PEER REVIEW DRAFT - DO NOT CITE OR QUOTE

xvEPA

United States

Environmental Protection Agency

Office of Chemical Safety and
Pollution Prevention

Draft Risk Evaluation for
Perchloroethylene

Systematic Review Supplemental File:

Data Extraction Tables of Environmental Fate and

Transport Studies

CASRN: 127-18-4

CI CI

CI CI

April 2020


-------
PEER REVIEW DRAFT - DO NOT CITE OR QUOTE

Table of Contents

Table 1. Biodegradation Study Summary for Perchloroethylene	

Table 2. Bioconcentration Study Summary for Perchloroethylene	

Table 3. Photolysis Study Summary for Perchloroethylene	

Table 4. Hydrolysis Study Summary for Perchloroethylene	

Table 5. Sorption Study Summary for Perchloroethylene	

Table 6. Other Fate Endpoints Study Summary for Perchloroethylene

EPI Suite™ Model Outputs	

References	


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Interagency Review Draft Document. Do Not Release or Distribute.

Table 1. Biodegradation Study Summary for Perchloroethylene

















Data

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Quality
Evaluatio
n Results
of Full
Study
Report

Water





Digested
sludge:
Preconditione
d with
methane or





Biodegradation

parameter:
percent removal









Aerobic
bottle test
initial mass
= 37 ng





fbased on active

bottles and
expected mass"):
Methane culture:
0%/20d
(reported as -
5%); phenol
culture: -

The reviewer





Aerobic serum bottle
test

phenol
bacteria,
municipal
digester
sludge from
the batch
reactor
cultures

aerobic

20 days

agreed with
this study's
overall quality
level.

Long et

aL
C19931

High









15%/20d











other: Pure

















culture: T.

















versicolor













Pure culture aerobic
biodegradation

5 mg/L

(ATCC#4523
0);

maintained

by

subculturing
on 2% malt
extract agar
slants (pH
4.5) at room
temperature.
Subcultures
were
routinely

aerobic

9 days

Biodegradation
parameter: rate
constant:
0.20 to 0.28
nmol h1 mg1 dry
weight of
biomass/3d

The reviewer
agreed with
this study's
overall quality
level.

Long et

al.
("19931

High


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report





made every
30 days.













Reductive
dechlorination in semi-
continuous digester
using a mixed culture
inoculum

50 irmol/L

anaerobic
microorganis
ms: Mixed
culture
isolated from
sludge of
urban
wastewater
treatment
plant (Bourg-
en-Bresse
France);
methanogenic
, sulfate-
reducing,
acetogenic
bacteria

anaerobic

37 days

Biodegradation
parameter:
percent
dechlorination:
100%/37 days

Biodegradation

parameter:
dechlorination
rate:

5.2	nmol/mg
protein/day

Biodegradation
parameter:
removal rate:

3.3	|iM day-1,
calc. during first
9 days; conc. of
trichloroethylen

e increased at
the same rate
during this time

The reviewer
agreed with
this study's
overall quality
level.

Cabirol
et al.
f19961

High

Non-guideline; closed
system, incubated in

the dark at 35 C,
inverted to minimize
gas leakage

<200 ng/L

activated
sludge,
adapted; To
the medium
was added
lOml/L of a
methanogenic

anaerobic

57 days

Biodegradation

parameter:
concentration

finitial
concentration:
200 ug/Ll:

The reviewer
agreed with
this study's
overall quality
level.

Bouwer

and
Mccartv

("19831

High


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report





mixed
culture,
grown in a
laboratory-
scale digester
fed waste-
activated
sludge, xylan
and cellulose.





160 |ig/L after

19d;
1.63 to
<10.7
irmol/L

other: First-
generation
and sixth-

anaerobic

Sixth
generatio
n:

Biodegradation

parameter:
Dercent removal

The reviewer
agreed with
this study's

Freedma

n and

High


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

reactor with an



generation



Methanol

via

overall quality

Gossett



anaerobic enrichment



enrichment



42 to 110

dechlorination:

level.

("19891



culture



culture



days;

>99% (0.15 to











obtained



Glucose

0.81%











from semi-



25 to 114

remaining);











continuous



days;

Biodegradation











reactor,



semi-

parameter:











operated at



continuou

dechlorination











35C with



s

products:











digested



operation

Ultimate











sludge



16-90

product: ethene:











obtained



days

intermediates











from



followed

products: vinvl











anaerobic



by

chloride(major),











digester



incubatio

TCE, 1,2-DCEs;











seeded from



n period

Biodegradation











Ithaca



7-30 days

parameter:











wastewater





dechlorination











treatment





rate: after 309











plant





days 36.4 |.unol

















PCE consumed,

















4.90 nmolVC

















and 12.0 |imol

















ethene

















remained.

















Reductive

















dechlorination

















was not suitable

















unless an

















electron donor

















was present








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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

Non-guideline
incubation

10 mg/L

other: aquifer

material -
Traverse City
Microcosms

anaerobic

250 days

Biodegradation

parameter:
transformation
rate: -4.43+/-
0.95 |iM/day.
Similar results
obtained in the
presence of
toluene,
ethylbenzene or
benzoate.

The reviewer
agreed with
this study's
overall quality
level.

Edwards
et al.
("19921

High

Non-guideline
incubation

<10 mg/L

other; aquifer
material -
Pensacola
Microcosms

anaerobic

250 days

Biodeeradation

parameter:
transformation
rate: -1.45+/-
0.34 |iM/day
(day 1-40) and -
2.16+/-0.34
l_iM/day (day

116-131).
Similar results
obtained in the

presence of
toluene under

the same
conditions but
not when no
other organic
compounds
were present
with a stable
toluene

The reviewer
agreed with
this study's
overall quality
level.

Edwards
et al.

("19921

High


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Interagency Review Draft Document. Do Not Release or Distribute.

















Data

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Quality
Evaluatio
n Results
of Full
Study
Report











degrading
suspended

















consortia

















derived from the

















Pensacola

















microcosms.

















Biodegradation

















parameter:
transformation







Non-guideline
incubation

<10 mg/L

other; aquifer
material -
Tyndall
Airforce Base

anaerobic

85 days

rate in toluene
amended
sample: 0.013+/-
0.066 |iM/day.

PCE not
transformed in
the presence of
benzoate or
phenol.

The reviewer
agreed with
this study's
overall quality

Edwards
et al.
("19921

High





Microcosms





level.















Biodegradation

















parameter: test

substance
transformation

rate: 0.0
|iMol/mg total
suspended
solids/h

The reviewer





non-guideline;
screening test

6.5 |rm

other;
Hanford soil
microcosms

aerobic

30 hours

agreed with
this study's
overall quality
level.

Kim et

aL

("20001

High

non-guideline

anaerobic
biodegradation
experiment

17-176
Hg/mL

other;
methanogenic
mixed culture
grown in a
laboratory-
scale

anaerobic

16 weeks

Biodegradation

parameter:
concentration:
56 |ig/L after
16w for 176

The reviewer
agreed with
this study's
overall quality
level.

Bouwer
et al.
119811

High


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report





digester fed
waste-
activated
sludge





|ig/L initial
concentration;
20 |ig/L after
16w for 36 |ig/L

initial
concentration;
7 |ig/L after 16w
for 17 |ig/L
initial
concentration;
limited
degradation







Static-culture flask-
screening test

5 and 10
mg/L

sewage,
domestic,
non-adapted;
Settled
domestic
wastewater

aerobic

28 days
(includes
7-day
static
incubatio
n and 3
weekly
subcultur
es)

Biodegradation

parameter:
percent removal
45%/7d and
87%/28d (5
mg/L initial
concentration);
30%/7d and
84%/28d (10
mg/L initial
concentration)
Significant
degradation with
rapid adaptation

The reviewer
agreed with
this study's
overall quality
level.

