United States Environmental Protection Agency	Office of Research and Development

National Exposure Research Laboratory
Research Abstract

Government Performance Results Act (GPRA) Goal 1
Annual Performance Measure 220

Significant Research Findings:

A Probabilistic Exposure Model Capable of Estimating
Population Exposures to PM Components

Scientific	EPA's National Ambient Air Quality Standards (NAAQS) for particulate matter

Problem and	(PM) are largely based on studies that have shown consistent associations between

Policy Issues	increases in PM concentrations measured at outdoor sites within a community and

the occurrence of adverse health effects in the population living there. However,
the PM concentrations measured in outdoor air may not be the same as in the air
people breathe during their daily activities, for example while indoors at home,
work, or school, or when traveling in vehicles. Understanding actual personal
exposures to PM provides an important link between PM regulatory monitoring
and the risk of adverse health effects.

The National Research Council (NRC) lists understanding PM exposures as one of
the ten highest priority research areas for PM. (Cf. Research Priorities for
Airborne Particulate Matter: IV. Continuing Research Progress National
Academies Press, 2004.) The first two NRC Research Topics focus on
understanding exposures of susceptible subpopulations, such as the elderly and
children, to PM mass concentrations and how these exposures relate to
concentrations measured at outdoor community sites. The second Research Topic
extends the exposure research to the potentially toxic components of PM, such as
sulfate, nitrate, various metals, and organic and elemental carbon, as well as to the
different PM size fractions, including the ultra-fine fraction.

To address these research areas identified by the NRC, new data and models are
needed that can estimate individual, subpopulation, and general population
exposures to PM (and its biologically important constituents) and to relate those
exposures to PM concentrations measured at outdoor sites.

Research	EPA's National Exposure Research Laboratory (NERL) has developed a model to

Approach	estimate distribution of PM exposures (amount available in the air for an

individual to breathe) and intake dose (amount inhaled into the lungs) for the
general population or for a targeted sub-population. U.S. census data built into the
model are used to create the simulated population. Human activity pattern data,
also built into the model, are assigned to each simulated individual to account for
the way people interact with their environment. The user is only required to
provide ambient PM concentration data, which can be monitoring data or output
from an air quality dispersion model. PM concentrations in the indoor locations
where people spend much of their time (such as home, work, or school) are
calculated using algorithms that depend on the outdoor PM concentration, but also


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account for indoor PM sources. Each individual's exposure profile is then
calculated from the time spent in each location and the PM concentration in that
location. Activity-specific inhalation rates while in each location are also
calculated by the model and combined with the exposure concentrations to
estimate an intake-dose profile for each individual. Daily-averaged values are
calculated from the daily exposure and dose profiles, and then combined to
provide distributions for the user-defined population. Statistical methods are used
to incorporate variability and uncertainty into the model input parameters. Model
output includes estimates of the contribution to exposure and intake-dose
distributions from both outdoor and indoor sources of PM.

Results and	The result of this research is Version 2.0 of the Stochastic Human Exposure and

Impact	Dose Simulation (SHEDS) model for PM. The EPA SHEDS-PM 2.0 model

estimates the range in PM exposure and/or intake-dose across a population of
interest, and percentage of estimated exposures above a certain level. The model
includes a user-friendly interface that allows the user to define the model run
scenario and input data, as well as to analyze and display the results.

The availability of data on PM constituents needed as input to the SHEDS-PM 2.0
model can vary significantly between the different PM species. The model is
structured to allow the user to provide the required inputs based on the level of
information available for that particular PM component. For example, the user has
different options for specifying the relationship between the outdoor air
concentrations of a PM component and the concentrations in locations where
people spend their time.

The model results can be used to assess potential exposures to PM components for
a community of interest, to estimate the impact of different air concentration
patterns resulting from possible emissions reduction strategies on population
exposures, and to improve exposure characterization in epidemiology studies.

Collaboration with EPA/NERL on this research effort included contributions from
Science Applications International Corporation (SAIC).

Examples of recent publications from this study include the following:

Burke, J., Zufall, M., Ozkaynak, H. A Population exposure model for particulate matter: case study
results for PM2.5 in Philadelphia, PA. Journal of Exposure Analysis and Environmental
Epidemiology (2001) 11, 470-489.

Burke, J., Vedantham, R., McCurdy, T., Xue, J., Ozkaynak, H. "A Population Exposure Model for
Particulate Matter: SHEDS-PM' Presented at the 21st annual conference of the American
Association of Aerosol Research (AAAR) Charlotte, NC. October, 2002.

Burke, J.M., Vedantham, R., McCurdy, T., Xue, J., Ozkaynak, H. "SHEDS-PM: A population
exposure model for predicting distributions of PM exposure and dose from both outdoor and
indoor PM sources" Presented at the 13th annual conference of the International Society of
Exposure Analysis, Stresa, Italy, September, 2003.

Future Research Recent human exposure measurement studies have produced data on PM

components from residential indoor, outdoor, and personal exposure samples. As
more of the data from these studies become available, EPA/NERL will use the
data to refine the SHEDS-PM 2.0 model inputs and to evaluate model predictions.

A longer term goal is to use observational data and SHEDS exposure model
predictions to describe and understand human exposures to particulates derived
from various source types, since recent findings show a variety of health effects

Research
Collaboration
and Research
Products


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associated with PM from specific sources. EPA/NERL will combine source
apportionment techniques with exposure models to evaluate the ambient-personal
exposure relationship for PM from various sources. EPA/NERL will also
investigate the influence of the spatial distribution of sources on exposure.

Contacts for	Questions and inquiries can be directed to the principal investigator:

Additional	T	~	^

Information	Janet M Burke' Ph D

U.S. EPA, Office of Research and Development

National Exposure Research Laboratory
Mail Drop E205-02
109 T.W. Alexander Drive
Research Triangle Park, NC 27711
Phone: 919-541-0820
E-mail: burke.janet@epa.gov

Federal funding for this research was administered under EPA Contract No.
69W99002 and 68W00122 to Science Applications International Corporation
(SAIC).


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