v>EPA

United States
Environmental Protection
Agency

METHOD 561: DETERMINATION OF ENDOTHALL,
GLYPHOSATE, GLUFOSINATE, AND
AMINOMETHYLPHOSPHONIC ACID IN DRINKING WATER
BY DIRECT AQUEOUS INJECTION AND LIQUID
CHROMATOGRAPHY/TANDEM MASS SPECTROMETRY


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Technical questions concerning this analytical method should be addressed to:

William A. Adams, Ph.D.

U.S. EPA, Office of Ground Water and Drinking Water, Standards and Risk Management Division,
Technical Support Branch, 26 W. Martin Luther King Dr. Cincinnati, OH 45268
Phone:(513)569-7656
adams.william@epa.gov

Questions concerning this document or policy should be addressed to: safewater@epa.gov

Office of Water (MS-140)

EPA Document No. 815-R-25-013
EPA contract 68HERC22C0058
August 2025

Authors

Alan Zaffiro, APTIM (Cincinnati, OH) and Leah Villegas Ph.D., APTIM (Cincinnati, OH)

Contractor's role did not include establishing Agency policy.

Anthony Giovengo, Ph.D., U.S. EPA (Cincinnati, OH) and William A. Adams, Ph.D., U.S. EPA (Cincinnati,
OH)

Acknowledgements

Laura Rosenblum, Ph.D., APTIM (Cincinnati, OH)

The following organizations completed a validation study in their laboratories using this method,
provided valuable feedback on the method procedures and reviewed the draft method manuscript:

Shodex - Resonac America, Inc. (New York, NY)

Eurofins Eaton Analytical, LLC (South Bend, IN)

Merit Laboratories, Inc. (East Lansing, Ml)

Agilent Technologies, Inc. (Santa Clara, CA)

Disclaimer

This analytical method may support a variety of monitoring applications. Publication of the method, in
and of itself, does not establish a requirement, although the use of this method may be specified by the
EPA or a state through independent actions. Terms such as "must" or "required," as used in this
document, refer to procedures that are to be followed to conform with the method. References to
specific brands and catalog numbers are included only as examples and do not imply endorsement of
the products. Such reference does not preclude the use of equivalent products from other vendors or
suppliers.

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Table of Contents

1	Scope and Application	1

2	Method Summary	2

3	Definitions	2

4	Interferences	4

5	Safety	6

6	Equipment and Supplies	6

7	Reagents and Standards	8

8	Sample Collection, Preservation, and Storage	12

9	Quality Control	12

10	Calibration and Standardization	18

11	Procedure	21

12	Data Analysis and Calculations	22

13	Method Performance	23

14	Pollution Prevention	24

15	Waste Management	24

16	References	24

17	Tables, Figures and Method Performance Data	25

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Tables

Table 1. Preparation of Synthetic Matrix Solution	10

Table 2. Preparation of Internal Standard Stocks from Neat Materials	10

Table 3. HPLC Method Conditions for Sample Injections	25

Table 4. HPLC Conditions for EDTA Pre-lnjections and Gradient Recycle	25

Table 5. ESI Method Conditions	26

Table 6. Analyte RTs, MRMs, and MS/MS Method Conditions	26

Table 7. LCMRL Results	26

Table 8. Precision and Accuracy Data for Reagent Water	27

Table 9. Precision and Accuracy Data for a Ground Water Matrix	27

Table 10. Precision and Accuracy Data for a Surface Water Matrix	27

Table 11. Precision and Accuracy Data Synthetic Sample Matrix	28

Table 12. Precision and Accuracy Data for a Finished Surface Water with Orthophosate Anti-Corrosive
Agent	28

Table 13. Aqueous Sample Holding Time Data for a Ground Water Matrix	29

Table 14. Aqueous Sample Holding Time Data for a Surface Water Matrix	29

Table 15. Initial Demonstration of Capability (IDC) Quality Control Requirements	30

Table 16. Ongoing Quality Control Requirements	31

Figures

Figure 1. Relative Retention of Early Eluting Preservatives to the Method Analytes in High-Hardness
Water	32

Figure 2. Relative Retention of Late Eluting Preservatives to the Method Analytes in High-Hardness
Water	33

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1 Scope and Application

Method 561 is a liquid chromatography-tandem mass spectrometry (LC-MS/MS) method for the
determination of endothall, glyphosate, glufosinate, and aminomethylphosphonic acid in drinking water
using direct aqueous injection. This method gives instructions for a single bimodal LC column. At the
time of publication, the authors could not identify other columns capable of separating the method
analytes with acceptable efficiency and resolving these analytes from matrix interferences. A procedure
is provided in this method for demonstrating acceptable performance for alternate columns as they
become available.

Method 561 requires the use of MS/MS in Multiple Reaction Monitoring (MRM) mode to enhance
selectivity. Accuracy and precision data have been generated in reagent water, high-hardness synthetic
matrix, and drinking water for the compounds included in the analyte List. Method performance data
were generated with an injection volume of 2 piL to minimize matrix effects. This method is intended for
use by analysts skilled in the operation of LC-MS/MS instrumentation and the interpretation of the
associated data.

Analyte List

Analyte

Abbreviation

CASRN

Aminomethylphosphonic acid

AM PA

1066-51-9

Endothall

END

145-73-3

Glufosinate

GLU

51276-47-2

Glyphosate

GLY

1071-83-6

1.1	Lowest Concentration Minimum Reporting Limits

The lowest concentration minimum reporting level (LCMRL) is the lowest concentration for which the
future recovery is predicted to fall between 50 and 150% with high confidence (99%). Single-laboratory
LCMRLs determined for the method analytes during method development are reported in Table 7. The
procedure used to determine the LCMRL is described elsewhere.- Laboratories using this method are
not required to determine LCMRLs, but they must demonstrate that they are able to meet the minimum
reporting level (MRL) (Sect. 3.11) for each analyte per the procedure described in Section 9.1.4.

1.2	Method Flexibility

1.2.1 General Flexibility Requirements

At a minimum, one isotopically labeled analogue must be used as an internal standard for each analyte.
Changes may not be made to sample preservation and the quality control (QC) requirements.
Automated sample preparation techniques were not investigated during method development.
However, the laboratory may use automated sample preparation provided all quality control
requirements are met.

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1.2.2 Chromatographic Flexibility Requirements

The authors identified only one column capable of separating the method analytes and resolving them
from the preservatives (sodium omadine and ethylenediaminetetraacetic acid - EDTA) and common
anions in drinking water (chloride, nitrate, and sulfate). If the laboratory selects an LC column or LC
conditions different from those used to develop the method, the laboratory must demonstrate that the
preservatives and common anions elute within the analytical run, preventing them from building up on
the column. The procedure to identify retention times for the preservatives and matrix components is
provided in Section 9.3 to assist the user in meeting this requirement. The analyst must then perform
the procedures outlined in the Initial Demonstration of Capability (IDC, Sect. 9.1), verify that all QC
acceptance criteria in this method (Sect. 9.2) are met, and verify method performance in synthetic
matrix and a representative sample matrix (Sect. 9.3.3).

2	Method Summary

Drinking water samples are collected in 120 mL bottles containing sodium carbonate and the
preservative, sodium omadine. Sodium omadine reduces residual chlorine and, in excess, serves as a
biocide to prevent microbial growth during sample storage. Sodium carbonate raises sample pH to
approximately 11. Calcium precipitates at this pH as insoluble calcium carbonate. This step prevents
interference from the calcium-trisodium ethylenediaminetetraacetic acid (EDTA) complex that elutes
near the endothall-d6 internal standard. Prior to analysis, the samples are filtered to remove
precipitated calcium carbonate. EDTA is added to the filtered aliquot to prevent chelation of the method
analytes with metals, including alkaline earth metals. Finally, isotopically labeled analogues of the
method analytes are added to the samples as internal standards. An aliquot of the filtered sample is
injected onto the bimodal LC column, with anion exchange properties, specified in Section 6.9 that
separates the method analytes from the following common anions (matrix components) in drinking
water: chloride, sulfate, and nitrate, and the method preservatives: EDTA, EDTA complexed with Ca,
EDTA complexed with Mg, and sodium omadine, the latter eluted as the deprotonated pyrithione anion.
Prior to each sample injection, the column is conditioned with a 5 piL injection of 5 mmol EDTA in
aqueous buffer and then recycled to starting mobile phase conditions. This technique prevents band
broadening and fronting of the glyphosate peak caused by metals in the HPLC flow path. The matrix
components and preservatives in the column eluate are diverted to waste; the analytes of interest are
directed into the ESI-MS/MS system. The method analytes are qualitatively identified via retention time
and a unique mass transition. The concentration of each analyte is calculated using the integrated peak
area and the internal standard technique.

3	Definitions

3.1	Analysis Batch

A set of samples that are analyzed on the same instrument during a 24-hour period that begins and ends
with the analysis of the appropriate Continuing Calibration Check (CCC) standards. Additional CCCs may
be required depending on the length of the Analysis Batch and the number of field samples.

3.2	Continuing Calibration Check (CCC)

A calibration standard that is analyzed periodically to verify the accuracy of the existing calibration.

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3.3	Field Duplicates (FD)

Separate samples collected at the same time and sampling location, shipped, and stored under identical
conditions. Method precision, including the contribution from sample collection procedures, is
estimated from the analysis of Field Duplicates. Field Duplicates are used to prepare Laboratory Fortified
Sample Matrix and Laboratory Fortified Sample Matrix Duplicate QC samples.

3.4	Internal Standards

Isotopically labeled analogues of the method analytes that are added to the sample at a consistent
concentration prior to LC-MS/MS analysis.

3.5	Internal Standard Quantitation Technique

An analytical technique for measuring analyte concentration using the ratio of the peak area of the
native analyte to that of an isotopically labeled analogue added to the original sample in a known
amount.