Tabak et

al.
119811

High

Granular sludge from
USAB reactor treating
sugar beet refinery
wastewater

1000-1500
nmol/batch

activated
sludge,
industrial,
non-adapted;

Granular
sludge from

anaerobic

65 days

Biodegradation
parameter: rate
constant f first

order
transformation
kinetics"): 0.048

The reviewer
agreed with
this study's
overall quality
level.

van
Eekert
et al.

f2oon

High


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report





USAB reactor
treating sugar
beet refinery
wastewater





day-lg-1 volatile
suspended
solids;
Biodeeradation
parameter:
product:
trichloroethene;

Some
disappearance of
test substance
was seen in
presence of
autoclaved
sludge.







Other; Static
microcosms

4.2 mg/L

natural
water/sedim

ent:
freshwater;
Sediment
included
muck from
vegetation
decay and
marl
(carbonaceou
s precipitate

of algal
growth). 4g
muck or 6g
marl used.

aerobic

16 weeks

Biodegradation

parameter:
Concentration

(ug/L) of
degradation
products f95%
confidence
interval in
parentheses'):
Trichloroethene:
Week 0 - ND;

Week 2 -
510(4,175);
Week 16 - Trace.
Cis-DCE: Wk 0 -

ND, wk 2 -
300(1,360), wk
16 ND. Trans-

The reviewer
agreed with
this study's
overall quality
level.

Parsons
et al.
("19851

High


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Interagency Review Draft Document. Do Not Release or Distribute.

















Data

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Quality
Evaluatio
n Results
of Full
Study
Report











DCE: WkO-ND,

















weeks 2 and 4 -

















trace, wk 16 -

















ND.

















Transformation

















was not

















observed in

















nonviable

















microcosms











anaerobic

















microorganis





Biodegradation











ms; Pure
cultures





parameter:
percent removal:







Pure culture anaerobic

dehalogenation;
isolation of strain and
optimization of growth

50-200
mmol/L

(strain TT4EQ
obtained

from
anaerobic
sediments
from a stream
in

Massachusett
s

contaminated
with TCE and
toluene

anaerobic

10 days

100%/10d;
Biodegradation
parameter:
degradation
products:
trichloroethylen

e and cis-
dichloroethylene

. No abiotic
dehalogenation
was observed.

The reviewer
agreed with
this study's
overall quality
level.

Krumhol
z et al.
f19961

High

Non-guideline

3.33 |Tg/mL
[approx.]

other; muck

from the
Everglades

anaerobic

30 days

Biodegradation
parameter: Half-
life: 34 days



Wood et

aL
ri98ii

High

Reductive
dechlorination in a
semi-continuous
reactor with an

>3.5 <55
irmol/L

other;
Methanol-

PCE
Enrichment

anaerobic

195 days

Biodegradation

parameter:
percent removal
via

The reviewer
agreed with
this study's

Di Stefan
o et al.
ri99ii

High


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

anaerobic enrichment
culture



culture using
a

methanogenic

bacterium
and a method

reference
(HER028022
94)





dechlorination:

100%/2-4d;
Biodegradation
parameter:
degradation
products:
ethene with very
little or no vinyl
chloride and

negligible
quantities of
trichloroethene
and

dichloroethene
isomers.

overall quality
level.





Non-guideline; other



other:
Anaerobic
mixed culture
known to be
capable of
dechlorinatin
g PCE to
ethene
seeded with

aquifer
material from

a PCE-
contaminated

site in
Victoria, TX

anaerobic

1 hour

Biodeeradation

parameter:
Dechlorination
rate: 77 |iM/day

The reviewer
agreed with
this study's
overall quality
level.

Hasten

and
Mccartv

("19991

High

Non-guideline; other

6.98 mg/L

activated
sludge

aerobic/anaer
obic

14 days

Biodeeradation
Darameter:

The reviewer
agreed with

Kastner

("19911

High


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report





(adaptation

not
specified);
enrichment
cultures from
contaminated
groundwaters
from site
former
solvent-
recycling
factor in
Germany





percent removal:
anaerobic:
0%/14d
Biodegradation

parameter:
removal: aerobic
changed to
anaerobic
conditions: some
transformation/

14d;
Biodegradation
parameter:
degradation
products: 100%
transformation
of PCE to cis-1,2-
dichloroethylene
(cDCE)
in aerobically

prepared
medium with
nitrogen atm

this study's
overall quality
level.





Influents and effluents
of 27 Korean WWTPs
screened for 22
chemicals



activated
sludge,
industrial
(adaptation

not
specified);
Various
treatment
processes

not specified

3 months

Biodesradation

parameter:
percent removal

f aver age.
estimated from
graph!: 72%

Removal
Percentage %
(degradation,

The reviewer
agreed with
this study's
overall quality
level.

Lee et al.

f.20151

High


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report





used: 15 used
activated
sludge
process,
remaining

used
sequencing
batch
reactors,
biological
nutrient
removal
process,
chemical
coagulation

and
sedimentatio
n, or contact
oxidation.





volatilization,
sorption to
solids, all
included in
"removal")







Continuous flow
column study

110 mg/L

anaerobic
microorganis
ms

anaerobic

2- or 4-
days
detention
time

Biodegradation

parameter:
percent removal:

99.98%
Biodeeradation
parameter:
Degradation
products:
trichloroethylen
e,

dichloroethylene
, vinyl chloride,
and carbon

The reviewer
downgraded
this study's
overall quality

rating. They
noted: Control
groups were
not reported,
limiting study
evaluation.

Voeel

and
Mccartv

("19851

Low


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report











dioxide; a
stepwise
degradation
scheme was
proposed.







Continuous-flow
column study

0.76 mg/L

anaerobic
microorganis
ms;

Methanogenic
bacteria

anaerobic

10 and 22
days

Biodegradation

parameter:
concentration:
300 |ig/L to 5
lig/L-

Biodegradation
parameter:
Degradation
products:
trichloroethylen
e,

dichloroethylene
, vinyl chloride,
and carbon
dioxide; a
stepwise
degradation
scheme was
proposed.

The reviewer
agreed with
this study's
overall quality
level.

Voeel

and
Mccartv

("19851

High





other; Pure
cultures:
Pseudomonas
stutzeri 0X1,
Luria-Bertani

growth
medium at 30
C

aerobic

24 hours

Biodegradation
parameter:
Degradation
products: 65%
chloride ion
generated

Initial
degradation

The reviewer
agreed with
this study's
overall quality
level.

Rvoo et

al.

T20001

High


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report











rates
determined by
sampling every 7
min for up to 2
hours







Non-guideline

91 mg/L

PCE-MeOH
enrichment
culture, yeast
extract

anaerobic

60 days

Biodegradation
parameter:

reaction
conditions:
Hydrogen was
able to serve as
the electron
donor in
reductive
dechlorination of
perchloroethyle
ne to vinyl
chloride and
ethylene over
periods of 14-40
days.

The reviewer
agreed with
this study's
overall quality
level.

Di Stefan
o et al.
119921

High

Simulated seasonal
field study



natural
water:
marine; NR

aerobic



Biodegradation
parameter: half-
lives: 25 d
(spring), 14 d
(summer), 12 d

(winter)
Volatilization
dominated the
loss of test
material

The reviewer
agreed with
this study's
overall quality
level.

Wakeha
m et al.

("19831

Medium


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

Simulated seasonal
field study

0.5 to 2
irmol/L

natural
water:
marine; NR

aerobic

24 hours

Biodegradation
parameter: half-
lives poisoned
with HsCl? and
not poisoned,
respectively:
12.1 d and 12.0
d;

Based on the
half-lives with
and without
HgC12 poisoning,
the loss of test
material was
determined to be
primarily by
volatilization.

