv. CaCCh/L. 24 ppm total dissolved solids) obtained from Grand
River, Madison, Ohio, and ground (well) water (EFS-625; pH 8.0, 242 mg equiv. CaCO.VL. 348 ppm total dissolved
solids) obtained from Rock Creek, Ohio, were used (p. 14; Appendix A, pp. 91-92). Water characterization was
performed by Agvise Laboratories, Northwood, North Dakota.

4	Means, standard deviations and RSDs were reviewer-calculated based on all reported recovery values. Rules of
significant figures were followed when reporting results. The study author only used five values for statistics.
Recovery values which were deemed outliers were omitted, and the samples were replaced with additional samples.

III. Method Characteristics

In the ECM and ILV, the method LOQs in water were 0.10 |ig/L for Pyrethrin I (pyrethrin I,
jasmolin I, and cinerin I) and 0.0818 |ig/L for Pyrethrin II (pyrethrin II, jasmolin II, and cinerin II;
pp. 19-22, 25-26 of MRID 50475402; pp. 6, 25 of MRID 50475401). In the ECM and ILV, the
LOQ was defined as the lowest fortification level successfully tested. In the ECM, it was noted that
background noise should not exceed 20% of the LOQ. In the ECM and ILV, the method LODs were
0.0132 |ig/L in ground water and 0.0138 |ig/L in surface water for Pyrethrin I and 0.0181 |ig/L in
ground water and 0.00986 |ig/L in surface water for Pyrethrin II. In the ECM, the LOD was
calculated as the standard deviation at the LOQ multiplied by to.99, where to.99 equalled 3.143 for n-1
degrees of freedom where n = 7. The LOD was not justified in the ILV.

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Pvrethrins (PC 069001)

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Table 4. Method Characteristics for Pyrethrins in Water.

Analyte1

Pyrethrin I

Pyrethrin II

Limit of

Quantitation

(LOQ)

ECM

0.10 ng/L

0.0818 ng/L

ILV

Limit of

Detection (LOD)

ECM

Nominal

Not reported

Calculated

0.0132 |ig/L (ground)
0.0138 |ig/L (surface)

0.0181 |ig/L (ground)
0.00986 ng/L (surface)

ILV2

0.0132 |ig/L (ground)
0.0138 |ig/L (surface)

0.0181 |ig/L (ground)
0.00986 ng/L (surface)

Linearity
(calibration curve
r2 and

concentration
range)

ECM

Ground

r2 = 0.99625

r2 = 0.99435

Surface

r2 = 0.99290

r2 = 0.99768

ILV

Ground

r2 = 0.99393

r2 = 0.9983

Surface

r2 = 0.99643

r2 = 0.99853

Range

0.05-0.50 ng/L

0.0409-0.409 (ig/L
0.0409-0.327 jig/L (ILV/surface)

Repeatable

ECM4

Yes at LOQ and lOxLOQ in one surface water and one ground water
matrices (characterized).

ILV5-6

Yes at lOxLOQ in one surface water and one ground water matrices
(characterized).

No at LOQ [mean 67.8% and RSD
34.6% (ground); surface water, RSD
44% (surface)].

No at LOQ [RSD 28.1% (ground);
RSD 35% (surface)].

Reproducible

No at LOQ
Yes at lOxLOQ

Specific

ECM

Yes, matrix interferences were < 7% of the LOQ (based on peak area) for
each of the three components. Baseline noise interference was more
significant in chromatograms of jasmolin I/II.

ILV

Yes, matrix interferences were < 6% of the LOQ (based on peak area) for
each of the three components. Baseline noise interference was more
significant in chromatograms of jasmolin I/II and cinerin I/II.