3.6	Laboratory Fortified Blank (LFB)

A volume of reagent water, containing method preservatives, to which known quantities of the method
analytes are added. The LFB is used during the IDC (Sect. 9.1) to verify method performance for
precision and accuracy.

3.7	Laboratory Fortified Sample Matrix (LFSM)

An aliquot of a field sample to which known quantities of the method analytes are added. The purpose
of the LSFM is to determine whether the sample matrix contributes bias to the analytical results.

3.8	Laboratory Fortified Sample Matrix Duplicate (LFSMD)

A Field Duplicate of the sample used to prepare the LFSM that is fortified and analyzed identically to the
LFSM. The LFSMD is used instead of the Field Duplicate to assess method precision when the method
analytes are rarely found at concentrations greater than the Minimum Reporting Levels.

3.9	Laboratory Reagent Blank (LRB)

An aliquot of reagent water, including preservatives fortified with the internal standards and processed
identically to a field sample. An LRB is included in each Analysis Batch to determine if the method
analytes or other interferences are introduced from the laboratory environment, the reagents, or
glassware.

3.10	Lowest Concentration Minimum Reporting Level (LCMRL)

The single-laboratory LCMRL is the lowest spiking concentration such that the probability of spike
recovery in the 50% to 150% range is at least 99%.-

3.11	Minimum Reporting Level (MRL)

The minimum concentration that may be reported by a laboratory as a quantified value for a method
analyte. For each method analyte, the concentration of the lowest calibration standard must be at, or
below, the MRL and the laboratory must demonstrate its ability to meet the MRL per the criteria defined
in Section 9.1.4.

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3.12	Precursor Ion

The gas-phase species corresponding to the method analyte that is produced in the electrospray
ionization interface. During tandem mass spectrometry, or MS/MS, the precursor ion is mass selected
and fragmented by collision-activated dissociation to produce distinctive product ions of smaller mass to
charge (m/z) ratio. For this method, the precursor ion is usually the deprotonated molecule ([M - H]~) of
the method analyte.

3.13	Primary Dilution Standard (PDS)

A solution that contains method analytes (or internal standards) prepared from stock standards. PDS
solutions are used to fortify QC samples and diluted to prepare calibration standards.

3.14	Procedural Calibration Standard

A solution of the method analytes, internal standards, and method preservatives prepared in reagent
water. The procedural calibration standards are used to calibrate the instrument response with respect
to analyte concentration.

3.15	Product Ion

One of the fragment ions that is produced in MS/MS by collision-activated dissociation of the precursor
ion.

3.16	Quality Control Sample (QCS)

A solution containing the method analytes at a known concentration that is obtained from a source
external to the laboratory and different from the source of calibration standards. The purpose of the
QCS is to verify the accuracy of the primary calibration standards.

3.17	Stock Standard Solution

A concentrated standard that is prepared in the laboratory using assayed reference materials or that is
purchased from a commercial source with a Certificate of Analysis.

3.18	Synthetic Sample Matrix

A synthetic matrix representing a solution of high concentrations of common anions (chloride, nitrate,
and sulfate) in drinking water using alkaline earth metal salts (calcium and magnesium) prepared in
reagent water with prescribed concentrations of sample preservatives. Procedural calibration standards,
prepared by fortifying the synthetic sample matrix with the method analytes, are used to verify method
performance when analyzing high ionic content samples with alternate LC columns. Instructions for
preparing the synthetic sample matrix are provided in Section 7.9.

4 Interferences

The information in this section was informed by the authors' experience with the Shodex VT-50 2D
column (Sect. 6.9), used to develop the method and collect method performance data. However, the
potential negative effects of high ionic concentrations of synthetic sample matrix components and
preservatives must be equally evaluated and demonstrated when using alternate column technologies.

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4.1	Labware, Reagents and Equipment

Method interferences may be caused by contaminants in solvents, reagents, including reagent water,
sample bottles and caps, and other sample processing hardware that may lead to discrete artifacts or
elevated baselines in the chromatograms. Laboratories must demonstrate that these items are not
contributing to interference by analyzing LRBs as described in Section 9.2.1.

4.2	Interference from Matrix Anions

In addition to the method analytes, anion exchange columns, such as the Shodex VT-50 2D, retain
anionic species in drinking water, including the method preservatives which are anionic in the basic
mobile phase. Anionic complexes of EDTA with Ca and Mg are also retained. Figure 1 and Figure 2 are
chromatograms showing the elution order of the method analytes and these matrix anions. High
concentrations of matrix anions could cause instrument response suppression, band broadening, and
low recovery. However, for the bimodal Shodex column, none of these effects were observed at the
synthetic matrix concentrations listed in this section in the presence of the method preservatives
(sodium omadine, sodium carbonate, and EDTA) and an injection volume of 2 piL.

The authors verified method performance for matrix anions using synthetic matrix containing the three
most common anions in drinking water: chloride at 390 mg/L, nitrate at 44 mg/L, and sulfate at 250
mg/L. These concentrations represent, or exceed, the EPA Primary Drinking Water Standard maximum
contaminant level (MCL) for nitrate and the Secondary Drinking Water Standard MCLs for chloride and
sulfate.

To represent the worst case for high-hardness water, the authors consulted drinking water surveys for
water hardness in North American drinking water (e.g., Morr 2006- and Azoulay 2001-) and hardness
measurements made on local drinking water from aquifer sources. Morr reported up to 350 mg/L
hardness as calcium carbonate. The authors measured between 330 mg/L and 350 mg/L in a local
drinking water prepared from a groundwater source. With a formula weight of 100 mg/mmol for
calcium carbonate, 350 mg/L equals 3.52 mmol, corresponding to 141 mg/L of Ca (atomic weight = 40
mg/mmol), assuming the hardness is entirely due to Ca and no Mg is present. The Azoulay survey found
up to 48 mg/L (2.0 mmol) as Mg, atomic weight 24.3 mg/mmol. Therefore, synthetic matrix used to
verify method performance contained 141 mg/L Ca and 48 mg/L Mg. The combined hardness of this
synthetic matrix is 547 mg/L based on calcium carbonate equivalents.

4.3	Interference from Metals in the HPLC System and Samples
4.3.1 Analyte Complexes with Metals

Glyphosate is known to form complexes with metals in aqueous solution, including alkaline earth
metals, Ca and Mg-. As stated in EPA Method 548.1-, endothall complexes with Ca and Mg in drinking
water and source waters. To prevent formation of these undesired complexes, EDTA, as trisodium
ethylenediaminetetraacetic acid hydrate, is added to the samples after filtration in the laboratory at a
concentration of 2.5 mmol, the molar equivalent to 250 mg/L water hardness expressed as calcium
carbonate. 2.5 mmol EDTA is sufficient to complex the highest levels of Mg expected in drinking water
(2.0 mmol, 48 mg/L) and any Ca not removed during the precipitation step of the sample preparation
procedure.

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4.3.2	Chromatographic Interference from Ca-EDTA Complex

For the Shodex VT-50 2D column, the calcium-EDTA complex elutes near endothall and glyphosate
under the chromatographic conditions of this method and produces an MRM transition identical to that
used for the endothall-d6 internal standard. Although baseline separated, very high levels of Ca result in
a broad calcium EDTA peak that interferes with the endothall internal standard peak. Because there is
no alternate transition for endothall-d6, calcium must be removed during sample preparation by adding
sodium carbonate to field samples and subsequent filtration in the laboratory.

4.3.3	Magnesium-EDTA Complex

Calcium is effectively removed as insoluble calcium carbonate during the sample filtration step;
however, magnesium hydroxide forms a colloidal solution that is not removed during the filtration step.
At 48 mg/L (2.0 mmol) as Mg and a 2 piL injection volume, the authors observed no suppression of
analyte response when using the Shodex VT-50 2D column.

4.3.4	Effect of Metals on Glyphosate Peak Shape

The authors observed deterioration of glyphosate peak shape, revealed as bad broadening and fronting,
for new and aged Shodex VT-50 2D columns. Glyphosate may be sensitive to metals in the HPLC flow
path. The authors demonstrated that an EDTA pre-injection eliminates this degradation in column
efficiency. This method requires an injection of EDTA prior to each sample injection.

4.4 Organic Matrix Interferences

Matrix interferences may be caused by natural organic contaminants that are co-injected from the
sample. The extent of organic matrix interferences was assessed using drinking water from a surface
water source fortified with the method analytes. With an injection size of 2 piL, acceptable recoveries
were observed in the presence of total organic carbon (TOC) greater than 2 mg/L C.

5	Safety

Each chemical should be treated as a potential health hazard and exposure to these chemicals should be
minimized. Each laboratory is responsible for maintaining an awareness of OSHA regulations regarding
safe handling of chemicals used in this method. A reference file of safety data sheets should be made
available to all personnel involved in the chemical analysis.

6	Equipment and Supplies

References to specific brands and catalog numbers are included as examples only and do not imply
endorsement of the products. Such reference does not preclude the use of equivalent products from
other vendors or suppliers.

6.1	Sample Containers

120 mL (4 oz.) amber glass bottles with Teflon-lined septa.

6.2	Autosampler Vials
Glass with Teflon-lined closures.

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6.3	Sample Vials

Glass with Teflon-lined septa, 15 mL size recommended.

6.4	Micro Syringes

Liquid or gas tight syringes sized to transfer stock standards that cannot be measured using micro
pipettes with polypropylene tips.

6.5	Pipets

Automatic or manual micro pipettes with polypropylene tips may be used to prepare calibration
standards, add internal standards, and fortify samples to prepare quality control samples.

Capable of weighing to the nearest 0.0001 g.

6.6	pH Meter

Used to adjust the pH of the aqueous ammonium bicarbonate mobile phase.

6.7	Syringes and Filters

To filter field and QC samples, procedural calibration standards, and laboratory reagent blanks.

6.7.1	Plastic Syringes

Polypropylene syringes with rubber-tipped plungers, 10 mL size recommended.