The reviewer
agreed with
this study's
overall quality
level.

Wakeha
m et al.

("19831

Medium

Degradation in muck-
water

200 ng

natural
water;
Everglades
muck and

water
collected on
Feb 12,1979

not specified

70 days

Biodegradation

parameter:
percent removal:
100%/70 days
Biodegradation
parameter: half-
life: 33.8 days

(primary
degradation)

The reviewer
downgraded
this study's
overall quality
rating. They
noted: The

starting
material had
reported
impurities.

Dow
Chemica

1 ("19801

Medium

The influent and
effluent concentrations
of several VOCs were

measured at two
WWTPs and compared



activated
sludge,
industrial,
adapted

aerobic



Biodegradation

parameter:
predicted DCM
biodegradation
removal: WWTP

The reviewer
agreed with
this study's
overall quality
level.

Namkun

e and
Rittman
n ("19871

Medium


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

to a model developed
by the authors that
estimated VOC

removal by
volatilization,
adsorption, and
biodegradation based

on the WWTP
operational conditions.









#1: 84% (mainly

by

volatilization);

WWTP #2:
83.1% (mainly
by volatilization)







Degradation/dechlorin
ation using an
enrichment culture

300 and 600
irmol/L

other;
Enrichment
culture of
over 98%
Dehalococcoi
des, obtained
in 3 phases;
microcosm
set up with
groundwater

from
chlorinated
ethene-
contaminated
anaerobic
aquifer in
Bitterfeld
Germany;
preparation
methods
described
briefly and
referenced

anaerobic

120 days

Biodegradation

parameter:
percent removal:
100%/110d;
Biodegradation
parameter:
degradation
products: vinvl
chloride, ethene

The reviewer
agreed with
this study's
overall quality
level.

Cichocka
et al.
f20101

Medium


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Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

Anaerobic continuous-
flow column studies

>4.4 |ig/L
and <20.5
mg/L

anaerobic
bacteria;
Methanogenic
bacteria in a
continuous
column;
active
methanogenic
conditions
established
over several
years through

periodic
treatment of

different
organic waste
streams

anaerobic

22 days;
Liquid
detention
in large
column =
6 days;
small
column =
2-4 days

Biodegradation

parameter:
percent removal:
98-99.98%
(primary
reduction during
the small column
experiments);
Biodegradation

parameter:
concentration:
300 |ig/L was

reduced to
below 5 |ig/L
(the large
column
experiments)

The reviewer
downgraded
this study's
overall quality

rating. They
noted: Control
groups were
not reported,
limiting study
evaluation.

Vogel

and
Mccartv

("19851

Low

calculation



not specified

anaerobic



Biodegradation
parameter:
reduction
potential for
transformation
half-reactions:
PCE to TCE -0.7
volts at 0 and
lOOdegC.

The reviewer
downgraded
this study's
overall quality
rating. They
noted: Study
reports
calculated
estimates with
limited details
for endpoints
related to fate
(thermodynam
ic property).

Haas
and
Shock
119991

Low


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

Anaerobic
biodegradation

1.06 mg/L

anaerobic

sludge;
anaerobic
microorganis
ms from a
municipal

waste
treatment
plant

anaerobic

100 days

Biodegradation

parameter:
percent removal:
100%/40d

The reviewer
downgraded
this study's
overall quality
rating. They
noted: Due to

limited
information,
evaluation of
the

reasonableness

of the study
results was not
possible.

Gossett
("19851

Low

non-guideline aerobic
biodegradation
experiment

8.8+/-15%
and 74+/-
15% |.ig/mL

other;
Primary
sewage
effluent Palo
Alto, CA,
Water
Pollution
Control
Facility

aerobic

25 weeks

Biodegradation
parameter:

percent
remaining:
120-125%
relative to
control samples;
limited
degradation

The reviewer
downgraded
this study's
overall quality

rating. They
noted: Greater
than 100% of
test substance
was remaining
relative to the
controls after
25 weeks.

Bouwer
et al.
ri98n

Low

Pure culture study
using anaerobic
methanogenic bacteria

>1 to <3
mg/L

Methanosarci
na sp. strain

anaerobic

13 days

Biodegradation
parameter: rate
constant:
5.7-6.0
nmol/day;

Species specific
biodegradation
study excluded.

Fatherm

re and
Bovd
119881

Unaccepta
ble


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report











Biodegradation
parameter: CH4
production rate

constant:
180 nmol/day
during the active

phase of
methanogenesis







Batch sewage sludge
microcosm experiment



digested
sludge;
digester
sludge from

several
industrial and
municipal

sewage
treatment
plants canton

de Vaud
(Switzerland]

anaerobic



Biodegradation

parameter:
percent removal
in test svstem:
No degradation
or loss occurs

Biodegradation
results were
not reported
for

Perchloroethyl
ene.

Balsieer
et al.

T200S1

Unaccepta
ble


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

Anaerobic
biodegradation with
municipal solid waste
(MSW), biowaste,
and/or compost

4 to 5
mg/kg

other;
Digester filled
with MSW,
biowaste, or
compost;
MSW from
unsorted
waste from
households,
trade and
communities,
organic waste
from private
households of
Hamburg
Germany

anaerobic

Not
specified;

likely
>130 days

Biodegradation

parameter:
degradation rate
in test svstem:

PCE was
degraded at a
low rate under
acidic conditions
and at a higher

rate in the
methane phase
(however, only

very low
concentrations
of perc initially

added were
found in the gas
phase, attributed
to adsorption

and rapid
decomposition

The study did
not include or
report control
groups to
validate the
system used.

Deioser

and
Ste eman
n ("19971

Unaccepta
ble

Degradation in open
and closed systems

>0.1 to <1
ppm

natural
water:
marine;
Seawater
collected
from outside
Lysekil on the
Swedish
Coast

not specified

14 days

Biodegradation

parameter:
percent removal

in open-light,
closed-light, and
closed-dark

svstems.
respectivelv:
50%, 40%, 54%

Serious
uncertainties
or limitations
were identified

in sampling
methods of the
outcome of
interest. In
addition, loss
from leaks in
valves and

lensen

and
Rosenbe

rg
("19751

Unaccepta
ble


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report













open test
systems were
likely to have a

substantial
impact on the
results, making
the study
unusable.





non-guideline;
Modified shake flask

closed bottle
biodegradation test



not specified

aerobic



Biodegradation

parameter:
percent removal:
0%/21d
Possibly
multiple studies
(1) Acclimation
period with
adaptive
transfers after
48 or 72h with

and without
lactose; (2) No
biodegradation
after 2 Id
acclimation
period in a river
die-away study
without co-
substrate

Testing
methods and
conditions
were not
reported, and
data provided

were
insufficient to

interpret
results in this

secondary
source; citing
HERO ID
18157,
Mudder, T. I.

and J. L.
Musterman
(1982).

ECHA
f2017bl

Unaccepta
ble

inhibition of gas
production to
anaerobic sludge from

1000mg/L

sewage,
domestic
(adaptation
not

anaerobic

48 hours

Parameter:
inhibition of gas

production:
7.3% inhibition

Study
describes
inhibition of
gas production

Dow
Chem Co

("19771

Low


-------
Interagency Review Draft Document. Do Not Release or Distribute.

















Data



Initial
Concentrati
on











Affiliate

Quality
Evaluatio
n Results
of Full
Study
Report

Study Type (year)

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

d

Referen
ce

an operating municipal
sludge digester



specified); Mt
Pleasant MI
WWTP





at 10 mg/L; 20%
inhibition at 100
mg/L; 36% at
300 mg/L; 50%
at 550 mg/L
after 48h

not

biodegradation

rates or
transformation
pathways.