Data were obtained from pp. 19-22, 25-26 (LOQ/LOD); Tables 1-4, pp. 29-32 (recovery results); Figures 1-20, pp. 33-
52 (chromatograms); Figures 21-24, pp. 53-56 (calibration curves) of MRID 50475402; pp. 6, 25 (LOQ/LOD); Tables
1-2, pp. 20-21 and Tables A-l to A-4, pp. 29-31 (recovery results); Figures 1-4, pp. 38-41 (calibration curves); Figures

9-28, pp. 46-65 (chromatograms) of MRID 50475401; DER Attachment 2. Analytes were identified using one ion

transition; a confirmation method is usually not required when LC/MS or GC/MS is used as the primary method for

quantifying residues.

Red values indicate discrepancies with meeting guideline requirements.

1	Pyrethrins = Pyrethrin Concentrate (BAS 383 HB I), which consists of six different esters grouped as such: Pyrethrin I
(pyrethrin I, jasmolin I, and cinerin I) and Pyrethrin II (pyrethrin II, jasmolin II, and cinerin II). Pyrethrin Concentrate
(% purities) = 29.46% Pyrethrin I, 24.02% Pyrethrin II, 53.48% Total Pyrethrins.

2	ILV LODs were reported from the ECM.

3	ILV coefficient of determination (r2) values were reviewer-generated from reported regression data from Figures 1-4,
pp. 38-41 of MRID 50475402 since the study author did not report these values (DER Attachment 2). Linear
regression equations were used.

4	In the ECM, surface (river) water (pH 7.6, 85 mg equiv. CaCO.VL. 0.53 mmhos/cm conductivity) obtained from
Taunton River, Taunton, Massachusetts, and ground (well) water (pH 6.24, 84 mg equiv. CaCO.VL. 20 mg/L
alkalinity, 642 |iS/cm conductivity) obtained from Rock Creek, Olio, were used (p. 12 of MRID 50475402). Water
characterization was performed by Agvise Laboratories, Northwood, North Dakota.

5	In the ILV, surface (river) water (EFS-629; pH 8.3, 104 mg equiv. CaCO.VL. 24 ppm total dissolved solids) obtained
from Grand River, Madison, Ohio, and ground (well) water (EFS-625; pH 8.0, 242 mg equiv. CaCOs/L, 348 ppm
total dissolved solids) obtained from Rock Creek, Ohio, were used (p. 14; Appendix A, pp. 91-92 of MRID
50475401). Water characterization was performed by Agvise Laboratories, Northwood, North Dakota.

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6 The ILV validated the ECM in the second trial for pyrethrins in water with insignificant modifications of the
analytical instrumentation and parameters; however, through the failure of the LOQ fortification in the first trial, the
ILV learned that Fisher acetonitrile must be used for the sample processing since problems have occurred when other
sources of acetonitrile have been used for pyrethrins (pp. 15-16, 18, 24-25; Appendix E, pp. 127-130 of MRID
50475401). After switching from Sigma-Aldrich to Fisher brand acetonitrile, the ILV successfully validated the
ECM. The ECM did not contain a statement that the use of Fisher-brand acetonitrile was critical; an Updated ECM
should be submitted specifying the source of the acetonitrile as Fisher as critical.

Linearity is satisfactory when r2 > 0.995.

IV. Method Deficiencies and Reviewer's Comments

1.	An updated ECM was not submitted incorporating the fact that the source of the acetonitrile
was critical. After the failure of the LOQ fortification in the first trial, the ILV presumed that
matrix effects caused suppression of the analyte signal. After some communication with the
Study Monitor and testing, the ILV determined that matrix effects were not the cause. The
Study Monitor informed the ILV that Fisher acetonitrile must be used for the sample
processing since problems have occurred when other sources of acetonitrile have been used
for pyrethrins. The ILV communicated that Sigma-Aldrich acetonitrile had been used in
previous trials. After switching from Sigma-Aldrich to Fisher brand acetonitrile, the ILV
successfully validated the ECM. The ECM did not contain a statement that the use of Fisher-
brand acetonitrile was critical; an Updated ECM should be submitted specifying the source
of the acetonitrile as Fisher as critical. The use of the Fisher brand acetonitrile by the ILV
was necessary for the successful validation of the ECM method.