6.7.2	Syringe Filters, 0.45 [am glass fiber

GE Whatman 25 mm glass fiber, 0.45 micrometer pore size, Cat. No. 6894-2504, or equivalent.

6.8	LC-MS/MS System

6.8.1	LC System

The LC system must provide consistent sample injection volumes and be capable of performing binary
linear gradients at a constant flow rate. To improve the inertness of the sample path, the authors
replaced the metal mobile phase delivery tubing from the autosampler to the guard column with 0.0050
inch i.d. polyetheretherketone (PEEK) tubing.

6.8.2	Bimodal Guard Column

Shodex (Resonac America, Inc., New York, NY) HILICpak VT-50G 2A, 10 x 2.0 mm i.d., 5 micrometer
particle size, PEEK housing, polyvinyl alcohol substrate with quaternary ammonium group.

6.8.3	Guard Column Coupler

PEEK tubing: 0.010 inch i.d. used during method development.

6.8.4	Bimodal Analytical Column

Shodex (Resonac America, Inc., New York, NY) HILICpak VT-50 2D, 150 x 2.0 mm i.d., 5 micrometer
particle size. PEEK housing, polyvinyl alcohol substrate with quaternary ammonium group. The
maximum recommended column pressure for the bimodal column is 1450 psig. If the operating pressure

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at 40 °C is close to this limit, identify the i.d. of the post-column tubing and replace with tubing of a
greater diameter. The authors replaced the 0.0040 inch i.d. capillary, supplied by the instrument
manufacturer, between the column exit and the post-column divert valve with 0.010 inch i.d. PEEK
tubing to prevent the column from exceeding the 1450 psig pressure limit.

6.8.5	Electrospray Ionization Tandem Mass Spectrometer (ESI-MS/MS)

The mass spectrometer must be capable of electrospray ionization in the negative ion mode. The system
must be capable of performing MS/MS to produce unique product ions for the method analytes within
specified retention time windows. A minimum of 10 scans across the chromatographic peak is needed to
ensure adequate precision. The LC-MS/MS must have the capability to program multiple divert windows
to direct the column eluate to waste when the analytes are not eluting.

6.8.6	MS/MS Data System

An interfaced data system is required to acquire, store, and output MS data. The computer software
must have the capability of processing stored data by recognizing a chromatographic peak within a given
retention time window. The software must allow integration of the abundance of any specific ion
between specified time or scan number limits. The software must be able to construct a linear
regression or quadratic regression calibration curve and calculate analyte concentrations using the
internal standard technique.

7 Reagents and Standards

HPLC or LC-MS-grade reagents must be used, if available. Otherwise, all reagents must conform to the
specifications of the Committee on Analytical Reagents of the American Chemical Society (ACS), where
such specifications are available. Other grades may be used if the reagent is demonstrated to be free of
analytes and interferences and all requirements of the IDC are met when using these reagents. The
concentrations of analyte stocks, internal standard stocks, PDS solutions, and calibration standards
listed in this section were used to develop this method and are included only as examples.

Preparation instructions for mobile phases assume the use of the Shodex VT-50 2D column and a binary
HPLC pumping system. Quaternary LC pumps may be used. Laboratories are responsible for developing
appropriate mobile phase systems for alternate column technologies.

7.1	Reagent Water

Purified water which does not contain any measurable quantities of any method analytes or interfering
compounds greater than one-third of the MRL for each method analyte.

7.2	Acetonitrile

H3CN, CASRN 75-05-8, HPLC or LC-MS grade.

7.3	1% Acetonitrile Solution

For use diluting stock standards to prepare PDS (spiking) solutions and to reconstitute internal standards
if purchased as the neat materials. Combine 10 mL of pure acetonitrile with 990 mL of reagent water.

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7.4	Ammonium Bicarbonate

NH4HCO3, CASRN 1066-33-7, HPLC grade, molecular weight equals 79.056 g/mol.

7.5	Ammonium Hydroxide

NH4OH, CASRN 1336-21-6, approximately 56.6% in water as ammonium hydroxide (w/w), approximately
28% in water as ammonia, approximately 14.5 N (Fisher Scientific, Cat. No. A669, Certified ACS Plus
grade, or equivalent).

7.6	Mobile Phase Preparation

7.6.1	50 mmol Ammonium Bicarbonate, pH 9.2 (Mobile Phase A)

To prepare 1 L, add 3.95 g ammonium bicarbonate to 1 L of reagent water. Adjust pH to 9.2 with
ammonium hydroxide. This mobile phase must be replaced every 2 weeks. Analyte and matrix
component retention times increase as the buffer ages.

7.6.2	55% Acetonitrile (Mobile Phase B)

To prepare 0.50 L, separately measure 275 mL of acetonitrile and 225 mL reagent water. Combine in a
mobile phase bottle. This mobile phase may be used until exhausted.

7.7	Preservatives

7.7.1	Sodium Omadine-

C5H4NNaOS, CASRN 3811-73-2. Sodium omadine is added to sample bottles to reduce residual chlorine
and acts as a microbial growth inhibitor in drinking water samples. Reference number six provides
information on the properties of sodium omadine.

7.7.2	Sodium Carbonate, Anhydrous Powder

Na2C03, CASRN 497-19-8. Sodium carbonate is added to sample bottles to raise sample pH to
approximately 11.

7.8	Ethylenediaminetetraacetic acid trisodium salt hydrate

CASRN 85715-60-2, molecular weight equals 376.2 mg/mmol. Ethylenediaminetetraacetic acid (EDTA)
complexes with metals, including alkaline earth metals, that could otherwise complex with endothall,
glyphosate, AMPA, and glufosinate. EDTA is added to samples in the laboratory after filtration. EDTA is
also used to prepare the pre-injection solution (Section 7.8.2).

7.8.1	EDTA Preservative, 45 mg/mL

Dissolve 4,500 mg ethylenediaminetetraacetic acid trisodium salt hydrate in 100 mL reagent water.

7.8.2	EDTA Pre-injection Solution, 5.0 mmol

Dissolve 188 mg of ethylenediaminetetraacetic acid trisodium salt hydrate in 100 mL of 50 mmol
ammonium bicarbonate, pH 9.2 buffer. The pre-injection solution is used to condition the HPLC column
between each run. This treatment narrows the width and prevents fronting of the glyphosate peak.

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7.9 Synthetic Sample Matrix Preparation

Procedural calibration standards prepared in synthetic matrix are used to confirm acceptable analyte
recovery for alternate LC columns in the presence of common matrix ions in drinking water. Section 4.2
provides an explanation for the selection of the concentrations prescribed for the synthetic matrix.
Obtain common forms of the following salts at 99% purity, or greater: sodium nitrate, calcium chloride,
ammonium sulfate, and magnesium chloride. Table 1 gives the required concentration of each species in
the synthetic matrix solution and other information helpful for preparing this solution.

Table 1. Preparation of Synthetic Matrix Solution

COMPOUND

Mass of Salt Used

Concentration

(Formula Weight, mg/mmole)





I\I03" (62) from NaN03 (85)

60.7 mg NaN03

44 mg/L

CI" (35.45) from CaCI2 • 2H20 (147)

518 mg CaCI2-2H20

250 mg/L

CI" (35.45) from MgCI2 (95.21)

188 mg MgCI2

140 mg/L

Total Cl"



390 mg/L

Ca2+ (40) from CaCI2-2H20 (147)

From same addition above

141 mg/L (3.5 mmol)

Mg2+ (24.3) MgCI2 (95.21)

From same addition above

48 mg/L (2.0 mmol)

S042" (96) from (NH4)2S04 (132)

344 mg

250 mg/L

7.10	ESI Interface Gases
7.10.1 Nitrogen Nebulizer Gas

Nitrogen, used as a nebulizer gas in the ESI interface and as collision gas in some MS/MS platforms,
should meet or exceed the instrument manufacturer's specifications.

7.11	Argon

Used as collision gas in MS/MS instruments. Argon should meet or exceed instrument manufacturer's
specifications. Nitrogen may be used as the collision gas if recommended by the instrument
manufacturer.

7.12	Analyte Stock Standards

The solution concentrations listed in this section were used to develop this method and are included
only as examples. Obtain certified solutions of the method analytes in water. Typical concentrations are

1000-2000 ng/mL.

7.13	Internal Standards Stocks

During method development the internal standards required for use with this method were acquired as
neat materials. Table 2 lists the labeled analogues selected by the authors. Other labeled analogues may
be substituted, although the analyst must ensure that the QC requirements defined in Section 9.2.7 are
met. If purchased as neat materials, reconstitute with 1% acetonitrile in reagent water with sonication.
The authors took the additional step of rinsing the 1.5 mL ampoule with pH 9.2 ammonium bicarbonate
buffer (Sect. 7.6.1) several times to ensure complete transfer of the solid material into a 60 mL vial; then
brought to 40 mL final volume with 1% acetonitrile.

Table 2. Preparation of Internal Standard Stocks from Neat Materials

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Compound

Vendor

Cat. No.

Mass Used

Volume3

Stock, |o.g/mL

AMPA -d2

CDNb

D-8135

10 mg

40 mL

250

Glufosinate-

CDN

D-7962

10 mg

40 mL

250 as the

ds- HCI









hydrochloride

Endothall-c/6

CDN

D-7289

10 mg

40 mL

250 as the

monohydrate









hydrate

(MW=210)











Glyphosate-c/2

CDN

D-8030

10 mg

40 mL

250

a Reconstituted in water plus 1% acetonitrile with sonication.
b CDN Isotopes, Inc., or equivalent.