Biodegradation







non-guideline;
Degradation in muck-
water

200 ng

Everglades
muck and

water
collected on
Feb 12,1979

Not specified;
anaerobic
conditions
assumed

70 days

parameter:
unspecified:
100% after 70

days;
Biodegradation
parameter: half-
life: 33.8 days

(primary
degradation).
The estimated
time to complete
decay of200ug

Testing
conditions
were not
reported, and
data provided

were
insufficient to

Dow
Chemica

1 ("19801

Medium











interpret
results.















appears to be
approximately
70 days.







Sediment











Biodegradation







other; Non-guideline

500 ng/L

natural
water/sedim

ent:
freshwater

aerobic/anaer
obic

436d

parameter:
percent removal:
90% on days
338-436;
16% during day
140-337

The reviewer
agreed with
this study's
overall quality
level.

Chene et

aL
f20101

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

Static microcosm with

muck and surface
water in sealed septum
bottles

100

sewage,
domestic,
non-adapted

anaerobic

21 days

Biodegradation

parameter:
percent removal:
72.2%/21d

The reviewer
agreed with
this study's
overall quality
level.

Parsons
et al.
("19841

Medium

other; Reductive
dechlorination in
anaerobic sediment;
column and batch
studies

>0.6 to <9
irmol/L

natural
water/sedim
ent

anaerobic

Continuo
us-flow
column
>300
days;
batch >44
days

Biodegradation
parameter:
degradation
product: 95-98%
PCE was
recovered as
ethane under
steady-state
column
conditions in the
presence of
lactate

The reviewer
downgraded
this study's
overall quality
rating. They
noted: No
control groups
or validation
were reported.

de Bruin
et al.
("19921

Low

Anaerobic
biodegradation in Ni
contaminated
sediment

600 |Tmol/L

Anaerobic,
nutrient poor

sediment,
contaminated

with
chloroethene

and nickel,
collected at a
depth of 15m
near a former
metalworking
industrial
plant in the
Netherlands;
microbial pop

anaerobic

1 year (52
wks]

Biodeeradation
parameter:
degradation
products:
Ethene/ethane
production was
observed after
31 weeks; the
addition of
sulfate and
lactate were
necessary for
microbial
activity;
approximately 1

The reviewer
downgraded
this study's
overall quality

rating. They
noted: Specific
results stating
degradation
rates and/or
half-lives were
not reported.

Drzvzga
et al.

("20021

Low


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report





range10A2-
10A3 cells/g
of sediment
under sulfate
reducing
conditions





mM chloride was
detected in the
effluent
(background
from control was
0.5mM]







Microbial reductive
dechlorination of PCE
in sediment
microcosms

55 mmol/L

sewage,
domestic,
non-adapted

anaerobic



Biodegradation

parameter:
dechlorination
products:
Reductive
dechlorination of

PCE in
sediments from

3 locations
generated more
trans-DCE than

cis-DCE;
sediment from
one location
generated a
lower trans-/cis-
DCE ratio

The reviewer
downgraded
this study's
overall quality
rating. They
noted: Due to

limited
information,
evaluation of
the

reasonableness

of the study
results was not
possible.

Chene et

al.
f20101

Low

Soil


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Initial
Concentrati
on

Inoculum
Source

(An)aerobic
Status

Duration

Result

Comments

Affiliate
d

Referen
ce

Data
Quality
Evaluatio
n Results
of Full
Study
Report

Other; Biodegradation
in a continuous flow
system. Long-term
operation of a sand
column fed methanol
and concentrations of
PCE under anaerobic
continuous flow
conditions.

>12 to <720
irmol/L

Biomass from
an anaerobic
digester at
the

Metropolitan
Toronto Main
Treatment
Plant

anaerobic

2.5 years

Biodegradation

parameter:
removal rates
fthree different
column zones'):

1.23-1.60
|.unol/(h mg of
protein) at 0-15
cm; 0.21-0.26
|iMol/(h mg of
protein) at 0-30

cm; and 0.11-
0.13 |imol/(h mg
of protein) at 0-
45 cm.

The reviewer
downgraded
this study's
overall quality
rating. They

noted:
Continuous
flow reactor
with a sand
column that's
fed PCE and
methanol;
experiment a
treatment
system, the
study may not
be relevant to

fate and
environmental
degradation
and therefore
not applicable
to fate
assessment.

Isalou et

al.
f19981

Low


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Table 2. Bioconcentration Study Summary for Perch lor oethylene

Study Type
(year)

Initial
Concentratio
n

Species

Duration

Result

Comments

Affiliated
Referenc
e

Data
Quality
Evaluation
Results of
Full Study
Report

Bioconcentratio
n in Bluegill
sunfish:
Aquarium with
well-water and

modified
continuous-flow
proportional

dilution
apparatus for

chemical
introduction

3.43±1.53
^g/L

Bluegill
sunfish
(Lepomis
macrochirus
) 100 per
aquarium

Tetrachloroethylen
e 21 days; Test: 28

days or until
equilibrium; water
and fish samples

collected
periodically until

apparent
equilibrium was
reached or the max

exposure of28
days was reached

Bioconcentration
parameter: BCF:
49 (bluegill);

Bioconcentration
parameter: half-life:
< 1 day

The reviewer
agreed with this
study's overall
quality level. This
study is related to

another study,
HERO ID 3970785,

Echa.
Bioaccumulation:
aquatic/sediment:
Tetrachloroethylen
e. 2017.

Barrows
et al.
f19801

High









Bioconcentration
parameter: BCF DfUl:
118 (algae, uptake);







Kinetic uptake
measured via a
13C method and
ECD-GC method

0.22 or 0.50
mg/L

Skeletonema
costatum

72 hours

Bioconcentration
parameter:
BCF D(T): 113 (algae);
derived from exp data
for % inhibition and

exposure
concentration with
time

The reviewer
agreed with this
study's overall
quality level.

Wane et
al. P19961

High

Kinetic uptake
measured via a
13C method and
ECD-GC method

0.22 or 0.50
mg/L

Heterosigma
akashiwo

72 hours

Bioconcentration
parameter: BCF DfUl:
312 (algae, uptake);

Bioconcentration
parameter:
BCF D(T): 280 (algae);

The reviewer
agreed with this
study's overall
quality level.

Wang et

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type
(year)

Initial
Concentratio
n

Species

Duration

Result

Comments

Affiliated
Referenc
e

Data
Quality
Evaluation
Results of
Full Study
Report









derived from exp data
for % inhibition and

exposure
concentration with
time







"Bioaccumulatio
n test of a
chemical
substance in fish

or shellfish"
provided in "the
Notice on the
Test Method
Concerning New
Chemical
Substances"

0.1 and 0.01
ppm

Cyprinus
carpio

8 weeks

Bioconcentration
parameter: BCF:
25.8-77.1 [high);
28.4-75.7 (low) (carp)

The reviewer
agreed with this
study's overall
quality level. The
BCF study is also
available from the
NITE website.

Kawasaki
f19801

High

Uptake-
clearance of a
Perc commercial
product

0.06121 and
0.650 ppm

Rainbow
trout (Salmo
gairdneri]

48-hour exposure
followed by 144-
hour clearance

Bioconcentration
parameter: BCF:
39.7 (rainbow trout)

The reviewer
agreed with this
study's overall
quality level.

Dow
Chemical
fl9731

High

Method
described by
Branson et al
1974 for
determination of
BCF in Rainbow
trout

Two
concentration
s an order of
magnitude
apart

Salmo
gairdneri



Bioconcentration
parameter: BCF:
39.6 ± 5.5 (rainbow
trout)

The reviewer
agreed with this
study's overall
quality level.

Neelv et

;

Medium

Not specified



Golden ide
(Leuciscus
idus)



Bioconcentration

parameter:
unspecified: 90
(Golden ide)

Limited study
information
provided (i.e. study
controls not
reported).