2.	ILV performance data at the LOQs was unacceptable in both water matrices: Pyrethrin I
(ground water, mean 67.8% and RSD 34.6%; surface water, RSD 44%) and Pyrethrin II
(ground water, RSD 28.1%; surface water RSD 35%; Tables 1-2, pp. 20-21; Tables A-l to
A-4, pp. 29-31; DER Attachment 2). LOQ recovery statistics were reviewer-calculated
based on all reported recovery values (n = 6 or 7). The study author only used five values for
statistics. Recovery values which were deemed outliers were omitted, and the samples were
replaced with additional samples; subsequent statistics calculated by the study author were
acceptable. OCSPP guidelines state that acceptable mean recoveries and relative standard
deviations (RSD) are 70-120%) and <20%, respectively, at the LOQ and higher fortifications.

Since the ILV did not provide acceptable data at the LOQ for the analytes in either water
matrix, the reproducibility of the method was not demonstrated in the submitted method
validation set.

3.	ILV linearity was not satisfactory for Pyrethrin I in ground water, r2 = 0.9939 (Figures 1-4,
pp. 38-41 of MRID 50475401; DER Attachment 2). Coefficient of determination (r2) values
were reviewer-generated for three of the four calibration curves since the study author did
not report these values. Linear regression equations from reported regression data were used.

ECM linearity was not satisfactory for Pyrethrin I in surface water, r2 = 0.9929, and was not
satisfactory for Pyrethrin II in ground water, r2 = 0.99435 (Figures 21-24, pp. 53-56 of
MRID 50475402).

Linearity is satisfactory when r2 > 0.995.

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MRIDs 50475402/50475401

4.	The communications between the ILV Study Director and the CSPA Study Monitor were
documented (p. 26; Appendix E, pp. 127-130 of MRID 50475401). Communications
involved trial successes and failures, as well as procedure clarification (specifically the
dichloromethane extraction procedure and not allowing the extract to be reduced to dryness).
The reviewer noted that the CSPA Study Monitor involved the Smithers Study Director after
the ILV Study Director asked him to check with the method developer, and this
communication was forwarded to the ILV Study Director. However, the reviewer did not
deem this interaction to be collusion since the Smithers Study Director only clarified and re-
emphasized points of the method. The Smithers Study Director did not direct supplementary
work or modifications to the ILV.

The reviewer noted that the solution to the ILV LOQ performance data problem came from
the Study Monitor talking to another chemist familiar with analyzing pyrethrins (Appendix
E, p. 129 of MRID 50475401). The reviewer would have liked this chemist to have been
identified.

5.	Method LODs were not reported by the ECM or ILV; calculated LODs were provided. The
estimations of the LOQ and LOD in ECM and ILV were not based on scientifically
acceptable procedures as defined in 40 CFR Part 136 (pp. 19-22, 25-26 of MRID 50475402;
pp. 6, 25 of MRID 50475401). In the ECM and ILV, the LOQ was defined as the lowest
fortification level successfully tested. In the ECM, it was noted that background noise
should not exceed 20% of the LOQ. In the ECM, the LOD was calculated as the standard
deviation at the LOQ multiplied by to.99, where to.99 equalled 3.143 for n-1 degrees of
freedom where n = 7. The LOD was not justified in the ILV. Detection limits should not be
based on arbitrary values.

6.	The reviewer noted the following typographical error: PYRI in the Figure Title should have
been PYR II (Figure 20, p. 52 of MRID 50475402).

7.	It was reported for the ILV that one sample set of 13 samples required ca. 8 hours including
calculation of results (p. 25 of MRID 50475401).

V. References

U.S. Environmental Protection Agency. 2012. Ecological Effects Test Guidelines, OCSPP

850.6100, Environmental Chemistry Methods and Associated Independent Laboratory
Validation. Office of Chemical Safety and Pollution Prevention, Washington, DC. EPA 712-
C-001.