7.14	Analyte PDS

The analyte PDS is used to prepare the calibration standards and to fortify LFBs, LFSMs and LFSMDs with
the method analytes. Prepare the analyte PDS by combining and diluting the analyte stock standards in
water with 1% acetonitrile added. Select nominal analyte concentrations for the PDS such that at least
10 piL of the PDS are used to fortify samples and prepare standard solutions. More than one PDS
concentration may be necessary to meet this requirement. If preparing calibration standards and QC
samples in 120 mL bottles (Sect. 7.16), an analyte PDS prepared at 20,000 ng/L for AMPA, glufosinate,
and glyphosate and 10,000 ng/Lfor endothall is appropriate. The user may modify the relative
concentrations of the individual analytes based on the confirmed MRLs and the desired monitoring
range.

7.15	Internal Standard PDS

Prepare the internal standard PDS by combining and diluting the internal standard stocks in water with
1% acetonitrile added. Select nominal analyte concentrations for the PDS such that at least 10 piL of the
PDS are used to fortify samples and prepare standard solutions. During method development, the
internal standard PDS was prepared at a single concentration of 15 ng/mL. For collection of
performance data, an 80 piL aliquot of the internal standard PDS was added to 12 mL of filtered sample
to give a concentration of 100 ng/Lfor each internal standard.

7.16	Procedural Calibration Standards

Prepare a series of calibration standards of at least five levels by diluting the analyte PDS into reagent
water in 120 mL bottles containing the method preservatives: 7.5 mg/sodium omadine (75 mg/L) and
530 mg anhydrous sodium carbonate (0.050 M, 5.3 g/L). The order of addition is as follows: Weigh the
preservatives, sodium carbonate (530 mg) and sodium omadine (7.5 mg) into the sample bottles. Add
100 mL reagent water. Mix until the solids are dissolved. Add an appropriate aliquot of the analyte PDS
(Sect. 7.1.4) to establish each calibration level. Filter, add EDTA, and fortify with internal standards as
instructed in Sections 11.4 through 11.6. The lowest calibration standard must be at, or below, the MRL
for each analyte. The calibration standards may also be used as Continuing Calibration Checks (CCCs).
For the collection of method performance data, the concentration of the internal standards was 100
Hg/L. For AMPA, glufosinate, and glyphosate, the analyte calibration ranged from 10 ng/L to 400 ng/L
and for endothall, 5.0 ng/L to 200 ng/L.

7.17	Storage Temperatures for Standards Solutions

Refrigerate stock standards and PDS solutions unless the vendor recommends otherwise. Do not freeze.
During method development, no change in analyte concentrations was observed over a period of 6 to 12

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months. Warm PDS and stock standards to room temperature prior to use. Calibration standards may be
used for 6 months if evaporation is avoided.

8	Sample Collection, Preservation, and Storage

8.1	Sample Bottle Preparation

8.1.1	Sample Containers

Amber glass bottles with PTFE-lined screw caps, 120 mL (4 oz.) volume recommended. If recycling
bottles, include a rinse with tap water and a few drops of acetic acid to remove scale formed by
precipitation of calcium carbonate. When recycling sample containers, use new septa to avoid
contamination with method analytes during sampling.

8.1.2	Addition Of Preservatives

Prior to shipment to the field, add sodium omadine and anhydrous sodium carbonate to the sample
containers to produce concentrations of 75 mg/L and 5.3 g/L (0.050 M), respectively, in the field
samples. For example, a 100 mL sample requires 7.5 mg of sodium omadine and 530 mg of sodium
carbonate.

8.1.3	Collection Procedure

Open the tap and allow the system to flush until the water temperature has stabilized. Collect samples
from the flowing system. Samples do not need to be collected headspace free. After collecting the
sample, cap the bottle and agitate by hand until the sodium carbonate is dissolved. If using 120 mL
bottles, 4 oz., estimate the 100 mL level and fill approximately to that mark.

8.1.4	QC Samples

Collect enough Field Duplicates to satisfy the requirement of analyzing one Field Duplicate in each
Analysis Batch of 20 samples. Collect enough samples in triplicate to satisfy the requirement of at least
one LFSM and LFSMD in each Analysis Batch of 20 samples.

8.2	Sample Shipment and Storage

Samples must be shipped on ice. Samples are valid if any ice remains in the cooler when it is received at
the laboratory or bottles are received within 2 days of collection and below 10 °C. Once at the
laboratory, samples must be stored at, or below, 6 °C until analysis. Samples must not be frozen.

8.3	Sample Holding Time

Analyze samples as soon as possible. Samples must be in contact with the sodium carbonate used to
precipitate out metals for at least an hour, which includes both field samples and laboratory prepared
QC samples. Samples must be analyzed within 28 days of collection.

9	Quality Control

QC procedures include the IDC and ongoing QC requirements. This section describes each QC
parameter, its required frequency, and the performance criteria that must be met in order to satisfy
method objectives. The QC criteria discussed in the following sections are summarized in Table 15 and

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Table 16. These QC requirements are considered the minimum for an acceptable QC program.
Laboratories are encouraged to institute additional QC practices to meet their specific needs.

9.1 Initial Demonstration of Capability

The IDC must be successfully performed prior to analyzing field samples. The IDC must be repeated if
changes are made to analytical parameters not previously validated during the IDC. This may include, for
example, changing the injection volume, selecting alternate quantitation ions, substituting internal
standards, and extending the calibration range. Prior to conducting the IDC, the analyst must meet the
calibration requirements outlined in Section 10. The same calibration range used during the IDC must be
used for the analysis of field samples.

9.1.1	Demonstration of Low System Background

Prepare an LRB following the steps in Section 11.2. Filter, add EDTA, and fortify with internal standards
as instructed in Sections 11.4 through 11.6. Analyze the LRB in a valid Analysis Batch immediately after
injecting the highest calibration standard in the selected calibration range. Confirm that the blank is free
from contamination as defined in Section 9.2.1. If the LRB results fail, the carryover or system
contamination must be eliminated. Adjust the rinse settings of the sample introduction system or
reduce the concentration of the highest standard in the calibration range. Perform an initial calibration
and repeat the demonstration of low system background.

9.1.2	Demonstration of Precision

9.1.2.1	Prepare Seven Laboratory Fortified Blanks (LFBs)

Collect 100 mL of reagent water in 120 mL bottles containing the method preservatives, sodium
carbonate and sodium omadine (Sect. 8.1.2). Fortify near the midpoint of the initial calibration curve
with an appropriate volume of Analyte PDS (Sect. 7.14). Filter, add EDTA, and fortify with internal
standards as instructed in Sections 11.4 through 11.6.

9.1.2.2	Evaluate Precision

Analyze seven replicate LFBs in a valid Analysis Batch (seven LFBs and an LRB). The percent relative
standard deviation (%RSD) of the concentrations of the replicate analyses must be less than 20% for all
method analytes.

9.1.3	Demonstration of Accuracy

Using the same set of replicate data generated for Section 9.1.2, calculate the average percent recovery.
The average recovery for each analyte must be within a range of 70-130%.

9.1.4	Minimum Reporting Level (MRL) Confirmation

Establish a target concentration for the MRL (Sect. 3.12) based on the intended use of the method. If
there is a programmatic MRL requirement, the laboratory MRL must be set at, or below, this level.
Establishing the MRL concentration too low may cause repeated failure of ongoing QC requirements.

Perform an initial calibration following the procedures in Section 10.3. The lowest calibration standard
used to establish the initial calibration (as well as the low-level CCC) must be at, or below, the MRL.
Confirm the laboratory's ability to meet the MRL following the procedure outlined below.

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9.1.4.1	Prepare and Analyze MRL Samples

Prepare seven LFBs at, or below, the proposed MRL concentration. Collect 100 mL of reagent water in
120 mL bottles containing the method preservatives, sodium carbonate and sodium omadine (Sect.
8.1.2). Fortify with an appropriate volume of Analyte PDS (Sect. 7.14). Filter, add EDTA, and fortify with
internal standards as instructed in Sections 11.4 through 11.6. Analyze the LFBs in a valid Analysis Batch.

9.1.4.2	Calculate MRL Statistics

Calculate the mean and standard deviation for each analyte in these replicates. Determine the Half
Range for the Prediction Interval of Results (HRpir) using the following equation:

HRpir = 3.963S

Where,

5 = the standard deviation and 3.963 is a constant value for seven replicates.-

Calculate the Upper and Lower Limits for the Prediction Interval of Results (PIR = Mean ± HRpir) as shown
below. These equations are only defined for seven replicate samples.

Mean + HRp,r

Upper PIR Limit =		—-	 x 100

Fortified Concentration

Mean — HRpir

Lower PIR Limit = —		——	 x 100

Fortified. Concentration

9.1.4.3	MRL Acceptance Criteria

The laboratory's ability to meet the MRL is confirmed if the Upper PIR Limit is less than, or equal to,
150%; and the Lower PIR Limit is greater than, or equal to, 50%. If these criteria are not met, the MRL
has been set too low and must be confirmed again at a higher concentration.

9.1.5 Calibration Verification

Analyze a QCS (Sect. 9.2.10) to confirm the accuracy of the primary calibration standards.

9.2 Ongoing QC Requirements

This section describes the ongoing QC elements that must be included when processing and analyzing
field samples.

9.2.1 Laboratory Reagent Blank (LRB)

A new LRB must be prepared for each Analysis Batch. Each lot of syringes and filters must be checked for
interferences. If a new lot is required to complete an Analysis Batch, an additional LRB must be prepared
utilizing the new lot. Background concentrations of method analytes must be less than one-third the
MRL. If method analytes are detected in the LRB at concentrations greater than or equal to this level,
then all positive field sample results (i.e., results at, or above, the MRL) for those analytes are invalid for
all samples in the Analysis Batch. Subtracting blank values from sample results is not permitted.

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9.2.2	Estimating Background Concentrations

Although quantitative data below the MRL may not be accurate enough for data reporting, such data
are useful in determining the magnitude of background interference. Therefore, the analyte
concentrations in the LRB may be estimated by extrapolation when results are below the MRL.