Freitag et
al. fl9851

Unacceptabl
e


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type
(year)

Initial
Concentratio
n

Species

Duration

Result

Comments

Affiliated
Referenc
e

Data
Quality
Evaluation
Results of
Full Study
Report

Monitoring of
halogenated
hydrocarbons in
mollusks and

fish and
comparison to
concentrations
in seawater



Bassinum
undatum;
Modiolus,

Pecten
maximus;
Conger,
Gadus
morhua,
Pollachius

birens,
Scylliorhinu
s canicula,
Trisopterus
luscus



Bioconcentration
parameter: monitoring:
Relative to their
seawater levels these
compounds were only

slightly enriched;
usually by a factor of 2
- 25x (snails, scallops,
eels, marine fish)

Bioconcentration

parameter:
concentration in
organs:
brain>gill>liver>muscl
e; exceptions were
noted

The test substance
concentration in
seawater was not
reported. Results
provided are a
range of BCF (2-
2 5x) that are not
test compound or
organism specific.

Dickson
and Rilev
f19761

Unacceptabl
e

Long term
accumulation
experiment in

apparatus
similar to that
used for acute
tox

determination

0.03 and 0.3
mg/L

Dab

10 days and up to 3
months (3-35
days)

Bioconcentration
parameter:
accumulation factor in

organs:
5-9 times for flesh and
200-400 times for liver
(dab)

The study did not

report crucial
details on method,
sampling and
organisms.

Pearson

and
Mcconnell
C19751

Unacceptabl
e

Bioaccumulation

; purge-trap
method using a
Dean-stark
apparatus

5 and 100
lig/L

Mytilus
edulis

8 and 21 days

Bioconcentration
parameter: BAF:
25.7 (mussel)

Foreign language
paper with abstract
and data tables in
English. Full text
article review
needed when
available in English.

Saisho et
al. f19941

Unacceptabl
e


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Table 3. Photolysis Study Summary for Perchloroethylene

Study Type
(year)

Wavelength Range

Duration

Result

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of Full
Study Report

Air

Other; calculation

Atmospheric
lifetime in three
regimes of the
troposphere
based on OH
Reaction rate
constant





Photodegradation
parameter:
Tropospheric
lifetime at 288 K.
263 K. and 260 K.

respectivelv:
80,119, and 251
days

The reviewer agreed

with this study's
overall quality level.

U.S. EPA ("19871

High

Other; Test
material injected
into quartz flask
containing air to
give

concentrations in
the range of 10-7
to 10-4 by mass.

Outdoor light



Photodegradation
parameter: direct
photolvsis half-
life:

50%/12 weeks

Testing conditions
were not reported,
and data provided
were very general;
concentration of test

material not
specified. Ambient

air used for
experiment was not
subject to any
pretreatment or
analysis; climate and
conditions were not
controlled.

Pearson and
Mcconneii f19751

Unacceptable

Water

Direct photolysis
in quartz tubes

366 nm

5 days

Photodegradation
parameter: direct
photolvsis:
Negligible

The reviewer agreed

with this study's
overall quality level.

Chodola et al.

fl9891

High

Photodegradation
in water (indirect
photolysis)

185-254 nm

60 minutes

Photodegradation
parameter:
indirect
photolvsis rate
constants:

The reviewer agreed

with this study's
overall quality level.

Shiravama et al.

f20011

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type
(year)

Wavelength Range

Duration

Result

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of Full
Study Report







0.221 kdeg min1
(oxygenated) and
0.287 kdeg min-
ifoxygen free)
Photodegradation
parameter:
indirect
photolvsis half-
lives:
3.75 min
(oxygenated) and
3.39 min (oxygen
free)







Nonguideline lab
study - direct
photolysis

sunlight

1 year

Photodegradation
parameter: direct
photolvsis half-
life:

50%/8.8 months

The reviewer agreed

with this study's
overall quality level.
Related HERO ID,
Echa.

Phototransformation

in water:
Tetrachloroethylene.
2017.

Dilline et al.
fl9751

High

Photoinduced
reductive
dechlorination in
water containing
ferrous and/or
sulfide ions

Intensity 530±20 lux

33 days

Photodegradation
parameter:
indirect:
reductive
dechlorination:
No appreciable
degradation was
observed with
any medium with
or without
photolysis

The reviewer agreed

with this study's
overall quality level.

Dooneand Wu
119921

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Table 4. Hydrolysis Study Summary for Perchloroethylene

Study Type
(year)

PH

T emperature

Duration

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of
Full Study
Report

Nonguideline;
hydrolysis
study

4 and 9.2

4 and 502C (at both
pH values)

7 days

Hvdrolvsis
parameter:
conditions for
reaction:
Under acidic and
basic conditions,

the percent
difference of areas

at 4 and 502C
ranged between -

14% to +1%
indicating that the

chance for
transformation of
tetrachloroethylene
by hydrolysis
under
environmentally
relevant conditions
of temperature and
pH is minimal.

The reviewer
agreed with this
study's overall
quality level.

Chodola et

al. ("19891

High

Nonguideline
lab study in
Pyrex tubes
with light-

proof
container,
shaken every

2-weeks,
water purged
with air for
15 min prior



approx. 252C

1 year

Hvdrolvsis
parameter: half-
life:

50%/8.8 months

The reviewer
agreed with this
study's overall
quality level.

Dilling et al.
("19751

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type
(year)

PH

T emperature

Duration

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of
Full Study
Report

to addition of
chlorinated
compounds















Alkaline
homogenous

hydrolysis
experiments;
a range of pH

and
temperature
evaluated.
Arrhenius
temperature
dependence
assumed.

2-14

130-1702C

30 min to several
days (for all test
materials; specific

duration for
tetrachloroethylene
not specified)

Hvdrolvsis
parameter: half-life

fpH 7.25 °C1:
50%/9.9xl08 years

The reviewer
agreed with this
study's overall
quality level.

leffers et al.
119891

Medium

Table 5. Sorption Study Summary for Perch lor oethylene

Study Type (year)

Sorbent Source

Sorbent
Qualities
(clay/silt/sand,
OC, pH)

Duration

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of
Full Study
Report

Other; Non-guideline
study using bottle-point
method for isotherm
experiments

Filtrasorb 400
activated carbon
at 500 and 1500

m/u

Background
organic matter
was treated old

municipal
landfill leachate

DOC 300 mg/L

2 weeks

Sorption
parameter: Kf:
MilliO water:
7.071 ±0.09
(mg/g)/(ng/L)

and
l/n = 0.4412
±0.0061

The reviewer agreed

with this study's
overall quality level.

Serial et al.
f19941

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Sorbent Source

Sorbent
Qualities
(clay/silt/sand,
OC, pH)

Duration

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of
Full Study
Report



in Dover,
Delaware













OECD Guideline 106

(Adsorption -
Desorption Using a
Batch Equilibrium
Method)

7 samples of
Danish clayey till
from three sites
at depths of 2.4
to 9.5 m below
the surface (4
contaminated; 3
uncontaminated)

foc% 0.02-0.08;
% Clay content
23.0-27.0; 4
samples
reduced clayey
till; 3 samples
oxidized clayey
till



Sorption
parameter: Kd

f3 sites,
oxidized clavl:

1.55±0.08,
1.03±0.02, and
0.84±0.05;

Sorption
parameter: Kd

f4 sites,
reduced clavl:
2.41+0.07,
2.16±0.05,
2.45±0.08, and

I.81±0.14;

Sorption
parameter: Kf

f oxidized
clavl:

II.25±3.80;

Sorption
parameter: Kf

(2 sites,
reduced clavl:
21.30±4.11

and
32.56±14.3

The reviewer agreed

with this study's
overall quality level.