40 CFR Part 136. Appendix B. Definition and Procedure for the Determination of the Method
Detection Limit-Revision 1.11, pp. 317-319.

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MRIDs 50475402/50475401

DER Attachment 1: Chemical Names and Structures.

Pyrethrin I
IUPAC Name:

CAS Name:
CAS Number:
SMILES String:

[(lS)-2-methyl-4-oxo-3-[(2Z)-penta-2,4-dienyl]cyclopent-2-en-l-yl]
(lR,3R)-2,2-dimethyl-3 -(2-methylprop-1 -enyl )cyclopropane-1 -carboxylate
Not reported
121-21-1

CC1=C(C(=0)C[C@@H]10C(=0)[C@@H]2[C@H](C2(C)C)C=C(C)C)
C/C=C\C=C

Cinerin I
IUPAC Name:

CAS Name:
CAS Number:
SMILES String:

[(lR)-3-[(Z)-but-2-enyl]-2-methyl-4-oxocyclopent-2-en-l-yl] (lR,3R)-2,2-
dimethyl-3-(2-methylprop-1 -enyl )cyclopropane-1 -carboxylate
Not reported
25402-06-6

C/C=C\CC1=C([C@@H](CC1=0)0C(=0)[C@@H]2[C@H](C2(C)C)C=C(
C)C)C

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Pvrethrins (PC 069001)

MRIDs 50475402/50475401

Jasmolin I
IUPAC Name:

CAS Name:
CAS Number:
SMILES String:

[(lS)-2-methyl-4-oxo-3-[(Z)-pent-2-enyl]cyclopent-2-en-l-yl] (lR,3R)-2,2-
dimethyl-3-(2-methylprop-1 -enyl )cyclopropane-1 -carboxylate
Not reported
4466-14-2

CC/C=C\CC1=C([C@H](CC1=0)0C(=0)[C@@H]2[C@H](C2(C)C)C=C(
C)C)C



	

/

Pyrethin II
IUPAC Name:

CAS Name:
CAS Number:
SMILES String:

[(1 S)-2-methyl-4-o\o-3-[(2E)-penta-2,4-dienyl]cyclopent-2-en-1 -yl]

(lR,3R)-3-[(E)-3-methoxy-2-methyl-3-oxoprop-l-enyl]-2,2-
di m ethyl cy cl opropane-1 -carboxylate
Not reported
Not reported

CC1=C(C(=0)C[C@@H]10C(=0)[C@@H]2[C@H](C2(C)C)/C=C(\C)/C
(=0)OC)C/C=C/C=C

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Pvrethrins (PC 069001)

MRIDs 50475402/50475401

Cinerin II
IUPAC Name:

CAS Name:
CAS Number:
SMILES String:

[(1 S)-3-[(Z)-but-2-enyl]-2-methyl-4-o\ocyclopent-2-en-1 -yl] (1 R,3R)-3-

[(E)-3 -methoxy-2-methyl-3 -oxoprop-1 -enyl]-2,2-dimethyl cyclopropane-1 -

carboxylate

Not reported

121-20-0

C/C=C\CC1=C([C@H](CC1=0)0C(=0)[C@@H]2[C@H](C2(C)C)/C=C(\
C)/C(=0)OC)C

Jasmolin II
IUPAC Name:

CAS Name:
CAS Number:
SMILES String:

[(lS)-2-methyl-4-oxo-3-[(Z)-pent-2-enyl]cyclopent-2-en-l-yl] (lR,3R)-3-
[(E)-3-metho\y-2-methyl-3 -oxoprop-1 -enyl]-2,2-dimethyl cyclopropane-1 -
carboxylate
Not reported
1172-63-0

CC/C=C\CC1=C([C@H](CC1=0)0C(=0)[C@@H]2[C@H](C2(C)C)/C=C
(\C)/C(=0)OC)C

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