9.2.3	Evaluation of Background when Analytes Exceed the Calibration Range

After analysis of a sample in which method analytes exceed the calibration range, one or more LRBs
must be analyzed (to detect potential carryover) until the system meets the LRB acceptance criteria. If
this occurs during an automated sequence, examine the results of samples analyzed following the
sample that exceeded the calibration range. If the analytes that exceeded the calibration range in the
previous sample are detected at, or above, the MRL, these samples are invalid. If the affected analytes
do not exceed the MRL, these subsequent samples may be reported.

9.2.4	Continuing Calibration Check (CCC)

Analyze CCC standards at the beginning of each Analysis Batch, after every tenth field sample, and at the
end of the Analysis Batch. See Section 10.4 for concentration requirements and acceptance criteria for
CCCs.

9.2.5	Laboratory Fortified Blank

Because this method utilizes procedural calibration standards, which are fortified reagent waters, there
is no difference between the LFB and the Continuing Calibration Check standard. Consequently, the
analysis of a separate LFB is not required as part of the ongoing QC; however, the term "LFB" is used for
clarity in the IDC.

9.2.6	Internal Standard Areas

The analyst must monitor the peak areas of the internal standards in all injections of the Analysis Batch.
The internal standard responses (as indicated by peak area) in any chromatographic run must be within
50-150% of the average area measured during the initial calibration. If an internal standard area for a
sample does not meet these criteria, analyze the original filtered sample in a subsequent Analysis Batch.
Alternately, a fresh aliquot of the original field sample may be filtered and fortified with internal
standards and EDTA for the repeat analysis.

9.2.7	Laboratory Fortified Sample Matrix (LFSM)

Within each Analysis Batch, analyze a minimum of one LFSM. The native concentrations of the analytes
in the sample matrix must be determined in a separate field sample and subtracted from the measured
values in the LFSM. If various sample matrices are analyzed regularly, for example, drinking water
processed from ground water and surface water sources, collect performance data for each source.

9.2.7.1 Prepare the LFSM

Prepare the LFSM by fortifying a Field Duplicate with an appropriate amount of the analyte PDS (Sect.
7.14). Filter, add EDTA, and fortify with internal standards as instructed in Sections 11.4 through 11.6.
Generally, select a spiking concentration that is greater than, or equal to, the native concentration for
the analytes. Selecting a duplicate aliquot of a sample that has already been analyzed aids in the
selection of an appropriate spiking level. If this is not possible, use historical data when selecting a
fortifying concentration.

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9.2.7.2	Calculate the Percent Recovery
Calculate the percent recovery (%R) using the equation:

04-5)

o/0 R =	x 100

Where,

A = measured concentration in the fortified sample,

B = measured concentration in the unfortified sample, and
C = fortification concentration.

To obtain meaningful percent recovery results, correct the measured values in the LFSM and LFSMD for
the native levels in the unfortified samples, even if the native values are less than the MRL.

9.2.7.3	Evaluate Analyte Recovery in the LFSM

Results for analytes fortified at concentrations near or at the MRL (within a factor of two times the MRL
concentration) must be within 50-150% of the true value. Results for analytes fortified at all other
concentrations must be within 70-130% of the true value. If the accuracy for any analyte falls outside
the designated range, and the performance for that analyte in the CCCs of the Analysis Batch is shown to
be in control, the recovery is judged matrix biased. Report the result for the corresponding analyte in
the unfortified sample as "suspect-matrix".

9.2.8 Laboratory Fortified Sample Matrix Duplicate (LFSMD) or Field Duplicate (FD)

Within each Analysis Batch, analyze a minimum of one Field Duplicate or one Laboratory Fortified
Sample Matrix Duplicate. If the method analytes are not routinely observed in field samples, analyze an
LFSMD rather than an FD.

9.2.8.1	Calculate the RPD for the LFSM and LFSMD

If an LFSMD is analyzed instead of a Field Duplicate, calculate the RPD using the equation:

| LFSMD - LFSM \

RPD ~ (LFSMD + LFSM)/2 * 10°

9.2.8.2	Acceptance Criterion for the RPD of the LFSM and LFSMD

RPDs for duplicate LFSMs must be less than, or equal to, 30% for each analyte. Greater variability may
be observed when the matrix is fortified at analyte concentrations near or at the MRL (within a factor of
two times the MRL concentration). LFSMs at these concentrations must have RPDs that are less than, or
equal to, 50%. If the RPD of an analyte falls outside the designated range, the precision is judged matrix
influenced. Report the result for the corresponding analyte in the unfortified sample as "suspect-
matrix".

9.2.8.3	Calculate the RPD for Field Duplicates

Calculate the relative percent difference (RPD) for duplicate measurements (FD1 and FD2) using the
equation:

|FDi — FD21
RPD = ' ^ ' x 100
(FDi + FD2)/2

9.2.8.4	Acceptance Criterion for Field Duplicates

RPDs for Field Duplicates must be less than, or equal to, 30% for each analyte. Greater variability may be
observed when Field Duplicates have analyte concentrations that are near or at the MRL (within a factor

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of two times the MRL concentration). At these concentrations, Field Duplicates must have RPDs that are
less than, or equal to, 50%. If the RPD of an analyte falls outside the designated range, the precision is
judged matrix influenced. Report the result for the corresponding analyte in the unfortified sample as
"suspect-matrix"

9.2.9 Calibration Verification using QCS

A QCS (as defined in Sect. 3.17) must be analyzed during the IDC, and then every 3 to 6 months
thereafter. Collect 100 mL of reagent water in a 120 mL bottle containing the method preservatives,
sodium carbonate and sodium omadine (Sect. 8.1.2). Fortify near the midpoint of the calibration range
with an appropriate volume of the QCS stock standards. Filter, add EDTA, and fortify with internal
standards as instructed in Sections 11.4 through 11.6. The acceptance criterion for the QCS is 80-120%
of the true value. If the accuracy for any analyte fails the recovery criterion, prepare fresh standard
dilutions and repeat the QCS evaluation.

9.3 Alternate Column QC Requirements

The analyst is not permitted to modify the chromatographic conditions for the column specified in this
method. These conditions were optimized during method development for the Shodex VT-50 2D column
to ensure that matrix ions and method preservatives elute from the analytical column each run—and
these components are separated from the method analytes. If an alternate column is chosen, the
laboratory must demonstrate that the alternate column is capable of similar performance. The following
steps are required to confirm acceptable performance for alternate columns.

9.3.1	Determine RTs of Analytes and Matrix Components

Prepare calibration standards in both reagent water and in synthetic matrix (Sect. 7.9). Optimize
separation of the method analytes by analyzing calibration standards. Using calibration standards
prepared in synthetic matrix, determine the retention times of m/z 35 and 37 CI"; m/z 62 N03~; m/z 97
and 99 S042~; m/z 291 uncomplexed EDTA; m/z 329 EDTA complexed with Ca; m/z 313 EDTA complexed
with Mg and omadine (detected as the pyrithione anion, m/z 126). Adjust the gradient as necessary to
ensure that the matrix components listed above are separated as much as possible from the method
analytes. Complete separation may not be possible; however, the column may not be used if the co-
elution of matrix components causes QC failures during the IDC (Sect. 9.3.2).

9.3.2	Repeat the IDC

Establish an acceptable initial calibration (Sect. 10.3) using the alternate column and the modified
conditions. Repeat the procedures of the IDC (Sect. 9.1).

9.3.3	Document Performance in Synthetic Matrix and Representative Sample Matrices
The analyst is required to evaluate and demonstrate precision (Sect. 9.1.2) and accuracy (Sect. 9.1.3) for
the alternate column in synthetic matrix (Sect. 7.9) and real matrices that span the range of waters that
the laboratory analyzes. This additional step is required because modifications that perform acceptably
in the IDC, which is conducted in reagent water, could fail ongoing method QC requirements in real
matrices. This is particularly important for methods subject to matrix effects, such as LC-MS/MS-based
methods and for ion chromatography columns that retain ionic matrix components. For a laboratory
that routinely analyzes finished drinking water from municipal treatment plants that process ground
water, surface water, or a blend of surface and ground water, finished drinking waters derived from a

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surface water with moderate to high total organic carbon (e.g., 2 mg/L or greater) and from a hard
ground water (e.g., 250 mg/L calcium carbonate equivalent, or greater) are recommended.

10 Calibration and Standardization

Demonstration and documentation of acceptable MS calibration and initial analyte calibration are
required before performing the IDC and prior to analyzing field samples. The initial calibration should be
repeated each time a major instrument modification or maintenance is performed.

10.1	MS/MS Optimization

10.1.1	Mass Calibration

Calibrate the mass spectrometer with the calibration compounds and procedures specified by the
manufacturer.

10.1.2	MS Parameters

During the development of this method, instrumental parameters were optimized for the precursor and
product ions listed in Table 6. Product ions other than those listed may be selected; however, the
analyst should avoid using ions with lower mass or common ions that may not provide sufficient
discrimination between the analytes of interest and co-eluting interferences.

10.1.2.1	Precursor Ion

Optimize the response of the precursor ion ([M - H]~) for each analyte following manufacturer's
guidance. Analyte concentrations of 5 ng/mL introduced to the ESI-MS/MS via split infusion into mobile
phase were used for this step during method development. Vary the MS parameters (source voltages,
source and desolvation temperatures, gas flows, etc.) until optimal analyte responses are determined.
The electrospray parameters used during method development are listed in Table 5 and Table 6. The
analytes may have different optimal parameters, requiring some compromise on the final operating
conditions.

10.1.2.2	Product Ion

Optimize the product ion for each analyte following the manufacturer's guidance. See Table 6 for
MS/MS collision energies used to collect method performance data.