Lu et al.
f.20111

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Sorbent Source

Sorbent
Qualities
(clay/silt/sand,
OC, pH)

Duration

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of
Full Study
Report









Sorption
parameter: log
Kd fcalculated
from log Kd =

0.590 log
Kow-1.5611
f oxidized
clavl:
3.29, 3.54, and
3.62
Sorption
parameter: los
Kd fcalculated
from log Kd =

0.590 log
Kow-1.5611
f reduced
clavl: 3.78.
3.86, 3.69, and
3.41







Other; Non-guideline
study

pulverized
sediment (5-50
g] with a known
volume of
synthetic
groundwater (5-
17 mL] and mass

of PCE, from
methanol stock
solution, was
either flame
sealed into a
glass ampoule or
sealed with a

Three samples
consisted of
sand and gravel
and three
samples
consisted of
medium to fine
sand.



Sorption
parameter:
Kd: sand and

gravel:
0.82,1.16, and
1.92

Sorption
parameter:
Kd: medium to

fine sand:
0.8,1.16, and
0.82

The reviewer agreed

with this study's
overall quality level.

Wane et al.
f20131

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Sorbent Source

Sorbent
Qualities
(clay/silt/sand,
OC, pH)

Duration

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of
Full Study
Report



PTFE-lined butyl
rubber septum
into serum vial













Other; Sorption on
wastewater solids
(isotherm test)

Wastewater
solids collected
from three
different
municipal
WWTP near
Cincinnati, OH

Mixed-liquor
solids, primary

sludge,
anaerobically
digested sludge



Sorption
parameter:
adsorption
coefficient K:

primarv
sludge, mixed-
liquor solids
and digested.

sludge,
respectivelv:
0.60, 0.90,
0.70

Sorption
parameter: log

Kp: primarv
sludse. mixed-
liquor solids
and digested.

sludge,
respectivelv:
2.90,3.01,
3.09

The reviewer agreed

with this study's
overall quality level.

Dobbs et al.
119891

High

Other; Vapor
partitioning/ adsorption
in aquifer solids

Aquifer solids

from
contaminated
aquifers in
Livermore
Valleys CA with

low natural
organic matter

Sand clay and
silt: Surface
area: 13-29
m2/g; Organic
content 0.0064-
0.11%; particle
diameter: <75-
150 |im; Sand



Sorption
parameter: Kf:
0.0048
(nonlinear
isotherm 1/n
= 0.62)

The reviewer agreed

with this study's
overall quality level.

Farrell and
Reinhard
f19941

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Sorbent Source

Sorbent
Qualities
(clay/silt/sand,
OC, pH)

Duration

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of
Full Study
Report



sediment with

sand-sized
aggregates in
clay and silt

portion: internal
porosity 0.54
mL/g; pore
diameter: 69
Angstrom











Other; Vapor
partitioning/ adsorption
in aquifer solids

Aquifer solids

from
contaminated
aquifers in Santa
Clara CA
consisting of
fragments of
sedimentary
rocks (54%),
single grains
(30%), igneous

and
metamorphic
rock fragments
(16%)

Column solids
were in
equilibrium
with 100%
relative
humidity;
desorption
isotherms
measured with
stepwise batch

techniques;
solids allowed
to adsorb PCE
vapors at ca.
79% saturation
and equilibrated
for 1 week,
purged and
equilibrate for
another 1-3
week



Sorption
parameter: Kf:
0.0054
(nonlinear
isotherm 1/n
= 0.43)

The reviewer agreed

with this study's
overall quality level.

Farrell and
Reinhard
f19941

High

Secondary source,
based on several
experimental studies







Sorption
parameter:
Koc:
141
(log Koc =
2.15)

The reviewer
downgraded this
study's overall
quality rating. They
noted: Limited

information
reported in this
secondary source

ECHA

f.2017al

Unacceptable


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Study Type (year)

Sorbent Source

Sorbent
Qualities
(clay/silt/sand,
OC, pH)

Duration

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of
Full Study
Report











and unable to
confirm study
results with cited
reference HEROID

3839195, ECB
(2005). European

Union risk
assessment report:
Tetrachloroethylene.

Part 1 -
Environment. United
Kingdom, European
Commission - Joint

Research Centre
Institute for Health

and Consumer
Protection European
Chemicals Bureau.

57.





Table 6. Other Fate Endpoints Study Summary for Perchloroethylene

System

Study Type (year)

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of Full
Study Report

Measured concentrations
of tetrachloroethylene in
sediments of Scheldt
Estuary and water
samples from Southern
North Sea

Partitioning based on

measurements in
sediments of Scheldt
Estuary and water
Southern North Sea

Parameter: log Koc fsw.
ecQl

1.58 (Log Koc, sw: 0.94,
1.83,1.99,2.34; Log Koc
0.92,1.82,1.96,2.26)

The reviewer agreed
with this study's overall
quality level.

Roose et al.

f2oon

High


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Interagency Review Draft Document. Do Not Release or Distribute.

System

Study Type (year)

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of Full
Study Report





Biodeeradation







Anaerobic batch fed
reactor

digested sludge; Municipal
anaerobic digester sludge

parameter: test reactor
influent/effluent
comparison:
.Average reactor influent

of Perc = 120 ug/L,
average reactor effluent
= 3 ug/L

The reviewer agreed
with this study's overall
quality level.

Lone et al.
("19931

High





Biodegradation







Aerobic batch fed reactor

digested sludge; Municipal
anaerobic digester sludge

parameter: test reactor
influent/effluent
comparison:
Average reactor influent
= 160 ug/L; average
reactor effluent = 42
ug/L

The reviewer agreed
with this study's overall
quality level.

Lone et al.
("19931

High





Parameter: WWTP











influent/effluent











comparison:
Tetrachloroethene was











detected in 94% of







Analysis of NYC
municipal wastewaters;



influent samples and
74% of effluent samples;







Influent and effluent
samples were collected

Analysis of NYC municipal
wastewaters from 1989-

the concentration range
detected in influent was

The reviewer agreed
with this study's overall

Stubin et al.
("19961

High

from 14 Water Pollution

1993

5-78 |ig/L and effluent

quality level.



Control Plants in New



was 1-69 |ig/L.







York City



Tetrachloroethene was
one of five commonly

observed volatiles
detected; present in at
least a third or more of
all the samples analyzed.







VOCs injected into water



Parameter: percent

The reviewer

Tancrede et

Low

line of shower and glass



volatilization at 25 °C. 33

downgraded this study's

al. (19921


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Interagency Review Draft Document. Do Not Release or Distribute.

System

Study Type (year)

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of Full
Study Report

syringes were used to
collect air and water
samples.



°C. and 42 °C.
respectivelv:
56% +/-7%, 66% +/"?%
and 68% +/-7%

Parameter: percent
volatilization at 42 °C bv

flow rates:
69% +/-7% at flow rate
9.7 L/min and 68% +/-
7% at flow rate 13.5
L/min

overall quality rating.
They noted: Study

investigated
volatilization from
shower water. Study
results may not be
relevant to a
specific/designated Fate
endpoint.





Desorption profiles
obtained from PCE alone
and PCE mixed with TCE
in sediment

Diffusion/desorption on
natural solids

Parameter: Diffusion rate

constant of PCE alone
and PCE in mix with TCE.

respectivelv: 5.00E-
4/min (95%CI: 0.02E-4,
initial sorbed mass: 8.1
|ig/g) and 7.33E-4/min
(95%CI: 0.05E-4, initial
sorbed mass: 9.2 ng/g]

The reviewer agreed
with this study's overall
quality level.