10.2	Chromatographic Conditions, Shodex VT-50 2D Column

Establish LC operating parameters for analyte separation as specified in Table 3. Create a second
gradient method for the EDTA pre-injections as specified in Table 4. The authors optimized these
conditions for the Shodex VT-50 2D column to ensure that common matrix ions and method
preservatives elute from the analytical column each run—and these components are separated as much
as possible from the method analytes. Figure 1 and Figure 2 show the location of the matrix anions and
preservatives relative to the method analytes.

For the Shodex VT-50 SD column, it is recommended that laboratories utilize the entire gradient
specified in Table 3. including the 17 minute hold time at 90% mobile phase A after the analytes elute.
As shown in Figure 2 , the hold time is necessary to elute uncomplexed EDTA, detected as m/z 291 [H4-
EDTA- H]~, introduced onto the column from the sample injection and the EDTA pre-injection. Figure 2

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also gives the location of EDTA complexed with Ca, detected as m/z 329 [H4-EDTA - 3H + Ca]~ and EDTA
complexed with Mg, detected as m/z 313 [H4-EDTA - 3H + Mg]~ relative to the method analytes. If a
laboratory chooses to use different chromatographic conditions see the flexibility requirement
described in Section 1.2.2.

10.2.1	Equilibrate the Column

Begin heating the column to 40 °C. Establish a flow of 0.10 mL/min at 90% A (50 mmol ammonium
bicarbonate, pH 9.2) and 10% solvent B (55 % acetonitrile). When the system pressure stabilizes,
increase the flow rate to 0.20 mL/min.

10.2.2	EDTA Pre-injections

The laboratory must Inject 5 piL of the 5.0 mmol EDTA pre-injection solution (Sect. 7.8.2). Method
development used the LC conditions listed in Table 4. This gradient recycles the column to 10% A in
preparation for sample injections. If a laboratory chooses to use different chromatographic conditions
see the flexibility requirement described in Section 1.2.2. The EDTA pre-injection must be run prior to
each standard, field sample, and QC sample in the sequence.

10.2.3	Establish LC-MS/MS Retention Times, MRM Windows, and Divert Windows
Inject a mid- to high-level calibration standard under the LC conditions specified in Table 3.

10.2.3.1	Retention Times

Determine the retention times of each method analyte. The retention times observed during collection
of the method performance data are listed in Table 6.

10.2.3.2	MRM Windows

During method development, the chromatogram was divided into two windows—also called segments
or functions. AMPA and glufosinate were monitored during the first MRM window; glyphosate and
endothall were monitored in the second MRM window.

10.2.3.3	Matrix Divert Windows

The instructions in this subsection apply to the Shodex VT-50 2D column and any alternate column
technology. Divert column eluent to waste when analytes are not eluting. Enough time should be
allowed for the baseline to stabilize between the valve switch that begins each analyte elution window
and the appearance of the subsequent analyte signal. If the valve switch is too close to the analyte, the
starting point of the analyte peak may be difficult to distinguish from the baseline disruption, especially
for low analyte concentrations. Verify that analyte signals have returned to baseline before the valve
switch that begins the following matrix divert window.

10.3 Initial Calibration

Prepare a set of at least five procedural calibration standards as described in Section 7.16 to generate
linear or quadratic calibration curves. The analyte concentrations in the lowest calibration standard
must be at, or below, the MRL. Field samples must be quantified using a calibration curve that spans the
same concentration range used to collect the IDC data (Sect. 9.1), i.e., analysts are not permitted to use
a restricted calibration range to meet the IDC criteria and then use a larger dynamic range during
analysis of field samples.

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10.3.1 Calibration Acceptance Criteria

Evaluate the initial calibration by calculating the concentration of each analyte as an unknown against its
regression equation. For calibration levels that are less than, or equal to, the MRL, the result for each
analyte should be within 50-150% of the true value. All other calibration points should be within 70-
130% of their true value. If these criteria cannot be met, the analyst could have difficulty meeting
ongoing QC criteria. In this case, corrective action is recommended such as reanalyzing the calibration
standards, restricting the range of calibration, or performing instrument maintenance. If the cause for
failure to meet the criteria is due to contamination or standard degradation, prepare fresh calibration
standards and repeat the initial calibration.

10.4	Continuing Calibration

Analyze a CCC to verify the initial calibration at the beginning of each Analysis Batch, after every tenth
field sample, and at the end of each Analysis Batch. The beginning CCC for each Analysis Batch must be
at, or below, the MRL for each analyte. This CCC verifies instrument sensitivity prior to the analysis of
samples. Alternate subsequent CCCs between the mid and high calibration levels. Verify that the CCC
meets the criteria in the following sections.

10.4.1	Internal Standard Responses in CCCs

The absolute area of the quantitation ion for each internal standard must be within 50-150% of the
average area measured during the initial calibration. If these limits are exceeded, samples analyzed since
the last acceptable CCC are invalid and corrective action is necessary (Sect. 10.5).

10.4.2	Analyte Responses in CCCs

Calculate the concentration of each method analyte in the CCC. Each analyte fortified at a level less
than, or equal to, the MRL must be within 50-150% of the true value. The concentration of the analytes
in CCCs fortified at all other levels must be within 70-130%. If these limits are exceeded, then all data
for the failed analytes must be considered invalid. Any field samples analyzed since the last acceptable
CCC that are still within holding time must be reanalyzed after an acceptable calibration has been
restored.

10.4.2.1 Exception for High Recovery

If the CCC fails because the calculated concentration is greater than 130% (150% for the low-level CCC)
for a method analyte, and field sample extracts show no concentrations above the MRL for that analyte,
non-detects may be reported without re-analysis. Corrective action (Section 10.5) evaluating and
correcting the high bias for the CCCs is required when this high-bias CCC occurs.

10.5	Corrective Action

Failure to meet the CCC QC performance criteria requires corrective action. Following a minor remedial
action, such as servicing the autosampler or flushing the column, check the calibration with a mid-level
CCC and a CCC at the MRL, or recalibrate according to Section 10.3. If internal standard and calibration
failures persist, maintenance may be required, such as servicing the LC-MS/MS system or replacing the
guard column. These latter measures constitute major maintenance, and the analyst must return to the
initial calibration step (Sect. 10.3).

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11 Procedure

The following instructions are based on filtering 12 mL of the original sample volume of 100 mL. Other
filtering volumes may be used.

11.1	Prepare Fortified Matrix Samples

Fortify LFSMs and LFSMDs with an appropriate volume of Analyte PDS (Sect. 7.14). Use separate
duplicate field samples for the LFSM, LFSMD, and an unfortified sample to determine native analyte
concentration. Fortify analytes into the original sample before the filtration step.

11.2	Prepare the LRB

Collect 100 mL of reagent water in a 120 mL bottle containing the method preservatives, sodium
carbonate and sodium omadine (Sect. 8.1.2).

11.3	Field Duplicates

Select a Field Duplicate pair associated with the samples in the Analysis Batch. Subsampling from a
single field sample is not permitted.

11.4	Filter Samples

Shake stored samples and then separately filter exactly 12 mL of the field samples, LRB, field duplicates,
and LFSMs into 15 mL vials. See Section 6.7 for syringe and filter specifications.

11.5	Add EDTA

Add 250 piL of the 45 mg/mL EDTA solution (Sect. 7.8.1) to the 12 mL of filtered sample. The
concentration of trisodium EDTA hydrate is 950 mg/L (2.5 mM).

11.6	Addition of Internal Standards

Add 80 piL of the internal standard PDS (Sect. 7.15) to each sample, then cap and invert to mix. The
concentration of each internal standard is 100 ng/L. The concentration of the internal standards must be
the same in the samples as in the calibration standards.

11.7	Sample Analysis

The EDTA pre-injection must be run prior to each standard, field sample, and QC sample in the sequence
(Sect. 10.2.2).

11.7.1	Establish LC-MS/MS Operating Conditions

Establish MS/MS operating conditions per the procedures in Section 10.1 and chromatographic
conditions per Section 10.2. Establish a valid initial calibration following the procedures in Section 10.3
or confirm that the existing calibration is still valid by analyzing a low-level CCC. If establishing an initial
calibration for the first time, complete the IDC prior to analyzing field samples.

11.7.2	Verify Divert Windows

The analyst must ensure that each analyte and internal standard peak elutes entirely within the assigned
window during each Analysis Batch. Make this observation by viewing the quantitation ion for each
analyte in the CCCs analyzed during an Analysis Batch. If an internal standard or analyte peak drifts out

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of the assigned window into the divert window, then data for that analyte is invalid in all injections
acquired since the last valid CCC. Retention times increase by approximately one minute as the buffer
ages over two weeks. The authors recommend verifying divert windows after analyzing the low CCC to
begin each Analysis Batch and before running the LRB and subsequent samples.

11.7.3 Sample Analysis

Analyze field and QC samples in a properly sequenced Analysis Batch as described in Section 11.8.
11.8 Analysis Batch Sequence

An Analysis Batch is a sequence of samples, analyzed within a 24-hour period, of no more than 20 field
samples and includes all required QC samples (LRB, CCCs, the LFSM and LFSMD (or FD)). The required QC
samples and the EDTA pre-injections are not included in counting the maximum field sample total of 20.
LC-MS/MS conditions for the Analysis Batch must be the same as those used during calibration.

11.8.1	Analyze Initial CCC

After a valid calibration is established, begin every Analysis Batch by analyzing an initial low-level CCC at,
or below, the MRL. This initial CCC must be within 50-150% of the true value for each method analyte
and must pass the internal standard area response criterion (Sect. 10.4.1). The initial CCC confirms that
the calibration is still valid. Failure to meet the QC criteria may indicate that recalibration is required
prior to analyzing samples.

11.8.2	Analyze Field and QC Samples

After the initial CCC, continue the Analysis Batch by analyzing an LRB, followed by the field samples and
QC samples. Analyze a mid- or high-level CCC after every ten field samples and at the end of each
Analysis Batch. Do not count QC samples (LRBs, FDs, LFSMs, LFSMDs) when calculating the required
frequency of CCCs.