C2.Q..Q1)

High

Modified EPA method
624

Stripping of volatile
organics from wastewater

Parameter: WWTP
influent/effluent
comparison:
88 and 139 |ig/m3 max
off gas samples; avg
influent and effluent:
0.2 |ig/L in water and 40
and 43 |ig/m3 in off gas
at skyway, influent and
effluent: 0.3 and 0.2 |ig/L
in water and 82 and 115
|ig/m3 in off gas at
highland creek

The reviewer agreed
with this study's overall
quality level.

Bell et al.

("19931

High


-------
Interagency Review Draft Document. Do Not Release or Distribute.

System

Study Type (year)

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of Full
Study Report

VOC's were measured in
water samples between
November 2006-June
2008; by comparing STE
and post-RO samples
matched to plant and
date the overall
treatment efficiency was
calculated as a
proportion of the
removal

Monitoring of water
samples and correlation to
treatment efficiency

Parameter: WWTP
removal efficiencv:
The median removal
efficiency was 91.2% for
tetrachloroethene; STE
samples (n=29): 86.2%
detections; post-MF
samples (n=9): 88.9%

detections; post-RO
samples (n=27): 14.8%
detections

The reviewer agreed
with this study's overall
quality level.

Rodriguez et
al. C20121

High

gravimetric
measurements by a
Mettler H54 balance

evaporation rates of
solutes from water

Parameter: volatilization
rates at 23.2 °C and 3.5
°C. respectively:
1.36E5 g/cm2-s and
4.77E4 g/cm2-s

The reviewer agreed
with this study's overall
quality level.

Chiou et al.

("19801

High

Refers to Hill et al.

Volatilization rate study
for high-volatility
compounds

Parameter: volatilization

rate constant ratios
kvC/kvo: 0.52 +/- 0.09

The reviewer agreed
with this study's overall
quality level.

Smith et al.

("19801

High

Concentrations in air,
water and sludge phases
analyzed under four
different operational
circumstances evaluating
single and combined
effects of aeration and
sludge addition on phase
distributions; sludge

added prior to
experiments; aeration
3rd-10th hour

Fugacity model approach
to VOC fate in WWTP

Parameter: partitioning:
The concentrations of the
VOCs
in the air, water, and
sludge phases of the
bioreactor were analyzed
regularly. Mass
distributions indicated
that Perc was mainly
present in the water
phase throughout the
four treatment stages;
less than 1% of the total
mass was subject to
biological sorption
and/or degradation by

The reviewer agreed
with this study's overall
quality level.

Chen et al.
("20141

High


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Interagency Review Draft Document. Do Not Release or Distribute.

System

Study Type (year)

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of Full
Study Report





the sludge; water
aeration resulted in
increased partitioning to
the air phase with a
negative impact on
biological removal; Perc

mass distribution
throughout the 4 stages:
~99% water, ~0.4% air,
less than 0.1% sludge







Reductive
dehalogenation
measured in static
microcosms with 8 mL
leachate and 10 mM PCE
under 80%-N2:10%-

C02: 10%-H2
atmosphere with and
without organic carbon
amendments

Dehalogenation of PCE in
landfill leachates with and
without organic carbon
amendments under
anaerobic conditions

Extent of dehalogenation
was correlated with the
availability of organic
carbon; 19% degradation
after 14 days in low
carbon Cell 8 leachate
and almost all PCE and
some TCE degradation
after 30 days; greater
than 75% degradation
after 14 days in high car

The reviewer agreed
with this study's overall
quality level.

Leahv and
Shrevef20001

High



Concentration in seawater
and air

Parameter: seawater to

air flux:
0.02-160.4 (mean 34.3)
nmol nr2 d1

The reviewer agreed
with this study's overall
quality level.

He et al.
f20131

High

200 rpm stirring of the
solution with a shallow
pitch

propeller stirrer in still
air



Parameter: volatilization
half-life: 27.1 min

The reviewer agreed
with this study's overall
quality level.

Dillii

High

Transformation study
under anaerobic
conditions

non-guideline

Parameter: abiotic
dechlorination in the
presence of iron half-
lives at 50 °C and 23 °C
respectively:

The reviewer agreed
with this study's overall
quality level.

Schreier and
Reinhard

("19941

Medium


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Interagency Review Draft Document. Do Not Release or Distribute.

System

Study Type (year)

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of Full
Study Report





20d+/-4 and 38d+/-25;
dechlorination did not
occur in the presence of
manganese







wastewater flow: 41.5,
21,852,2390, 499,110
and 30.5 1/min. Volatile
organic loading rate:

14.6,	4.6,292,286,19,
5.29, 0.395 kg/L. Feed

ratio: 9.6,10.5,28.8, NA,

14.7,	7.1,1.4 kg/kg for
plants A-G respectively

7 steam stripper
operations are reported

Parameter: percent
removal from steam
stripper operations:
>99.2 and >99.89
removal from plant C and

D, respectively, no
removal plants A, B, E-G.

The reviewer agreed
with this study's overall
quality level.

Blanev 119891

Medium





Parameter: 8h TWA in
air:

150,280, 3800, 380 ppb;

Parameter: air
concentration:
0-20 ppm v/v;

Parameter: WW
concentration:
0.19-47 ng/L







Mill Creek, Little Miami
River, and Muddy Creek
treatment plants



The reviewer
downgraded this study's
overall quality rating.
They noted: The
volatility is reported for
3 sites in open systems.

Dunovantet
al. f19861

Low

continuous release of
chemicals and steady
hydrological parameters
assumed to develop a
steady-state model for
estimating concentration
in river

Hydrological data and
monitoring samples are
used to calculate
volatilization

Parameter half-life in
river:

4-6 d;

Perc release from the
river is variable with an
average value of 0.6%.
Mainly removed by
volatilization.

The analytical method
used for detection of the
test substance was not
reported.

Briieeemann

and Trace
("19881

Unacceptable


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Interagency Review Draft Document. Do Not Release or Distribute.

System

Study Type (year)

Results

Comments

Affiliated
Reference

Data Quality
Evaluation
Results of Full
Study Report

Full scale Wet Air
Oxidation [WAO] of
solvent still bottoms and
general organic waste
details are reported by

Radimsky and Shah
1985; parameters used
to measure performance
were COD, BOD, and
DOC; off-gas emissions
measured by THC as
methane;

Wet air oxidation
performance data

Parameter: percent
removal from test

svstem:
95.35% Effluent
concentration solvent
still bottoms of
tetrachloroethylene = 40
mg/L

Due to limited
information, evaluation
of the reasonableness of
the study results was not
possible.

Matienzo
("19891

Unacceptable

Performance data was
collected on full scale

batch fractional
distillation systems as
referenced in the source
document

Distillation performance
data

Parameter: performance
of test svstem:

Mean solvent
concentration of
distillation residues:
tetrachloroethylene 12
reported values, mean
concentration = 4;
feasible treatment level =
3.0 mg/kg

Due to limited
information, evaluation
of the reasonableness of
the study results was not
possible.

Matienzo
("19891

Unacceptable

Samples taken from
WWTP to evaluate air
stripping and removal of
Perc/PCE

Partitioning in activated
sludge plant

Parameter: percent
removal from WWTP:
78% removal of Perc/
PCE by full scale aeration
basin

Parameter: gas-liquid
phase partition
coefficient:
avg. 600 (+/-86) and 611
C+/-369) fng/LI/fng/L]

Study evaluates removal
based on air stripping.

The extent of air
stripping is a function of

the compound pchem
properties and a function
of WWTP design and
operation.

Parker et al.
("19931

Unacceptable


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Interagency Review Draft Document. Do Not Release or Distribute.

EPI Suite™ Model Outputs

SMILES : C(=C(C1)C1)(C1)C1
CHEM : TETRACHLOROETHENE
MOL FOR: C2 CL4
MOLWT : 165.83

	EPI SUMMARY (v4.11)	

Physical Property Inputs:

Log Kow (octanol-water): 3.40
Boiling Point (deg C) : 121.30
Melting Point (deg C) : -22.30
Vapor Pressure (mm Hg) : 18.5
Water Solubility (mg/L): 206
Henry LC (atm-m3/mole) : 0.0177

Log Octanol-Water Partition Coef (SRC):

Log Kow (KOWWIN vl.69 estimate) = 2.97
Log Kow (Exper. database match) = 3.40
Exper. Ref: HANSCH,C ET AL. (1995)

Boiling Pt, Melting Pt, Vapor Pressure Estimations (MPBPVP vl.43):

Boiling Pt (deg C): 114.28 (Adapted Stein & Brown method)

Melting Pt (deg C): -60.56 (Mean or Weighted MP)

VP(mm Hg,25 deg C): 17.8 (Mean VP of Antoine & Grain methods)

VP (Pa, 25 deg C) : 2.37E+003 (Mean VP of Antoine & Grain methods)
MP (exp database): -22.3 deg C
BP (exp database): 121.3 deg C

VP (exp database): 1.85E+01 mm Hg (2.47E+003 Pa) at 25 deg C

Water Solubility Estimate from Log Kow (WSKOW vl.42):

Water Solubility at 25 deg C (mg/L): 134.3
log Kow used: 3.40 (user entered)
melt pt used: -22.30 deg C

Water Sol (Exper. database match) = 206 mg/L (25 deg C)

Exper. Ref: HORVATH,AL ET AL. (1999)

Water Sol Estimate from Fragments:

Wat Sol (vl.01 est) = 247.12 mg/L

ECOSAR Class Program (ECOSARvl.ll):

Class(es) found:

Vinyl/Allyl Halides

Henrys Law Constant (25 deg C) [HENRYWIN v3.20]:

Bond Method : 1.65E-002 atm-m3/mole (1.67E+003 Pa-m3/mole)

Group Method: 1.77E-002 atm-m3/mole (1.80E+003 Pa-m3/mole)

Exper Database: 1.77E-02 atm-m3/mole (1.79E+003 Pa-m3/mole)

For Henry LC Comparison Purposes:

User-Entered Henry LC: 1.770E-002 atm-m3/mole (1.793E+003 Pa-m3/mole)
Henrys LC [via VP/WSol estimate using User-Entered or Estimated values]:
HLC: 1.960E-002 atm-m3/mole (1.986E+003 Pa-m3/mole)


-------
Interagency Review Draft Document. Do Not Release or Distribute.

VP: 18.5 mm Hg (source: User-Entered)

WS: 206 mg/L (source: User-Entered)

Log Octanol-Air Partition Coefficient (25 deg C) [KOAWIN vl.10]:

Log Kow used: 3.40 (user entered)

Log Kaw used: -0.140 (user entered)

Log Koa (KOAWIN vl.10 estimate): 3.540

Log Koa (experimental database): 3.480

Probability of Rapid Biodegradation (BIOWIN v4.10):

Biowinl (Linear Model) : 0.2230

Biowin2 (Non-Linear Model) : 0.0012

Expert Survey Biodegradation Results:

Biowin3 (Ultimate Survey Model): 2.1400 (months )

Biowin4 (Primary Survey Model) : 3.2060 (weeks )

MITI Biodegradation Probability:

Biowin5 (MITI Linear Model) : 0.3626

Biowin6 (MITI Non-Linear Model): 0.0227

Anaerobic Biodegradation Probability:

Biowin7 (Anaerobic Linear Model): 0.7775

Ready Biodegradability Prediction: NO

Hydrocarbon Biodegradation (BioHCwin vl.01):

Structure incompatible with current estimation method!

Sorption to aerosols (25 Dec C)[AEROWIN vl.00]:

Vapor pressure (liquid/subcooled): 2.47E+003 Pa (18.5 mm Hg)

Log Koa (Exp database): 3.480

Kp (particle/gas partition coef. (m3/ug)):

Mackay model : 1.22E-009

Octanol/air (Koa) model: 7.41E-010

Fraction sorbed to airborne particulates (phi):

Junge-Pankow model : 4.39E-008

Mackay model : 9.73E-008

Octanol/air (Koa) model: 5.93E-008

Atmospheric Oxidation (25 deg C) [AopWin vl.92]:

Hydroxyl Radicals Reaction:

OVERALL OH Rate Constant = 0.2139 E-12 cm3/molecule-sec
Half-Life = 49.998 Days (12-hr day; 1.5E6 OH/cm3)

Ozone Reaction:

OVERALL Ozone Rate Constant = 0.000073 E-17 cm3/molecule-sec

Half-Life = 15660.362 Days (at 7E11 mol/cm3)

Fraction sorbed to airborne particulates (phi):

7.06E-008 (Junge-Pankow, Mackay avg)

5.93E-008 (Koamethod)

Note: the sorbed fraction may be resistant to atmospheric oxidation

Soil Adsorption Coefficient (KOCWIN v2.00):

Koc : 94.94 L/kg (MCI method)

Log Koc: 1.977 (MCI method)


-------
Interagency Review Draft Document. Do Not Release or Distribute.

Koc : 892.2 L/kg (Kow method)

Log Koc: 2.950 (Kow method)

Experimental Log Koc: 2.4 (database)

Aqueous Base/Acid-Catalyzed Hydrolysis (25 deg C) [HYDROWIN v2.00]:
Rate constants can NOT be estimated for this structure!

Bioaccumulation Estimates (BCFBAF v3.01):

Log BCF from regression-based method = 1.910 (BCF = 81.34 L/kg wet-wt)
Log Biotransformation Half-life (HL) = 0.5257 days (HL = 3.355 days)
Log BCF Arnot-Gobas method (upper trophic) = 1.663 (BCF = 46.04)
Log BAF Arnot-Gobas method (upper trophic) = 1.663 (BAF = 46.04)
log Kow used: 3.40 (user entered)

Volatilization from Water:

Henry LC: 0.0177 atm-m3/mole (entered by user)

Half-Life from Model River: 1.357 hours

Half-Life from Model Lake : 122.8 hours (5.116 days)

Removal in Wastewater Treatment:

Total removal:	87.91 percent

Total biodegradation: 0.05 percent
Total sludge adsorption: 6.32 percent
Total to Air:	81.53 percent

(using 10000 hr Bio P,A,S)

Removal in Wastewater Treatment:

Total removal:	88.20 percent

Total biodegradation: 2.12 percent
Total sludge adsorption: 6.29 percent
Total to Air:	79.79 percent

(using Biowin/EPA draft method)

Level III Fugacity Model: (MCI Method)

Mass Amount Half-Life Emissions
(percent) (hr) (kg/hr)

Air 46	1.6e+003 1000

Water 46.8 1.44e+003 1000
Soil 6.87 2.88e+003 1000
Sediment 0.314 1.3e+004 0
Persistence Time: 181 hr

Level III Fugacity Model: (MCI Method with Water percents)

Mass Amount Half-Life Emissions

(percent) (hr) (kg/hr)

Air 46	1.6e+003 1000

Water 46.8 1.44e+003 1000

water (46.8)

biota (0.00587)

suspended sediment (0.00666)

Soil 6.87 2.88e+003 1000


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Interagency Review Draft Document. Do Not Release or Distribute.

Sediment 0.314 1.3e+004 0
Persistence Time: 181 hr

Level III Fugacity Model: (EQC Default)

Mass Amount Half-Life Emissions

(percent) (hr) (kg/hr)

Air 29.1 1.6e+003 1000

Water 30.4 1.44e+003 1000

water (30.3)

biota (0.00381)

suspended sediment (0.0469)

Soil 38.4 2.88e+003 1000

Sediment 2.03	1.3e+004 0

Persistence Time: 279 hr


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Interagency Review Draft Document. Do Not Release or Distribute.

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