11.8.3	Analyze Final CCC

The last injection of the Analysis Batch must be a mid- or high-level CCC. The acquisition start time of the
final CCC must be within 24 hours of the acquisition start time of the low-level CCC at the beginning of
the Analysis Batch. More than one Analysis Batch within a 24-hour period is permitted.

11.8.4	Initial Calibration Frequency

A full calibration curve is not required before starting a new Analysis Batch. A previous calibration can be
confirmed by running an initial, low-level CCC followed by an LRB. If a new calibration curve is analyzed,
an Analysis Batch run immediately thereafter must begin with a low-level CCC and an LRB.

12 Data Analysis and Calculations

12.1 Identify Peaks of Interest

At the conclusion of data acquisition, use the same software settings established during the calibration
procedure to identify peaks of interest in the predetermined retention time windows. Confirm the
identity of each analyte by comparison of its retention time with that of the corresponding analyte peak
in a recent CCC.

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12.2	Calculate Analyte Concentrations

Calculate analyte concentrations using the multipoint calibration. Report only those values that fall
between the MRL and the highest calibration standard.

12.3	Significant Figures

Calculations must use all available digits of precision, but final reported concentrations should be
rounded to an appropriate number of significant figures (one digit of uncertainty), typically two, and not
more than three significant figures.

12.4	Exceeding the Calibration Range

The analyst must not extrapolate beyond the established calibration range. If an analyte result exceeds
the range of the initial calibration curve, the filtered sample may be diluted using reagent water
containing the appropriate amount of internal standard added to match the original level. Re-inject the
diluted sample. Incorporate the dilution factor into final concentration calculations. The resulting data
must be annotated as a dilution, and the reported MRLs must reflect the dilution factor.

13 Method Performance

Method performance data were collected using the Shodex bimodal LC column specified in Section 6.9
and an injection volume of 2 piL.

13.1	Precision, Accuracy, and LCMRL Results

Tables for these data are presented in Section 17. Single-laboratory LCMRLs are presented in Table 7.
Single-laboratory precision and accuracy data are presented for five water matrices: reagent water
(Table 8). high-hardness matrix from a ground water source (Table 9). high-TOC matrix from a surface
water source (Table 10). synthetic sample matrix prepared per the formulation in Section 7.9 (Table 11).
and finished drinking water from a surface water source, containing an orthophosphate anti-corrosive
agent (Table 12).

13.2	Analyte Stability Study in High-Hardness Matrix

Samples from a high-hardness matrix from a ground water source were inoculated with microbial-rich
water from an impacted surface source and fortified with the method analytes. These samples were
stored as required in this method. The percent change from the initial analyzed concentration observed
after 7, 14, 21, 28, and 42 days is presented in Table 13 .

13.3	Analyte Stability Study in High-TOC Matrix

Samples from a high-TOC matrix from a surface water source were inoculated with microbial-rich water
from an impacted surface source and fortified the method analytes. These samples were stored as
required in this method. The percent change from the initial analyzed concentration observed after 14,
and 35 days is presented in Table 14.

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14 Pollution Prevention

For information about pollution prevention applicable to laboratory operations described in this
method, consult: Less is Better, Guide to Minimizing Waste in Laboratories, a publication available from
the American Chemical Society (accessed January 2024) at www.acs.org.

15	Waste Management

Laboratory waste management practices should be consistent with all applicable rules and regulations,
and that laboratories protect the air, water, and land by minimizing and controlling all releases from
fume hoods and bench operations. In addition, compliance is required with any sewage discharge
permits and regulations, particularly the hazardous waste identification rules and land disposal
restrictions.

16	References

1.	US EPA. Technical Basis for the Lowest Concentration Minimum Reporting Level (LCMRL) Calculator;
EPA 815-R-11-001; Office of Water: Cincinnati, OH, December 2010.

2.	Morr, S.; Cuartas, E., M.D.; et al. How Much Calcium is in your Drinking Water? A Survey of Calcium
Concentrations in Bottled and Tap Water and their Significance for Medical Treatment and Drug
Administration. HSS Journal. 2006, 2, 130-135.

3.	Azoulay, A.; Eisenberg, M. J.; et al. Comparison of the Mineral Content of Tap Water and Bottled
Waters. J. Gen. Internal Medicine. 2001, 16, 168-175.

4.	Thelem, K.D.; Jackson E.P; and Penner, D. The Basis for the Hard-Water Antagonism of Glyphosate
Activity. Weed Science. 1995, Volume 43, 541-548.

5.	U.S. EPA. Method 548.1: Determination of Endothall in Drinking Water by Ion-Exchange extraction,
Acidic Methanol Methylation and Gas Chromatography/Mass Spectrometry, Revision 1.0. 1992

6.	Sodium Omadine™ 40%, Product Fact Sheet, https://monsonco.com/wp-
content/uploads/2019/09/Sodium-Omadine-40.-TDS.pdf, accessed January 2023.

7.	US EPA. Statistical Protocol for the Determination of the Single-Laboratory Lowest Concentration
Minimum Reporting Level (LCMRL) and Validation of Laboratory Performance at or Below the
Minimum Reporting Level (MRL); EPA 815-R-05-006; Office of Water: Cincinnati, OH, November
2004.

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17 Tables, Figures and Method Performance Data

Table 3. HPLC Method Conditions for Sample lnjections°'b'c'd

Time, min

percentage of 50 mmol ammonium
bicarbonate, pH 9.2

percentage of 55% acetonitrile

Initial

10

90

0.1

10

90

7.0

50

50

10

50

50

10.01

55

45

15

55

45

18

80

20

18.01

90

10

35

90

10

a Guard Column = Shodex HILICpak VT-50G 2A, 10 x 2.0 mm i.d. 5 pirn dp
b Analytical Column = Shodex HILICpak VT-50 2D, 150 x 2.0 mm i.d. 5 pim dp

c Method performance data were collected under these conditions at an injection volume of 2 piL.
d Column Flow = 0.2 mL/min, Column Temperature = 40 °C

Table 4. HPLC Conditions for EDTA Pre-lnjections and Gradient Recycle°

Time
(min)

percentage of 50 mmol ammonium
bicarbonate, pH 9.2

percentage of 55% acetonitrile

Initial

90

10

3.0

10

90

8.0

10

90

a Method performance data were collected under these conditions using an EDTA injection volume of

5 \il.

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Table 5. ESI Method Conditions

ESI Conditions3



Polarity

Negative ion

Capillary needle voltage

2.5 kV

Cone gas flow

200 L/hour

Cone voltage (all analytes)

20 V

Nitrogen desolvation gas

800 L/hour

Desolvation gas temperature

400 °C

a Method performance data were collected using a Waters (Milford, MA) Xevo TQ Absolute.
Table 6. Analyte RTs, MRMs, and MS/MS Method Conditions

Analyte

Segment

Retention
Time

Precursor Ion (m/z)

Product lonc [m/z)

Collision Energy (V)

AMPA

1

9.13

110

63

12

AM PA-d2

1

9.00

112

63

12

GLU

1

10.67

180

85

18

GLU-c/s

1

10.50

188

89

18

END

2

17.37

185

141

14

END-de

2

17.30

191

147

14

GLY

2

17.47

168

63

16

GLY-d2

2

17.33

170

63

16

a An LC-MS/MS chromatogram of the analytes obtained using these parameters and a Waters

(Milford, MA) Xevo TQ Absolute is shown in Figure 1 and Figure 2.
b Precursor and product ions listed in this table are nominal masses.
c Argon used as collision gas.

Table 7. LCMRL Results

Analyte

LCMRL Fortification Levels (|ag/L)

Calculated LCMRL (ng/L)

AMPA

0.0, 1.0, 2.0, 4.0, 5.0, 6.0, 8.0, 10

1.4

Glufosinate

0.0, 0.50, 1.0, 2.0, 4.0, 5.0, 6.0, 8.0, 10

2.1

Endothall

0.0, 0.50, 1.0, 2.0, 2.5, 3.0, 4.0, 5.0

1.6

Glyphosate

0.0, 0.50, 1.0, 2.0, 4.0, 5.0, 6.0, 8.0, 10

2.2

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Table 8. Precision and Accuracy Data for Reagent Water

Analyte

Low Fortification
(Hg/L)

Mean %Ra
(n=7)

%RSDa

High Fortification
(Hg/L)

Mean %R
(i=5)

%RSD

AM PA

10

81.2

8.1

150

98.9

2.4

Glufosinate

10

98.8

4.2

150

101

1.6

Endothall

5

92.8

2.9

75

102

3.8

Glyphosate

10

81.5

4.2

150

100

3.6

a %R = percent recovery; %RSD = percent re ative standard deviation
Table 9. Precision and Accuracy Data for a Ground Water Matrix°

Analyte

Low Fortification
(Hg/L)

Mean %Rbc
(i=5)

%RSDb

High Fortification
(Hg/L)

Mean %R
(i=5)

%RSD

AM PA

10

86.9

4.8

150

101

1.0

Glufosinate

10

97.2

2.0

150

103

1.9

Endothall

5.0

90.8

6.4

75

101

0.86

Glyphosate

10

89.7

2.6

150

99.1

1.7

a Ground water matrix was sampled after the clarifier and prior to water softener within the drinking
water treatment plant. Hardness = 338 mg/L as CaC03, pH = 8.2 at 20 °C, Free Cl2 = 0.10 mg/L, Total
Cl2 = 0.17 mg/L.

b %R = percent recovery, corrected for native concentration; %RSD = percent relative standard

deviation.
c Corrected for native concentration

Table 10. Precision and Accuracy Data for a Surface Water Matrix°

Analyte

Low Fortification
(Hg/L)

Mean %Rbc
(i=5)

%RSDb

High Fortification
(Hg/L)

Mean %R
(i=5)

%RSD

AM PA

10

85.9

6.0

150

99.6

2.4

Glufosinate

10

101

2.0

150

102

2.8

Endothall

5

92.7

2.6

75

99.7

2.3

Glyphosate

10

92.2

4.1

150

101

1.8

a Surface water matrix was sampled after the clarifier and prior to granular activated carbon within
the drinking water treatment plant and chlorinated in our laboratory. Hardness = 122 mg/L as
CaC03, pH = 8.4 at 20 °C, Free Cl2 = 0.82 mg/L, Total Cl2 = 1.26 mg/L, Total Organic Carbon (TOC) =
2.7 mg/L C.

b %R = percent recovery; %RSD = percent relative standard deviation.
c Corrected for native concentration.

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Table 11. Precision and Accuracy Data for a Synthetic Sample Matrix°

Analyte

Fortification (ng/L)

Mean %Rb'c(n=5)

%RSDb

AM PA

80

103

6.6

Glufosinate

80

107

6.7

Endothall

40

103

4.9

Glyphosate

80

99.9

5.8

a Synthetic matrix was prepared with 141 mg/L Ca2+, 48 mg/L Mg2+, 44 mg/L N03 , 390 mg/L CI , 250
mg/L S042".

b %R = percent recovery; %RSD = percent relative standard deviation.
c Corrected for native concentration.

Table 12. Precision and Accuracy Data for a Finished Surface Water with Orthophosphate Anti-
Corrosive Agent"

Analyte

Fortification (ng/L)

Mean %Rb,c (n=5)

%RSDb

AM PA

40

100

1.7

Glufosinate

40

101

1.6

Endothall

20

101

1.9

Glyphosate

40

104

1.5

a Surface water matrix was sampled after the clarifier and prior to granular activated carbon within
the drinking water treatment plant and chlorinated in our laboratory. Hardness = 117 mg/L as
CaC03, pH = 8.62 at 20 °C, Free Cl2 = 1.22 mg/L, Total Cl2 = 1.38 mg/L, Total Organic Carbon (TOC) =
2.1 mg/LC.

b %R = percent recovery; %RSD = percent relative standard deviation.
c Corrected for native concentration.

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Table 13. Aqueous Sample Holding Time Data for a Ground Water Matrix°'b

Analyte

Fortified
Cone.
(Hg/L)

Day
Zero
Mean
(Hg/L)

Day
Zero
%RSD

Day 7
%Changeb

Day 7
%RSD

Day 14
%Change

Day
14
%RSD

Day 21
%Change

Day
21
%RSD

Day 28
%Change

Day
28
%RSD

Day 42
%Change

Day
42
%RSD

AM PA

150

151

1.0

0.52

2.6

0.58

2.8

0.79

1.6

1.0

1.9

0.87

1.9

Glufosinate

150

155

1.9

-1.6

1.7

-1.2

0.71

-0.89

1.7

-1.2

1.2

-1.4

1.9

Endothall

75

75.7

0.86

-0.10

0.61

1.9

1.3

0.65

0.85

0.76

1.4

1.0

0.52

Glyphosate

150

149

1.7

-1.9

2.1

2.7

0.45

2.6

1.2

3.4

1.4

4.0

0.92

a Ground water matrix was sampled after the clarifier and prior to the water softener within the drinking water treatment plant. Hardness = 338 mg/L as

CaC03, pH = 8.2 at 20 °C, Free Cl2 = 0.10 mg/L, Total Cl2 = 0.17 mg/L, n=5.
b %Change = percent change from Day Zero calculated as follows: (Day X mean concentration - Day Zero mean concentration) / Day Zero mean
concentration * 100%, where X is the analysis day.

Table 14. Aqueous Sample Holding Time Data for a Surface Water Matrixa,b

Analyte

Fortified
Cone. (|ig/L)

Day Zero
Mean
(Hg/L)

Day
Zero
%RSD

Day 14
%Change

Day 14 %RSD

Day 35
%Change

Day 35 %RSD

AM PA

150

149

2.2

-3.1

12

-5.6

13

Glufosinate

150

152

2.5

-4.8

8.3

-6.8

10

Endothall

75

74.8

2.3

0.93

1.4

-1.4

4.1

Glyphosate

150

151

1.6

-4.2

12

-3.4

14

a Surface water matrix was sampled after the clarifier and prior to granular activated carbon within the drinking water treatment plant and chlorinated in

our laboratory. Hardness = 122 mg/L as CaC03, pH = 8.4 at 20 °C, Free Cl2 = 0.82 mg/L, Total Cl2 = 1.26 mg/L, Total Organic Carbon (TOC) = 2.7 mg/L C, n=5.
b %Change = percent change from Day Zero calculated as follows: (Day X mean concentration - Day Zero mean concentration) / Day Zero mean
concentration * 100%, where X is the analysis day.

561-29


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Table 15. Initial Demonstration of Capability (IDC) Quality Control Requirements

Method
Reference

Requirement

Specification and Frequency

Acceptance Criteria

Section 10

Establish LC-MS/MS
conditions, establish
retention times and
divert windows

Prior to conducting the IDC

Each analyte and internal standard peak must elute
entirely within the MRM window (Sect. 11.4.2).

Section 10.3

Initial calibration

Use the internal standard calibration technique to
generate a linear or quadratic calibration curve.
Use at least 5 standard concentrations. Evaluate
the calibration curve as described in Section
10.3.1.

When each calibration standard is calculated as an
unknown using the calibration curve, the lowest
level standard should be within 50-150% of the true
value. All other levels should be within 70-130% of
the true value.

Section 9.1.1

Demonstration of low
system background

Analyze a Laboratory Reagent Blank (LRB) after the
highest standard in the calibration range.

Demonstrate that the method analytes are less than
one-third of the Minimum Reporting Level (MRL).

Section 9.1.2

Demonstration of
precision

Analyze 7 replicate Laboratory Fortified Blanks (LFBs)
near the mid-range concentration.

Percent relative standard deviation must be <20%.

Section 9.1.3

Demonstration of
accuracy

Calculate mean recovery for replicates used in Section
9.1.2.

Mean recovery within 70-130% of the true value.

Section 9.1.4

MRL confirmation

Fortify and analyze 7 replicate LFBs at the proposed
MRL concentration. Confirm that the Upper Prediction
Interval of Results (PIR) and Lower PIR meet the
recovery criteria.

Upper PIR <150%
Lower PIR >50%

Section 9.1.5

Calibration Verification

Analyze mid-level QCS.

Results must be within 80-120% of the true value.

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Table 16. Ongoing Quality Control Requirements

Method
Reference

Requirement

Specification and Frequency

Acceptance Criteria

Section 10.3

Initial calibration

Use the internal standard calibration technique to
generate a linear or quadratic calibration curve. Use
at least 5 standard concentrations. Evaluate the
calibration curve as described in Section 10.3.1.

When each calibration standard is calculated as an
unknown using the calibration curve, the lowest level
standard should be within 50-150% of the true value.
All other levels should be within 70-130% of the true
value.

Section 10.4

Continuing
Calibration Check
(CCC)

Verify initial calibration by analyzing a low-level CCC
(concentrations at, or below, the MRL for each analyte)
at the beginning of each Analysis Batch. Subsequent
CCCs are required after every tenth field sample and to
complete the batch.

The lowest level CCC must be within 50-150% of the
true value. All other levels must be within 70-130% of
the true value. Verify that each internal standard and
analyte peak elutes entirely within the MRM window
(Sect. 11.4.2).

Section 9.2.1

Laboratory Reagent
Blank (LRB)

With each Analysis Batch, analyze one LRB for each lot
number of filters used to prepare samples.

Demonstrate that all method analytes are below one-
third the Minimum Reporting Level (MRL), and that
possible interference from reagents and glassware do
not prevent identification and quantitation of method
analytes.

Section 9.2.7

Internal standards

Internal standards are added to all standards and
samples.

Peak area counts for each internal standard in
samples and CCCs must be within 50-150% of the
average peak area in the initial calibration.

Section 9.2.8

Laboratory Fortified
Sample Matrix
(LFSM)

Include one LFSM per Analysis Batch. Fortify the LFSM
with method analytes at a concentration close to but
greater than the native concentrations (if known).

For analytes fortified at concentrations <2 x the MRL,
the result must be within 50-150% of the true value;
70-130% of the true value if fortified at
concentrations greater than 2 x the MRL.

Section 9.2.9

Laboratory Fortified
Sample Matrix
Duplicate (LFSMD) or
Field Duplicate (FD)

Include at least one LFSMD or FD with each Analysis
Batch.

For LFSMDs or FDs, relative percent differences must
be <30% (<50% if analyte concentration <2 x the
MRL).

Section 9.2.2

Field Reagent Blank
(FRB)

Analyze the FRB if any analyte is detected in the
associated field samples.

If an analyte detected in the field sample is present in
the associated FRB at greater than one-third the MRL,
the results for that analyte are invalid.

Section 9.2.10

Calibration
Verification using
QCS

Perform a Calibration Verification at least quarterly.

Results must be within 80-120% of the true value.

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Figure 1. Relative Retention of Early Eluting Preservatives to the Method Analytes in High-Hardness Watera'b

1.0-

0.8-

0.6-

0.4-

0.2-

0.0

Chloride 	Sodium Omadine

AMPA 	Nitrate 	Glu

8

9	10

Time (min)

a Acquired using a Waters (Milford, MA) Xevo TQ Absolute. AMPA, GLU, and GLY at 40 ng/L; END at 20 ng/L.
b Sodium omadine was observed as the pyrithione anion at m/z 126.

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Figure 2. Relative Retention of Late Eluting Preservatives to the Method Analytes in High-Hardness Water°

1.0-

	EDTA-Ca

- EDTA-Mg

Gly

	End

	Sulfate

	Free EDTA

Time (min)

Acquired using a Waters (Milford, MA) Xevo TQ Absolute. AMPA, GLU, and GLY at 40 ng/L; END at 20 ng/L.

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